Articles | Volume 24, issue 15
https://doi.org/10.5194/acp-24-8865-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-24-8865-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue overview
| 
13 Aug 2024
Special issue overview |
| 13 Aug 2024
| 13 Aug 2024
Overview: quasi-Lagrangian observations of Arctic air mass transformations – introduction and initial results of the HALO–(𝒜 𝒞)3 aircraft campaign
Manfred Wendisch
CORRESPONDING AUTHOR
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
Susanne Crewell
Institut für Geophysik und Meteorologie (IGM), Universität zu Köln, Cologne, Germany
André Ehrlich
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
Andreas Herber
Physik der Atmosphäre Bremerhaven, Alfred–Wegener–Institut, Helmholtz–Zentrum für Polar– und Meeresforschung (AWI), Bremerhaven, Germany
Benjamin Kirbus
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
Christof Lüpkes
Physik der Atmosphäre Bremerhaven, Alfred–Wegener–Institut, Helmholtz–Zentrum für Polar– und Meeresforschung (AWI), Bremerhaven, Germany
Mario Mech
Institut für Geophysik und Meteorologie (IGM), Universität zu Köln, Cologne, Germany
Steven J. Abel
Met Office, Exeter, United Kingdom
Elisa F. Akansu
Atmosphärische Mikrophysik, Leibniz–Institut für Troposphärenforschung (TROPOS), Leipzig, Germany
Felix Ament
Meteorologisches Institut, Universität Hamburg, Hamburg, Germany
Clémantyne Aubry
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Laboratoire Atmosphères, Milieux et Observations Spatiales (LATMOS), Centre National de la Recherche Scientifique (CNRS), Guyancourt, France
Sebastian Becker
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
Stephan Borrmann
Abteilung für Partikelchemie, Max-Planck-Institut für Chemie (MPIC), Mainz, Germany
Institut für Physik der Atmosphäre (IPA), Johannes Gutenberg-Universität, Mainz, Germany
Heiko Bozem
Institut für Physik der Atmosphäre (IPA), Johannes Gutenberg-Universität, Mainz, Germany
Marlen Brückner
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
Hans-Christian Clemen
Abteilung für Partikelchemie, Max-Planck-Institut für Chemie (MPIC), Mainz, Germany
Sandro Dahlke
Physik der Atmosphäre, Alfred–Wegener–Institut, Helmholtz–Zentrum für Polar– und Meeresforschung (AWI), Potsdam, Germany
Georgios Dekoutsidis
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Julien Delanoë
Laboratoire Atmosphères, Milieux et Observations Spatiales (LATMOS), Centre National de la Recherche Scientifique (CNRS), Guyancourt, France
Elena De La Torre Castro
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Institut für Physik der Atmosphäre (IPA), Johannes Gutenberg-Universität, Mainz, Germany
Faculteit Luchtvaart- en Ruimtevaarttechniek, Technische Universiteit Delft, Delft, the Netherlands
Henning Dorff
Meteorologisches Institut, Universität Hamburg, Hamburg, Germany
Regis Dupuy
Laboratoire de Météorologie Physique (LaMP), Université Clermont Auvergne, Centre National de la Recherche Scientifique (CNRS), Clermont-Ferrand, France
Oliver Eppers
Abteilung für Partikelchemie, Max-Planck-Institut für Chemie (MPIC), Mainz, Germany
Florian Ewald
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Geet George
Klimaphysik, Max-Planck-Institut für Meteorologie (MPI-M), Hamburg, Germany
now at: Faculty of Civil Engineering and Geosciences, Delft University of Technology (TU Delft), Delft, the Netherlands
Irina V. Gorodetskaya
Centro de Estudos do Ambiente e do Mar (CESAM), Universidade de Aveiro, Aveiro, Portugal
Sarah Grawe
Atmosphärische Mikrophysik, Leibniz–Institut für Troposphärenforschung (TROPOS), Leipzig, Germany
Silke Groß
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Jörg Hartmann
Physik der Atmosphäre Bremerhaven, Alfred–Wegener–Institut, Helmholtz–Zentrum für Polar– und Meeresforschung (AWI), Bremerhaven, Germany
Silvia Henning
Atmosphärische Mikrophysik, Leibniz–Institut für Troposphärenforschung (TROPOS), Leipzig, Germany
Lutz Hirsch
Klimaphysik, Max-Planck-Institut für Meteorologie (MPI-M), Hamburg, Germany
Evelyn Jäkel
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
Philipp Joppe
Abteilung für Partikelchemie, Max-Planck-Institut für Chemie (MPIC), Mainz, Germany
Institut für Physik der Atmosphäre (IPA), Johannes Gutenberg-Universität, Mainz, Germany
Olivier Jourdan
Laboratoire de Météorologie Physique (LaMP), Université Clermont Auvergne, Centre National de la Recherche Scientifique (CNRS), Clermont-Ferrand, France
Zsofia Jurányi
Physik der Atmosphäre Bremerhaven, Alfred–Wegener–Institut, Helmholtz–Zentrum für Polar– und Meeresforschung (AWI), Bremerhaven, Germany
Michail Karalis
Department of Meteorology and Bolin Centre for Climate research, Stockholm University, Stockholm, Sweden
Mona Kellermann
Atmosphärische Mikrophysik, Leibniz–Institut für Troposphärenforschung (TROPOS), Leipzig, Germany
Marcus Klingebiel
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
Michael Lonardi
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
now at: Extreme Environments Research Laboratory (EERL), Ecole Polytechnique Fédérale de Lausanne (EPFL), Sion, Switzerland
Johannes Lucke
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Faculteit Luchtvaart- en Ruimtevaarttechniek, Technische Universiteit Delft, Delft, the Netherlands
Anna E. Luebke
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
Maximilian Maahn
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
Nina Maherndl
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
Marion Maturilli
Physik der Atmosphäre, Alfred–Wegener–Institut, Helmholtz–Zentrum für Polar– und Meeresforschung (AWI), Potsdam, Germany
Bernhard Mayer
Meteorologisches Institut, Ludwig-Maximilians-Universität München, Munich, Germany
Johanna Mayer
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Stephan Mertes
Atmosphärische Mikrophysik, Leibniz–Institut für Troposphärenforschung (TROPOS), Leipzig, Germany
Janosch Michaelis
Physik der Atmosphäre Bremerhaven, Alfred–Wegener–Institut, Helmholtz–Zentrum für Polar– und Meeresforschung (AWI), Bremerhaven, Germany
now at: Maritime Klimatologie, Maritim-klimatologische Analysen und Produkte, Deutscher Wetterdienst (DWD), Hamburg, Germany
Michel Michalkov
Atmosphärische Mikrophysik, Leibniz–Institut für Troposphärenforschung (TROPOS), Leipzig, Germany
Guillaume Mioche
Laboratoire de Météorologie Physique (LaMP), Université Clermont Auvergne, Centre National de la Recherche Scientifique (CNRS), Clermont-Ferrand, France
Manuel Moser
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Institut für Physik der Atmosphäre (IPA), Johannes Gutenberg-Universität, Mainz, Germany
Hanno Müller
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
Roel Neggers
Institut für Geophysik und Meteorologie (IGM), Universität zu Köln, Cologne, Germany
Davide Ori
Institut für Geophysik und Meteorologie (IGM), Universität zu Köln, Cologne, Germany
Daria Paul
Institut für Geophysik und Meteorologie (IGM), Universität zu Köln, Cologne, Germany
Fiona M. Paulus
Institut für Geophysik und Meteorologie (IGM), Universität zu Köln, Cologne, Germany
Christian Pilz
Atmosphärische Mikrophysik, Leibniz–Institut für Troposphärenforschung (TROPOS), Leipzig, Germany
Felix Pithan
Physik der Atmosphäre Bremerhaven, Alfred–Wegener–Institut, Helmholtz–Zentrum für Polar– und Meeresforschung (AWI), Bremerhaven, Germany
Mira Pöhlker
Atmosphärische Mikrophysik, Leibniz–Institut für Troposphärenforschung (TROPOS), Leipzig, Germany
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
Veronika Pörtge
Meteorologisches Institut, Ludwig-Maximilians-Universität München, Munich, Germany
Maximilian Ringel
Meteorologisches Institut, Universität Hamburg, Hamburg, Germany
Nils Risse
Institut für Geophysik und Meteorologie (IGM), Universität zu Köln, Cologne, Germany
Gregory C. Roberts
Scripps Institution of Oceanography, University of California San Diego, La Jolla, USA
Sophie Rosenburg
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
Johannes Röttenbacher
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
Janna Rückert
Institut für Umweltphysik (IUP), Universität Bremen, Bremen, Germany
Michael Schäfer
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
Jonas Schaefer
Atmosphärische Mikrophysik, Leibniz–Institut für Troposphärenforschung (TROPOS), Leipzig, Germany
Vera Schemann
Institut für Geophysik und Meteorologie (IGM), Universität zu Köln, Cologne, Germany
Imke Schirmacher
Institut für Geophysik und Meteorologie (IGM), Universität zu Köln, Cologne, Germany
Jörg Schmidt
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
Sebastian Schmidt
Department of Atmospheric and Oceanic Sciences, Laboratory for Atmospheric and Space Physics (LASP), University of Colorado Boulder, Boulder, CO, USA
Johannes Schneider
Abteilung für Partikelchemie, Max-Planck-Institut für Chemie (MPIC), Mainz, Germany
Sabrina Schnitt
Institut für Geophysik und Meteorologie (IGM), Universität zu Köln, Cologne, Germany
Anja Schwarz
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
Holger Siebert
Atmosphärische Mikrophysik, Leibniz–Institut für Troposphärenforschung (TROPOS), Leipzig, Germany
Harald Sodemann
Geophysical Institute, University of Bergen, Bergen, Norway
Bjerknes Centre for Climate Research, Bergen, Norway
Tim Sperzel
Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Leipzig, Germany
now at: Abteilung Klima und Umwelt, Deutscher Wetterdienst, Offenbach am Main, Germany
Gunnar Spreen
Institut für Umweltphysik (IUP), Universität Bremen, Bremen, Germany
Bjorn Stevens
Klimaphysik, Max-Planck-Institut für Meteorologie (MPI-M), Hamburg, Germany
Frank Stratmann
Atmosphärische Mikrophysik, Leibniz–Institut für Troposphärenforschung (TROPOS), Leipzig, Germany
Gunilla Svensson
Department of Meteorology and Bolin Centre for Climate research, Stockholm University, Stockholm, Sweden
Christian Tatzelt
Atmosphärische Mikrophysik, Leibniz–Institut für Troposphärenforschung (TROPOS), Leipzig, Germany
Thomas Tuch
Atmosphärische Mikrophysik, Leibniz–Institut für Troposphärenforschung (TROPOS), Leipzig, Germany
Timo Vihma
Finnish Meteorological Institute (FMI), Helsinki, Finland
Christiane Voigt
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Institut für Physik der Atmosphäre (IPA), Johannes Gutenberg-Universität, Mainz, Germany
Lea Volkmer
Meteorologisches Institut, Ludwig-Maximilians-Universität München, Munich, Germany
Andreas Walbröl
Institut für Geophysik und Meteorologie (IGM), Universität zu Köln, Cologne, Germany
Anna Weber
Meteorologisches Institut, Ludwig-Maximilians-Universität München, Munich, Germany
Birgit Wehner
Atmosphärische Mikrophysik, Leibniz–Institut für Troposphärenforschung (TROPOS), Leipzig, Germany
Bruno Wetzel
Atmosphärische Mikrophysik, Leibniz–Institut für Troposphärenforschung (TROPOS), Leipzig, Germany
Martin Wirth
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Tobias Zinner
Meteorologisches Institut, Ludwig-Maximilians-Universität München, Munich, Germany
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CloudSat’s relatively coarse spatial resolution, low sensitivity, and blind zone limit its assessment of Arctic low-level clouds, which affect the surface energy balance. We compare cloud fractions from CloudSat and finely resolved airborne radar observations to determine CloudSat’s limitations. Cloudsat overestimates cloud fractions above its blind zone, especially during cold-air outbreaks over open water, and misses a cloud fraction of 32 % and half of the precipitation inside its blind zone.
Olivia Linke, Johannes Quaas, Finja Baumer, Sebastian Becker, Jan Chylik, Sandro Dahlke, André Ehrlich, Dörthe Handorf, Christoph Jacobi, Heike Kalesse-Los, Luca Lelli, Sina Mehrdad, Roel A. J. Neggers, Johannes Riebold, Pablo Saavedra Garfias, Niklas Schnierstein, Matthew D. Shupe, Chris Smith, Gunnar Spreen, Baptiste Verneuil, Kameswara S. Vinjamuri, Marco Vountas, and Manfred Wendisch
Atmos. Chem. Phys., 23, 9963–9992, https://doi.org/10.5194/acp-23-9963-2023, https://doi.org/10.5194/acp-23-9963-2023, 2023
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Lapse rate feedback (LRF) is a major driver of the Arctic amplification (AA) of climate change. It arises because the warming is stronger at the surface than aloft. Several processes can affect the LRF in the Arctic, such as the omnipresent temperature inversion. Here, we compare multimodel climate simulations to Arctic-based observations from a large research consortium to broaden our understanding of these processes, find synergy among them, and constrain the Arctic LRF and AA.
Manfred Wendisch, Johannes Stapf, Sebastian Becker, André Ehrlich, Evelyn Jäkel, Marcus Klingebiel, Christof Lüpkes, Michael Schäfer, and Matthew D. Shupe
Atmos. Chem. Phys., 23, 9647–9667, https://doi.org/10.5194/acp-23-9647-2023, https://doi.org/10.5194/acp-23-9647-2023, 2023
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Atmospheric radiation measurements have been conducted during two field campaigns using research aircraft. The data are analyzed to see if the near-surface air in the Arctic is warmed or cooled if warm–humid air masses from the south enter the Arctic or cold–dry air moves from the north from the Arctic to mid-latitude areas. It is important to study these processes and to check if climate models represent them well. Otherwise it is not possible to reliably forecast the future Arctic climate.
Sophie Rosenburg, Charlotte Lange, Evelyn Jäkel, Michael Schäfer, André Ehrlich, and Manfred Wendisch
Atmos. Meas. Tech., 16, 3915–3930, https://doi.org/10.5194/amt-16-3915-2023, https://doi.org/10.5194/amt-16-3915-2023, 2023
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Snow layer melting and melt pond formation on Arctic sea ice are important seasonal processes affecting the surface reflection and energy budget. Sea ice reflectivity was surveyed by airborne imaging spectrometers in May–June 2017. Adapted retrieval approaches were applied to find snow layer liquid water fraction, snow grain effective radius, and melt pond depth. The retrievals show the potential and limitations of spectral airborne imaging to map melting snow layer and melt pond properties.
Manuel Moser, Christiane Voigt, Tina Jurkat-Witschas, Valerian Hahn, Guillaume Mioche, Olivier Jourdan, Régis Dupuy, Christophe Gourbeyre, Alfons Schwarzenboeck, Johannes Lucke, Yvonne Boose, Mario Mech, Stephan Borrmann, André Ehrlich, Andreas Herber, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys., 23, 7257–7280, https://doi.org/10.5194/acp-23-7257-2023, https://doi.org/10.5194/acp-23-7257-2023, 2023
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This study provides a comprehensive microphysical and thermodynamic phase analysis of low-level clouds in the northern Fram Strait, above the sea ice and the open ocean, during spring and summer. Using airborne in situ cloud data, we show that the properties of Arctic low-level clouds vary significantly with seasonal meteorological situations and surface conditions. The observations presented in this study can help one to assess the role of clouds in the Arctic climate system.
Sebastian Becker, André Ehrlich, Michael Schäfer, and Manfred Wendisch
Atmos. Chem. Phys., 23, 7015–7031, https://doi.org/10.5194/acp-23-7015-2023, https://doi.org/10.5194/acp-23-7015-2023, 2023
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This study analyses the variability of the warming or cooling effect of clouds on the Arctic surface. Therefore, aircraft radiation measurements were performed over sea ice and open ocean during three seasonally different campaigns. It is found that clouds cool the open-ocean surface most strongly in summer. Over sea ice, clouds warm the surface in spring but have a neutral effect in summer. Due to the variable sea ice extent, clouds warm the surface during spring but cool it during late summer.
Dmitry G. Chechin, Christof Lüpkes, Jörg Hartmann, André Ehrlich, and Manfred Wendisch
Atmos. Chem. Phys., 23, 4685–4707, https://doi.org/10.5194/acp-23-4685-2023, https://doi.org/10.5194/acp-23-4685-2023, 2023
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Clouds represent a very important component of the Arctic climate system, as they strongly reduce the amount of heat lost to space from the sea ice surface. Properties of clouds, as well as their persistence, strongly depend on the complex interaction of such small-scale properties as phase transitions, radiative transfer and turbulence. In this study we use airborne observations to learn more about the effect of clouds and radiative cooling on turbulence in comparison with other factors.
André Ehrlich, Martin Zöger, Andreas Giez, Vladyslav Nenakhov, Christian Mallaun, Rolf Maser, Timo Röschenthaler, Anna E. Luebke, Kevin Wolf, Bjorn Stevens, and Manfred Wendisch
Atmos. Meas. Tech., 16, 1563–1581, https://doi.org/10.5194/amt-16-1563-2023, https://doi.org/10.5194/amt-16-1563-2023, 2023
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Measurements of the broadband radiative energy budget from aircraft are needed to study the effect of clouds, aerosol particles, and surface conditions on the Earth's energy budget. However, the moving aircraft introduces challenges to the instrument performance and post-processing of the data. This study introduces a new radiometer package, outlines a greatly simplifying method to correct thermal offsets, and provides exemplary measurements of solar and thermal–infrared irradiance.
Yunfan Liu, Hang Su, Siwen Wang, Chao Wei, Wei Tao, Mira L. Pöhlker, Christopher Pöhlker, Bruna A. Holanda, Ovid O. Krüger, Thorsten Hoffmann, Manfred Wendisch, Paulo Artaxo, Ulrich Pöschl, Meinrat O. Andreae, and Yafang Cheng
Atmos. Chem. Phys., 23, 251–272, https://doi.org/10.5194/acp-23-251-2023, https://doi.org/10.5194/acp-23-251-2023, 2023
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The origins of the abundant cloud condensation nuclei (CCN) in the upper troposphere (UT) of the Amazon remain unclear. With model developments of new secondary organic aerosol schemes and constrained by observation, we show that strong aerosol nucleation and condensation in the UT is triggered by biogenic organics, and organic condensation is key for UT CCN production. This UT CCN-producing mechanism may prevail over broader vegetation canopies and deserves emphasis in aerosol–climate feedback.
Sebastian Becker, André Ehrlich, Evelyn Jäkel, Tim Carlsen, Michael Schäfer, and Manfred Wendisch
Atmos. Meas. Tech., 15, 2939–2953, https://doi.org/10.5194/amt-15-2939-2022, https://doi.org/10.5194/amt-15-2939-2022, 2022
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Airborne radiation measurements are used to characterize the solar directional reflection of a mixture of Arctic sea ice and open-ocean surfaces in the transition zone between both surface types. The mixture reveals reflection properties of both surface types. It is shown that the directional reflection of the mixture can be reconstructed from the directional reflection of the individual surfaces, accounting for the special conditions present in the transition zone.
Michael Schäfer, Kevin Wolf, André Ehrlich, Christoph Hallbauer, Evelyn Jäkel, Friedhelm Jansen, Anna Elizabeth Luebke, Joshua Müller, Jakob Thoböll, Timo Röschenthaler, Bjorn Stevens, and Manfred Wendisch
Atmos. Meas. Tech., 15, 1491–1509, https://doi.org/10.5194/amt-15-1491-2022, https://doi.org/10.5194/amt-15-1491-2022, 2022
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The new airborne thermal infrared imager VELOX is introduced. It measures two-dimensional fields of spectral thermal infrared radiance or brightness temperature within the large atmospheric window. The technical specifications as well as necessary calibration and correction procedures are presented. Example measurements from the first field deployment are analysed with respect to cloud coverage and cloud top altitude.
Anna E. Luebke, André Ehrlich, Michael Schäfer, Kevin Wolf, and Manfred Wendisch
Atmos. Chem. Phys., 22, 2727–2744, https://doi.org/10.5194/acp-22-2727-2022, https://doi.org/10.5194/acp-22-2727-2022, 2022
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A combination of aircraft and satellite observations is used to show how the characteristics of tropical shallow clouds interact with incoming and outgoing energy. A complete depiction of these clouds is challenging to obtain, but such data are useful for understanding how models can correctly represent them. The amount of cloud is found to be the most important factor, while other cloud characteristics become increasingly impactful when more cloud is present.
Ramon Campos Braga, Barbara Ervens, Daniel Rosenfeld, Meinrat O. Andreae, Jan-David Förster, Daniel Fütterer, Lianet Hernández Pardo, Bruna A. Holanda, Tina Jurkat-Witschas, Ovid O. Krüger, Oliver Lauer, Luiz A. T. Machado, Christopher Pöhlker, Daniel Sauer, Christiane Voigt, Adrian Walser, Manfred Wendisch, Ulrich Pöschl, and Mira L. Pöhlker
Atmos. Chem. Phys., 21, 17513–17528, https://doi.org/10.5194/acp-21-17513-2021, https://doi.org/10.5194/acp-21-17513-2021, 2021
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Interactions of aerosol particles with clouds represent a large uncertainty in estimates of climate change. Properties of aerosol particles control their ability to act as cloud condensation nuclei. Using aerosol measurements in the Amazon, we performed model studies to compare predicted and measured cloud droplet number concentrations at cloud bases. Our results confirm previous estimates of particle hygroscopicity in this region.
Heike Konow, Florian Ewald, Geet George, Marek Jacob, Marcus Klingebiel, Tobias Kölling, Anna E. Luebke, Theresa Mieslinger, Veronika Pörtge, Jule Radtke, Michael Schäfer, Hauke Schulz, Raphaela Vogel, Martin Wirth, Sandrine Bony, Susanne Crewell, André Ehrlich, Linda Forster, Andreas Giez, Felix Gödde, Silke Groß, Manuel Gutleben, Martin Hagen, Lutz Hirsch, Friedhelm Jansen, Theresa Lang, Bernhard Mayer, Mario Mech, Marc Prange, Sabrina Schnitt, Jessica Vial, Andreas Walbröl, Manfred Wendisch, Kevin Wolf, Tobias Zinner, Martin Zöger, Felix Ament, and Bjorn Stevens
Earth Syst. Sci. Data, 13, 5545–5563, https://doi.org/10.5194/essd-13-5545-2021, https://doi.org/10.5194/essd-13-5545-2021, 2021
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The German research aircraft HALO took part in the research campaign EUREC4A in January and February 2020. The focus area was the tropical Atlantic east of the island of Barbados. We describe the characteristics of the 15 research flights, provide auxiliary information, derive combined cloud mask products from all instruments that observe clouds on board the aircraft, and provide code examples that help new users of the data to get started.
Ramon Campos Braga, Daniel Rosenfeld, Ovid O. Krüger, Barbara Ervens, Bruna A. Holanda, Manfred Wendisch, Trismono Krisna, Ulrich Pöschl, Meinrat O. Andreae, Christiane Voigt, and Mira L. Pöhlker
Atmos. Chem. Phys., 21, 14079–14088, https://doi.org/10.5194/acp-21-14079-2021, https://doi.org/10.5194/acp-21-14079-2021, 2021
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Quantifying the precipitation within clouds is crucial for our understanding of the Earth's hydrological cycle. Using in situ measurements of cloud and rain properties over the Amazon Basin and Atlantic Ocean, we show here a linear relationship between the effective radius (re) and precipitation water content near the tops of convective clouds for different pollution states and temperature levels. Our results emphasize the role of re to determine both initiation and amount of precipitation.
Bjorn Stevens, Sandrine Bony, David Farrell, Felix Ament, Alan Blyth, Christopher Fairall, Johannes Karstensen, Patricia K. Quinn, Sabrina Speich, Claudia Acquistapace, Franziska Aemisegger, Anna Lea Albright, Hugo Bellenger, Eberhard Bodenschatz, Kathy-Ann Caesar, Rebecca Chewitt-Lucas, Gijs de Boer, Julien Delanoë, Leif Denby, Florian Ewald, Benjamin Fildier, Marvin Forde, Geet George, Silke Gross, Martin Hagen, Andrea Hausold, Karen J. Heywood, Lutz Hirsch, Marek Jacob, Friedhelm Jansen, Stefan Kinne, Daniel Klocke, Tobias Kölling, Heike Konow, Marie Lothon, Wiebke Mohr, Ann Kristin Naumann, Louise Nuijens, Léa Olivier, Robert Pincus, Mira Pöhlker, Gilles Reverdin, Gregory Roberts, Sabrina Schnitt, Hauke Schulz, A. Pier Siebesma, Claudia Christine Stephan, Peter Sullivan, Ludovic Touzé-Peiffer, Jessica Vial, Raphaela Vogel, Paquita Zuidema, Nicola Alexander, Lyndon Alves, Sophian Arixi, Hamish Asmath, Gholamhossein Bagheri, Katharina Baier, Adriana Bailey, Dariusz Baranowski, Alexandre Baron, Sébastien Barrau, Paul A. Barrett, Frédéric Batier, Andreas Behrendt, Arne Bendinger, Florent Beucher, Sebastien Bigorre, Edmund Blades, Peter Blossey, Olivier Bock, Steven Böing, Pierre Bosser, Denis Bourras, Pascale Bouruet-Aubertot, Keith Bower, Pierre Branellec, Hubert Branger, Michal Brennek, Alan Brewer, Pierre-Etienne Brilouet, Björn Brügmann, Stefan A. Buehler, Elmo Burke, Ralph Burton, Radiance Calmer, Jean-Christophe Canonici, Xavier Carton, Gregory Cato Jr., Jude Andre Charles, Patrick Chazette, Yanxu Chen, Michal T. Chilinski, Thomas Choularton, Patrick Chuang, Shamal Clarke, Hugh Coe, Céline Cornet, Pierre Coutris, Fleur Couvreux, Susanne Crewell, Timothy Cronin, Zhiqiang Cui, Yannis Cuypers, Alton Daley, Gillian M. Damerell, Thibaut Dauhut, Hartwig Deneke, Jean-Philippe Desbios, Steffen Dörner, Sebastian Donner, Vincent Douet, Kyla Drushka, Marina Dütsch, André Ehrlich, Kerry Emanuel, Alexandros Emmanouilidis, Jean-Claude Etienne, Sheryl Etienne-Leblanc, Ghislain Faure, Graham Feingold, Luca Ferrero, Andreas Fix, Cyrille Flamant, Piotr Jacek Flatau, Gregory R. Foltz, Linda Forster, Iulian Furtuna, Alan Gadian, Joseph Galewsky, Martin Gallagher, Peter Gallimore, Cassandra Gaston, Chelle Gentemann, Nicolas Geyskens, Andreas Giez, John Gollop, Isabelle Gouirand, Christophe Gourbeyre, Dörte de Graaf, Geiske E. de Groot, Robert Grosz, Johannes Güttler, Manuel Gutleben, Kashawn Hall, George Harris, Kevin C. Helfer, Dean Henze, Calvert Herbert, Bruna Holanda, Antonio Ibanez-Landeta, Janet Intrieri, Suneil Iyer, Fabrice Julien, Heike Kalesse, Jan Kazil, Alexander Kellman, Abiel T. Kidane, Ulrike Kirchner, Marcus Klingebiel, Mareike Körner, Leslie Ann Kremper, Jan Kretzschmar, Ovid Krüger, Wojciech Kumala, Armin Kurz, Pierre L'Hégaret, Matthieu Labaste, Tom Lachlan-Cope, Arlene Laing, Peter Landschützer, Theresa Lang, Diego Lange, Ingo Lange, Clément Laplace, Gauke Lavik, Rémi Laxenaire, Caroline Le Bihan, Mason Leandro, Nathalie Lefevre, Marius Lena, Donald Lenschow, Qiang Li, Gary Lloyd, Sebastian Los, Niccolò Losi, Oscar Lovell, Christopher Luneau, Przemyslaw Makuch, Szymon Malinowski, Gaston Manta, Eleni Marinou, Nicholas Marsden, Sebastien Masson, Nicolas Maury, Bernhard Mayer, Margarette Mayers-Als, Christophe Mazel, Wayne McGeary, James C. McWilliams, Mario Mech, Melina Mehlmann, Agostino Niyonkuru Meroni, Theresa Mieslinger, Andreas Minikin, Peter Minnett, Gregor Möller, Yanmichel Morfa Avalos, Caroline Muller, Ionela Musat, Anna Napoli, Almuth Neuberger, Christophe Noisel, David Noone, Freja Nordsiek, Jakub L. Nowak, Lothar Oswald, Douglas J. Parker, Carolyn Peck, Renaud Person, Miriam Philippi, Albert Plueddemann, Christopher Pöhlker, Veronika Pörtge, Ulrich Pöschl, Lawrence Pologne, Michał Posyniak, Marc Prange, Estefanía Quiñones Meléndez, Jule Radtke, Karim Ramage, Jens Reimann, Lionel Renault, Klaus Reus, Ashford Reyes, Joachim Ribbe, Maximilian Ringel, Markus Ritschel, Cesar B. Rocha, Nicolas Rochetin, Johannes Röttenbacher, Callum Rollo, Haley Royer, Pauline Sadoulet, Leo Saffin, Sanola Sandiford, Irina Sandu, Michael Schäfer, Vera Schemann, Imke Schirmacher, Oliver Schlenczek, Jerome Schmidt, Marcel Schröder, Alfons Schwarzenboeck, Andrea Sealy, Christoph J. Senff, Ilya Serikov, Samkeyat Shohan, Elizabeth Siddle, Alexander Smirnov, Florian Späth, Branden Spooner, M. Katharina Stolla, Wojciech Szkółka, Simon P. de Szoeke, Stéphane Tarot, Eleni Tetoni, Elizabeth Thompson, Jim Thomson, Lorenzo Tomassini, Julien Totems, Alma Anna Ubele, Leonie Villiger, Jan von Arx, Thomas Wagner, Andi Walther, Ben Webber, Manfred Wendisch, Shanice Whitehall, Anton Wiltshire, Allison A. Wing, Martin Wirth, Jonathan Wiskandt, Kevin Wolf, Ludwig Worbes, Ethan Wright, Volker Wulfmeyer, Shanea Young, Chidong Zhang, Dongxiao Zhang, Florian Ziemen, Tobias Zinner, and Martin Zöger
Earth Syst. Sci. Data, 13, 4067–4119, https://doi.org/10.5194/essd-13-4067-2021, https://doi.org/10.5194/essd-13-4067-2021, 2021
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The EUREC4A field campaign, designed to test hypothesized mechanisms by which clouds respond to warming and benchmark next-generation Earth-system models, is presented. EUREC4A comprised roughly 5 weeks of measurements in the downstream winter trades of the North Atlantic – eastward and southeastward of Barbados. It was the first campaign that attempted to characterize the full range of processes and scales influencing trade wind clouds.
Ulrike Egerer, André Ehrlich, Matthias Gottschalk, Hannes Griesche, Roel A. J. Neggers, Holger Siebert, and Manfred Wendisch
Atmos. Chem. Phys., 21, 6347–6364, https://doi.org/10.5194/acp-21-6347-2021, https://doi.org/10.5194/acp-21-6347-2021, 2021
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This paper describes a case study of a three-day period with a persistent humidity inversion above a mixed-phase cloud layer in the Arctic. It is based on measurements with a tethered balloon, complemented with results from a dedicated high-resolution large-eddy simulation. Both methods show that the humidity layer acts to provide moisture to the cloud layer through downward turbulent transport. This supply of additional moisture can contribute to the persistence of Arctic clouds.
Johannes Stapf, André Ehrlich, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-279, https://doi.org/10.5194/acp-2021-279, 2021
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Airborne observations of the surface radiative energy budget in the marginal sea ice zone (the region between open ocean and closed sea ice) are presented. Atmospheric thermodynamic profiles and surface properties change on small spatial scales in this area and influence the impact of clouds on the radiative energy budget. The radiation budget over sea ice is compared to available studies in the Arctic and the influence of cold air outbreaks and warm air intrusions is illustrated.
Evelyn Jäkel, Tim Carlsen, André Ehrlich, Manfred Wendisch, Michael Schäfer, Sophie Rosenburg, Konstantina Nakoudi, Marco Zanatta, Gerit Birnbaum, Veit Helm, Andreas Herber, Larysa Istomina, Linlu Mei, and Anika Rohde
The Cryosphere Discuss., https://doi.org/10.5194/tc-2021-14, https://doi.org/10.5194/tc-2021-14, 2021
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Different approaches to retrieve the optical-equivalent snow grain size using satellite, airborne, and ground-based observations were evaluated and compared to modeled data. The study is focused on low Sun and partly rough surface conditions encountered North of Greenland in March/April 2018. We proposed an adjusted airborne retrieval method to reduce the retrieval uncertainty.
Johannes Quaas, Antti Arola, Brian Cairns, Matthew Christensen, Hartwig Deneke, Annica M. L. Ekman, Graham Feingold, Ann Fridlind, Edward Gryspeerdt, Otto Hasekamp, Zhanqing Li, Antti Lipponen, Po-Lun Ma, Johannes Mülmenstädt, Athanasios Nenes, Joyce E. Penner, Daniel Rosenfeld, Roland Schrödner, Kenneth Sinclair, Odran Sourdeval, Philip Stier, Matthias Tesche, Bastiaan van Diedenhoven, and Manfred Wendisch
Atmos. Chem. Phys., 20, 15079–15099, https://doi.org/10.5194/acp-20-15079-2020, https://doi.org/10.5194/acp-20-15079-2020, 2020
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Anthropogenic pollution particles – aerosols – serve as cloud condensation nuclei and thus increase cloud droplet concentration and the clouds' reflection of sunlight (a cooling effect on climate). This Twomey effect is poorly constrained by models and requires satellite data for better quantification. The review summarizes the challenges in properly doing so and outlines avenues for progress towards a better use of aerosol retrievals and better retrievals of droplet concentrations.
Tim Carlsen, Gerit Birnbaum, André Ehrlich, Veit Helm, Evelyn Jäkel, Michael Schäfer, and Manfred Wendisch
The Cryosphere, 14, 3959–3978, https://doi.org/10.5194/tc-14-3959-2020, https://doi.org/10.5194/tc-14-3959-2020, 2020
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The angular reflection of solar radiation by snow surfaces is particularly anisotropic and highly variable. We measured the angular reflection from an aircraft using a digital camera in Antarctica in 2013/14 and studied its variability: the anisotropy increases with a lower Sun but decreases for rougher surfaces and larger snow grains. The applied methodology allows for a direct comparison with satellite observations, which generally underestimated the anisotropy measured within this study.
Jan Kretzschmar, Johannes Stapf, Daniel Klocke, Manfred Wendisch, and Johannes Quaas
Atmos. Chem. Phys., 20, 13145–13165, https://doi.org/10.5194/acp-20-13145-2020, https://doi.org/10.5194/acp-20-13145-2020, 2020
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This study compares simulations with the ICON model at the kilometer scale to airborne radiation and cloud microphysics observations that have been derived during the ACLOUD aircraft campaign around Svalbard, Norway, in May/June 2017. We find an overestimated surface warming effect of clouds compared to the observations in our setup. This bias was reduced by considering subgrid-scale vertical motion in the activation of cloud condensation nuclei in the two-moment microphysical scheme used.
Li Li, Zhengqiang Li, Wenyuan Chang, Yang Ou, Philippe Goloub, Chengzhe Li, Kaitao Li, Qiaoyun Hu, Jianping Wang, and Manfred Wendisch
Atmos. Chem. Phys., 20, 10845–10864, https://doi.org/10.5194/acp-20-10845-2020, https://doi.org/10.5194/acp-20-10845-2020, 2020
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Dust Aerosol Observation-Kashi (DAO-K) campaign was conducted near the Taklimakan Desert in April 2019 to obtain comprehensive aerosol, atmosphere, and surface parameters. Estimations of aerosol solar radiative forcing by a radiative transfer (RT) model were improved based on the measured aerosol parameters, additionally considering atmospheric profiles and diurnal variations of surface albedo. RT simulations agree well with simultaneous irradiance observations, even in dust-polluted conditions.
Johannes Stapf, André Ehrlich, Evelyn Jäkel, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys., 20, 9895–9914, https://doi.org/10.5194/acp-20-9895-2020, https://doi.org/10.5194/acp-20-9895-2020, 2020
Tobias Donth, Evelyn Jäkel, André Ehrlich, Bernd Heinold, Jacob Schacht, Andreas Herber, Marco Zanatta, and Manfred Wendisch
Atmos. Chem. Phys., 20, 8139–8156, https://doi.org/10.5194/acp-20-8139-2020, https://doi.org/10.5194/acp-20-8139-2020, 2020
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Solar radiative effects of Arctic black carbon (BC) particles (suspended in the atmosphere and in the surface snowpack) were quantified under cloudless and cloudy conditions. An atmospheric and a snow radiative transfer model were coupled to account for radiative interactions between both compartments. It was found that (i) the warming effect of BC in the snowpack overcompensates for the atmospheric BC cooling effect, and (ii) clouds tend to reduce the atmospheric BC cooling and snow BC warming.
Elena Ruiz-Donoso, André Ehrlich, Michael Schäfer, Evelyn Jäkel, Vera Schemann, Susanne Crewell, Mario Mech, Birte Solveig Kulla, Leif-Leonard Kliesch, Roland Neuber, and Manfred Wendisch
Atmos. Chem. Phys., 20, 5487–5511, https://doi.org/10.5194/acp-20-5487-2020, https://doi.org/10.5194/acp-20-5487-2020, 2020
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Mixed-phase clouds, formed of water droplets and ice crystals, appear frequently in Arctic regions. Characterizing the distribution of liquid water and ice inside the cloud appropriately is important because it influences the cloud's impact on the surface temperature. In this study, we combined images of the cloud top with measurements inside the cloud to analyze in detail the 3D spatial distribution of liquid and ice in two mixed-phase clouds occurring under different meteorological scenarios.
Bruna A. Holanda, Mira L. Pöhlker, David Walter, Jorge Saturno, Matthias Sörgel, Jeannine Ditas, Florian Ditas, Christiane Schulz, Marco Aurélio Franco, Qiaoqiao Wang, Tobias Donth, Paulo Artaxo, Henrique M. J. Barbosa, Stephan Borrmann, Ramon Braga, Joel Brito, Yafang Cheng, Maximilian Dollner, Johannes W. Kaiser, Thomas Klimach, Christoph Knote, Ovid O. Krüger, Daniel Fütterer, Jošt V. Lavrič, Nan Ma, Luiz A. T. Machado, Jing Ming, Fernando G. Morais, Hauke Paulsen, Daniel Sauer, Hans Schlager, Johannes Schneider, Hang Su, Bernadett Weinzierl, Adrian Walser, Manfred Wendisch, Helmut Ziereis, Martin Zöger, Ulrich Pöschl, Meinrat O. Andreae, and Christopher Pöhlker
Atmos. Chem. Phys., 20, 4757–4785, https://doi.org/10.5194/acp-20-4757-2020, https://doi.org/10.5194/acp-20-4757-2020, 2020
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Biomass burning smoke from African savanna and grassland is transported across the South Atlantic Ocean in defined layers within the free troposphere. The combination of in situ aircraft and ground-based measurements aided by satellite observations showed that these layers are transported into the Amazon Basin during the early dry season. The influx of aged smoke, enriched in black carbon and cloud condensation nuclei, has important implications for the Amazonian aerosol and cloud cycling.
Fan Mei, Jian Wang, Jennifer M. Comstock, Ralf Weigel, Martina Krämer, Christoph Mahnke, John E. Shilling, Johannes Schneider, Christiane Schulz, Charles N. Long, Manfred Wendisch, Luiz A. T. Machado, Beat Schmid, Trismono Krisna, Mikhail Pekour, John Hubbe, Andreas Giez, Bernadett Weinzierl, Martin Zoeger, Mira L. Pöhlker, Hans Schlager, Micael A. Cecchini, Meinrat O. Andreae, Scot T. Martin, Suzane S. de Sá, Jiwen Fan, Jason Tomlinson, Stephen Springston, Ulrich Pöschl, Paulo Artaxo, Christopher Pöhlker, Thomas Klimach, Andreas Minikin, Armin Afchine, and Stephan Borrmann
Atmos. Meas. Tech., 13, 661–684, https://doi.org/10.5194/amt-13-661-2020, https://doi.org/10.5194/amt-13-661-2020, 2020
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In 2014, the US DOE G1 aircraft and the German HALO aircraft overflew the Amazon basin to study how aerosols influence cloud cycles under a clean condition and around a tropical megacity. This paper describes how to meaningfully compare similar measurements from two research aircraft and identify the potential measurement issue. We also discuss the uncertainty range for each measurement for further usage in model evaluation and satellite data validation.
Pascal Polonik, Christoph Knote, Tobias Zinner, Florian Ewald, Tobias Kölling, Bernhard Mayer, Meinrat O. Andreae, Tina Jurkat-Witschas, Thomas Klimach, Christoph Mahnke, Sergej Molleker, Christopher Pöhlker, Mira L. Pöhlker, Ulrich Pöschl, Daniel Rosenfeld, Christiane Voigt, Ralf Weigel, and Manfred Wendisch
Atmos. Chem. Phys., 20, 1591–1605, https://doi.org/10.5194/acp-20-1591-2020, https://doi.org/10.5194/acp-20-1591-2020, 2020
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A realistic representation of cloud–aerosol interactions is central to accurate climate projections. Here we combine observations collected during the ACRIDICON-CHUVA campaign with chemistry-transport simulations to evaluate the model’s ability to represent the indirect effects of biomass burning aerosol on cloud microphysics. We find an upper limit for the model sensitivity on cloud condensation nuclei concentrations well below the levels reached during the burning season in the Amazon Basin.
André Ehrlich, Manfred Wendisch, Christof Lüpkes, Matthias Buschmann, Heiko Bozem, Dmitri Chechin, Hans-Christian Clemen, Régis Dupuy, Olliver Eppers, Jörg Hartmann, Andreas Herber, Evelyn Jäkel, Emma Järvinen, Olivier Jourdan, Udo Kästner, Leif-Leonard Kliesch, Franziska Köllner, Mario Mech, Stephan Mertes, Roland Neuber, Elena Ruiz-Donoso, Martin Schnaiter, Johannes Schneider, Johannes Stapf, and Marco Zanatta
Earth Syst. Sci. Data, 11, 1853–1881, https://doi.org/10.5194/essd-11-1853-2019, https://doi.org/10.5194/essd-11-1853-2019, 2019
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During the Arctic CLoud Observations Using airborne measurements during polar Day (ACLOUD) campaign, two research aircraft (Polar 5 and 6) jointly performed 22 research flights over the transition zone between open ocean and closed sea ice. The data set combines remote sensing and in situ measurement of cloud, aerosol, and trace gas properties, as well as turbulent and radiative fluxes, which will be used to study Arctic boundary layer and mid-level clouds and their role in Arctic amplification.
Ulrike Egerer, Matthias Gottschalk, Holger Siebert, André Ehrlich, and Manfred Wendisch
Atmos. Meas. Tech., 12, 4019–4038, https://doi.org/10.5194/amt-12-4019-2019, https://doi.org/10.5194/amt-12-4019-2019, 2019
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In this study, we introduce the new tethered balloon system BELUGA, which includes different modular instrument packages for measuring turbulence and radiation in the atmospheric boundary layer. BELUGA was deployed in an Arctic field campaign in 2017, providing details of boundary layer processes in combination with low-level clouds. Those processes are still not fully understood and in situ measurements in the Arctic improve our understanding of the Arctic response in terms of global warming.
Evelyn Jäkel, Johannes Stapf, Manfred Wendisch, Marcel Nicolaus, Wolfgang Dorn, and Annette Rinke
The Cryosphere, 13, 1695–1708, https://doi.org/10.5194/tc-13-1695-2019, https://doi.org/10.5194/tc-13-1695-2019, 2019
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The sea ice surface albedo parameterization of a coupled regional climate model was validated against aircraft measurements performed in May–June 2017 north of Svalbard. The albedo parameterization was run offline from the model using the measured parameters surface temperature and snow depth to calculate the surface albedo and the individual fractions of the ice surface subtypes. An adjustment of the variables and additionally accounting for cloud cover reduced the root-mean-squared error.
Kevin Wolf, André Ehrlich, Marek Jacob, Susanne Crewell, Martin Wirth, and Manfred Wendisch
Atmos. Meas. Tech., 12, 1635–1658, https://doi.org/10.5194/amt-12-1635-2019, https://doi.org/10.5194/amt-12-1635-2019, 2019
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Using passive spectral solar radiation and active lidar, radar, and microwave measurements with HALO during NARVAL-II, the cloud droplet number concentration of shallow trade wind cumulus is estimated. With stepwise inclusion of the different instruments into the retrieval, the benefits of the synergetic approach based on artificial measurements and two cloud cases are demonstrated. Significant improvement with the synergetic method compared to the solar-radiation-only method is reported.
Tobias Zinner, Ulrich Schwarz, Tobias Kölling, Florian Ewald, Evelyn Jäkel, Bernhard Mayer, and Manfred Wendisch
Atmos. Meas. Tech., 12, 1167–1181, https://doi.org/10.5194/amt-12-1167-2019, https://doi.org/10.5194/amt-12-1167-2019, 2019
Erlend M. Knudsen, Bernd Heinold, Sandro Dahlke, Heiko Bozem, Susanne Crewell, Irina V. Gorodetskaya, Georg Heygster, Daniel Kunkel, Marion Maturilli, Mario Mech, Carolina Viceto, Annette Rinke, Holger Schmithüsen, André Ehrlich, Andreas Macke, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys., 18, 17995–18022, https://doi.org/10.5194/acp-18-17995-2018, https://doi.org/10.5194/acp-18-17995-2018, 2018
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The paper describes the synoptic development during the ACLOUD/PASCAL airborne and ship-based field campaign near Svalbard in spring 2017. This development is presented using near-surface and upperair meteorological observations, satellite, and model data. We first present time series of these data, from which we identify and characterize three key periods. Finally, we put our observations in historical and regional contexts and compare our findings to other Arctic field campaigns.
Emma Järvinen, Olivier Jourdan, David Neubauer, Bin Yao, Chao Liu, Meinrat O. Andreae, Ulrike Lohmann, Manfred Wendisch, Greg M. McFarquhar, Thomas Leisner, and Martin Schnaiter
Atmos. Chem. Phys., 18, 15767–15781, https://doi.org/10.5194/acp-18-15767-2018, https://doi.org/10.5194/acp-18-15767-2018, 2018
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Using light diffraction it is possible to detect microscopic features within ice particles that have not yet been fully characterized. Here, this technique was applied in airborne measurements, where it was found that majority of atmospheric ice particles have features that significantly change the way ice particles interact with solar light. The microscopic features make ice-containing clouds more reflective than previously thought, which could have consequences for predicting our climate.
Christiane Schulz, Johannes Schneider, Bruna Amorim Holanda, Oliver Appel, Anja Costa, Suzane S. de Sá, Volker Dreiling, Daniel Fütterer, Tina Jurkat-Witschas, Thomas Klimach, Christoph Knote, Martina Krämer, Scot T. Martin, Stephan Mertes, Mira L. Pöhlker, Daniel Sauer, Christiane Voigt, Adrian Walser, Bernadett Weinzierl, Helmut Ziereis, Martin Zöger, Meinrat O. Andreae, Paulo Artaxo, Luiz A. T. Machado, Ulrich Pöschl, Manfred Wendisch, and Stephan Borrmann
Atmos. Chem. Phys., 18, 14979–15001, https://doi.org/10.5194/acp-18-14979-2018, https://doi.org/10.5194/acp-18-14979-2018, 2018
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Aerosol chemical composition measurements in the tropical upper troposphere over the Amazon region show that 78 % of the aerosol in the upper troposphere consists of organic matter. Up to 20 % of the organic aerosol can be attributed to isoprene epoxydiol secondary organic aerosol (IEPOX-SOA). Furthermore, organic nitrates were identified, suggesting a connection to the IEPOX-SOA formation.
Michael Schäfer, Katharina Loewe, André Ehrlich, Corinna Hoose, and Manfred Wendisch
Atmos. Chem. Phys., 18, 13115–13133, https://doi.org/10.5194/acp-18-13115-2018, https://doi.org/10.5194/acp-18-13115-2018, 2018
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Airborne observed horizontal fields of cloud optical thickness are compared with semi-idealized large eddy simulations of Arctic stratus. The comparison focuses on horizontal cloud inhomogeneities and directional features of the small-scale cloud structures. Using inhomogeneity parameters and autocorrelation analysis it is investigated, if the observed small-scale cloud inhomogeneities can be represented by the model. Forcings for cloud inhomogeneities are investigated in a sensitivity study.
Jorge Saturno, Florian Ditas, Marloes Penning de Vries, Bruna A. Holanda, Mira L. Pöhlker, Samara Carbone, David Walter, Nicole Bobrowski, Joel Brito, Xuguang Chi, Alexandra Gutmann, Isabella Hrabe de Angelis, Luiz A. T. Machado, Daniel Moran-Zuloaga, Julian Rüdiger, Johannes Schneider, Christiane Schulz, Qiaoqiao Wang, Manfred Wendisch, Paulo Artaxo, Thomas Wagner, Ulrich Pöschl, Meinrat O. Andreae, and Christopher Pöhlker
Atmos. Chem. Phys., 18, 10391–10405, https://doi.org/10.5194/acp-18-10391-2018, https://doi.org/10.5194/acp-18-10391-2018, 2018
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This study uses satellite observations to track volcanic emissions in eastern Congo and their subsequent transport across the Atlantic Ocean into the Amazon Basin. Aircraft and ground-based observations are used to characterize the influence of volcanogenic aerosol on the chemical and microphysical properties of Amazonian aerosols. Further, this work is an illustrative example of the conditions and dynamics driving the transatlantic transport of African emissions to South America.
Luiz A. T. Machado, Alan J. P. Calheiros, Thiago Biscaro, Scott Giangrande, Maria A. F. Silva Dias, Micael A. Cecchini, Rachel Albrecht, Meinrat O. Andreae, Wagner F. Araujo, Paulo Artaxo, Stephan Borrmann, Ramon Braga, Casey Burleyson, Cristiano W. Eichholz, Jiwen Fan, Zhe Feng, Gilberto F. Fisch, Michael P. Jensen, Scot T. Martin, Ulrich Pöschl, Christopher Pöhlker, Mira L. Pöhlker, Jean-François Ribaud, Daniel Rosenfeld, Jaci M. B. Saraiva, Courtney Schumacher, Ryan Thalman, David Walter, and Manfred Wendisch
Atmos. Chem. Phys., 18, 6461–6482, https://doi.org/10.5194/acp-18-6461-2018, https://doi.org/10.5194/acp-18-6461-2018, 2018
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This overview discuss the main precipitation processes and their sensitivities to environmental conditions in the Central Amazon Basin. It presents a review of the knowledge acquired about cloud processes and rainfall formation in Amazonas. In addition, this study provides a characterization of the seasonal variation and rainfall sensitivities to topography, surface cover, and aerosol concentration. Airplane measurements were evaluated to characterize and contrast cloud microphysical properties.
Trismono C. Krisna, Manfred Wendisch, André Ehrlich, Evelyn Jäkel, Frank Werner, Ralf Weigel, Stephan Borrmann, Christoph Mahnke, Ulrich Pöschl, Meinrat O. Andreae, Christiane Voigt, and Luiz A. T. Machado
Atmos. Chem. Phys., 18, 4439–4462, https://doi.org/10.5194/acp-18-4439-2018, https://doi.org/10.5194/acp-18-4439-2018, 2018
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The optical thickness and particle effective radius of a cirrus above liquid water clouds and a DCC topped by an anvil cirrus are retrieved based on SMART and MODIS radiance measurements. For the cirrus, retrieved particle effective radius are validated with corresponding in situ data using a vertical weighting method. This approach allows to assess the measurements, retrieval algorithms, and derived cloud products.
Meinrat O. Andreae, Armin Afchine, Rachel Albrecht, Bruna Amorim Holanda, Paulo Artaxo, Henrique M. J. Barbosa, Stephan Borrmann, Micael A. Cecchini, Anja Costa, Maximilian Dollner, Daniel Fütterer, Emma Järvinen, Tina Jurkat, Thomas Klimach, Tobias Konemann, Christoph Knote, Martina Krämer, Trismono Krisna, Luiz A. T. Machado, Stephan Mertes, Andreas Minikin, Christopher Pöhlker, Mira L. Pöhlker, Ulrich Pöschl, Daniel Rosenfeld, Daniel Sauer, Hans Schlager, Martin Schnaiter, Johannes Schneider, Christiane Schulz, Antonio Spanu, Vinicius B. Sperling, Christiane Voigt, Adrian Walser, Jian Wang, Bernadett Weinzierl, Manfred Wendisch, and Helmut Ziereis
Atmos. Chem. Phys., 18, 921–961, https://doi.org/10.5194/acp-18-921-2018, https://doi.org/10.5194/acp-18-921-2018, 2018
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We made airborne measurements of aerosol particle concentrations and properties over the Amazon Basin. We found extremely high concentrations of very small particles in the region between 8 and 14 km altitude all across the basin, which had been recently formed by gas-to-particle conversion at these altitudes. This makes the upper troposphere a very important source region of atmospheric particles with significant implications for the Earth's climate system.
Micael A. Cecchini, Luiz A. T. Machado, Manfred Wendisch, Anja Costa, Martina Krämer, Meinrat O. Andreae, Armin Afchine, Rachel I. Albrecht, Paulo Artaxo, Stephan Borrmann, Daniel Fütterer, Thomas Klimach, Christoph Mahnke, Scot T. Martin, Andreas Minikin, Sergej Molleker, Lianet H. Pardo, Christopher Pöhlker, Mira L. Pöhlker, Ulrich Pöschl, Daniel Rosenfeld, and Bernadett Weinzierl
Atmos. Chem. Phys., 17, 14727–14746, https://doi.org/10.5194/acp-17-14727-2017, https://doi.org/10.5194/acp-17-14727-2017, 2017
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This study introduces and explores the concept of gamma phase space. This space is able to represent all possible variations in the cloud droplet size distributions (DSDs). The methodology was applied to recent in situ aircraft measurements over the Amazon. It is shown that the phase space is able to represent several processes occurring in the clouds in a simple manner. The consequences for cloud studies, modeling, and the representation of the transition from warm to mixed phase are discussed.
Ramon Campos Braga, Daniel Rosenfeld, Ralf Weigel, Tina Jurkat, Meinrat O. Andreae, Manfred Wendisch, Ulrich Pöschl, Christiane Voigt, Christoph Mahnke, Stephan Borrmann, Rachel I. Albrecht, Sergej Molleker, Daniel A. Vila, Luiz A. T. Machado, and Lucas Grulich
Atmos. Chem. Phys., 17, 14433–14456, https://doi.org/10.5194/acp-17-14433-2017, https://doi.org/10.5194/acp-17-14433-2017, 2017
Tim Carlsen, Gerit Birnbaum, André Ehrlich, Johannes Freitag, Georg Heygster, Larysa Istomina, Sepp Kipfstuhl, Anaïs Orsi, Michael Schäfer, and Manfred Wendisch
The Cryosphere, 11, 2727–2741, https://doi.org/10.5194/tc-11-2727-2017, https://doi.org/10.5194/tc-11-2727-2017, 2017
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The optical size of snow grains (ropt) affects the reflectivity of snow surfaces and thus the local surface energy budget in particular in polar regions. The temporal evolution of ropt retrieved from ground-based, airborne, and spaceborne remote sensing could reproduce optical in situ measurements for a 2-month period in central Antarctica (2013/14). The presented validation study provided a unique testbed for retrievals of ropt under Antarctic conditions where in situ data are scarce.
Anja Costa, Jessica Meyer, Armin Afchine, Anna Luebke, Gebhard Günther, James R. Dorsey, Martin W. Gallagher, Andre Ehrlich, Manfred Wendisch, Darrel Baumgardner, Heike Wex, and Martina Krämer
Atmos. Chem. Phys., 17, 12219–12238, https://doi.org/10.5194/acp-17-12219-2017, https://doi.org/10.5194/acp-17-12219-2017, 2017
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The paper presents 38 h of in situ cloud spectrometer observations of microphysical cloud properties in the Arctic, midlatitudes and tropics. The clouds are classified via particle concentrations, size distributions, and – as a novelty – small particle aspherical fractions. Cloud-type profiles are given for different temperatures and locations. The results confine regions where different cloud transformation processes occurred and emphasise the importance of small particle shape detection.
Marcus Klingebiel, André Ehrlich, Fanny Finger, Timo Röschenthaler, Suad Jakirlić, Matthias Voigt, Stefan Müller, Rolf Maser, Manfred Wendisch, Peter Hoor, Peter Spichtinger, and Stephan Borrmann
Atmos. Meas. Tech., 10, 3485–3498, https://doi.org/10.5194/amt-10-3485-2017, https://doi.org/10.5194/amt-10-3485-2017, 2017
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Microphysical and radiation measurements were collected with the unique AIRcraft TOwed Sensor Shuttle (AIRTOSS) – Learjet tandem platform. It is a combination of a Learjet 35A research aircraft and an instrumented aerodynamic bird, which can be detached from and retracted back to the aircraft during flight.
AIRTOSS and Learjet are equipped with radiative, cloud microphysical, trace gas,
and meteorological instruments to study cirrus clouds.
André Ehrlich, Eike Bierwirth, Larysa Istomina, and Manfred Wendisch
Atmos. Meas. Tech., 10, 3215–3230, https://doi.org/10.5194/amt-10-3215-2017, https://doi.org/10.5194/amt-10-3215-2017, 2017
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In the Arctic, uncertainties in passive solar remote sensing of cloud properties arise from uncertainties in the assumed spectral surface albedo, mainly determined by the generally unknown effective snow grain size. Therefore, a retrieval method is presented that simultaneously derives liquid water cloud and snow surface parameters, including cloud optical thickness, droplet effective radius, and effective snow grain size. Airborne measurements were used to test the retrieval procedure.
Micael A. Cecchini, Luiz A. T. Machado, Meinrat O. Andreae, Scot T. Martin, Rachel I. Albrecht, Paulo Artaxo, Henrique M. J. Barbosa, Stephan Borrmann, Daniel Fütterer, Tina Jurkat, Christoph Mahnke, Andreas Minikin, Sergej Molleker, Mira L. Pöhlker, Ulrich Pöschl, Daniel Rosenfeld, Christiane Voigt, Bernadett Weinzierl, and Manfred Wendisch
Atmos. Chem. Phys., 17, 10037–10050, https://doi.org/10.5194/acp-17-10037-2017, https://doi.org/10.5194/acp-17-10037-2017, 2017
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We study the effects of aerosol particles and updraft speed on the warm phase of Amazonian clouds. We expand the sensitivity analysis usually found in the literature by concomitantly considering cloud evolution and the effects on droplet size distribution (DSD) shape. The quantitative results show that particle concentration is the primary driver for the vertical profiles of effective diameter and droplet concentration in the warm phase of Amazonian convective clouds.
Evelyn Jäkel, Manfred Wendisch, Trismono C. Krisna, Florian Ewald, Tobias Kölling, Tina Jurkat, Christiane Voigt, Micael A. Cecchini, Luiz A. T. Machado, Armin Afchine, Anja Costa, Martina Krämer, Meinrat O. Andreae, Ulrich Pöschl, Daniel Rosenfeld, and Tianle Yuan
Atmos. Chem. Phys., 17, 9049–9066, https://doi.org/10.5194/acp-17-9049-2017, https://doi.org/10.5194/acp-17-9049-2017, 2017
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Vertical profiles of the cloud particle phase state in tropical deep convective clouds (DCCs) were investigated using airborne imaging spectrometer measurements during the ACRIDICON-CHUVA campaign, which was conducted over the Brazilian rainforest in September 2014. A phase discrimination retrieval was applied to observations of clouds formed in different aerosol conditions. The profiles were compared to in situ and satellite measurements.
Ramon Campos Braga, Daniel Rosenfeld, Ralf Weigel, Tina Jurkat, Meinrat O. Andreae, Manfred Wendisch, Mira L. Pöhlker, Thomas Klimach, Ulrich Pöschl, Christopher Pöhlker, Christiane Voigt, Christoph Mahnke, Stephan Borrmann, Rachel I. Albrecht, Sergej Molleker, Daniel A. Vila, Luiz A. T. Machado, and Paulo Artaxo
Atmos. Chem. Phys., 17, 7365–7386, https://doi.org/10.5194/acp-17-7365-2017, https://doi.org/10.5194/acp-17-7365-2017, 2017
Kevin Wolf, André Ehrlich, Tilman Hüneke, Klaus Pfeilsticker, Frank Werner, Martin Wirth, and Manfred Wendisch
Atmos. Chem. Phys., 17, 4283–4303, https://doi.org/10.5194/acp-17-4283-2017, https://doi.org/10.5194/acp-17-4283-2017, 2017
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The potential of airborne radiance measurements in the sideward and nadir directions for cirrus remote sensing is investigated. Therefore radiative transfer simulations were used and the sensitivity of upward radiance with respect to optical thickness, effective radius, surface albedo, wavelength and viewing angle was studied. It was shown that sideward observations lead to more accurate retrieval results. Investigating a case study of ML-CIRRUS, these findings are confirmed.
Michael Schäfer, Eike Bierwirth, André Ehrlich, Evelyn Jäkel, Frank Werner, and Manfred Wendisch
Atmos. Chem. Phys., 17, 2359–2372, https://doi.org/10.5194/acp-17-2359-2017, https://doi.org/10.5194/acp-17-2359-2017, 2017
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Cloud optical thickness fields, retrieved from solar spectral radiance measurements, are used to investigate the directional structure of horizontal cloud inhomogeneities with scalar one-dimensional inhomogeneity parameters, two-dimensional auto-correlation functions, and two-dimensional Fourier analysis. The investigations reveal that it is not sufficient to quantify horizontal cloud inhomogeneities by one-dimensional inhomogeneity parameters; two-dimensional parameters are necessary.
Fanny Finger, Frank Werner, Marcus Klingebiel, André Ehrlich, Evelyn Jäkel, Matthias Voigt, Stephan Borrmann, Peter Spichtinger, and Manfred Wendisch
Atmos. Chem. Phys., 16, 7681–7693, https://doi.org/10.5194/acp-16-7681-2016, https://doi.org/10.5194/acp-16-7681-2016, 2016
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Solar spectra of optical layer properties of cirrus have been derived from the first truly collocated airborne radiation measurements using an aircraft and a towed sensor platform. The measured layer properties differ slightly due to horizontal cirrus inhomogeneities and the influence of low-level water clouds. Applying a 1-D radiative transfer model sensitivity studies were performed. It was found that if a low-level cloud is not considered, the solar cooling of the cirrus is strongly overestimated.
S. T. Martin, P. Artaxo, L. A. T. Machado, A. O. Manzi, R. A. F. Souza, C. Schumacher, J. Wang, M. O. Andreae, H. M. J. Barbosa, J. Fan, G. Fisch, A. H. Goldstein, A. Guenther, J. L. Jimenez, U. Pöschl, M. A. Silva Dias, J. N. Smith, and M. Wendisch
Atmos. Chem. Phys., 16, 4785–4797, https://doi.org/10.5194/acp-16-4785-2016, https://doi.org/10.5194/acp-16-4785-2016, 2016
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The Observations and Modeling of the Green Ocean Amazon (GoAmazon2014/5) Experiment took place in central Amazonia throughout 2014 and 2015. The experiment focused on the complex links among vegetation, atmospheric chemistry, and aerosol production on the one hand and their connections to aerosols, clouds, and precipitation on the other, especially when altered by urban pollution. This article serves as an introduction to the special issue of publications presenting findings of this experiment.
E. Jäkel, B. Mey, R. Levy, X. Gu, T. Yu, Z. Li, D. Althausen, B. Heese, and M. Wendisch
Atmos. Meas. Tech., 8, 5237–5249, https://doi.org/10.5194/amt-8-5237-2015, https://doi.org/10.5194/amt-8-5237-2015, 2015
A. Ehrlich and M. Wendisch
Atmos. Meas. Tech., 8, 3671–3684, https://doi.org/10.5194/amt-8-3671-2015, https://doi.org/10.5194/amt-8-3671-2015, 2015
M. Schäfer, E. Bierwirth, A. Ehrlich, E. Jäkel, and M. Wendisch
Atmos. Chem. Phys., 15, 8147–8163, https://doi.org/10.5194/acp-15-8147-2015, https://doi.org/10.5194/acp-15-8147-2015, 2015
M. Klingebiel, A. de Lozar, S. Molleker, R. Weigel, A. Roth, L. Schmidt, J. Meyer, A. Ehrlich, R. Neuber, M. Wendisch, and S. Borrmann
Atmos. Chem. Phys., 15, 617–631, https://doi.org/10.5194/acp-15-617-2015, https://doi.org/10.5194/acp-15-617-2015, 2015
C. Fricke, A. Ehrlich, E. Jäkel, B. Bohn, M. Wirth, and M. Wendisch
Atmos. Chem. Phys., 14, 1943–1958, https://doi.org/10.5194/acp-14-1943-2014, https://doi.org/10.5194/acp-14-1943-2014, 2014
M. Schäfer, E. Bierwirth, A. Ehrlich, F. Heyner, and M. Wendisch
Atmos. Meas. Tech., 6, 1855–1868, https://doi.org/10.5194/amt-6-1855-2013, https://doi.org/10.5194/amt-6-1855-2013, 2013
E. Bierwirth, A. Ehrlich, M. Wendisch, J.-F. Gayet, C. Gourbeyre, R. Dupuy, A. Herber, R. Neuber, and A. Lampert
Atmos. Meas. Tech., 6, 1189–1200, https://doi.org/10.5194/amt-6-1189-2013, https://doi.org/10.5194/amt-6-1189-2013, 2013
E. Jäkel, J. Walter, and M. Wendisch
Atmos. Meas. Tech., 6, 539–547, https://doi.org/10.5194/amt-6-539-2013, https://doi.org/10.5194/amt-6-539-2013, 2013
E. Jäkel, M. Wendisch, and B. Mayer
Atmos. Meas. Tech., 6, 527–537, https://doi.org/10.5194/amt-6-527-2013, https://doi.org/10.5194/amt-6-527-2013, 2013
Henning Dorff, Florian Ewald, Heike Konow, Mario Mech, Davide Ori, Vera Schemann, Andreas Walbröl, Manfred Wendisch, and Felix Ament
Atmos. Chem. Phys., 25, 8329–8354, https://doi.org/10.5194/acp-25-8329-2025, https://doi.org/10.5194/acp-25-8329-2025, 2025
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Using observations of an Arctic atmospheric river (AR) from a long-range research aircraft, we analyse how moisture transported into the Arctic by the AR is transformed and how it interacts with the Arctic environment. The moisture transport divergence is the main driver of local moisture change over time. Surface precipitation and evaporation are rather weak when averaged over extended AR sectors, although considerable heterogeneity of precipitation within the AR is observed.
Zsófia Jurányi, Christof Lüpkes, Frank Stratmann, Jörg Hartmann, Jonas Schaefer, Anna-Marie Jörss, Alexander Schulz, Bruno Wetzel, David Simon, Eduard Gebhard, Maximilian Stöhr, Paula Hofmann, Dirk Kalmbach, Sarah Grawe, Manfred Wendisch, and Andreas Herber
Atmos. Meas. Tech., 18, 3477–3494, https://doi.org/10.5194/amt-18-3477-2025, https://doi.org/10.5194/amt-18-3477-2025, 2025
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Understanding the lowest layers of the atmosphere is crucial for climate research, especially in the Arctic. Our study introduces the T-Bird, an aircraft-towed platform designed to measure turbulence and aerosol properties at extremely low altitudes. Traditional aircraft cannot access this region, making the T-Bird a breakthrough for capturing critical atmospheric data. Its first deployment over the Arctic demonstrated its potential to improve our understanding of polar processes.
Nina Maherndl, Alessandro Battaglia, Anton Kötsche, and Maximilian Maahn
Atmos. Meas. Tech., 18, 3287–3304, https://doi.org/10.5194/amt-18-3287-2025, https://doi.org/10.5194/amt-18-3287-2025, 2025
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Accurate measurements of ice water content (IWC) and snowfall rate (SR) are challenging due to high spatial variability and limitations of our measurement techniques. Here, we present a novel method to derive IWC and SR from W-band cloud radar observations, considering the degree of riming. We also investigate the use of the liquid water path (LWP) as a proxy for the occurrence of riming. LWP is easier to measure, so that the method can be applied to both ground-based and space-based instruments.
Elena Shevnina, Timo Vihma, Miguel Potes, and Tuomas Naakka
EGUsphere, https://doi.org/10.5194/egusphere-2025-1964, https://doi.org/10.5194/egusphere-2025-1964, 2025
This preprint is open for discussion and under review for Hydrology and Earth System Sciences (HESS).
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The study first estimated the summertime evaporation over lakes located in coastal Antarctica with direct (eddy-covariance) measurements collected during two austral summers (December–January) in 2017–2018 and 2019–2020. The lake evaporation was on average 1.6 mm d-1 in the ice break-up period, and it doubled in the ice free period. The bulk aerodynamic method with a site-specific transfer coefficient of moisture well reproduced the observed day-to-day variations in evaporation over lakes.
Guillaume Feger, Jean-Pierre Chaboureau, Thibaut Dauhut, Julien Delanoë, and Pierre Coutris
Atmos. Chem. Phys., 25, 7447–7465, https://doi.org/10.5194/acp-25-7447-2025, https://doi.org/10.5194/acp-25-7447-2025, 2025
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Saharan air at the trade wind layer, cold pools, and dry upper troposphere has these three main factors inhibiting the cyclogenesis of the Pierre Henri mesoscale convective system. The findings were obtained through observations made during two flights of the Clouds-Atmospheric Dynamics-Dust Interactions in West Africa (CADDIWA) campaign and a convection-permitting simulation run with the Meso-NH model. They provide new insights into the complex dynamics of cyclogenesis in the Cabo Verde region and challenge the existing model of the Saharan Air Layer (SAL).
Kerstin Ebell, Christian Buhren, Rosa Gierens, Giovanni Chellini, Melanie Lauer, Andreas Walbröl, Sandro Dahlke, Pavel Krobot, and Mario Mech
Atmos. Chem. Phys., 25, 7315–7342, https://doi.org/10.5194/acp-25-7315-2025, https://doi.org/10.5194/acp-25-7315-2025, 2025
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Ground-based observations of precipitation are rare in the Arctic. Since 2017, additional temporally highly resolved precipitation measurements have been carried out by a precipitation gauge and an optical precipitation sensor at Ny-Ålesund, Svalbard. These new data facilitate the distinction between liquid and solid precipitation. Using reanalysis data, we also find that water vapor transport contributes strongly to precipitation and especially to extreme precipitation events.
Linda Forster, Anna Weber, and Bernhard Mayer
EGUsphere, https://doi.org/10.5194/egusphere-2025-1369, https://doi.org/10.5194/egusphere-2025-1369, 2025
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
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CrystalTrace is a Monte Carlo raytracing algorithm for simulating radiative transfer in ice clouds with different crystal shapes and orientations. Integrated into libradtran’s MYSTIC solver, it enables efficient, realistic simulations of ice alongside water clouds. By computing single-scattering properties online at the crystal scale, it eliminates the need for precomputed lookup tables, improving efficiency and angular resolution for satellite, airborne, and ground-based observation retrievals.
Gregor Köcher and Tobias Zinner
EGUsphere, https://doi.org/10.5194/egusphere-2025-2475, https://doi.org/10.5194/egusphere-2025-2475, 2025
This preprint is open for discussion and under review for Geoscientific Model Development (GMD).
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Simulations of convective precipitation events with microphysics schemes of varying complexity are statistically evaluated against polarimetric radar observations. Convective precipitation is potentially hazardous and difficult to predict. Cloud microphysics schemes contribute significantly to this uncertainty. Depending on the microphysics used, the simulated precipitation distribution varies significantly. The main reason for these differences are the underlying rain drop size distributions.
Anna Weber, Gregor Köcher, and Bernhard Mayer
EGUsphere, https://doi.org/10.5194/egusphere-2025-2554, https://doi.org/10.5194/egusphere-2025-2554, 2025
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
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A neural-network-based fast forward operator for polarized 3D radiative transfer is presented. The forward operator uses the new independent column local half-sphere approximation (IDEFAX). Polarized radiances simulated with IFEDAX and the forward operator were validated against full 3D radiative transfer simulations with MYSTIC and show a significantly improved representation of 3D radiative effects compared to the plane-parallel independent column approximation at comparable computation times.
Anna Breuninger, Philipp Joppe, Jonas Wilsch, Cornelis Schwenk, Heiko Bozem, Nicolas Emig, Laurin Merkel, Rainer Rossberg, Timo Keber, Arthur Kutschka, Philipp Waleska, Stefan Hofmann, Sarah Richter, Florian Ungeheuer, Konstantin Dörholt, Thorsten Hoffmann, Annette Miltenberger, Johannes Schneider, Peter Hoor, and Alexander L. Vogel
EGUsphere, https://doi.org/10.5194/egusphere-2025-3129, https://doi.org/10.5194/egusphere-2025-3129, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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This study investigates molecular organic aerosol composition in the upper troposphere and lower stratosphere from an airborne campaign over Central Europe in summer 2024. Via ultra-high-performance liquid chromatography and high-resolution mass spectrometry of tropospheric and stratospheric filter samples, we identified various organic compounds. Our findings underscore the significant cross-tropopause transport of biogenic secondary organic aerosol and anthropogenic pollutants.
Heiko Bozem, Philipp Joppe, Yun Li, Nicolas Emig, Armin Afchine, Anna Breuninger, Joachim Curtius, Stefan Hofmann, Sadath Ismayil, Konrad Kandler, Daniel Kunkel, Arthur Kutschka, Hans-Christoph Lachnitt, Andreas Petzold, Sarah Richter, Timo Röschenthaler, Christian Rolf, Lisa Schneider, Johannes Schneider, Alexander Vogel, and Peter Hoor
EGUsphere, https://doi.org/10.5194/egusphere-2025-3175, https://doi.org/10.5194/egusphere-2025-3175, 2025
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
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Deployed on a Learjet as a tandem measurement platform during TPEx I (TropoPause composition gradients and mixing Experiment) campaign in June 2024, the new TPC-TOSS (TropoPause Composition Towed Sensor Shuttle) system delivers high-resolution in situ data on ozone, aerosol, clouds, and key weather parameters. Laboratory and in-flight tests confirmed its precision and stability. Observed gradients near the tropopause reveal active mixing and transport processes in the tropopause region.
Masatomo Fujiwara, Bomin Sun, Anthony Reale, Domenico Cimini, Salvatore Larosa, Lori Borg, Christoph von Rohden, Michael Sommer, Ruud Dirksen, Marion Maturilli, Holger Vömel, Rigel Kivi, Bruce Ingleby, Ryan J. Kramer, Belay Demoz, Fabio Madonna, Fabien Carminati, Owen Lewis, Brett Candy, Christopher Thomas, David Edwards, Noersomadi, Kensaku Shimizu, and Peter Thorne
Atmos. Meas. Tech., 18, 2919–2955, https://doi.org/10.5194/amt-18-2919-2025, https://doi.org/10.5194/amt-18-2919-2025, 2025
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We assess and illustrate the benefits of high-altitude attainment of balloon-borne radiosonde soundings up to and beyond 10 hPa level from various aspects. We show that the extra costs and technical challenges involved in consistent attainment of high ascents are more than outweighed by the benefits for a broad variety of real-time and delayed-mode applications. Consistent attainment of high ascents should therefore be pursued across the balloon observational network.
Aymeric Dziduch, Guillaume Mioche, Quentin Coopman, Clément Bazantay, Julien Delanoë, and Olivier Jourdan
EGUsphere, https://doi.org/10.5194/egusphere-2025-2698, https://doi.org/10.5194/egusphere-2025-2698, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Low-level clouds play a central role in the Arctic climate, modulating the surface energy budget with competing warming and cooling effects. In this study, radar-lidar satellite products are used to investigate the geographical and seasonal variations of different cloud types observed over eight years. Oceanic regions are characterized by high occurrences of low-level mixed-phase clouds, which are influenced by atmospheric stability conditions, surface temperatures and cold air outbreaks.
Aino Ovaska, Elio Rauth, Daniel Holmberg, Paulo Artaxo, John Backman, Benjamin Bergmans, Don Collins, Marco Aurélio Franco, Shahzad Gani, Roy M. Harrison, Rakes K. Hooda, Tareq Hussein, Antti-Pekka Hyvärinen, Kerneels Jaars, Adam Kristensson, Markku Kulmala, Lauri Laakso, Ari Laaksonen, Nikolaos Mihalopoulos, Colin O'Dowd, Jakub Ondracek, Tuukka Petäjä, Kristina Plauškaitė, Mira Pöhlker, Ximeng Qi, Peter Tunved, Ville Vakkari, Alfred Wiedensohler, Kai Puolamäki, Tuomo Nieminen, Veli-Matti Kerminen, Victoria A. Sinclair, and Pauli Paasonen
Aerosol Research Discuss., https://doi.org/10.5194/ar-2025-18, https://doi.org/10.5194/ar-2025-18, 2025
Preprint under review for AR
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We trained machine learning models to estimate the number of aerosol particles large enough to form clouds and generated daily estimates for the entire globe. The models performed well in many continental regions but struggled in remote and marine areas. Still, this approach offers a way to quantify these particles in areas that lack direct measurements, helping us understand their influence on clouds and climate on a global scale.
Théophane Costabloz, Frédéric Burnet, Christine Lac, Pauline Martinet, Julien Delanoë, Susana Jorquera, and Maroua Fathalli
Atmos. Chem. Phys., 25, 6539–6573, https://doi.org/10.5194/acp-25-6539-2025, https://doi.org/10.5194/acp-25-6539-2025, 2025
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This study documents vertical profiles of liquid water content (LWC) in fogs from in situ measurements collected during the SOFOG3D field campaign in 2019–2020. The analysis of 140 vertical profiles reveals a reverse trend in LWC, maximum values at ground decreasing with height, during stable conditions in optically thin fogs, evolving towards quasi-adiabatic characteristics when fogs become thick. These results offer new perspectives for better constraining fog numerical simulations.
Ann Kristin Naumann, Monika Esch, and Bjorn Stevens
Atmos. Chem. Phys., 25, 6429–6444, https://doi.org/10.5194/acp-25-6429-2025, https://doi.org/10.5194/acp-25-6429-2025, 2025
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This study explores how uncertainties in the representation of microphysical processes affect the tropical condensate distribution in the global storm-resolving model ICON. The results point to the importance of the fall speed of hydrometeor particles and to a simple relationship: the faster a condensate falls, the less there is of it. Implications for the energy balance and precipitation properties are discussed.
Sandrine Bony, Basile Poujol, Brett McKim, Nicolas Rochetin, Marie Lothon, Julia Windmiller, Nicolas Maury, Clarisse Dufaux, Louis Jaffeux, Patrick Chazette, and Julien Delanoë
EGUsphere, https://doi.org/10.5194/egusphere-2025-2839, https://doi.org/10.5194/egusphere-2025-2839, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Space photographs of the Earth show that clouds form diverse, common but poorly understood cloud patterns. The analysis of observations gathered from research aircraft over the tropical ocean shows that the merging of thermals and clouds in the first kilometer of the atmosphere plays a key role in controlling the size, depth and spacing of clouds. This reveals a fundamental process through which clouds interact with each other and with their environment.
Patrick Konjari, Christian Rolf, Martina Krämer, Armin Afchine, Nicole Spelten, Irene Bartolome Garcia, Annette Miltenberger, Nicolar Emig, Philipp Joppe, Johannes Schneider, Yun Li, Andreas Petzold, Heiko Bozem, and Peter Hoor
EGUsphere, https://doi.org/10.5194/egusphere-2025-2847, https://doi.org/10.5194/egusphere-2025-2847, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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We investigated how a powerful storm over southern Sweden in June 2024 transported ice particles and moist air into the normally dry stratosphere. We observed unusually high water vapor and ice levels up to 1.5 kilometers above the tropopause. Although the extra water vapor lasted only a few days to weeks, it shows how such storms can temporarily alter the upper atmosphere’s composition.
Kevin Wolf, Evelyn Jäkel, André Ehrlich, Michael Schäfer, Hannes Feilhauer, Andreas Huth, Alexandra Weigelt, and Manfred Wendisch
Biogeosciences, 22, 2909–2933, https://doi.org/10.5194/bg-22-2909-2025, https://doi.org/10.5194/bg-22-2909-2025, 2025
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This paper reports an investigation of the influence of clouds on vegetation albedo using a coupled atmosphere–vegetation radiative transfer model. Both models are iteratively linked to simulate cloud–vegetation–radiation interactions over canopies more realistically. Solar, spectral, and broadband irradiances have been simulated under varying cloud conditions. The simulated irradiances were used to investigate the spectral and broadband effect of clouds on vegetation albedo.
Ewan Crosbie, Johnathan W. Hair, Amin R. Nehrir, Richard A. Ferrare, Chris Hostetler, Taylor Shingler, David Harper, Marta Fenn, James Collins, Rory Barton-Grimley, Brian Collister, K. Lee Thornhill, Christiane Voigt, Simon Kirschler, and Armin Sorooshian
Atmos. Meas. Tech., 18, 2639–2658, https://doi.org/10.5194/amt-18-2639-2025, https://doi.org/10.5194/amt-18-2639-2025, 2025
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A method was developed to extract information from airborne lidar observations about the distribution of ice and liquid water within clouds. The method specifically targets signatures of horizontal and vertical gradients in ice and water that appear in the polarization of the lidar signals. The method was tested against direct measurements of the cloud properties collected by a second aircraft.
Qiang Li and Silke Groß
EGUsphere, https://doi.org/10.5194/egusphere-2025-2052, https://doi.org/10.5194/egusphere-2025-2052, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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This study presents the cirrus occurrence and optical properties at high- and midlatitudes using the satellite lidar measurements. The results indicate the differences in cirrus occurrence and optical properties across latitudes. Besides seasonality, the cirrus extinction and depolarization show a consistent decrease with increasing latitude. The potential causes are discussed and it turns out that aerosol particles show much larger concentrations at midlatitudes than at high-latitudes.
Kevin Ohneiser, Patric Seifert, Willi Schimmel, Fabian Senf, Tom Gaudek, Martin Radenz, Audrey Teisseire, Veronika Ettrichrätz, Teresa Vogl, Nina Maherndl, Nils Pfeifer, Jan Henneberger, Anna J. Miller, Nadja Omanovic, Christopher Fuchs, Huiying Zhang, Fabiola Ramelli, Robert Spirig, Anton Kötsche, Heike Kalesse-Los, Maximilian Maahn, Heather Corden, Alexis Berne, Majid Hajipour, Hannes Griesche, Julian Hofer, Ronny Engelmann, Annett Skupin, Albert Ansmann, and Holger Baars
EGUsphere, https://doi.org/10.5194/egusphere-2025-2482, https://doi.org/10.5194/egusphere-2025-2482, 2025
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This study focuses on a seeder-feeder cloud system on 8 Jan 2024 in Eriswil, Switzerland. It is shown how the interaction of these cloud systems changes the cloud microphysical properties and the precipitation patterns. A big set of advanced remote-sensing techniques and retrieval algorithms are applied, so that a detailed view on the seeder-feeder cloud system is available. The gained knowledge can be used to improve weather models and weather forecasts.
Denghui Ji, Christoph Ritter, Xiaoyu Sun, Manuel Moser, Christiane Voigt, Mathias Palm, and Justus Notholt
EGUsphere, https://doi.org/10.5194/egusphere-2025-1932, https://doi.org/10.5194/egusphere-2025-1932, 2025
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We discovered a process where large aerosols help small water droplets in Arctic clouds grow, even when conditions normally favor ice. Unlike the traditional view, this process may explain how liquid and ice can coexist in cold clouds. Based on theory and aircraft data, our findings provide new insight into the microphysics of mixed-phase clouds, which could improve understanding of how Arctic clouds affect climate.
Gregor Neumann, Andreas Marsing, Theresa Harlass, Daniel Sauer, Simon Braun, Magdalena Pühl, Christopher Heckl, Paul Stock, Elena De La Torre Castro, Valerian Hahn, Anke Roiger, Christiane Voigt, Simon Unterstraßer, Jean Cammas, Charles Renard, Roberta Vasenden, Arnold Vasenden, and Tina Jurkat-Witschas
EGUsphere, https://doi.org/10.5194/egusphere-2025-2026, https://doi.org/10.5194/egusphere-2025-2026, 2025
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
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This study presents the first successful in-flight emission characterization of a turboprop engine using a fully autonomous airborne measurement platform, offering new insights into the atmospheric impacts of regional aviation. By equipping the high-altitude Grob G 520 Egrett with a suite of custom and modified commercial instruments, we demonstrate precise, high-resolution measurements of aerosol particles, trace gases, and contrail ice in the engine exhaust plume at cruise altitudes.
Manfred Wendisch, Benjamin Kirbus, Davide Ori, Matthew D. Shupe, Susanne Crewell, Harald Sodemann, and Vera Schemann
EGUsphere, https://doi.org/10.5194/egusphere-2025-2062, https://doi.org/10.5194/egusphere-2025-2062, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Aircraft observations of air parcels moving into and out of the Arctic are reported. From the data, heating and cooling as well as drying and moistening of the air masses along their way into and out of the Arctic could be measured for the first time. These data enable to evaluate if numerical weather prediction models are able to accurately represent these air mass transformations. This work helps to model the future climate changes in the Arctic, which are important for mid-latitude weather.
Kaiqi Wang, Kai Bi, Shuling Chen, Markus Hartmann, Zhijun Wu, Jiyu Gao, Xiaoyu Xu, Yuhan Cheng, Mengyu Huang, Yunbo Chen, Huiwen Xue, Bingbing Wang, Yaqiong Hu, Xiongying Zhang, Xincheng Ma, Ruijie Li, Ping Tian, Ottmar Möhler, Heike Wex, Frank Startmann, Jie Chen, and Xianda Gong
EGUsphere, https://doi.org/10.5194/egusphere-2025-1873, https://doi.org/10.5194/egusphere-2025-1873, 2025
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Understanding how ice forms in clouds is crucial for predicting weather and climate; however, accurately measuring the ice-nucleating particles that trigger ice formation remains challenging. We developed an advanced instrument called the Freezing Ice Nucleation Detection Analyzer. By refining temperature control, automating freezing detection, and rigorously testing, we demonstrated that this instrument can reliably measure ice-nucleating particles across diverse conditions.
Kevin Wolf, Evelyn Jäkel, André Ehrlich, Michael Schäfer, Hannes Feilhauer, Andreas Huth, and Manfred Wendisch
EGUsphere, https://doi.org/10.5194/egusphere-2025-2082, https://doi.org/10.5194/egusphere-2025-2082, 2025
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This paper presents combined atmosphere-vegetation radiative transfer simulations to systematically investigate cloud-induced biases in remotely sensed vegetation indices (VIs) derived from below-cloud measurements. The biases in VIs have been investigated for the general case of two-band VIs, and for the special cases of the normalized difference vegetation index (NDVI), the normalized difference water index (NDWI), and the enhanced vegetation index (EVI).
Florian Tornow, Ann Fridlind, George Tselioudis, Brian Cairns, Andrew Ackerman, Seethala Chellappan, David Painemal, Paquita Zuidema, Christiane Voigt, Simon Kirschler, and Armin Sorooshian
Atmos. Chem. Phys., 25, 5053–5074, https://doi.org/10.5194/acp-25-5053-2025, https://doi.org/10.5194/acp-25-5053-2025, 2025
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The recent NASA campaign ACTIVATE (Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment) performed 71 tandem flights in mid-latitude marine cold-air outbreaks off the US eastern seaboard. We provide meteorological and cloud transition stage context, allowing us to identify days that are most suitable for Lagrangian modeling and analysis. Surveyed cloud properties show signatures of cloud microphysical processes, such as cloud-top entrainment and secondary ice formation.
Albert Ansmann, Cristofer Jimenez, Johanna Roschke, Johannes Bühl, Kevin Ohneiser, Ronny Engelmann, Martin Radenz, Hannes Griesche, Julian Hofer, Dietrich Althausen, Daniel A. Knopf, Sandro Dahlke, Tom Gaudek, Patric Seifert, and Ulla Wandinger
Atmos. Chem. Phys., 25, 4847–4866, https://doi.org/10.5194/acp-25-4847-2025, https://doi.org/10.5194/acp-25-4847-2025, 2025
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In this study, we focus on the potential impact of wildfire smoke on cirrus formation. For the first time, state-of-the-art aerosol and cirrus observations with lidar and radar, presented in this paper (Part 1 of a series of two articles), are closely linked to the comprehensive modeling of gravity-wave-induced ice nucleation in cirrus evolution processes, presented in a companion paper (Part 2). We found a clear impact of wildfire smoke on cirrus evolution.
Dennis Niedermeier, Rasmus Hoffmann, Silvio Schmalfuss, Wiebke Frey, Fabian Senf, Olaf Hellmuth, Mira Pöhlker, and Frank Stratmann
Aerosol Research, 3, 219–230, https://doi.org/10.5194/ar-3-219-2025, https://doi.org/10.5194/ar-3-219-2025, 2025
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This study examines the deliquescence behavior of NaCl particles in a turbulent humidity field using the wind tunnel LACIS-T (Turbulent Leipzig Aerosol Cloud Interaction Simulator). The results show that turbulent relative humidity (RH) fluctuations affect the number of deliquesced particles, depending on the mean RH, strength of humidity fluctuations, and particle residence time. It turns out that, in addition to the mean RH, it is essential to consider humidity fluctuations and particle history when determining the phase state of the deliquescent particles.
Philipp Joppe, Johannes Schneider, Jonas Wilsch, Heiko Bozem, Anna Breuninger, Joachim Curtius, Martin Ebert, Nicolas Emig, Peter Hoor, Sadath Ismayil, Konrad Kandler, Daniel Kunkel, Isabel Kurth, Hans-Christoph Lachnitt, Yun Li, Annette Miltenberger, Sarah Richter, Christian Rolf, Lisa Schneider, Cornelis Schwenk, Nicole Spelten, Alexander L. Vogel, Yafang Cheng, and Stephan Borrmann
EGUsphere, https://doi.org/10.5194/egusphere-2025-1346, https://doi.org/10.5194/egusphere-2025-1346, 2025
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We show measurements of a filament with biomass burning influence transported by a warm conveyor belt (WCB) into the tropopause region over Europe. The pollution originates from Canadian forest fires and is transported in the lower troposphere towards Europe. The WCB transport is followed by mixing with air masses of stratospheric chemical signatures. We hypothesize that this mixing leads to a change in the vertical gradient of the potential temperature.
Yu-Wen Chen, K. Sebastian Schmidt, Hong Chen, Steven T. Massie, Susan S. Kulawik, and Hironobu Iwabuchi
Atmos. Meas. Tech., 18, 1859–1884, https://doi.org/10.5194/amt-18-1859-2025, https://doi.org/10.5194/amt-18-1859-2025, 2025
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CO2 column-averaged dry-air mole fractions can be retrieved from space using spectrometers like OCO-2. However, nearby clouds induce spectral distortions that bias these retrievals beyond the accuracy needed for global CO2 source and sink assessments. This study employs a physics-based linearization approach to represent 3D cloud effects and introduces radiance-level mitigation techniques for actual OCO-2 data, enabling the operational implementation of these corrections.
Logan Thomas Mitchell, Connor J. Flynn, Kristina Pistone, Samuel E. LeBlanc, K. Sebastian Schmidt, and Jens Redemann
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2025-31, https://doi.org/10.5194/essd-2025-31, 2025
Preprint under review for ESSD
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During 2016–2018, NASA conducted an airborne field campaign over the Southeast Atlantic Ocean to study biomass burning aerosols emitted from Southern African fires. These aerosols then interact with stratocumulus clouds over the Southeast Atlantic, which is difficult for climate models to account for. Our instrument, 4STAR, determines aerosol radiative properties. A dataset was already created for 2016, but additional quality control was required to address instrument issues for 2017 and 2018.
Meloë S. F. Kacenelenbogen, Ralph Kuehn, Nandana Amarasinghe, Kerry Meyer, Edward Nowottnick, Mark Vaughan, Hong Chen, Sebastian Schmidt, Richard Ferrare, John Hair, Robert Levy, Hongbin Yu, Paquita Zuidema, Robert Holz, and Willem Marais
EGUsphere, https://doi.org/10.5194/egusphere-2025-1403, https://doi.org/10.5194/egusphere-2025-1403, 2025
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Aerosols perturb the radiation balance of the Earth-atmosphere system. To reduce the uncertainty in quantifying present-day climate change, we combine two satellite sensors and a model to assess the aerosol effects on radiation in all-sky conditions. Satellite-based and coincident aircraft measurements of aerosol radiative effects agree well over the Southeast Atlantic. This constitutes a crucial first evaluation before we apply our method to more years and regions of the world.
Denghui Ji, Mathias Palm, Matthias Buschmann, Kerstin Ebell, Marion Maturilli, Xiaoyu Sun, and Justus Notholt
Atmos. Chem. Phys., 25, 3889–3904, https://doi.org/10.5194/acp-25-3889-2025, https://doi.org/10.5194/acp-25-3889-2025, 2025
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Our study explores how certain aerosols, like sea salt, affect infrared heat radiation in the Arctic, potentially speeding up warming. We used advanced technology to measure aerosol composition and found that these particles grow with humidity, significantly increasing their heat-trapping effect in the infrared region, especially in winter. Our findings suggest these aerosols could be a key factor in Arctic warming, emphasizing the importance of understanding aerosols for climate prediction.
Yubing Cheng, Bin Cheng, Roberta Pirazzini, Amy R. Macfarlane, Timo Vihma, Wolfgang Dorn, Ruzica Dadic, Martin Schneebeli, Stefanie Arndt, and Annette Rinke
EGUsphere, https://doi.org/10.5194/egusphere-2025-1164, https://doi.org/10.5194/egusphere-2025-1164, 2025
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We study snow density from the MOSAiC expedition. Several snow density schemes were tested and compared with observation. A thermodynamic ice model was employed to assess the impact of snow density and precipitation on the thermal regime of sea ice. The parameterized mean snow densities are consistent with observations. Increased snow density reduces snow and ice temperatures, promoting ice growth, while increased precipitation leads to warmer snow and ice temperatures and reduced ice thickness.
André Ehrlich, Susanne Crewell, Andreas Herber, Marcus Klingebiel, Christof Lüpkes, Mario Mech, Sebastian Becker, Stephan Borrmann, Heiko Bozem, Matthias Buschmann, Hans-Christian Clemen, Elena De La Torre Castro, Henning Dorff, Regis Dupuy, Oliver Eppers, Florian Ewald, Geet George, Andreas Giez, Sarah Grawe, Christophe Gourbeyre, Jörg Hartmann, Evelyn Jäkel, Philipp Joppe, Olivier Jourdan, Zsófia Jurányi, Benjamin Kirbus, Johannes Lucke, Anna E. Luebke, Maximilian Maahn, Nina Maherndl, Christian Mallaun, Johanna Mayer, Stephan Mertes, Guillaume Mioche, Manuel Moser, Hanno Müller, Veronika Pörtge, Nils Risse, Greg Roberts, Sophie Rosenburg, Johannes Röttenbacher, Michael Schäfer, Jonas Schaefer, Andreas Schäfler, Imke Schirmacher, Johannes Schneider, Sabrina Schnitt, Frank Stratmann, Christian Tatzelt, Christiane Voigt, Andreas Walbröl, Anna Weber, Bruno Wetzel, Martin Wirth, and Manfred Wendisch
Earth Syst. Sci. Data, 17, 1295–1328, https://doi.org/10.5194/essd-17-1295-2025, https://doi.org/10.5194/essd-17-1295-2025, 2025
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This paper provides an overview of the HALO–(AC)3 aircraft campaign data sets, the campaign-specific instrument operation, data processing, and data quality. The data set comprises in situ and remote sensing observations from three research aircraft: HALO, Polar 5, and Polar 6. All data are published in the PANGAEA database by instrument-separated data subsets. It is highlighted how the scientific analysis of the HALO–(AC)3 data benefits from the coordinated operation of three aircraft.
Sebastian Becker, André Ehrlich, Michael Schäfer, and Manfred Wendisch
EGUsphere, https://doi.org/10.5194/egusphere-2025-1210, https://doi.org/10.5194/egusphere-2025-1210, 2025
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Clouds interact with solar radiation and can alter the surface temperature. The strength of this cloud impact is driven by cloud properties as well as solar elevation and surface reflection. Since these dependences are poorly represented in climate models, cloud, surface, and radiation observations are used to quantify the contributions of the drivers in the Arctic. It is shown that the weaker surface reflection dominates the stronger cooling effect of clouds over open ocean compared to sea ice.
Joshua Jeremias Müller, Michael Schäfer, Sophie Rosenburg, André Ehrlich, and Manfred Wendisch
EGUsphere, https://doi.org/10.5194/amt-2024-3967, https://doi.org/10.5194/amt-2024-3967, 2025
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We retrieved high-resolution maps of Arctic surface temperature and type using airborne thermal infrared imagery from the HALO-(𝒜𝒞)3 campaign. Our study highlights small-scale surface variability, complementing satellite observations. Surface temperature was retrieved via radiative transfer simulations, while surface type was classified using machine learning. Additionally, we analyzed segment sizes of each surface type, presenting results based on their distance from the sea-ice edge.
Felix Pithan, Ann Kristin Naumann, and Marion Maturilli
Atmos. Chem. Phys., 25, 3269–3285, https://doi.org/10.5194/acp-25-3269-2025, https://doi.org/10.5194/acp-25-3269-2025, 2025
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Representing the exchange of air masses between the Arctic and mid-latitudes and the associated cloud formation is difficult for climate models. We compare climate model output to temperature and humidity measurements from weather balloons to provide suggestions for model improvements. Cold biases mostly occur in air that is exported from the Arctic. Models that compute the number of ice particles in a cloud better represent humidity than models that assume a fixed number of ice particles.
Cristofer Jimenez, Albert Ansmann, Kevin Ohneiser, Hannes Griesche, Ronny Engelmann, Martin Radenz, Julian Hofer, Dietrich Althausen, Daniel Alexander Knopf, Sandro Dahlke, Johannes Bühl, Holger Baars, Patric Seifert, and Ulla Wandinger
EGUsphere, https://doi.org/10.5194/egusphere-2025-967, https://doi.org/10.5194/egusphere-2025-967, 2025
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Using advanced remote sensing on the icebreaker Polarstern, we studied mixed-phase clouds (MPCs) in the central Arctic during the 2019–2020 MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) campaign. For the first time, lidar and radar techniques tracked the year-round evolution of liquid and ice phases in MPCs. The study provides cloud statistics and explores key processes driving cloud longevity, offering new insights into Arctic cloud formation and persistence.
Silke Groß, Volker Freudenthaler, Moritz Haarig, Albert Ansmann, Carlos Toledano, David Mateos, Petra Seibert, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Josef Gasteiger, Maximilian Dollner, Anne Tipka, Manuel Schöberl, Marilena Teri, and Bernadett Weinzierl
Atmos. Chem. Phys., 25, 3191–3211, https://doi.org/10.5194/acp-25-3191-2025, https://doi.org/10.5194/acp-25-3191-2025, 2025
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Aerosols contribute to the largest uncertainties in climate change predictions. The eastern Mediterranean is a hotspot for aerosols with natural and anthropogenic contributions. We present lidar measurements performed during A-LIFE (Absorbing aerosol layers in a changing climate: aging, lifetime and dynamics) to characterize aerosols and aerosol mixtures. We extend current lidar classification and separation schemes and compare them to classification schemes using different methods.
Harald Sodemann
EGUsphere, https://doi.org/10.5194/egusphere-2025-574, https://doi.org/10.5194/egusphere-2025-574, 2025
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The WaterSip software locates regions where precipitation comes from. WaterSip evaluates of the water budget of the air masses, providing information on the conditions during evaporation, transport, and arrival at the target area. WaterSip can be easily configured and writes gridded output files. Guidance is given on where uncertainties arise using a case study, and best practices are recommended. This manuscript supports the comparison of different methods to find precipitation sources.
Christian Heske, Florian Ewald, and Silke Groß
EGUsphere, https://doi.org/10.5194/egusphere-2025-691, https://doi.org/10.5194/egusphere-2025-691, 2025
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This study proposes a new technique to augment polarimetric radar measurements of the national German operational radar network with vertically looking cloud radars. The method is tested in two different case studies by comparison to dedicated scanning radars revealing promising results. Future usage of the method is motivated by analyzing the coverage of the operational radar network finding advantageous locations with good radar coverage.
Ziming Wang, Luca Bugliaro, Klaus Gierens, Michaela I. Hegglin, Susanne Rohs, Andreas Petzold, Stefan Kaufmann, and Christiane Voigt
Atmos. Chem. Phys., 25, 2845–2861, https://doi.org/10.5194/acp-25-2845-2025, https://doi.org/10.5194/acp-25-2845-2025, 2025
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Upper-tropospheric relative humidity bias in the ERA5 weather model is corrected by 10 % by an artificial neural network using aircraft in-service humidity data and thermodynamic and dynamical variables. The improved skills of the weather model will advance cirrus research, weather forecasts, and measures for contrail reduction.
Tereza Uhlíková, Timo Vihma, Alexey Yu Karpechko, and Petteri Uotila
The Cryosphere, 19, 1031–1046, https://doi.org/10.5194/tc-19-1031-2025, https://doi.org/10.5194/tc-19-1031-2025, 2025
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To better understand the local, regional, and global impacts of the recent rapid sea-ice decline in the Arctic, one of the key issues is to quantify the effects of sea-ice concentration on the surface radiative fluxes. We analyse these effects utilising four data sets called atmospheric reanalyses, and we evaluate uncertainties in these effects arising from inter-reanalysis differences in the sensitivity of the surface radiative fluxes to sea-ice concentration.
Hairu Ding, Bjorn Stevens, and Hauke Schmidt
EGUsphere, https://doi.org/10.5194/egusphere-2025-876, https://doi.org/10.5194/egusphere-2025-876, 2025
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This study examines the physical link between subtropical highs and stratocumulus variability. Using reanalysis data, we test two proposed pathways—one at the surface and one in the free troposphere—but find that neither is a dominant mechanism for stratocumulus variability on seasonal and interannual timescales. These results challenge the assumed influence of subtropical highs on stratocumulus and highlight the need for further research into lower tropospheric stability dynamics.
Anton Kötsche, Alexander Myagkov, Leonie von Terzi, Maximilian Maahn, Veronika Ettrichrätz, Teresa Vogl, Alexander Ryzhkov, Petar Bukovcic, Davide Ori, and Heike Kalesse-Los
EGUsphere, https://doi.org/10.5194/egusphere-2025-734, https://doi.org/10.5194/egusphere-2025-734, 2025
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Our study combines radar observations of snowf with snowfall camera observations on the ground to enhance our understanding of radar variables and snowfall properties. We found that values of an important radar variable (KDP) can be related to many different snow particle properties and number concentrations. We were able to constrain which particle sizes contribute to KDP by using computer models of snowflakes and showed which microphysical processes during snow formation can influence KDP.
Kira Zeider, Kayla McCauley, Sanja Dmitrovic, Leong Wai Siu, Yonghoon Choi, Ewan C. Crosbie, Joshua P. DiGangi, Glenn S. Diskin, Simon Kirschler, John B. Nowak, Michael A. Shook, Kenneth L. Thornhill, Christiane Voigt, Edward L. Winstead, Luke D. Ziemba, Paquita Zuidema, and Armin Sorooshian
Atmos. Chem. Phys., 25, 2407–2422, https://doi.org/10.5194/acp-25-2407-2025, https://doi.org/10.5194/acp-25-2407-2025, 2025
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In situ aircraft data collected over the northwest Atlantic Ocean are utilized to compare aerosol conditions and turbulence between near-surface and below-cloud-base altitudes for different regimes of coupling strength between those two levels, along with how cloud microphysical properties vary across those regimes. Stronger coupling yields more homogenous aerosol structure vertically along with higher cloud drop concentrations and sea salt influence in clouds.
Benjamin Heutte, Nora Bergner, Hélène Angot, Jakob B. Pernov, Lubna Dada, Jessica A. Mirrielees, Ivo Beck, Andrea Baccarini, Matthew Boyer, Jessie M. Creamean, Kaspar R. Daellenbach, Imad El Haddad, Markus M. Frey, Silvia Henning, Tiia Laurila, Vaios Moschos, Tuukka Petäjä, Kerri A. Pratt, Lauriane L. J. Quéléver, Matthew D. Shupe, Paul Zieger, Tuija Jokinen, and Julia Schmale
Atmos. Chem. Phys., 25, 2207–2241, https://doi.org/10.5194/acp-25-2207-2025, https://doi.org/10.5194/acp-25-2207-2025, 2025
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Limited aerosol measurements in the central Arctic hinder our understanding of aerosol–climate interactions in the region. Our year-long observations of aerosol physicochemical properties during the MOSAiC expedition reveal strong seasonal variations in aerosol chemical composition, where the short-term variability is heavily affected by storms in the Arctic. Local wind-generated particles are shown to be an important source of cloud seeds, especially in autumn.
Hans Segura, Xabier Pedruzo-Bagazgoitia, Philipp Weiss, Sebastian K. Müller, Thomas Rackow, Junhong Lee, Edgar Dolores-Tesillos, Imme Benedict, Matthias Aengenheyster, Razvan Aguridan, Gabriele Arduini, Alexander J. Baker, Jiawei Bao, Swantje Bastin, Eulàlia Baulenas, Tobias Becker, Sebastian Beyer, Hendryk Bockelmann, Nils Brüggemann, Lukas Brunner, Suvarchal K. Cheedela, Sushant Das, Jasper Denissen, Ian Dragaud, Piotr Dziekan, Madeleine Ekblom, Jan Frederik Engels, Monika Esch, Richard Forbes, Claudia Frauen, Lilli Freischem, Diego García-Maroto, Philipp Geier, Paul Gierz, Álvaro González-Cervera, Katherine Grayson, Matthew Griffith, Oliver Gutjahr, Helmuth Haak, Ioan Hadade, Kerstin Haslehner, Shabeh ul Hasson, Jan Hegewald, Lukas Kluft, Aleksei Koldunov, Nikolay Koldunov, Tobias Kölling, Shunya Koseki, Sergey Kosukhin, Josh Kousal, Peter Kuma, Arjun U. Kumar, Rumeng Li, Nicolas Maury, Maximilian Meindl, Sebastian Milinski, Kristian Mogensen, Bimochan Niraula, Jakub Nowak, Divya Sri Praturi, Ulrike Proske, Dian Putrasahan, René Redler, David Santuy, Domokos Sármány, Reiner Schnur, Patrick Scholz, Dmitry Sidorenko, Dorian Spät, Birgit Sützl, Daisuke Takasuka, Adrian Tompkins, Alejandro Uribe, Mirco Valentini, Menno Veerman, Aiko Voigt, Sarah Warnau, Fabian Wachsmann, Marta Wacławczyk, Nils Wedi, Karl-Hermann Wieners, Jonathan Wille, Marius Winkler, Yuting Wu, Florian Ziemen, Janos Zimmermann, Frida A.-M. Bender, Dragana Bojovic, Sandrine Bony, Simona Bordoni, Patrice Brehmer, Marcus Dengler, Emanuel Dutra, Saliou Faye, Erich Fischer, Chiel van Heerwaarden, Cathy Hohenegger, Heikki Järvinen, Markus Jochum, Thomas Jung, Johann H. Jungclaus, Noel S. Keenlyside, Daniel Klocke, Heike Konow, Martina Klose, Szymon Malinowski, Olivia Martius, Thorsten Mauritsen, Juan Pedro Mellado, Theresa Mieslinger, Elsa Mohino, Hanna Pawłowska, Karsten Peters-von Gehlen, Abdoulaye Sarré, Pajam Sobhani, Philip Stier, Lauri Tuppi, Pier Luigi Vidale, Irina Sandu, and Bjorn Stevens
EGUsphere, https://doi.org/10.5194/egusphere-2025-509, https://doi.org/10.5194/egusphere-2025-509, 2025
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The nextGEMS project developed two Earth system models that resolve processes of the order of 10 km, giving more fidelity to the representation of local phenomena, globally. In its fourth cycle, nextGEMS performed simulations with coupled ocean, land, and atmosphere over the 2020–2049 period under the SSP3-7.0 scenario. Here, we provide an overview of nextGEMS, insights into the model development, and the realism of multi-decadal, kilometer-scale simulations.
Inge Wiekenkamp, Anna Katharina Lehmann, Alexander Bütow, Jörg Hartmann, Stefan Metzger, Thomas Ruhtz, Christian Wille, Mathias Zöllner, and Torsten Sachs
Atmos. Meas. Tech., 18, 749–772, https://doi.org/10.5194/amt-18-749-2025, https://doi.org/10.5194/amt-18-749-2025, 2025
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Airborne eddy covariance platforms are crucial to measure three-dimensional wind and turbulent matter and energy transport between the surface and the atmosphere at larger scales. In this study, we introduce a new airborne eddy covariance platform (Schleicher ASK-16) and demonstrate that this platform is able to accurately measure turbulent fluxes and wind vectors. Data from this platform can help to build bridges between local tower measurements and remote-sensing-based products.
Theresa Mathes, Heather Guy, John Prytherch, Julia Kojoj, Ian Brooks, Sonja Murto, Paul Zieger, Birgit Wehner, Michael Tjernström, and Andreas Held
EGUsphere, https://doi.org/10.5194/egusphere-2025-183, https://doi.org/10.5194/egusphere-2025-183, 2025
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The Arctic is warming faster than the global average and aerosol-cloud-sea-ice interactions are crucial for studying its climate system. During the ARTofMELT Expedition 2023, particle and sensible heat fluxes were measured over multiple surfaces. Wide lead surfaces acted as particle sources with the strongest sensible heat fluxes, while closed ice surfaces acted as a particle sink. This study improves methods to measure these interactions, enhancing our understanding of Arctic climate processes.
Astrid B. Gjelsvik, Robert O. David, Tim Carlsen, Franziska Hellmuth, Stefan Hofer, Zachary McGraw, Harald Sodemann, and Trude Storelvmo
Atmos. Chem. Phys., 25, 1617–1637, https://doi.org/10.5194/acp-25-1617-2025, https://doi.org/10.5194/acp-25-1617-2025, 2025
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Ice formation in clouds has a substantial impact on radiation and precipitation and must be realistically simulated in order to understand present and future Arctic climate. Rare aerosols known as ice-nucleating particles can play an important role in cloud ice formation, but their representation in global climate models is not well suited for the Arctic. In this study, the simulation of cloud phase is improved when the representation of these particles is constrained by Arctic observations.
Claudia Christine Stephan and Bjorn Stevens
Atmos. Chem. Phys., 25, 1209–1226, https://doi.org/10.5194/acp-25-1209-2025, https://doi.org/10.5194/acp-25-1209-2025, 2025
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Tropical precipitation cluster area and intensity distributions follow power laws, but the physical processes responsible for this behavior remain unknown. We analyze global simulations that realistically represent precipitation processes. We consider Earth-like planets as well as virtual planets to realize different types of large-scale dynamics. Our finding is that power laws in Earth’s precipitation cluster statistics stem from the robust power laws in Earth’s atmospheric wind field.
Marcus Klingebiel, André Ehrlich, Micha Gryschka, Nils Risse, Nina Maherndl, Imke Schirmacher, Sophie Rosenburg, Sabine Hörnig, Manuel Moser, Evelyn Jäkel, Michael Schäfer, Hartwig Deneke, Mario Mech, Christiane Voigt, and Manfred Wendisch
EGUsphere, https://doi.org/10.5194/egusphere-2025-201, https://doi.org/10.5194/egusphere-2025-201, 2025
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Our study is using aircraft measurements from the HALO-(𝒜𝒞)³ campaign to investigate the transition from organized Arctic cloud street structures to more scattered cloud shapes. We show that lower wind speeds cause this transition. In addition we look at the changes of the cloud coverage, the height of the clouds, the cloud particles and the radiative properties.
Johanna Roschke, Jonas Witthuhn, Marcus Klingebiel, Moritz Haarig, Andreas Foth, Anton Kötsche, and Heike Kalesse-Los
Atmos. Meas. Tech., 18, 487–508, https://doi.org/10.5194/amt-18-487-2025, https://doi.org/10.5194/amt-18-487-2025, 2025
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We present a technique to discriminate between the Cloudnet target classification of "drizzle or rain" and sea salt aerosols that is applicable to marine Cloudnet sites. The method is crucial for investigating the occurrence of precipitation and significantly improves the Cloudnet target classification scheme for measurements over the Barbados Cloud Observatory (BCO). A first-ever analysis of the Cloudnet product including the new "haze echo" target over 2 years at the BCO is presented.
Johannes Schneider, Christiane Schulz, Florian Rubach, Anna Ludwig, Jonas Wilsch, Philipp Joppe, Christian Gurk, Sergej Molleker, Laurent Poulain, Florian Obersteiner, Torsten Gehrlein, Harald Bönisch, Andreas Zahn, Peter Hoor, Nicolas Emig, Heiko Bozem, Stephan Borrmann, and Markus Hermann
EGUsphere, https://doi.org/10.5194/egusphere-2024-3969, https://doi.org/10.5194/egusphere-2024-3969, 2025
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IAGOS-CARIBIC operates an instrumented container laboratory on commercial regular passenger flights to obtain a long-term representative data set on the composition of the upper troposphere and lowermost stratosphere. Here we report on the development on a fully automated aerosol mass spectrometer for this project. We present technical specifications, necessary modifications for the automation, instrument calibration and comparisons, detection limits, and first in-flight data.
Olivia G. Norman, Colette L. Heald, Solomon Bililign, Pedro Campuzano-Jost, Hugh Coe, Marc N. Fiddler, Jaime R. Green, Jose L. Jimenez, Katharina Kaiser, Jin Liao, Ann M. Middlebrook, Benjamin A. Nault, John B. Nowak, Johannes Schneider, and André Welti
Atmos. Chem. Phys., 25, 771–795, https://doi.org/10.5194/acp-25-771-2025, https://doi.org/10.5194/acp-25-771-2025, 2025
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This study finds that one component of secondary inorganic aerosols, nitrate, is greatly overestimated by a global atmospheric chemistry model compared to observations from 11 flight campaigns. None of the loss and production pathways explored can explain the nitrate bias alone. The model’s inability to capture the variability in the observations remains and requires future investigation to avoid biases in policy-related studies (i.e., air quality, health, climate impacts of these aerosols).
Shravan Deshmukh, Laurent Poulain, Birgit Wehner, Silvia Henning, Jean-Eudes Petit, Pauline Fombelle, Olivier Favez, Hartmut Herrmann, and Mira Pöhlker
Atmos. Chem. Phys., 25, 741–758, https://doi.org/10.5194/acp-25-741-2025, https://doi.org/10.5194/acp-25-741-2025, 2025
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Aerosol hygroscopicity has been investigated at a sub-urban site in Paris; analysis shows the sub-saturated regime's measured hygroscopicity and the chemically derived hygroscopic growth, shedding light on the large effect of external particle mixing and its influence on predicting hygroscopicity.
Lukas Pfitzenmaier, Pavlos Kollias, Nils Risse, Imke Schirmacher, Bernat Puigdomenech Treserras, and Katia Lamer
Geosci. Model Dev., 18, 101–115, https://doi.org/10.5194/gmd-18-101-2025, https://doi.org/10.5194/gmd-18-101-2025, 2025
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The Python tool Orbital-Radar transfers suborbital radar data (ground-based, airborne, and forward-simulated numerical weather prediction model) into synthetic spaceborne cloud profiling radar data, mimicking platform-specific instrument characteristics, e.g. EarthCARE or CloudSat. The tool's novelty lies in simulating characteristic errors and instrument noise. Thus, existing data sets are transferred into synthetic observations and can be used for satellite calibration–validation studies.
Michail Karalis, Gunilla Svensson, Manfred Wendisch, and Michael Tjernström
EGUsphere, https://doi.org/10.5194/egusphere-2024-3709, https://doi.org/10.5194/egusphere-2024-3709, 2025
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During the spring Arctic warm-air intrusion captured by HALO-(𝒜𝒞)3, the airmass demonstrated a column-like structure. We built a Lagrangian modeling framework using a single-column model (AOSCM) to simulate the airmass transformation. Comparing to observations, reanalysis and forecast data, we found that the AOSCM can successfully reproduce the main features of the transformation. The framework can be used for future model development to improve Arctic weather and climate prediction.
Larysa Istomina, Hannah Niehaus, and Gunnar Spreen
The Cryosphere, 19, 83–105, https://doi.org/10.5194/tc-19-83-2025, https://doi.org/10.5194/tc-19-83-2025, 2025
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Melt water puddles, or melt ponds on top of the Arctic sea ice, are a good measure of the Arctic climate state. In the context of recent climate warming, the Arctic has warmed about 4 times faster than the rest of the world, and a long-term dataset of the melt pond fraction is needed to be able to model the future development of the Arctic climate. We present such a dataset, produce 2002–2023 trends and highlight a potential melt regime shift with drastic regional trends of + 20 % per decade.
Huihui Wu, Fanny Peers, Jonathan W. Taylor, Chenjie Yu, Steven J. Abel, Paul A. Barrett, Jamie Trembath, Keith Bower, Jim M. Haywood, and Hugh Coe
EGUsphere, https://doi.org/10.5194/egusphere-2024-3975, https://doi.org/10.5194/egusphere-2024-3975, 2025
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This study investigates the transport history of African Biomass-Burning aerosols (BBAs) over the southeast Atlantic (SEA), and the relationship between transported BBAs and clouds around Ascension Island using in-situ airborne measurements. The work provides critical simplified parameterizations of aerosol-cloud interaction for improving the evaluation of radiative forcing over the SEA. It also identifies key entrainment regions for understanding the vertical transport process of African BBAs.
Daniele Zannoni, Hans Christian Steen-Larsen, Harald Sodemann, Iris Thurnherr, Cyrille Flamant, Patrick Chazette, Julien Totems, Martin Werner, and Myriam Raybaut
EGUsphere, https://doi.org/10.5194/egusphere-2024-3394, https://doi.org/10.5194/egusphere-2024-3394, 2025
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High resolution airborne observations reveal that mixing between the free troposphere and surface evapotranspiration flux primarly modulates the water vapor isotopic composition in the lower troposphere. Water vapor isotopes structure variations occur on the scale of 100s of m, underlying the utility of stable isotopes for studying microscale atmospheric dynamics. This study also provides the basis for better validation of water vapor isotopes remote sensing retrievals with surface observations.
Diana Francis, Ricardo Fonseca, Narendra Nelli, Petra Heil, Jonathan Wille, Irina Gorodetskaya, and Robert Massom
EGUsphere, https://doi.org/10.5194/egusphere-2024-3535, https://doi.org/10.5194/egusphere-2024-3535, 2025
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This study investigates the impact of atmospheric rivers and associated atmospheric dynamics on sea-ice thickness and snow depth at a coastal site in East Antarctica during July–November 2022 using in-situ measurements and numerical modelling. The passage of an atmospheric river induced a reduction of up to 0.06 m in both fields. Precipitation occurred from the convergence of katabatic winds with advected low-latitude moist air.
Tabea Rettelbach, Ingmar Nitze, Inge Grünberg, Jennika Hammar, Simon Schäffler, Daniel Hein, Matthias Gessner, Tilman Bucher, Jörg Brauchle, Jörg Hartmann, Torsten Sachs, Julia Boike, and Guido Grosse
Earth Syst. Sci. Data, 16, 5767–5798, https://doi.org/10.5194/essd-16-5767-2024, https://doi.org/10.5194/essd-16-5767-2024, 2024
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Permafrost landscapes in the Arctic are rapidly changing due to climate warming. Here, we publish aerial images and elevation models with very high spatial detail that help study these landscapes in northwestern Canada and Alaska. The images were collected using the Modular Aerial Camera System (MACS). This dataset has significant implications for understanding permafrost landscape dynamics in response to climate change. It is publicly available for further research.
Martanda Gautam, Alexander Theis, Jackson Seymore, Moritz Hey, Stephan Borrmann, Karoline Diehl, Subir K. Mitra, and Miklós Szakáll
EGUsphere, https://doi.org/10.5194/egusphere-2024-3917, https://doi.org/10.5194/egusphere-2024-3917, 2024
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We investigated the retention of chemical species and their binary mixtures during freezing of raindrops via acoustic levitation. Our results reveal high retention-nearly all substances being fully retained during freezing. This could be attributed to faster freezing time compared to slower mass expulsion time, along with ice-shell formation during freezing. This result helps improve our understanding of interaction between ice microphysical processes and chemistry in deep convective clouds.
Christine Borchers, Jackson Seymore, Martanda Gautam, Konstantin Dörholt, Yannik Müller, Andreas Arndt, Laura Gömmer, Florian Ungeheuer, Miklós Szakáll, Stephan Borrmann, Alexander Theis, Alexander L. Vogel, and Thorsten Hoffmann
Atmos. Chem. Phys., 24, 13961–13974, https://doi.org/10.5194/acp-24-13961-2024, https://doi.org/10.5194/acp-24-13961-2024, 2024
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Riming, a crucial process in cloud dynamics, influences the vertical distribution of compounds in the atmosphere. Experiments in Mainz's wind tunnel investigated retention coefficients of organic compounds under varying conditions. Findings suggest a correlation between the Henry's law constant and retention, applicable even to complex organic molecules.
Erin N. Raif, Sarah L. Barr, Mark D. Tarn, James B. McQuaid, Martin I. Daily, Steven J. Abel, Paul A. Barrett, Keith N. Bower, Paul R. Field, Kenneth S. Carslaw, and Benjamin J. Murray
Atmos. Chem. Phys., 24, 14045–14072, https://doi.org/10.5194/acp-24-14045-2024, https://doi.org/10.5194/acp-24-14045-2024, 2024
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Ice-nucleating particles (INPs) allow ice to form in clouds at temperatures warmer than −35°C. We measured INP concentrations over the Norwegian and Barents seas in weather events where cold air is ejected from the Arctic. These concentrations were among the highest measured in the Arctic. It is likely that the INPs were transported to the Arctic from distant regions. These results show it is important to consider hemispheric-scale INP processes to understand INP concentrations in the Arctic.
Karl Kortum, Suman Singha, and Gunnar Spreen
EGUsphere, https://doi.org/10.5194/egusphere-2024-3351, https://doi.org/10.5194/egusphere-2024-3351, 2024
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Improved sea ice observations are essential to understanding the processes that lead to the strong warming effect currently being observed in the Arctic. In this work, we combine complementary satellite measurement techniques and find remarkable correlations between the two observations. This allows us to expand the coverage of ice topography measurements to a scope and resolution that could not previously be observed.
Nina Maherndl, Manuel Moser, Imke Schirmacher, Aaron Bansemer, Johannes Lucke, Christiane Voigt, and Maximilian Maahn
Atmos. Chem. Phys., 24, 13935–13960, https://doi.org/10.5194/acp-24-13935-2024, https://doi.org/10.5194/acp-24-13935-2024, 2024
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It is not clear why ice crystals in clouds occur in clusters. Here, airborne measurements of clouds in mid-latitudes and high latitudes are used to study the spatial variability of ice. Further, we investigate the influence of riming, which occurs when liquid droplets freeze onto ice crystals. We find that riming enhances the occurrence of ice clusters. In the Arctic, riming leads to ice clustering at spatial scales of 3–5 km. This is due to updrafts and not higher amounts of liquid water.
Lukas Kluft, Bjorn Stevens, Manfred Brath, and Stefan A. Buehler
EGUsphere, https://doi.org/10.5194/egusphere-2024-3829, https://doi.org/10.5194/egusphere-2024-3829, 2024
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Using a single column model, we investigate the effect of the vertical distribution of clouds on climate sensitivity. We show that, depending on their height, clouds can mask or unmask the radiative response of the clear-sky atmosphere. Our single column model yields an all-sky climate sensitivity of 2.2 K, slightly less than the clear-sky value. This value can be interpreted as a baseline to which changes in surface albedo and an assumed reduction in cloud albedo would add.
Yifan Yang, Thomas Müller, Laurent Poulain, Samira Atabakhsh, Bruna A. Holanda, Jens Voigtländer, Shubhi Arora, and Mira L. Pöhlker
EGUsphere, https://doi.org/10.5194/egusphere-2024-3539, https://doi.org/10.5194/egusphere-2024-3539, 2024
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Black carbon (BC) is the major atmospheric aerosol that can absorb light and influence climate. We measured the physical properties of BC at a background site in Germany. In summer, BC particles were smaller and the mixture with other atmospheric components occurred during the daytime. In winter, emissions from residential heating significantly influenced BC's properties. Understanding these characteristics of BC can help improve aerosol optics simulation accuracy.
Lea Volkmer, Tobias Kölling, Tobias Zinner, and Bernhard Mayer
Atmos. Meas. Tech., 17, 6807–6817, https://doi.org/10.5194/amt-17-6807-2024, https://doi.org/10.5194/amt-17-6807-2024, 2024
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The importance of the consideration of cloud motion for the stereographic determination of cloud top height from aircraft observations is demonstrated using measurements of the airborne spectrometer of the Munich Aerosol Cloud Scanner (specMACS). A method for cloud motion correction using model winds from the European Centre for Medium-Range Weather Forecasts is presented and validated using both real measurements and realistic radiative transfer simulations.
Claudia Emde, Veronika Pörtge, Mihail Manev, and Bernhard Mayer
Atmos. Meas. Tech., 17, 6769–6789, https://doi.org/10.5194/amt-17-6769-2024, https://doi.org/10.5194/amt-17-6769-2024, 2024
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We introduce an innovative method to retrieve the cloud fraction and optical thickness of liquid water clouds over the ocean based on polarimetry. This is well suited for satellite observations providing multi-angle polarization measurements. Cloud fraction and cloud optical thickness can be derived from measurements at two viewing angles: one within the cloudbow and one in the sun glint region.
Phuc Thi Minh Ha, Yugo Kanaya, Kazuyo Yamaji, Syuichi Itahashi, Satoru Chatani, Takashi Sekiya, Maria Dolores Andrés Hernández, John Philip Burrows, Hans Schlager, Michael Lichtenstern, Mira Poehlker, and Bruna Holanda
EGUsphere, https://doi.org/10.5194/egusphere-2024-2064, https://doi.org/10.5194/egusphere-2024-2064, 2024
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Black carbon and CO are important to climate change. EMeRGe airborne observation can identify the suitability of emission inventories used in CMAQv5.0.2 model for Asian polluted regions. GFEDv4.1s is suitable for fire emissions. Anthropogenic BC and CO emissions from Philippines (REASv2.1) are insufficient. The estimated Chinese emissions in 2018 are 0.65±0.25 TgBC, 166±65 TgCO and 12.4±4.8 PgCO2, suggesting a reduction and increment for China's BC and CO emissions in the HTAPv2.2z inventory.
Zhenhai Zhang, F. Martin Ralph, Xun Zou, Brian Kawzenuk, Minghua Zheng, Irina V. Gorodetskaya, Penny M. Rowe, and David H. Bromwich
The Cryosphere, 18, 5239–5258, https://doi.org/10.5194/tc-18-5239-2024, https://doi.org/10.5194/tc-18-5239-2024, 2024
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Atmospheric rivers (ARs) are long, narrow corridors of strong water vapor transport in the atmosphere. ARs play an important role in extreme weather in polar regions, including heavy rain and/or snow, heat waves, and surface melt. The standard AR scale is developed based on the midlatitude climate and is insufficient for polar regions. This paper introduces an extended version of the AR scale tuned to polar regions, aiming to quantify polar ARs objectively based on their strength and impact.
Imke Schirmacher, Sabrina Schnitt, Marcus Klingebiel, Nina Maherndl, Benjamin Kirbus, André Ehrlich, Mario Mech, and Susanne Crewell
Atmos. Chem. Phys., 24, 12823–12842, https://doi.org/10.5194/acp-24-12823-2024, https://doi.org/10.5194/acp-24-12823-2024, 2024
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During Arctic marine cold-air outbreaks, cold air flows from sea ice over open water. Roll circulations evolve, forming cloud streets. We investigate the initial circulation and cloud development using high-resolution airborne measurements. We compute the distance an air mass traveled over water (fetch) from back trajectories. Cloud streets form at 15 km fetch, cloud cover strongly increases at around 20 km, and precipitation forms at around 30 km.
Christoph Kiemle, Andreas Fix, Christian Fruck, Gerhard Ehret, and Martin Wirth
Atmos. Meas. Tech., 17, 6569–6578, https://doi.org/10.5194/amt-17-6569-2024, https://doi.org/10.5194/amt-17-6569-2024, 2024
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Nitrous oxide is the third most important greenhouse gas modified by human activities after carbon dioxide and methane. This study examines the feasibility of airborne differential absorption lidar to quantify emissions from agriculture, fossil fuel combustion, industry, and biomass burning. Simulations show that a technically realizable and affordable mid-infrared lidar system will be able to measure the nitrous oxide column concentration enhancements with sufficient precision.
Julia Pikmann, Frank Drewnick, Friederike Fachinger, and Stephan Borrmann
Atmos. Chem. Phys., 24, 12295–12321, https://doi.org/10.5194/acp-24-12295-2024, https://doi.org/10.5194/acp-24-12295-2024, 2024
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Cooking activities can contribute substantially to indoor and ambient aerosol. We performed a comprehensive study with laboratory measurements cooking 19 different dishes and ambient measurements at two Christmas markets measuring various particle properties and trace gases of emissions in real time. Similar emission characteristics were observed for dishes with the same preparation method, mainly due to similar cooking temperature and use of oil, with barbecuing as an especially strong source.
Rémy Lapere, Louis Marelle, Pierre Rampal, Laurent Brodeau, Christian Melsheimer, Gunnar Spreen, and Jennie L. Thomas
Atmos. Chem. Phys., 24, 12107–12132, https://doi.org/10.5194/acp-24-12107-2024, https://doi.org/10.5194/acp-24-12107-2024, 2024
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Elongated open-water areas in sea ice, called leads, can release marine aerosols into the atmosphere. In the Arctic, this source of atmospheric particles could play an important role for climate. However, the amount, seasonality and spatial distribution of such emissions are all mostly unknown. Here, we propose a first parameterization for sea spray aerosols emitted through leads in sea ice and quantify their impact on aerosol populations in the high Arctic.
Sven Krautwurst, Christian Fruck, Sebastian Wolff, Jakob Borchardt, Oke Huhs, Konstantin Gerilowski, Michał Gałkowski, Christoph Kiemle, Mathieu Quatrevalet, Martin Wirth, Christian Mallaun, John P. Burrows, Christoph Gerbig, Andreas Fix, Hartmut Bösch, and Heinrich Bovensmann
EGUsphere, https://doi.org/10.5194/egusphere-2024-3182, https://doi.org/10.5194/egusphere-2024-3182, 2024
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Anomalously high CH4 emissions from landfills in Madrid, Spain, have been observed by satellite measurements in recent years. Our investigations of these waste facilities using passive and active airborne remote sensing measurements confirm these high emission rates with values of up to 13 th-1 during the overflight and show excellent agreement between the two techniques. A large fraction of the emissions is attributed to active landfill sites.
Andreas Walbröl, Hannes J. Griesche, Mario Mech, Susanne Crewell, and Kerstin Ebell
Atmos. Meas. Tech., 17, 6223–6245, https://doi.org/10.5194/amt-17-6223-2024, https://doi.org/10.5194/amt-17-6223-2024, 2024
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We developed retrievals of integrated water vapour (IWV), temperature profiles, and humidity profiles from ground-based passive microwave remote sensing measurements gathered during the MOSAiC expedition. We demonstrate and quantify the benefit of combining low- and high-frequency microwave radiometers to improve humidity profiling and IWV estimates by comparing the retrieved quantities to single-instrument retrievals and reference datasets (radiosondes).
Hannah Niehaus, Gunnar Spreen, Larysa Istomina, and Marcel Nicolaus
EGUsphere, https://doi.org/10.5194/egusphere-2024-3127, https://doi.org/10.5194/egusphere-2024-3127, 2024
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Melt ponds on Arctic sea ice affect how much solar energy is absorbed, influencing ice melt and climate change. This study used satellite data from 2017–2023 to examine how these ponds vary across regions and seasons. The results show that the surface fraction of melt ponds is more stable in the Central Arctic, with air temperature and ice surface roughness playing key roles in their formation. Understanding these patterns can help to improve climate models and predictions for Arctic warming.
Theresa Harlass, Rebecca Dischl, Stefan Kaufmann, Raphael Märkl, Daniel Sauer, Monika Scheibe, Paul Stock, Tiziana Bräuer, Andreas Dörnbrack, Anke Roiger, Hans Schlager, Ulrich Schumann, Magdalena Pühl, Tobias Schripp, Tobias Grein, Linda Bondorf, Charles Renard, Maxime Gauthier, Mark Johnson, Darren Luff, Paul Madden, Peter Swann, Denise Ahrens, Reetu Sallinen, and Christiane Voigt
Atmos. Chem. Phys., 24, 11807–11822, https://doi.org/10.5194/acp-24-11807-2024, https://doi.org/10.5194/acp-24-11807-2024, 2024
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Emissions from aircraft have a direct impact on our climate. Here, we present airborne and ground-based measurement data of nitrogen oxides that were collected in the exhaust of an Airbus aircraft. We study the impact of burning fossil and sustainable aviation fuel on nitrogen oxide emissions at different engine settings related to combustor temperature, pressure and fuel flow. Further, we compare observations with engine emission models.
Soodabeh Namdari, Sanja Dmitrovic, Gao Chen, Yonghoon Choi, Ewan Crosbie, Joshua P. DiGangi, Glenn S. Diskin, Richard A. Ferrare, Johnathan W. Hair, Simon Kirschler, John B. Nowak, Kenneth L. Thornhill, Christiane Voigt, Holger Vömel, Xubin Zeng, and Armin Sorooshian
EGUsphere, https://doi.org/10.5194/egusphere-2024-3024, https://doi.org/10.5194/egusphere-2024-3024, 2024
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We conducted this study to assess the accuracy of airborne measurements of wind, temperature, and humidity, essential for understanding atmospheric processes. Using data from NASA's ACTIVATE campaign, we compared measurements from the TAMMS and DLH aboard a Falcon aircraft with dropsondes from a King Air, matching data points based on location and time using statistical methods. The study showed strong agreement, confirming the reliability of these methods for advancing climate models.
Johanna Tjernström, Michael Gallagher, Jareth Holt, Gunilla Svensson, Matthew D. Shupe, Jonathan J. Day, Lara Ferrighi, Siri Jodha Khalsa, Leslie M. Hartten, Ewan O'Connor, Zen Mariani, and Øystein Godøy
EGUsphere, https://doi.org/10.5194/egusphere-2024-2088, https://doi.org/10.5194/egusphere-2024-2088, 2024
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The value of numerical weather predictions can be enhanced in several ways, one is to improve the representations of small-scale processes in models. To understand what needs to be improved, the model results need to be evaluated. Following standardized principles, a file format has been defined to be as similar as possible for both observational and model data. Python packages and toolkits are presented as a community resource in the production of the files and evaluation analysis.
Rebecca Dischl, Daniel Sauer, Christiane Voigt, Theresa Harlaß, Felicitas Sakellariou, Raphael Märkl, Ulrich Schumann, Monika Scheibe, Stefan Kaufmann, Anke Roiger, Andreas Dörnbrack, Charles Renard, Maxime Gauthier, Peter Swann, Paul Madden, Darren Luff, Mark Johnson, Denise Ahrens, Reetu Sallinen, Tobias Schripp, Georg Eckel, Uwe Bauder, and Patrick Le Clercq
Atmos. Chem. Phys., 24, 11255–11273, https://doi.org/10.5194/acp-24-11255-2024, https://doi.org/10.5194/acp-24-11255-2024, 2024
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In-flight measurements of aircraft emissions burning 100 % sustainable aviation fuel (SAF) show reduced particle number concentrations up to 41 % compared to conventional jet fuel. Particle emissions are dependent on engine power setting, flight altitude, and fuel composition. Engine models show a good correlation with measurement results. Future increased prevalence of SAF can positively influence the climate impact of aviation.
Andrew W. Seidl, Aina Johannessen, Alena Dekhtyareva, Jannis M. Huss, Marius O. Jonassen, Alexander Schulz, Ove Hermansen, Christoph K. Thomas, and Harald Sodemann
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-293, https://doi.org/10.5194/essd-2024-293, 2024
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ISLAS2020 set out to measure the stable water isotopic composition of Arctic moisture. By not only measuring at different sites around Ny-Ålesund, Svalbard, but also measuring at variable heights above surface level, we aim to characterize processes that produce or modify the isotopic composition. We also collect precipitation samples from sites that were typically downstream of Ny-Ålesund, so as to capture the isotopic composition during removal from the atmospheric water cycle.
Xiaoli Shen, David M. Bell, Hugh Coe, Naruki Hiranuma, Fabian Mahrt, Nicholas A. Marsden, Claudia Mohr, Daniel M. Murphy, Harald Saathoff, Johannes Schneider, Jacqueline Wilson, Maria A. Zawadowicz, Alla Zelenyuk, Paul J. DeMott, Ottmar Möhler, and Daniel J. Cziczo
Atmos. Chem. Phys., 24, 10869–10891, https://doi.org/10.5194/acp-24-10869-2024, https://doi.org/10.5194/acp-24-10869-2024, 2024
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Single-particle mass spectrometry (SPMS) is commonly used to measure the chemical composition and mixing state of aerosol particles. Intercomparison of SPMS instruments was conducted. All instruments reported similar size ranges and common spectral features. The instrument-specific detection efficiency was found to be more dependent on particle size than type. All differentiated secondary organic aerosol, soot, and soil dust but had difficulties differentiating among minerals and dusts.
Cassidy Soloff, Taiwo Ajayi, Yonghoon Choi, Ewan C. Crosbie, Joshua P. DiGangi, Glenn S. Diskin, Marta A. Fenn, Richard A. Ferrare, Francesca Gallo, Johnathan W. Hair, Miguel Ricardo A. Hilario, Simon Kirschler, Richard H. Moore, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Christiane Voigt, Edward L. Winstead, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 24, 10385–10408, https://doi.org/10.5194/acp-24-10385-2024, https://doi.org/10.5194/acp-24-10385-2024, 2024
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Using aircraft measurements over the northwestern Atlantic between the US East Coast and Bermuda and trajectory modeling of continental outflow, we identify trace gas and particle properties that exhibit gradients with offshore distance and quantify these changes with high-resolution measurements of concentrations and particle chemistry, size, and scattering properties. This work furthers our understanding of the complex interactions between continental and marine environments.
Theresa Kiszler, Davide Ori, and Vera Schemann
Atmos. Chem. Phys., 24, 10039–10053, https://doi.org/10.5194/acp-24-10039-2024, https://doi.org/10.5194/acp-24-10039-2024, 2024
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Microphysical processes impact the phase-partitioning of clouds. In this study we evaluate these processes while focusing on low-level Arctic clouds. To achieve this we used an extensive simulation set in combination with a new diagnostic tool. This study presents our findings on the relevance of these processes and their behaviour under different thermodynamic regimes.
Shuaiqi Tang, Hailong Wang, Xiang-Yu Li, Jingyi Chen, Armin Sorooshian, Xubin Zeng, Ewan Crosbie, Kenneth L. Thornhill, Luke D. Ziemba, and Christiane Voigt
Atmos. Chem. Phys., 24, 10073–10092, https://doi.org/10.5194/acp-24-10073-2024, https://doi.org/10.5194/acp-24-10073-2024, 2024
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We examined marine boundary layer clouds and their interactions with aerosols in the E3SM single-column model (SCM) for a case study. The SCM shows good agreement when simulating the clouds with high-resolution models. It reproduces the relationship between cloud droplet and aerosol particle number concentrations as produced in global models. However, the relationship between cloud liquid water and droplet number concentration is different, warranting further investigation.
Nils Risse, Mario Mech, Catherine Prigent, Gunnar Spreen, and Susanne Crewell
The Cryosphere, 18, 4137–4163, https://doi.org/10.5194/tc-18-4137-2024, https://doi.org/10.5194/tc-18-4137-2024, 2024
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Passive microwave observations from satellites are crucial for monitoring Arctic sea ice and atmosphere. To do this effectively, it is important to understand how sea ice emits microwaves. Through unique Arctic sea ice observations, we improved our understanding, identified four distinct emission types, and expanded current knowledge to include higher frequencies. These findings will enhance our ability to monitor the Arctic climate and provide valuable information for new satellite missions.
Filippo Emilio Scarsi, Alessandro Battaglia, Maximilian Maahn, and Stef Lhermitte
EGUsphere, https://doi.org/10.5194/egusphere-2024-1917, https://doi.org/10.5194/egusphere-2024-1917, 2024
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Snowfall measurements at high latitudes are crucial for estimating ice sheet mass balance. Spaceborne radar and radiometer missions help estimate snowfall but face uncertainties. This work evaluates uncertainties in snowfall estimates from a fixed near-nadir radar (CloudSat-like) and a conically scanning radar (WIVERN-like), determining that WIVERN will provide much better estimates than CloudSat, and at much smaller spatial and temporal scales.
Lara Foth, Wolfgang Dorn, Annette Rinke, Evelyn Jäkel, and Hannah Niehaus
The Cryosphere, 18, 4053–4064, https://doi.org/10.5194/tc-18-4053-2024, https://doi.org/10.5194/tc-18-4053-2024, 2024
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It is demonstrated that the explicit consideration of the cloud dependence of the snow surface albedo in a climate model results in a more realistic simulation of the surface albedo during the snowmelt period in late May and June. Although this improvement appears to be relatively insubstantial, it has significant impact on the simulated sea-ice volume and extent in the model due to an amplification of the snow/sea-ice albedo feedback, one of the main contributors to Arctic amplification.
Johanna Mayer, Bernhard Mayer, Luca Bugliaro, Ralf Meerkötter, and Christiane Voigt
Atmos. Meas. Tech., 17, 5161–5185, https://doi.org/10.5194/amt-17-5161-2024, https://doi.org/10.5194/amt-17-5161-2024, 2024
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This study uses radiative transfer calculations to characterize the relation of two satellite channel combinations (namely infrared window brightness temperature differences – BTDs – of SEVIRI) to the thermodynamic cloud phase. A sensitivity analysis reveals the complex interplay of cloud parameters and their contribution to the observed phase dependence of BTDs. This knowledge helps to design optimal cloud-phase retrievals and to understand their potential and limitations.
Taiwo Ajayi, Yonghoon Choi, Ewan C. Crosbie, Joshua P. DiGangi, Glenn S. Diskin, Marta A. Fenn, Richard A. Ferrare, Johnathan W. Hair, Miguel Ricardo A. Hilario, Chris A. Hostetler, Simon Kirschler, Richard H. Moore, Taylor J. Shingler, Michael A. Shook, Cassidy Soloff, Kenneth L. Thornhill, Christiane Voigt, Edward L. Winstead, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 24, 9197–9218, https://doi.org/10.5194/acp-24-9197-2024, https://doi.org/10.5194/acp-24-9197-2024, 2024
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This study uses airborne data to examine vertical profiles of trace gases, aerosol particles, and meteorological variables over a remote marine area (Bermuda). Results show distinct differences based on both air mass source region (North America, Ocean, Caribbean/North Africa) and altitude for a given air mass type. This work highlights the sensitivity of remote marine areas to long-range transport and the importance of considering the vertical dependence of trace gas and aerosol properties.
Luiz A. T. Machado, Jürgen Kesselmeier, Santiago Botía, Hella van Asperen, Meinrat O. Andreae, Alessandro C. de Araújo, Paulo Artaxo, Achim Edtbauer, Rosaria R. Ferreira, Marco A. Franco, Hartwig Harder, Sam P. Jones, Cléo Q. Dias-Júnior, Guido G. Haytzmann, Carlos A. Quesada, Shujiro Komiya, Jost Lavric, Jos Lelieveld, Ingeborg Levin, Anke Nölscher, Eva Pfannerstill, Mira L. Pöhlker, Ulrich Pöschl, Akima Ringsdorf, Luciana Rizzo, Ana M. Yáñez-Serrano, Susan Trumbore, Wanda I. D. Valenti, Jordi Vila-Guerau de Arellano, David Walter, Jonathan Williams, Stefan Wolff, and Christopher Pöhlker
Atmos. Chem. Phys., 24, 8893–8910, https://doi.org/10.5194/acp-24-8893-2024, https://doi.org/10.5194/acp-24-8893-2024, 2024
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Composite analysis of gas concentration before and after rainfall, during the day and night, gives insight into the complex relationship between trace gas variability and precipitation. The analysis helps us to understand the sources and sinks of trace gases within a forest ecosystem. It elucidates processes that are not discernible under undisturbed conditions and contributes to a deeper understanding of the trace gas life cycle and its intricate interactions with cloud dynamics in the Amazon.
Baseerat Romshoo, Jaikrishna Patil, Tobias Michels, Thomas Müller, Marius Kloft, and Mira Pöhlker
Atmos. Chem. Phys., 24, 8821–8846, https://doi.org/10.5194/acp-24-8821-2024, https://doi.org/10.5194/acp-24-8821-2024, 2024
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Through the use of our machine-learning-based optical model, realistic BC morphologies can be incorporated into atmospheric science applications that require highly accurate results with minimal computational resources. The results of the study demonstrate that the predictions of single-scattering albedo (ω) and mass absorption cross-section (MAC) were improved over the conventional Mie-based predictions when using the machine learning method.
Di Chen, Qizhen Sun, and Timo Vihma
EGUsphere, https://doi.org/10.5194/egusphere-2024-2359, https://doi.org/10.5194/egusphere-2024-2359, 2024
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We investigates the variations and trends in Arctic sea ice during summer and autumn, focusing on the impacts of sea surface temperature (SST) and surface air temperature (SAT). Both SST and SAT significantly influence Arctic sea ice concentration. SST affects both interannual variations and decadal trends, while SAT primarily influences interannual variations. Additionally, SAT's impact on sea ice concentration leads by seven months, due to a stronger warming trend in winter than in summer.
Henning Dorff, Heike Konow, Vera Schemann, and Felix Ament
Atmos. Chem. Phys., 24, 8771–8795, https://doi.org/10.5194/acp-24-8771-2024, https://doi.org/10.5194/acp-24-8771-2024, 2024
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Using synthetic dropsondes, we assess how discrete spatial sampling and temporal evolution during flight affect the accuracy of real sonde-based moisture transport divergence in Arctic atmospheric rivers (ARs). Non-instantaneous sampling during temporal AR evolution deteriorates the divergence values more than spatial undersampling. Moisture advection is the dominating factor but most sensitive to the sampling method. We suggest a minimum of seven sondes to resolve the AR divergence components.
Jonathan J. Day, Gunilla Svensson, Barbara Casati, Taneil Uttal, Siri-Jodha Khalsa, Eric Bazile, Elena Akish, Niramson Azouz, Lara Ferrighi, Helmut Frank, Michael Gallagher, Øystein Godøy, Leslie M. Hartten, Laura X. Huang, Jareth Holt, Massimo Di Stefano, Irene Suomi, Zen Mariani, Sara Morris, Ewan O'Connor, Roberta Pirazzini, Teresa Remes, Rostislav Fadeev, Amy Solomon, Johanna Tjernström, and Mikhail Tolstykh
Geosci. Model Dev., 17, 5511–5543, https://doi.org/10.5194/gmd-17-5511-2024, https://doi.org/10.5194/gmd-17-5511-2024, 2024
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The YOPP site Model Intercomparison Project (YOPPsiteMIP), which was designed to facilitate enhanced weather forecast evaluation in polar regions, is discussed here, focussing on describing the archive of forecast data and presenting a multi-model evaluation at Arctic supersites during February and March 2018. The study highlights an underestimation in boundary layer temperature variance that is common across models and a related inability to forecast cold extremes at several of the sites.
Johannes Röttenbacher, André Ehrlich, Hanno Müller, Florian Ewald, Anna E. Luebke, Benjamin Kirbus, Robin J. Hogan, and Manfred Wendisch
Atmos. Chem. Phys., 24, 8085–8104, https://doi.org/10.5194/acp-24-8085-2024, https://doi.org/10.5194/acp-24-8085-2024, 2024
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Weather prediction models simplify the physical processes related to light scattering by clouds consisting of complex ice crystals. Whether these simplifications are the cause for uncertainties in their prediction can be evaluated by comparing them with measurement data. Here we do this for Arctic ice clouds over sea ice using airborne measurements from two case studies. The model performs well for thick ice clouds but not so well for thin ones. This work can be used to improve the model.
Andreas Walbröl, Janosch Michaelis, Sebastian Becker, Henning Dorff, Kerstin Ebell, Irina Gorodetskaya, Bernd Heinold, Benjamin Kirbus, Melanie Lauer, Nina Maherndl, Marion Maturilli, Johanna Mayer, Hanno Müller, Roel A. J. Neggers, Fiona M. Paulus, Johannes Röttenbacher, Janna E. Rückert, Imke Schirmacher, Nils Slättberg, André Ehrlich, Manfred Wendisch, and Susanne Crewell
Atmos. Chem. Phys., 24, 8007–8029, https://doi.org/10.5194/acp-24-8007-2024, https://doi.org/10.5194/acp-24-8007-2024, 2024
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To support the interpretation of the data collected during the HALO-(AC)3 campaign, which took place in the North Atlantic sector of the Arctic from 7 March to 12 April 2022, we analyze how unusual the weather and sea ice conditions were with respect to the long-term climatology. From observations and ERA5 reanalysis, we found record-breaking warm air intrusions and a large variety of marine cold air outbreaks. Sea ice concentration was mostly within the climatological interquartile range.
Niklas Karbach, Lisa Höhler, Peter Hoor, Heiko Bozem, Nicole Bobrowski, and Thorsten Hoffmann
Atmos. Meas. Tech., 17, 4081–4086, https://doi.org/10.5194/amt-17-4081-2024, https://doi.org/10.5194/amt-17-4081-2024, 2024
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The system presented here can accurately generate and reproduce a stable flow of gas mixtures of known concentrations over several days using ambient air as a dilution medium. In combination with the small size and low weight of the system, this enables the calibration of hydrogen sensors in the field, reducing the influence of matrix effects on the accuracy of the sensor. The system is inexpensive to assemble and easy to maintain, which is the key to reliable measurement results.
Johanna Mayer, Luca Bugliaro, Bernhard Mayer, Dennis Piontek, and Christiane Voigt
Atmos. Meas. Tech., 17, 4015–4039, https://doi.org/10.5194/amt-17-4015-2024, https://doi.org/10.5194/amt-17-4015-2024, 2024
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ProPS (PRObabilistic cloud top Phase retrieval for SEVIRI) is a method to detect clouds and their thermodynamic phase with a geostationary satellite, distinguishing between clear sky and ice, mixed-phase, supercooled and warm liquid clouds. It uses a Bayesian approach based on the lidar–radar product DARDAR. The method allows studying cloud phases, especially mixed-phase and supercooled clouds, rarely observed from geostationary satellites. This can be used for comparison with climate models.
Taneil Uttal, Leslie M. Hartten, Siri Jodha Khalsa, Barbara Casati, Gunilla Svensson, Jonathan Day, Jareth Holt, Elena Akish, Sara Morris, Ewan O'Connor, Roberta Pirazzini, Laura X. Huang, Robert Crawford, Zen Mariani, Øystein Godøy, Johanna A. K. Tjernström, Giri Prakash, Nicki Hickmon, Marion Maturilli, and Christopher J. Cox
Geosci. Model Dev., 17, 5225–5247, https://doi.org/10.5194/gmd-17-5225-2024, https://doi.org/10.5194/gmd-17-5225-2024, 2024
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A Merged Observatory Data File (MODF) format to systematically collate complex atmosphere, ocean, and terrestrial data sets collected by multiple instruments during field campaigns is presented. The MODF format is also designed to be applied to model output data, yielding format-matching Merged Model Data Files (MMDFs). MODFs plus MMDFs will augment and accelerate the synergistic use of model results with observational data to increase understanding and predictive skill.
Philipp Joppe, Johannes Schneider, Katharina Kaiser, Horst Fischer, Peter Hoor, Daniel Kunkel, Hans-Christoph Lachnitt, Andreas Marsing, Lenard Röder, Hans Schlager, Laura Tomsche, Christiane Voigt, Andreas Zahn, and Stephan Borrmann
Atmos. Chem. Phys., 24, 7499–7522, https://doi.org/10.5194/acp-24-7499-2024, https://doi.org/10.5194/acp-24-7499-2024, 2024
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From aircraft measurements in the upper troposphere/lower stratosphere, we find a correlation between the ozone and particulate sulfate in the lower stratosphere. The correlation exhibits some variability over the measurement period exceeding the background sulfate-to-ozone correlation. From our analysis, we conclude that gas-to-particle conversion of volcanic sulfur dioxide leads to observed enhanced sulfate aerosol mixing ratios.
Zen Mariani, Sara M. Morris, Taneil Uttal, Elena Akish, Robert Crawford, Laura Huang, Jonathan Day, Johanna Tjernström, Øystein Godøy, Lara Ferrighi, Leslie M. Hartten, Jareth Holt, Christopher J. Cox, Ewan O'Connor, Roberta Pirazzini, Marion Maturilli, Giri Prakash, James Mather, Kimberly Strong, Pierre Fogal, Vasily Kustov, Gunilla Svensson, Michael Gallagher, and Brian Vasel
Earth Syst. Sci. Data, 16, 3083–3124, https://doi.org/10.5194/essd-16-3083-2024, https://doi.org/10.5194/essd-16-3083-2024, 2024
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During the Year of Polar Prediction (YOPP), we increased measurements in the polar regions and have made dedicated efforts to centralize and standardize all of the different types of datasets that have been collected to facilitate user uptake and model–observation comparisons. This paper is an overview of those efforts and a description of the novel standardized Merged Observation Data Files (MODFs), including a description of the sites, data format, and instruments.
Clémantyne Aubry, Julien Delanoë, Silke Groß, Florian Ewald, Frédéric Tridon, Olivier Jourdan, and Guillaume Mioche
Atmos. Meas. Tech., 17, 3863–3881, https://doi.org/10.5194/amt-17-3863-2024, https://doi.org/10.5194/amt-17-3863-2024, 2024
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Radar–lidar synergy is used to retrieve ice, supercooled water and mixed-phase cloud properties, making the most of the radar sensitivity to ice crystals and the lidar sensitivity to supercooled droplets. A first analysis of the output of the algorithm run on the satellite data is compared with in situ data during an airborne Arctic field campaign, giving a mean percent error of 49 % for liquid water content and 75 % for ice water content.
Karina McCusker, Anthony J. Baran, Chris Westbrook, Stuart Fox, Patrick Eriksson, Richard Cotton, Julien Delanoë, and Florian Ewald
Atmos. Meas. Tech., 17, 3533–3552, https://doi.org/10.5194/amt-17-3533-2024, https://doi.org/10.5194/amt-17-3533-2024, 2024
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Polarised radiative transfer simulations are performed using an atmospheric model based on in situ measurements. These are compared to large polarisation measurements to explore whether such measurements can provide information on cloud ice, e.g. particle shape and orientation. We find that using oriented particle models with shapes based on imagery generally allows for accurate simulations. However, results are sensitive to shape assumptions such as the choice of single crystals or aggregates.
Ewan Crosbie, Luke D. Ziemba, Michael A. Shook, Taylor Shingler, Johnathan W. Hair, Armin Sorooshian, Richard A. Ferrare, Brian Cairns, Yonghoon Choi, Joshua DiGangi, Glenn S. Diskin, Chris Hostetler, Simon Kirschler, Richard H. Moore, David Painemal, Claire Robinson, Shane T. Seaman, K. Lee Thornhill, Christiane Voigt, and Edward Winstead
Atmos. Chem. Phys., 24, 6123–6152, https://doi.org/10.5194/acp-24-6123-2024, https://doi.org/10.5194/acp-24-6123-2024, 2024
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Marine clouds are found to clump together in regions or lines, readily discernible from satellite images of the ocean. While clustering is also a feature of deep storm clouds, we focus on smaller cloud systems associated with fair weather and brief localized showers. Two aircraft sampled the region around these shallow systems: one incorporated measurements taken within, adjacent to, and below the clouds, while the other provided a survey from above using remote sensing techniques.
Roger Teoh, Zebediah Engberg, Ulrich Schumann, Christiane Voigt, Marc Shapiro, Susanne Rohs, and Marc E. J. Stettler
Atmos. Chem. Phys., 24, 6071–6093, https://doi.org/10.5194/acp-24-6071-2024, https://doi.org/10.5194/acp-24-6071-2024, 2024
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The radiative forcing (RF) due to aviation contrails is comparable to that caused by CO2. We estimate that global contrail net RF in 2019 was 62.1 mW m−2. This is ~1/2 the previous best estimate for 2018. Contrail RF varies regionally due to differences in conditions required for persistent contrails. COVID-19 reduced contrail RF by 54% in 2020 relative to 2019. Globally, 2 % of all flights account for 80 % of the annual contrail energy forcing, suggesting a opportunity to mitigate contrail RF.
Georgios Dekoutsidis, Martin Wirth, and Silke Groß
Atmos. Chem. Phys., 24, 5971–5987, https://doi.org/10.5194/acp-24-5971-2024, https://doi.org/10.5194/acp-24-5971-2024, 2024
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For decades the earth's temperature has been rising. The Arctic regions are warming faster. Cirrus clouds can contribute to this phenomenon. During warm-air intrusions, air masses are transported into the Arctic from the mid-latitudes. The HALO-(AC)3 campaign took place to measure cirrus during intrusion events and under normal conditions. We study the two cloud types based on these measurements and find differences in their geometry, relative humidity distribution and vertical structure.
Junghwa Lee, Patric Seifert, Tempei Hashino, Maximilian Maahn, Fabian Senf, and Oswald Knoth
Atmos. Chem. Phys., 24, 5737–5756, https://doi.org/10.5194/acp-24-5737-2024, https://doi.org/10.5194/acp-24-5737-2024, 2024
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Spectral bin model simulations of an idealized supercooled stratiform cloud were performed with the AMPS model for variable CCN and INP concentrations. We performed radar forward simulations with PAMTRA to transfer the simulations into radar observational space. The derived radar reflectivity factors were compared to observational studies of stratiform mixed-phase clouds. These studies report a similar response of the radar reflectivity factor to aerosol perturbations as we found in our study.
Valery Shcherbakov, Frédéric Szczap, Guillaume Mioche, and Céline Cornet
Atmos. Meas. Tech., 17, 3011–3028, https://doi.org/10.5194/amt-17-3011-2024, https://doi.org/10.5194/amt-17-3011-2024, 2024
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We performed Monte Carlo simulations of single-wavelength lidar signals from multi-layered clouds with special attention focused on the multiple-scattering (MS) effect in regions of the cloud-free molecular atmosphere. The MS effect on lidar signals always decreases with the increasing distance from the cloud far edge. The decrease is the direct consequence of the fact that the forward peak of particle phase functions is much larger than the receiver field of view.
Finn Burgemeister, Marco Clemens, and Felix Ament
Earth Syst. Sci. Data, 16, 2317–2332, https://doi.org/10.5194/essd-16-2317-2024, https://doi.org/10.5194/essd-16-2317-2024, 2024
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Knowledge of small-scale rainfall variability is needed for hydro-meteorological applications in urban areas. Therefore, we present an open-access data set covering reanalyzed radar reflectivities and rainfall estimates measured by a weather radar at high spatio-temporal resolution in the urban environment of Hamburg between 2013 and 2021. We describe the data reanalysis, outline the measurement’s performance for long time periods, and discuss open issues and limitations of the data set.
Johanna S. Seidel, Alexei A. Kiselev, Alice Keinert, Frank Stratmann, Thomas Leisner, and Susan Hartmann
Atmos. Chem. Phys., 24, 5247–5263, https://doi.org/10.5194/acp-24-5247-2024, https://doi.org/10.5194/acp-24-5247-2024, 2024
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Clouds often contain several thousand times more ice crystals than aerosol particles catalyzing ice formation. This phenomenon, commonly known as ice multiplication, is often explained by secondary ice formation due to the collisions between falling ice particles and droplets. In this study, we mimic this riming process. Contrary to earlier experiments, we found no efficient ice multiplication, which fundamentally questions the importance of the rime-splintering mechanism.
Karl Kortum, Suman Singha, Gunnar Spreen, Nils Hutter, Arttu Jutila, and Christian Haas
The Cryosphere, 18, 2207–2222, https://doi.org/10.5194/tc-18-2207-2024, https://doi.org/10.5194/tc-18-2207-2024, 2024
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A dataset of 20 radar satellite acquisitions and near-simultaneous helicopter-based surveys of the ice topography during the MOSAiC expedition is constructed and used to train a variety of deep learning algorithms. The results give realistic insights into the accuracy of retrieval of measured ice classes using modern deep learning models. The models able to learn from the spatial distribution of the measured sea ice classes are shown to have a clear advantage over those that cannot.
Declan L. Finney, Alan M. Blyth, Martin Gallagher, Huihui Wu, Graeme J. Nott, Michael I. Biggerstaff, Richard G. Sonnenfeld, Martin Daily, Dan Walker, David Dufton, Keith Bower, Steven Böing, Thomas Choularton, Jonathan Crosier, James Groves, Paul R. Field, Hugh Coe, Benjamin J. Murray, Gary Lloyd, Nicholas A. Marsden, Michael Flynn, Kezhen Hu, Navaneeth M. Thamban, Paul I. Williams, Paul J. Connolly, James B. McQuaid, Joseph Robinson, Zhiqiang Cui, Ralph R. Burton, Gordon Carrie, Robert Moore, Steven J. Abel, Dave Tiddeman, and Graydon Aulich
Earth Syst. Sci. Data, 16, 2141–2163, https://doi.org/10.5194/essd-16-2141-2024, https://doi.org/10.5194/essd-16-2141-2024, 2024
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The DCMEX (Deep Convective Microphysics Experiment) project undertook an aircraft- and ground-based measurement campaign of New Mexico deep convective clouds during July–August 2022. The campaign coordinated a broad range of instrumentation measuring aerosol, cloud physics, radar signals, thermodynamics, dynamics, electric fields, and weather. The project's objectives included the utilisation of these data with satellite observations to study the anvil cloud radiative effect.
Bjorn Stevens, Stefan Adami, Tariq Ali, Hartwig Anzt, Zafer Aslan, Sabine Attinger, Jaana Bäck, Johanna Baehr, Peter Bauer, Natacha Bernier, Bob Bishop, Hendryk Bockelmann, Sandrine Bony, Guy Brasseur, David N. Bresch, Sean Breyer, Gilbert Brunet, Pier Luigi Buttigieg, Junji Cao, Christelle Castet, Yafang Cheng, Ayantika Dey Choudhury, Deborah Coen, Susanne Crewell, Atish Dabholkar, Qing Dai, Francisco Doblas-Reyes, Dale Durran, Ayoub El Gaidi, Charlie Ewen, Eleftheria Exarchou, Veronika Eyring, Florencia Falkinhoff, David Farrell, Piers M. Forster, Ariane Frassoni, Claudia Frauen, Oliver Fuhrer, Shahzad Gani, Edwin Gerber, Debra Goldfarb, Jens Grieger, Nicolas Gruber, Wilco Hazeleger, Rolf Herken, Chris Hewitt, Torsten Hoefler, Huang-Hsiung Hsu, Daniela Jacob, Alexandra Jahn, Christian Jakob, Thomas Jung, Christopher Kadow, In-Sik Kang, Sarah Kang, Karthik Kashinath, Katharina Kleinen-von Königslöw, Daniel Klocke, Uta Kloenne, Milan Klöwer, Chihiro Kodama, Stefan Kollet, Tobias Kölling, Jenni Kontkanen, Steve Kopp, Michal Koran, Markku Kulmala, Hanna Lappalainen, Fakhria Latifi, Bryan Lawrence, June Yi Lee, Quentin Lejeun, Christian Lessig, Chao Li, Thomas Lippert, Jürg Luterbacher, Pekka Manninen, Jochem Marotzke, Satoshi Matsouoka, Charlotte Merchant, Peter Messmer, Gero Michel, Kristel Michielsen, Tomoki Miyakawa, Jens Müller, Ramsha Munir, Sandeep Narayanasetti, Ousmane Ndiaye, Carlos Nobre, Achim Oberg, Riko Oki, Tuba Özkan-Haller, Tim Palmer, Stan Posey, Andreas Prein, Odessa Primus, Mike Pritchard, Julie Pullen, Dian Putrasahan, Johannes Quaas, Krishnan Raghavan, Venkatachalam Ramaswamy, Markus Rapp, Florian Rauser, Markus Reichstein, Aromar Revi, Sonakshi Saluja, Masaki Satoh, Vera Schemann, Sebastian Schemm, Christina Schnadt Poberaj, Thomas Schulthess, Cath Senior, Jagadish Shukla, Manmeet Singh, Julia Slingo, Adam Sobel, Silvina Solman, Jenna Spitzer, Philip Stier, Thomas Stocker, Sarah Strock, Hang Su, Petteri Taalas, John Taylor, Susann Tegtmeier, Georg Teutsch, Adrian Tompkins, Uwe Ulbrich, Pier-Luigi Vidale, Chien-Ming Wu, Hao Xu, Najibullah Zaki, Laure Zanna, Tianjun Zhou, and Florian Ziemen
Earth Syst. Sci. Data, 16, 2113–2122, https://doi.org/10.5194/essd-16-2113-2024, https://doi.org/10.5194/essd-16-2113-2024, 2024
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To manage Earth in the Anthropocene, new tools, new institutions, and new forms of international cooperation will be required. Earth Virtualization Engines is proposed as an international federation of centers of excellence to empower all people to respond to the immense and urgent challenges posed by climate change.
Richard Maier, Fabian Jakub, Claudia Emde, Mihail Manev, Aiko Voigt, and Bernhard Mayer
Geosci. Model Dev., 17, 3357–3383, https://doi.org/10.5194/gmd-17-3357-2024, https://doi.org/10.5194/gmd-17-3357-2024, 2024
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Based on the TenStream solver, we present a new method to accelerate 3D radiative transfer towards the speed of currently used 1D solvers. Using a shallow-cumulus-cloud time series, we evaluate the performance of this new solver in terms of both speed and accuracy. Compared to a 3D benchmark simulation, we show that our new solver is able to determine much more accurate irradiances and heating rates than a 1D δ-Eddington solver, even when operated with a similar computational demand.
Ilias Fountoulakis, Alexandra Tsekeri, Stelios Kazadzis, Vassilis Amiridis, Angelos Nersesian, Maria Tsichla, Emmanouil Proestakis, Antonis Gkikas, Kyriakoula Papachristopoulou, Vasileios Barlakas, Claudia Emde, and Bernhard Mayer
Atmos. Chem. Phys., 24, 4915–4948, https://doi.org/10.5194/acp-24-4915-2024, https://doi.org/10.5194/acp-24-4915-2024, 2024
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In our study we provide an assessment, through a sensitivity study, of the limitations of models to calculate the dust direct radiative effect (DRE) due to the underrepresentation of its size, refractive index (RI), and shape. Our results indicate the necessity of including more realistic sizes and RIs for dust particles in dust models, in order to derive better estimations of the dust direct radiative effects.
Behrooz Keshtgar, Aiko Voigt, Bernhard Mayer, and Corinna Hoose
Atmos. Chem. Phys., 24, 4751–4769, https://doi.org/10.5194/acp-24-4751-2024, https://doi.org/10.5194/acp-24-4751-2024, 2024
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Cloud-radiative heating (CRH) affects extratropical cyclones but is uncertain in weather and climate models. We provide a framework to quantify uncertainties in CRH within an extratropical cyclone due to four factors and show that the parameterization of ice optical properties contributes significantly to uncertainty in CRH. We also argue that ice optical properties, by affecting CRH on spatial scales of 100 km, are relevant for the large-scale dynamics of extratropical cyclones.
Martin Ebert, Ralf Weigel, Stephan Weinbruch, Lisa Schneider, Konrad Kandler, Stefan Lauterbach, Franziska Köllner, Felix Plöger, Gebhard Günther, Bärbel Vogel, and Stephan Borrmann
Atmos. Chem. Phys., 24, 4771–4788, https://doi.org/10.5194/acp-24-4771-2024, https://doi.org/10.5194/acp-24-4771-2024, 2024
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Particles were collected during the flight campaign StratoClim 2017 within the Asian tropopause aerosol layer (ATAL). Refractory particles from seven different flights were characterized by scanning and transmission electron microscopy (SEM, TEM). The most abundant refractory particles are silicates and non-volatile organics. The most important sources are combustion processes at the ground and the agitation of soil material. During one flight, small cinnabar particles (HgS) were also detected.
Hanno Müller, André Ehrlich, Evelyn Jäkel, Johannes Röttenbacher, Benjamin Kirbus, Michael Schäfer, Robin J. Hogan, and Manfred Wendisch
Atmos. Chem. Phys., 24, 4157–4175, https://doi.org/10.5194/acp-24-4157-2024, https://doi.org/10.5194/acp-24-4157-2024, 2024
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A weather model is used to compare solar radiation with measurements from an aircraft campaign in the Arctic. Model and observations agree on the downward radiation but show differences in the radiation reflected by the surface and the clouds, which in the model is too low above sea ice and too high above open ocean. The model–observation bias is reduced above open ocean by a realistic fraction of clouds and less cloud liquid water and above sea ice by less dark sea ice and more cloud droplets.
Gabriela R. Unfer, Luiz A. T. Machado, Paulo Artaxo, Marco A. Franco, Leslie A. Kremper, Mira L. Pöhlker, Ulrich Pöschl, and Christopher Pöhlker
Atmos. Chem. Phys., 24, 3869–3882, https://doi.org/10.5194/acp-24-3869-2024, https://doi.org/10.5194/acp-24-3869-2024, 2024
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Amazonian aerosols and their interactions with precipitation were studied by understanding them in a 3D space based on three parameters that characterize the concentration and size distribution of aerosols. The results showed characteristic arrangements regarding seasonal and diurnal cycles, as well as when interacting with precipitation. The use of this 3D space appears to be a promising tool for aerosol population analysis and for model validation and parameterization.
Benjamin Kirbus, Imke Schirmacher, Marcus Klingebiel, Michael Schäfer, André Ehrlich, Nils Slättberg, Johannes Lucke, Manuel Moser, Hanno Müller, and Manfred Wendisch
Atmos. Chem. Phys., 24, 3883–3904, https://doi.org/10.5194/acp-24-3883-2024, https://doi.org/10.5194/acp-24-3883-2024, 2024
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A research aircraft is used to track the changes in air temperature, moisture, and cloud properties for air that moves from cold Arctic sea ice onto warmer oceanic waters. The measurements are compared to two reanalysis models named ERA5 and CARRA. The biggest differences are found for air temperature over the sea ice and moisture over the ocean. CARRA data are more accurate than ERA5 because they better simulate the sea ice, the transition from sea ice to open ocean, and the forming clouds.
Raphael Satoru Märkl, Christiane Voigt, Daniel Sauer, Rebecca Katharina Dischl, Stefan Kaufmann, Theresa Harlaß, Valerian Hahn, Anke Roiger, Cornelius Weiß-Rehm, Ulrike Burkhardt, Ulrich Schumann, Andreas Marsing, Monika Scheibe, Andreas Dörnbrack, Charles Renard, Maxime Gauthier, Peter Swann, Paul Madden, Darren Luff, Reetu Sallinen, Tobias Schripp, and Patrick Le Clercq
Atmos. Chem. Phys., 24, 3813–3837, https://doi.org/10.5194/acp-24-3813-2024, https://doi.org/10.5194/acp-24-3813-2024, 2024
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In situ measurements of contrails from a large passenger aircraft burning 100 % sustainable aviation fuel (SAF) show a 56 % reduction in contrail ice crystal numbers compared to conventional Jet A-1. Results from a climate model initialized with the observations suggest a significant decrease in radiative forcing from contrails. Our study confirms that future increased use of low aromatic SAF can reduce the climate impact from aviation.
Lea Volkmer, Veronika Pörtge, Fabian Jakub, and Bernhard Mayer
Atmos. Meas. Tech., 17, 1703–1719, https://doi.org/10.5194/amt-17-1703-2024, https://doi.org/10.5194/amt-17-1703-2024, 2024
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Three-dimensional radiative transfer simulations are used to evaluate the performance of retrieval algorithms in the derivation of cloud geometry (cloud top heights) and cloud droplet size distributions from two-dimensional polarized radiance measurements of the airborne spectrometer of the Munich Aerosol Cloud Scanner. The cloud droplet size distributions are derived for the effective radius and variance. The simulations are based on cloud data from highly resolved large-eddy simulations.
Luisa von Albedyll, Stefan Hendricks, Nils Hutter, Dmitrii Murashkin, Lars Kaleschke, Sascha Willmes, Linda Thielke, Xiangshan Tian-Kunze, Gunnar Spreen, and Christian Haas
The Cryosphere, 18, 1259–1285, https://doi.org/10.5194/tc-18-1259-2024, https://doi.org/10.5194/tc-18-1259-2024, 2024
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Leads (openings in sea ice cover) are created by sea ice dynamics. Because they are important for many processes in the Arctic winter climate, we aim to detect them with satellites. We present two new techniques to detect lead widths of a few hundred meters at high spatial resolution (700 m) and independent of clouds or sun illumination. We use the MOSAiC drift 2019–2020 in the Arctic for our case study and compare our new products to other existing lead products.
Evelyn Jäkel, Sebastian Becker, Tim R. Sperzel, Hannah Niehaus, Gunnar Spreen, Ran Tao, Marcel Nicolaus, Wolfgang Dorn, Annette Rinke, Jörg Brauchle, and Manfred Wendisch
The Cryosphere, 18, 1185–1205, https://doi.org/10.5194/tc-18-1185-2024, https://doi.org/10.5194/tc-18-1185-2024, 2024
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The results of the surface albedo scheme of a coupled regional climate model were evaluated against airborne and ground-based measurements conducted in the European Arctic in different seasons between 2017 and 2022. We found a seasonally dependent bias between measured and modeled surface albedo for cloudless and cloudy situations. The strongest effects of the albedo model bias on the net irradiance were most apparent in the presence of optically thin clouds.
Nina Maherndl, Manuel Moser, Johannes Lucke, Mario Mech, Nils Risse, Imke Schirmacher, and Maximilian Maahn
Atmos. Meas. Tech., 17, 1475–1495, https://doi.org/10.5194/amt-17-1475-2024, https://doi.org/10.5194/amt-17-1475-2024, 2024
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In some clouds, liquid water droplets can freeze onto ice crystals (riming). Riming leads to the formation of snowflakes. We show two ways to quantify riming using aircraft data collected in the Arctic. One aircraft had a cloud radar, while the other aircraft was measuring directly in cloud. The first method compares radar and direct observations. The second looks at snowflake shape. Both methods agree, except when there were gaps in the cloud. This improves our ability to understand riming.
Anil Kumar Mandariya, Junteng Wu, Anne Monod, Paola Formenti, Bénédicte Picquet-Varrault, Mathieu Cazaunau, Stephan Mertes, Laurent Poulain, Antonin Berge, Edouard Pangui, Andreas Tilgner, Thomas Schaefer, Liang Wen, Hartmut Herrmann, and Jean-François Doussin
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-206, https://doi.org/10.5194/amt-2023-206, 2024
Publication in AMT not foreseen
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An optimized and controlled protocol for generating quasi-adiabatic expansion clouds under simulated dark and light conditions was presented. The irradiated clouds clearly showed a gradual activation of seed particles into droplets. In contrast, non-irradiated clouds faced a flash activation. This paper will lay the foundation for multiphase photochemical studies implying water-soluble volatile organic compounds and particulate matter formation during cloud formation-evaporation cycles.
Anna Weber, Tobias Kölling, Veronika Pörtge, Andreas Baumgartner, Clemens Rammeloo, Tobias Zinner, and Bernhard Mayer
Atmos. Meas. Tech., 17, 1419–1439, https://doi.org/10.5194/amt-17-1419-2024, https://doi.org/10.5194/amt-17-1419-2024, 2024
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In this work, we introduce the 2D RGB polarization-resolving cameras of the airborne hyperspectral and polarized imaging system specMACS. A full characterization and calibration of the cameras including a geometric calibration as well as a radiometric characterization is provided, allowing for the computation of absolute calibrated, georeferenced Stokes vectors rotated into the scattering plane. We validate the calibration by comparing sunglint measurements to radiative transfer simulations.
Adrien Deroubaix, Marco Vountas, Benjamin Gaubert, Maria Dolores Andrés Hernández, Stephan Borrmann, Guy Brasseur, Bruna Holanda, Yugo Kanaya, Katharina Kaiser, Flora Kluge, Ovid Oktavian Krüger, Inga Labuhn, Michael Lichtenstern, Klaus Pfeilsticker, Mira Pöhlker, Hans Schlager, Johannes Schneider, Guillaume Siour, Basudev Swain, Paolo Tuccella, Kameswara S. Vinjamuri, Mihalis Vrekoussis, Benjamin Weyland, and John P. Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2024-516, https://doi.org/10.5194/egusphere-2024-516, 2024
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This study assesses atmospheric composition using air quality models during aircraft campaigns in Europe and Asia, focusing on carbonaceous aerosols and trace gases. While carbon monoxide is well modeled, other pollutants have moderate to weak agreement with observations. Wind speed modeling is reliable for identifying pollution plumes, where models tend to overestimate concentrations. This highlights challenges in accurately modeling aerosol and trace gas composition, particularly in cities.
Adrien Deroubaix, Marco Vountas, Benjamin Gaubert, Maria Dolores Andrés Hernández, Stephan Borrmann, Guy Brasseur, Bruna Holanda, Yugo Kanaya, Katharina Kaiser, Flora Kluge, Ovid Oktavian Krüger, Inga Labuhn, Michael Lichtenstern, Klaus Pfeilsticker, Mira Pöhlker, Hans Schlager, Johannes Schneider, Guillaume Siour, Basudev Swain, Paolo Tuccella, Kameswara S. Vinjamuri, Mihalis Vrekoussis, Benjamin Weyland, and John P. Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2024-521, https://doi.org/10.5194/egusphere-2024-521, 2024
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This study explores the proportional relationships between carbonaceous aerosols (black and organic carbon) and trace gases using airborne measurements from two campaigns in Europe and East Asia. Differences between regions were found, but air quality models struggled to reproduce them accurately. We show that these proportional relationships can help to constrain models and can be used to infer aerosol concentrations from satellite observations of trace gases, especially in urban areas.
Tereza Uhlíková, Timo Vihma, Alexey Yu Karpechko, and Petteri Uotila
The Cryosphere, 18, 957–976, https://doi.org/10.5194/tc-18-957-2024, https://doi.org/10.5194/tc-18-957-2024, 2024
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A prerequisite for understanding the local, regional, and hemispherical impacts of Arctic sea-ice decline on the atmosphere is to quantify the effects of sea-ice concentration (SIC) on the sensible and latent heat fluxes in the Arctic. We analyse these effects utilising four data sets called atmospheric reanalyses, and we evaluate uncertainties in these effects arising from inter-reanalysis differences in SIC and in the sensitivity of the latent and sensible heat fluxes to SIC.
Larissa Lacher, Michael P. Adams, Kevin Barry, Barbara Bertozzi, Heinz Bingemer, Cristian Boffo, Yannick Bras, Nicole Büttner, Dimitri Castarede, Daniel J. Cziczo, Paul J. DeMott, Romy Fösig, Megan Goodell, Kristina Höhler, Thomas C. J. Hill, Conrad Jentzsch, Luis A. Ladino, Ezra J. T. Levin, Stephan Mertes, Ottmar Möhler, Kathryn A. Moore, Benjamin J. Murray, Jens Nadolny, Tatjana Pfeuffer, David Picard, Carolina Ramírez-Romero, Mickael Ribeiro, Sarah Richter, Jann Schrod, Karine Sellegri, Frank Stratmann, Benjamin E. Swanson, Erik S. Thomson, Heike Wex, Martin J. Wolf, and Evelyn Freney
Atmos. Chem. Phys., 24, 2651–2678, https://doi.org/10.5194/acp-24-2651-2024, https://doi.org/10.5194/acp-24-2651-2024, 2024
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Aerosol particles that trigger ice formation in clouds are important for the climate system but are very rare in the atmosphere, challenging measurement techniques. Here we compare three cloud chambers and seven methods for collecting aerosol particles on filters for offline analysis at a mountaintop station. A general good agreement of the methods was found when sampling aerosol particles behind a whole air inlet, supporting their use for obtaining data that can be implemented in models.
Hannah Niehaus, Larysa Istomina, Marcel Nicolaus, Ran Tao, Aleksey Malinka, Eleonora Zege, and Gunnar Spreen
The Cryosphere, 18, 933–956, https://doi.org/10.5194/tc-18-933-2024, https://doi.org/10.5194/tc-18-933-2024, 2024
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Melt ponds are puddles of meltwater which form on Arctic sea ice in the summer period. They are darker than the ice cover and lead to increased absorption of solar energy. Global climate models need information about the Earth's energy budget. Thus satellite observations are used to monitor the surface fractions of melt ponds, ocean, and sea ice in the entire Arctic. We present a new physically based algorithm that can separate these three surface types with uncertainty below 10 %.
Andrea Cuesta-Mosquera, Kristina Glojek, Griša Močnik, Luka Drinovec, Asta Gregorič, Martin Rigler, Matej Ogrin, Baseerat Romshoo, Kay Weinhold, Maik Merkel, Dominik van Pinxteren, Hartmut Herrmann, Alfred Wiedensohler, Mira Pöhlker, and Thomas Müller
Atmos. Chem. Phys., 24, 2583–2605, https://doi.org/10.5194/acp-24-2583-2024, https://doi.org/10.5194/acp-24-2583-2024, 2024
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This study evaluated the air pollution and climate impacts of residential-wood-burning particle emissions from a rural European site. The authors investigate the optical and physical properties that connect the aerosol emissions with climate by evaluating atmospheric radiative impacts via simple-forcing calculations. The study contributes to reducing the lack of information on the understanding of the optical properties of air pollution from anthropogenic sources.
Robert Hanfland, Dominik Brunner, Christiane Voigt, Alina Fiehn, Anke Roiger, and Margit Pattantyús-Ábrahám
Atmos. Chem. Phys., 24, 2511–2534, https://doi.org/10.5194/acp-24-2511-2024, https://doi.org/10.5194/acp-24-2511-2024, 2024
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To show that the three-dimensional dispersion of plumes simulated by the Atmospheric Radionuclide Transport Model within the planetary boundary layer agrees with real plumes, we identify the most important input parameters and analyse the turbulence properties of five different turbulence models in very unstable stratification conditions using their deviation from the well-mixed state. Simulations show that one model agrees slightly better in unstable stratification conditions.
Hauke Schmidt, Sebastian Rast, Jiawei Bao, Amrit Cassim, Shih-Wei Fang, Diego Jimenez-de la Cuesta, Paul Keil, Lukas Kluft, Clarissa Kroll, Theresa Lang, Ulrike Niemeier, Andrea Schneidereit, Andrew I. L. Williams, and Bjorn Stevens
Geosci. Model Dev., 17, 1563–1584, https://doi.org/10.5194/gmd-17-1563-2024, https://doi.org/10.5194/gmd-17-1563-2024, 2024
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A recent development in numerical simulations of the global atmosphere is the increase in horizontal resolution to grid spacings of a few kilometers. However, the vertical grid spacing of these models has not been reduced at the same rate as the horizontal grid spacing. Here, we assess the effects of much finer vertical grid spacings, in particular the impacts on cloud quantities and the atmospheric energy balance.
Michael Lonardi, Elisa F. Akansu, André Ehrlich, Mauro Mazzola, Christian Pilz, Matthew D. Shupe, Holger Siebert, and Manfred Wendisch
Atmos. Chem. Phys., 24, 1961–1978, https://doi.org/10.5194/acp-24-1961-2024, https://doi.org/10.5194/acp-24-1961-2024, 2024
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Profiles of thermal-infrared irradiance were measured at two Arctic sites. The presence or lack of clouds influences the vertical structure of these observations. In particular, the cloud top region is a source of radiative energy that can promote cooling and mixing in the cloud layer. Simulations are used to further characterize how the amount of water in the cloud modifies this forcing. A case study additionally showcases the evolution of the radiation profiles in a dynamic atmosphere.
Maximilian Maahn, Dmitri Moisseev, Isabelle Steinke, Nina Maherndl, and Matthew D. Shupe
Atmos. Meas. Tech., 17, 899–919, https://doi.org/10.5194/amt-17-899-2024, https://doi.org/10.5194/amt-17-899-2024, 2024
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The open-source Video In Situ Snowfall Sensor (VISSS) is a novel instrument for characterizing particle shape, size, and sedimentation velocity in snowfall. It combines a large observation volume with relatively high resolution and a design that limits wind perturbations. The open-source nature of the VISSS hardware and software invites the community to contribute to the development of the instrument, which has many potential applications in atmospheric science and beyond.
Gina C. Jozef, John J. Cassano, Sandro Dahlke, Mckenzie Dice, Christopher J. Cox, and Gijs de Boer
Atmos. Chem. Phys., 24, 1429–1450, https://doi.org/10.5194/acp-24-1429-2024, https://doi.org/10.5194/acp-24-1429-2024, 2024
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Observations collected during MOSAiC were used to identify the range in vertical structure and stability of the central Arctic lower atmosphere through a self-organizing map analysis. Characteristics of wind features (such as low-level jets) and atmospheric moisture features (such as clouds) were analyzed in the context of the varying vertical structure and stability. Thus, the results of this paper give an overview of the thermodynamic and kinematic features of the central Arctic atmosphere.
Sabrina Schnitt, Andreas Foth, Heike Kalesse-Los, Mario Mech, Claudia Acquistapace, Friedhelm Jansen, Ulrich Löhnert, Bernhard Pospichal, Johannes Röttenbacher, Susanne Crewell, and Bjorn Stevens
Earth Syst. Sci. Data, 16, 681–700, https://doi.org/10.5194/essd-16-681-2024, https://doi.org/10.5194/essd-16-681-2024, 2024
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This publication describes the microwave radiometric measurements performed during the EUREC4A campaign at Barbados Cloud Observatory (BCO) and aboard RV Meteor and RV Maria S Merian. We present retrieved integrated water vapor (IWV), liquid water path (LWP), and temperature and humidity profiles as a unified, quality-controlled, multi-site data set on a 3 s temporal resolution for a core period between 19 January 2020 and 14 February 2020.
Basudev Swain, Marco Vountas, Adrien Deroubaix, Luca Lelli, Yanick Ziegler, Soheila Jafariserajehlou, Sachin S. Gunthe, Andreas Herber, Christoph Ritter, Hartmut Bösch, and John P. Burrows
Atmos. Meas. Tech., 17, 359–375, https://doi.org/10.5194/amt-17-359-2024, https://doi.org/10.5194/amt-17-359-2024, 2024
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Aerosols are suspensions of particles dispersed in the air. In this study, we use a novel retrieval of satellite data to investigate an optical property of aerosols, the aerosol optical depth, in the high Arctic to assess their direct and indirect roles in climate change. This study demonstrates that the presented approach shows good quality and very promising potential.
Cheikh Dione, Martial Haeffelin, Frédéric Burnet, Christine Lac, Guylaine Canut, Julien Delanoë, Jean-Charles Dupont, Susana Jorquera, Pauline Martinet, Jean-François Ribaud, and Felipe Toledo
Atmos. Chem. Phys., 23, 15711–15731, https://doi.org/10.5194/acp-23-15711-2023, https://doi.org/10.5194/acp-23-15711-2023, 2023
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This paper documents the role of thermodynamics and turbulence in the fog life cycle over southwestern France. It is based on a unique dataset collected during the SOFOG3D field campaign in autumn and winter 2019–2020. The paper gives a threshold for turbulence driving the different phases of the fog life cycle and the role of advection in the night-time dissipation of fog. The results can be operationalised to nowcast fog and improve short-range forecasts in numerical weather prediction models.
Elisa F. Akansu, Sandro Dahlke, Holger Siebert, and Manfred Wendisch
Atmos. Chem. Phys., 23, 15473–15489, https://doi.org/10.5194/acp-23-15473-2023, https://doi.org/10.5194/acp-23-15473-2023, 2023
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The height of the mixing layer is an important measure of the surface-level distribution of energy or other substances. The experimental determination of this height is associated with large uncertainties, particularly under stable conditions that we often find during the polar night or in the presence of clouds. We present a reference method using turbulence measurements on a tethered balloon, which allows us to evaluate approaches based on radiosondes or surface observations.
Ulrike Egerer, Holger Siebert, Olaf Hellmuth, and Lise Lotte Sørensen
Atmos. Chem. Phys., 23, 15365–15373, https://doi.org/10.5194/acp-23-15365-2023, https://doi.org/10.5194/acp-23-15365-2023, 2023
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Low-level jets (LLJs) are strong winds near the surface and occur frequently in the Arctic in stable conditions. Using tethered-balloon profile measurements in Greenland, we analyze a multi-hour period with an LLJ that later weakens and finally collapses. Increased shear-induced turbulence at the LLJ bounds mostly does not reach the ground until the LLJ collapses. Our findings support the hypothesis that a passive tracer can be advected with an LLJ and mixed down when the LLJ collapses.
Marcus Klingebiel, André Ehrlich, Elena Ruiz-Donoso, Nils Risse, Imke Schirmacher, Evelyn Jäkel, Michael Schäfer, Kevin Wolf, Mario Mech, Manuel Moser, Christiane Voigt, and Manfred Wendisch
Atmos. Chem. Phys., 23, 15289–15304, https://doi.org/10.5194/acp-23-15289-2023, https://doi.org/10.5194/acp-23-15289-2023, 2023
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In this study we explain how we use aircraft measurements from two Arctic research campaigns to identify cloud properties (like droplet size) over sea-ice and ice-free ocean. To make sure that our measurements make sense, we compare them with other observations. Our results show, e.g., larger cloud droplets in early summer than in spring. Moreover, the cloud droplets are also larger over ice-free ocean than compared to sea ice. In the future, our data can be used to improve climate models.
Lejiang Yu, Shiyuan Zhong, Timo Vihma, Cuijuan Sui, and Bo Sun
EGUsphere, https://doi.org/10.5194/egusphere-2023-2436, https://doi.org/10.5194/egusphere-2023-2436, 2023
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In contrary to the current understanding, there can be a strong connection between ENSO and the South Atlantic Subtropical Dipole (SASD). It is highly probable that the robust inverse correlation between ENSO and SASD will persist in the future. The ENSO-SASD correlation exhibits substantial multi-decadal variability over the course of a century. The change in the ENSO-SASD relation can be linked to changes in ENSO regime and convective activities over the central South Pacific Ocean.
Giovanni Chellini, Rosa Gierens, Kerstin Ebell, Theresa Kiszler, Pavel Krobot, Alexander Myagkov, Vera Schemann, and Stefan Kneifel
Earth Syst. Sci. Data, 15, 5427–5448, https://doi.org/10.5194/essd-15-5427-2023, https://doi.org/10.5194/essd-15-5427-2023, 2023
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We present a comprehensive quality-controlled dataset of remote sensing observations of low-level mixed-phase clouds (LLMPCs) taken at the high Arctic site of Ny-Ålesund, Svalbard, Norway. LLMPCs occur frequently in the Arctic region, and substantially warm the surface. However, our understanding of microphysical processes in these clouds is incomplete. This dataset includes a comprehensive set of variables which allow for extensive investigation of such processes in LLMPCs at the site.
Bjorn Stevens and Lukas Kluft
Atmos. Chem. Phys., 23, 14673–14689, https://doi.org/10.5194/acp-23-14673-2023, https://doi.org/10.5194/acp-23-14673-2023, 2023
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A simple model is introduced to account for the spectral diversity of radiant energy transfer. It provides an improved basis for assessing the different ways in which clouds influence Earth’s climate sensitivity, demonstrating how many cloud effects depend on the existing cloud climatology. Given existing assessments of changes in cloud albedo with warming, it is determined that clouds reduce Earth's climate sensitivity as compared to what it would be in a counterfactual world without clouds.
Leonie Villiger, Marina Dütsch, Sandrine Bony, Marie Lothon, Stephan Pfahl, Heini Wernli, Pierre-Etienne Brilouet, Patrick Chazette, Pierre Coutris, Julien Delanoë, Cyrille Flamant, Alfons Schwarzenboeck, Martin Werner, and Franziska Aemisegger
Atmos. Chem. Phys., 23, 14643–14672, https://doi.org/10.5194/acp-23-14643-2023, https://doi.org/10.5194/acp-23-14643-2023, 2023
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This study evaluates three numerical simulations performed with an isotope-enabled weather forecast model and investigates the coupling between shallow trade-wind cumulus clouds and atmospheric circulations on different scales. We show that the simulations reproduce key characteristics of shallow trade-wind clouds as observed during the field experiment EUREC4A and that the spatial distribution of stable-water-vapour isotopes is shaped by the overturning circulation associated with these clouds.
Pablo Saavedra Garfias, Heike Kalesse-Los, Luisa von Albedyll, Hannes Griesche, and Gunnar Spreen
Atmos. Chem. Phys., 23, 14521–14546, https://doi.org/10.5194/acp-23-14521-2023, https://doi.org/10.5194/acp-23-14521-2023, 2023
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An important Arctic climate process is the release of heat fluxes from sea ice openings to the atmosphere that influence the clouds. The characterization of this process is the objective of this study. Using synergistic observations from the MOSAiC expedition, we found that single-layer cloud properties show significant differences when clouds are coupled or decoupled to the water vapour transport which is used as physical link between the upwind sea ice openings and the cloud under observation.
Barbara Harm-Altstädter, Konrad Bärfuss, Lutz Bretschneider, Martin Schön, Jens Bange, Ralf Käthner, Radovan Krejci, Mauro Mazzola, Kihong Park, Falk Pätzold, Alexander Peuker, Rita Traversi, Birgit Wehner, and Astrid Lampert
Aerosol Research, 1, 39–64, https://doi.org/10.5194/ar-1-39-2023, https://doi.org/10.5194/ar-1-39-2023, 2023
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We present observations of aerosol particles and meteorological parameters in the horizontal and vertical distribution measured with uncrewed aerial systems in the Arctic. The field campaign was carried out during the snow melting season, when ultrafine aerosol particles (UFPs) with a size between 3 and 12 nm occurred frequently. A high variability of the measured UFPs was identified in the spatial scale, which was strongly associated with different atmospheric boundary layer properties.
Gina C. Jozef, Robert Klingel, John J. Cassano, Björn Maronga, Gijs de Boer, Sandro Dahlke, and Christopher J. Cox
Earth Syst. Sci. Data, 15, 4983–4995, https://doi.org/10.5194/essd-15-4983-2023, https://doi.org/10.5194/essd-15-4983-2023, 2023
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Observations from the MOSAiC expedition relating to lower-atmospheric temperature, wind, stability, moisture, and surface radiation budget from radiosondes, a meteorological tower, radiation station, and ceilometer were compiled to create a dataset which describes the thermodynamic and kinematic state of the central Arctic lower atmosphere between October 2019 and September 2020. This paper describes the methods used to develop this lower-atmospheric properties dataset.
Harald Sodemann, Alena Dekhtyareva, Alvaro Fernandez, Andrew Seidl, and Jenny Maccali
Atmos. Meas. Tech., 16, 5181–5203, https://doi.org/10.5194/amt-16-5181-2023, https://doi.org/10.5194/amt-16-5181-2023, 2023
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We describe a device that allows one to produce a continuous stream of water vapour with a specified level of humidity. As a main innovation, we can mix waters with different water isotope composition. Through a series of tests we show that the performance characteristics of the device are in line with specifications. We present two laboratory applications where the device proves useful, first in characterizing instruments, and second for the analysis of water contained in stalagmites.
Tiina Nygård, Lukas Papritz, Tuomas Naakka, and Timo Vihma
Weather Clim. Dynam., 4, 943–961, https://doi.org/10.5194/wcd-4-943-2023, https://doi.org/10.5194/wcd-4-943-2023, 2023
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Despite the general warming trend, wintertime cold-air outbreaks in Europe have remained nearly as extreme and as common as decades ago. In this study, we identify six principal cold anomaly types over Europe in 1979–2020. We show the origins of various physical processes and their contributions to the formation of cold wintertime air masses.
James Barry, Stefanie Meilinger, Klaus Pfeilsticker, Anna Herman-Czezuch, Nicola Kimiaie, Christopher Schirrmeister, Rone Yousif, Tina Buchmann, Johannes Grabenstein, Hartwig Deneke, Jonas Witthuhn, Claudia Emde, Felix Gödde, Bernhard Mayer, Leonhard Scheck, Marion Schroedter-Homscheidt, Philipp Hofbauer, and Matthias Struck
Atmos. Meas. Tech., 16, 4975–5007, https://doi.org/10.5194/amt-16-4975-2023, https://doi.org/10.5194/amt-16-4975-2023, 2023
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Measured power data from solar photovoltaic (PV) systems contain information about the state of the atmosphere. In this work, power data from PV systems in the Allgäu region in Germany were used to determine the solar irradiance at each location, using state-of-the-art simulation and modelling. The results were validated using concurrent measurements of the incoming solar radiation in each case. If applied on a wider scale, this algorithm could help improve weather and climate models.
Francesco Cairo, Martina Krämer, Armin Afchine, Guido Di Donfrancesco, Luca Di Liberto, Sergey Khaykin, Lorenza Lucaferri, Valentin Mitev, Max Port, Christian Rolf, Marcel Snels, Nicole Spelten, Ralf Weigel, and Stephan Borrmann
Atmos. Meas. Tech., 16, 4899–4925, https://doi.org/10.5194/amt-16-4899-2023, https://doi.org/10.5194/amt-16-4899-2023, 2023
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Cirrus clouds have been observed over the Himalayan region between 10 km and the tropopause at 17–18 km. Data from backscattersonde, hygrometers, and particle cloud spectrometers have been compared to assess their consistency. Empirical relationships between optical parameters accessible with remote sensing lidars and cloud microphysical parameters (such as ice water content, particle number and surface area density, and particle aspherical fraction) have been established.
Pierre Grzegorczyk, Sudha Yadav, Florian Zanger, Alexander Theis, Subir K. Mitra, Stephan Borrmann, and Miklós Szakáll
Atmos. Chem. Phys., 23, 13505–13521, https://doi.org/10.5194/acp-23-13505-2023, https://doi.org/10.5194/acp-23-13505-2023, 2023
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Secondary ice production generates high concentrations of ice crystals in clouds. These processes have been poorly understood. We conducted experiments at the wind tunnel laboratory of the Johannes Gutenberg University, Mainz, on graupel–graupel and graupel–snowflake collisions. From these experiments fragment number, size, cross-sectional area, and aspect ratio were determined.
Elena De La Torre Castro, Tina Jurkat-Witschas, Armin Afchine, Volker Grewe, Valerian Hahn, Simon Kirschler, Martina Krämer, Johannes Lucke, Nicole Spelten, Heini Wernli, Martin Zöger, and Christiane Voigt
Atmos. Chem. Phys., 23, 13167–13189, https://doi.org/10.5194/acp-23-13167-2023, https://doi.org/10.5194/acp-23-13167-2023, 2023
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In this study, we show the differences in the microphysical properties between high-latitude (HL) cirrus and mid-latitude (ML) cirrus over the Arctic, North Atlantic, and central Europe during summer. The in situ measurements are combined with backward trajectories to investigate the influence of the region on cloud formation. We show that HL cirrus are characterized by a lower concentration of larger ice crystals when compared to ML cirrus.
Gina C. Jozef, John J. Cassano, Sandro Dahlke, Mckenzie Dice, Christopher J. Cox, and Gijs de Boer
Atmos. Chem. Phys., 23, 13087–13106, https://doi.org/10.5194/acp-23-13087-2023, https://doi.org/10.5194/acp-23-13087-2023, 2023
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Observations from the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) were used to determine the frequency of occurrence of various central Arctic lower atmospheric stability regimes and how the stability regimes transition between each other. Wind and radiation observations were analyzed in the context of stability regime and season to reveal the relationships between Arctic atmospheric stability and mechanically and radiatively driven turbulent forcings.
Albert Ansmann, Kevin Ohneiser, Ronny Engelmann, Martin Radenz, Hannes Griesche, Julian Hofer, Dietrich Althausen, Jessie M. Creamean, Matthew C. Boyer, Daniel A. Knopf, Sandro Dahlke, Marion Maturilli, Henriette Gebauer, Johannes Bühl, Cristofer Jimenez, Patric Seifert, and Ulla Wandinger
Atmos. Chem. Phys., 23, 12821–12849, https://doi.org/10.5194/acp-23-12821-2023, https://doi.org/10.5194/acp-23-12821-2023, 2023
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The 1-year MOSAiC (2019–2020) expedition with the German ice breaker Polarstern was the largest polar field campaign ever conducted. The Polarstern, with our lidar aboard, drifted with the pack ice north of 85° N for more than 7 months (October 2019 to mid-May 2020). We measured the full annual cycle of aerosol conditions in terms of aerosol optical and cloud-process-relevant properties. We observed a strong contrast between polluted winter and clean summer aerosol conditions.
Sarah Grawe, Conrad Jentzsch, Jonas Schaefer, Heike Wex, Stephan Mertes, and Frank Stratmann
Atmos. Meas. Tech., 16, 4551–4570, https://doi.org/10.5194/amt-16-4551-2023, https://doi.org/10.5194/amt-16-4551-2023, 2023
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Measurements of ice-nucleating particle (INP) concentrations are valuable for the simulation of cloud properties. In recent years, filter sampling in combination with offline INP measurements has become increasingly popular. However, most sampling is ground-based, and the vertical transport of INPs is not well quantified. The High-volume flow aERosol particle filter sAmpler (HERA) for applications on board aircraft was developed to expand the sparse dataset of INP concentrations at cloud level.
Simon Kirschler, Christiane Voigt, Bruce E. Anderson, Gao Chen, Ewan C. Crosbie, Richard A. Ferrare, Valerian Hahn, Johnathan W. Hair, Stefan Kaufmann, Richard H. Moore, David Painemal, Claire E. Robinson, Kevin J. Sanchez, Amy J. Scarino, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Edward L. Winstead, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 23, 10731–10750, https://doi.org/10.5194/acp-23-10731-2023, https://doi.org/10.5194/acp-23-10731-2023, 2023
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In this study we present an overview of liquid and mixed-phase clouds and precipitation in the marine boundary layer over the western North Atlantic Ocean. We compare microphysical properties of pure liquid clouds to mixed-phase clouds and show that the initiation of the ice phase in mixed-phase clouds promotes precipitation. The observational data presented in this study are well suited for investigating the processes that give rise to liquid and mixed-phase clouds, ice, and precipitation.
Angela Mynard, Joss Kent, Eleanor R. Smith, Andy Wilson, Kirsty Wivell, Noel Nelson, Matthew Hort, James Bowles, David Tiddeman, Justin M. Langridge, Benjamin Drummond, and Steven J. Abel
Atmos. Meas. Tech., 16, 4229–4261, https://doi.org/10.5194/amt-16-4229-2023, https://doi.org/10.5194/amt-16-4229-2023, 2023
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Air quality models are key in understanding complex air pollution processes and assist in developing strategies to mitigate the impacts of air pollution. The ability of regional air quality models to skilfully represent pollutant distributions aloft is important to enabling their skilful prediction at the surface. To assist in model development and evaluation, a long-term, quality-assured dataset of the 3-D distribution of key pollutants was collected over the United Kingdom (2019–2022).
Alexander Mchedlishvili, Christof Lüpkes, Alek Petty, Michel Tsamados, and Gunnar Spreen
The Cryosphere, 17, 4103–4131, https://doi.org/10.5194/tc-17-4103-2023, https://doi.org/10.5194/tc-17-4103-2023, 2023
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In this study we looked at sea ice–atmosphere drag coefficients, quantities that help with characterizing the friction between the atmosphere and sea ice, and vice versa. Using ICESat-2, a laser altimeter that measures elevation differences by timing how long it takes for photons it sends out to return to itself, we could map the roughness, i.e., how uneven the surface is. From roughness we then estimate drag force, the frictional force between sea ice and the atmosphere, across the Arctic.
Imke Schirmacher, Pavlos Kollias, Katia Lamer, Mario Mech, Lukas Pfitzenmaier, Manfred Wendisch, and Susanne Crewell
Atmos. Meas. Tech., 16, 4081–4100, https://doi.org/10.5194/amt-16-4081-2023, https://doi.org/10.5194/amt-16-4081-2023, 2023
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CloudSat’s relatively coarse spatial resolution, low sensitivity, and blind zone limit its assessment of Arctic low-level clouds, which affect the surface energy balance. We compare cloud fractions from CloudSat and finely resolved airborne radar observations to determine CloudSat’s limitations. Cloudsat overestimates cloud fractions above its blind zone, especially during cold-air outbreaks over open water, and misses a cloud fraction of 32 % and half of the precipitation inside its blind zone.
Olivia Linke, Johannes Quaas, Finja Baumer, Sebastian Becker, Jan Chylik, Sandro Dahlke, André Ehrlich, Dörthe Handorf, Christoph Jacobi, Heike Kalesse-Los, Luca Lelli, Sina Mehrdad, Roel A. J. Neggers, Johannes Riebold, Pablo Saavedra Garfias, Niklas Schnierstein, Matthew D. Shupe, Chris Smith, Gunnar Spreen, Baptiste Verneuil, Kameswara S. Vinjamuri, Marco Vountas, and Manfred Wendisch
Atmos. Chem. Phys., 23, 9963–9992, https://doi.org/10.5194/acp-23-9963-2023, https://doi.org/10.5194/acp-23-9963-2023, 2023
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Lapse rate feedback (LRF) is a major driver of the Arctic amplification (AA) of climate change. It arises because the warming is stronger at the surface than aloft. Several processes can affect the LRF in the Arctic, such as the omnipresent temperature inversion. Here, we compare multimodel climate simulations to Arctic-based observations from a large research consortium to broaden our understanding of these processes, find synergy among them, and constrain the Arctic LRF and AA.
Qian Xiao, Jiaoshi Zhang, Yang Wang, Luke D. Ziemba, Ewan Crosbie, Edward L. Winstead, Claire E. Robinson, Joshua P. DiGangi, Glenn S. Diskin, Jeffrey S. Reid, K. Sebastian Schmidt, Armin Sorooshian, Miguel Ricardo A. Hilario, Sarah Woods, Paul Lawson, Snorre A. Stamnes, and Jian Wang
Atmos. Chem. Phys., 23, 9853–9871, https://doi.org/10.5194/acp-23-9853-2023, https://doi.org/10.5194/acp-23-9853-2023, 2023
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Using recent airborne measurements, we show that the influences of anthropogenic emissions, transport, convective clouds, and meteorology lead to new particle formation (NPF) under a variety of conditions and at different altitudes in tropical marine environments. NPF is enhanced by fresh urban emissions in convective outflow but is suppressed in air masses influenced by aged urban emissions where reactive precursors are mostly consumed while particle surface area remains relatively high.
Philip Rostosky and Gunnar Spreen
The Cryosphere, 17, 3867–3881, https://doi.org/10.5194/tc-17-3867-2023, https://doi.org/10.5194/tc-17-3867-2023, 2023
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During winter, storms entering the Arctic region can bring warm air into the cold environment. Strong increases in air temperature modify the characteristics of the Arctic snow and ice cover. The Arctic sea ice cover can be monitored by satellites observing the natural emission of the Earth's surface. In this study, we show that during warm air intrusions the change in the snow characteristics influences the satellite-derived sea ice cover, leading to a false reduction of the estimated ice area.
Manfred Wendisch, Johannes Stapf, Sebastian Becker, André Ehrlich, Evelyn Jäkel, Marcus Klingebiel, Christof Lüpkes, Michael Schäfer, and Matthew D. Shupe
Atmos. Chem. Phys., 23, 9647–9667, https://doi.org/10.5194/acp-23-9647-2023, https://doi.org/10.5194/acp-23-9647-2023, 2023
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Atmospheric radiation measurements have been conducted during two field campaigns using research aircraft. The data are analyzed to see if the near-surface air in the Arctic is warmed or cooled if warm–humid air masses from the south enter the Arctic or cold–dry air moves from the north from the Arctic to mid-latitude areas. It is important to study these processes and to check if climate models represent them well. Otherwise it is not possible to reliably forecast the future Arctic climate.
Sophie Rosenburg, Charlotte Lange, Evelyn Jäkel, Michael Schäfer, André Ehrlich, and Manfred Wendisch
Atmos. Meas. Tech., 16, 3915–3930, https://doi.org/10.5194/amt-16-3915-2023, https://doi.org/10.5194/amt-16-3915-2023, 2023
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Snow layer melting and melt pond formation on Arctic sea ice are important seasonal processes affecting the surface reflection and energy budget. Sea ice reflectivity was surveyed by airborne imaging spectrometers in May–June 2017. Adapted retrieval approaches were applied to find snow layer liquid water fraction, snow grain effective radius, and melt pond depth. The retrievals show the potential and limitations of spectral airborne imaging to map melting snow layer and melt pond properties.
Amelie U. Schmitt, Felix Ament, Alessandro C. de Araújo, Marta Sá, and Paulo Teixeira
Atmos. Chem. Phys., 23, 9323–9346, https://doi.org/10.5194/acp-23-9323-2023, https://doi.org/10.5194/acp-23-9323-2023, 2023
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Tall vegetation in forests affects the exchange of heat and moisture between the atmosphere and the land surface. We compared measurements from the Amazon Tall Tower Observatory to results from a land surface model to identify model shortcomings. Our results suggest that soil temperatures in the model could be improved by incorporating a separate canopy layer which represents the heat storage within the forest.
Dimitri Castarède, Zoé Brasseur, Yusheng Wu, Zamin A. Kanji, Markus Hartmann, Lauri Ahonen, Merete Bilde, Markku Kulmala, Tuukka Petäjä, Jan B. C. Pettersson, Berko Sierau, Olaf Stetzer, Frank Stratmann, Birgitta Svenningsson, Erik Swietlicki, Quynh Thu Nguyen, Jonathan Duplissy, and Erik S. Thomson
Atmos. Meas. Tech., 16, 3881–3899, https://doi.org/10.5194/amt-16-3881-2023, https://doi.org/10.5194/amt-16-3881-2023, 2023
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Clouds play a key role in Earth’s climate by influencing the surface energy budget. Certain types of atmospheric aerosols, called ice-nucleating particles (INPs), induce the formation of ice in clouds and, thus, often initiate precipitation formation. The Portable Ice Nucleation Chamber 2 (PINCii) is a new instrument developed to study ice formation and to conduct ambient measurements of INPs, allowing us to investigate the sources and properties of the atmospheric aerosols that can act as INPs.
Jake J. Gristey, K. Sebastian Schmidt, Hong Chen, Daniel R. Feldman, Bruce C. Kindel, Joshua Mauss, Mathew van den Heever, Maria Z. Hakuba, and Peter Pilewskie
Atmos. Meas. Tech., 16, 3609–3630, https://doi.org/10.5194/amt-16-3609-2023, https://doi.org/10.5194/amt-16-3609-2023, 2023
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The concept of a satellite-based camera is demonstrated for sampling the angular distribution of outgoing radiance from Earth needed to generate data products for new radiation budget spectral channels.
Melanie Lauer, Annette Rinke, Irina Gorodetskaya, Michael Sprenger, Mario Mech, and Susanne Crewell
Atmos. Chem. Phys., 23, 8705–8726, https://doi.org/10.5194/acp-23-8705-2023, https://doi.org/10.5194/acp-23-8705-2023, 2023
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We present a new method to analyse the influence of atmospheric rivers (ARs), cyclones, and fronts on the precipitation in the Arctic, based on two campaigns: ACLOUD (early summer 2017) and AFLUX (early spring 2019). There are differences between both campaign periods: in early summer, the precipitation is mostly related to ARs and fronts, especially when they are co-located, while in early spring, cyclones isolated from ARs and fronts contributed most to the precipitation.
Shijie Peng, Qinghua Yang, Matthew D. Shupe, Xingya Xi, Bo Han, Dake Chen, Sandro Dahlke, and Changwei Liu
Atmos. Chem. Phys., 23, 8683–8703, https://doi.org/10.5194/acp-23-8683-2023, https://doi.org/10.5194/acp-23-8683-2023, 2023
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Due to a lack of observations, the structure of the Arctic atmospheric boundary layer (ABL) remains to be further explored. By analyzing a year-round radiosonde dataset collected over the Arctic sea-ice surface, we found the annual cycle of the ABL height (ABLH) is primarily controlled by the evolution of ABL thermal structure, and the surface conditions also show a high correlation with ABLH variation. In addition, the Arctic ABLH is found to be decreased in summer compared with 20 years ago.
Amelie U. Schmitt and Christof Lüpkes
The Cryosphere, 17, 3115–3136, https://doi.org/10.5194/tc-17-3115-2023, https://doi.org/10.5194/tc-17-3115-2023, 2023
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In the last few decades, the region between Greenland and Svalbard has experienced the largest loss of Arctic sea ice in winter. We analyze how changes in air temperature, humidity and wind in this region differ for winds that originate from sea ice covered areas and from the open ocean. The largest impacts of sea ice cover are found for temperatures close to the ice edge and up to a distance of 500 km. Up to two-thirds of the observed temperature variability is related to sea ice changes.
Armin Sorooshian, Mikhail D. Alexandrov, Adam D. Bell, Ryan Bennett, Grace Betito, Sharon P. Burton, Megan E. Buzanowicz, Brian Cairns, Eduard V. Chemyakin, Gao Chen, Yonghoon Choi, Brian L. Collister, Anthony L. Cook, Andrea F. Corral, Ewan C. Crosbie, Bastiaan van Diedenhoven, Joshua P. DiGangi, Glenn S. Diskin, Sanja Dmitrovic, Eva-Lou Edwards, Marta A. Fenn, Richard A. Ferrare, David van Gilst, Johnathan W. Hair, David B. Harper, Miguel Ricardo A. Hilario, Chris A. Hostetler, Nathan Jester, Michael Jones, Simon Kirschler, Mary M. Kleb, John M. Kusterer, Sean Leavor, Joseph W. Lee, Hongyu Liu, Kayla McCauley, Richard H. Moore, Joseph Nied, Anthony Notari, John B. Nowak, David Painemal, Kasey E. Phillips, Claire E. Robinson, Amy Jo Scarino, Joseph S. Schlosser, Shane T. Seaman, Chellappan Seethala, Taylor J. Shingler, Michael A. Shook, Kenneth A. Sinclair, William L. Smith Jr., Douglas A. Spangenberg, Snorre A. Stamnes, Kenneth L. Thornhill, Christiane Voigt, Holger Vömel, Andrzej P. Wasilewski, Hailong Wang, Edward L. Winstead, Kira Zeider, Xubin Zeng, Bo Zhang, Luke D. Ziemba, and Paquita Zuidema
Earth Syst. Sci. Data, 15, 3419–3472, https://doi.org/10.5194/essd-15-3419-2023, https://doi.org/10.5194/essd-15-3419-2023, 2023
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The NASA Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) produced a unique dataset for research into aerosol–cloud–meteorology interactions. HU-25 Falcon and King Air aircraft conducted systematic and spatially coordinated flights over the northwest Atlantic Ocean. This paper describes the ACTIVATE flight strategy, instrument and complementary dataset products, data access and usage details, and data application notes.
Valerian Hahn, Ralf Meerkötter, Christiane Voigt, Sonja Gisinger, Daniel Sauer, Valéry Catoire, Volker Dreiling, Hugh Coe, Cyrille Flamant, Stefan Kaufmann, Jonas Kleine, Peter Knippertz, Manuel Moser, Philip Rosenberg, Hans Schlager, Alfons Schwarzenboeck, and Jonathan Taylor
Atmos. Chem. Phys., 23, 8515–8530, https://doi.org/10.5194/acp-23-8515-2023, https://doi.org/10.5194/acp-23-8515-2023, 2023
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During the DACCIWA campaign in West Africa, we found a 35 % increase in the cloud droplet concentration that formed in a polluted compared with a less polluted environment and a decrease of 17 % in effective droplet diameter. Radiative transfer simulations, based on the measured cloud properties, reveal that these low-level polluted clouds radiate only 2.6 % more energy back to space, compared with a less polluted cloud. The corresponding additional decrease in temperature is rather small.
Silke Groß, Tina Jurkat-Witschas, Qiang Li, Martin Wirth, Benedikt Urbanek, Martina Krämer, Ralf Weigel, and Christiane Voigt
Atmos. Chem. Phys., 23, 8369–8381, https://doi.org/10.5194/acp-23-8369-2023, https://doi.org/10.5194/acp-23-8369-2023, 2023
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Aviation-emitted aerosol can have an impact on cirrus clouds. We present optical and microphysical properties of mid-latitude cirrus clouds which were formed under the influence of aviation-emitted aerosol or which were formed under rather pristine conditions. We find that cirrus clouds affected by aviation-emitted aerosol show larger values of the particle linear depolarization ratio, larger mean effective ice particle diameters and decreased ice particle number concentrations.
Marco Zanatta, Stephan Mertes, Olivier Jourdan, Regis Dupuy, Emma Järvinen, Martin Schnaiter, Oliver Eppers, Johannes Schneider, Zsófia Jurányi, and Andreas Herber
Atmos. Chem. Phys., 23, 7955–7973, https://doi.org/10.5194/acp-23-7955-2023, https://doi.org/10.5194/acp-23-7955-2023, 2023
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Black carbon (BC) particles influence the Arctic radiative balance. Vertical measurements of black carbon were conducted during the ACLOUD campaign in the European Arctic to study the interaction of BC with clouds. This study shows that clouds influence the vertical variability of BC properties across the inversion layer and that multiple activation and transformation mechanisms of BC may occur in the presence of low-level, persistent, mixed-phase clouds.
Emma Järvinen, Franziska Nehlert, Guanglang Xu, Fritz Waitz, Guillaume Mioche, Regis Dupuy, Olivier Jourdan, and Martin Schnaiter
Atmos. Chem. Phys., 23, 7611–7633, https://doi.org/10.5194/acp-23-7611-2023, https://doi.org/10.5194/acp-23-7611-2023, 2023
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The Arctic is warming faster than other regions. Arctic low-level mixed-phase clouds, where ice crystals and liquid droplets co-exist, are thought to have an important role in Arctic warming. Here we show airborne measurements of vertical distribution of liquid and ice particles and their relative abundance. Ice particles are found in relative warm clouds, which can be explained by multiplication of existing ice crystals. However, the role of ice particles in redistributing sun light is minimal.
Manuel Moser, Christiane Voigt, Tina Jurkat-Witschas, Valerian Hahn, Guillaume Mioche, Olivier Jourdan, Régis Dupuy, Christophe Gourbeyre, Alfons Schwarzenboeck, Johannes Lucke, Yvonne Boose, Mario Mech, Stephan Borrmann, André Ehrlich, Andreas Herber, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys., 23, 7257–7280, https://doi.org/10.5194/acp-23-7257-2023, https://doi.org/10.5194/acp-23-7257-2023, 2023
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This study provides a comprehensive microphysical and thermodynamic phase analysis of low-level clouds in the northern Fram Strait, above the sea ice and the open ocean, during spring and summer. Using airborne in situ cloud data, we show that the properties of Arctic low-level clouds vary significantly with seasonal meteorological situations and surface conditions. The observations presented in this study can help one to assess the role of clouds in the Arctic climate system.
Philipp Gregor, Tobias Zinner, Fabian Jakub, and Bernhard Mayer
Atmos. Meas. Tech., 16, 3257–3271, https://doi.org/10.5194/amt-16-3257-2023, https://doi.org/10.5194/amt-16-3257-2023, 2023
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This work introduces MACIN, a model for short-term forecasting of direct irradiance for solar energy applications. MACIN exploits cloud images of multiple cameras to predict irradiance. The model is applied to artificial images of clouds from a weather model. The artificial cloud data allow for a more in-depth evaluation and attribution of errors compared with real data. Good performance of derived cloud information and significant forecast improvements over a baseline forecast were found.
Samira Atabakhsh, Laurent Poulain, Gang Chen, Francesco Canonaco, André S. H. Prévôt, Mira Pöhlker, Alfred Wiedensohler, and Hartmut Herrmann
Atmos. Chem. Phys., 23, 6963–6988, https://doi.org/10.5194/acp-23-6963-2023, https://doi.org/10.5194/acp-23-6963-2023, 2023
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The study focuses on the aerosol chemical variations found in the rural-background station of Melpitz based on ACSM and MAAP measurements. Source apportionment on both organic aerosol (OA) and black carbon (eBC) was performed, and source seasonality was also linked to air mass trajectories. Overall, three anthropogenic sources were identified in OA and eBC plus two additional aged OA. Our results demonstrate the influence of transported coal-combustion-related OA even during summer time.
Sebastian Becker, André Ehrlich, Michael Schäfer, and Manfred Wendisch
Atmos. Chem. Phys., 23, 7015–7031, https://doi.org/10.5194/acp-23-7015-2023, https://doi.org/10.5194/acp-23-7015-2023, 2023
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This study analyses the variability of the warming or cooling effect of clouds on the Arctic surface. Therefore, aircraft radiation measurements were performed over sea ice and open ocean during three seasonally different campaigns. It is found that clouds cool the open-ocean surface most strongly in summer. Over sea ice, clouds warm the surface in spring but have a neutral effect in summer. Due to the variable sea ice extent, clouds warm the surface during spring but cool it during late summer.
Gregor Köcher, Tobias Zinner, and Christoph Knote
Atmos. Chem. Phys., 23, 6255–6269, https://doi.org/10.5194/acp-23-6255-2023, https://doi.org/10.5194/acp-23-6255-2023, 2023
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Polarimetric radar observations of 30 d of convective precipitation events are used to statistically analyze 5 state-of-the-art microphysics schemes of varying complexity. The frequency and area of simulated heavy-precipitation events are in some cases significantly different from those observed, depending on the microphysics scheme. Analysis of simulated particle size distributions and reflectivities shows that some schemes have problems reproducing the correct particle size distributions.
Abdanour Irbah, Julien Delanoë, Gerd-Jan van Zadelhoff, David P. Donovan, Pavlos Kollias, Bernat Puigdomènech Treserras, Shannon Mason, Robin J. Hogan, and Aleksandra Tatarevic
Atmos. Meas. Tech., 16, 2795–2820, https://doi.org/10.5194/amt-16-2795-2023, https://doi.org/10.5194/amt-16-2795-2023, 2023
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The Cloud Profiling Radar (CPR) and ATmospheric LIDar (ATLID) aboard the EarthCARE satellite are used to probe the Earth's atmosphere by measuring cloud and aerosol profiles. ATLID is sensitive to aerosols and small cloud particles and CPR to large ice particles, snowflakes and raindrops. It is the synergy of the measurements of these two instruments that allows a better classification of the atmospheric targets and the description of the associated products, which are the subject of this paper.
Vishnu Nandan, Rosemary Willatt, Robbie Mallett, Julienne Stroeve, Torsten Geldsetzer, Randall Scharien, Rasmus Tonboe, John Yackel, Jack Landy, David Clemens-Sewall, Arttu Jutila, David N. Wagner, Daniela Krampe, Marcus Huntemann, Mallik Mahmud, David Jensen, Thomas Newman, Stefan Hendricks, Gunnar Spreen, Amy Macfarlane, Martin Schneebeli, James Mead, Robert Ricker, Michael Gallagher, Claude Duguay, Ian Raphael, Chris Polashenski, Michel Tsamados, Ilkka Matero, and Mario Hoppmann
The Cryosphere, 17, 2211–2229, https://doi.org/10.5194/tc-17-2211-2023, https://doi.org/10.5194/tc-17-2211-2023, 2023
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We show that wind redistributes snow on Arctic sea ice, and Ka- and Ku-band radar measurements detect both newly deposited snow and buried snow layers that can affect the accuracy of snow depth estimates on sea ice. Radar, laser, meteorological, and snow data were collected during the MOSAiC expedition. With frequent occurrence of storms in the Arctic, our results show that
wind-redistributed snow needs to be accounted for to improve snow depth estimates on sea ice from satellite radars.
Astrid Fremme, Paul J. Hezel, Øyvind Seland, and Harald Sodemann
Weather Clim. Dynam., 4, 449–470, https://doi.org/10.5194/wcd-4-449-2023, https://doi.org/10.5194/wcd-4-449-2023, 2023
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We study the atmospheric moisture transport into eastern China for past, present, and future climate. Hence, we use different climate and weather prediction model data with a moisture source identification method. We find that while the moisture to first order originates mostly from similar regions, smaller changes consistently point to differences in the recycling of precipitation over land between different climates. Some differences are larger between models than between different climates.
Ulrike Egerer, John J. Cassano, Matthew D. Shupe, Gijs de Boer, Dale Lawrence, Abhiram Doddi, Holger Siebert, Gina Jozef, Radiance Calmer, Jonathan Hamilton, Christian Pilz, and Michael Lonardi
Atmos. Meas. Tech., 16, 2297–2317, https://doi.org/10.5194/amt-16-2297-2023, https://doi.org/10.5194/amt-16-2297-2023, 2023
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This paper describes how measurements from a small uncrewed aircraft system can be used to estimate the vertical turbulent heat energy exchange between different layers in the atmosphere. This is particularly important for the atmosphere in the Arctic, as turbulent exchange in this region is often suppressed but is still important to understand how the atmosphere interacts with sea ice. We present three case studies from the MOSAiC field campaign in Arctic sea ice in 2020.
Jan Chylik, Dmitry Chechin, Regis Dupuy, Birte S. Kulla, Christof Lüpkes, Stephan Mertes, Mario Mech, and Roel A. J. Neggers
Atmos. Chem. Phys., 23, 4903–4929, https://doi.org/10.5194/acp-23-4903-2023, https://doi.org/10.5194/acp-23-4903-2023, 2023
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Arctic low-level clouds play an important role in the ongoing warming of the Arctic. Unfortunately, these clouds are not properly represented in weather forecast and climate models. This study tries to cover this gap by focusing on clouds over open water during the spring, observed by research aircraft near Svalbard. The study combines the high-resolution model with sets of observational data. The results show the importance of processes that involve both ice and the liquid water in the clouds.
Steven T. Massie, Heather Cronk, Aronne Merrelli, Sebastian Schmidt, and Steffen Mauceri
Atmos. Meas. Tech., 16, 2145–2166, https://doi.org/10.5194/amt-16-2145-2023, https://doi.org/10.5194/amt-16-2145-2023, 2023
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This paper provides insights into the effects of clouds on Orbiting Carbon Observatory (OCO-2) measurements of CO2. Calculations are carried out that indicate the extent to which this satellite experiment underestimates CO2, due to these cloud effects, as a function of the distance between the surface observation footprint and the nearest cloud. The paper discusses how to lessen the influence of these cloud effects.
Dmitry G. Chechin, Christof Lüpkes, Jörg Hartmann, André Ehrlich, and Manfred Wendisch
Atmos. Chem. Phys., 23, 4685–4707, https://doi.org/10.5194/acp-23-4685-2023, https://doi.org/10.5194/acp-23-4685-2023, 2023
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Clouds represent a very important component of the Arctic climate system, as they strongly reduce the amount of heat lost to space from the sea ice surface. Properties of clouds, as well as their persistence, strongly depend on the complex interaction of such small-scale properties as phase transitions, radiative transfer and turbulence. In this study we use airborne observations to learn more about the effect of clouds and radiative cooling on turbulence in comparison with other factors.
Kevin C. H. Sze, Heike Wex, Markus Hartmann, Henrik Skov, Andreas Massling, Diego Villanueva, and Frank Stratmann
Atmos. Chem. Phys., 23, 4741–4761, https://doi.org/10.5194/acp-23-4741-2023, https://doi.org/10.5194/acp-23-4741-2023, 2023
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Ice-nucleating particles (INPs) play an important role in cloud formation and thus in our climate. But little is known about the abundance and properties of INPs, especially in the Arctic, where the temperature increases almost 4 times as fast as that of the rest of the globe. We observe higher INP concentrations and more biological INPs in summer than in winter, likely from local sources. We also provide three equations for estimating INP concentrations in models at different times of the year.
Armin Blanke, Andrew J. Heymsfield, Manuel Moser, and Silke Trömel
Atmos. Meas. Tech., 16, 2089–2106, https://doi.org/10.5194/amt-16-2089-2023, https://doi.org/10.5194/amt-16-2089-2023, 2023
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We present an evaluation of current retrieval techniques in the ice phase applied to polarimetric radar measurements with collocated in situ observations of aircraft conducted over the Olympic Mountains, Washington State, during winter 2015. Radar estimates of ice properties agreed most with aircraft observations in regions with pronounced radar signatures, but uncertainties were identified that indicate issues of some retrievals, particularly in warmer temperature regimes.
Hong Chen, K. Sebastian Schmidt, Steven T. Massie, Vikas Nataraja, Matthew S. Norgren, Jake J. Gristey, Graham Feingold, Robert E. Holz, and Hironobu Iwabuchi
Atmos. Meas. Tech., 16, 1971–2000, https://doi.org/10.5194/amt-16-1971-2023, https://doi.org/10.5194/amt-16-1971-2023, 2023
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We introduce the Education and Research 3D Radiative Transfer Toolbox (EaR3T) and propose a radiance self-consistency approach for quantifying and mitigating 3D bias in legacy airborne and spaceborne imagery retrievals due to spatially inhomogeneous clouds and surfaces.
Samuel Kwakye, Heike Kalesse-Los, Maximilian Maahn, Patric Seifert, Roel van Klink, Christian Wirth, and Johannes Quaas
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-69, https://doi.org/10.5194/amt-2023-69, 2023
Publication in AMT not foreseen
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Insect numbers in the atmosphere can be calculated using polarimetric weather radar but they have to be identified and separated from other echoes, especially weather phenomena. Here, the separation is demonstrated using three machine-learning algorithms and insect count data from suction traps and the nature of radar measurements of different radar echoes is revealed. Random forest is the best separating algorithm and insect echoes radar measurements are distinct.
Felix Pithan, Marylou Athanase, Sandro Dahlke, Antonio Sánchez-Benítez, Matthew D. Shupe, Anne Sledd, Jan Streffing, Gunilla Svensson, and Thomas Jung
Geosci. Model Dev., 16, 1857–1873, https://doi.org/10.5194/gmd-16-1857-2023, https://doi.org/10.5194/gmd-16-1857-2023, 2023
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Evaluating climate models usually requires long observational time series, but we present a method that also works for short field campaigns. We compare climate model output to observations from the MOSAiC expedition in the central Arctic Ocean. All models show how the arrival of a warm air mass warms the Arctic in April 2020, but two models do not show the response of snow temperature to the diurnal cycle. One model has too little liquid water and too much ice in clouds during cold days.
Heike Kalesse-Los, Anton Kötsche, Andreas Foth, Johannes Röttenbacher, Teresa Vogl, and Jonas Witthuhn
Atmos. Meas. Tech., 16, 1683–1704, https://doi.org/10.5194/amt-16-1683-2023, https://doi.org/10.5194/amt-16-1683-2023, 2023
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The Virga-Sniffer, a new modular open-source Python package tool to characterize full precipitation evaporation (so-called virga) from ceilometer cloud base height and vertically pointing cloud radar reflectivity time–height fields, is described. Results of its first application to RV Meteor observations during the EUREC4A field experiment in January–February 2020 are shown. About half of all detected clouds with bases below the trade inversion height were found to produce virga.
André Ehrlich, Martin Zöger, Andreas Giez, Vladyslav Nenakhov, Christian Mallaun, Rolf Maser, Timo Röschenthaler, Anna E. Luebke, Kevin Wolf, Bjorn Stevens, and Manfred Wendisch
Atmos. Meas. Tech., 16, 1563–1581, https://doi.org/10.5194/amt-16-1563-2023, https://doi.org/10.5194/amt-16-1563-2023, 2023
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Measurements of the broadband radiative energy budget from aircraft are needed to study the effect of clouds, aerosol particles, and surface conditions on the Earth's energy budget. However, the moving aircraft introduces challenges to the instrument performance and post-processing of the data. This study introduces a new radiometer package, outlines a greatly simplifying method to correct thermal offsets, and provides exemplary measurements of solar and thermal–infrared irradiance.
Steffen Mauceri, Steven Massie, and Sebastian Schmidt
Atmos. Meas. Tech., 16, 1461–1476, https://doi.org/10.5194/amt-16-1461-2023, https://doi.org/10.5194/amt-16-1461-2023, 2023
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The Orbiting Carbon Observatory-2 makes space-based measurements of reflected sunlight. Using a retrieval algorithm these measurements are converted to CO2 concentrations in the atmosphere. However, the converted CO2 concentrations contain errors for observations close to clouds. Using a simple machine learning approach, we developed a model to correct these remaining errors. The model is able to reduce errors over land and ocean by 20 % and 40 %, respectively.
Wenkai Guo, Polona Itkin, Suman Singha, Anthony P. Doulgeris, Malin Johansson, and Gunnar Spreen
The Cryosphere, 17, 1279–1297, https://doi.org/10.5194/tc-17-1279-2023, https://doi.org/10.5194/tc-17-1279-2023, 2023
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Sea ice maps are produced to cover the MOSAiC Arctic expedition (2019–2020) and divide sea ice into scientifically meaningful classes. We use a high-resolution X-band synthetic aperture radar dataset and show how image brightness and texture systematically vary across the images. We use an algorithm that reliably corrects this effect and achieve good results, as evaluated by comparisons to ground observations and other studies. The sea ice maps are useful as a basis for future MOSAiC studies.
Julia Pikmann, Lasse Moormann, Frank Drewnick, and Stephan Borrmann
Atmos. Meas. Tech., 16, 1323–1341, https://doi.org/10.5194/amt-16-1323-2023, https://doi.org/10.5194/amt-16-1323-2023, 2023
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Aerosols measured in complex environments are usually a mixture of emissions from different sources. To characterize sources individually, we developed a sampling system for particles and organic trace gases which is coupled to real-time data of physical and chemical aerosol properties, gas concentrations, and meteorological variables. Using suitable sampling conditions for individual aerosols which are compared with the real-time data the desired aerosols are sampled separately from each other.
Pragya Vishwakarma, Julien Delanoë, Susana Jorquera, Pauline Martinet, Frederic Burnet, Alistair Bell, and Jean-Charles Dupont
Atmos. Meas. Tech., 16, 1211–1237, https://doi.org/10.5194/amt-16-1211-2023, https://doi.org/10.5194/amt-16-1211-2023, 2023
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Cloud observations are necessary to characterize the cloud properties at local and global scales. The observations must be translated to cloud geophysical parameters. This paper presents the estimation of liquid water content (LWC) using radar and microwave radiometer (MWR) measurements. Liquid water path from MWR scales LWC and retrieves the scaling factor (ln a). The retrievals are compared with in situ observations. A climatology of ln a is built to estimate LWC using only radar information.
Georgios Dekoutsidis, Silke Groß, Martin Wirth, Martina Krämer, and Christian Rolf
Atmos. Chem. Phys., 23, 3103–3117, https://doi.org/10.5194/acp-23-3103-2023, https://doi.org/10.5194/acp-23-3103-2023, 2023
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Cirrus clouds affect Earth's atmosphere, deeming our study important. Here we use water vapor measurements by lidar and study the relative humidity (RHi) within and around midlatitude cirrus clouds. We find high supersaturations in the cloud-free air and within the clouds, especially near the cloud top. We study two cloud types with different formation processes. Finally, we conclude that the shape of the distribution of RHi can be used as an indicator of different cloud evolutionary stages.
Dominik Brunner, Gerrit Kuhlmann, Stephan Henne, Erik Koene, Bastian Kern, Sebastian Wolff, Christiane Voigt, Patrick Jöckel, Christoph Kiemle, Anke Roiger, Alina Fiehn, Sven Krautwurst, Konstantin Gerilowski, Heinrich Bovensmann, Jakob Borchardt, Michal Galkowski, Christoph Gerbig, Julia Marshall, Andrzej Klonecki, Pascal Prunet, Robert Hanfland, Margit Pattantyús-Ábrahám, Andrzej Wyszogrodzki, and Andreas Fix
Atmos. Chem. Phys., 23, 2699–2728, https://doi.org/10.5194/acp-23-2699-2023, https://doi.org/10.5194/acp-23-2699-2023, 2023
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We evaluated six atmospheric transport models for their capability to simulate the CO2 plumes from two of the largest power plants in Europe by comparing the models against aircraft observations collected during the CoMet (Carbon Dioxide and Methane Mission) campaign in 2018. The study analyzed how realistically such plumes can be simulated at different model resolutions and how well the planned European satellite mission CO2M will be able to quantify emissions from power plants.
Chuan-Yao Lin, Wan-Chin Chen, Yi-Yun Chien, Charles C. K. Chou, Chian-Yi Liu, Helmut Ziereis, Hans Schlager, Eric Förster, Florian Obersteiner, Ovid O. Krüger, Bruna A. Holanda, Mira L. Pöhlker, Katharina Kaiser, Johannes Schneider, Birger Bohn, Klaus Pfeilsticker, Benjamin Weyland, Maria Dolores Andrés Hernández, and John P. Burrows
Atmos. Chem. Phys., 23, 2627–2647, https://doi.org/10.5194/acp-23-2627-2023, https://doi.org/10.5194/acp-23-2627-2023, 2023
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During the EMeRGe campaign in Asia, atmospheric pollutants were measured on board the HALO aircraft. The WRF-Chem model was employed to evaluate the biomass burning (BB) plume transported from Indochina and its impact on the downstream areas. The combination of BB aerosol enhancement with cloud water resulted in a reduction in incoming shortwave radiation at the surface in southern China and the East China Sea, which potentially has significant regional climate implications.
Yun Li, Christoph Mahnke, Susanne Rohs, Ulrich Bundke, Nicole Spelten, Georgios Dekoutsidis, Silke Groß, Christiane Voigt, Ulrich Schumann, Andreas Petzold, and Martina Krämer
Atmos. Chem. Phys., 23, 2251–2271, https://doi.org/10.5194/acp-23-2251-2023, https://doi.org/10.5194/acp-23-2251-2023, 2023
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The radiative effect of aviation-induced cirrus is closely related to ambient conditions and its microphysical properties. Our study investigated the occurrence of contrail and natural cirrus measured above central Europe in spring 2014. It finds that contrail cirrus appears frequently in the pressure range 200 to 245 hPa and occurs more often in slightly ice-subsaturated environments than expected. Avoiding slightly ice-subsaturated regions by aviation might help mitigate contrail cirrus.
Andrew W. Seidl, Harald Sodemann, and Hans Christian Steen-Larsen
Atmos. Meas. Tech., 16, 769–790, https://doi.org/10.5194/amt-16-769-2023, https://doi.org/10.5194/amt-16-769-2023, 2023
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It is challenging to make field measurements of stable water isotopes in the Arctic. To this end, we present a modular stable-water-isotope analyzer profiling system. The system operated for a 2-week field campaign on Svalbard during the Arctic winter. We evaluate the system’s performance and analyze any potential impact that the field conditions might have had on the isotopic measurements and the system's ability to resolve isotope gradients in the lowermost layer of the atmosphere.
Ziming Wang, Luca Bugliaro, Tina Jurkat-Witschas, Romy Heller, Ulrike Burkhardt, Helmut Ziereis, Georgios Dekoutsidis, Martin Wirth, Silke Groß, Simon Kirschler, Stefan Kaufmann, and Christiane Voigt
Atmos. Chem. Phys., 23, 1941–1961, https://doi.org/10.5194/acp-23-1941-2023, https://doi.org/10.5194/acp-23-1941-2023, 2023
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Differences in the microphysical properties of contrail cirrus and natural cirrus in a contrail outbreak situation during the ML-CIRRUS campaign over the North Atlantic flight corridor can be observed from in situ measurements. The cirrus radiative effect in the area of the outbreak, derived from satellite observation-based radiative transfer modeling, is warming in the early morning and cooling during the day.
Veronika Pörtge, Tobias Kölling, Anna Weber, Lea Volkmer, Claudia Emde, Tobias Zinner, Linda Forster, and Bernhard Mayer
Atmos. Meas. Tech., 16, 645–667, https://doi.org/10.5194/amt-16-645-2023, https://doi.org/10.5194/amt-16-645-2023, 2023
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In this work, we analyze polarized cloudbow observations by the airborne camera system specMACS to retrieve the cloud droplet size distribution defined by the effective radius (reff) and the effective variance (veff). Two case studies of trade-wind cumulus clouds observed during the EUREC4A field campaign are presented. The results are combined into maps of reff and veff with a very high spatial resolution (100 m × 100 m) that allow new insights into cloud microphysics.
Adriana Bailey, Franziska Aemisegger, Leonie Villiger, Sebastian A. Los, Gilles Reverdin, Estefanía Quiñones Meléndez, Claudia Acquistapace, Dariusz B. Baranowski, Tobias Böck, Sandrine Bony, Tobias Bordsdorff, Derek Coffman, Simon P. de Szoeke, Christopher J. Diekmann, Marina Dütsch, Benjamin Ertl, Joseph Galewsky, Dean Henze, Przemyslaw Makuch, David Noone, Patricia K. Quinn, Michael Rösch, Andreas Schneider, Matthias Schneider, Sabrina Speich, Bjorn Stevens, and Elizabeth J. Thompson
Earth Syst. Sci. Data, 15, 465–495, https://doi.org/10.5194/essd-15-465-2023, https://doi.org/10.5194/essd-15-465-2023, 2023
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One of the novel ways EUREC4A set out to investigate trade wind clouds and their coupling to the large-scale circulation was through an extensive network of isotopic measurements in water vapor, precipitation, and seawater. Samples were taken from the island of Barbados, from aboard two aircraft, and from aboard four ships. This paper describes the full collection of EUREC4A isotopic in situ data and guides readers to complementary remotely sensed water vapor isotope ratios.
Cathy Hohenegger, Peter Korn, Leonidas Linardakis, René Redler, Reiner Schnur, Panagiotis Adamidis, Jiawei Bao, Swantje Bastin, Milad Behravesh, Martin Bergemann, Joachim Biercamp, Hendryk Bockelmann, Renate Brokopf, Nils Brüggemann, Lucas Casaroli, Fatemeh Chegini, George Datseris, Monika Esch, Geet George, Marco Giorgetta, Oliver Gutjahr, Helmuth Haak, Moritz Hanke, Tatiana Ilyina, Thomas Jahns, Johann Jungclaus, Marcel Kern, Daniel Klocke, Lukas Kluft, Tobias Kölling, Luis Kornblueh, Sergey Kosukhin, Clarissa Kroll, Junhong Lee, Thorsten Mauritsen, Carolin Mehlmann, Theresa Mieslinger, Ann Kristin Naumann, Laura Paccini, Angel Peinado, Divya Sri Praturi, Dian Putrasahan, Sebastian Rast, Thomas Riddick, Niklas Roeber, Hauke Schmidt, Uwe Schulzweida, Florian Schütte, Hans Segura, Radomyra Shevchenko, Vikram Singh, Mia Specht, Claudia Christine Stephan, Jin-Song von Storch, Raphaela Vogel, Christian Wengel, Marius Winkler, Florian Ziemen, Jochem Marotzke, and Bjorn Stevens
Geosci. Model Dev., 16, 779–811, https://doi.org/10.5194/gmd-16-779-2023, https://doi.org/10.5194/gmd-16-779-2023, 2023
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Models of the Earth system used to understand climate and predict its change typically employ a grid spacing of about 100 km. Yet, many atmospheric and oceanic processes occur on much smaller scales. In this study, we present a new model configuration designed for the simulation of the components of the Earth system and their interactions at kilometer and smaller scales, allowing an explicit representation of the main drivers of the flow of energy and matter by solving the underlying equations.
Haley M. Royer, Mira L. Pöhlker, Ovid Krüger, Edmund Blades, Peter Sealy, Nurun Nahar Lata, Zezhen Cheng, Swarup China, Andrew P. Ault, Patricia K. Quinn, Paquita Zuidema, Christopher Pöhlker, Ulrich Pöschl, Meinrat Andreae, and Cassandra J. Gaston
Atmos. Chem. Phys., 23, 981–998, https://doi.org/10.5194/acp-23-981-2023, https://doi.org/10.5194/acp-23-981-2023, 2023
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This paper presents atmospheric particle chemical composition and measurements of aerosol water uptake properties collected at Ragged Point, Barbados, during the winter of 2020. The result of this study indicates the importance of small African smoke particles for cloud droplet formation in the tropical North Atlantic and highlights the large spatial and temporal pervasiveness of smoke over the Atlantic Ocean.
Andreas Schäfler, Michael Sprenger, Heini Wernli, Andreas Fix, and Martin Wirth
Atmos. Chem. Phys., 23, 999–1018, https://doi.org/10.5194/acp-23-999-2023, https://doi.org/10.5194/acp-23-999-2023, 2023
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In this study, airborne lidar profile measurements of H2O and O3 across a midlatitude jet stream are combined with analyses in tracer–trace space and backward trajectories. We highlight that transport and mixing processes in the history of the observed air masses are governed by interacting tropospheric weather systems on synoptic timescales. We show that these weather systems play a key role in the high variability of the paired H2O and O3 distributions near the tropopause.
Behrooz Keshtgar, Aiko Voigt, Corinna Hoose, Michael Riemer, and Bernhard Mayer
Weather Clim. Dynam., 4, 115–132, https://doi.org/10.5194/wcd-4-115-2023, https://doi.org/10.5194/wcd-4-115-2023, 2023
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Forecasting extratropical cyclones is challenging due to many physical factors influencing their behavior. One such factor is the impact of heating and cooling of the atmosphere by the interaction between clouds and radiation. In this study, we show that cloud-radiative heating (CRH) increases the intensity of an idealized cyclone and affects its predictability. We find that CRH affects the cyclone mostly via increasing latent heat release and subsequent changes in the synoptic circulation.
Andreas Marsing, Ralf Meerkötter, Romy Heller, Stefan Kaufmann, Tina Jurkat-Witschas, Martina Krämer, Christian Rolf, and Christiane Voigt
Atmos. Chem. Phys., 23, 587–609, https://doi.org/10.5194/acp-23-587-2023, https://doi.org/10.5194/acp-23-587-2023, 2023
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We employ highly resolved aircraft measurements of profiles of the ice water content (IWC) in Arctic cirrus clouds in winter and spring, when solar irradiation is low. Using radiation transfer calculations, we assess the cloud radiative effect over different surfaces like snow or ocean. The variability in the IWC of the clouds affects their overall radiative effect and drives internal processes. This helps understand the role of cirrus in a rapidly changing Arctic environment.
Yunfan Liu, Hang Su, Siwen Wang, Chao Wei, Wei Tao, Mira L. Pöhlker, Christopher Pöhlker, Bruna A. Holanda, Ovid O. Krüger, Thorsten Hoffmann, Manfred Wendisch, Paulo Artaxo, Ulrich Pöschl, Meinrat O. Andreae, and Yafang Cheng
Atmos. Chem. Phys., 23, 251–272, https://doi.org/10.5194/acp-23-251-2023, https://doi.org/10.5194/acp-23-251-2023, 2023
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The origins of the abundant cloud condensation nuclei (CCN) in the upper troposphere (UT) of the Amazon remain unclear. With model developments of new secondary organic aerosol schemes and constrained by observation, we show that strong aerosol nucleation and condensation in the UT is triggered by biogenic organics, and organic condensation is key for UT CCN production. This UT CCN-producing mechanism may prevail over broader vegetation canopies and deserves emphasis in aerosol–climate feedback.
Christian Melsheimer, Gunnar Spreen, Yufang Ye, and Mohammed Shokr
The Cryosphere, 17, 105–126, https://doi.org/10.5194/tc-17-105-2023, https://doi.org/10.5194/tc-17-105-2023, 2023
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It is necessary to know the type of Antarctic sea ice present – first-year ice (grown in one season) or multiyear ice (survived one summer melt) – to understand and model its evolution, as the ice types behave and react differently. We have adapted and extended an existing method (originally for the Arctic), and now, for the first time, daily maps of Antarctic sea ice types can be derived from microwave satellite data. This will allow a new data set from 2002 well into the future to be built.
Lejiang Yu, Shiyuan Zhong, Timo Vihma, Cuijuan Sui, and Bo Sun
Atmos. Chem. Phys., 23, 345–353, https://doi.org/10.5194/acp-23-345-2023, https://doi.org/10.5194/acp-23-345-2023, 2023
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Previous studies have noted a significant relationship between the Subtropical Indian Ocean Dipole and the South Atlantic Ocean Dipole indices, but little is known about the stability of their relationship. We found a significant positive correlation between the two indices prior to the year 2000 but an insignificant correlation afterwards.
Johannes Lucke, Tina Jurkat-Witschas, Romy Heller, Valerian Hahn, Matthew Hamman, Wolfgang Breitfuss, Venkateshwar Reddy Bora, Manuel Moser, and Christiane Voigt
Atmos. Meas. Tech., 15, 7375–7394, https://doi.org/10.5194/amt-15-7375-2022, https://doi.org/10.5194/amt-15-7375-2022, 2022
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Flight testing in icing conditions requires instruments that are able to accurately measure the liquid water content of supercooled large droplets (SLDs). This work finds that the 12 mm cone of the Nevzorov hot-wire probe has excellent collection properties for SLDs. We also derive a correction to compensate for the low collision efficiency of small droplets with the cone. The results provide a procedure to evaluate LWC measurements of the 12 mm cone during wind tunnel and airborne experiments.
Qiang Li and Silke Groß
Atmos. Chem. Phys., 22, 15963–15980, https://doi.org/10.5194/acp-22-15963-2022, https://doi.org/10.5194/acp-22-15963-2022, 2022
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The IPCC report identified that cirrus clouds have a significant impact on the radiation balance comparable to the CO2 effects, which, however, is still hard to parameterize. The current study investigates the possible impact of aviation on cirrus properties based on the analysis of 10-year lidar measurements of CALIPSO. The results reveal that there is a significant positive trend in cirrus depolarization ratio in the last 10 years before COVID-19, which is strongly correlated with aviation.
Yuan Wang, Silvia Henning, Laurent Poulain, Chunsong Lu, Frank Stratmann, Yuying Wang, Shengjie Niu, Mira L. Pöhlker, Hartmut Herrmann, and Alfred Wiedensohler
Atmos. Chem. Phys., 22, 15943–15962, https://doi.org/10.5194/acp-22-15943-2022, https://doi.org/10.5194/acp-22-15943-2022, 2022
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Aerosol particle activation affects cloud, precipitation, radiation, and thus the global climate. Its long-term measurements are important but still scarce. In this study, more than 4 years of measurements at a central European station were analyzed. The overall characteristics and seasonal changes of aerosol particle activation are summarized. The power-law fit between particle hygroscopicity factor and diameter was recommended for predicting cloud
condensation nuclei number concentration.
Julie Thérèse Pasquier, Jan Henneberger, Fabiola Ramelli, Annika Lauber, Robert Oscar David, Jörg Wieder, Tim Carlsen, Rosa Gierens, Marion Maturilli, and Ulrike Lohmann
Atmos. Chem. Phys., 22, 15579–15601, https://doi.org/10.5194/acp-22-15579-2022, https://doi.org/10.5194/acp-22-15579-2022, 2022
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It is important to understand how ice crystals and cloud droplets form in clouds, as their concentrations and sizes determine the exact radiative properties of the clouds. Normally, ice crystals form from aerosols, but we found evidence for the formation of additional ice crystals from the original ones over a large temperature range within Arctic clouds. In particular, additional ice crystals were formed during collisions of several ice crystals or during the freezing of large cloud droplets.
Konstantin Krüger, Andreas Schäfler, Martin Wirth, Martin Weissmann, and George C. Craig
Atmos. Chem. Phys., 22, 15559–15577, https://doi.org/10.5194/acp-22-15559-2022, https://doi.org/10.5194/acp-22-15559-2022, 2022
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A comprehensive data set of airborne lidar water vapour profiles is compared with ERA5 reanalyses for a robust characterization of the vertical structure of the mid-latitude lower-stratospheric moist bias. We confirm a moist bias of up to 55 % at 1.3 km altitude above the tropopause and uncover a decreasing bias beyond. Collocated O3 and H2O observations reveal a particularly strong bias in the mixing layer, indicating insufficiently modelled transport processes fostering the bias.
Baseerat Romshoo, Mira Pöhlker, Alfred Wiedensohler, Sascha Pfeifer, Jorge Saturno, Andreas Nowak, Krzysztof Ciupek, Paul Quincey, Konstantina Vasilatou, Michaela N. Ess, Maria Gini, Konstantinos Eleftheriadis, Chris Robins, François Gaie-Levrel, and Thomas Müller
Atmos. Meas. Tech., 15, 6965–6989, https://doi.org/10.5194/amt-15-6965-2022, https://doi.org/10.5194/amt-15-6965-2022, 2022
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Black carbon (BC) is often assumed to be spherically shaped, causing uncertainties in its optical properties when modelled. This study investigates different modelling techniques for the optical properties of BC by comparing them to laboratory measurements. We provide experimental support for emphasizing the use of appropriate size representation (polydisperse size method) and morphological representation (aggregate morphology) for optical modelling and parameterization scheme development of BC.
Christian Pilz, Sebastian Düsing, Birgit Wehner, Thomas Müller, Holger Siebert, Jens Voigtländer, and Michael Lonardi
Atmos. Meas. Tech., 15, 6889–6905, https://doi.org/10.5194/amt-15-6889-2022, https://doi.org/10.5194/amt-15-6889-2022, 2022
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Tethered balloon observations are highly valuable for aerosol studies in the lowest part of the atmosphere. This study presents a newly developed platform called CAMP with four aerosol instruments for balloon-borne measurements in the Arctic. Laboratory characterizations and evaluations of the instruments and results of a first field deployment are shown. A case study highlights CAMP's capabilities and the importance of airborne aerosol studies for interpretation of ground-based observations.
Linda Forster and Bernhard Mayer
Atmos. Chem. Phys., 22, 15179–15205, https://doi.org/10.5194/acp-22-15179-2022, https://doi.org/10.5194/acp-22-15179-2022, 2022
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We present a novel retrieval using ground-based imaging observations of halo displays together with radiative transfer simulations to help improve our understanding of ice crystal properties representative of cirrus clouds. Analysis of 4400 calibrated HaloCam images featuring a 22° halo revealed aggregates of hexagonal columns of 20 µm effective radius with a mixture of about 37 % smooth and 63% severely roughened surfaces as the best match in general.
Laura Tomsche, Andreas Marsing, Tina Jurkat-Witschas, Johannes Lucke, Stefan Kaufmann, Katharina Kaiser, Johannes Schneider, Monika Scheibe, Hans Schlager, Lenard Röder, Horst Fischer, Florian Obersteiner, Andreas Zahn, Martin Zöger, Jos Lelieveld, and Christiane Voigt
Atmos. Chem. Phys., 22, 15135–15151, https://doi.org/10.5194/acp-22-15135-2022, https://doi.org/10.5194/acp-22-15135-2022, 2022
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The detection of sulfur compounds in the upper troposphere (UT) and lower stratosphere (LS) is a challenge. In-flight measurements of SO2 and sulfate aerosol were performed during the BLUESKY mission in spring 2020 under exceptional atmospheric conditions. Reduced sinks in the dry UTLS and lower but still significant air traffic influenced the enhanced SO2 in the UT, and aged volcanic plumes enhanced the LS sulfate aerosol impacting the atmospheric radiation budget and global climate.
Paul A. Barrett, Steven J. Abel, Hugh Coe, Ian Crawford, Amie Dobracki, James Haywood, Steve Howell, Anthony Jones, Justin Langridge, Greg M. McFarquhar, Graeme J. Nott, Hannah Price, Jens Redemann, Yohei Shinozuka, Kate Szpek, Jonathan W. Taylor, Robert Wood, Huihui Wu, Paquita Zuidema, Stéphane Bauguitte, Ryan Bennett, Keith Bower, Hong Chen, Sabrina Cochrane, Michael Cotterell, Nicholas Davies, David Delene, Connor Flynn, Andrew Freedman, Steffen Freitag, Siddhant Gupta, David Noone, Timothy B. Onasch, James Podolske, Michael R. Poellot, Sebastian Schmidt, Stephen Springston, Arthur J. Sedlacek III, Jamie Trembath, Alan Vance, Maria A. Zawadowicz, and Jianhao Zhang
Atmos. Meas. Tech., 15, 6329–6371, https://doi.org/10.5194/amt-15-6329-2022, https://doi.org/10.5194/amt-15-6329-2022, 2022
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To better understand weather and climate, it is vital to go into the field and collect observations. Often measurements take place in isolation, but here we compared data from two aircraft and one ground-based site. This was done in order to understand how well measurements made on one platform compared to those made on another. Whilst this is easy to do in a controlled laboratory setting, it is more challenging in the real world, and so these comparisons are as valuable as they are rare.
Hossein Dadashazar, Andrea F. Corral, Ewan Crosbie, Sanja Dmitrovic, Simon Kirschler, Kayla McCauley, Richard Moore, Claire Robinson, Joseph S. Schlosser, Michael Shook, K. Lee Thornhill, Christiane Voigt, Edward Winstead, Luke Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 22, 13897–13913, https://doi.org/10.5194/acp-22-13897-2022, https://doi.org/10.5194/acp-22-13897-2022, 2022
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Multi-season airborne data over the northwestern Atlantic show that organic mass fraction and the relative amount of oxygenated organics within that fraction are enhanced in droplet residual particles as compared to particles below and above cloud. In-cloud aqueous processing is shown to be a potential driver of this compositional shift in cloud. This implies that aerosol–cloud interactions in the region reduce aerosol hygroscopicity due to the jump in the organic : sulfate ratio in cloud.
Oliver Appel, Franziska Köllner, Antonis Dragoneas, Andreas Hünig, Sergej Molleker, Hans Schlager, Christoph Mahnke, Ralf Weigel, Max Port, Christiane Schulz, Frank Drewnick, Bärbel Vogel, Fred Stroh, and Stephan Borrmann
Atmos. Chem. Phys., 22, 13607–13630, https://doi.org/10.5194/acp-22-13607-2022, https://doi.org/10.5194/acp-22-13607-2022, 2022
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This paper clarifies the chemical composition of the Asian tropopause aerosol layer (ATAL) by means of airborne in situ aerosol mass spectrometry (AMS). Ammonium nitrate and organics are found to significantly contribute to the particle layer, while sulfate does not show a layered structure. An analysis of the single-particle mass spectra suggests that secondary particle formation and subsequent growth dominate the particle composition, rather than condensation on pre-existing primary particles.
Huan Yu, Claudia Emde, Arve Kylling, Ben Veihelmann, Bernhard Mayer, Kerstin Stebel, and Michel Van Roozendael
Atmos. Meas. Tech., 15, 5743–5768, https://doi.org/10.5194/amt-15-5743-2022, https://doi.org/10.5194/amt-15-5743-2022, 2022
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In this study, we have investigated the impact of 3D clouds on the tropospheric NO2 retrieval from UV–visible sensors. We applied standard NO2 retrieval methods including cloud corrections to synthetic data generated by the 3D radiative transfer model. A sensitivity study was done for synthetic data, and dependencies on various parameters were investigated. Possible mitigation strategies were investigated and compared based on 3D simulations and observed data.
Antonis Dragoneas, Sergej Molleker, Oliver Appel, Andreas Hünig, Thomas Böttger, Markus Hermann, Frank Drewnick, Johannes Schneider, Ralf Weigel, and Stephan Borrmann
Atmos. Meas. Tech., 15, 5719–5742, https://doi.org/10.5194/amt-15-5719-2022, https://doi.org/10.5194/amt-15-5719-2022, 2022
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The ERICA is a specially designed aerosol particle mass spectrometer for in situ, real-time chemical composition analysis of aerosols. It can operate completely autonomously, in the absence of an instrument operator. Its design has enabled its operation under harsh conditions, like those experienced in the upper troposphere and lower stratosphere, aboard unpressurized high-altitude research aircraft. The instrument has successfully participated in several aircraft operations around the world.
Julienne Stroeve, Vishnu Nandan, Rosemary Willatt, Ruzica Dadic, Philip Rostosky, Michael Gallagher, Robbie Mallett, Andrew Barrett, Stefan Hendricks, Rasmus Tonboe, Michelle McCrystall, Mark Serreze, Linda Thielke, Gunnar Spreen, Thomas Newman, John Yackel, Robert Ricker, Michel Tsamados, Amy Macfarlane, Henna-Reetta Hannula, and Martin Schneebeli
The Cryosphere, 16, 4223–4250, https://doi.org/10.5194/tc-16-4223-2022, https://doi.org/10.5194/tc-16-4223-2022, 2022
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Impacts of rain on snow (ROS) on satellite-retrieved sea ice variables remain to be fully understood. This study evaluates the impacts of ROS over sea ice on active and passive microwave data collected during the 2019–20 MOSAiC expedition. Rainfall and subsequent refreezing of the snowpack significantly altered emitted and backscattered radar energy, laying important groundwork for understanding their impacts on operational satellite retrievals of various sea ice geophysical variables.
Alessandro Carlo Maria Savazzi, Louise Nuijens, Irina Sandu, Geet George, and Peter Bechtold
Atmos. Chem. Phys., 22, 13049–13066, https://doi.org/10.5194/acp-22-13049-2022, https://doi.org/10.5194/acp-22-13049-2022, 2022
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Winds are of great importance for the transport of energy and moisture in the atmosphere. In this study we use measurements from the EUREC4A field campaign and several model experiments to understand the wind bias in the forecasts produced by the European Centre for Medium-Range Weather Forecasts. We are able to link the model errors to heights above 2 km and to the representation of the diurnal cycle of winds: the model makes the winds too slow in the morning and too strong in the evening.
Alistair Bell, Pauline Martinet, Olivier Caumont, Frédéric Burnet, Julien Delanoë, Susana Jorquera, Yann Seity, and Vinciane Unger
Atmos. Meas. Tech., 15, 5415–5438, https://doi.org/10.5194/amt-15-5415-2022, https://doi.org/10.5194/amt-15-5415-2022, 2022
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Cloud radars and microwave radiometers offer the potential to improve fog forecasts when assimilated into a high-resolution model. As this process can be complex, a retrieval of model variables is sometimes made as a first step. In this work, results from a 1D-Var algorithm for the retrieval of temperature, humidity and cloud liquid water content are presented. The algorithm is applied first to a synthetic dataset and then to a dataset of real measurements from a recent field campaign.
Willi Schimmel, Heike Kalesse-Los, Maximilian Maahn, Teresa Vogl, Andreas Foth, Pablo Saavedra Garfias, and Patric Seifert
Atmos. Meas. Tech., 15, 5343–5366, https://doi.org/10.5194/amt-15-5343-2022, https://doi.org/10.5194/amt-15-5343-2022, 2022
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This study introduces the novel Doppler radar spectra-based machine learning approach VOODOO (reVealing supercOOled liquiD beyOnd lidar attenuatiOn). VOODOO is a powerful probability-based extension to the existing Cloudnet hydrometeor target classification, enabling the detection of liquid-bearing cloud layers beyond complete lidar attenuation via user-defined p* threshold. VOODOO performs best for (multi-layer) stratiform and deep mixed-phase clouds with liquid water path > 100 g m−2.
Marco A. Giorgetta, William Sawyer, Xavier Lapillonne, Panagiotis Adamidis, Dmitry Alexeev, Valentin Clément, Remo Dietlicher, Jan Frederik Engels, Monika Esch, Henning Franke, Claudia Frauen, Walter M. Hannah, Benjamin R. Hillman, Luis Kornblueh, Philippe Marti, Matthew R. Norman, Robert Pincus, Sebastian Rast, Daniel Reinert, Reiner Schnur, Uwe Schulzweida, and Bjorn Stevens
Geosci. Model Dev., 15, 6985–7016, https://doi.org/10.5194/gmd-15-6985-2022, https://doi.org/10.5194/gmd-15-6985-2022, 2022
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This work presents a first version of the ICON atmosphere model that works not only on CPUs, but also on GPUs. This GPU-enabled ICON version is benchmarked on two GPU machines and a CPU machine. While the weak scaling is very good on CPUs and GPUs, the strong scaling is poor on GPUs. But the high performance of GPU machines allowed for first simulations of a short period of the quasi-biennial oscillation at very high resolution with explicit convection and gravity wave forcing.
Vikas Nataraja, Sebastian Schmidt, Hong Chen, Takanobu Yamaguchi, Jan Kazil, Graham Feingold, Kevin Wolf, and Hironobu Iwabuchi
Atmos. Meas. Tech., 15, 5181–5205, https://doi.org/10.5194/amt-15-5181-2022, https://doi.org/10.5194/amt-15-5181-2022, 2022
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A convolutional neural network (CNN) is introduced to retrieve cloud optical thickness (COT) from passive cloud imagery. The CNN, trained on large eddy simulations from the Sulu Sea, learns from spatial information at multiple scales to reduce cloud inhomogeneity effects. By considering the spatial context of a pixel, the CNN outperforms the traditional independent pixel approximation (IPA) across several cloud morphology metrics.
Marcel Zauner-Wieczorek, Martin Heinritzi, Manuel Granzin, Timo Keber, Andreas Kürten, Katharina Kaiser, Johannes Schneider, and Joachim Curtius
Atmos. Chem. Phys., 22, 11781–11794, https://doi.org/10.5194/acp-22-11781-2022, https://doi.org/10.5194/acp-22-11781-2022, 2022
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We present measurements of ambient ions in the free troposphere and lower stratosphere over Europe in spring 2020. We observed nitrate and hydrogen sulfate, amongst others. From their ratio, the number concentrations of gaseous sulfuric acid were inferred. Nitrate increased towards the stratosphere, whilst sulfuric acid was slightly decreased there. The average values for sulfuric acid were 1.9 to 7.8 × 105 cm-3. Protonated pyridine was identified in an altitude range of 4.6 to 8.5 km.
Leonie von Terzi, José Dias Neto, Davide Ori, Alexander Myagkov, and Stefan Kneifel
Atmos. Chem. Phys., 22, 11795–11821, https://doi.org/10.5194/acp-22-11795-2022, https://doi.org/10.5194/acp-22-11795-2022, 2022
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We present a statistical analysis of ice microphysical processes (IMP) in mid-latitude clouds. Combining various radar approaches, we find that the IMP active at −20 to −10 °C seems to be the main driver of ice particle size, shape and concentration. The strength of aggregation at −20 to −10 °C correlates with the increase in concentration and aspect ratio of locally formed ice particles. Despite ongoing aggregation, the concentration of ice particles stays enhanced until −4 °C.
Roger Teoh, Ulrich Schumann, Edward Gryspeerdt, Marc Shapiro, Jarlath Molloy, George Koudis, Christiane Voigt, and Marc E. J. Stettler
Atmos. Chem. Phys., 22, 10919–10935, https://doi.org/10.5194/acp-22-10919-2022, https://doi.org/10.5194/acp-22-10919-2022, 2022
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Aircraft condensation trails (contrails) contribute to over half of the climate forcing attributable to aviation. This study uses historical air traffic and weather data to simulate contrails in the North Atlantic over 5 years, from 2016 to 2021. We found large intra- and inter-year variability in contrail radiative forcing and observed a 66 % reduction due to COVID-19. Most warming contrails predominantly result from night-time flights in winter.
Simon F. Reifenberg, Anna Martin, Matthias Kohl, Sara Bacer, Zaneta Hamryszczak, Ivan Tadic, Lenard Röder, Daniel J. Crowley, Horst Fischer, Katharina Kaiser, Johannes Schneider, Raphael Dörich, John N. Crowley, Laura Tomsche, Andreas Marsing, Christiane Voigt, Andreas Zahn, Christopher Pöhlker, Bruna A. Holanda, Ovid Krüger, Ulrich Pöschl, Mira Pöhlker, Patrick Jöckel, Marcel Dorf, Ulrich Schumann, Jonathan Williams, Birger Bohn, Joachim Curtius, Hardwig Harder, Hans Schlager, Jos Lelieveld, and Andrea Pozzer
Atmos. Chem. Phys., 22, 10901–10917, https://doi.org/10.5194/acp-22-10901-2022, https://doi.org/10.5194/acp-22-10901-2022, 2022
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In this work we use a combination of observational data from an aircraft campaign and model results to investigate the effect of the European lockdown due to COVID-19 in spring 2020. Using model results, we show that the largest relative changes to the atmospheric composition caused by the reduced emissions are located in the upper troposphere around aircraft cruise altitude, while the largest absolute changes are present at the surface.
Xianda Gong, Martin Radenz, Heike Wex, Patric Seifert, Farnoush Ataei, Silvia Henning, Holger Baars, Boris Barja, Albert Ansmann, and Frank Stratmann
Atmos. Chem. Phys., 22, 10505–10525, https://doi.org/10.5194/acp-22-10505-2022, https://doi.org/10.5194/acp-22-10505-2022, 2022
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The sources of ice-nucleating particles (INPs) are poorly understood in the Southern Hemisphere (SH). We studied INPs in the boundary layer in the southern Patagonia region. No seasonal cycle of INP concentrations was observed. The majority of INPs are biogenic particles, likely from local continental sources. The INP concentrations are higher when strong precipitation occurs. While previous studies focused on marine INP sources in SH, we point out the importance of continental sources of INPs.
Meryl Wimmer, Gwendal Rivière, Philippe Arbogast, Jean-Marcel Piriou, Julien Delanoë, Carole Labadie, Quitterie Cazenave, and Jacques Pelon
Weather Clim. Dynam., 3, 863–882, https://doi.org/10.5194/wcd-3-863-2022, https://doi.org/10.5194/wcd-3-863-2022, 2022
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The effect of deep convection representation on the jet stream above the cold front of an extratropical cyclone is investigated in the global numerical weather prediction model ARPEGE. Two simulations using different deep convection schemes are compared with (re)analysis datasets and NAWDEX airborne observations. A deeper jet stream is observed with the less active scheme. The diabatic origin of this difference is interpreted by backward Lagrangian trajectories and potential vorticity budgets.
Bastian Kirsch, Cathy Hohenegger, Daniel Klocke, Rainer Senke, Michael Offermann, and Felix Ament
Earth Syst. Sci. Data, 14, 3531–3548, https://doi.org/10.5194/essd-14-3531-2022, https://doi.org/10.5194/essd-14-3531-2022, 2022
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Conventional observation networks are too coarse to resolve the horizontal structure of kilometer-scale atmospheric processes. We present the FESST@HH field experiment that took place in Hamburg (Germany) during summer 2020 and featured a dense network of 103 custom-built, low-cost weather stations. The data set is capable of providing new insights into the structure of convective cold pools and the nocturnal urban heat island and variations of local temperature fluctuations.
Janine Lückerath, Andreas Held, Holger Siebert, Michel Michalkow, and Birgit Wehner
Atmos. Chem. Phys., 22, 10007–10021, https://doi.org/10.5194/acp-22-10007-2022, https://doi.org/10.5194/acp-22-10007-2022, 2022
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Three different methods were applied to estimate the vertical aerosol particle flux in the marine boundary layer (MBL) and between the MBL and free troposphere. For the first time, aerosol fluxes derived from these three methods were estimated and compared using airborne aerosol measurements using data from the ACORES field campaign in the northeastern Atlantic Ocean in July 2017. The amount of fluxes was small and directed up and down for different cases, but the methods were applicable.
Carlton Xavier, Metin Baykara, Robin Wollesen de Jonge, Barbara Altstädter, Petri Clusius, Ville Vakkari, Roseline Thakur, Lisa Beck, Silvia Becagli, Mirko Severi, Rita Traversi, Radovan Krejci, Peter Tunved, Mauro Mazzola, Birgit Wehner, Mikko Sipilä, Markku Kulmala, Michael Boy, and Pontus Roldin
Atmos. Chem. Phys., 22, 10023–10043, https://doi.org/10.5194/acp-22-10023-2022, https://doi.org/10.5194/acp-22-10023-2022, 2022
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The focus of this work is to study and improve our understanding of processes involved in the formation and growth of new particles in a remote Arctic marine environment. We run the 1D model ADCHEM along air mass trajectories arriving at Ny-Ålesund in May 2018. The model finds that ion-mediated H2SO4–NH3 nucleation can explain the observed new particle formation at Ny-Ålesund. The growth of particles is driven via H2SO4 condensation and formation of methane sulfonic acid in the aqueous phase.
Elena Shevnina, Miguel Potes, Timo Vihma, Tuomas Naakka, Pankaj Ramji Dhote, and Praveen Kumar Thakur
The Cryosphere, 16, 3101–3121, https://doi.org/10.5194/tc-16-3101-2022, https://doi.org/10.5194/tc-16-3101-2022, 2022
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The evaporation over an ice-free glacial lake was measured in January 2018, and the uncertainties inherent to five indirect methods were quantified. Results show that in summer up to 5 mm of water evaporated daily from the surface of the lake located in Antarctica. The indirect methods underestimated the evaporation over the lake's surface by up to 72 %. The results are important for estimating the evaporation over polar regions where a growing number of glacial lakes have recently been evident.
Christian Tatzelt, Silvia Henning, André Welti, Andrea Baccarini, Markus Hartmann, Martin Gysel-Beer, Manuela van Pinxteren, Robin L. Modini, Julia Schmale, and Frank Stratmann
Atmos. Chem. Phys., 22, 9721–9745, https://doi.org/10.5194/acp-22-9721-2022, https://doi.org/10.5194/acp-22-9721-2022, 2022
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We present the abundance and origin of cloud-relevant aerosol particles in the preindustral-like conditions of the Southern Ocean (SO) during austral summer. Cloud condensation nuclei (CCN) and ice-nucleating particles (INP) were measured during a circum-Antarctic scientific cruise with in situ instrumentation and offline filter measurements, respectively. Transport processes were found to play an equally important role as local sources for both the CCN and INP population of the SO.
Alexander D. Harrison, Daniel O'Sullivan, Michael P. Adams, Grace C. E. Porter, Edmund Blades, Cherise Brathwaite, Rebecca Chewitt-Lucas, Cassandra Gaston, Rachel Hawker, Ovid O. Krüger, Leslie Neve, Mira L. Pöhlker, Christopher Pöhlker, Ulrich Pöschl, Alberto Sanchez-Marroquin, Andrea Sealy, Peter Sealy, Mark D. Tarn, Shanice Whitehall, James B. McQuaid, Kenneth S. Carslaw, Joseph M. Prospero, and Benjamin J. Murray
Atmos. Chem. Phys., 22, 9663–9680, https://doi.org/10.5194/acp-22-9663-2022, https://doi.org/10.5194/acp-22-9663-2022, 2022
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The formation of ice in clouds fundamentally alters cloud properties; hence it is important we understand the special aerosol particles that can nucleate ice when immersed in supercooled cloud droplets. In this paper we show that African desert dust that has travelled across the Atlantic to the Caribbean nucleates ice much less well than we might have expected.
Zezhen Cheng, Megan Morgenstern, Bo Zhang, Matthew Fraund, Nurun Nahar Lata, Rhenton Brimberry, Matthew A. Marcus, Lynn Mazzoleni, Paulo Fialho, Silvia Henning, Birgit Wehner, Claudio Mazzoleni, and Swarup China
Atmos. Chem. Phys., 22, 9033–9057, https://doi.org/10.5194/acp-22-9033-2022, https://doi.org/10.5194/acp-22-9033-2022, 2022
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We observed a high abundance of liquid and internally mixed particles in samples collected in the North Atlantic free troposphere during summer. We also found several solid and semisolid particles for different emission sources and transport patterns. Our results suggest that considering the mixing state, emission source, and transport patterns of particles is necessary to estimate their phase state in the free troposphere, which is critical for predicting their effects on climate.
Jakub L. Nowak, Robert Grosz, Wiebke Frey, Dennis Niedermeier, Jędrzej Mijas, Szymon P. Malinowski, Linda Ort, Silvio Schmalfuß, Frank Stratmann, Jens Voigtländer, and Tadeusz Stacewicz
Atmos. Meas. Tech., 15, 4075–4089, https://doi.org/10.5194/amt-15-4075-2022, https://doi.org/10.5194/amt-15-4075-2022, 2022
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A high-resolution infrared hygrometer (FIRH) was adapted to measure humidity and its rapid fluctuations in turbulence inside a moist-air wind tunnel LACIS-T where two air streams of different temperature and humidity are mixed. The measurement was achieved from outside the tunnel through its glass windows and provided an agreement with a reference dew-point hygrometer placed inside. The characterization of humidity complements previous investigations of velocity and temperature fields.
Gina Jozef, John Cassano, Sandro Dahlke, and Gijs de Boer
Atmos. Meas. Tech., 15, 4001–4022, https://doi.org/10.5194/amt-15-4001-2022, https://doi.org/10.5194/amt-15-4001-2022, 2022
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During the MOSAiC expedition, meteorological conditions over the lowest 1 km of the atmosphere were sampled with the DataHawk2 uncrewed aircraft system. These data were used to identify the best method for atmospheric boundary layer height detection by comparing visually identified subjective boundary layer height to that identified by several objective automated detection methods. The results show a bulk Richardson number-based approach gives the best estimate of boundary layer height.
Ovid O. Krüger, Bruna A. Holanda, Sourangsu Chowdhury, Andrea Pozzer, David Walter, Christopher Pöhlker, Maria Dolores Andrés Hernández, John P. Burrows, Christiane Voigt, Jos Lelieveld, Johannes Quaas, Ulrich Pöschl, and Mira L. Pöhlker
Atmos. Chem. Phys., 22, 8683–8699, https://doi.org/10.5194/acp-22-8683-2022, https://doi.org/10.5194/acp-22-8683-2022, 2022
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The abrupt reduction in human activities during the first COVID-19 lockdown created unprecedented atmospheric conditions. We took the opportunity to quantify changes in black carbon (BC) as a major anthropogenic air pollutant. Therefore, we measured BC on board a research aircraft over Europe during the lockdown and compared the results to measurements from 2017. With model simulations we account for different weather conditions and find a lockdown-related decrease in BC of 41 %.
Eleni Tetoni, Florian Ewald, Martin Hagen, Gregor Köcher, Tobias Zinner, and Silke Groß
Atmos. Meas. Tech., 15, 3969–3999, https://doi.org/10.5194/amt-15-3969-2022, https://doi.org/10.5194/amt-15-3969-2022, 2022
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We use the C-band POLDIRAD and the Ka-band MIRA-35 to perform snowfall dual-wavelength polarimetric radar measurements. We develop an ice microphysics retrieval for mass, apparent shape, and median size of the particle size distribution by comparing observations to T-matrix ice spheroid simulations while varying the mass–size relationship. We furthermore show how the polarimetric measurements from POLDIRAD help to narrow down ambiguities between ice particle shape and size.
Simon Kirschler, Christiane Voigt, Bruce Anderson, Ramon Campos Braga, Gao Chen, Andrea F. Corral, Ewan Crosbie, Hossein Dadashazar, Richard A. Ferrare, Valerian Hahn, Johannes Hendricks, Stefan Kaufmann, Richard Moore, Mira L. Pöhlker, Claire Robinson, Amy J. Scarino, Dominik Schollmayer, Michael A. Shook, K. Lee Thornhill, Edward Winstead, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 22, 8299–8319, https://doi.org/10.5194/acp-22-8299-2022, https://doi.org/10.5194/acp-22-8299-2022, 2022
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In this study we show that the vertical velocity dominantly impacts the cloud droplet number concentration (NC) of low-level clouds over the western North Atlantic in the winter and summer season, while the cloud condensation nuclei concentration, aerosol size distribution and chemical composition impact NC within a season. The observational data presented in this study can evaluate and improve the representation of aerosol–cloud interactions for a wide range of conditions.
Dongwei Fu, Larry Di Girolamo, Robert M. Rauber, Greg M. McFarquhar, Stephen W. Nesbitt, Jesse Loveridge, Yulan Hong, Bastiaan van Diedenhoven, Brian Cairns, Mikhail D. Alexandrov, Paul Lawson, Sarah Woods, Simone Tanelli, Sebastian Schmidt, Chris Hostetler, and Amy Jo Scarino
Atmos. Chem. Phys., 22, 8259–8285, https://doi.org/10.5194/acp-22-8259-2022, https://doi.org/10.5194/acp-22-8259-2022, 2022
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Satellite-retrieved cloud microphysics are widely used in climate research because of their central role in water and energy cycles. Here, we provide the first detailed investigation of retrieved cloud drop sizes from in situ and various satellite and airborne remote sensing techniques applied to real cumulus cloud fields. We conclude that the most widely used passive remote sensing method employed in climate research produces high biases of 6–8 µm (60 %–80 %) caused by 3-D radiative effects.
Henning Dorff, Heike Konow, and Felix Ament
Atmos. Meas. Tech., 15, 3641–3661, https://doi.org/10.5194/amt-15-3641-2022, https://doi.org/10.5194/amt-15-3641-2022, 2022
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This study elaborates how aircraft-based horizontal geometries of trade wind cumuli differ whether a one-dimensional profiling radar or a two-dimensional imager is used. Cloud size distributions are examined in terms of sensitivity to sample size, resolution, and instrument field of view. While the radar cannot reproduce the double power law distribution due to coarse resolution and restriction to vertical transects, the imager also reveals the elliptic cloud structure enhancing with wind speed.
Arve Kylling, Claudia Emde, Huan Yu, Michel van Roozendael, Kerstin Stebel, Ben Veihelmann, and Bernhard Mayer
Atmos. Meas. Tech., 15, 3481–3495, https://doi.org/10.5194/amt-15-3481-2022, https://doi.org/10.5194/amt-15-3481-2022, 2022
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Atmospheric trace gases such as nitrogen dioxide (NO2) may be measured by satellite instruments sensitive to solar ultraviolet–visible radiation reflected from Earth and its atmosphere. For a single pixel, clouds in neighbouring pixels may affect the radiation and hence the retrieved trace gas amount. We found that for a solar zenith angle less than about 40° this cloud-related NO2 bias is typically below 10 %, while for larger solar zenith angles the NO2 bias is on the order of tens of percent.
Manuel Gutleben, Silke Groß, Christian Heske, and Martin Wirth
Atmos. Chem. Phys., 22, 7319–7330, https://doi.org/10.5194/acp-22-7319-2022, https://doi.org/10.5194/acp-22-7319-2022, 2022
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The main transportation route of Saharan mineral dust particles leads over the subtropical Atlantic Ocean and is subject to a seasonal variation. This study investigates the characteristics of wintertime transatlantic dust transport towards the Caribbean by means of airborne lidar measurements. It is found that dust particles are transported at low atmospheric altitudes (<3.5 km) embedded in a relatively moist mixture with two other particle types, namely marine and biomass-burning particles.
Annakaisa von Lerber, Mario Mech, Annette Rinke, Damao Zhang, Melanie Lauer, Ana Radovan, Irina Gorodetskaya, and Susanne Crewell
Atmos. Chem. Phys., 22, 7287–7317, https://doi.org/10.5194/acp-22-7287-2022, https://doi.org/10.5194/acp-22-7287-2022, 2022
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Snowfall is an important climate indicator. However, microphysical snowfall processes are challenging for atmospheric models. In this study, the performance of a regional climate model is evaluated in modeling the spatial and temporal distribution of Arctic snowfall when compared to CloudSat satellite observations. Excellent agreement in averaged annual snowfall rates is found, and the shown methodology offers a promising diagnostic tool to investigate the shown differences further.
Theresa Mieslinger, Bjorn Stevens, Tobias Kölling, Manfred Brath, Martin Wirth, and Stefan A. Buehler
Atmos. Chem. Phys., 22, 6879–6898, https://doi.org/10.5194/acp-22-6879-2022, https://doi.org/10.5194/acp-22-6879-2022, 2022
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The trades are home to a plethora of small cumulus clouds that are often barely visible to the human eye and difficult to detect with active and passive remote sensing methods. With the help of a new method and by means of high-resolution data we can detect small and particularly thin clouds. We find that optically thin clouds are a common phenomenon in the trades, covering a large area and influencing the radiative effect of clouds if they are undetected and contaminate the cloud-free signal.
Andreas Hünig, Oliver Appel, Antonis Dragoneas, Sergej Molleker, Hans-Christian Clemen, Frank Helleis, Thomas Klimach, Franziska Köllner, Thomas Böttger, Frank Drewnick, Johannes Schneider, and Stephan Borrmann
Atmos. Meas. Tech., 15, 2889–2921, https://doi.org/10.5194/amt-15-2889-2022, https://doi.org/10.5194/amt-15-2889-2022, 2022
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We have serially combined the two well-established methods for in situ real-time measurement of fine particle chemical composition, the single-particle laser ablation method and the flash evaporation with electron impact ionization method, into a novel instrument. Here we present the design; instrument characteristics, as derived from laboratory and field measurements; and results from the first field deployment during the 2017 StratoClim aircraft campaign.
Sebastian Becker, André Ehrlich, Evelyn Jäkel, Tim Carlsen, Michael Schäfer, and Manfred Wendisch
Atmos. Meas. Tech., 15, 2939–2953, https://doi.org/10.5194/amt-15-2939-2022, https://doi.org/10.5194/amt-15-2939-2022, 2022
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Airborne radiation measurements are used to characterize the solar directional reflection of a mixture of Arctic sea ice and open-ocean surfaces in the transition zone between both surface types. The mixture reveals reflection properties of both surface types. It is shown that the directional reflection of the mixture can be reconstructed from the directional reflection of the individual surfaces, accounting for the special conditions present in the transition zone.
M. Dolores Andrés Hernández, Andreas Hilboll, Helmut Ziereis, Eric Förster, Ovid O. Krüger, Katharina Kaiser, Johannes Schneider, Francesca Barnaba, Mihalis Vrekoussis, Jörg Schmidt, Heidi Huntrieser, Anne-Marlene Blechschmidt, Midhun George, Vladyslav Nenakhov, Theresa Harlass, Bruna A. Holanda, Jennifer Wolf, Lisa Eirenschmalz, Marc Krebsbach, Mira L. Pöhlker, Anna B. Kalisz Hedegaard, Linlu Mei, Klaus Pfeilsticker, Yangzhuoran Liu, Ralf Koppmann, Hans Schlager, Birger Bohn, Ulrich Schumann, Andreas Richter, Benjamin Schreiner, Daniel Sauer, Robert Baumann, Mariano Mertens, Patrick Jöckel, Markus Kilian, Greta Stratmann, Christopher Pöhlker, Monica Campanelli, Marco Pandolfi, Michael Sicard, José L. Gómez-Amo, Manuel Pujadas, Katja Bigge, Flora Kluge, Anja Schwarz, Nikos Daskalakis, David Walter, Andreas Zahn, Ulrich Pöschl, Harald Bönisch, Stephan Borrmann, Ulrich Platt, and John P. Burrows
Atmos. Chem. Phys., 22, 5877–5924, https://doi.org/10.5194/acp-22-5877-2022, https://doi.org/10.5194/acp-22-5877-2022, 2022
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EMeRGe provides a unique set of in situ and remote sensing airborne measurements of trace gases and aerosol particles along selected flight routes in the lower troposphere over Europe. The interpretation uses also complementary collocated ground-based and satellite measurements. The collected data help to improve the current understanding of the complex spatial distribution of trace gases and aerosol particles resulting from mixing, transport, and transformation of pollution plumes over Europe.
Manuela van Pinxteren, Tiera-Brandy Robinson, Sebastian Zeppenfeld, Xianda Gong, Enno Bahlmann, Khanneh Wadinga Fomba, Nadja Triesch, Frank Stratmann, Oliver Wurl, Anja Engel, Heike Wex, and Hartmut Herrmann
Atmos. Chem. Phys., 22, 5725–5742, https://doi.org/10.5194/acp-22-5725-2022, https://doi.org/10.5194/acp-22-5725-2022, 2022
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A class of marine particles (transparent exopolymer particles, TEPs) that is ubiquitously found in the world oceans was measured for the first time in ambient marine aerosol particles and marine cloud waters in the tropical Atlantic Ocean. TEPs are likely to have good properties for influencing clouds. We show that TEPs are transferred from the ocean to the marine atmosphere via sea-spray formation and our results suggest that they can also form directly in aerosol particles and in cloud water.
Sandrine Bony, Marie Lothon, Julien Delanoë, Pierre Coutris, Jean-Claude Etienne, Franziska Aemisegger, Anna Lea Albright, Thierry André, Hubert Bellec, Alexandre Baron, Jean-François Bourdinot, Pierre-Etienne Brilouet, Aurélien Bourdon, Jean-Christophe Canonici, Christophe Caudoux, Patrick Chazette, Michel Cluzeau, Céline Cornet, Jean-Philippe Desbios, Dominique Duchanoy, Cyrille Flamant, Benjamin Fildier, Christophe Gourbeyre, Laurent Guiraud, Tetyana Jiang, Claude Lainard, Christophe Le Gac, Christian Lendroit, Julien Lernould, Thierry Perrin, Frédéric Pouvesle, Pascal Richard, Nicolas Rochetin, Kevin Salaün, Alfons Schwarzenboeck, Guillaume Seurat, Bjorn Stevens, Julien Totems, Ludovic Touzé-Peiffer, Gilles Vergez, Jessica Vial, Leonie Villiger, and Raphaela Vogel
Earth Syst. Sci. Data, 14, 2021–2064, https://doi.org/10.5194/essd-14-2021-2022, https://doi.org/10.5194/essd-14-2021-2022, 2022
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The French ATR42 research aircraft participated in the EUREC4A international field campaign that took place in 2020 over the tropical Atlantic, east of Barbados. We present the extensive instrumentation of the aircraft, the research flights and the different measurements. We show that the ATR measurements of humidity, wind, aerosols and cloudiness in the lower atmosphere are robust and consistent with each other. They will make it possible to advance understanding of cloud–climate interactions.
Mireia Papke Chica, Valerian Hahn, Tiziana Braeuer, Elena de la Torre Castro, Florian Ewald, Mathias Gergely, Simon Kirschler, Luca Bugliaro Goggia, Stefanie Knobloch, Martina Kraemer, Johannes Lucke, Johanna Mayer, Raphael Maerkl, Manuel Moser, Laura Tomsche, Tina Jurkat-Witschas, Martin Zoeger, Christian von Savigny, and Christiane Voigt
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-255, https://doi.org/10.5194/acp-2022-255, 2022
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The mixed-phase temperature regime in convective clouds challenges our understanding of microphysical and radiative cloud properties. We provide a rare and unique dataset of aircraft in situ measurements in a strong mid-latitude convective system. We find that mechanisms initiating ice nucleation and growth strongly depend on temperature, relative humidity, and vertical velocity and variate within the measured system, resulting in altitude dependent changes of the cloud liquid and ice fraction.
Xianda Gong, Heike Wex, Thomas Müller, Silvia Henning, Jens Voigtländer, Alfred Wiedensohler, and Frank Stratmann
Atmos. Chem. Phys., 22, 5175–5194, https://doi.org/10.5194/acp-22-5175-2022, https://doi.org/10.5194/acp-22-5175-2022, 2022
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We conducted 10 yr measurements to characterize the atmospheric aerosol at Cabo Verde. An unsupervised machine learning algorithm, K-means, was implemented to study the aerosol types. Cloud condensation nuclei number concentrations during dust periods were 2.5 times higher than marine periods. The long-term data sets, together with the aerosol classification, can be used as a basis to improve understanding of annual cycles of aerosol, and aerosol-cloud interactions in the North Atlantic.
Janosch Michaelis, Amelie U. Schmitt, Christof Lüpkes, Jörg Hartmann, Gerit Birnbaum, and Timo Vihma
Earth Syst. Sci. Data, 14, 1621–1637, https://doi.org/10.5194/essd-14-1621-2022, https://doi.org/10.5194/essd-14-1621-2022, 2022
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A major goal of the Springtime Atmospheric Boundary Layer Experiment (STABLE) aircraft campaign was to observe atmospheric conditions during marine cold-air outbreaks (MCAOs) originating from the sea-ice-covered Arctic ocean. Quality-controlled measurements of several meteorological variables collected during 15 vertical aircraft profiles and by 22 dropsondes are presented. The comprehensive data set may be used for validating model results to improve the understanding of future trends in MCAOs.
Hanna K. Lappalainen, Tuukka Petäjä, Timo Vihma, Jouni Räisänen, Alexander Baklanov, Sergey Chalov, Igor Esau, Ekaterina Ezhova, Matti Leppäranta, Dmitry Pozdnyakov, Jukka Pumpanen, Meinrat O. Andreae, Mikhail Arshinov, Eija Asmi, Jianhui Bai, Igor Bashmachnikov, Boris Belan, Federico Bianchi, Boris Biskaborn, Michael Boy, Jaana Bäck, Bin Cheng, Natalia Chubarova, Jonathan Duplissy, Egor Dyukarev, Konstantinos Eleftheriadis, Martin Forsius, Martin Heimann, Sirkku Juhola, Vladimir Konovalov, Igor Konovalov, Pavel Konstantinov, Kajar Köster, Elena Lapshina, Anna Lintunen, Alexander Mahura, Risto Makkonen, Svetlana Malkhazova, Ivan Mammarella, Stefano Mammola, Stephany Buenrostro Mazon, Outi Meinander, Eugene Mikhailov, Victoria Miles, Stanislav Myslenkov, Dmitry Orlov, Jean-Daniel Paris, Roberta Pirazzini, Olga Popovicheva, Jouni Pulliainen, Kimmo Rautiainen, Torsten Sachs, Vladimir Shevchenko, Andrey Skorokhod, Andreas Stohl, Elli Suhonen, Erik S. Thomson, Marina Tsidilina, Veli-Pekka Tynkkynen, Petteri Uotila, Aki Virkkula, Nadezhda Voropay, Tobias Wolf, Sayaka Yasunaka, Jiahua Zhang, Yubao Qiu, Aijun Ding, Huadong Guo, Valery Bondur, Nikolay Kasimov, Sergej Zilitinkevich, Veli-Matti Kerminen, and Markku Kulmala
Atmos. Chem. Phys., 22, 4413–4469, https://doi.org/10.5194/acp-22-4413-2022, https://doi.org/10.5194/acp-22-4413-2022, 2022
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We summarize results during the last 5 years in the northern Eurasian region, especially from Russia, and introduce recent observations of the air quality in the urban environments in China. Although the scientific knowledge in these regions has increased, there are still gaps in our understanding of large-scale climate–Earth surface interactions and feedbacks. This arises from limitations in research infrastructures and integrative data analyses, hindering a comprehensive system analysis.
Luca Bugliaro, Dennis Piontek, Stephan Kox, Marius Schmidl, Bernhard Mayer, Richard Müller, Margarita Vázquez-Navarro, Daniel M. Peters, Roy G. Grainger, Josef Gasteiger, and Jayanta Kar
Nat. Hazards Earth Syst. Sci., 22, 1029–1054, https://doi.org/10.5194/nhess-22-1029-2022, https://doi.org/10.5194/nhess-22-1029-2022, 2022
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The monitoring of ash dispersion in the atmosphere is an important task for satellite remote sensing since ash represents a threat to air traffic. We present an AI-based method that retrieves the spatial extension and properties of volcanic ash clouds with high temporal resolution during day and night by means of geostationary satellite measurements. This algorithm, trained on realistic observations simulated with a radiative transfer model, runs operationally at the German Weather Service.
Valery Shcherbakov, Frédéric Szczap, Alaa Alkasem, Guillaume Mioche, and Céline Cornet
Atmos. Meas. Tech., 15, 1729–1754, https://doi.org/10.5194/amt-15-1729-2022, https://doi.org/10.5194/amt-15-1729-2022, 2022
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We performed extensive Monte Carlo (MC) simulations of lidar signals and developed an empirical model to account for the multiple scattering in the lidar signals. The simulations have taken into consideration four types of lidar configurations (the ground based, the airborne, the CALIOP, and the ATLID) and four types of particles (coarse aerosol, water cloud, jet-stream cirrus, and cirrus).
The empirical model has very good quality of MC data fitting for all considered cases.
Claudia Emde, Huan Yu, Arve Kylling, Michel van Roozendael, Kerstin Stebel, Ben Veihelmann, and Bernhard Mayer
Atmos. Meas. Tech., 15, 1587–1608, https://doi.org/10.5194/amt-15-1587-2022, https://doi.org/10.5194/amt-15-1587-2022, 2022
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Retrievals of trace gas concentrations from satellite observations can be affected by clouds in the vicinity, either by shadowing or by scattering of radiation from clouds in the clear region. We used a Monte Carlo radiative transfer model to generate synthetic satellite observations, which we used to test retrieval algorithms and to quantify the error of retrieved NO2 vertical column density due to cloud scattering.
Helmut Ziereis, Peter Hoor, Jens-Uwe Grooß, Andreas Zahn, Greta Stratmann, Paul Stock, Michael Lichtenstern, Jens Krause, Vera Bense, Armin Afchine, Christian Rolf, Wolfgang Woiwode, Marleen Braun, Jörn Ungermann, Andreas Marsing, Christiane Voigt, Andreas Engel, Björn-Martin Sinnhuber, and Hermann Oelhaf
Atmos. Chem. Phys., 22, 3631–3654, https://doi.org/10.5194/acp-22-3631-2022, https://doi.org/10.5194/acp-22-3631-2022, 2022
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Airborne observations were conducted in the lowermost Arctic stratosphere during the winter of 2015/2016. The observed distribution of reactive nitrogen shows clear indications of nitrification in mid-winter and denitrification in late winter. This was caused by the formation of polar stratospheric cloud particles, which were observed during several flights. The sedimentation and evaporation of these particles and the descent of air masses cause a redistribution of reactive nitrogen.
Marco A. Franco, Florian Ditas, Leslie A. Kremper, Luiz A. T. Machado, Meinrat O. Andreae, Alessandro Araújo, Henrique M. J. Barbosa, Joel F. de Brito, Samara Carbone, Bruna A. Holanda, Fernando G. Morais, Janaína P. Nascimento, Mira L. Pöhlker, Luciana V. Rizzo, Marta Sá, Jorge Saturno, David Walter, Stefan Wolff, Ulrich Pöschl, Paulo Artaxo, and Christopher Pöhlker
Atmos. Chem. Phys., 22, 3469–3492, https://doi.org/10.5194/acp-22-3469-2022, https://doi.org/10.5194/acp-22-3469-2022, 2022
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In Central Amazonia, new particle formation in the planetary boundary layer is rare. Instead, there is the appearance of sub-50 nm aerosols with diameters larger than about 20 nm that eventually grow to cloud condensation nuclei size range. Here, 254 growth events were characterized which have higher predominance in the wet season. About 70 % of them showed direct relation to convective downdrafts, while 30 % occurred partly under clear-sky conditions, evidencing still unknown particle sources.
Michael Schäfer, Kevin Wolf, André Ehrlich, Christoph Hallbauer, Evelyn Jäkel, Friedhelm Jansen, Anna Elizabeth Luebke, Joshua Müller, Jakob Thoböll, Timo Röschenthaler, Bjorn Stevens, and Manfred Wendisch
Atmos. Meas. Tech., 15, 1491–1509, https://doi.org/10.5194/amt-15-1491-2022, https://doi.org/10.5194/amt-15-1491-2022, 2022
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The new airborne thermal infrared imager VELOX is introduced. It measures two-dimensional fields of spectral thermal infrared radiance or brightness temperature within the large atmospheric window. The technical specifications as well as necessary calibration and correction procedures are presented. Example measurements from the first field deployment are analysed with respect to cloud coverage and cloud top altitude.
Matthew S. Norgren, John Wood, K. Sebastian Schmidt, Bastiaan van Diedenhoven, Snorre A. Stamnes, Luke D. Ziemba, Ewan C. Crosbie, Michael A. Shook, A. Scott Kittelman, Samuel E. LeBlanc, Stephen Broccardo, Steffen Freitag, and Jeffrey S. Reid
Atmos. Meas. Tech., 15, 1373–1394, https://doi.org/10.5194/amt-15-1373-2022, https://doi.org/10.5194/amt-15-1373-2022, 2022
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A new spectral instrument (SPN-S), with the ability to partition solar radiation into direct and diffuse components, is used in airborne settings to study the optical properties of aerosols and cirrus. It is a low-cost and mechanically simple system but has higher measurement uncertainty than existing standards. This challenge is overcome by utilizing the unique measurement capabilities to develop new retrieval techniques. Validation is done with data from two NASA airborne research campaigns.
Alexander Myagkov and Davide Ori
Atmos. Meas. Tech., 15, 1333–1354, https://doi.org/10.5194/amt-15-1333-2022, https://doi.org/10.5194/amt-15-1333-2022, 2022
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This study provides equations to characterize random errors of spectral polarimetric observations from cloud radars. The results can be used for a broad spectrum of applications. For instance, accurate error characterization is essential for advanced retrievals of microphysical properties of clouds and precipitation. Moreover, error characterization allows for the use of measurements from polarimetric cloud radars to potentially improve weather forecasts.
Adrien Deroubaix, Laurent Menut, Cyrille Flamant, Peter Knippertz, Andreas H. Fink, Anneke Batenburg, Joel Brito, Cyrielle Denjean, Cheikh Dione, Régis Dupuy, Valerian Hahn, Norbert Kalthoff, Fabienne Lohou, Alfons Schwarzenboeck, Guillaume Siour, Paolo Tuccella, and Christiane Voigt
Atmos. Chem. Phys., 22, 3251–3273, https://doi.org/10.5194/acp-22-3251-2022, https://doi.org/10.5194/acp-22-3251-2022, 2022
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During the summer monsoon in West Africa, pollutants emitted in urbanized areas modify cloud cover and precipitation patterns. We analyze these patterns with the WRF-CHIMERE model, integrating the effects of aerosols on meteorology, based on the numerous observations provided by the Dynamics-Aerosol-Climate-Interactions campaign. This study adds evidence to recent findings that increased pollution levels in West Africa delay the breakup time of low-level clouds and reduce precipitation.
Gregor Köcher, Tobias Zinner, Christoph Knote, Eleni Tetoni, Florian Ewald, and Martin Hagen
Atmos. Meas. Tech., 15, 1033–1054, https://doi.org/10.5194/amt-15-1033-2022, https://doi.org/10.5194/amt-15-1033-2022, 2022
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We present a setup for systematic characterization of differences between numerical weather models and radar observations for convective weather situations. Radar observations providing dual-wavelength and polarimetric variables to infer information about hydrometeor shapes and sizes are compared against simulations using microphysics schemes of varying complexity. Differences are found in ice and liquid phase, pointing towards issues of some schemes in reproducing particle size distributions.
Anna E. Luebke, André Ehrlich, Michael Schäfer, Kevin Wolf, and Manfred Wendisch
Atmos. Chem. Phys., 22, 2727–2744, https://doi.org/10.5194/acp-22-2727-2022, https://doi.org/10.5194/acp-22-2727-2022, 2022
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A combination of aircraft and satellite observations is used to show how the characteristics of tropical shallow clouds interact with incoming and outgoing energy. A complete depiction of these clouds is challenging to obtain, but such data are useful for understanding how models can correctly represent them. The amount of cloud is found to be the most important factor, while other cloud characteristics become increasingly impactful when more cloud is present.
Rupert Holzinger, Oliver Eppers, Kouji Adachi, Heiko Bozem, Markus Hartmann, Andreas Herber, Makoto Koike, Dylan B. Millet, Nobuhiro Moteki, Sho Ohata, Frank Stratmann, and Atsushi Yoshida
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-95, https://doi.org/10.5194/acp-2022-95, 2022
Revised manuscript not accepted
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In spring 2018 the research aircraft Polar 5 conducted flights in the Arctic atmosphere. The flight operation was from Station Nord in Greenland, 1700 km north of the Arctic Circle (81°43'N, 17°47'W). Using a mass spectrometer we measured more than 100 organic compounds in the air. We found a clear signature of natural organic compounds that are transported from forests to the high Arctic. These compounds have the potential to change the cloud cover and energy budget of the Arctic region.
Alexander Mchedlishvili, Gunnar Spreen, Christian Melsheimer, and Marcus Huntemann
The Cryosphere, 16, 471–487, https://doi.org/10.5194/tc-16-471-2022, https://doi.org/10.5194/tc-16-471-2022, 2022
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In this paper we show that the activity leading to the open-ocean polynyas near the Maud Rise seamount that have occurred repeatedly from 1974–1976 as well as 2016–2017 does not simply stop for polynya-free years. Using apparent sea ice thickness retrieval, we have identified anomalies where there is thinning of sea ice on a scale that is comparable to that of the polynya events of 2016–2017. These anomalies took place in 2010, 2013, 2014 and 2018.
Simon Pfreundschuh, Stuart Fox, Patrick Eriksson, David Duncan, Stefan A. Buehler, Manfred Brath, Richard Cotton, and Florian Ewald
Atmos. Meas. Tech., 15, 677–699, https://doi.org/10.5194/amt-15-677-2022, https://doi.org/10.5194/amt-15-677-2022, 2022
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We test a novel method to remotely measure ice particles in clouds. This is important because such measurements are required to improve climate and weather models. The method combines a radar with newly developed sensors measuring microwave radiation at very short wavelengths. We use observations made from aircraft flying above the cloud and compare them to real measurements from inside the cloud. This works well given that one can model the ice particles in the cloud sufficiently well.
Anna A. Shestakova, Dmitry G. Chechin, Christof Lüpkes, Jörg Hartmann, and Marion Maturilli
Atmos. Chem. Phys., 22, 1529–1548, https://doi.org/10.5194/acp-22-1529-2022, https://doi.org/10.5194/acp-22-1529-2022, 2022
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This article presents a comprehensive analysis of the easterly orographic wind episode which occurred over Svalbard on 30–31 May 2017. This wind caused a significant temperature rise on the lee side of the mountains and greatly intensified the snowmelt. This episode was investigated on the basis of measurements collected during the ACLOUD/PASCAL field campaigns with the help of numerical modeling.
Teresa Vogl, Maximilian Maahn, Stefan Kneifel, Willi Schimmel, Dmitri Moisseev, and Heike Kalesse-Los
Atmos. Meas. Tech., 15, 365–381, https://doi.org/10.5194/amt-15-365-2022, https://doi.org/10.5194/amt-15-365-2022, 2022
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We are using machine learning techniques, a type of artificial intelligence, to detect graupel formation in clouds. The measurements used as input to the machine learning framework were performed by cloud radars. Cloud radars are instruments located at the ground, emitting radiation with wavelenghts of a few millimeters vertically into the cloud and measuring the back-scattered signal. Our novel technique can be applied to different radar systems and different weather conditions.
Carolina Viceto, Irina V. Gorodetskaya, Annette Rinke, Marion Maturilli, Alfredo Rocha, and Susanne Crewell
Atmos. Chem. Phys., 22, 441–463, https://doi.org/10.5194/acp-22-441-2022, https://doi.org/10.5194/acp-22-441-2022, 2022
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We focus on anomalous moisture transport events known as atmospheric rivers (ARs). During ACLOUD and PASCAL, three AR events were identified: 30 May, 6 June, and 9 June 2017. We explore their spatio-temporal evolution and precipitation patterns using measurements, reanalyses, and a model. We show the importance of the following: Atlantic and Siberian pathways during spring–summer in the Arctic, AR-associated heat/moisture increase, precipitation phase transition, and high-resolution datasets.
Claudia Acquistapace, Richard Coulter, Susanne Crewell, Albert Garcia-Benadi, Rosa Gierens, Giacomo Labbri, Alexander Myagkov, Nils Risse, and Jan H. Schween
Earth Syst. Sci. Data, 14, 33–55, https://doi.org/10.5194/essd-14-33-2022, https://doi.org/10.5194/essd-14-33-2022, 2022
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This publication describes the unprecedented high-resolution cloud and precipitation dataset collected by two radars deployed on the Maria S. Merian research vessel. The ship operated in the west Atlantic Ocean during the measurement campaign called EUREC4A, between 19 January and 19 February 2020. The data collected are crucial to investigate clouds and precipitation and understand how they form and change over the ocean, where it is so difficult to measure them.
Sonja Murto, Rodrigo Caballero, Gunilla Svensson, and Lukas Papritz
Weather Clim. Dynam., 3, 21–44, https://doi.org/10.5194/wcd-3-21-2022, https://doi.org/10.5194/wcd-3-21-2022, 2022
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This study uses reanalysis data to investigate the role of atmospheric blocking, prevailing high-pressure systems and mid-latitude cyclones in driving high-Arctic wintertime warm extreme events. These events are mainly preceded by Ural and Scandinavian blocks, which are shown to be significantly influenced and amplified by cyclones in the North Atlantic. It also highlights processes that need to be well captured in climate models for improving their representation of Arctic wintertime climate.
Hélène Bresson, Annette Rinke, Mario Mech, Daniel Reinert, Vera Schemann, Kerstin Ebell, Marion Maturilli, Carolina Viceto, Irina Gorodetskaya, and Susanne Crewell
Atmos. Chem. Phys., 22, 173–196, https://doi.org/10.5194/acp-22-173-2022, https://doi.org/10.5194/acp-22-173-2022, 2022
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Arctic warming is pronounced, and one factor in this is the poleward atmospheric transport of heat and moisture. This study assesses the 4D structure of an Arctic moisture intrusion event which occurred in June 2017. For the first time, high-resolution pan-Arctic ICON simulations are performed and compared with global models, reanalysis, and observations. Results show the added value of high resolution in the event representation and the impact of the intrusion on the surface energy fluxes.
Sabrina P. Cochrane, K. Sebastian Schmidt, Hong Chen, Peter Pilewskie, Scott Kittelman, Jens Redemann, Samuel LeBlanc, Kristina Pistone, Michal Segal Rozenhaimer, Meloë Kacenelenbogen, Yohei Shinozuka, Connor Flynn, Rich Ferrare, Sharon Burton, Chris Hostetler, Marc Mallet, and Paquita Zuidema
Atmos. Meas. Tech., 15, 61–77, https://doi.org/10.5194/amt-15-61-2022, https://doi.org/10.5194/amt-15-61-2022, 2022
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This work presents heating rates derived from aircraft observations from the 2016 and 2017 field campaigns of ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS). We separate the total heating rates into aerosol and gas (primarily water vapor) absorption and explore some of the co-variability of heating rate profiles and their primary drivers, leading to the development of a new concept: the heating rate efficiency (HRE; the heating rate per unit aerosol extinction).
Martin Hagen, Florian Ewald, Silke Groß, Lothar Oswald, David A. Farrell, Marvin Forde, Manuel Gutleben, Johann Heumos, Jens Reimann, Eleni Tetoni, Gregor Köcher, Eleni Marinou, Christoph Kiemle, Qiang Li, Rebecca Chewitt-Lucas, Alton Daley, Delando Grant, and Kashawn Hall
Earth Syst. Sci. Data, 13, 5899–5914, https://doi.org/10.5194/essd-13-5899-2021, https://doi.org/10.5194/essd-13-5899-2021, 2021
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The German polarimetric weather radar Poldirad was deployed for the international campaign EUREC4A on Barbados. The focus was monitoring clouds and precipitation in the trade wind region east of Barbados. Observations were with a temporal sequence of 5 min and a maximum range of 375 km. Examples of mesoscale precipitation patterns, rain rate accumulation, diurnal cycle, and vertical distribution show the potential for further studies on the life cycle of precipitating shallow cumulus clouds.
Luiz A. T. Machado, Marco A. Franco, Leslie A. Kremper, Florian Ditas, Meinrat O. Andreae, Paulo Artaxo, Micael A. Cecchini, Bruna A. Holanda, Mira L. Pöhlker, Ivan Saraiva, Stefan Wolff, Ulrich Pöschl, and Christopher Pöhlker
Atmos. Chem. Phys., 21, 18065–18086, https://doi.org/10.5194/acp-21-18065-2021, https://doi.org/10.5194/acp-21-18065-2021, 2021
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Several studies evaluate aerosol–cloud interactions, but only a few attempted to describe how clouds modify aerosol properties. This study evaluates the effect of weather events on the particle size distribution at the ATTO, combining remote sensing and in situ data. Ultrafine, Aitken and accumulation particles modes have different behaviors for the diurnal cycle and for rainfall events. This study opens up new scientific questions that need to be pursued in detail in new field campaigns.
Ramon Campos Braga, Barbara Ervens, Daniel Rosenfeld, Meinrat O. Andreae, Jan-David Förster, Daniel Fütterer, Lianet Hernández Pardo, Bruna A. Holanda, Tina Jurkat-Witschas, Ovid O. Krüger, Oliver Lauer, Luiz A. T. Machado, Christopher Pöhlker, Daniel Sauer, Christiane Voigt, Adrian Walser, Manfred Wendisch, Ulrich Pöschl, and Mira L. Pöhlker
Atmos. Chem. Phys., 21, 17513–17528, https://doi.org/10.5194/acp-21-17513-2021, https://doi.org/10.5194/acp-21-17513-2021, 2021
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Interactions of aerosol particles with clouds represent a large uncertainty in estimates of climate change. Properties of aerosol particles control their ability to act as cloud condensation nuclei. Using aerosol measurements in the Amazon, we performed model studies to compare predicted and measured cloud droplet number concentrations at cloud bases. Our results confirm previous estimates of particle hygroscopicity in this region.
Silke Trömel, Clemens Simmer, Ulrich Blahak, Armin Blanke, Sabine Doktorowski, Florian Ewald, Michael Frech, Mathias Gergely, Martin Hagen, Tijana Janjic, Heike Kalesse-Los, Stefan Kneifel, Christoph Knote, Jana Mendrok, Manuel Moser, Gregor Köcher, Kai Mühlbauer, Alexander Myagkov, Velibor Pejcic, Patric Seifert, Prabhakar Shrestha, Audrey Teisseire, Leonie von Terzi, Eleni Tetoni, Teresa Vogl, Christiane Voigt, Yuefei Zeng, Tobias Zinner, and Johannes Quaas
Atmos. Chem. Phys., 21, 17291–17314, https://doi.org/10.5194/acp-21-17291-2021, https://doi.org/10.5194/acp-21-17291-2021, 2021
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The article introduces the ACP readership to ongoing research in Germany on cloud- and precipitation-related process information inherent in polarimetric radar measurements, outlines pathways to inform atmospheric models with radar-based information, and points to remaining challenges towards an improved fusion of radar polarimetry and atmospheric modelling.
Heike Konow, Florian Ewald, Geet George, Marek Jacob, Marcus Klingebiel, Tobias Kölling, Anna E. Luebke, Theresa Mieslinger, Veronika Pörtge, Jule Radtke, Michael Schäfer, Hauke Schulz, Raphaela Vogel, Martin Wirth, Sandrine Bony, Susanne Crewell, André Ehrlich, Linda Forster, Andreas Giez, Felix Gödde, Silke Groß, Manuel Gutleben, Martin Hagen, Lutz Hirsch, Friedhelm Jansen, Theresa Lang, Bernhard Mayer, Mario Mech, Marc Prange, Sabrina Schnitt, Jessica Vial, Andreas Walbröl, Manfred Wendisch, Kevin Wolf, Tobias Zinner, Martin Zöger, Felix Ament, and Bjorn Stevens
Earth Syst. Sci. Data, 13, 5545–5563, https://doi.org/10.5194/essd-13-5545-2021, https://doi.org/10.5194/essd-13-5545-2021, 2021
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The German research aircraft HALO took part in the research campaign EUREC4A in January and February 2020. The focus area was the tropical Atlantic east of the island of Barbados. We describe the characteristics of the 15 research flights, provide auxiliary information, derive combined cloud mask products from all instruments that observe clouds on board the aircraft, and provide code examples that help new users of the data to get started.
Sebastian Landwehr, Michele Volpi, F. Alexander Haumann, Charlotte M. Robinson, Iris Thurnherr, Valerio Ferracci, Andrea Baccarini, Jenny Thomas, Irina Gorodetskaya, Christian Tatzelt, Silvia Henning, Rob L. Modini, Heather J. Forrer, Yajuan Lin, Nicolas Cassar, Rafel Simó, Christel Hassler, Alireza Moallemi, Sarah E. Fawcett, Neil Harris, Ruth Airs, Marzieh H. Derkani, Alberto Alberello, Alessandro Toffoli, Gang Chen, Pablo Rodríguez-Ros, Marina Zamanillo, Pau Cortés-Greus, Lei Xue, Conor G. Bolas, Katherine C. Leonard, Fernando Perez-Cruz, David Walton, and Julia Schmale
Earth Syst. Dynam., 12, 1295–1369, https://doi.org/10.5194/esd-12-1295-2021, https://doi.org/10.5194/esd-12-1295-2021, 2021
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The Antarctic Circumnavigation Expedition surveyed a large number of variables describing the dynamic state of ocean and atmosphere, freshwater cycle, atmospheric chemistry, ocean biogeochemistry, and microbiology in the Southern Ocean. To reduce the dimensionality of the dataset, we apply a sparse principal component analysis and identify temporal patterns from diurnal to seasonal cycles, as well as geographical gradients and
hotspotsof interaction. Code and data are open access.
Markus Jesswein, Heiko Bozem, Hans-Christoph Lachnitt, Peter Hoor, Thomas Wagenhäuser, Timo Keber, Tanja Schuck, and Andreas Engel
Atmos. Chem. Phys., 21, 17225–17241, https://doi.org/10.5194/acp-21-17225-2021, https://doi.org/10.5194/acp-21-17225-2021, 2021
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This study presents and compares inorganic chlorine (Cly) derived from observations with the HALO research aircraft in the Antarctic late winter–early fall 2019 and the Arctic winter 2015–2016. Trend-corrected correlations from the Northern Hemisphere show excellent agreement with those from the Southern Hemisphere. After observation allocation inside and outside the vortex based on N2O measurements, results of the two campaigns reveal substantial differences in Cly within the respective vortex.
Markus Karrer, Axel Seifert, Davide Ori, and Stefan Kneifel
Atmos. Chem. Phys., 21, 17133–17166, https://doi.org/10.5194/acp-21-17133-2021, https://doi.org/10.5194/acp-21-17133-2021, 2021
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Modeling precipitation is of great relevance, e.g., for mitigating damage caused by extreme weather. A key component in accurate precipitation modeling is aggregation, i.e., sticking together of snowflakes. Simulating aggregation is difficult due to multiple parameters that are not well-known. Knowing how these parameters affect aggregation can help its simulation. We put new parameters in the model and select a combination of parameters with which the model can simulate observations better.
Larissa Lacher, Hans-Christian Clemen, Xiaoli Shen, Stephan Mertes, Martin Gysel-Beer, Alireza Moallemi, Martin Steinbacher, Stephan Henne, Harald Saathoff, Ottmar Möhler, Kristina Höhler, Thea Schiebel, Daniel Weber, Jann Schrod, Johannes Schneider, and Zamin A. Kanji
Atmos. Chem. Phys., 21, 16925–16953, https://doi.org/10.5194/acp-21-16925-2021, https://doi.org/10.5194/acp-21-16925-2021, 2021
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We investigate ice-nucleating particle properties at Jungfraujoch during the 2017 joint INUIT/CLACE field campaign, to improve the knowledge about those rare particles in a cloud-relevant environment. By quantifying ice-nucleating particles in parallel to single-particle mass spectrometry measurements, we find that mineral dust and aged sea spray particles are potential candidates for ice-nucleating particles. Our findings are supported by ice residual analysis and source region modeling.
Tiziana Bräuer, Christiane Voigt, Daniel Sauer, Stefan Kaufmann, Valerian Hahn, Monika Scheibe, Hans Schlager, Felix Huber, Patrick Le Clercq, Richard H. Moore, and Bruce E. Anderson
Atmos. Chem. Phys., 21, 16817–16826, https://doi.org/10.5194/acp-21-16817-2021, https://doi.org/10.5194/acp-21-16817-2021, 2021
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Over half of aviation climate impact is caused by contrails. Biofuels can reduce the ice crystal numbers in contrails and mitigate the climate impact. The experiment ECLIF II/NDMAX in 2018 assessed the effects of biofuels on contrails and aviation emissions. The NASA DC-8 aircraft performed measurements inside the contrail of the DLR A320. One reference fuel and two blends of the biofuel HEFA and kerosene are analysed. We find a max reduction of contrail ice numbers through biofuel use of 40 %.
Sebastian Düsing, Albert Ansmann, Holger Baars, Joel C. Corbin, Cyrielle Denjean, Martin Gysel-Beer, Thomas Müller, Laurent Poulain, Holger Siebert, Gerald Spindler, Thomas Tuch, Birgit Wehner, and Alfred Wiedensohler
Atmos. Chem. Phys., 21, 16745–16773, https://doi.org/10.5194/acp-21-16745-2021, https://doi.org/10.5194/acp-21-16745-2021, 2021
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The work deals with optical properties of aerosol particles in dried and atmospheric states. Based on two measurement campaigns in the rural background of central Europe, different measurement approaches were compared with each other, such as modeling based on Mie theory and direct in situ or remote sensing measurements. Among others, it was shown that the aerosol extinction-to-backscatter ratio is relative humidity dependent, and refinement with respect to the model input parameters is needed.
Geet George, Bjorn Stevens, Sandrine Bony, Robert Pincus, Chris Fairall, Hauke Schulz, Tobias Kölling, Quinn T. Kalen, Marcus Klingebiel, Heike Konow, Ashley Lundry, Marc Prange, and Jule Radtke
Earth Syst. Sci. Data, 13, 5253–5272, https://doi.org/10.5194/essd-13-5253-2021, https://doi.org/10.5194/essd-13-5253-2021, 2021
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Dropsondes measure atmospheric parameters such as temperature, pressure, humidity and horizontal winds. The EUREC4A field campaign deployed 1215 dropsondes during January–February 2020 in the north Atlantic trade-wind region in order to characterize the thermodynamic and the dynamic structure of the atmosphere, primarily at horizontal scales of ~ 200 km. We present JOANNE, the dataset that provides these dropsonde measurements and thereby a rich characterization of the trade-wind atmosphere.
Najin Kim, Yafang Cheng, Nan Ma, Mira L. Pöhlker, Thomas Klimach, Thomas F. Mentel, Ovid O. Krüger, Ulrich Pöschl, and Hang Su
Atmos. Meas. Tech., 14, 6991–7005, https://doi.org/10.5194/amt-14-6991-2021, https://doi.org/10.5194/amt-14-6991-2021, 2021
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A broad supersaturation scanning CCN (BS2-CCN) system, in which particles are exposed to a range of supersaturation simultaneously, can measure a broad range of CCN activity distribution with a high time resolution. We describe how the BS2-CCN system can be effectively calibrated and which factors can affect the calibration curve. Intercomparison experiments between typical DMA-CCN and BS2-CCN measurements to evaluate the BS2-CCN system showed high correlation and good agreement.
Sho Ohata, Makoto Koike, Atsushi Yoshida, Nobuhiro Moteki, Kouji Adachi, Naga Oshima, Hitoshi Matsui, Oliver Eppers, Heiko Bozem, Marco Zanatta, and Andreas B. Herber
Atmos. Chem. Phys., 21, 15861–15881, https://doi.org/10.5194/acp-21-15861-2021, https://doi.org/10.5194/acp-21-15861-2021, 2021
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Vertical profiles of black carbon (BC) in the Arctic were measured during the PAMARCMiP aircraft-based experiment in spring 2018 and compared with those observed during previous aircraft campaigns in 2008, 2010, and 2015. Their differences were explained primarily by the year-to-year variation of biomass burning activities in northern midlatitudes over Eurasia. Our observations provide a bases to evaluate numerical model simulations that assess the BC radiative effects in the Arctic spring.
Hossein Dadashazar, Majid Alipanah, Miguel Ricardo A. Hilario, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Andrew J. Peters, Amy Jo Scarino, Michael Shook, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Bo Zhang, Luke Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 21, 16121–16141, https://doi.org/10.5194/acp-21-16121-2021, https://doi.org/10.5194/acp-21-16121-2021, 2021
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This study investigates precipitation impacts on long-range transport of North American outflow over the western North Atlantic Ocean (WNAO). Results demonstrate that precipitation scavenging plays a significant role in modifying surface aerosol concentrations over the WNAO, especially in winter and spring due to large-scale scavenging processes. This study highlights how precipitation impacts surface aerosol properties with relevance for other marine regions vulnerable to continental outflow.
Gwendal Rivière, Meryl Wimmer, Philippe Arbogast, Jean-Marcel Piriou, Julien Delanoë, Carole Labadie, Quitterie Cazenave, and Jacques Pelon
Weather Clim. Dynam., 2, 1011–1031, https://doi.org/10.5194/wcd-2-1011-2021, https://doi.org/10.5194/wcd-2-1011-2021, 2021
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Inacurracies in representing processes occurring at spatial scales smaller than the grid scales of the weather forecast models are important sources of forecast errors. This is the case of deep convection representation in models with 10 km grid spacing. We performed simulations of a real extratropical cyclone using a model with different representations of deep convection. These forecasts lead to different behaviors in the ascending air masses of the cyclone and the jet stream aloft.
Yu-Wen Chen, Yi-Chun Chen, Charles C.-K. Chou, Hui-Ming Hung, Shih-Yu Chang, Lisa Eirenschmalz, Michael Lichtenstern, Helmut Ziereis, Hans Schlager, Greta Stratmann, Katharina Kaiser, Johannes Schneider, Stephan Borrmann, Florian Obersteiner, Eric Förster, Andreas Zahn, Wei-Nai Chen, Po-Hsiung Lin, Shuenn-Chin Chang, Maria Dolores Andrés Hernández, Pao-Kuan Wang, and John P. Burrows
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-788, https://doi.org/10.5194/acp-2021-788, 2021
Preprint withdrawn
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By presenting an approach using EMeRGe-Asia airborne field measurements and surface observations, this study shows that the fraction of OH reactivity due to SO2-OH reaction has a significant correlation with the sulfate concentration. Approximately 30 % of sulfate is produced by SO2-OH reaction. Our results underline the importance of SO2-OH gas-phase oxidation in sulfate formation, and demonstrate that the method can be applied to other regions and under different meteorological conditions.
Kevin Ohneiser, Albert Ansmann, Alexandra Chudnovsky, Ronny Engelmann, Christoph Ritter, Igor Veselovskii, Holger Baars, Henriette Gebauer, Hannes Griesche, Martin Radenz, Julian Hofer, Dietrich Althausen, Sandro Dahlke, and Marion Maturilli
Atmos. Chem. Phys., 21, 15783–15808, https://doi.org/10.5194/acp-21-15783-2021, https://doi.org/10.5194/acp-21-15783-2021, 2021
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The highlight of the lidar measurements during the 1-year MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition of the German icebreaker Polarstern (October 2019–October 2020) was the detection of a persistent, 10 km deep Siberian wildfire smoke layer in the upper troposphere and lower stratosphere (UTLS) from about 7–8 km to 17–18 km height that could potentially have impacted the record-breaking ozone depletion over the Arctic in the spring of 2020.
Jonas Hamperl, Clément Capitaine, Jean-Baptiste Dherbecourt, Myriam Raybaut, Patrick Chazette, Julien Totems, Bruno Grouiez, Laurence Régalia, Rosa Santagata, Corinne Evesque, Jean-Michel Melkonian, Antoine Godard, Andrew Seidl, Harald Sodemann, and Cyrille Flamant
Atmos. Meas. Tech., 14, 6675–6693, https://doi.org/10.5194/amt-14-6675-2021, https://doi.org/10.5194/amt-14-6675-2021, 2021
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Laser active remote sensing of tropospheric water vapor is a promising technology for enhancing our understanding of processes governing the global hydrological cycle. We investigate the potential of a ground-based lidar to monitor the main water vapor isotopes at high spatio-temporal resolutions in the lower troposphere. Using a realistic end-to-end simulator, we show that high-precision measurements can be achieved within a range of 1.5 km, in mid-latitude or tropical environments.
Christoph Mahnke, Ralf Weigel, Francesco Cairo, Jean-Paul Vernier, Armin Afchine, Martina Krämer, Valentin Mitev, Renaud Matthey, Silvia Viciani, Francesco D'Amato, Felix Ploeger, Terry Deshler, and Stephan Borrmann
Atmos. Chem. Phys., 21, 15259–15282, https://doi.org/10.5194/acp-21-15259-2021, https://doi.org/10.5194/acp-21-15259-2021, 2021
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In 2017, in situ aerosol measurements were conducted aboard the M55 Geophysica in the Asian monsoon region. The vertical particle mixing ratio profiles show a distinct layer (15–18.5 km), the Asian tropopause aerosol layer (ATAL). The backscatter ratio (BR) was calculated based on the aerosol size distributions and compared with the BRs detected by a backscatter probe and a lidar aboard M55, and by the CALIOP lidar. All four methods show enhanced BRs in the ATAL altitude range (max. at 17.5 km).
Qiang Li and Silke Groß
Atmos. Chem. Phys., 21, 14573–14590, https://doi.org/10.5194/acp-21-14573-2021, https://doi.org/10.5194/acp-21-14573-2021, 2021
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Aircraft emit exhaust gases and particles directly into the atmosphere, which may contribute to climate change. We present a significant reduction in the occurrence rate and particle linear depolarization ratio of cirrus clouds based on the analysis of measurements with the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) satellite during COVID-19 when air traffic was significantly reduced. The findings imply that these clouds formed with less influence from aviation.
Ramon Campos Braga, Daniel Rosenfeld, Ovid O. Krüger, Barbara Ervens, Bruna A. Holanda, Manfred Wendisch, Trismono Krisna, Ulrich Pöschl, Meinrat O. Andreae, Christiane Voigt, and Mira L. Pöhlker
Atmos. Chem. Phys., 21, 14079–14088, https://doi.org/10.5194/acp-21-14079-2021, https://doi.org/10.5194/acp-21-14079-2021, 2021
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Quantifying the precipitation within clouds is crucial for our understanding of the Earth's hydrological cycle. Using in situ measurements of cloud and rain properties over the Amazon Basin and Atlantic Ocean, we show here a linear relationship between the effective radius (re) and precipitation water content near the tops of convective clouds for different pollution states and temperature levels. Our results emphasize the role of re to determine both initiation and amount of precipitation.
Bernd Schalge, Gabriele Baroni, Barbara Haese, Daniel Erdal, Gernot Geppert, Pablo Saavedra, Vincent Haefliger, Harry Vereecken, Sabine Attinger, Harald Kunstmann, Olaf A. Cirpka, Felix Ament, Stefan Kollet, Insa Neuweiler, Harrie-Jan Hendricks Franssen, and Clemens Simmer
Earth Syst. Sci. Data, 13, 4437–4464, https://doi.org/10.5194/essd-13-4437-2021, https://doi.org/10.5194/essd-13-4437-2021, 2021
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In this study, a 9-year simulation of complete model output of a coupled atmosphere–land-surface–subsurface model on the catchment scale is discussed. We used the Neckar catchment in SW Germany as the basis of this simulation. Since the dataset includes the full model output, it is not only possible to investigate model behavior and interactions between the component models but also use it as a virtual truth for comparison of, for example, data assimilation experiments.
Ralf Weigel, Christoph Mahnke, Manuel Baumgartner, Martina Krämer, Peter Spichtinger, Nicole Spelten, Armin Afchine, Christian Rolf, Silvia Viciani, Francesco D'Amato, Holger Tost, and Stephan Borrmann
Atmos. Chem. Phys., 21, 13455–13481, https://doi.org/10.5194/acp-21-13455-2021, https://doi.org/10.5194/acp-21-13455-2021, 2021
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In July and August 2017, the StratoClim mission took place in Nepal with eight flights of the M-55 Geophysica at up to 20 km in the Asian monsoon anticyclone. New particle formation (NPF) next to cloud ice was detected in situ by abundant nucleation-mode aerosols (> 6 nm) along with ice particles (> 3 µm). NPF was observed mainly below the tropopause, down to 15 % being non-volatile residues. Observed intra-cloud NPF indicates its importance for the composition in the tropical tropopause layer.
Ronny Engelmann, Albert Ansmann, Kevin Ohneiser, Hannes Griesche, Martin Radenz, Julian Hofer, Dietrich Althausen, Sandro Dahlke, Marion Maturilli, Igor Veselovskii, Cristofer Jimenez, Robert Wiesen, Holger Baars, Johannes Bühl, Henriette Gebauer, Moritz Haarig, Patric Seifert, Ulla Wandinger, and Andreas Macke
Atmos. Chem. Phys., 21, 13397–13423, https://doi.org/10.5194/acp-21-13397-2021, https://doi.org/10.5194/acp-21-13397-2021, 2021
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A Raman lidar was operated aboard the icebreaker Polarstern during MOSAiC and monitored aerosol and cloud layers in the central Arctic up to 30 km height. The article provides an overview of the spectrum of aerosol profiling observations and shows aerosol–cloud interaction studies for liquid-water and ice clouds. A highlight was the detection of a 10 km deep wildfire smoke layer over the North Pole up to 17 km height from the fire season of 2019, which persisted over the whole winter period.
Bjorn Stevens, Sandrine Bony, David Farrell, Felix Ament, Alan Blyth, Christopher Fairall, Johannes Karstensen, Patricia K. Quinn, Sabrina Speich, Claudia Acquistapace, Franziska Aemisegger, Anna Lea Albright, Hugo Bellenger, Eberhard Bodenschatz, Kathy-Ann Caesar, Rebecca Chewitt-Lucas, Gijs de Boer, Julien Delanoë, Leif Denby, Florian Ewald, Benjamin Fildier, Marvin Forde, Geet George, Silke Gross, Martin Hagen, Andrea Hausold, Karen J. Heywood, Lutz Hirsch, Marek Jacob, Friedhelm Jansen, Stefan Kinne, Daniel Klocke, Tobias Kölling, Heike Konow, Marie Lothon, Wiebke Mohr, Ann Kristin Naumann, Louise Nuijens, Léa Olivier, Robert Pincus, Mira Pöhlker, Gilles Reverdin, Gregory Roberts, Sabrina Schnitt, Hauke Schulz, A. Pier Siebesma, Claudia Christine Stephan, Peter Sullivan, Ludovic Touzé-Peiffer, Jessica Vial, Raphaela Vogel, Paquita Zuidema, Nicola Alexander, Lyndon Alves, Sophian Arixi, Hamish Asmath, Gholamhossein Bagheri, Katharina Baier, Adriana Bailey, Dariusz Baranowski, Alexandre Baron, Sébastien Barrau, Paul A. Barrett, Frédéric Batier, Andreas Behrendt, Arne Bendinger, Florent Beucher, Sebastien Bigorre, Edmund Blades, Peter Blossey, Olivier Bock, Steven Böing, Pierre Bosser, Denis Bourras, Pascale Bouruet-Aubertot, Keith Bower, Pierre Branellec, Hubert Branger, Michal Brennek, Alan Brewer, Pierre-Etienne Brilouet, Björn Brügmann, Stefan A. Buehler, Elmo Burke, Ralph Burton, Radiance Calmer, Jean-Christophe Canonici, Xavier Carton, Gregory Cato Jr., Jude Andre Charles, Patrick Chazette, Yanxu Chen, Michal T. Chilinski, Thomas Choularton, Patrick Chuang, Shamal Clarke, Hugh Coe, Céline Cornet, Pierre Coutris, Fleur Couvreux, Susanne Crewell, Timothy Cronin, Zhiqiang Cui, Yannis Cuypers, Alton Daley, Gillian M. Damerell, Thibaut Dauhut, Hartwig Deneke, Jean-Philippe Desbios, Steffen Dörner, Sebastian Donner, Vincent Douet, Kyla Drushka, Marina Dütsch, André Ehrlich, Kerry Emanuel, Alexandros Emmanouilidis, Jean-Claude Etienne, Sheryl Etienne-Leblanc, Ghislain Faure, Graham Feingold, Luca Ferrero, Andreas Fix, Cyrille Flamant, Piotr Jacek Flatau, Gregory R. Foltz, Linda Forster, Iulian Furtuna, Alan Gadian, Joseph Galewsky, Martin Gallagher, Peter Gallimore, Cassandra Gaston, Chelle Gentemann, Nicolas Geyskens, Andreas Giez, John Gollop, Isabelle Gouirand, Christophe Gourbeyre, Dörte de Graaf, Geiske E. de Groot, Robert Grosz, Johannes Güttler, Manuel Gutleben, Kashawn Hall, George Harris, Kevin C. Helfer, Dean Henze, Calvert Herbert, Bruna Holanda, Antonio Ibanez-Landeta, Janet Intrieri, Suneil Iyer, Fabrice Julien, Heike Kalesse, Jan Kazil, Alexander Kellman, Abiel T. Kidane, Ulrike Kirchner, Marcus Klingebiel, Mareike Körner, Leslie Ann Kremper, Jan Kretzschmar, Ovid Krüger, Wojciech Kumala, Armin Kurz, Pierre L'Hégaret, Matthieu Labaste, Tom Lachlan-Cope, Arlene Laing, Peter Landschützer, Theresa Lang, Diego Lange, Ingo Lange, Clément Laplace, Gauke Lavik, Rémi Laxenaire, Caroline Le Bihan, Mason Leandro, Nathalie Lefevre, Marius Lena, Donald Lenschow, Qiang Li, Gary Lloyd, Sebastian Los, Niccolò Losi, Oscar Lovell, Christopher Luneau, Przemyslaw Makuch, Szymon Malinowski, Gaston Manta, Eleni Marinou, Nicholas Marsden, Sebastien Masson, Nicolas Maury, Bernhard Mayer, Margarette Mayers-Als, Christophe Mazel, Wayne McGeary, James C. McWilliams, Mario Mech, Melina Mehlmann, Agostino Niyonkuru Meroni, Theresa Mieslinger, Andreas Minikin, Peter Minnett, Gregor Möller, Yanmichel Morfa Avalos, Caroline Muller, Ionela Musat, Anna Napoli, Almuth Neuberger, Christophe Noisel, David Noone, Freja Nordsiek, Jakub L. Nowak, Lothar Oswald, Douglas J. Parker, Carolyn Peck, Renaud Person, Miriam Philippi, Albert Plueddemann, Christopher Pöhlker, Veronika Pörtge, Ulrich Pöschl, Lawrence Pologne, Michał Posyniak, Marc Prange, Estefanía Quiñones Meléndez, Jule Radtke, Karim Ramage, Jens Reimann, Lionel Renault, Klaus Reus, Ashford Reyes, Joachim Ribbe, Maximilian Ringel, Markus Ritschel, Cesar B. Rocha, Nicolas Rochetin, Johannes Röttenbacher, Callum Rollo, Haley Royer, Pauline Sadoulet, Leo Saffin, Sanola Sandiford, Irina Sandu, Michael Schäfer, Vera Schemann, Imke Schirmacher, Oliver Schlenczek, Jerome Schmidt, Marcel Schröder, Alfons Schwarzenboeck, Andrea Sealy, Christoph J. Senff, Ilya Serikov, Samkeyat Shohan, Elizabeth Siddle, Alexander Smirnov, Florian Späth, Branden Spooner, M. Katharina Stolla, Wojciech Szkółka, Simon P. de Szoeke, Stéphane Tarot, Eleni Tetoni, Elizabeth Thompson, Jim Thomson, Lorenzo Tomassini, Julien Totems, Alma Anna Ubele, Leonie Villiger, Jan von Arx, Thomas Wagner, Andi Walther, Ben Webber, Manfred Wendisch, Shanice Whitehall, Anton Wiltshire, Allison A. Wing, Martin Wirth, Jonathan Wiskandt, Kevin Wolf, Ludwig Worbes, Ethan Wright, Volker Wulfmeyer, Shanea Young, Chidong Zhang, Dongxiao Zhang, Florian Ziemen, Tobias Zinner, and Martin Zöger
Earth Syst. Sci. Data, 13, 4067–4119, https://doi.org/10.5194/essd-13-4067-2021, https://doi.org/10.5194/essd-13-4067-2021, 2021
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The EUREC4A field campaign, designed to test hypothesized mechanisms by which clouds respond to warming and benchmark next-generation Earth-system models, is presented. EUREC4A comprised roughly 5 weeks of measurements in the downstream winter trades of the North Atlantic – eastward and southeastward of Barbados. It was the first campaign that attempted to characterize the full range of processes and scales influencing trade wind clouds.
Thomas Krumpen, Luisa von Albedyll, Helge F. Goessling, Stefan Hendricks, Bennet Juhls, Gunnar Spreen, Sascha Willmes, H. Jakob Belter, Klaus Dethloff, Christian Haas, Lars Kaleschke, Christian Katlein, Xiangshan Tian-Kunze, Robert Ricker, Philip Rostosky, Janna Rückert, Suman Singha, and Julia Sokolova
The Cryosphere, 15, 3897–3920, https://doi.org/10.5194/tc-15-3897-2021, https://doi.org/10.5194/tc-15-3897-2021, 2021
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We use satellite data records collected along the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) drift to categorize ice conditions that shaped and characterized the floe and surroundings during the expedition. A comparison with previous years is made whenever possible. The aim of this analysis is to provide a basis and reference for subsequent research in the six main research areas of atmosphere, ocean, sea ice, biogeochemistry, remote sensing and ecology.
Bin Cheng, Yubing Cheng, Timo Vihma, Anna Kontu, Fei Zheng, Juha Lemmetyinen, Yubao Qiu, and Jouni Pulliainen
Earth Syst. Sci. Data, 13, 3967–3978, https://doi.org/10.5194/essd-13-3967-2021, https://doi.org/10.5194/essd-13-3967-2021, 2021
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Climate change strongly impacts the Arctic, with clear signs of higher air temperature and more precipitation. A sustainable observation programme has been carried out in Lake Orajärvi in Sodankylä, Finland. The high-quality air–snow–ice–water temperature profiles have been measured every winter since 2009. The data can be used to investigate the lake ice surface heat balance and the role of snow in lake ice mass balance and parameterization of snow-to-ice transformation in snow/ice models.
Ralf Weigel, Christoph Mahnke, Manuel Baumgartner, Antonis Dragoneas, Bärbel Vogel, Felix Ploeger, Silvia Viciani, Francesco D'Amato, Silvia Bucci, Bernard Legras, Beiping Luo, and Stephan Borrmann
Atmos. Chem. Phys., 21, 11689–11722, https://doi.org/10.5194/acp-21-11689-2021, https://doi.org/10.5194/acp-21-11689-2021, 2021
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In July and August 2017, eight StratoClim mission flights of the Geophysica reached up to 20 km in the Asian monsoon anticyclone. New particle formation (NPF) was identified in situ by abundant nucleation-mode aerosols (6–15 nm in diameter) with mixing ratios of up to 50 000 mg−1. NPF occurred most frequently at 12–16 km with fractions of non-volatile residues of down to 15 %. Abundance and productivity of observed NPF indicate its ability to promote the Asian tropopause aerosol layer.
Mira L. Pöhlker, Minghui Zhang, Ramon Campos Braga, Ovid O. Krüger, Ulrich Pöschl, and Barbara Ervens
Atmos. Chem. Phys., 21, 11723–11740, https://doi.org/10.5194/acp-21-11723-2021, https://doi.org/10.5194/acp-21-11723-2021, 2021
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Clouds cool our atmosphere. The role of small aerosol particles in affecting them represents one of the largest uncertainties in current estimates of climate change. Traditionally it is assumed that cloud droplets only form particles of diameters ~ 100 nm (
accumulation mode). Previous studies suggest that this can also occur in smaller particles (
Aitken mode). Our study provides a general framework to estimate under which aerosol and cloud conditions Aitken mode particles affect clouds.
Yongbiao Weng, Aina Johannessen, and Harald Sodemann
Weather Clim. Dynam., 2, 713–737, https://doi.org/10.5194/wcd-2-713-2021, https://doi.org/10.5194/wcd-2-713-2021, 2021
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High-resolution measurements of stable isotopes in near-surface vapour and precipitation show a
W-shaped evolution during a 24 h land-falling atmospheric river event in southern Norway. We distinguish contributions from below-cloud processes, weather system characteristics, and moisture source conditions during different stages of the event. Rayleigh distillation models need to be expanded by additional processes to accurately predict isotopes in surface precipitation from stratiform clouds.
Markus Hartmann, Xianda Gong, Simonas Kecorius, Manuela van Pinxteren, Teresa Vogl, André Welti, Heike Wex, Sebastian Zeppenfeld, Hartmut Herrmann, Alfred Wiedensohler, and Frank Stratmann
Atmos. Chem. Phys., 21, 11613–11636, https://doi.org/10.5194/acp-21-11613-2021, https://doi.org/10.5194/acp-21-11613-2021, 2021
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Ice-nucleating particles (INPs) are not well characterized in the Arctic despite their importance for the Arctic energy budget. Little is known about their nature (mineral or biological) and sources (terrestrial or marine, long-range transport or local). We find indications that, at the beginning of the melt season, a local, biogenic, probably marine source is likely, but significant enrichment of INPs has to take place from the ocean to the aerosol phase.
Benjamin Männel, Florian Zus, Galina Dick, Susanne Glaser, Maximilian Semmling, Kyriakos Balidakis, Jens Wickert, Marion Maturilli, Sandro Dahlke, and Harald Schuh
Atmos. Meas. Tech., 14, 5127–5138, https://doi.org/10.5194/amt-14-5127-2021, https://doi.org/10.5194/amt-14-5127-2021, 2021
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Within the MOSAiC expedition, GNSS was used to monitor variations in atmospheric water vapor. Based on 15 months of continuously tracked data, coordinates and hourly zenith total delays (ZTDs) were determined using kinematic precise point positioning. The derived ZTD values agree within few millimeters with ERA5 and terrestrial GNSS and VLBI stations. The derived integrated water vapor corresponds to the frequently launched radiosondes (0.08 ± 0.04 kg m−2, rms of the differences of 1.47 kg m−2).
Florian Ewald, Silke Groß, Martin Wirth, Julien Delanoë, Stuart Fox, and Bernhard Mayer
Atmos. Meas. Tech., 14, 5029–5047, https://doi.org/10.5194/amt-14-5029-2021, https://doi.org/10.5194/amt-14-5029-2021, 2021
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In this study, we show how solar radiance observations can be used to validate and further constrain ice cloud microphysics retrieved from the synergy of radar–lidar measurements. Since most radar–lidar retrievals rely on a global assumption about the ice particle shape, ice water content and particle size biases are to be expected in individual cloud regimes. In this work, we identify and correct these biases by reconciling simulated and measured solar radiation reflected from these clouds.
Patrick Chazette, Cyrille Flamant, Harald Sodemann, Julien Totems, Anne Monod, Elsa Dieudonné, Alexandre Baron, Andrew Seidl, Hans Christian Steen-Larsen, Pascal Doira, Amandine Durand, and Sylvain Ravier
Atmos. Chem. Phys., 21, 10911–10937, https://doi.org/10.5194/acp-21-10911-2021, https://doi.org/10.5194/acp-21-10911-2021, 2021
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To gain understanding on the vertical structure of atmospheric water vapour above mountain lakes and to assess its link to the isotopic composition of the lake water and small-scale dynamics, the L-WAIVE field campaign was conducted in the Annecy valley in the French Alps in June 2019. Based on a synergy between ground-based, boat-borne, and airborne measuring platforms, significant gradients of isotopic content have been revealed at the transitions to the lake and to the free troposphere.
Jakub L. Nowak, Holger Siebert, Kai-Erik Szodry, and Szymon P. Malinowski
Atmos. Chem. Phys., 21, 10965–10991, https://doi.org/10.5194/acp-21-10965-2021, https://doi.org/10.5194/acp-21-10965-2021, 2021
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Turbulence properties in two cases of a marine stratocumulus-topped boundary layer have been compared using high-resolution helicopter-borne in situ measurements. In the coupled one, small-scale turbulence was close to isotropic and reasonably followed inertial range scaling according to Kolmogorov theory. In the decoupled one, turbulence was more anisotropic and the scaling deviated from theory. This was more pronounced in the cloud and subcloud layers in comparison to the surface mixed layer.
Jun Inoue, Yutaka Tobo, Kazutoshi Sato, Fumikazu Taketani, and Marion Maturilli
Atmos. Meas. Tech., 14, 4971–4987, https://doi.org/10.5194/amt-14-4971-2021, https://doi.org/10.5194/amt-14-4971-2021, 2021
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A cloud particle sensor (CPS) sonde is an observing system to obtain the signals of the phase, size, and the number of cloud particles. Based on the field experiments in the Arctic regions and numerical experiments, we proposed a method to correct the CPS sonde data and found that the CPS sonde system can appropriately observe the liquid cloud if our correction method is applied.
Alistair Bell, Pauline Martinet, Olivier Caumont, Benoît Vié, Julien Delanoë, Jean-Charles Dupont, and Mary Borderies
Atmos. Meas. Tech., 14, 4929–4946, https://doi.org/10.5194/amt-14-4929-2021, https://doi.org/10.5194/amt-14-4929-2021, 2021
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This paper presents work towards making retrievals on the liquid water content in fog and low clouds. Future retrievals will rely on a radar simulator and high-resolution forecast. In this work, real observations are used to assess the errors associated with the simulator and forecast. A selection method to reduce errors associated with the forecast is proposed. It is concluded that the distribution of errors matches the requirements for future retrievals.
Pierre-Etienne Brilouet, Marie Lothon, Jean-Claude Etienne, Pascal Richard, Sandrine Bony, Julien Lernoult, Hubert Bellec, Gilles Vergez, Thierry Perrin, Julien Delanoë, Tetyana Jiang, Frédéric Pouvesle, Claude Lainard, Michel Cluzeau, Laurent Guiraud, Patrice Medina, and Theotime Charoy
Earth Syst. Sci. Data, 13, 3379–3398, https://doi.org/10.5194/essd-13-3379-2021, https://doi.org/10.5194/essd-13-3379-2021, 2021
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During the EUREC4A field experiment that took place over the tropical Atlantic Ocean east of Barbados, the French ATR 42 environment research aircraft of SAFIRE aimed to characterize the shallow cloud properties near cloud base and the turbulent structure of the subcloud layer. The high-frequency measurements of wind, temperature and humidity as well as their translation in terms of turbulent fluctuations, turbulent moments and characteristic length scales of turbulence are presented.
Hossein Dadashazar, David Painemal, Majid Alipanah, Michael Brunke, Seethala Chellappan, Andrea F. Corral, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Claire Robinson, Amy Jo Scarino, Michael Shook, Kenneth Sinclair, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Xubin Zeng, Luke Ziemba, Paquita Zuidema, and Armin Sorooshian
Atmos. Chem. Phys., 21, 10499–10526, https://doi.org/10.5194/acp-21-10499-2021, https://doi.org/10.5194/acp-21-10499-2021, 2021
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This study investigates the seasonal cycle of cloud drop number concentration (Nd) over the western North Atlantic Ocean (WNAO) using multiple datasets. Reasons for the puzzling discrepancy between the seasonal cycles of Nd and aerosol concentration were identified. Results indicate that Nd is highest in winter (when aerosol proxy values are often lowest) due to conditions both linked to cold-air outbreaks and that promote greater droplet activation.
Susanne Crewell, Kerstin Ebell, Patrick Konjari, Mario Mech, Tatiana Nomokonova, Ana Radovan, David Strack, Arantxa M. Triana-Gómez, Stefan Noël, Raul Scarlat, Gunnar Spreen, Marion Maturilli, Annette Rinke, Irina Gorodetskaya, Carolina Viceto, Thomas August, and Marc Schröder
Atmos. Meas. Tech., 14, 4829–4856, https://doi.org/10.5194/amt-14-4829-2021, https://doi.org/10.5194/amt-14-4829-2021, 2021
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Water vapor (WV) is an important variable in the climate system. Satellite measurements are thus crucial to characterize the spatial and temporal variability in WV and how it changed over time. In particular with respect to the observed strong Arctic warming, the role of WV still needs to be better understood. However, as shown in this paper, a detailed understanding is still hampered by large uncertainties in the various satellite WV products, showing the need for improved methods to derive WV.
Hyunju Jung, Ann Kristin Naumann, and Bjorn Stevens
Atmos. Chem. Phys., 21, 10337–10345, https://doi.org/10.5194/acp-21-10337-2021, https://doi.org/10.5194/acp-21-10337-2021, 2021
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We analyze the behavior of organized convection in a large-scale flow by imposing a mean flow to idealized simulations. In the mean flow, organized convection initially propagates slower than the mean wind speed and becomes stationary. The initial upstream and downstream difference in surface fluxes becomes symmetric as the surface momentum flux acts as a drag, resulting in the stationarity. Meanwhile, the surface enthalpy flux has a minor role in the propagation of the convection.
Anja Rösel, Sinead Louise Farrell, Vishnu Nandan, Jaqueline Richter-Menge, Gunnar Spreen, Dmitry V. Divine, Adam Steer, Jean-Charles Gallet, and Sebastian Gerland
The Cryosphere, 15, 2819–2833, https://doi.org/10.5194/tc-15-2819-2021, https://doi.org/10.5194/tc-15-2819-2021, 2021
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Recent observations in the Arctic suggest a significant shift towards a snow–ice regime caused by deep snow on thin sea ice which may result in a flooding of the snowpack. These conditions cause the brine wicking and saturation of the basal snow layers which lead to a subsequent underestimation of snow depth from snow radar mesurements. As a consequence the calculated sea ice thickness will be biased towards higher values.
Nina Črnivec and Bernhard Mayer
Geosci. Model Dev., 14, 3663–3682, https://doi.org/10.5194/gmd-14-3663-2021, https://doi.org/10.5194/gmd-14-3663-2021, 2021
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This study aims to advance the cloud–radiation interplay treatment in global weather and climate prediction, focusing on cloud horizontal inhomogeneity misrepresentation. We explore the potential of the Tripleclouds method for diverse cloud types, namely the stratocumulus, cirrus and cumulonimbus. The validity of global cloud variability estimate with various condensate distribution assumptions is assessed. Optimizations for overcast and extremely heterogeneous cloudiness are further endorsed.
Linlu Mei, Vladimir Rozanov, Evelyn Jäkel, Xiao Cheng, Marco Vountas, and John P. Burrows
The Cryosphere, 15, 2781–2802, https://doi.org/10.5194/tc-15-2781-2021, https://doi.org/10.5194/tc-15-2781-2021, 2021
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This paper presents a new snow property retrieval algorithm from satellite observations. This is Part 2 of two companion papers and shows the results and validation. The paper performs the new retrieval algorithm on the Sea and Land
Surface Temperature Radiometer (SLSTR) instrument and compares the retrieved snow properties with ground-based measurements, aircraft measurements and other satellite products.
Marco Zanatta, Andreas Herber, Zsófia Jurányi, Oliver Eppers, Johannes Schneider, and Joshua P. Schwarz
Atmos. Chem. Phys., 21, 9329–9342, https://doi.org/10.5194/acp-21-9329-2021, https://doi.org/10.5194/acp-21-9329-2021, 2021
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Saline snow samples were collected from the sea ice in the Fram Strait. Laboratory experiments revealed that sea salt can bias the quantification of black carbon with a laser-induced incandescence technique. The maximum underestimation was quantified to reach values of 80 %–90 %. This salt-induced interference is reported here for the first time and should be considered in future studies aiming to quantify black carbon in snow in marine environments.
Olivier Bock, Pierre Bosser, Cyrille Flamant, Erik Doerflinger, Friedhelm Jansen, Romain Fages, Sandrine Bony, and Sabrina Schnitt
Earth Syst. Sci. Data, 13, 2407–2436, https://doi.org/10.5194/essd-13-2407-2021, https://doi.org/10.5194/essd-13-2407-2021, 2021
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Measurements from a network of Global Navigation Satellite System (GNSS) receivers operated from the eastern Caribbean islands are used to monitor the total water vapour content in the atmosphere during the EUREC4A field campaign. These data help describe the moisture environment of mesoscale cloud patterns in the trade winds with high temporal sampling. They are also useful to assess the accuracy of collocated radiosonde measurements and numerical weather model reanalyses.
Ulrich Schumann, Ian Poll, Roger Teoh, Rainer Koelle, Enrico Spinielli, Jarlath Molloy, George S. Koudis, Robert Baumann, Luca Bugliaro, Marc Stettler, and Christiane Voigt
Atmos. Chem. Phys., 21, 7429–7450, https://doi.org/10.5194/acp-21-7429-2021, https://doi.org/10.5194/acp-21-7429-2021, 2021
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The roughly 70 % reduction of air traffic during the COVID-19 pandemic from March–August 2020 compared to 2019 provides a test case for the relationship between air traffic density, contrails, and their radiative forcing of climate change. This paper investigates the induced traffic and contrail changes in a model study. Besides strong weather changes, the model results indicate aviation-induced cirrus and top-of-the-atmosphere irradiance changes, which can be tested with observations.
Eugene F. Mikhailov, Mira L. Pöhlker, Kathrin Reinmuth-Selzle, Sergey S. Vlasenko, Ovid O. Krüger, Janine Fröhlich-Nowoisky, Christopher Pöhlker, Olga A. Ivanova, Alexey A. Kiselev, Leslie A. Kremper, and Ulrich Pöschl
Atmos. Chem. Phys., 21, 6999–7022, https://doi.org/10.5194/acp-21-6999-2021, https://doi.org/10.5194/acp-21-6999-2021, 2021
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Subpollen particles are a relatively new subset of atmospheric aerosol particles. When pollen grains rupture, they release cytoplasmic fragments known as subpollen particles (SPPs). We found that SPPs, containing a broad spectrum of biopolymers and hydrocarbons, exhibit abnormally high water uptake. This effect may influence the life cycle of SPPs and the related direct and indirect impacts on radiation budget as well as reinforce their allergic potential.
Franziska Köllner, Johannes Schneider, Megan D. Willis, Hannes Schulz, Daniel Kunkel, Heiko Bozem, Peter Hoor, Thomas Klimach, Frank Helleis, Julia Burkart, W. Richard Leaitch, Amir A. Aliabadi, Jonathan P. D. Abbatt, Andreas B. Herber, and Stephan Borrmann
Atmos. Chem. Phys., 21, 6509–6539, https://doi.org/10.5194/acp-21-6509-2021, https://doi.org/10.5194/acp-21-6509-2021, 2021
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We present in situ observations of vertically resolved particle chemical composition in the summertime Arctic lower troposphere. Our analysis demonstrates the strong vertical contrast between particle properties within the boundary layer and aloft. Emissions from vegetation fires and anthropogenic sources in northern Canada, Europe, and East Asia influenced particle composition in the free troposphere. Organics detected in Arctic aerosol particles can partly be identified as dicarboxylic acids.
Patricia K. Quinn, Elizabeth J. Thompson, Derek J. Coffman, Sunil Baidar, Ludovic Bariteau, Timothy S. Bates, Sebastien Bigorre, Alan Brewer, Gijs de Boer, Simon P. de Szoeke, Kyla Drushka, Gregory R. Foltz, Janet Intrieri, Suneil Iyer, Chris W. Fairall, Cassandra J. Gaston, Friedhelm Jansen, James E. Johnson, Ovid O. Krüger, Richard D. Marchbanks, Kenneth P. Moran, David Noone, Sergio Pezoa, Robert Pincus, Albert J. Plueddemann, Mira L. Pöhlker, Ulrich Pöschl, Estefania Quinones Melendez, Haley M. Royer, Malgorzata Szczodrak, Jim Thomson, Lucia M. Upchurch, Chidong Zhang, Dongxiao Zhang, and Paquita Zuidema
Earth Syst. Sci. Data, 13, 1759–1790, https://doi.org/10.5194/essd-13-1759-2021, https://doi.org/10.5194/essd-13-1759-2021, 2021
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ATOMIC took place in the northwestern tropical Atlantic during January and February of 2020 to gather information on shallow atmospheric convection, the effects of aerosols and clouds on the ocean surface energy budget, and mesoscale oceanic processes. Measurements made from the NOAA RV Ronald H. Brown and assets it deployed (instrumented mooring and uncrewed seagoing vehicles) are described herein to advance widespread use of the data by the ATOMIC and broader research communities.
Ulrike Egerer, André Ehrlich, Matthias Gottschalk, Hannes Griesche, Roel A. J. Neggers, Holger Siebert, and Manfred Wendisch
Atmos. Chem. Phys., 21, 6347–6364, https://doi.org/10.5194/acp-21-6347-2021, https://doi.org/10.5194/acp-21-6347-2021, 2021
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This paper describes a case study of a three-day period with a persistent humidity inversion above a mixed-phase cloud layer in the Arctic. It is based on measurements with a tethered balloon, complemented with results from a dedicated high-resolution large-eddy simulation. Both methods show that the humidity layer acts to provide moisture to the cloud layer through downward turbulent transport. This supply of additional moisture can contribute to the persistence of Arctic clouds.
Johannes Stapf, André Ehrlich, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-279, https://doi.org/10.5194/acp-2021-279, 2021
Preprint withdrawn
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Airborne observations of the surface radiative energy budget in the marginal sea ice zone (the region between open ocean and closed sea ice) are presented. Atmospheric thermodynamic profiles and surface properties change on small spatial scales in this area and influence the impact of clouds on the radiative energy budget. The radiation budget over sea ice is compared to available studies in the Arctic and the influence of cold air outbreaks and warm air intrusions is illustrated.
Iris Thurnherr, Katharina Hartmuth, Lukas Jansing, Josué Gehring, Maxi Boettcher, Irina Gorodetskaya, Martin Werner, Heini Wernli, and Franziska Aemisegger
Weather Clim. Dynam., 2, 331–357, https://doi.org/10.5194/wcd-2-331-2021, https://doi.org/10.5194/wcd-2-331-2021, 2021
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Extratropical cyclones are important for the transport of moisture from low to high latitudes. In this study, we investigate how the isotopic composition of water vapour is affected by horizontal temperature advection associated with extratropical cyclones using measurements and modelling. It is shown that air–sea moisture fluxes induced by this horizontal temperature advection lead to the strong variability observed in the isotopic composition of water vapour in the marine boundary layer.
Sebastian Wolff, Gerhard Ehret, Christoph Kiemle, Axel Amediek, Mathieu Quatrevalet, Martin Wirth, and Andreas Fix
Atmos. Meas. Tech., 14, 2717–2736, https://doi.org/10.5194/amt-14-2717-2021, https://doi.org/10.5194/amt-14-2717-2021, 2021
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We report on CO2 emissions of a coal-fired power plant derived from flight measurements performed with the IPDA lidar CHARM-F during the CoMet campaign in spring 2018. Despite the results being in broad agreement with reported emissions, we observe strong variations between successive flyovers. Using a high-resolution large eddy simulation, we identify strong atmospheric turbulence as the cause for the variations and recommend more favorable measurement conditions for future campaign planning.
Maxi Boettcher, Andreas Schäfler, Michael Sprenger, Harald Sodemann, Stefan Kaufmann, Christiane Voigt, Hans Schlager, Donato Summa, Paolo Di Girolamo, Daniele Nerini, Urs Germann, and Heini Wernli
Atmos. Chem. Phys., 21, 5477–5498, https://doi.org/10.5194/acp-21-5477-2021, https://doi.org/10.5194/acp-21-5477-2021, 2021
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Warm conveyor belts (WCBs) are important airstreams in extratropical cyclones, often leading to the formation of intense precipitation. We present a case study that involves aircraft, lidar and radar observations of water and clouds in a WCB ascending from western Europe across the Alps towards the Baltic Sea during the field campaigns HyMeX and T-NAWDEX-Falcon in October 2012. A probabilistic trajectory measure and an airborne tracer experiment were used to confirm the long pathway of the WCB.
Hong Chen, Sebastian Schmidt, Michael D. King, Galina Wind, Anthony Bucholtz, Elizabeth A. Reid, Michal Segal-Rozenhaimer, William L. Smith, Patrick C. Taylor, Seiji Kato, and Peter Pilewskie
Atmos. Meas. Tech., 14, 2673–2697, https://doi.org/10.5194/amt-14-2673-2021, https://doi.org/10.5194/amt-14-2673-2021, 2021
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In this paper, we accessed the shortwave irradiance derived from MODIS cloud optical properties by using aircraft measurements. We developed a data aggregation technique to parameterize spectral surface albedo by snow fraction in the Arctic. We found that undetected clouds have the most significant impact on the imagery-derived irradiance. This study suggests that passive imagery cloud detection could be improved through a multi-pixel approach that would make it more dependable in the Arctic.
Daniela Krampe, Frank Kauker, Marie Dumont, and Andreas Herber
The Cryosphere Discuss., https://doi.org/10.5194/tc-2021-100, https://doi.org/10.5194/tc-2021-100, 2021
Manuscript not accepted for further review
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Reliable and detailed Arctic snow data are limited. Evaluation of the performance of atmospheric reanalysis compared to measurements in northeast Greenland generally show good agreement. Both data sets are applied to an Alpine snow model and the performance for Arctic conditions is investigated: Simulated snow depth evolution is reliable, but vertical snow profiles show weaknesses. These are smaller with an adapted parametrisation for the density of newly fallen snow for harsh Arctic conditions.
Andreas Schäfler, Andreas Fix, and Martin Wirth
Atmos. Chem. Phys., 21, 5217–5234, https://doi.org/10.5194/acp-21-5217-2021, https://doi.org/10.5194/acp-21-5217-2021, 2021
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First-ever, collocated ozone and water vapor lidar observations across the tropopause are applied to investigate the extratropical transition layer (ExTL). The combined view of a quasi-instantaneous cross section and its tracer–tracer depiction allows us to analyze the ExTL shape and composition and the formation of mixing lines in relation to the dynamic situation. Such lidar data are relevant for future upper-tropospheric and lower-stratospheric investigations and model validations.
Yu Zhang, Tingting Zhu, Gunnar Spreen, Christian Melsheimer, Marcus Huntemann, Nick Hughes, Shengkai Zhang, and Fei Li
The Cryosphere Discuss., https://doi.org/10.5194/tc-2021-85, https://doi.org/10.5194/tc-2021-85, 2021
Revised manuscript not accepted
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We developed an algorithm for ice-water classification using Sentinel-1 data during melting seasons in the Fram Strait. The proposed algorithm has the OA of nearly 90 % with STD less than 10 %. The comparison of sea ice concentration demonstrate that it can provide detailed information of sea ice with the spatial resolution of 1km. The time series shows the average June to September sea ice area does not change so much in 2015–2017 and 2019–2020, but it has a significant decrease in 2018.
Franziska Aemisegger, Raphaela Vogel, Pascal Graf, Fabienne Dahinden, Leonie Villiger, Friedhelm Jansen, Sandrine Bony, Bjorn Stevens, and Heini Wernli
Weather Clim. Dynam., 2, 281–309, https://doi.org/10.5194/wcd-2-281-2021, https://doi.org/10.5194/wcd-2-281-2021, 2021
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The interaction of clouds in the trade wind region with the atmospheric flow is complex and at the heart of uncertainties associated with climate projections. In this study, a natural tracer of atmospheric circulation is used to establish a link between air originating from dry regions of the midlatitudes and the occurrence of specific cloud patterns. Two pathways involving transport within midlatitude weather systems are identified, by which air is brought into the trades within 5–10 d.
David L. A. Flack, Gwendal Rivière, Ionela Musat, Romain Roehrig, Sandrine Bony, Julien Delanoë, Quitterie Cazenave, and Jacques Pelon
Weather Clim. Dynam., 2, 233–253, https://doi.org/10.5194/wcd-2-233-2021, https://doi.org/10.5194/wcd-2-233-2021, 2021
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The representation of an extratropical cyclone in simulations of two climate models is studied by comparing them to observations of the international field campaign NAWDEX. We show that the current resolution used to run climate model projections (more than 100 km) is not enough to represent the life cycle accurately, but the use of 50 km resolution is good enough. Despite these encouraging results, cloud properties (partitioning liquid and solid) are found to be far from the observations.
Davide Ori, Leonie von Terzi, Markus Karrer, and Stefan Kneifel
Geosci. Model Dev., 14, 1511–1531, https://doi.org/10.5194/gmd-14-1511-2021, https://doi.org/10.5194/gmd-14-1511-2021, 2021
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Snowflakes have very complex shapes, and modeling their properties requires vast computing power. We produced a large number of realistic snowflakes and modeled their average properties by leveraging their fractal structure. Our approach allows modeling the properties of big ensembles of snowflakes, taking into account their natural variability, at a much lower cost. This enables the usage of remote sensing instruments, such as radars, to monitor the evolution of clouds and precipitation.
Sebastian O'Shea, Jonathan Crosier, James Dorsey, Louis Gallagher, Waldemar Schledewitz, Keith Bower, Oliver Schlenczek, Stephan Borrmann, Richard Cotton, Christopher Westbrook, and Zbigniew Ulanowski
Atmos. Meas. Tech., 14, 1917–1939, https://doi.org/10.5194/amt-14-1917-2021, https://doi.org/10.5194/amt-14-1917-2021, 2021
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The number, shape, and size of ice crystals in clouds are important properties that influence the Earth's radiation budget, cloud evolution, and precipitation formation. This work suggests that one of the most widely used methods for in situ measurements of these properties has significant uncertainties and biases. We suggest methods that dramatically improve these measurements, which can be applied to past and future datasets from these instruments.
Duseong S. Jo, Alma Hodzic, Louisa K. Emmons, Simone Tilmes, Rebecca H. Schwantes, Michael J. Mills, Pedro Campuzano-Jost, Weiwei Hu, Rahul A. Zaveri, Richard C. Easter, Balwinder Singh, Zheng Lu, Christiane Schulz, Johannes Schneider, John E. Shilling, Armin Wisthaler, and Jose L. Jimenez
Atmos. Chem. Phys., 21, 3395–3425, https://doi.org/10.5194/acp-21-3395-2021, https://doi.org/10.5194/acp-21-3395-2021, 2021
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Secondary organic aerosol (SOA) is a major component of submicron particulate matter, but there are a lot of uncertainties in the future prediction of SOA. We used CESM 2.1 to investigate future IEPOX SOA concentration changes. The explicit chemistry predicted substantial changes in IEPOX SOA depending on the future scenario, but the parameterization predicted weak changes due to simplified chemistry, which shows the importance of correct physicochemical dependencies in future SOA prediction.
Miklós Szakáll, Michael Debertshäuser, Christian Philipp Lackner, Amelie Mayer, Oliver Eppers, Karoline Diehl, Alexander Theis, Subir Kumar Mitra, and Stephan Borrmann
Atmos. Chem. Phys., 21, 3289–3316, https://doi.org/10.5194/acp-21-3289-2021, https://doi.org/10.5194/acp-21-3289-2021, 2021
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The freezing of cloud drops is promoted by ice-nucleating particles immersed in the drops. This process is essential to understand ice and subsequent precipitation formation in clouds. We investigated the efficiency of several particle types to trigger immersion freezing with two single-drop levitation techniques: a wind tunnel and an acoustic levitator. The evaluation accounted for different conditions during our two series of experiments, which is also applicable to future comparison studies.
Fanny Peers, Peter Francis, Steven J. Abel, Paul A. Barrett, Keith N. Bower, Michael I. Cotterell, Ian Crawford, Nicholas W. Davies, Cathryn Fox, Stuart Fox, Justin M. Langridge, Kerry G. Meyer, Steven E. Platnick, Kate Szpek, and Jim M. Haywood
Atmos. Chem. Phys., 21, 3235–3254, https://doi.org/10.5194/acp-21-3235-2021, https://doi.org/10.5194/acp-21-3235-2021, 2021
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Satellite observations at high temporal resolution are a valuable asset to monitor the transport of biomass burning plumes and the cloud diurnal cycle in the South Atlantic, but they need to be validated. Cloud and above-cloud aerosol properties retrieved from SEVIRI are compared against MODIS and measurements from the CLARIFY-2017 campaign. While some systematic differences are observed between SEVIRI and MODIS, the overall agreement in the cloud and aerosol properties is very satisfactory.
Inken Knop, Stephan E. Bansmer, Valerian Hahn, and Christiane Voigt
Atmos. Meas. Tech., 14, 1761–1781, https://doi.org/10.5194/amt-14-1761-2021, https://doi.org/10.5194/amt-14-1761-2021, 2021
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Knowledge on droplet size and concentration is essential for several applications of atomizers. After having developed a new spray system for our icing wind tunnel, we did intercomparison tests of different droplet measurement techniques including two commercial probes. The probes proved the good repeatability of the spray conditions and showed good overall agreement in measuring size and concentration. Furthermore, we could identify limitations and error sources of the measuring techniques.
Steven T. Massie, Heather Cronk, Aronne Merrelli, Christopher O'Dell, K. Sebastian Schmidt, Hong Chen, and David Baker
Atmos. Meas. Tech., 14, 1475–1499, https://doi.org/10.5194/amt-14-1475-2021, https://doi.org/10.5194/amt-14-1475-2021, 2021
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The OCO-2 science team is working to retrieve CO2 measurements that can be used by the carbon cycle community to calculate regional sources and sinks of CO2. The retrieved data, however, are in need of improvements in accuracy. This paper discusses several ways in which 3D cloud metrics (such as the distance of a measurement to the nearest cloud) can be used to account for cloud effects in the OCO-2 CO2 data files.
Rosaria E. Pileci, Robin L. Modini, Michele Bertò, Jinfeng Yuan, Joel C. Corbin, Angela Marinoni, Bas Henzing, Marcel M. Moerman, Jean P. Putaud, Gerald Spindler, Birgit Wehner, Thomas Müller, Thomas Tuch, Arianna Trentini, Marco Zanatta, Urs Baltensperger, and Martin Gysel-Beer
Atmos. Meas. Tech., 14, 1379–1403, https://doi.org/10.5194/amt-14-1379-2021, https://doi.org/10.5194/amt-14-1379-2021, 2021
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Black carbon (BC), which is an important constituent of atmospheric aerosols, remains difficult to quantify due to various limitations of available methods. This study provides an extensive comparison of co-located field measurements, applying two methods based on different principles. It was shown that both methods indeed quantify the same aerosol property – BC mass concentration. The level of agreement that can be expected was quantified, and some reasons for discrepancy were identified.
Claudia Christine Stephan, Sabrina Schnitt, Hauke Schulz, Hugo Bellenger, Simon P. de Szoeke, Claudia Acquistapace, Katharina Baier, Thibaut Dauhut, Rémi Laxenaire, Yanmichel Morfa-Avalos, Renaud Person, Estefanía Quiñones Meléndez, Gholamhossein Bagheri, Tobias Böck, Alton Daley, Johannes Güttler, Kevin C. Helfer, Sebastian A. Los, Almuth Neuberger, Johannes Röttenbacher, Andreas Raeke, Maximilian Ringel, Markus Ritschel, Pauline Sadoulet, Imke Schirmacher, M. Katharina Stolla, Ethan Wright, Benjamin Charpentier, Alexis Doerenbecher, Richard Wilson, Friedhelm Jansen, Stefan Kinne, Gilles Reverdin, Sabrina Speich, Sandrine Bony, and Bjorn Stevens
Earth Syst. Sci. Data, 13, 491–514, https://doi.org/10.5194/essd-13-491-2021, https://doi.org/10.5194/essd-13-491-2021, 2021
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The EUREC4A field campaign took place in the western tropical Atlantic during January and February 2020. A total of 811 radiosondes, launched regularly (usually 4-hourly) from Barbados, and 4 ships measured wind, temperature, and relative humidity. They sampled atmospheric variability associated with different ocean surface conditions, synoptic variability, and mesoscale convective organization. The methods of data collection and post-processing for the radiosonde data are described here.
Jens Redemann, Robert Wood, Paquita Zuidema, Sarah J. Doherty, Bernadette Luna, Samuel E. LeBlanc, Michael S. Diamond, Yohei Shinozuka, Ian Y. Chang, Rei Ueyama, Leonhard Pfister, Ju-Mee Ryoo, Amie N. Dobracki, Arlindo M. da Silva, Karla M. Longo, Meloë S. Kacenelenbogen, Connor J. Flynn, Kristina Pistone, Nichola M. Knox, Stuart J. Piketh, James M. Haywood, Paola Formenti, Marc Mallet, Philip Stier, Andrew S. Ackerman, Susanne E. Bauer, Ann M. Fridlind, Gregory R. Carmichael, Pablo E. Saide, Gonzalo A. Ferrada, Steven G. Howell, Steffen Freitag, Brian Cairns, Brent N. Holben, Kirk D. Knobelspiesse, Simone Tanelli, Tristan S. L'Ecuyer, Andrew M. Dzambo, Ousmane O. Sy, Greg M. McFarquhar, Michael R. Poellot, Siddhant Gupta, Joseph R. O'Brien, Athanasios Nenes, Mary Kacarab, Jenny P. S. Wong, Jennifer D. Small-Griswold, Kenneth L. Thornhill, David Noone, James R. Podolske, K. Sebastian Schmidt, Peter Pilewskie, Hong Chen, Sabrina P. Cochrane, Arthur J. Sedlacek, Timothy J. Lang, Eric Stith, Michal Segal-Rozenhaimer, Richard A. Ferrare, Sharon P. Burton, Chris A. Hostetler, David J. Diner, Felix C. Seidel, Steven E. Platnick, Jeffrey S. Myers, Kerry G. Meyer, Douglas A. Spangenberg, Hal Maring, and Lan Gao
Atmos. Chem. Phys., 21, 1507–1563, https://doi.org/10.5194/acp-21-1507-2021, https://doi.org/10.5194/acp-21-1507-2021, 2021
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Southern Africa produces significant biomass burning emissions whose impacts on regional and global climate are poorly understood. ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) is a 5-year NASA investigation designed to study the key processes that determine these climate impacts. The main purpose of this paper is to familiarize the broader scientific community with the ORACLES project, the dataset it produced, and the most important initial findings.
Evelyn Jäkel, Tim Carlsen, André Ehrlich, Manfred Wendisch, Michael Schäfer, Sophie Rosenburg, Konstantina Nakoudi, Marco Zanatta, Gerit Birnbaum, Veit Helm, Andreas Herber, Larysa Istomina, Linlu Mei, and Anika Rohde
The Cryosphere Discuss., https://doi.org/10.5194/tc-2021-14, https://doi.org/10.5194/tc-2021-14, 2021
Preprint withdrawn
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Different approaches to retrieve the optical-equivalent snow grain size using satellite, airborne, and ground-based observations were evaluated and compared to modeled data. The study is focused on low Sun and partly rough surface conditions encountered North of Greenland in March/April 2018. We proposed an adjusted airborne retrieval method to reduce the retrieval uncertainty.
Sabrina P. Cochrane, K. Sebastian Schmidt, Hong Chen, Peter Pilewskie, Scott Kittelman, Jens Redemann, Samuel LeBlanc, Kristina Pistone, Meloë Kacenelenbogen, Michal Segal Rozenhaimer, Yohei Shinozuka, Connor Flynn, Amie Dobracki, Paquita Zuidema, Steven Howell, Steffen Freitag, and Sarah Doherty
Atmos. Meas. Tech., 14, 567–593, https://doi.org/10.5194/amt-14-567-2021, https://doi.org/10.5194/amt-14-567-2021, 2021
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Based on observations from the 2016 and 2017 field campaigns of ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS), this work establishes an observationally driven link from mid-visible aerosol optical depth (AOD) and other scene parameters to broadband shortwave irradiance (and by extension the direct aerosol radiative effect, DARE). The majority of the case-to-case DARE variability within the ORACLES dataset is attributable to the dependence on AOD and scene albedo.
Jim M. Haywood, Steven J. Abel, Paul A. Barrett, Nicolas Bellouin, Alan Blyth, Keith N. Bower, Melissa Brooks, Ken Carslaw, Haochi Che, Hugh Coe, Michael I. Cotterell, Ian Crawford, Zhiqiang Cui, Nicholas Davies, Beth Dingley, Paul Field, Paola Formenti, Hamish Gordon, Martin de Graaf, Ross Herbert, Ben Johnson, Anthony C. Jones, Justin M. Langridge, Florent Malavelle, Daniel G. Partridge, Fanny Peers, Jens Redemann, Philip Stier, Kate Szpek, Jonathan W. Taylor, Duncan Watson-Parris, Robert Wood, Huihui Wu, and Paquita Zuidema
Atmos. Chem. Phys., 21, 1049–1084, https://doi.org/10.5194/acp-21-1049-2021, https://doi.org/10.5194/acp-21-1049-2021, 2021
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Every year, the seasonal cycle of biomass burning from agricultural practices in Africa creates a huge plume of smoke that travels many thousands of kilometres over the Atlantic Ocean. This study provides an overview of a measurement campaign called the cloud–aerosol–radiation interaction and forcing for year 2017 (CLARIFY-2017) and documents the rationale, deployment strategy, observations, and key results from the campaign which utilized the heavily equipped FAAM atmospheric research aircraft.
Johannes Schneider, Ralf Weigel, Thomas Klimach, Antonis Dragoneas, Oliver Appel, Andreas Hünig, Sergej Molleker, Franziska Köllner, Hans-Christian Clemen, Oliver Eppers, Peter Hoppe, Peter Hoor, Christoph Mahnke, Martina Krämer, Christian Rolf, Jens-Uwe Grooß, Andreas Zahn, Florian Obersteiner, Fabrizio Ravegnani, Alexey Ulanovsky, Hans Schlager, Monika Scheibe, Glenn S. Diskin, Joshua P. DiGangi, John B. Nowak, Martin Zöger, and Stephan Borrmann
Atmos. Chem. Phys., 21, 989–1013, https://doi.org/10.5194/acp-21-989-2021, https://doi.org/10.5194/acp-21-989-2021, 2021
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During five aircraft missions, we detected aerosol particles containing meteoric material in the lower stratosphere. The stratospheric measurements span a latitude range from 15 to 68° N, and we find that at potential temperature levels of more than 40 K above the tropopause; particles containing meteoric material occur at similar abundance fractions across latitudes and seasons. We conclude that meteoric material is efficiently distributed between high and low latitudes by isentropic mixing.
Kamil Mróz, Alessandro Battaglia, Stefan Kneifel, Leonie von Terzi, Markus Karrer, and Davide Ori
Atmos. Meas. Tech., 14, 511–529, https://doi.org/10.5194/amt-14-511-2021, https://doi.org/10.5194/amt-14-511-2021, 2021
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The article examines the relationship between the characteristics of rain and the properties of the ice cloud from which the rain originated. Our results confirm the widely accepted assumption that the mass flux through the melting zone is well preserved with an exception of extreme aggregation and riming conditions. Moreover, it is shown that the mean (mass-weighted) size of particles above and below the melting zone is strongly linked, with the former being on average larger.
Tobias Sebastian Finn, Gernot Geppert, and Felix Ament
Hydrol. Earth Syst. Sci. Discuss., https://doi.org/10.5194/hess-2020-672, https://doi.org/10.5194/hess-2020-672, 2021
Revised manuscript not accepted
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Through the lens of recent developments in hydrological modelling and data assimilation, we hourly update the soil moisture with ensemble data assimilation and sparse 2-metre-temperature observations in a coupled limited area model system. In idealized experiments, we improve the soil moisture analysis by coupled data assimilation across the atmosphere-land interface. We conclude that we can merge the separated assimilation cycles for the atmosphere and land surface into one single cycle.
Jinfeng Yuan, Robin Lewis Modini, Marco Zanatta, Andreas B. Herber, Thomas Müller, Birgit Wehner, Laurent Poulain, Thomas Tuch, Urs Baltensperger, and Martin Gysel-Beer
Atmos. Chem. Phys., 21, 635–655, https://doi.org/10.5194/acp-21-635-2021, https://doi.org/10.5194/acp-21-635-2021, 2021
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Black carbon (BC) aerosols contribute substantially to climate warming due to their unique light absorption capabilities. We performed field measurements at a central European background site in winter and found that variability in the absorption efficiency of BC particles is driven mainly by their internal mixing state. Our results suggest that, at this site, knowing the BC mixing state is sufficient to describe BC light absorption enhancements due to the lensing effect in good approximation.
Nicolas Blanchard, Florian Pantillon, Jean-Pierre Chaboureau, and Julien Delanoë
Weather Clim. Dynam., 2, 37–53, https://doi.org/10.5194/wcd-2-37-2021, https://doi.org/10.5194/wcd-2-37-2021, 2021
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Rare aircraft observations in the warm conveyor belt outflow associated with an extratropical cyclone are complemented with convection-permitting simulations. They reveal a complex tropopause structure with two jet stream cores, from which one is reinforced by bands of negative potential vorticity. They show that negative potential vorticity takes its origin in mid-level convection, which indirectly accelerates the jet stream and, thus, may influence the downstream large-scale circulation.
Lena Frey, Frida A.-M. Bender, and Gunilla Svensson
Atmos. Chem. Phys., 21, 577–595, https://doi.org/10.5194/acp-21-577-2021, https://doi.org/10.5194/acp-21-577-2021, 2021
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We investigate the vertical distribution of aerosol in the climate model NorESM1-M in five regions of marine stratocumulus clouds. We thereby analyze the total aerosol extinction to facilitate a comparison with satellite data. We find that the model underestimates aerosol extinction throughout the troposphere, especially elevated aerosol layers. Further, we perform sensitivity experiments to identify the processes most important for vertical aerosol distribution in our model.
Frédéric Szczap, Alaa Alkasem, Guillaume Mioche, Valery Shcherbakov, Céline Cornet, Julien Delanoë, Yahya Gour, Olivier Jourdan, Sandra Banson, and Edouard Bray
Atmos. Meas. Tech., 14, 199–221, https://doi.org/10.5194/amt-14-199-2021, https://doi.org/10.5194/amt-14-199-2021, 2021
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Spaceborne lidar and radar are suitable tools to investigate cloud vertical properties on a global scale. This paper presents the McRALI code that provides simulations of lidar and radar signals from the EarthCARE mission. Regarding radar signals, cloud heterogeneity induces a severe bias in velocity estimates. Regarding lidar signals, multiple scattering is not negligible. Our results also give some insight into the reliability of lidar signal modeling using independent column approximation.
Felipe Toledo, Julien Delanoë, Martial Haeffelin, Jean-Charles Dupont, Susana Jorquera, and Christophe Le Gac
Atmos. Meas. Tech., 13, 6853–6875, https://doi.org/10.5194/amt-13-6853-2020, https://doi.org/10.5194/amt-13-6853-2020, 2020
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Cloud observations are essential to rainfall, fog and climate change forecasts. One key instrument for these observations is cloud radar. Yet, discrepancies are found when comparing radars from different ground stations or satellites. Our work presents a calibration methodology for cloud radars based on reference targets, including an analysis of the uncertainty sources. The method enables the calibration of reference instruments to improve the quality and value of the cloud radar network data.
André Welti, E. Keith Bigg, Paul J. DeMott, Xianda Gong, Markus Hartmann, Mike Harvey, Silvia Henning, Paul Herenz, Thomas C. J. Hill, Blake Hornblow, Caroline Leck, Mareike Löffler, Christina S. McCluskey, Anne Marie Rauker, Julia Schmale, Christian Tatzelt, Manuela van Pinxteren, and Frank Stratmann
Atmos. Chem. Phys., 20, 15191–15206, https://doi.org/10.5194/acp-20-15191-2020, https://doi.org/10.5194/acp-20-15191-2020, 2020
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Ship-based measurements of maritime ice nuclei concentrations encompassing all oceans are compiled. From this overview it is found that maritime ice nuclei concentrations are typically 10–100 times lower than over continents, while concentrations are surprisingly similar in different oceanic regions. The analysis of the influence of ship emissions shows no effect on the data, making ship-based measurements an efficient strategy for the large-scale exploration of ice nuclei concentrations.
Ourania Soupiona, Alexandros Papayannis, Panagiotis Kokkalis, Romanos Foskinis, Guadalupe Sánchez Hernández, Pablo Ortiz-Amezcua, Maria Mylonaki, Christina-Anna Papanikolaou, Nikolaos Papagiannopoulos, Stefanos Samaras, Silke Groß, Rodanthi-Elisavet Mamouri, Lucas Alados-Arboledas, Aldo Amodeo, and Basil Psiloglou
Atmos. Chem. Phys., 20, 15147–15166, https://doi.org/10.5194/acp-20-15147-2020, https://doi.org/10.5194/acp-20-15147-2020, 2020
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51 dust events over the Mediterranean from EARLINET were studied regarding the aerosol geometrical, optical and microphysical properties and radiative forcing. We found δp532 values of 0.24–0.28, LR532 values of 49–52 sr and AOT532 of 0.11–0.40. The aerosol mixing state was also examined. Depending on the dust properties, intensity and solar zenith angle, the estimated solar radiative forcing ranged from −59 to −22 W m−2 at the surface and from −24 to −1 W m−2 at the TOA (cooling effect).
Johannes Quaas, Antti Arola, Brian Cairns, Matthew Christensen, Hartwig Deneke, Annica M. L. Ekman, Graham Feingold, Ann Fridlind, Edward Gryspeerdt, Otto Hasekamp, Zhanqing Li, Antti Lipponen, Po-Lun Ma, Johannes Mülmenstädt, Athanasios Nenes, Joyce E. Penner, Daniel Rosenfeld, Roland Schrödner, Kenneth Sinclair, Odran Sourdeval, Philip Stier, Matthias Tesche, Bastiaan van Diedenhoven, and Manfred Wendisch
Atmos. Chem. Phys., 20, 15079–15099, https://doi.org/10.5194/acp-20-15079-2020, https://doi.org/10.5194/acp-20-15079-2020, 2020
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Anthropogenic pollution particles – aerosols – serve as cloud condensation nuclei and thus increase cloud droplet concentration and the clouds' reflection of sunlight (a cooling effect on climate). This Twomey effect is poorly constrained by models and requires satellite data for better quantification. The review summarizes the challenges in properly doing so and outlines avenues for progress towards a better use of aerosol retrievals and better retrievals of droplet concentrations.
Julienne Stroeve, Vishnu Nandan, Rosemary Willatt, Rasmus Tonboe, Stefan Hendricks, Robert Ricker, James Mead, Robbie Mallett, Marcus Huntemann, Polona Itkin, Martin Schneebeli, Daniela Krampe, Gunnar Spreen, Jeremy Wilkinson, Ilkka Matero, Mario Hoppmann, and Michel Tsamados
The Cryosphere, 14, 4405–4426, https://doi.org/10.5194/tc-14-4405-2020, https://doi.org/10.5194/tc-14-4405-2020, 2020
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This study provides a first look at the data collected by a new dual-frequency Ka- and Ku-band in situ radar over winter sea ice in the Arctic Ocean. The instrument shows potential for using both bands to retrieve snow depth over sea ice, as well as sensitivity of the measurements to changing snow and atmospheric conditions.
Maximilian Weitzel, Subir K. Mitra, Miklós Szakáll, Jacob P. Fugal, and Stephan Borrmann
Atmos. Chem. Phys., 20, 14889–14901, https://doi.org/10.5194/acp-20-14889-2020, https://doi.org/10.5194/acp-20-14889-2020, 2020
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The properties of ice crystals smaller than 150 µm in diameter were investigated in a cold-room laboratory using digital holography and microscopy. Automated image processing has been used to determine the track of falling ice crystals, and collected crystals were melted and scanned under a microscope to infer particle mass. A parameterization relating particle size and mass was determined which describes ice crystals in this size range more accurately than existing relationships.
Larysa Istomina, Henrik Marks, Marcus Huntemann, Georg Heygster, and Gunnar Spreen
Atmos. Meas. Tech., 13, 6459–6472, https://doi.org/10.5194/amt-13-6459-2020, https://doi.org/10.5194/amt-13-6459-2020, 2020
Marek Jacob, Pavlos Kollias, Felix Ament, Vera Schemann, and Susanne Crewell
Geosci. Model Dev., 13, 5757–5777, https://doi.org/10.5194/gmd-13-5757-2020, https://doi.org/10.5194/gmd-13-5757-2020, 2020
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We compare clouds in different cloud-resolving atmosphere simulations with airborne remote sensing observations. The focus is on warm shallow clouds in the Atlantic trade wind region. Those clouds are climatologically important but challenging for climate models. We use forward operators to apply instrument-specific thresholds for cloud detection to model outputs. In this comparison, the higher-resolution model better reproduces the layered cloud structure.
Anna Gialitaki, Alexandra Tsekeri, Vassilis Amiridis, Romain Ceolato, Lucas Paulien, Anna Kampouri, Antonis Gkikas, Stavros Solomos, Eleni Marinou, Moritz Haarig, Holger Baars, Albert Ansmann, Tatyana Lapyonok, Anton Lopatin, Oleg Dubovik, Silke Groß, Martin Wirth, Maria Tsichla, Ioanna Tsikoudi, and Dimitris Balis
Atmos. Chem. Phys., 20, 14005–14021, https://doi.org/10.5194/acp-20-14005-2020, https://doi.org/10.5194/acp-20-14005-2020, 2020
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Stratospheric smoke particles are found to significantly depolarize incident light, while this effect is also accompanied by a strong spectral dependence. We utilize scattering simulations to show that this behaviour can be attributed to the near-spherical shape of the particles. We also examine whether an extension of the current AERONET scattering model to include the near-spherical shapes could be of benefit to the AERONET retrieval for stratospheric smoke associated with enhanced PLDR.
Marvin Heidkamp, Felix Ament, Philipp de Vrese, and Andreas Chlond
Earth Syst. Dynam. Discuss., https://doi.org/10.5194/esd-2020-75, https://doi.org/10.5194/esd-2020-75, 2020
Publication in ESD not foreseen
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This study deals with leaf thermoregulation, a process that describes the ability of leaves to buffer against ambient temperatures. In the past, this effect has been investigated at the leaf scale, but not on the canopy or global scale. Here we try to close this scientific gap by studying the large-scale effect of leaf thermoregulation using the Max Planck Institute's Earth system model. We believe that our study provides valuable insights for modelers and observers.
Maialen Iturbide, José M. Gutiérrez, Lincoln M. Alves, Joaquín Bedia, Ruth Cerezo-Mota, Ezequiel Cimadevilla, Antonio S. Cofiño, Alejandro Di Luca, Sergio Henrique Faria, Irina V. Gorodetskaya, Mathias Hauser, Sixto Herrera, Kevin Hennessy, Helene T. Hewitt, Richard G. Jones, Svitlana Krakovska, Rodrigo Manzanas, Daniel Martínez-Castro, Gemma T. Narisma, Intan S. Nurhati, Izidine Pinto, Sonia I. Seneviratne, Bart van den Hurk, and Carolina S. Vera
Earth Syst. Sci. Data, 12, 2959–2970, https://doi.org/10.5194/essd-12-2959-2020, https://doi.org/10.5194/essd-12-2959-2020, 2020
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We present an update of the IPCC WGI reference regions used in AR5 for the synthesis of climate change information. This revision was guided by the basic principles of climatic consistency and model representativeness (in particular for the new CMIP6 simulations). We also present a new dataset of monthly CMIP5 and CMIP6 spatially aggregated information using the new reference regions and describe a worked example of how to use this dataset to inform regional climate change studies.
Tim Carlsen, Gerit Birnbaum, André Ehrlich, Veit Helm, Evelyn Jäkel, Michael Schäfer, and Manfred Wendisch
The Cryosphere, 14, 3959–3978, https://doi.org/10.5194/tc-14-3959-2020, https://doi.org/10.5194/tc-14-3959-2020, 2020
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The angular reflection of solar radiation by snow surfaces is particularly anisotropic and highly variable. We measured the angular reflection from an aircraft using a digital camera in Antarctica in 2013/14 and studied its variability: the anisotropy increases with a lower Sun but decreases for rougher surfaces and larger snow grains. The applied methodology allows for a direct comparison with satellite observations, which generally underestimated the anisotropy measured within this study.
Lixia Liu, Yafang Cheng, Siwen Wang, Chao Wei, Mira L. Pöhlker, Christopher Pöhlker, Paulo Artaxo, Manish Shrivastava, Meinrat O. Andreae, Ulrich Pöschl, and Hang Su
Atmos. Chem. Phys., 20, 13283–13301, https://doi.org/10.5194/acp-20-13283-2020, https://doi.org/10.5194/acp-20-13283-2020, 2020
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This modeling paper reveals how aerosol–cloud interactions (ACIs) and aerosol–radiation interactions (ARIs) induced by biomass burning (BB) aerosols act oppositely on radiation, cloud, and precipitation in the Amazon during the dry season. The varying relative significance of ACIs and ARIs with BB aerosol concentration leads to a nonlinear dependence of the total climate response on BB aerosol loading and features the growing importance of ARIs at high aerosol loading.
Hans-Christian Clemen, Johannes Schneider, Thomas Klimach, Frank Helleis, Franziska Köllner, Andreas Hünig, Florian Rubach, Stephan Mertes, Heike Wex, Frank Stratmann, André Welti, Rebecca Kohl, Fabian Frank, and Stephan Borrmann
Atmos. Meas. Tech., 13, 5923–5953, https://doi.org/10.5194/amt-13-5923-2020, https://doi.org/10.5194/amt-13-5923-2020, 2020
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We improved the efficiency of a single-particle mass spectrometer with a newly developed aerodynamic lens system, delayed ion extraction, and better electric shielding. The new components result in significantly improved particle analysis and sample statistics. This is particularly important for measurements of low-number-density particles, such as ice-nucleating particles, and for aircraft-based measurements at high altitudes or where high temporal and spatial resolution is required.
Jan Kretzschmar, Johannes Stapf, Daniel Klocke, Manfred Wendisch, and Johannes Quaas
Atmos. Chem. Phys., 20, 13145–13165, https://doi.org/10.5194/acp-20-13145-2020, https://doi.org/10.5194/acp-20-13145-2020, 2020
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This study compares simulations with the ICON model at the kilometer scale to airborne radiation and cloud microphysics observations that have been derived during the ACLOUD aircraft campaign around Svalbard, Norway, in May/June 2017. We find an overestimated surface warming effect of clouds compared to the observations in our setup. This bias was reduced by considering subgrid-scale vertical motion in the activation of cloud condensation nuclei in the two-moment microphysical scheme used.
Huihui Wu, Jonathan W. Taylor, Kate Szpek, Justin M. Langridge, Paul I. Williams, Michael Flynn, James D. Allan, Steven J. Abel, Joseph Pitt, Michael I. Cotterell, Cathryn Fox, Nicholas W. Davies, Jim Haywood, and Hugh Coe
Atmos. Chem. Phys., 20, 12697–12719, https://doi.org/10.5194/acp-20-12697-2020, https://doi.org/10.5194/acp-20-12697-2020, 2020
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Airborne measurements of highly aged biomass burning aerosols (BBAs) over the remote southeast Atlantic provide unique aerosol parameters for climate models. Our observations demonstrate the persistence of strongly absorbing BBAs across wide regions of the South Atlantic. We also found significant vertical variation in the single-scattering albedo of these BBAs, as a function of relative chemical composition and size. Aerosol properties in the marine BL are suggested to be separated from the FT.
Jie Gong, Xiping Zeng, Dong L. Wu, S. Joseph Munchak, Xiaowen Li, Stefan Kneifel, Davide Ori, Liang Liao, and Donifan Barahona
Atmos. Chem. Phys., 20, 12633–12653, https://doi.org/10.5194/acp-20-12633-2020, https://doi.org/10.5194/acp-20-12633-2020, 2020
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This work provides a novel way of using polarized passive microwave measurements to study the interlinked cloud–convection–precipitation processes. The magnitude of differences between polarized radiances is found linked to ice microphysics (shape, size, orientation and density), mesoscale dynamic and thermodynamic structures, and surface precipitation. We conclude that passive sensors with multiple polarized channel pairs may serve as cheaper and useful substitutes for spaceborne radar sensors.
Manuel Gutleben, Silke Groß, Martin Wirth, and Bernhard Mayer
Atmos. Chem. Phys., 20, 12313–12327, https://doi.org/10.5194/acp-20-12313-2020, https://doi.org/10.5194/acp-20-12313-2020, 2020
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Airborne lidar measurements in the vicinity of Barbados are used to investigate radiative effects of long-range-transported Saharan air layers. Derived atmospheric heating rates indicate that observed enhanced water vapor concentrations inside these layers are the main drivers for dust vertical mixing inside the layers. Additionally, they may play a major role for the suppression of subjacent convective cloud development.
Ting Lei, Nan Ma, Juan Hong, Thomas Tuch, Xin Wang, Zhibin Wang, Mira Pöhlker, Maofa Ge, Weigang Wang, Eugene Mikhailov, Thorsten Hoffmann, Ulrich Pöschl, Hang Su, Alfred Wiedensohler, and Yafang Cheng
Atmos. Meas. Tech., 13, 5551–5567, https://doi.org/10.5194/amt-13-5551-2020, https://doi.org/10.5194/amt-13-5551-2020, 2020
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We present the design of a nano-hygroscopicity tandem differential mobility analyzer (nano-HTDMA) apparatus that enables high accuracy and precision in hygroscopic growth measurements of aerosol nanoparticles with diameters less than 10 nm. We further introduce comprehensive methods for system calibration and validation of the performance of the system. We then study the size dependence of the deliquescence and the efflorescence of aerosol nanoparticles for sizes down to 6 nm.
Nicolas Blanchard, Florian Pantillon, Jean-Pierre Chaboureau, and Julien Delanoë
Weather Clim. Dynam., 1, 617–634, https://doi.org/10.5194/wcd-1-617-2020, https://doi.org/10.5194/wcd-1-617-2020, 2020
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The study presents the first results from the airborne RASTA observations measured during the North Atlantic Waveguide and Downstream Impact Experiment (NAWDEX). Our combined Eulerian–Lagrangian analysis found three types of organized convection (frontal, banded and mid-level) in the warm conveyor belt (WCB) of the Stalactite cyclone. The results emphasize that convection embedded in WCBs occurs in a coherent and organized manner rather than as isolated cells.
Yohei Shinozuka, Meloë S. Kacenelenbogen, Sharon P. Burton, Steven G. Howell, Paquita Zuidema, Richard A. Ferrare, Samuel E. LeBlanc, Kristina Pistone, Stephen Broccardo, Jens Redemann, K. Sebastian Schmidt, Sabrina P. Cochrane, Marta Fenn, Steffen Freitag, Amie Dobracki, Michal Segal-Rosenheimer, and Connor J. Flynn
Atmos. Chem. Phys., 20, 11275–11285, https://doi.org/10.5194/acp-20-11275-2020, https://doi.org/10.5194/acp-20-11275-2020, 2020
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To help satellite retrieval of aerosols and studies of their radiative effects, we demonstrate that daytime aerosol optical depth over low-level clouds is similar to that in neighboring clear skies at the same heights. Based on recent airborne lidar and sun photometer observations above the southeast Atlantic, the mean AOD difference at 532 nm is between 0 and -0.01, when comparing the cloudy and clear sides of cloud edges, with each up to 20 km wide.
Hamish Gordon, Paul R. Field, Steven J. Abel, Paul Barrett, Keith Bower, Ian Crawford, Zhiqiang Cui, Daniel P. Grosvenor, Adrian A. Hill, Jonathan Taylor, Jonathan Wilkinson, Huihui Wu, and Ken S. Carslaw
Atmos. Chem. Phys., 20, 10997–11024, https://doi.org/10.5194/acp-20-10997-2020, https://doi.org/10.5194/acp-20-10997-2020, 2020
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The Met Office's Unified Model is widely used both for weather forecasting and climate prediction. We present the first version of the model in which both aerosol and cloud particle mass and number concentrations are allowed to evolve separately and independently, which is important for studying how aerosols affect weather and climate. We test the model against aircraft observations near Ascension Island in the Atlantic, focusing on how aerosols can "activate" to become cloud droplets.
Li Li, Zhengqiang Li, Wenyuan Chang, Yang Ou, Philippe Goloub, Chengzhe Li, Kaitao Li, Qiaoyun Hu, Jianping Wang, and Manfred Wendisch
Atmos. Chem. Phys., 20, 10845–10864, https://doi.org/10.5194/acp-20-10845-2020, https://doi.org/10.5194/acp-20-10845-2020, 2020
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Dust Aerosol Observation-Kashi (DAO-K) campaign was conducted near the Taklimakan Desert in April 2019 to obtain comprehensive aerosol, atmosphere, and surface parameters. Estimations of aerosol solar radiative forcing by a radiative transfer (RT) model were improved based on the measured aerosol parameters, additionally considering atmospheric profiles and diurnal variations of surface albedo. RT simulations agree well with simultaneous irradiance observations, even in dust-polluted conditions.
Christof G. Beer, Johannes Hendricks, Mattia Righi, Bernd Heinold, Ina Tegen, Silke Groß, Daniel Sauer, Adrian Walser, and Bernadett Weinzierl
Geosci. Model Dev., 13, 4287–4303, https://doi.org/10.5194/gmd-13-4287-2020, https://doi.org/10.5194/gmd-13-4287-2020, 2020
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Mineral dust aerosol plays an important role in the climate system. Previously, dust emissions have often been represented in global models by prescribed monthly-mean emission fields representative of a specific year. We now apply an online calculation of wind-driven dust emissions. This results in an improved agreement with observations, due to a better representation of the highly variable dust emissions. Increasing the model resolution led to an additional performance gain.
Nina Črnivec and Bernhard Mayer
Atmos. Chem. Phys., 20, 10733–10755, https://doi.org/10.5194/acp-20-10733-2020, https://doi.org/10.5194/acp-20-10733-2020, 2020
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Unresolved interaction between clouds and atmospheric radiation is a source of uncertainty in weather and climate models. The present study highlights the potential of the state-of-the-art Tripleclouds radiative solver for shallow cumulus clouds, exposing the significance of properly representing subgrid cloud horizontal heterogeneity. The Tripleclouds concept was thereby incorporated in the widely employed δ-Eddington two-stream radiation scheme within the comprehensive libRadtran library.
Mario Mech, Maximilian Maahn, Stefan Kneifel, Davide Ori, Emiliano Orlandi, Pavlos Kollias, Vera Schemann, and Susanne Crewell
Geosci. Model Dev., 13, 4229–4251, https://doi.org/10.5194/gmd-13-4229-2020, https://doi.org/10.5194/gmd-13-4229-2020, 2020
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The Passive and Active Microwave TRAnsfer tool (PAMTRA) is a public domain software package written in Python and Fortran for the simulation of microwave remote sensing observations. PAMTRA models the interaction of radiation with gases, clouds, precipitation, and the surface using either in situ observations or model output as input parameters. The wide range of applications is demonstrated for passive (radiometer) and active (radar) instruments on ground, airborne, and satellite platforms.
W. Richard Leaitch, John K. Kodros, Megan D. Willis, Sarah Hanna, Hannes Schulz, Elisabeth Andrews, Heiko Bozem, Julia Burkart, Peter Hoor, Felicia Kolonjari, John A. Ogren, Sangeeta Sharma, Meng Si, Knut von Salzen, Allan K. Bertram, Andreas Herber, Jonathan P. D. Abbatt, and Jeffrey R. Pierce
Atmos. Chem. Phys., 20, 10545–10563, https://doi.org/10.5194/acp-20-10545-2020, https://doi.org/10.5194/acp-20-10545-2020, 2020
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Black carbon is a factor in the warming of the Arctic atmosphere due to its ability to absorb light, but the uncertainty is high and few observations have been made in the high Arctic above 80° N. We combine airborne and ground-based observations in the springtime Arctic, at and above 80° N, with simulations from a global model to show that light absorption by black carbon may be much larger than modelled. However, the uncertainty remains high.
Philipp J. Griewank, Thijs Heus, Neil P. Lareau, and Roel A. J. Neggers
Atmos. Chem. Phys., 20, 10211–10230, https://doi.org/10.5194/acp-20-10211-2020, https://doi.org/10.5194/acp-20-10211-2020, 2020
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The idea that larger shallow cumulus clouds have stronger updrafts than small shallow cumulus clouds is as intuitive as it is old. In this paper we gather years of upward-pointing laser measurements from a plain in Oklahoma and combine them with 28 d of high-resolution simulations. Our approach, which has much more data than previous studies, confirms that updraft strength and cloud size are linked and that the simulations reproduce the observed cloud wind and moisture structure.
Leighton A. Regayre, Julia Schmale, Jill S. Johnson, Christian Tatzelt, Andrea Baccarini, Silvia Henning, Masaru Yoshioka, Frank Stratmann, Martin Gysel-Beer, Daniel P. Grosvenor, and Ken S. Carslaw
Atmos. Chem. Phys., 20, 10063–10072, https://doi.org/10.5194/acp-20-10063-2020, https://doi.org/10.5194/acp-20-10063-2020, 2020
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The amount of energy reflected back into space because of man-made particles is highly uncertain. Processes related to naturally occurring particles cause most of the uncertainty, but these processes are poorly constrained by present-day measurements. We show that measurements over the Southern Ocean, far from pollution sources, efficiently reduce climate model uncertainties. Our results pave the way to designing experiments and measurement campaigns that reduce this uncertainty even further.
Johannes Stapf, André Ehrlich, Evelyn Jäkel, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys., 20, 9895–9914, https://doi.org/10.5194/acp-20-9895-2020, https://doi.org/10.5194/acp-20-9895-2020, 2020
James D. Annan, Julia C. Hargreaves, Thorsten Mauritsen, and Bjorn Stevens
Earth Syst. Dynam., 11, 709–719, https://doi.org/10.5194/esd-11-709-2020, https://doi.org/10.5194/esd-11-709-2020, 2020
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In this paper we explore the potential of variability for constraining the equilibrium response of the climate system to external forcing. We show that the constraint is inherently skewed, with a long tail to high sensitivity, and that while the variability may contain some useful information, it is unlikely to generate a tight constraint.
Christa Genz, Roland Schrödner, Bernd Heinold, Silvia Henning, Holger Baars, Gerald Spindler, and Ina Tegen
Atmos. Chem. Phys., 20, 8787–8806, https://doi.org/10.5194/acp-20-8787-2020, https://doi.org/10.5194/acp-20-8787-2020, 2020
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Atmospheric aerosols are the precondition for the formation of cloud droplets and thus have a large influence on cloud properties. Concentrations of cloud condensation nuclei of the period with highest aerosol concentrations over central Europe are uncertain. In this work, modeled estimates of CCN from today and the mid-1980s are compared to available in situ and remote sensing observations. A scaling factor between today and the 1980s for the CCN concentrations has been derived.
Linda Forster, Meinhard Seefeldner, Andreas Baumgartner, Tobias Kölling, and Bernhard Mayer
Atmos. Meas. Tech., 13, 3977–3991, https://doi.org/10.5194/amt-13-3977-2020, https://doi.org/10.5194/amt-13-3977-2020, 2020
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We present a procedure for both the geometric and absolute radiometric characterization of the weather-proof RGB camera HaloCamRAW, which is part of our automated halo observation system HaloCam, designed for the quantitative analysis of halo displays. By comparing the calibrated HaloCamRAW radiances of a 22° halo scene with radiative transfer simulations, we demonstrate the potential of developing a retrieval method for ice crystal properties, such as size, shape, and surface roughness.
Tuukka Petäjä, Ella-Maria Duplissy, Ksenia Tabakova, Julia Schmale, Barbara Altstädter, Gerard Ancellet, Mikhail Arshinov, Yurii Balin, Urs Baltensperger, Jens Bange, Alison Beamish, Boris Belan, Antoine Berchet, Rossana Bossi, Warren R. L. Cairns, Ralf Ebinghaus, Imad El Haddad, Beatriz Ferreira-Araujo, Anna Franck, Lin Huang, Antti Hyvärinen, Angelika Humbert, Athina-Cerise Kalogridis, Pavel Konstantinov, Astrid Lampert, Matthew MacLeod, Olivier Magand, Alexander Mahura, Louis Marelle, Vladimir Masloboev, Dmitri Moisseev, Vaios Moschos, Niklas Neckel, Tatsuo Onishi, Stefan Osterwalder, Aino Ovaska, Pauli Paasonen, Mikhail Panchenko, Fidel Pankratov, Jakob B. Pernov, Andreas Platis, Olga Popovicheva, Jean-Christophe Raut, Aurélie Riandet, Torsten Sachs, Rosamaria Salvatori, Roberto Salzano, Ludwig Schröder, Martin Schön, Vladimir Shevchenko, Henrik Skov, Jeroen E. Sonke, Andrea Spolaor, Vasileios K. Stathopoulos, Mikko Strahlendorff, Jennie L. Thomas, Vito Vitale, Sterios Vratolis, Carlo Barbante, Sabine Chabrillat, Aurélien Dommergue, Konstantinos Eleftheriadis, Jyri Heilimo, Kathy S. Law, Andreas Massling, Steffen M. Noe, Jean-Daniel Paris, André S. H. Prévôt, Ilona Riipinen, Birgit Wehner, Zhiyong Xie, and Hanna K. Lappalainen
Atmos. Chem. Phys., 20, 8551–8592, https://doi.org/10.5194/acp-20-8551-2020, https://doi.org/10.5194/acp-20-8551-2020, 2020
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The role of polar regions is increasing in terms of megatrends such as globalization, new transport routes, demography, and the use of natural resources with consequent effects on regional and transported pollutant concentrations. Here we summarize initial results from our integrative project exploring the Arctic environment and pollution to deliver data products, metrics, and indicators for stakeholders.
Tobias Donth, Evelyn Jäkel, André Ehrlich, Bernd Heinold, Jacob Schacht, Andreas Herber, Marco Zanatta, and Manfred Wendisch
Atmos. Chem. Phys., 20, 8139–8156, https://doi.org/10.5194/acp-20-8139-2020, https://doi.org/10.5194/acp-20-8139-2020, 2020
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Solar radiative effects of Arctic black carbon (BC) particles (suspended in the atmosphere and in the surface snowpack) were quantified under cloudless and cloudy conditions. An atmospheric and a snow radiative transfer model were coupled to account for radiative interactions between both compartments. It was found that (i) the warming effect of BC in the snowpack overcompensates for the atmospheric BC cooling effect, and (ii) clouds tend to reduce the atmospheric BC cooling and snow BC warming.
Arantxa M. Triana-Gómez, Georg Heygster, Christian Melsheimer, Gunnar Spreen, Monia Negusini, and Boyan H. Petkov
Atmos. Meas. Tech., 13, 3697–3715, https://doi.org/10.5194/amt-13-3697-2020, https://doi.org/10.5194/amt-13-3697-2020, 2020
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In the Arctic, in situ measurements are sparse and standard remote sensing retrieval methods have problems. We present advances in a retrieval algorithm for vertically integrated water vapour tuned for polar regions. In addition to the initial sensor used (AMSU-B), we can now also use data from the successor instrument (MHS). Additionally, certain artefacts are now filtered out. Comparison with radiosondes shows the overall good performance of the updated algorithm.
Sergej Molleker, Frank Helleis, Thomas Klimach, Oliver Appel, Hans-Christian Clemen, Antonis Dragoneas, Christian Gurk, Andreas Hünig, Franziska Köllner, Florian Rubach, Christiane Schulz, Johannes Schneider, and Stephan Borrmann
Atmos. Meas. Tech., 13, 3651–3660, https://doi.org/10.5194/amt-13-3651-2020, https://doi.org/10.5194/amt-13-3651-2020, 2020
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A novel constant-pressure-inlet design for use in airborne aerosol particle mass spectrometry – an aerodynamic lens focuses aerosol particles into a vacuum chamber – is presented. The pressure of a few hectopascals at the lens is precisely controlled over a large flight altitude range up to 21 km. The constant pressure is achieved by changing the inner diameter of a properly scaled flexible O-ring acting as a critical orifice. Particle transmission at various inlet pressures is characterized.
Yongbiao Weng, Alexandra Touzeau, and Harald Sodemann
Atmos. Meas. Tech., 13, 3167–3190, https://doi.org/10.5194/amt-13-3167-2020, https://doi.org/10.5194/amt-13-3167-2020, 2020
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We find that the known mixing ratio dependence of laser spectrometers for water vapour isotope measurements varies with isotope composition. We have developed a scheme to correct for this isotope-composition-dependent bias. The correction is most substantial at low mixing ratios. Stability tests indicate that the first-order dependency is a constant instrument characteristic. Water vapour isotope measurements at low mixing ratios can now be corrected by following our proposed procedure.
Manuela van Pinxteren, Khanneh Wadinga Fomba, Nadja Triesch, Christian Stolle, Oliver Wurl, Enno Bahlmann, Xianda Gong, Jens Voigtländer, Heike Wex, Tiera-Brandy Robinson, Stefan Barthel, Sebastian Zeppenfeld, Erik Hans Hoffmann, Marie Roveretto, Chunlin Li, Benoit Grosselin, Veronique Daële, Fabian Senf, Dominik van Pinxteren, Malena Manzi, Nicolás Zabalegui, Sanja Frka, Blaženka Gašparović, Ryan Pereira, Tao Li, Liang Wen, Jiarong Li, Chao Zhu, Hui Chen, Jianmin Chen, Björn Fiedler, Wolf von Tümpling, Katie Alana Read, Shalini Punjabi, Alastair Charles Lewis, James Roland Hopkins, Lucy Jane Carpenter, Ilka Peeken, Tim Rixen, Detlef Schulz-Bull, María Eugenia Monge, Abdelwahid Mellouki, Christian George, Frank Stratmann, and Hartmut Herrmann
Atmos. Chem. Phys., 20, 6921–6951, https://doi.org/10.5194/acp-20-6921-2020, https://doi.org/10.5194/acp-20-6921-2020, 2020
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An introduction to a comprehensive field campaign performed at the Cape Verde Atmospheric Observatory regarding ocean–atmosphere interactions is given. Chemical, physical, biological and meteorological techniques were applied, and measurements of bulk water, the sea surface microlayer, cloud water and ambient aerosol particles took place. Oceanic compounds were found to be transferred to atmospheric aerosol and to the cloud level; however, sea spray contributions to CCN and INPs were limited.
Xiaoyong Yu, Annette Rinke, Wolfgang Dorn, Gunnar Spreen, Christof Lüpkes, Hiroshi Sumata, and Vladimir M. Gryanik
The Cryosphere, 14, 1727–1746, https://doi.org/10.5194/tc-14-1727-2020, https://doi.org/10.5194/tc-14-1727-2020, 2020
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This study presents an evaluation of Arctic sea ice drift speed for the period 2003–2014 in a state-of-the-art coupled regional model for the Arctic, called HIRHAM–NAOSIM. In particular, the dependency of the drift speed on the near-surface wind speed and sea ice conditions is presented. Effects of sea ice form drag included by an improved parameterization of the transfer coefficients for momentum and heat over sea ice are discussed.
Iris Thurnherr, Anna Kozachek, Pascal Graf, Yongbiao Weng, Dimitri Bolshiyanov, Sebastian Landwehr, Stephan Pfahl, Julia Schmale, Harald Sodemann, Hans Christian Steen-Larsen, Alessandro Toffoli, Heini Wernli, and Franziska Aemisegger
Atmos. Chem. Phys., 20, 5811–5835, https://doi.org/10.5194/acp-20-5811-2020, https://doi.org/10.5194/acp-20-5811-2020, 2020
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Stable water isotopes (SWIs) are tracers of moist atmospheric processes. We analyse the impact of large- to small-scale atmospheric processes and various environmental conditions on the variability of SWIs using ship-based SWI measurement in water vapour from the Atlantic and Southern Ocean. Furthermore, simultaneous measurements of SWIs at two altitudes are used to illustrate the potential of such measurements for future research to estimate sea spray evaporation and turbulent moisture fluxes.
Montserrat Costa-Surós, Odran Sourdeval, Claudia Acquistapace, Holger Baars, Cintia Carbajal Henken, Christa Genz, Jonas Hesemann, Cristofer Jimenez, Marcel König, Jan Kretzschmar, Nils Madenach, Catrin I. Meyer, Roland Schrödner, Patric Seifert, Fabian Senf, Matthias Brueck, Guido Cioni, Jan Frederik Engels, Kerstin Fieg, Ksenia Gorges, Rieke Heinze, Pavan Kumar Siligam, Ulrike Burkhardt, Susanne Crewell, Corinna Hoose, Axel Seifert, Ina Tegen, and Johannes Quaas
Atmos. Chem. Phys., 20, 5657–5678, https://doi.org/10.5194/acp-20-5657-2020, https://doi.org/10.5194/acp-20-5657-2020, 2020
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The impact of anthropogenic aerosols on clouds is a key uncertainty in climate change. This study analyses large-domain simulations with a new high-resolution model to investigate the differences in clouds between 1985 and 2013 comparing multiple observational datasets. The differences in aerosol and in cloud droplet concentrations are clearly detectable. For other quantities, the detection and attribution proved difficult, despite a substantial impact on the Earth's energy budget.
Elena Ruiz-Donoso, André Ehrlich, Michael Schäfer, Evelyn Jäkel, Vera Schemann, Susanne Crewell, Mario Mech, Birte Solveig Kulla, Leif-Leonard Kliesch, Roland Neuber, and Manfred Wendisch
Atmos. Chem. Phys., 20, 5487–5511, https://doi.org/10.5194/acp-20-5487-2020, https://doi.org/10.5194/acp-20-5487-2020, 2020
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Mixed-phase clouds, formed of water droplets and ice crystals, appear frequently in Arctic regions. Characterizing the distribution of liquid water and ice inside the cloud appropriately is important because it influences the cloud's impact on the surface temperature. In this study, we combined images of the cloud top with measurements inside the cloud to analyze in detail the 3D spatial distribution of liquid and ice in two mixed-phase clouds occurring under different meteorological scenarios.
Tatiana Nomokonova, Kerstin Ebell, Ulrich Löhnert, Marion Maturilli, and Christoph Ritter
Atmos. Chem. Phys., 20, 5157–5173, https://doi.org/10.5194/acp-20-5157-2020, https://doi.org/10.5194/acp-20-5157-2020, 2020
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This paper presents an influence of water vapor anomalies on cloud properties and their radiative effect at Ny-Ålesund. The study is based on a 2.5-year active and passive cloud observation and a radiative transfer model. The results show that moist and dry conditions are related to strong changes in cloud occurrence, phase partitioning, water path, and, consequently, modulate the surface radiative budget.
Bruna A. Holanda, Mira L. Pöhlker, David Walter, Jorge Saturno, Matthias Sörgel, Jeannine Ditas, Florian Ditas, Christiane Schulz, Marco Aurélio Franco, Qiaoqiao Wang, Tobias Donth, Paulo Artaxo, Henrique M. J. Barbosa, Stephan Borrmann, Ramon Braga, Joel Brito, Yafang Cheng, Maximilian Dollner, Johannes W. Kaiser, Thomas Klimach, Christoph Knote, Ovid O. Krüger, Daniel Fütterer, Jošt V. Lavrič, Nan Ma, Luiz A. T. Machado, Jing Ming, Fernando G. Morais, Hauke Paulsen, Daniel Sauer, Hans Schlager, Johannes Schneider, Hang Su, Bernadett Weinzierl, Adrian Walser, Manfred Wendisch, Helmut Ziereis, Martin Zöger, Ulrich Pöschl, Meinrat O. Andreae, and Christopher Pöhlker
Atmos. Chem. Phys., 20, 4757–4785, https://doi.org/10.5194/acp-20-4757-2020, https://doi.org/10.5194/acp-20-4757-2020, 2020
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Biomass burning smoke from African savanna and grassland is transported across the South Atlantic Ocean in defined layers within the free troposphere. The combination of in situ aircraft and ground-based measurements aided by satellite observations showed that these layers are transported into the Amazon Basin during the early dry season. The influx of aged smoke, enriched in black carbon and cloud condensation nuclei, has important implications for the Amazonian aerosol and cloud cycling.
Siddika Celik, Frank Drewnick, Friederike Fachinger, James Brooks, Eoghan Darbyshire, Hugh Coe, Jean-Daniel Paris, Philipp G. Eger, Jan Schuladen, Ivan Tadic, Nils Friedrich, Dirk Dienhart, Bettina Hottmann, Horst Fischer, John N. Crowley, Hartwig Harder, and Stephan Borrmann
Atmos. Chem. Phys., 20, 4713–4734, https://doi.org/10.5194/acp-20-4713-2020, https://doi.org/10.5194/acp-20-4713-2020, 2020
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Analysis of 252 ship emission plumes in the Mediterranean Sea and around the Arabian Peninsula examined particulate- and gas-phase characteristics. By identifying the corresponding ships, source features and plume age were determined. Emission factors (amount of pollutant per kilogram of fuel burned) were calculated and investigated for dependencies on source characteristics, atmospheric conditions, and transport time, providing insight into the most relevant influences on ship emissions.
Dennis Niedermeier, Jens Voigtländer, Silvio Schmalfuß, Daniel Busch, Jörg Schumacher, Raymond A. Shaw, and Frank Stratmann
Atmos. Meas. Tech., 13, 2015–2033, https://doi.org/10.5194/amt-13-2015-2020, https://doi.org/10.5194/amt-13-2015-2020, 2020
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In this paper, we present the new moist-air wind tunnel LACIS-T (Turbulent Leipzig Aerosol Cloud Interaction Simulator). It is used to study cloud physical processes in general and interactions between turbulence and cloud microphysical processes in particular. The operating principle of LACIS-T is explained, and the first results are depicted from deliquescence and droplet formation experiments observing clear indications on the effect of turbulence on these microphysical processes.
Steven J. Abel, Paul A. Barrett, Paquita Zuidema, Jianhao Zhang, Matt Christensen, Fanny Peers, Jonathan W. Taylor, Ian Crawford, Keith N. Bower, and Michael Flynn
Atmos. Chem. Phys., 20, 4059–4084, https://doi.org/10.5194/acp-20-4059-2020, https://doi.org/10.5194/acp-20-4059-2020, 2020
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In situ measurements of a free-tropospheric (FT) biomass burning aerosol plume in contact with the boundary layer inversion overriding a pocket of open cells (POC) and surrounding stratiform cloud are presented. The data highlight the contrasting thermodynamic, aerosol and cloud properties in the two cloud regimes and further demonstrate that the cloud regime plays a key role in regulating the flow of FT aerosols into the boundary layer, which has implications for the aerosol indirect effect.
Gary Lloyd, Thomas Choularton, Keith Bower, Jonathan Crosier, Martin Gallagher, Michael Flynn, James Dorsey, Dantong Liu, Jonathan W. Taylor, Oliver Schlenczek, Jacob Fugal, Stephan Borrmann, Richard Cotton, Paul Field, and Alan Blyth
Atmos. Chem. Phys., 20, 3895–3904, https://doi.org/10.5194/acp-20-3895-2020, https://doi.org/10.5194/acp-20-3895-2020, 2020
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Measurements of liquid and ice cloud particles were made using an aircraft to penetrate fresh growing convective clouds in the tropical Atlantic. We found small ice particles at surprisingly high temperatures just below freezing. At colder temperatures secondary ice processes rapidly generated high concentrations of ice crystals.
Maria P. Cadeddu, Virendra P. Ghate, and Mario Mech
Atmos. Meas. Tech., 13, 1485–1499, https://doi.org/10.5194/amt-13-1485-2020, https://doi.org/10.5194/amt-13-1485-2020, 2020
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A combination of ground-based active and passive observations is used to partition cloud and precipitation liquid water path in precipitating stratocumulous clouds. Results show that neglecting scattering effects from drizzle drops leads to 8–15 % overestimation of the liquid amount in the cloud. In closed-cell systems only ~20 % of the available drizzle in the cloud falls below the cloud base, compared to ~40 % in open-cell systems.
Mattia Righi, Johannes Hendricks, Ulrike Lohmann, Christof Gerhard Beer, Valerian Hahn, Bernd Heinold, Romy Heller, Martina Krämer, Michael Ponater, Christian Rolf, Ina Tegen, and Christiane Voigt
Geosci. Model Dev., 13, 1635–1661, https://doi.org/10.5194/gmd-13-1635-2020, https://doi.org/10.5194/gmd-13-1635-2020, 2020
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A new cloud microphysical scheme is implemented in the global EMAC-MADE3 aerosol model and evaluated. The new scheme features a detailed parameterization for aerosol-driven ice formation in cirrus clouds, accounting for the competition between homogeneous and heterogeneous ice formation processes. The comparison against satellite data and in situ measurements shows that the model performance is in line with similar global coupled models featuring ice cloud parameterizations.
Emmanuel Fontaine, Alfons Schwarzenboeck, Delphine Leroy, Julien Delanoë, Alain Protat, Fabien Dezitter, John Walter Strapp, and Lyle Edward Lilie
Atmos. Chem. Phys., 20, 3503–3553, https://doi.org/10.5194/acp-20-3503-2020, https://doi.org/10.5194/acp-20-3503-2020, 2020
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This study investigates properties of ice hydrometeors (shape, concentration, density, and size) in deep convective systems. The analysis focuses on similarities and differences over four locations in the tropical troposphere. It shows that measurements as a function of temperature and radar reflectivity factors tend to be similar in the four types of deep convective systems when concentrations of ice are larger than 0.1 g m-3.
Rosa Gierens, Stefan Kneifel, Matthew D. Shupe, Kerstin Ebell, Marion Maturilli, and Ulrich Löhnert
Atmos. Chem. Phys., 20, 3459–3481, https://doi.org/10.5194/acp-20-3459-2020, https://doi.org/10.5194/acp-20-3459-2020, 2020
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Multiyear statistics of persistent low-level mixed-phase clouds observed at an Arctic fjord environment in Svalbard are presented. The effects the local boundary layer (i.e. the fjords' wind climate and surface coupling), regional wind direction, and seasonality have on the cloud occurrence and properties are evaluated using a synergy of ground-based remote sensing methods and auxiliary data. The phenomena considered were found to modify the amount of liquid and ice in the studied clouds.
Lucas Höppler, Felix Gödde, Manuel Gutleben, Tobias Kölling, Bernhard Mayer, and Tobias Zinner
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-49, https://doi.org/10.5194/amt-2020-49, 2020
Publication in AMT not foreseen
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Clouds are considered as two-dimensional in many climate and weather models. This approach creates errors due to wrongly calculated solar or terrestrial radiative transfer. In order to reduce these errors, realistic three-dimensional clouds need to be retrieved or reproduced. This paper shows an approach to retrieve realistic three-dimensional clouds from an airplane, by combining the strengths of several active and passive remote sensing instruments.
Paul Ockenfuß, Claudia Emde, Bernhard Mayer, and Germar Bernhard
Atmos. Chem. Phys., 20, 1961–1976, https://doi.org/10.5194/acp-20-1961-2020, https://doi.org/10.5194/acp-20-1961-2020, 2020
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We model solar radiation as it would be measured on the Earth's surface in the core shadow of a total solar eclipse. Subsequently, we compare our results to observations during the total eclipse 2017 for ultraviolet, visible and near-infrared wavelengths. Moreover, we analyze the effect of the surface reflectance, the ozone profile, aerosol and the topography and give a visualization of the prevailing photons paths in the atmosphere during the eclipse.
Paul A. Barrett, Alan Blyth, Philip R. A. Brown, and Steven J. Abel
Atmos. Chem. Phys., 20, 1921–1939, https://doi.org/10.5194/acp-20-1921-2020, https://doi.org/10.5194/acp-20-1921-2020, 2020
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Here we present new in situ observations from altocumulus clouds made with a research aircraft. By carefully measuring the cloud top height, we are able to study the turbulence and cloud properties in high vertical resolution, something not presented before. The clouds contain both ice particles and liquid drops, even though the temperature is −30 °C. These measurements will hopefully assist future developers of climate models to verify and assess the performance of simulations.
Tobias Marke, Ulrich Löhnert, Vera Schemann, Jan H. Schween, and Susanne Crewell
Atmos. Chem. Phys., 20, 1723–1736, https://doi.org/10.5194/acp-20-1723-2020, https://doi.org/10.5194/acp-20-1723-2020, 2020
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In this study, land surface and atmosphere interactions are addressed using ground-based remote sensing, satellite products, and high-resolution large-eddy simulations. The focus is on water vapor transport from the surface into the atmosphere. Patterns found in long-term observations can be linked to properties of the surrounding land surface. The simulation results suggest that a different distribution of land use types has implications for boundary layer characteristics and clouds.
Fan Mei, Jian Wang, Jennifer M. Comstock, Ralf Weigel, Martina Krämer, Christoph Mahnke, John E. Shilling, Johannes Schneider, Christiane Schulz, Charles N. Long, Manfred Wendisch, Luiz A. T. Machado, Beat Schmid, Trismono Krisna, Mikhail Pekour, John Hubbe, Andreas Giez, Bernadett Weinzierl, Martin Zoeger, Mira L. Pöhlker, Hans Schlager, Micael A. Cecchini, Meinrat O. Andreae, Scot T. Martin, Suzane S. de Sá, Jiwen Fan, Jason Tomlinson, Stephen Springston, Ulrich Pöschl, Paulo Artaxo, Christopher Pöhlker, Thomas Klimach, Andreas Minikin, Armin Afchine, and Stephan Borrmann
Atmos. Meas. Tech., 13, 661–684, https://doi.org/10.5194/amt-13-661-2020, https://doi.org/10.5194/amt-13-661-2020, 2020
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In 2014, the US DOE G1 aircraft and the German HALO aircraft overflew the Amazon basin to study how aerosols influence cloud cycles under a clean condition and around a tropical megacity. This paper describes how to meaningfully compare similar measurements from two research aircraft and identify the potential measurement issue. We also discuss the uncertainty range for each measurement for further usage in model evaluation and satellite data validation.
Pascal Polonik, Christoph Knote, Tobias Zinner, Florian Ewald, Tobias Kölling, Bernhard Mayer, Meinrat O. Andreae, Tina Jurkat-Witschas, Thomas Klimach, Christoph Mahnke, Sergej Molleker, Christopher Pöhlker, Mira L. Pöhlker, Ulrich Pöschl, Daniel Rosenfeld, Christiane Voigt, Ralf Weigel, and Manfred Wendisch
Atmos. Chem. Phys., 20, 1591–1605, https://doi.org/10.5194/acp-20-1591-2020, https://doi.org/10.5194/acp-20-1591-2020, 2020
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A realistic representation of cloud–aerosol interactions is central to accurate climate projections. Here we combine observations collected during the ACRIDICON-CHUVA campaign with chemistry-transport simulations to evaluate the model’s ability to represent the indirect effects of biomass burning aerosol on cloud microphysics. We find an upper limit for the model sensitivity on cloud condensation nuclei concentrations well below the levels reached during the burning season in the Amazon Basin.
Xianda Gong, Heike Wex, Jens Voigtländer, Khanneh Wadinga Fomba, Kay Weinhold, Manuela van Pinxteren, Silvia Henning, Thomas Müller, Hartmut Herrmann, and Frank Stratmann
Atmos. Chem. Phys., 20, 1431–1449, https://doi.org/10.5194/acp-20-1431-2020, https://doi.org/10.5194/acp-20-1431-2020, 2020
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We characterized the aerosol particles in Cabo Verde at sea and cloud levels. We found four well-separable types of PNSDs, with the strongest differences between air masses coming from the ocean compared to from the African continent. During the strongest observed dust periods, CCN concentrations were 2.5 higher than during clean marine periods. The hygroscopicity of the particles did not vary much between different periods. Aerosol at sea level and on the mountaintop was well in agreement.
Xianda Gong, Heike Wex, Manuela van Pinxteren, Nadja Triesch, Khanneh Wadinga Fomba, Jasmin Lubitz, Christian Stolle, Tiera-Brandy Robinson, Thomas Müller, Hartmut Herrmann, and Frank Stratmann
Atmos. Chem. Phys., 20, 1451–1468, https://doi.org/10.5194/acp-20-1451-2020, https://doi.org/10.5194/acp-20-1451-2020, 2020
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In this study, we examined number concentrations of ice nucleating particles (INPs) at Cabo Verde in the oceanic sea surface microlayer and underlying seawater, in the air close to both sea level and cloud level, and in cloud water. The results show that most INPs are supermicron in size, that INP number concentrations in air fit well to those in cloud water and that sea spray aerosols at maximum contributed a small fraction of all INPs in the air at Cabo Verde.
Christine Pohl, Larysa Istomina, Steffen Tietsche, Evelyn Jäkel, Johannes Stapf, Gunnar Spreen, and Georg Heygster
The Cryosphere, 14, 165–182, https://doi.org/10.5194/tc-14-165-2020, https://doi.org/10.5194/tc-14-165-2020, 2020
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A spectral to broadband conversion is developed empirically that can be used in combination with the Melt Pond Detector algorithm to derive broadband albedo (300–3000 nm) of Arctic sea ice from MERIS data. It is validated and shows better performance compared to existing conversion methods. A comparison of MERIS broadband albedo with respective values from ERA5 reanalysis suggests a revision of the albedo values used in ERA5. MERIS albedo might be useful for improving albedo representation.
Hans Grob, Claudia Emde, Matthias Wiegner, Meinhard Seefeldner, Linda Forster, and Bernhard Mayer
Atmos. Meas. Tech., 13, 239–258, https://doi.org/10.5194/amt-13-239-2020, https://doi.org/10.5194/amt-13-239-2020, 2020
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Polarimetry has been established as an enhancement to classical photometry in aerosol remote sensing over the past years. We propose a fast and exact radiometric and polarimetric calibration method for polarized photometers. Additionally, a technique for correcting an alt-azimuthal mount is introduced.
These methods are applied to measurements obtained with our SSARA instrument during the A-LIFE field campaign. For 2 d, the data are subjected to an inversion of aerosol optical properties.
Vera Schemann and Kerstin Ebell
Atmos. Chem. Phys., 20, 475–485, https://doi.org/10.5194/acp-20-475-2020, https://doi.org/10.5194/acp-20-475-2020, 2020
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In this study, we apply a high-resolution model at the observation supersite Ny-Ålesund (Svalbard) to evaluate mixed-phase clouds. These clouds are a potential driver for the stronger warming in the Arctic compared to the global mean, but their representation in climate models is typically rather poor due to complex microphysical processes. The presented combination of high-resolution modeling and long-term state-of-the-art observations can lead to improved process understanding.
Sophie L. Haslett, Jonathan W. Taylor, Mathew Evans, Eleanor Morris, Bernhard Vogel, Alima Dajuma, Joel Brito, Anneke M. Batenburg, Stephan Borrmann, Johannes Schneider, Christiane Schulz, Cyrielle Denjean, Thierry Bourrianne, Peter Knippertz, Régis Dupuy, Alfons Schwarzenböck, Daniel Sauer, Cyrille Flamant, James Dorsey, Ian Crawford, and Hugh Coe
Atmos. Chem. Phys., 19, 15217–15234, https://doi.org/10.5194/acp-19-15217-2019, https://doi.org/10.5194/acp-19-15217-2019, 2019
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Three aircraft datasets from the DACCIWA campaign in summer 2016 are used here to show there is a background mass of pollution present in the lower atmosphere in southern West Africa. We suggest that this likely comes from biomass burning in central and southern Africa, which has been carried into the region over the Atlantic Ocean. This would have a negative health impact on populations living near the coast and may alter the impact of growing city emissions on cloud formation and the monsoon.
Heiko Bozem, Peter Hoor, Daniel Kunkel, Franziska Köllner, Johannes Schneider, Andreas Herber, Hannes Schulz, W. Richard Leaitch, Amir A. Aliabadi, Megan D. Willis, Julia Burkart, and Jonathan P. D. Abbatt
Atmos. Chem. Phys., 19, 15049–15071, https://doi.org/10.5194/acp-19-15049-2019, https://doi.org/10.5194/acp-19-15049-2019, 2019
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We present airborne trace gas measurements in the European and Canadian Arctic for July 2014 and April 2015. Based on CO and CO2 in situ data as well as 10 d kinematic back trajectories, we characterize the prevailing transport regimes and derive a tracer-based diagnostic for the determination of the polar dome boundary. Using the tracer-derived boundary, an analysis of the recent transport history of air masses within the polar dome reveals significant differences between spring and summer.
Sabrina P. Cochrane, K. Sebastian Schmidt, Hong Chen, Peter Pilewskie, Scott Kittelman, Jens Redemann, Samuel LeBlanc, Kristina Pistone, Meloë Kacenelenbogen, Michal Segal Rozenhaimer, Yohei Shinozuka, Connor Flynn, Steven Platnick, Kerry Meyer, Rich Ferrare, Sharon Burton, Chris Hostetler, Steven Howell, Steffen Freitag, Amie Dobracki, and Sarah Doherty
Atmos. Meas. Tech., 12, 6505–6528, https://doi.org/10.5194/amt-12-6505-2019, https://doi.org/10.5194/amt-12-6505-2019, 2019
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For two cases from the NASA ORACLES experiments, we retrieve aerosol and cloud properties and calculate a direct aerosol radiative effect (DARE). We investigate the relationship between DARE and the cloud albedo by specifying the albedo for which DARE transitions from a cooling to warming radiative effect. Our new aerosol retrieval algorithm is successful despite complexities associated with scenes that contain aerosols above clouds and decreases the uncertainty on retrieved aerosol parameters.
Anna T. Kunert, Mira L. Pöhlker, Kai Tang, Carola S. Krevert, Carsten Wieder, Kai R. Speth, Linda E. Hanson, Cindy E. Morris, David G. Schmale III, Ulrich Pöschl, and Janine Fröhlich-Nowoisky
Biogeosciences, 16, 4647–4659, https://doi.org/10.5194/bg-16-4647-2019, https://doi.org/10.5194/bg-16-4647-2019, 2019
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A screening of more than 100 strains from 65 different species revealed that the ice nucleation activity within the fungal genus Fusarium is more widespread than previously assumed. Filtration experiments suggest that the single cell-free Fusarium IN is smaller than 100 kDa (~ 6 nm) and that aggregates can be formed in solution. Exposure experiments, freeze–thaw cycles, and long-term storage tests demonstrate a high stability of Fusarium IN under atmospherically relevant conditions.
Ignacio Pisso, Espen Sollum, Henrik Grythe, Nina I. Kristiansen, Massimo Cassiani, Sabine Eckhardt, Delia Arnold, Don Morton, Rona L. Thompson, Christine D. Groot Zwaaftink, Nikolaos Evangeliou, Harald Sodemann, Leopold Haimberger, Stephan Henne, Dominik Brunner, John F. Burkhart, Anne Fouilloux, Jerome Brioude, Anne Philipp, Petra Seibert, and Andreas Stohl
Geosci. Model Dev., 12, 4955–4997, https://doi.org/10.5194/gmd-12-4955-2019, https://doi.org/10.5194/gmd-12-4955-2019, 2019
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We present the latest release of the Lagrangian transport model FLEXPART, which simulates the transport, diffusion, dry and wet deposition, radioactive decay, and 1st-order chemical reactions of atmospheric tracers. The model has been recently updated both technically and in the representation of physicochemical processes. We describe the changes, document the most recent input and output files, provide working examples, and introduce testing capabilities.
Carlos Toledano, Benjamín Torres, Cristian Velasco-Merino, Dietrich Althausen, Silke Groß, Matthias Wiegner, Bernadett Weinzierl, Josef Gasteiger, Albert Ansmann, Ramiro González, David Mateos, David Farrel, Thomas Müller, Moritz Haarig, and Victoria E. Cachorro
Atmos. Chem. Phys., 19, 14571–14583, https://doi.org/10.5194/acp-19-14571-2019, https://doi.org/10.5194/acp-19-14571-2019, 2019
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Ground-based sun photometers have been used to analyze the properties of long-range transported Saharan dust over Barbados. The measurements were carried out as part of the Saharan Aerosol Long-Range Transport and Aerosol–Cloud-Interaction Experiment (SALTRACE), carried out in the Caribbean in 2013. A variety of instruments, ground-based and airborne, were used in this research. In this paper, the sun photometer data are presented and related to data collected from other co-located instruments.
André Ehrlich, Manfred Wendisch, Christof Lüpkes, Matthias Buschmann, Heiko Bozem, Dmitri Chechin, Hans-Christian Clemen, Régis Dupuy, Olliver Eppers, Jörg Hartmann, Andreas Herber, Evelyn Jäkel, Emma Järvinen, Olivier Jourdan, Udo Kästner, Leif-Leonard Kliesch, Franziska Köllner, Mario Mech, Stephan Mertes, Roland Neuber, Elena Ruiz-Donoso, Martin Schnaiter, Johannes Schneider, Johannes Stapf, and Marco Zanatta
Earth Syst. Sci. Data, 11, 1853–1881, https://doi.org/10.5194/essd-11-1853-2019, https://doi.org/10.5194/essd-11-1853-2019, 2019
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During the Arctic CLoud Observations Using airborne measurements during polar Day (ACLOUD) campaign, two research aircraft (Polar 5 and 6) jointly performed 22 research flights over the transition zone between open ocean and closed sea ice. The data set combines remote sensing and in situ measurement of cloud, aerosol, and trace gas properties, as well as turbulent and radiative fluxes, which will be used to study Arctic boundary layer and mid-level clouds and their role in Arctic amplification.
Zsófia Jurányi and Rolf Weller
Atmos. Chem. Phys., 19, 14417–14430, https://doi.org/10.5194/acp-19-14417-2019, https://doi.org/10.5194/acp-19-14417-2019, 2019
Simonas Kecorius, Teresa Vogl, Pauli Paasonen, Janne Lampilahti, Daniel Rothenberg, Heike Wex, Sebastian Zeppenfeld, Manuela van Pinxteren, Markus Hartmann, Silvia Henning, Xianda Gong, Andre Welti, Markku Kulmala, Frank Stratmann, Hartmut Herrmann, and Alfred Wiedensohler
Atmos. Chem. Phys., 19, 14339–14364, https://doi.org/10.5194/acp-19-14339-2019, https://doi.org/10.5194/acp-19-14339-2019, 2019
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Arctic sea-ice retreat, atmospheric new particle formation (NPF), and aerosol–cloud interaction may all be linked via a positive feedback mechanism. Understanding the sources of cloud condensation nuclei (CCN) is an important piece in the Arctic amplification puzzle. We show that Arctic newly formed particles do not have to grow beyond the Aitken mode to act as CCN. This is important, because NPF occurrence in the Arctic is expected to increase, making it a significant contributor to CCN budget.
Andrea Spolaor, Elena Barbaro, David Cappelletti, Clara Turetta, Mauro Mazzola, Fabio Giardi, Mats P. Björkman, Federico Lucchetta, Federico Dallo, Katrine Aspmo Pfaffhuber, Hélène Angot, Aurelien Dommergue, Marion Maturilli, Alfonso Saiz-Lopez, Carlo Barbante, and Warren R. L. Cairns
Atmos. Chem. Phys., 19, 13325–13339, https://doi.org/10.5194/acp-19-13325-2019, https://doi.org/10.5194/acp-19-13325-2019, 2019
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The main aims of the study are to (a) detect whether mercury in the surface snow undergoes a daily cycle as determined in the atmosphere, (b) compare the mercury concentration in surface snow with the concentration in the atmosphere, (c) evaluate the effect of snow depositions, (d) detect whether iodine and bromine in the surface snow undergo a daily cycle, and (e) evaluate the role of metereological and atmospheric conditions. Different behaviours were determined during different seasons.
Horst Fischer, Raoul Axinte, Heiko Bozem, John N. Crowley, Cheryl Ernest, Stefan Gilge, Sascha Hafermann, Hartwig Harder, Korbinian Hens, Ruud H. H. Janssen, Rainer Königstedt, Dagmar Kubistin, Chinmay Mallik, Monica Martinez, Anna Novelli, Uwe Parchatka, Christian Plass-Dülmer, Andrea Pozzer, Eric Regelin, Andreas Reiffs, Torsten Schmidt, Jan Schuladen, and Jos Lelieveld
Atmos. Chem. Phys., 19, 11953–11968, https://doi.org/10.5194/acp-19-11953-2019, https://doi.org/10.5194/acp-19-11953-2019, 2019
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We use in situ observations of H2O2 to study the interplay between photochemistry, transport and deposition processes. The data were obtained during five ground-based field campaigns across Europe. A budget calculation indicates that the photochemical production rate was much larger than photochemical loss and that dry deposition is the dominant loss process. To reproduce the change in H2O2 mixing ratios after sunrise, a variable contribution of entrainment from the residual layer is required.
Mario Mech, Leif-Leonard Kliesch, Andreas Anhäuser, Thomas Rose, Pavlos Kollias, and Susanne Crewell
Atmos. Meas. Tech., 12, 5019–5037, https://doi.org/10.5194/amt-12-5019-2019, https://doi.org/10.5194/amt-12-5019-2019, 2019
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An improved understanding of Arctic mixed-phase clouds and their contribution to Arctic warming can be achieved by observations from airborne platforms with remote sensing instruments. Such an instrument is MiRAC combining active and passive techniques to gain information on the distribution of clouds, the occurrence of precipitation, and the amount of liquid and ice within the cloud. Operated during a campaign in Arctic summer, it could observe lower clouds often not seen by spaceborne radars.
Eleni Marinou, Matthias Tesche, Athanasios Nenes, Albert Ansmann, Jann Schrod, Dimitra Mamali, Alexandra Tsekeri, Michael Pikridas, Holger Baars, Ronny Engelmann, Kalliopi-Artemis Voudouri, Stavros Solomos, Jean Sciare, Silke Groß, Florian Ewald, and Vassilis Amiridis
Atmos. Chem. Phys., 19, 11315–11342, https://doi.org/10.5194/acp-19-11315-2019, https://doi.org/10.5194/acp-19-11315-2019, 2019
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We assess the feasibility of ground-based and spaceborne lidars to retrieve profiles of cloud-relevant aerosol concentrations and ice-nucleating particles. The retrieved profiles are in good agreement with airborne in situ measurements. Our methodology will be applied to satellite observations in the future so as to provide a global 3D product of cloud-relevant properties.
Jacob Schacht, Bernd Heinold, Johannes Quaas, John Backman, Ribu Cherian, Andre Ehrlich, Andreas Herber, Wan Ting Katty Huang, Yutaka Kondo, Andreas Massling, P. R. Sinha, Bernadett Weinzierl, Marco Zanatta, and Ina Tegen
Atmos. Chem. Phys., 19, 11159–11183, https://doi.org/10.5194/acp-19-11159-2019, https://doi.org/10.5194/acp-19-11159-2019, 2019
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The Arctic is warming faster than the rest of Earth. Black carbon (BC) aerosol contributes to this Arctic amplification by direct and indirect aerosol radiative effects while distributed in air or deposited on snow and ice. The aerosol-climate model ECHAM-HAM is used to estimate direct aerosol radiative effect (DRE). Airborne and near-surface BC measurements are used to evaluate the model and give an uncertainty range for the burden and DRE of Arctic BC caused by different emission inventories.
Xianda Gong, Heike Wex, Thomas Müller, Alfred Wiedensohler, Kristina Höhler, Konrad Kandler, Nan Ma, Barbara Dietel, Thea Schiebel, Ottmar Möhler, and Frank Stratmann
Atmos. Chem. Phys., 19, 10883–10900, https://doi.org/10.5194/acp-19-10883-2019, https://doi.org/10.5194/acp-19-10883-2019, 2019
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For the diverse aerosol on Cyprus, we found the following: new particle formation can be a source of cloud condensation nuclei. Particle hygroscopicity showed that particles ~<100 nm contained mostly organic material, while larger ones were more hygroscopic. Two separate methods obtained similar concentrations of ice-nucleating particles (INP), with mostly no evidence of a local origin. Different parameterizations overestimated INP concentration in this rather polluted region.
Andreas Marsing, Tina Jurkat-Witschas, Jens-Uwe Grooß, Stefan Kaufmann, Romy Heller, Andreas Engel, Peter Hoor, Jens Krause, and Christiane Voigt
Atmos. Chem. Phys., 19, 10757–10772, https://doi.org/10.5194/acp-19-10757-2019, https://doi.org/10.5194/acp-19-10757-2019, 2019
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We study the partitioning of inorganic chlorine into active (ozone-depleting) and reservoir species in the lowermost stratosphere of the Arctic polar vortex, using novel in situ aircraft measurements in winter 2015/2016. We observe a change in recovery pathways of the reservoirs HCl and ClONO2 with increasing potential temperature. A comparison with the CLaMS model relates the observations to the vortex-wide evolution and confirms unresolved discrepancies in the mid-winter HCl distribution.
Manuel Gutleben, Silke Groß, and Martin Wirth
Atmos. Chem. Phys., 19, 10659–10673, https://doi.org/10.5194/acp-19-10659-2019, https://doi.org/10.5194/acp-19-10659-2019, 2019
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This study concentrates on airborne lidar measurements conducted during the NARVAL field experiments over the western subtropical North Atlantic Ocean to study differences between shallow marine cloud macro-physical properties (i.e. cloud fraction, cloud top height, cloud length, cloud gap length) in Saharan-dust-laden and dust-free trade wind regions. Cloud top heights, cloud fractions and cloud lengths are found to be lower and smaller in Saharan-dust-laden compared to dust-free regions.
Fanny Peers, Peter Francis, Cathryn Fox, Steven J. Abel, Kate Szpek, Michael I. Cotterell, Nicholas W. Davies, Justin M. Langridge, Kerry G. Meyer, Steven E. Platnick, and Jim M. Haywood
Atmos. Chem. Phys., 19, 9595–9611, https://doi.org/10.5194/acp-19-9595-2019, https://doi.org/10.5194/acp-19-9595-2019, 2019
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The measurements from the geostationary satellite MSG/SEVIRI are used to retrieve the cloud and above-cloud aerosol properties over the South Atlantic. The technique relies on the spectral contrast and the magnitude of the signal in the visible to shortwave infrared region as well as the atmospheric correction based on forecasted water vapour profiles. The sensitivity analysis and the stability of the retrieval over time show great potential of the high-temporal-resolution observations.
Valentin Ludwig, Gunnar Spreen, Christian Haas, Larysa Istomina, Frank Kauker, and Dmitrii Murashkin
The Cryosphere, 13, 2051–2073, https://doi.org/10.5194/tc-13-2051-2019, https://doi.org/10.5194/tc-13-2051-2019, 2019
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Sea-ice concentration, the fraction of an area covered by sea ice, can be observed from satellites with different methods. We combine two methods to obtain a product which is better than either of the input measurements alone. The benefit of our product is demonstrated by observing the formation of an open water area which can now be observed with more detail. Additionally, we find that the open water area formed because the sea ice drifted in the opposite direction and faster than usual.
Helge Knoop, Felix Ament, and Björn Maronga
Adv. Sci. Res., 16, 143–148, https://doi.org/10.5194/asr-16-143-2019, https://doi.org/10.5194/asr-16-143-2019, 2019
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This paper proposes a new generic method to define and detect wind gusts from high-resolution wind velocity data. The method describes any specific gust by an amplitude and period and allows the detection of individual gusts in time using wavelet-analysis. The result of a full gust analysis using this method yields a so-called characteristic gust distribution for the respective wind velocity data, which can serve as a direct link to the physical impact a particular gust has on e.g. an aircraft.
Ulrike Egerer, Matthias Gottschalk, Holger Siebert, André Ehrlich, and Manfred Wendisch
Atmos. Meas. Tech., 12, 4019–4038, https://doi.org/10.5194/amt-12-4019-2019, https://doi.org/10.5194/amt-12-4019-2019, 2019
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In this study, we introduce the new tethered balloon system BELUGA, which includes different modular instrument packages for measuring turbulence and radiation in the atmospheric boundary layer. BELUGA was deployed in an Arctic field campaign in 2017, providing details of boundary layer processes in combination with low-level clouds. Those processes are still not fully understood and in situ measurements in the Arctic improve our understanding of the Arctic response in terms of global warming.
Kristina Pistone, Jens Redemann, Sarah Doherty, Paquita Zuidema, Sharon Burton, Brian Cairns, Sabrina Cochrane, Richard Ferrare, Connor Flynn, Steffen Freitag, Steven G. Howell, Meloë Kacenelenbogen, Samuel LeBlanc, Xu Liu, K. Sebastian Schmidt, Arthur J. Sedlacek III, Michal Segal-Rozenhaimer, Yohei Shinozuka, Snorre Stamnes, Bastiaan van Diedenhoven, Gerard Van Harten, and Feng Xu
Atmos. Chem. Phys., 19, 9181–9208, https://doi.org/10.5194/acp-19-9181-2019, https://doi.org/10.5194/acp-19-9181-2019, 2019
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Understanding how smoke particles interact with sunlight is important in calculating their effects on climate, since some smoke is more scattering (cooling) and some is more absorbing (heating). Knowing this proportion is important for both satellite observations and climate models. We measured smoke properties in a recent aircraft-based field campaign off the west coast of Africa and present a comparison of these properties as measured using the six different, independent techniques available.
Jan Chylik, Stephan Mertes, and Roel A. J. Neggers
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2019-637, https://doi.org/10.5194/acp-2019-637, 2019
Preprint withdrawn
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Arctic low-levels clouds play an important role in the Arctic warming, however they are not properly represented in weather and climate models. Among other issues, there are difficulties with balance of ice and liquid in clouds, as well as interaction between clouds and aerosols. In this model study, we focus on the way that variation in the concentration of aerosols affect the evolution of clouds and the turbulence. Model scenarios are based on the observations during the ACLOUD campaign.
Jonathan W. Taylor, Sophie L. Haslett, Keith Bower, Michael Flynn, Ian Crawford, James Dorsey, Tom Choularton, Paul J. Connolly, Valerian Hahn, Christiane Voigt, Daniel Sauer, Régis Dupuy, Joel Brito, Alfons Schwarzenboeck, Thierry Bourriane, Cyrielle Denjean, Phil Rosenberg, Cyrille Flamant, James D. Lee, Adam R. Vaughan, Peter G. Hill, Barbara Brooks, Valéry Catoire, Peter Knippertz, and Hugh Coe
Atmos. Chem. Phys., 19, 8503–8522, https://doi.org/10.5194/acp-19-8503-2019, https://doi.org/10.5194/acp-19-8503-2019, 2019
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Low-level clouds cover a wide area of southern West Africa (SWA) and play an important role in the region's climate, reflecting sunlight away from the surface. We performed aircraft measurements of aerosols and clouds over SWA during the 2016 summer monsoon and found pollution, and polluted clouds, across the whole region. Smoke from biomass burning in Central Africa is transported to West Africa, causing a polluted background which limits the effect of local pollution on cloud properties.
Christopher Pöhlker, David Walter, Hauke Paulsen, Tobias Könemann, Emilio Rodríguez-Caballero, Daniel Moran-Zuloaga, Joel Brito, Samara Carbone, Céline Degrendele, Viviane R. Després, Florian Ditas, Bruna A. Holanda, Johannes W. Kaiser, Gerhard Lammel, Jošt V. Lavrič, Jing Ming, Daniel Pickersgill, Mira L. Pöhlker, Maria Praß, Nina Löbs, Jorge Saturno, Matthias Sörgel, Qiaoqiao Wang, Bettina Weber, Stefan Wolff, Paulo Artaxo, Ulrich Pöschl, and Meinrat O. Andreae
Atmos. Chem. Phys., 19, 8425–8470, https://doi.org/10.5194/acp-19-8425-2019, https://doi.org/10.5194/acp-19-8425-2019, 2019
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The Amazon Tall Tower Observatory (ATTO) has been established to monitor the rain forest's biosphere–atmosphere exchange, which experiences the combined pressures from human-made deforestation and progressing climate change. This work is meant to be a reference study, which characterizes various geospatial properties of the ATTO footprint region and shows how the human-made transformation of Amazonia may impact future atmospheric observations at ATTO.
Heike Konow, Marek Jacob, Felix Ament, Susanne Crewell, Florian Ewald, Martin Hagen, Lutz Hirsch, Friedhelm Jansen, Mario Mech, and Bjorn Stevens
Earth Syst. Sci. Data, 11, 921–934, https://doi.org/10.5194/essd-11-921-2019, https://doi.org/10.5194/essd-11-921-2019, 2019
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High-resolution measurements of maritime clouds are relatively scarce. Airborne cloud radar, microwave radiometer and dropsonde observations are used to expand these data. The measurements are unified into one data set to enable easy joint analyses of several or all instruments together to gain insight into cloud properties and atmospheric state. The data set contains measurements from four campaigns between December 2013 and October 2016 over the tropical and midlatitude Atlantic.
Evelyn Jäkel, Johannes Stapf, Manfred Wendisch, Marcel Nicolaus, Wolfgang Dorn, and Annette Rinke
The Cryosphere, 13, 1695–1708, https://doi.org/10.5194/tc-13-1695-2019, https://doi.org/10.5194/tc-13-1695-2019, 2019
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The sea ice surface albedo parameterization of a coupled regional climate model was validated against aircraft measurements performed in May–June 2017 north of Svalbard. The albedo parameterization was run offline from the model using the measured parameters surface temperature and snow depth to calculate the surface albedo and the individual fractions of the ice surface subtypes. An adjustment of the variables and additionally accounting for cloud cover reduced the root-mean-squared error.
Nina Črnivec and Bernhard Mayer
Atmos. Chem. Phys., 19, 8083–8100, https://doi.org/10.5194/acp-19-8083-2019, https://doi.org/10.5194/acp-19-8083-2019, 2019
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The interaction between radiation and clouds represents a source of uncertainty in numerical weather prediction (NWP), due to both intrinsic problems of one-dimensional radiation schemes and poor representation of clouds. The underlying question addressed in this study is how large the bias is of radiative heating rates in NWP models for shallow cumulus clouds and how it scales with various parameters, such as solar zenith angle, surface albedo, cloud cover and liquid water path.
Marek Jacob, Felix Ament, Manuel Gutleben, Heike Konow, Mario Mech, Martin Wirth, and Susanne Crewell
Atmos. Meas. Tech., 12, 3237–3254, https://doi.org/10.5194/amt-12-3237-2019, https://doi.org/10.5194/amt-12-3237-2019, 2019
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Tropical clouds are a key climate component but are still not fully understood. Therefore, we analyze airborne remote sensing measurements that were taken in the dry and wet seasons over the Atlantic east of Barbados. From these we derive sub-kilometer resolution data of vertically integrated atmospheric water vapor and liquid water. Results show that although the humidity is lower in the dry season, clouds are more frequent, contain more water, and produce more rain than in the wet season.
José Dias Neto, Stefan Kneifel, Davide Ori, Silke Trömel, Jan Handwerker, Birger Bohn, Normen Hermes, Kai Mühlbauer, Martin Lenefer, and Clemens Simmer
Earth Syst. Sci. Data, 11, 845–863, https://doi.org/10.5194/essd-11-845-2019, https://doi.org/10.5194/essd-11-845-2019, 2019
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This study describes a 2-month dataset of ground-based, vertically pointing triple-frequency cloud radar observations recorded during the winter season 2015/2016 in Jülich, Germany. Intensive quality control has been applied to the unique long-term dataset, which allows the multifrequency signatures of ice and snow particles to be statistically analyzed for the first time. The analysis includes, for example, aggregation and its dependence on cloud temperature, riming, and onset of melting.
Maximilian Maahn, Fabian Hoffmann, Matthew D. Shupe, Gijs de Boer, Sergey Y. Matrosov, and Edward P. Luke
Atmos. Meas. Tech., 12, 3151–3171, https://doi.org/10.5194/amt-12-3151-2019, https://doi.org/10.5194/amt-12-3151-2019, 2019
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Cloud radars are unique instruments for observing cloud processes, but uncertainties in radar calibration have frequently limited data quality. Here, we present three novel methods for calibrating vertically pointing cloud radars. These calibration methods are based on microphysical processes of liquid clouds, such as the transition of cloud droplets to drizzle drops. We successfully apply the methods to cloud radar data from the North Slope of Alaska (NSA) and Oliktok Point (OLI) ARM sites.
Sebastian J. O'Shea, Jonathan Crosier, James Dorsey, Waldemar Schledewitz, Ian Crawford, Stephan Borrmann, Richard Cotton, and Aaron Bansemer
Atmos. Meas. Tech., 12, 3067–3079, https://doi.org/10.5194/amt-12-3067-2019, https://doi.org/10.5194/amt-12-3067-2019, 2019
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Optical array probe measurements of clouds are widely used to inform and validate numerical weather and climate models. In this paper, we discuss artefacts which may bias data from these instruments. Using laboratory and synthetic datasets, we demonstrate how greyscale analysis can be used to filter data, constraining the sample volume and improving data quality particularly at small sizes where their measurements are considered unreliable.
Astrid Fremme and Harald Sodemann
Hydrol. Earth Syst. Sci., 23, 2525–2540, https://doi.org/10.5194/hess-23-2525-2019, https://doi.org/10.5194/hess-23-2525-2019, 2019
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This study examines the evaporation sources of precipitation falling over the Yangtze River valley on China's east coast. The summer monsoon rainfall causes large seasonal and interannual variations which affect a large population. We found that evaporation from surrounding land regions is important, supplying more than half of the summertime precipitation. Extreme dry and wet summers are connected to contributions from specific land and ocean regions.
Constantino Listowski, Julien Delanoë, Amélie Kirchgaessner, Tom Lachlan-Cope, and John King
Atmos. Chem. Phys., 19, 6771–6808, https://doi.org/10.5194/acp-19-6771-2019, https://doi.org/10.5194/acp-19-6771-2019, 2019
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Using satellite cloud products we investigate the supercooled liquid-water (SLW) distribution Antarctic-wide for the first time. We demonstrate differences between the monthly evolution of the marine low-level mixed-phase clouds and that of the marine low-level pure SLW clouds. In addition to the temperature and sea ice fraction as factors explaining the low-level liquid-cloud seasonal cycle, ice nuclei emissions from open water may also be driving the mixed-phase cloud monthly evolution.
Quitterie Cazenave, Marie Ceccaldi, Julien Delanoë, Jacques Pelon, Silke Groß, and Andrew Heymsfield
Atmos. Meas. Tech., 12, 2819–2835, https://doi.org/10.5194/amt-12-2819-2019, https://doi.org/10.5194/amt-12-2819-2019, 2019
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The impact of ice clouds on the water cycle and radiative budget is still uncertain due to the complexity of cloud processes that makes it difficult to acquire adequate observations of ice cloud properties and parameterize them into climate and weather prediction models. In this paper we present the latest refinements brought to the DARDAR-CLOUD product, which contains ice cloud microphysical properties retrieved from the cloud radar and lidar measurements from the A-Train space mission.
Wenfeng Huang, Bin Cheng, Jinrong Zhang, Zheng Zhang, Timo Vihma, Zhijun Li, and Fujun Niu
Hydrol. Earth Syst. Sci., 23, 2173–2186, https://doi.org/10.5194/hess-23-2173-2019, https://doi.org/10.5194/hess-23-2173-2019, 2019
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Up to now, little has been known on ice thermodynamics and lake–atmosphere interaction over the Tibetan Plateau during ice-covered seasons due to a lack of field data. Here, model experiments on ice thermodynamics were conducted in a shallow lake using HIGHTSI. Water–ice heat flux was a major source of uncertainty for lake ice thickness. Heat and mass budgets were estimated within the vertical air–ice–water system. Strong ice sublimation occurred and was responsible for water loss during winter.
Lejiang Yu, Shiyuan Zhong, and Timo Vihma
The Cryosphere Discuss., https://doi.org/10.5194/tc-2019-38, https://doi.org/10.5194/tc-2019-38, 2019
Manuscript not accepted for further review
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Arctic sea ice cover has been decreasing in recent decades. The reason for the decrease remains unclear. In this study, we examine the contributions of the North Pacific SST anomalies to the decrease. There are global warming and Pacific Decadal Oscillation (PDO) modesof the North Pacific SST variability in boreal summer and autumn. The global warming mode explains 44.9% and 50.1% of the Arctic sea ice loss in boreal summer and autumn, respectively. There are 22.0% and 22.2% for PDO mode.
Mary Borderies, Olivier Caumont, Julien Delanoë, Véronique Ducrocq, Nadia Fourrié, and Pascal Marquet
Nat. Hazards Earth Syst. Sci., 19, 907–926, https://doi.org/10.5194/nhess-19-907-2019, https://doi.org/10.5194/nhess-19-907-2019, 2019
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The potential of W-band radar reflectivity to improve the quality of analyses and forecasts of heavy precipitation events in the Mediterranean area is investigated. The 1D + 3DVar assimilation method has been adapted to assimilate the W-band reflectivity in the Météo-France kilometre-scale NWP model AROME. The results suggest that the joint assimilation of W-band reflectivity and horizontal wind profiles lead to a slight improvement of moisture analyses and rainfall precipitation forecasts.
Mary Borderies, Olivier Caumont, Julien Delanoë, Véronique Ducrocq, and Nadia Fourrié
Nat. Hazards Earth Syst. Sci., 19, 821–835, https://doi.org/10.5194/nhess-19-821-2019, https://doi.org/10.5194/nhess-19-821-2019, 2019
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The study reports on the impact of the assimilation of wind data from airborne Doppler cloud-profiling radar in a kilometre-scale NWP model on predicting heavy precipitation events in the Mediterranean area. The positive impact of the assimilation of such data is particularly evidenced for a heavy precipitation event and results are slightly encouraging over a 45-day period. In addition, the impact of the length of the assimilation window in a 3h-3DVar assimilation system is investigated.
Heike Wex, Lin Huang, Wendy Zhang, Hayley Hung, Rita Traversi, Silvia Becagli, Rebecca J. Sheesley, Claire E. Moffett, Tate E. Barrett, Rossana Bossi, Henrik Skov, Anja Hünerbein, Jasmin Lubitz, Mareike Löffler, Olivia Linke, Markus Hartmann, Paul Herenz, and Frank Stratmann
Atmos. Chem. Phys., 19, 5293–5311, https://doi.org/10.5194/acp-19-5293-2019, https://doi.org/10.5194/acp-19-5293-2019, 2019
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We found an annual cycle for ice-nucleating particles in the Arctic. These particles are important for Arctic clouds, as they can change the lifetime of clouds. We suggest that higher concentrations of these particles in summertime originate from the Arctic biosphere (both marine and terrestrial). With a warming Arctic, these concentrations may increase further, influencing aerosol–cloud interactions and therewith the observed strong warming of the Arctic.
Maiken Vassel, Luisa Ickes, Marion Maturilli, and Corinna Hoose
Atmos. Chem. Phys., 19, 5111–5126, https://doi.org/10.5194/acp-19-5111-2019, https://doi.org/10.5194/acp-19-5111-2019, 2019
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Multilayer clouds are coexisting clouds at different heights. We evaluate measurements and find that Arctic multilayer clouds occur in 29 % of the investigated days at Ny-Ålesund, Svalbard. Multilayer clouds can interact by ice crystals falling from the upper cloud into the lower cloud. This is possible in 23 % of the investigated days, and in 9 % it is not possible. Weather models are still error-prone in the Arctic and we suggest that multilayer clouds should be included more in future work.
Katarzyna Karpińska, Jonathan F. E. Bodenschatz, Szymon P. Malinowski, Jakub L. Nowak, Steffen Risius, Tina Schmeissner, Raymond A. Shaw, Holger Siebert, Hengdong Xi, Haitao Xu, and Eberhard Bodenschatz
Atmos. Chem. Phys., 19, 4991–5003, https://doi.org/10.5194/acp-19-4991-2019, https://doi.org/10.5194/acp-19-4991-2019, 2019
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Observations of clouds at a mountain-top laboratory revealed for the first time the presence of “voids”, i.e., elongated volumes inside a cloud that are devoid of droplets. Theoretical and numerical analyses suggest that these voids are a result of strong and long-lasting vortex presence in turbulent air. If this is confirmed in further investigation, the effect may become an important part of models describing cloud evolution and rain formation.
Marc Mallet, Pierre Nabat, Paquita Zuidema, Jens Redemann, Andrew Mark Sayer, Martin Stengel, Sebastian Schmidt, Sabrina Cochrane, Sharon Burton, Richard Ferrare, Kerry Meyer, Pablo Saide, Hiren Jethva, Omar Torres, Robert Wood, David Saint Martin, Romain Roehrig, Christina Hsu, and Paola Formenti
Atmos. Chem. Phys., 19, 4963–4990, https://doi.org/10.5194/acp-19-4963-2019, https://doi.org/10.5194/acp-19-4963-2019, 2019
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The model is able to represent LWP but not the LCF. AOD is consistent over the continent but also over ocean (ACAOD). Differences are observed in SSA due to the absence of internal mixing in ALADIN-Climate. A significant regional gradient of the forcing at TOA is observed. An intense positive forcing is simulated over Gabon. Results highlight the significant effect of enhanced moisture on BBA extinction. The surface dimming modifies the energy budget.
Naruki Hiranuma, Kouji Adachi, David M. Bell, Franco Belosi, Hassan Beydoun, Bhaskar Bhaduri, Heinz Bingemer, Carsten Budke, Hans-Christian Clemen, Franz Conen, Kimberly M. Cory, Joachim Curtius, Paul J. DeMott, Oliver Eppers, Sarah Grawe, Susan Hartmann, Nadine Hoffmann, Kristina Höhler, Evelyn Jantsch, Alexei Kiselev, Thomas Koop, Gourihar Kulkarni, Amelie Mayer, Masataka Murakami, Benjamin J. Murray, Alessia Nicosia, Markus D. Petters, Matteo Piazza, Michael Polen, Naama Reicher, Yinon Rudich, Atsushi Saito, Gianni Santachiara, Thea Schiebel, Gregg P. Schill, Johannes Schneider, Lior Segev, Emiliano Stopelli, Ryan C. Sullivan, Kaitlyn Suski, Miklós Szakáll, Takuya Tajiri, Hans Taylor, Yutaka Tobo, Romy Ullrich, Daniel Weber, Heike Wex, Thomas F. Whale, Craig L. Whiteside, Katsuya Yamashita, Alla Zelenyuk, and Ottmar Möhler
Atmos. Chem. Phys., 19, 4823–4849, https://doi.org/10.5194/acp-19-4823-2019, https://doi.org/10.5194/acp-19-4823-2019, 2019
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A total of 20 ice nucleation measurement techniques contributed to investigate the immersion freezing behavior of cellulose particles – natural polymers. Our data showed several types of cellulose are able to nucleate ice as efficiently as some mineral dust samples and cellulose has the potential to be an important atmospheric ice-nucleating particle. Continued investigation/collaboration is necessary to obtain further insight into consistency or diversity of ice nucleation measurements.
Tatiana Nomokonova, Kerstin Ebell, Ulrich Löhnert, Marion Maturilli, Christoph Ritter, and Ewan O'Connor
Atmos. Chem. Phys., 19, 4105–4126, https://doi.org/10.5194/acp-19-4105-2019, https://doi.org/10.5194/acp-19-4105-2019, 2019
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In this study, properties of clouds at the French–German Arctic research station in Ny-Ålesund are related to in-cloud thermodynamic conditions. The dataset used was collected within the Arctic Amplification project with a set of active and passive remote instruments. The results are compared with a model output. Significant divergence in observations and modelling of single-layer ice and mixed-phase clouds was found.
Stephanie Fiedler, Bjorn Stevens, Matthew Gidden, Steven J. Smith, Keywan Riahi, and Detlef van Vuuren
Geosci. Model Dev., 12, 989–1007, https://doi.org/10.5194/gmd-12-989-2019, https://doi.org/10.5194/gmd-12-989-2019, 2019
Florian Ewald, Silke Groß, Martin Hagen, Lutz Hirsch, Julien Delanoë, and Matthias Bauer-Pfundstein
Atmos. Meas. Tech., 12, 1815–1839, https://doi.org/10.5194/amt-12-1815-2019, https://doi.org/10.5194/amt-12-1815-2019, 2019
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This study gives a summary of lessons learned during the absolute calibration of the airborne, high-power Ka-band cloud radar HAMP MIRA on board the German research aircraft HALO. The first part covers the internal calibration of the instrument where individual instrument components are characterized in the laboratory. In the second part, the internal calibration is validated with external reference sources like the ocean surface backscatter and different air- and spaceborne cloud radars.
Christoph Böhm, Odran Sourdeval, Johannes Mülmenstädt, Johannes Quaas, and Susanne Crewell
Atmos. Meas. Tech., 12, 1841–1860, https://doi.org/10.5194/amt-12-1841-2019, https://doi.org/10.5194/amt-12-1841-2019, 2019
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The cloud base height (CBH) is important for air traffic, for describing the energy budget of the Earth and for other applications. Ground-based CBH measurements are only available for individual sites and mostly limited to land. Satellites are a powerful tool for global coverage. While the cloud top height is derived operationally, the derivation of CBH from space is more difficult as the clouds hide their base. Here, we present a method to retrieve the CBH from multi-angle satellite data.
Florentin Lemonnier, Jean-Baptiste Madeleine, Chantal Claud, Christophe Genthon, Claudio Durán-Alarcón, Cyril Palerme, Alexis Berne, Niels Souverijns, Nicole van Lipzig, Irina V. Gorodetskaya, Tristan L'Ecuyer, and Norman Wood
The Cryosphere, 13, 943–954, https://doi.org/10.5194/tc-13-943-2019, https://doi.org/10.5194/tc-13-943-2019, 2019
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Evaluation of the vertical precipitation rate profiles of CloudSat radar by comparison with two surface-based micro-rain radars (MRR) located at two antarctic stations gives a near-perfect correlation between both datasets, even though climatic and geographic conditions are different for the stations. A better understanding and reassessment of CloudSat uncertainties ranging from −13 % up to +22 % confirms the robustness of the CloudSat retrievals of snowfall over Antarctica.
Kevin Wolf, André Ehrlich, Marek Jacob, Susanne Crewell, Martin Wirth, and Manfred Wendisch
Atmos. Meas. Tech., 12, 1635–1658, https://doi.org/10.5194/amt-12-1635-2019, https://doi.org/10.5194/amt-12-1635-2019, 2019
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Using passive spectral solar radiation and active lidar, radar, and microwave measurements with HALO during NARVAL-II, the cloud droplet number concentration of shallow trade wind cumulus is estimated. With stepwise inclusion of the different instruments into the retrieval, the benefits of the synergetic approach based on artificial measurements and two cloud cases are demonstrated. Significant improvement with the synergetic method compared to the solar-radiation-only method is reported.
Cătălin Paţilea, Georg Heygster, Marcus Huntemann, and Gunnar Spreen
The Cryosphere, 13, 675–691, https://doi.org/10.5194/tc-13-675-2019, https://doi.org/10.5194/tc-13-675-2019, 2019
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Sea ice thickness is important for representing atmosphere–ocean interactions in climate models. A validated satellite sea ice thickness measurement algorithm is transferred to a new sensor. The results offer a better temporal and spatial coverage of satellite measurements in the polar regions. Here we describe the calibration procedure between the two sensors, taking into account their technical differences. In addition a new filter for interference from artificial radio sources is implemented.
Jonathan P. D. Abbatt, W. Richard Leaitch, Amir A. Aliabadi, Allan K. Bertram, Jean-Pierre Blanchet, Aude Boivin-Rioux, Heiko Bozem, Julia Burkart, Rachel Y. W. Chang, Joannie Charette, Jai P. Chaubey, Robert J. Christensen, Ana Cirisan, Douglas B. Collins, Betty Croft, Joelle Dionne, Greg J. Evans, Christopher G. Fletcher, Martí Galí, Roya Ghahreman, Eric Girard, Wanmin Gong, Michel Gosselin, Margaux Gourdal, Sarah J. Hanna, Hakase Hayashida, Andreas B. Herber, Sareh Hesaraki, Peter Hoor, Lin Huang, Rachel Hussherr, Victoria E. Irish, Setigui A. Keita, John K. Kodros, Franziska Köllner, Felicia Kolonjari, Daniel Kunkel, Luis A. Ladino, Kathy Law, Maurice Levasseur, Quentin Libois, John Liggio, Martine Lizotte, Katrina M. Macdonald, Rashed Mahmood, Randall V. Martin, Ryan H. Mason, Lisa A. Miller, Alexander Moravek, Eric Mortenson, Emma L. Mungall, Jennifer G. Murphy, Maryam Namazi, Ann-Lise Norman, Norman T. O'Neill, Jeffrey R. Pierce, Lynn M. Russell, Johannes Schneider, Hannes Schulz, Sangeeta Sharma, Meng Si, Ralf M. Staebler, Nadja S. Steiner, Jennie L. Thomas, Knut von Salzen, Jeremy J. B. Wentzell, Megan D. Willis, Gregory R. Wentworth, Jun-Wei Xu, and Jacqueline D. Yakobi-Hancock
Atmos. Chem. Phys., 19, 2527–2560, https://doi.org/10.5194/acp-19-2527-2019, https://doi.org/10.5194/acp-19-2527-2019, 2019
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The Arctic is experiencing considerable environmental change with climate warming, illustrated by the dramatic decrease in sea-ice extent. It is important to understand both the natural and perturbed Arctic systems to gain a better understanding of how they will change in the future. This paper summarizes new insights into the relationships between Arctic aerosol particles and climate, as learned over the past five or so years by a large Canadian research consortium, NETCARE.
Tobias Zinner, Ulrich Schwarz, Tobias Kölling, Florian Ewald, Evelyn Jäkel, Bernhard Mayer, and Manfred Wendisch
Atmos. Meas. Tech., 12, 1167–1181, https://doi.org/10.5194/amt-12-1167-2019, https://doi.org/10.5194/amt-12-1167-2019, 2019
Florian Ewald, Tobias Zinner, Tobias Kölling, and Bernhard Mayer
Atmos. Meas. Tech., 12, 1183–1206, https://doi.org/10.5194/amt-12-1183-2019, https://doi.org/10.5194/amt-12-1183-2019, 2019
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This paper presents a new method for gaining insights into the vertical evolution of cloud droplet effective radii by using reflected solar radiation from cloud sides. The paper investigates how bi-spectral effective radius retrievals are affected by unknown cloud surface orientations and presents a method to mitigate this effect. Based on these findings, this study develops a statistical effective radius retrieval for airborne, side-looking imaging sensors.
Hannes Schulz, Marco Zanatta, Heiko Bozem, W. Richard Leaitch, Andreas B. Herber, Julia Burkart, Megan D. Willis, Daniel Kunkel, Peter M. Hoor, Jonathan P. D. Abbatt, and Rüdiger Gerdes
Atmos. Chem. Phys., 19, 2361–2384, https://doi.org/10.5194/acp-19-2361-2019, https://doi.org/10.5194/acp-19-2361-2019, 2019
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Aircraft vertical profiles of black carbon (BC) aerosol from the High Canadian Arctic have shown systematic variability in different levels of the cold, stably stratified polar dome. During spring and summer, efficiencies of BC supply by transport (often from gas flaring and wildfire-affected regions) were different in the lower dome than at higher levels, as apparent from changes in mean particle size and mixing ratios with CO. Summer BC concentrations were a factor of 10 lower than in spring.
Tobias Kölling, Tobias Zinner, and Bernhard Mayer
Atmos. Meas. Tech., 12, 1155–1166, https://doi.org/10.5194/amt-12-1155-2019, https://doi.org/10.5194/amt-12-1155-2019, 2019
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Imaging technology allows us to quickly gather information on larger cloud fields. Unlike using lidar or radar, it is difficult to obtain accurate position information about the observed clouds. This work presents a method to retrieve the missing position information using RGB images from an airborne video camera. Using field campaign data, we observe and explain a median offset of 126 m compared to lidar data and show that systematic errors across the measurement swath are well below 50 m.
Alexandra Gossart, Stephen P. Palm, Niels Souverijns, Jan T. M. Lenaerts, Irina V. Gorodetskaya, Stef Lhermitte, and Nicole P. M. van Lipzig
The Cryosphere Discuss., https://doi.org/10.5194/tc-2019-25, https://doi.org/10.5194/tc-2019-25, 2019
Manuscript not accepted for further review
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Blowing snow measurements are scarce, both in time and space over the Antarctic ice sheet. We compare here CALIPSO satellite blowing snow measurements, to ground-base remote sensing ceilometer retrievals at two coastal stations in East Antarctica. Results indicate that 95 % of the blowing snow occurs under cloudy conditions, and are missed by the satellite. In addition, difficulties arise if comparing point locations to satellite overpasses.
Timo Vihma, Petteri Uotila, Stein Sandven, Dmitry Pozdnyakov, Alexander Makshtas, Alexander Pelyasov, Roberta Pirazzini, Finn Danielsen, Sergey Chalov, Hanna K. Lappalainen, Vladimir Ivanov, Ivan Frolov, Anna Albin, Bin Cheng, Sergey Dobrolyubov, Viktor Arkhipkin, Stanislav Myslenkov, Tuukka Petäjä, and Markku Kulmala
Atmos. Chem. Phys., 19, 1941–1970, https://doi.org/10.5194/acp-19-1941-2019, https://doi.org/10.5194/acp-19-1941-2019, 2019
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The Arctic marine climate system, ecosystems, and socio-economic systems are changing rapidly. This calls for the establishment of a marine Arctic component of the Pan-Eurasian Experiment (MA-PEEX), for which we present a plan. The program will promote international collaboration; sustainable marine meteorological, sea ice, and oceanographic observations; advanced data management; and multidisciplinary research on the marine Arctic and its interaction with the Eurasian continent.
Claudio Durán-Alarcón, Brice Boudevillain, Christophe Genthon, Jacopo Grazioli, Niels Souverijns, Nicole P. M. van Lipzig, Irina V. Gorodetskaya, and Alexis Berne
The Cryosphere, 13, 247–264, https://doi.org/10.5194/tc-13-247-2019, https://doi.org/10.5194/tc-13-247-2019, 2019
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Precipitation is the main input in the surface mass balance of the Antarctic ice sheet, but it is still poorly understood due to a lack of observations in this region. We analyzed the vertical structure of the precipitation using multiyear observation of vertically pointing micro rain radars (MRRs) at two stations located in East Antarctica. The use of MRRs showed the potential to study the effect of climatology and hydrometeor microphysics on the vertical structure of Antarctic precipitation.
Pascal Graf, Heini Wernli, Stephan Pfahl, and Harald Sodemann
Atmos. Chem. Phys., 19, 747–765, https://doi.org/10.5194/acp-19-747-2019, https://doi.org/10.5194/acp-19-747-2019, 2019
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This article studies the interaction between falling rain and vapour with stable water isotopes. In particular, rain evaporation is relevant for several atmospheric processes, but remains difficult to quantify. A novel framework is introduced to facilitate the interpretation of stable water isotope observations in near-surface vapour and rain. The usefulness of this concept is demonstrated using observations at high time resolution from a cold front. Sensitivities are tested with a simple model.
Xiang-Yu Li, Gunilla Svensson, Axel Brandenburg, and Nils E. L. Haugen
Atmos. Chem. Phys., 19, 639–648, https://doi.org/10.5194/acp-19-639-2019, https://doi.org/10.5194/acp-19-639-2019, 2019
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The broadening of droplet size distributions in stratiform clouds, where the updraft velocity is almost zero, is puzzling. Without turbulence, the classical treatment of condensational growth of cloud droplets fails to explain this
broadening. We investigated the time evolution of droplet size distributions using direct numerical simulations, where turbulence is resolved into the smallest scales. We found that the broadening is due to the turbulence-facilitated supersaturation fluctuations.
Paul Herenz, Heike Wex, Alexander Mangold, Quentin Laffineur, Irina V. Gorodetskaya, Zoë L. Fleming, Marios Panagi, and Frank Stratmann
Atmos. Chem. Phys., 19, 275–294, https://doi.org/10.5194/acp-19-275-2019, https://doi.org/10.5194/acp-19-275-2019, 2019
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Atmospheric aerosol particles were observed in Antarctica, at the Belgian Princess Elisabeth station during three austral summers. Possible source regions for the particles were examined. Air that spent more than 90 %; of the time during 10 days over Antarctica had low and stable number concentrations, while the highest (new particle formation) and lowest (scavenging and wet deposition) concentrations were observed for air masses that were more strongly influenced by the Southern Ocean.
Megan D. Willis, Heiko Bozem, Daniel Kunkel, Alex K. Y. Lee, Hannes Schulz, Julia Burkart, Amir A. Aliabadi, Andreas B. Herber, W. Richard Leaitch, and Jonathan P. D. Abbatt
Atmos. Chem. Phys., 19, 57–76, https://doi.org/10.5194/acp-19-57-2019, https://doi.org/10.5194/acp-19-57-2019, 2019
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The vertical distribution of Arctic aerosol is an important driver of its climate impacts. We present vertically resolved measurements of aerosol composition and properties made in the High Arctic during spring on an aircraft platform. We explore how aerosol properties are related to transport history and show evidence of vertical trends in aerosol sources, transport mechanisms and composition. These results will help us to better understand aerosol–climate interactions in the Arctic.
Erlend M. Knudsen, Bernd Heinold, Sandro Dahlke, Heiko Bozem, Susanne Crewell, Irina V. Gorodetskaya, Georg Heygster, Daniel Kunkel, Marion Maturilli, Mario Mech, Carolina Viceto, Annette Rinke, Holger Schmithüsen, André Ehrlich, Andreas Macke, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys., 18, 17995–18022, https://doi.org/10.5194/acp-18-17995-2018, https://doi.org/10.5194/acp-18-17995-2018, 2018
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The paper describes the synoptic development during the ACLOUD/PASCAL airborne and ship-based field campaign near Svalbard in spring 2017. This development is presented using near-surface and upperair meteorological observations, satellite, and model data. We first present time series of these data, from which we identify and characterize three key periods. Finally, we put our observations in historical and regional contexts and compare our findings to other Arctic field campaigns.
Jessie M. Creamean, Rachel M. Kirpes, Kerri A. Pratt, Nicholas J. Spada, Maximilian Maahn, Gijs de Boer, Russell C. Schnell, and Swarup China
Atmos. Chem. Phys., 18, 18023–18042, https://doi.org/10.5194/acp-18-18023-2018, https://doi.org/10.5194/acp-18-18023-2018, 2018
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Warm-temperature ice nucleating particles (INPs) were observed during a springtime transition period of the melting of frozen surfaces in Northern Alaska. Such INPs were likely biological and from marine and terrestrial (tundra) sources. Influxes of these efficient INPs may have important implications for Arctic cloud ice formation and, consequently, the surface energy budget.
Michael Weger, Bernd Heinold, Christa Engler, Ulrich Schumann, Axel Seifert, Romy Fößig, Christiane Voigt, Holger Baars, Ulrich Blahak, Stephan Borrmann, Corinna Hoose, Stefan Kaufmann, Martina Krämer, Patric Seifert, Fabian Senf, Johannes Schneider, and Ina Tegen
Atmos. Chem. Phys., 18, 17545–17572, https://doi.org/10.5194/acp-18-17545-2018, https://doi.org/10.5194/acp-18-17545-2018, 2018
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The impact of desert dust on cloud formation is investigated for a major Saharan dust event over Europe by interactive regional dust modeling. Dust particles are very efficient ice-nucleating particles promoting the formation of ice crystals in clouds. The simulations show that the observed extensive cirrus development was likely related to the above-average dust load. The interactive dust–cloud feedback in the model significantly improves the agreement with aircraft and satellite observations.
Gary Lloyd, Thomas W. Choularton, Keith N. Bower, Martin W. Gallagher, Jonathan Crosier, Sebastian O'Shea, Steven J. Abel, Stuart Fox, Richard Cotton, and Ian A. Boutle
Atmos. Chem. Phys., 18, 17191–17206, https://doi.org/10.5194/acp-18-17191-2018, https://doi.org/10.5194/acp-18-17191-2018, 2018
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The work deals with cold weather outbreaks at high latitudes that often bring severe weather such as heavy snow, lightning and high winds but are poorly forecast by weather models. Here we made measurements of these events and the clouds associated with them using a research aircraft. We found that the properties of these clouds were often very different to what the models predicted, and these results can potentially be used to bring significant improvement to the forecasting of these events.
Amy Solomon, Gijs de Boer, Jessie M. Creamean, Allison McComiskey, Matthew D. Shupe, Maximilian Maahn, and Christopher Cox
Atmos. Chem. Phys., 18, 17047–17059, https://doi.org/10.5194/acp-18-17047-2018, https://doi.org/10.5194/acp-18-17047-2018, 2018
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The results of this study indicate that perturbations in ice nucleating particles (INPs) dominate over cloud condensation nuclei (CCN) perturbations in Arctic mixed-phase stratocumulus; i.e., an equivalent fractional decrease in CCN and INPs results in an increase in the cloud-top longwave cooling rate, even though the droplet effective radius increases and the cloud emissivity decreases. In addition, cloud-processing causes layering of aerosols with increased concentrations of CCN at cloud top.
Niels Souverijns, Alexandra Gossart, Stef Lhermitte, Irina V. Gorodetskaya, Jacopo Grazioli, Alexis Berne, Claudio Duran-Alarcon, Brice Boudevillain, Christophe Genthon, Claudio Scarchilli, and Nicole P. M. van Lipzig
The Cryosphere, 12, 3775–3789, https://doi.org/10.5194/tc-12-3775-2018, https://doi.org/10.5194/tc-12-3775-2018, 2018
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Snowfall observations over Antarctica are scarce and currently limited to information from the CloudSat satellite. Here, a first evaluation of the CloudSat snowfall record is performed using observations of ground-based precipitation radars. Results indicate an accurate representation of the snowfall climatology over Antarctica, despite the low overpass frequency of the satellite, outperforming state-of-the-art model estimates. Individual snowfall events are however not well represented.
Stefan Kaufmann, Christiane Voigt, Romy Heller, Tina Jurkat-Witschas, Martina Krämer, Christian Rolf, Martin Zöger, Andreas Giez, Bernhard Buchholz, Volker Ebert, Troy Thornberry, and Ulrich Schumann
Atmos. Chem. Phys., 18, 16729–16745, https://doi.org/10.5194/acp-18-16729-2018, https://doi.org/10.5194/acp-18-16729-2018, 2018
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We present an intercomparison of the airborne water vapor measurements during the ML-CIRRUS mission. Although the agreement of the hygrometers significantly improved compared to studies from recent decades, systematic differences remain under specific meteorological conditions. We compare the measurements to model data, where we observe a model wet bias in the lower stratosphere close to the tropopause, likely caused by a blurred humidity gradient in the model tropopause.
Anna T. Kunert, Mark Lamneck, Frank Helleis, Ulrich Pöschl, Mira L. Pöhlker, and Janine Fröhlich-Nowoisky
Atmos. Meas. Tech., 11, 6327–6337, https://doi.org/10.5194/amt-11-6327-2018, https://doi.org/10.5194/amt-11-6327-2018, 2018
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The new Twin-plate Ice Nucleation Assay with infrared detection for high-throughput droplet freezing experiments in microliter-sized droplets is introduced, which was tested and characterized with bacterial and fungal ice nuclei. It was applied to investigate the influence of chemical processing on the activity of biological ice nuclei, and aqueous extracts of atmospheric aerosols were studied for ice nuclei activity.
Paul J. DeMott, Ottmar Möhler, Daniel J. Cziczo, Naruki Hiranuma, Markus D. Petters, Sarah S. Petters, Franco Belosi, Heinz G. Bingemer, Sarah D. Brooks, Carsten Budke, Monika Burkert-Kohn, Kristen N. Collier, Anja Danielczok, Oliver Eppers, Laura Felgitsch, Sarvesh Garimella, Hinrich Grothe, Paul Herenz, Thomas C. J. Hill, Kristina Höhler, Zamin A. Kanji, Alexei Kiselev, Thomas Koop, Thomas B. Kristensen, Konstantin Krüger, Gourihar Kulkarni, Ezra J. T. Levin, Benjamin J. Murray, Alessia Nicosia, Daniel O'Sullivan, Andreas Peckhaus, Michael J. Polen, Hannah C. Price, Naama Reicher, Daniel A. Rothenberg, Yinon Rudich, Gianni Santachiara, Thea Schiebel, Jann Schrod, Teresa M. Seifried, Frank Stratmann, Ryan C. Sullivan, Kaitlyn J. Suski, Miklós Szakáll, Hans P. Taylor, Romy Ullrich, Jesus Vergara-Temprado, Robert Wagner, Thomas F. Whale, Daniel Weber, André Welti, Theodore W. Wilson, Martin J. Wolf, and Jake Zenker
Atmos. Meas. Tech., 11, 6231–6257, https://doi.org/10.5194/amt-11-6231-2018, https://doi.org/10.5194/amt-11-6231-2018, 2018
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The ability to measure ice nucleating particles is vital to quantifying their role in affecting clouds and precipitation. Methods for measuring droplet freezing were compared while co-sampling relevant particle types. Measurement correspondence was very good for ice nucleating particles of bacterial and natural soil origin, and somewhat more disparate for those of mineral origin. Results reflect recently improved capabilities and provide direction toward addressing remaining measurement issues.
Emma Järvinen, Olivier Jourdan, David Neubauer, Bin Yao, Chao Liu, Meinrat O. Andreae, Ulrike Lohmann, Manfred Wendisch, Greg M. McFarquhar, Thomas Leisner, and Martin Schnaiter
Atmos. Chem. Phys., 18, 15767–15781, https://doi.org/10.5194/acp-18-15767-2018, https://doi.org/10.5194/acp-18-15767-2018, 2018
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Using light diffraction it is possible to detect microscopic features within ice particles that have not yet been fully characterized. Here, this technique was applied in airborne measurements, where it was found that majority of atmospheric ice particles have features that significantly change the way ice particles interact with solar light. The microscopic features make ice-containing clouds more reflective than previously thought, which could have consequences for predicting our climate.
Akio Hansen, Felix Ament, Verena Grützun, and Andrea Lammert
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2018-259, https://doi.org/10.5194/gmd-2018-259, 2018
Publication in GMD not foreseen
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Clouds are responsible for large uncertainties in atmospheric models, whereby the evaluation is very challenging due to their complexity. The Cloudnet project uses multi-sensor observations to create a comprehensive Target Classification showing the cloud structure and phase, but there is no comparable model output available. The presented cloud classification algorithm generates a consistent product, which provides a comprehensive view on clouds and is used for further in-depth evaluation.
Christiane Voigt, Andreas Dörnbrack, Martin Wirth, Silke M. Groß, Michael C. Pitts, Lamont R. Poole, Robert Baumann, Benedikt Ehard, Björn-Martin Sinnhuber, Wolfgang Woiwode, and Hermann Oelhaf
Atmos. Chem. Phys., 18, 15623–15641, https://doi.org/10.5194/acp-18-15623-2018, https://doi.org/10.5194/acp-18-15623-2018, 2018
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The 2015–2016 stratospheric winter was the coldest in the 36-year climatological data record. The extreme conditions promoted the formation of persistent Arctic polar stratospheric ice clouds. An extended ice PSC detected by airborne lidar in January 2016 shows a second mode with higher particle depolarization ratios. Back-trajectories from the high-depol ice matched to CALIOP PSC curtains provide evidence for ice nucleation on NAT. The novel data consolidate our understanding of PSC formation.
Yoann Tellier, Clémence Pierangelo, Martin Wirth, Fabien Gibert, and Fabien Marnas
Atmos. Meas. Tech., 11, 5865–5884, https://doi.org/10.5194/amt-11-5865-2018, https://doi.org/10.5194/amt-11-5865-2018, 2018
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The French and German space agencies (CNES, DLR) are currently developing MERLIN, a satellite that will measure atmospheric concentration of methane, a powerful greenhouse gas. To reach the desired precision, horizontally averaging the measurements along the satellite track is performed but leads to a processing bias due to non-linear equations. This article studies the processing biases for several averaging schemes and bias correction algorithms and recommends a best approach to limit biases.
Hamish Gordon, Paul R. Field, Steven J. Abel, Mohit Dalvi, Daniel P. Grosvenor, Adrian A. Hill, Ben T. Johnson, Annette K. Miltenberger, Masaru Yoshioka, and Ken S. Carslaw
Atmos. Chem. Phys., 18, 15261–15289, https://doi.org/10.5194/acp-18-15261-2018, https://doi.org/10.5194/acp-18-15261-2018, 2018
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Smoke from African fires is frequently transported across the Atlantic Ocean, where it interacts with clouds. We simulate the interaction of the smoke with the clouds, and the consequences of this for the solar radiation the clouds reflect. The simulations use a new regional configuration of the UK Met Office climate model. Our simulations indicate that the properties of the clouds, in particular their height and reflectivity, and the fractional cloud cover, are strongly affected by the smoke.
Christiane Schulz, Johannes Schneider, Bruna Amorim Holanda, Oliver Appel, Anja Costa, Suzane S. de Sá, Volker Dreiling, Daniel Fütterer, Tina Jurkat-Witschas, Thomas Klimach, Christoph Knote, Martina Krämer, Scot T. Martin, Stephan Mertes, Mira L. Pöhlker, Daniel Sauer, Christiane Voigt, Adrian Walser, Bernadett Weinzierl, Helmut Ziereis, Martin Zöger, Meinrat O. Andreae, Paulo Artaxo, Luiz A. T. Machado, Ulrich Pöschl, Manfred Wendisch, and Stephan Borrmann
Atmos. Chem. Phys., 18, 14979–15001, https://doi.org/10.5194/acp-18-14979-2018, https://doi.org/10.5194/acp-18-14979-2018, 2018
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Aerosol chemical composition measurements in the tropical upper troposphere over the Amazon region show that 78 % of the aerosol in the upper troposphere consists of organic matter. Up to 20 % of the organic aerosol can be attributed to isoprene epoxydiol secondary organic aerosol (IEPOX-SOA). Furthermore, organic nitrates were identified, suggesting a connection to the IEPOX-SOA formation.
Kerstin Hartung, Gunilla Svensson, Hamish Struthers, Anna-Lena Deppenmeier, and Wilco Hazeleger
Geosci. Model Dev., 11, 4117–4137, https://doi.org/10.5194/gmd-11-4117-2018, https://doi.org/10.5194/gmd-11-4117-2018, 2018
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Single-column models have been used to develop weather and climate models for several decades. They decouple small-scale processes from large-scale forcing and allow us to test models in a controlled environment with reduced computational cost. Here, we present a fully coupled atmosphere–ocean single-column model, including sea ice. We demonstrate that it is a valuable tool to advance our understanding in marine and polar boundary layer processes and interactions of their coupled components.
Uwe Mikolajewicz, Florian Ziemen, Guido Cioni, Martin Claussen, Klaus Fraedrich, Marvin Heidkamp, Cathy Hohenegger, Diego Jimenez de la Cuesta, Marie-Luise Kapsch, Alexander Lemburg, Thorsten Mauritsen, Katharina Meraner, Niklas Röber, Hauke Schmidt, Katharina D. Six, Irene Stemmler, Talia Tamarin-Brodsky, Alexander Winkler, Xiuhua Zhu, and Bjorn Stevens
Earth Syst. Dynam., 9, 1191–1215, https://doi.org/10.5194/esd-9-1191-2018, https://doi.org/10.5194/esd-9-1191-2018, 2018
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Model experiments show that changing the sense of Earth's rotation has relatively little impact on the globally and zonally averaged energy budgets but leads to large shifts in continental climates and patterns of precipitation. The retrograde world is greener as the desert area shrinks. Deep water formation shifts from the North Atlantic to the North Pacific with subsequent changes in ocean overturning. Over large areas of the Indian Ocean, cyanobacteria dominate over bulk phytoplankton.
Odran Sourdeval, Edward Gryspeerdt, Martina Krämer, Tom Goren, Julien Delanoë, Armin Afchine, Friederike Hemmer, and Johannes Quaas
Atmos. Chem. Phys., 18, 14327–14350, https://doi.org/10.5194/acp-18-14327-2018, https://doi.org/10.5194/acp-18-14327-2018, 2018
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The number concentration of ice crystals (Ni) is a key cloud property that remains very uncertain due to difficulties in determining it using satellites. This lack of global observational constraints limits our ability to constrain this property in models responsible for predicting future climate. This pair of papers fills this gap by showing and analyzing the first rigorously evaluated global climatology of Ni, leading to new information shedding light on the processes that control high clouds.
Edward Gryspeerdt, Odran Sourdeval, Johannes Quaas, Julien Delanoë, Martina Krämer, and Philipp Kühne
Atmos. Chem. Phys., 18, 14351–14370, https://doi.org/10.5194/acp-18-14351-2018, https://doi.org/10.5194/acp-18-14351-2018, 2018
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The concentration of ice crystals in a cloud affects both the properties and the life cycle of the cloud. This work uses a new satellite retrieval to investigate controls on the ice crystal concentration at a global scale. Both temperature and vertical wind speed in a cloud have a strong impact on the concentration of ice crystals. The ice crystal number is also related to the aerosol environment; defining this relation opens up new ways to investigate human impacts on clouds and the climate.
Stine Eriksen Hammer, Stephan Mertes, Johannes Schneider, Martin Ebert, Konrad Kandler, and Stephan Weinbruch
Atmos. Chem. Phys., 18, 13987–14003, https://doi.org/10.5194/acp-18-13987-2018, https://doi.org/10.5194/acp-18-13987-2018, 2018
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It is important to study ice-nucleating particles in the environment to learn more about cloud formation. We studied the composition of ice particle residuals and total aerosol particles sampled in parallel during mixed-phase cloud events at Jungfraujoch and discovered that soot and complex secondary particles were not present. In contrast, silica, aluminosilicates, and other aluminosilicates were the most important ice particle residual groups at site temperatures between −11 and −18 °C.
Sarah Grawe, Stefanie Augustin-Bauditz, Hans-Christian Clemen, Martin Ebert, Stine Eriksen Hammer, Jasmin Lubitz, Naama Reicher, Yinon Rudich, Johannes Schneider, Robert Staacke, Frank Stratmann, André Welti, and Heike Wex
Atmos. Chem. Phys., 18, 13903–13923, https://doi.org/10.5194/acp-18-13903-2018, https://doi.org/10.5194/acp-18-13903-2018, 2018
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In this study, coal fly ash particles immersed in supercooled cloud droplets were analyzed concerning their freezing behavior. Additionally, physico-chemical particle properties (morphology, chemical composition, crystallography) were investigated. In combining both aspects, components that potentially contribute to the observed freezing behavior of the ash could be identified. Interactions at the particle-water interface, that depend on suspension time and influence freezing, are discussed.
Jens Voigtländer, Cedric Chou, Henner Bieligk, Tina Clauss, Susan Hartmann, Paul Herenz, Dennis Niedermeier, Georg Ritter, Frank Stratmann, and Zbigniew Ulanowski
Atmos. Chem. Phys., 18, 13687–13702, https://doi.org/10.5194/acp-18-13687-2018, https://doi.org/10.5194/acp-18-13687-2018, 2018
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Surface roughness of ice crystals has recently been acknowledged to strongly influence the radiative properties of cold clouds such as cirrus, but it is unclear how this roughness arises. The study investigates the origins of ice surface roughness under a variety of atmospherically relevant conditions, using a novel method to measure roughness quantitatively. It is found that faster growth leads to stronger roughness. Roughness also increases following repeated growth–sublimation cycles.
Elena Shevnina, Karoliina Pilli-Sihvola, Riina Haavisto, Timo Vihma, and Andrey Silaev
Hydrol. Earth Syst. Sci. Discuss., https://doi.org/10.5194/hess-2018-473, https://doi.org/10.5194/hess-2018-473, 2018
Manuscript not accepted for further review
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Projections of a potential hydropower production were evaluated in terms of probability of water resources available in the future. The future projections of annual river runoff were evaluated on average, as well as on low and high exceedance probabilities under several climate change scenarios. The main idea of the modelling method used is to simulate statistical estimators of annual river runoff (mean, variation and skewness) instead of runoff time series.
Michael Schäfer, Katharina Loewe, André Ehrlich, Corinna Hoose, and Manfred Wendisch
Atmos. Chem. Phys., 18, 13115–13133, https://doi.org/10.5194/acp-18-13115-2018, https://doi.org/10.5194/acp-18-13115-2018, 2018
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Airborne observed horizontal fields of cloud optical thickness are compared with semi-idealized large eddy simulations of Arctic stratus. The comparison focuses on horizontal cloud inhomogeneities and directional features of the small-scale cloud structures. Using inhomogeneity parameters and autocorrelation analysis it is investigated, if the observed small-scale cloud inhomogeneities can be represented by the model. Forcings for cloud inhomogeneities are investigated in a sensitivity study.
Jorge Saturno, Bruna A. Holanda, Christopher Pöhlker, Florian Ditas, Qiaoqiao Wang, Daniel Moran-Zuloaga, Joel Brito, Samara Carbone, Yafang Cheng, Xuguang Chi, Jeannine Ditas, Thorsten Hoffmann, Isabella Hrabe de Angelis, Tobias Könemann, Jošt V. Lavrič, Nan Ma, Jing Ming, Hauke Paulsen, Mira L. Pöhlker, Luciana V. Rizzo, Patrick Schlag, Hang Su, David Walter, Stefan Wolff, Yuxuan Zhang, Paulo Artaxo, Ulrich Pöschl, and Meinrat O. Andreae
Atmos. Chem. Phys., 18, 12817–12843, https://doi.org/10.5194/acp-18-12817-2018, https://doi.org/10.5194/acp-18-12817-2018, 2018
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Biomass burning emits light-absorbing aerosol particles that warm the atmosphere. One of them is the primarily emitted black carbon, which strongly absorbs radiation in the visible and UV spectral regions. Another one is the so-called brown carbon, a fraction of organic aerosol particles that are able to absorb radiation, especially in the UV spectral region. The contribution of both kinds of aerosol particles to light absorption over the Amazon rainforest is studied in this paper.
Christopher R. Williams, Maximilian Maahn, Joseph C. Hardin, and Gijs de Boer
Atmos. Meas. Tech., 11, 4963–4980, https://doi.org/10.5194/amt-11-4963-2018, https://doi.org/10.5194/amt-11-4963-2018, 2018
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This study presents three signal-processing methods to improve estimates derived from a vertically pointing 35 GHz cloud radar deployed at Oliktok Point, Alaska. The first method removes ground clutter from the Doppler velocity spectra. The second method estimates multiple peaks and high-order moments from the improved spectra. The third method removes high-frequency variability in high-order moments by shifting original 2 s spectra to a common reference before averaging over a 15 s interval.
Marvin Heidkamp, Andreas Chlond, and Felix Ament
Geosci. Model Dev., 11, 3465–3479, https://doi.org/10.5194/gmd-11-3465-2018, https://doi.org/10.5194/gmd-11-3465-2018, 2018
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The core of every climate model is the solution of the surface energy balance. Numerical approaches are mandatory to calculate the land's response to solar input. However, different numerical approaches should not affect the physical results. Here we develop a physical approach that determines how the available energy is divided into radiative and heat fluxes. A key element of this scheme is the inclusion of different types of heat storages in the canopy layer.
Suzane S. de Sá, Brett B. Palm, Pedro Campuzano-Jost, Douglas A. Day, Weiwei Hu, Gabriel Isaacman-VanWertz, Lindsay D. Yee, Joel Brito, Samara Carbone, Igor O. Ribeiro, Glauber G. Cirino, Yingjun Liu, Ryan Thalman, Arthur Sedlacek, Aaron Funk, Courtney Schumacher, John E. Shilling, Johannes Schneider, Paulo Artaxo, Allen H. Goldstein, Rodrigo A. F. Souza, Jian Wang, Karena A. McKinney, Henrique Barbosa, M. Lizabeth Alexander, Jose L. Jimenez, and Scot T. Martin
Atmos. Chem. Phys., 18, 12185–12206, https://doi.org/10.5194/acp-18-12185-2018, https://doi.org/10.5194/acp-18-12185-2018, 2018
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This study aimed at understanding and quantifying the changes in mass concentration and composition of submicron airborne particulate matter (PM) in Amazonia due to urban pollution. Downwind of Manaus, PM concentrations increased by up to 200 % under polluted compared with background conditions. The observed changes included contributions from both primary and secondary processes. The differences in organic PM composition suggested a shift in the pathways of secondary production with pollution.
Amelie Driemel, John Augustine, Klaus Behrens, Sergio Colle, Christopher Cox, Emilio Cuevas-Agulló, Fred M. Denn, Thierry Duprat, Masato Fukuda, Hannes Grobe, Martial Haeffelin, Gary Hodges, Nicole Hyett, Osamu Ijima, Ain Kallis, Wouter Knap, Vasilii Kustov, Charles N. Long, David Longenecker, Angelo Lupi, Marion Maturilli, Mohamed Mimouni, Lucky Ntsangwane, Hiroyuki Ogihara, Xabier Olano, Marc Olefs, Masao Omori, Lance Passamani, Enio Bueno Pereira, Holger Schmithüsen, Stefanie Schumacher, Rainer Sieger, Jonathan Tamlyn, Roland Vogt, Laurent Vuilleumier, Xiangao Xia, Atsumu Ohmura, and Gert König-Langlo
Earth Syst. Sci. Data, 10, 1491–1501, https://doi.org/10.5194/essd-10-1491-2018, https://doi.org/10.5194/essd-10-1491-2018, 2018
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The Baseline Surface Radiation Network (BSRN) collects and centrally archives high-quality ground-based radiation measurements in 1 min resolution. More than 10 300 months, i.e., > 850 years, of high-radiation data in 1 min resolution from the years 1992 to 2017 are available. The network currently comprises 59 stations collectively representing all seven continents as well as island-based stations in the Pacific, Atlantic, Indian and Arctic oceans.
Marion Maturilli and Kerstin Ebell
Earth Syst. Sci. Data, 10, 1451–1456, https://doi.org/10.5194/essd-10-1451-2018, https://doi.org/10.5194/essd-10-1451-2018, 2018
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We present a 25-year data record of cloud base height measured by ceilometer at the Ny-Ålesund, Svalbard, Arctic site. The long-term time series allows derivation of an annual cycle of the cloud occurrence frequency, revealing more frequent cloud cover in summer and the lowest cloud cover amount in April. The cloud base data further provide essential information for the interpretation of the surface radiation balance and contribute to understanding meteorological processes at high latitudes.
John K. Kodros, Sarah J. Hanna, Allan K. Bertram, W. Richard Leaitch, Hannes Schulz, Andreas B. Herber, Marco Zanatta, Julia Burkart, Megan D. Willis, Jonathan P. D. Abbatt, and Jeffrey R. Pierce
Atmos. Chem. Phys., 18, 11345–11361, https://doi.org/10.5194/acp-18-11345-2018, https://doi.org/10.5194/acp-18-11345-2018, 2018
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The mixing state of black carbon is one of the key uncertainties limiting the ability of models to estimate the direct radiative effect. In this work, we present aircraft measurements from the Canadian Arctic of coating thickness as a function of black carbon core diameter and black-carbon-containing particle number fractions. We use these measurements to inform estimates of the direct radiative effect in Arctic aerosol simulations.
Sören Johansson, Wolfgang Woiwode, Michael Höpfner, Felix Friedl-Vallon, Anne Kleinert, Erik Kretschmer, Thomas Latzko, Johannes Orphal, Peter Preusse, Jörn Ungermann, Michelle L. Santee, Tina Jurkat-Witschas, Andreas Marsing, Christiane Voigt, Andreas Giez, Martina Krämer, Christian Rolf, Andreas Zahn, Andreas Engel, Björn-Martin Sinnhuber, and Hermann Oelhaf
Atmos. Meas. Tech., 11, 4737–4756, https://doi.org/10.5194/amt-11-4737-2018, https://doi.org/10.5194/amt-11-4737-2018, 2018
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We present two-dimensional cross sections of temperature, HNO3, O3, ClONO2, H2O and CFC-12 from measurements of the GLORIA infrared limb imager during the POLSTRACC/GW-LCYCLE/SALSA aircraft campaigns in the Arctic winter 2015/2016. GLORIA sounded the atmosphere between 5 and 14 km with vertical resolutions of 0.4–1 km. Estimated errors are in the range of 1–2 K (temperature) and 10 %–20 % (trace gases). Comparisons to in situ instruments onboard the aircraft and to Aura/MLS are shown.
Jörg Hartmann, Martin Gehrmann, Katrin Kohnert, Stefan Metzger, and Torsten Sachs
Atmos. Meas. Tech., 11, 4567–4581, https://doi.org/10.5194/amt-11-4567-2018, https://doi.org/10.5194/amt-11-4567-2018, 2018
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We present new in-flight calibration procedures for airborne turbulence measurements that exploit suitable regular flight legs without the need for dedicated calibration patterns. Furthermore we estimate the accuracy of the airborne wind measurement and of the turbulent fluxes of the traces gases methane and carbon dioxide.
Brian H. Kahn, Hanii Takahashi, Graeme L. Stephens, Qing Yue, Julien Delanoë, Gerald Manipon, Evan M. Manning, and Andrew J. Heymsfield
Atmos. Chem. Phys., 18, 10715–10739, https://doi.org/10.5194/acp-18-10715-2018, https://doi.org/10.5194/acp-18-10715-2018, 2018
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The Atmospheric Infrared Sounder (AIRS) satellite instrument shows statistically significant global trends in ice cloud properties between September 2002 and August 2016. The trends are not explained by known AIRS instrument limitations. Significant differences in the ice cloud particle size is found between convective clouds and thin ice clouds in the tropics. These results will be a useful benchmark for other studies of global ice cloud properties.
Jorge Saturno, Florian Ditas, Marloes Penning de Vries, Bruna A. Holanda, Mira L. Pöhlker, Samara Carbone, David Walter, Nicole Bobrowski, Joel Brito, Xuguang Chi, Alexandra Gutmann, Isabella Hrabe de Angelis, Luiz A. T. Machado, Daniel Moran-Zuloaga, Julian Rüdiger, Johannes Schneider, Christiane Schulz, Qiaoqiao Wang, Manfred Wendisch, Paulo Artaxo, Thomas Wagner, Ulrich Pöschl, Meinrat O. Andreae, and Christopher Pöhlker
Atmos. Chem. Phys., 18, 10391–10405, https://doi.org/10.5194/acp-18-10391-2018, https://doi.org/10.5194/acp-18-10391-2018, 2018
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This study uses satellite observations to track volcanic emissions in eastern Congo and their subsequent transport across the Atlantic Ocean into the Amazon Basin. Aircraft and ground-based observations are used to characterize the influence of volcanogenic aerosol on the chemical and microphysical properties of Amazonian aerosols. Further, this work is an illustrative example of the conditions and dynamics driving the transatlantic transport of African emissions to South America.
Mira L. Pöhlker, Florian Ditas, Jorge Saturno, Thomas Klimach, Isabella Hrabě de Angelis, Alessandro C. Araùjo, Joel Brito, Samara Carbone, Yafang Cheng, Xuguang Chi, Reiner Ditz, Sachin S. Gunthe, Bruna A. Holanda, Konrad Kandler, Jürgen Kesselmeier, Tobias Könemann, Ovid O. Krüger, Jošt V. Lavrič, Scot T. Martin, Eugene Mikhailov, Daniel Moran-Zuloaga, Luciana V. Rizzo, Diana Rose, Hang Su, Ryan Thalman, David Walter, Jian Wang, Stefan Wolff, Henrique M. J. Barbosa, Paulo Artaxo, Meinrat O. Andreae, Ulrich Pöschl, and Christopher Pöhlker
Atmos. Chem. Phys., 18, 10289–10331, https://doi.org/10.5194/acp-18-10289-2018, https://doi.org/10.5194/acp-18-10289-2018, 2018
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This paper presents the aerosol and cloud condensation nuclei (CCN) variability for characteristic atmospheric states – such as biomass burning, long-range transport, and pristine rain forest conditions – in the vulnerable and climate-relevant Amazon Basin. It summarizes the key properties of aerosol and CCN and, thus, provides a basis for an in-depth analysis of aerosol–cloud interactions in the Amazon region.
Daniel Moran-Zuloaga, Florian Ditas, David Walter, Jorge Saturno, Joel Brito, Samara Carbone, Xuguang Chi, Isabella Hrabě de Angelis, Holger Baars, Ricardo H. M. Godoi, Birgit Heese, Bruna A. Holanda, Jošt V. Lavrič, Scot T. Martin, Jing Ming, Mira L. Pöhlker, Nina Ruckteschler, Hang Su, Yaqiang Wang, Qiaoqiao Wang, Zhibin Wang, Bettina Weber, Stefan Wolff, Paulo Artaxo, Ulrich Pöschl, Meinrat O. Andreae, and Christopher Pöhlker
Atmos. Chem. Phys., 18, 10055–10088, https://doi.org/10.5194/acp-18-10055-2018, https://doi.org/10.5194/acp-18-10055-2018, 2018
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This study presents multiple years of aerosol coarse mode observations at the remote ATTO site in the Amazon Basin. The results are discussed in light of the frequent and episodic long-range transport of Saharan dust plumes in the early wet season as well as the persistent background bioaerosol cycling in the rain forest ecosystem. This work provides a solid basis for future studies on the dynamic coarse mode aerosol cycling and its biogeochemical relevance in the Amazon.
Andrei Serafimovich, Stefan Metzger, Jörg Hartmann, Katrin Kohnert, Donatella Zona, and Torsten Sachs
Atmos. Chem. Phys., 18, 10007–10023, https://doi.org/10.5194/acp-18-10007-2018, https://doi.org/10.5194/acp-18-10007-2018, 2018
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In order to support the evaluation of coupled atmospheric–land-surface models we investigated spatial patterns of energy fluxes in relation to land-surface properties and upscaled airborne flux measurements to high resolution flux maps. A machine learning technique allows us to estimate environmental response functions between spatially and temporally resolved flux observations and corresponding biophysical and meteorological drivers.
Aurélien Chauvigné, Olivier Jourdan, Alfons Schwarzenboeck, Christophe Gourbeyre, Jean François Gayet, Christiane Voigt, Hans Schlager, Stefan Kaufmann, Stephan Borrmann, Sergej Molleker, Andreas Minikin, Tina Jurkat, and Ulrich Schumann
Atmos. Chem. Phys., 18, 9803–9822, https://doi.org/10.5194/acp-18-9803-2018, https://doi.org/10.5194/acp-18-9803-2018, 2018
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This paper demonstrates a new form of statistical analysis of contrail to cirrus evolution. The authors show well-separated analyses of the different stages of the contrail's evolution, which allows us to study their optical, microphysical, and chemical properties. These results could be used to develop representative parameterizations of the scattering and geometrical properties of the ice crystals’ shapes and sizes, observed in the visible wavelength range.
Armin Afchine, Christian Rolf, Anja Costa, Nicole Spelten, Martin Riese, Bernhard Buchholz, Volker Ebert, Romy Heller, Stefan Kaufmann, Andreas Minikin, Christiane Voigt, Martin Zöger, Jessica Smith, Paul Lawson, Alexey Lykov, Sergey Khaykin, and Martina Krämer
Atmos. Meas. Tech., 11, 4015–4031, https://doi.org/10.5194/amt-11-4015-2018, https://doi.org/10.5194/amt-11-4015-2018, 2018
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The ice water content (IWC) of cirrus clouds is an essential parameter that determines their radiative properties and is thus important for climate simulations. Experimental investigations of IWCs measured on board research aircraft reveal that their accuracy is influenced by the sampling position. IWCs detected at the aircraft roof deviate significantly from wing, side or bottom IWCs. The reasons are deflections of the gas streamlines and ice particle trajectories behind the aircraft cockpit.
Christine A. Shields, Jonathan J. Rutz, Lai-Yung Leung, F. Martin Ralph, Michael Wehner, Brian Kawzenuk, Juan M. Lora, Elizabeth McClenny, Tashiana Osborne, Ashley E. Payne, Paul Ullrich, Alexander Gershunov, Naomi Goldenson, Bin Guan, Yun Qian, Alexandre M. Ramos, Chandan Sarangi, Scott Sellars, Irina Gorodetskaya, Karthik Kashinath, Vitaliy Kurlin, Kelly Mahoney, Grzegorz Muszynski, Roger Pierce, Aneesh C. Subramanian, Ricardo Tome, Duane Waliser, Daniel Walton, Gary Wick, Anna Wilson, David Lavers, Prabhat, Allison Collow, Harinarayan Krishnan, Gudrun Magnusdottir, and Phu Nguyen
Geosci. Model Dev., 11, 2455–2474, https://doi.org/10.5194/gmd-11-2455-2018, https://doi.org/10.5194/gmd-11-2455-2018, 2018
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ARTMIP (Atmospheric River Tracking Method Intercomparison Project) is a community effort with the explicit goal of understanding the uncertainties, and the implications of those uncertainties, in atmospheric river science solely due to detection algorithm. ARTMIP strives to quantify these differences and provide guidance on appropriate algorithmic choices for the science question posed. Project goals, experimental design, and preliminary results are provided.
Ralf Becker, Marion Maturilli, Rolf Philipona, and Klaus Behrens
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2018-173, https://doi.org/10.5194/amt-2018-173, 2018
Revised manuscript not accepted
Barbara Altstädter, Andreas Platis, Michael Jähn, Holger Baars, Janine Lückerath, Andreas Held, Astrid Lampert, Jens Bange, Markus Hermann, and Birgit Wehner
Atmos. Chem. Phys., 18, 8249–8264, https://doi.org/10.5194/acp-18-8249-2018, https://doi.org/10.5194/acp-18-8249-2018, 2018
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This article describes the appearance of ultrafine aerosol particles (size < 12 nm) within the atmospheric boundary layer under cloudy conditions. New particle formation (NPF) was observed with the ALADINA unmanned aerial system in relation to increased turbulence near the inversion layer. Fast mixing processes and rapid dilution of surrounding air led to an insufficient particle growth rate, seen in sporadic clusters at ground. These events might not have been classified as NPF by surface data.
Niels Souverijns, Alexandra Gossart, Irina V. Gorodetskaya, Stef Lhermitte, Alexander Mangold, Quentin Laffineur, Andy Delcloo, and Nicole P. M. van Lipzig
The Cryosphere, 12, 1987–2003, https://doi.org/10.5194/tc-12-1987-2018, https://doi.org/10.5194/tc-12-1987-2018, 2018
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This work is the first to gain insight into the local surface mass balance over Antarctica using accurate long-term snowfall observations. A non-linear relationship between accumulation and snowfall is discovered, indicating that total surface mass balance measurements are not a good proxy for snowfall over Antarctica. Furthermore, the meteorological drivers causing changes in the local SMB are identified.
Aleksey Malinka, Eleonora Zege, Larysa Istomina, Georg Heygster, Gunnar Spreen, Donald Perovich, and Chris Polashenski
The Cryosphere, 12, 1921–1937, https://doi.org/10.5194/tc-12-1921-2018, https://doi.org/10.5194/tc-12-1921-2018, 2018
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Melt ponds occupy a large part of the Arctic sea ice in summer and strongly affect the radiative budget of the atmosphere–ice–ocean system. The melt pond reflectance is modeled in the framework of the radiative transfer theory and validated with field observations. It improves understanding of melting sea ice and enables better parameterization of the surface in Arctic atmospheric remote sensing (clouds, aerosols, trace gases) and re-evaluating Arctic climatic feedbacks at a new accuracy level.
Stephan E. Bansmer, Arne Baumert, Stephan Sattler, Inken Knop, Delphine Leroy, Alfons Schwarzenboeck, Tina Jurkat-Witschas, Christiane Voigt, Hugo Pervier, and Biagio Esposito
Atmos. Meas. Tech., 11, 3221–3249, https://doi.org/10.5194/amt-11-3221-2018, https://doi.org/10.5194/amt-11-3221-2018, 2018
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Snow, frost formation and ice cubes in our drinks are part of our daily life. But what about our technical innovations like aviation, electrical power transmission and wind-energy production, can they cope with icing? Icing Wind Tunnels are an ideal laboratory environment to answer that question. In this paper, we show how the icing wind tunnel in Braunschweig (Germany) was built and how we can use it for engineering and climate research.
Marta Tecla Falconi, Annakaisa von Lerber, Davide Ori, Frank Silvio Marzano, and Dmitri Moisseev
Atmos. Meas. Tech., 11, 3059–3079, https://doi.org/10.5194/amt-11-3059-2018, https://doi.org/10.5194/amt-11-3059-2018, 2018
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Estimating snowfall intensity from satellite and ground-based radar missions requires accurate retrieval models. Reflectivity–snowfall relations are obtained at cm and mm wavelengths using data recorded during the Biogenic Aerosols Effects on Clouds and Climate (BAECC) campaign in Finland. Lightly, moderately and heavily rimed snow cases are identified. Numerical simulations are performed to relate snowflake microphysical (video disdrometer) and multifrequency backscattering properties (radars).
Olga Henneberg, Felix Ament, and Verena Grützun
Atmos. Chem. Phys., 18, 6413–6425, https://doi.org/10.5194/acp-18-6413-2018, https://doi.org/10.5194/acp-18-6413-2018, 2018
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Soil moisture influences the occurrence of convective precipitation. An accurate knowledge of soil moisture might improve the prediction of convective cells.
But the model uncertainty overshadows the impact of soil moisture in convection resolving models. Only drastic soil moisture changes can exhibit the model uncertainties. Both the enhanced and reduced soil moisture result in a reduced precipitation rate. We point out the need for uncertainty estimations in soil moisture studies.
Luiz A. T. Machado, Alan J. P. Calheiros, Thiago Biscaro, Scott Giangrande, Maria A. F. Silva Dias, Micael A. Cecchini, Rachel Albrecht, Meinrat O. Andreae, Wagner F. Araujo, Paulo Artaxo, Stephan Borrmann, Ramon Braga, Casey Burleyson, Cristiano W. Eichholz, Jiwen Fan, Zhe Feng, Gilberto F. Fisch, Michael P. Jensen, Scot T. Martin, Ulrich Pöschl, Christopher Pöhlker, Mira L. Pöhlker, Jean-François Ribaud, Daniel Rosenfeld, Jaci M. B. Saraiva, Courtney Schumacher, Ryan Thalman, David Walter, and Manfred Wendisch
Atmos. Chem. Phys., 18, 6461–6482, https://doi.org/10.5194/acp-18-6461-2018, https://doi.org/10.5194/acp-18-6461-2018, 2018
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This overview discuss the main precipitation processes and their sensitivities to environmental conditions in the Central Amazon Basin. It presents a review of the knowledge acquired about cloud processes and rainfall formation in Amazonas. In addition, this study provides a characterization of the seasonal variation and rainfall sensitivities to topography, surface cover, and aerosol concentration. Airplane measurements were evaluated to characterize and contrast cloud microphysical properties.
Astrid Lampert, Jörg Hartmann, Falk Pätzold, Lennart Lobitz, Peter Hecker, Katrin Kohnert, Eric Larmanou, Andrei Serafimovich, and Torsten Sachs
Atmos. Meas. Tech., 11, 2523–2536, https://doi.org/10.5194/amt-11-2523-2018, https://doi.org/10.5194/amt-11-2523-2018, 2018
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We compared two different fast-response humidity sensors simultaneously on different airborne platforms. One is a particular, well-establed Lyman-alpha hygrometer that has been used for decades as the standard for fast airborne humidity measurements. However, it is not available any more. The other one is a hygrometer based on the absorption of infrared radiation, from LI-COR. For an environment of low vibrations, the LI-COR sensor is suitable for fast airborne water vapour measurements.
Klaus-Dirk Gottschaldt, Hans Schlager, Robert Baumann, Duy Sinh Cai, Veronika Eyring, Phoebe Graf, Volker Grewe, Patrick Jöckel, Tina Jurkat-Witschas, Christiane Voigt, Andreas Zahn, and Helmut Ziereis
Atmos. Chem. Phys., 18, 5655–5675, https://doi.org/10.5194/acp-18-5655-2018, https://doi.org/10.5194/acp-18-5655-2018, 2018
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This study places aircraft trace gas measurements from within the Asian summer monsoon anticyclone into the context of regional, intra- and interannual variability. We find that the processes reflected in the measurements are present throughout multiple simulated monsoon seasons. Dynamical instabilities, photochemical ozone production, lightning and entrainments from the lower troposphere and from the tropopause region determine the distinct composition of the anticyclone and its outflow.
André Welti, Konrad Müller, Zoë L. Fleming, and Frank Stratmann
Atmos. Chem. Phys., 18, 5307–5320, https://doi.org/10.5194/acp-18-5307-2018, https://doi.org/10.5194/acp-18-5307-2018, 2018
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We report on ambient concentrations of ice nuclei, measured on the Cabo Verde islands. Concentrations are found to exponentially increase by 7 orders of magnitude from −5 to −38 °C. At each temperature, the frequency distribution of observed concentrations can be described by a lognormal distribution, typical for random dilution of substances during transport. Random dilution is found to account for larger fluctuations in IN concentration than seasonal changes and changes in air mass origin.
Andrew E. Dessler, Thorsten Mauritsen, and Bjorn Stevens
Atmos. Chem. Phys., 18, 5147–5155, https://doi.org/10.5194/acp-18-5147-2018, https://doi.org/10.5194/acp-18-5147-2018, 2018
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One of the most important parameters in climate science is the equilibrium climate sensitivity (ECS). Estimates of this quantity based on 20th-century observations suggest low values of ECS (below 2 °C). We show that these calculations may be significantly in error. Together with other recent work on this problem, it seems probable that the ECS is larger than suggested by the 20th-century observations.
Paul Herenz, Heike Wex, Silvia Henning, Thomas Bjerring Kristensen, Florian Rubach, Anja Roth, Stephan Borrmann, Heiko Bozem, Hannes Schulz, and Frank Stratmann
Atmos. Chem. Phys., 18, 4477–4496, https://doi.org/10.5194/acp-18-4477-2018, https://doi.org/10.5194/acp-18-4477-2018, 2018
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The Arctic climate is changing much faster than other regions on Earth. Hence, it is necessary to investigate the processes that are liable for this phenomena and to document the current situation in the Arctic. Therefore, we measured the number and also the size of aerosol particles. It turned out that we captured the transition from the Arctic spring to the Arctic summer and that the according air masses show differences in particle properties. Also, the particles have a low water receptivity.
Trismono C. Krisna, Manfred Wendisch, André Ehrlich, Evelyn Jäkel, Frank Werner, Ralf Weigel, Stephan Borrmann, Christoph Mahnke, Ulrich Pöschl, Meinrat O. Andreae, Christiane Voigt, and Luiz A. T. Machado
Atmos. Chem. Phys., 18, 4439–4462, https://doi.org/10.5194/acp-18-4439-2018, https://doi.org/10.5194/acp-18-4439-2018, 2018
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The optical thickness and particle effective radius of a cirrus above liquid water clouds and a DCC topped by an anvil cirrus are retrieved based on SMART and MODIS radiance measurements. For the cirrus, retrieved particle effective radius are validated with corresponding in situ data using a vertical weighting method. This approach allows to assess the measurements, retrieval algorithms, and derived cloud products.
Christopher R. Yost, Kristopher M. Bedka, Patrick Minnis, Louis Nguyen, J. Walter Strapp, Rabindra Palikonda, Konstantin Khlopenkov, Douglas Spangenberg, William L. Smith Jr., Alain Protat, and Julien Delanoe
Atmos. Meas. Tech., 11, 1615–1637, https://doi.org/10.5194/amt-11-1615-2018, https://doi.org/10.5194/amt-11-1615-2018, 2018
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Accretion of cloud ice particles upon engine or instrument probe surfaces can cause engine malfunction or even power loss, and therefore it is important for aircraft to avoid flight through clouds that may have produced large quantities of ice particles. This study introduces a method by which potentially hazardous conditions can be detected using satellite imagery. It was found that potentially hazardous conditions were often located near or beneath very cold clouds and thunderstorm updrafts.
Jie Chen, Zhijun Wu, Stefanie Augustin-Bauditz, Sarah Grawe, Markus Hartmann, Xiangyu Pei, Zirui Liu, Dongsheng Ji, and Heike Wex
Atmos. Chem. Phys., 18, 3523–3539, https://doi.org/10.5194/acp-18-3523-2018, https://doi.org/10.5194/acp-18-3523-2018, 2018
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The ice nucleation activity of urban aerosols in the atmosphere of Beijing was detected in this study. Results showed that ice-nucleating particle (INP) concentrations were not influenced by the highly variable numbers of atmospheric particles, both in mass and particle number concentrations, implying that INP concentrations might not be influenced directly by anthropogenic activities, at least not down to roughly −25 °C and maybe even below.
Katrina M. Macdonald, Sangeeta Sharma, Desiree Toom, Alina Chivulescu, Andrew Platt, Mike Elsasser, Lin Huang, Richard Leaitch, Nathan Chellman, Joseph R. McConnell, Heiko Bozem, Daniel Kunkel, Ying Duan Lei, Cheol-Heon Jeong, Jonathan P. D. Abbatt, and Greg J. Evans
Atmos. Chem. Phys., 18, 3485–3503, https://doi.org/10.5194/acp-18-3485-2018, https://doi.org/10.5194/acp-18-3485-2018, 2018
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The sources of key contaminants in Arctic snow may be an important factor in understanding the rapid climate changes observed in the Arctic. Fresh snow samples collected frequently through the winter season were analyzed for major constituents. Temporally refined source apportionment via positive matrix factorization in conjunction with FLEXPART suggested potential source characteristics and locations. The identity of these sources and their relative contribution to key analytes is discussed.
Allison A. Wing, Kevin A. Reed, Masaki Satoh, Bjorn Stevens, Sandrine Bony, and Tomoki Ohno
Geosci. Model Dev., 11, 793–813, https://doi.org/10.5194/gmd-11-793-2018, https://doi.org/10.5194/gmd-11-793-2018, 2018
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RCEMIP, an intercomparison of multiple types of numerical models, is proposed. In RCEMIP, the climate system is modeled in an idealized manner with no spatial dependence of boundary conditions (i.e., sea surface temperature) or forcing (i.e., incoming sunlight). This set of simulations will be used to investigate how the amount of cloudiness changes with warming, how the clustering of clouds changes with warming, and how the state of the atmosphere in this idealized setup varies between models.
Julia Schmale, Silvia Henning, Stefano Decesari, Bas Henzing, Helmi Keskinen, Karine Sellegri, Jurgita Ovadnevaite, Mira L. Pöhlker, Joel Brito, Aikaterini Bougiatioti, Adam Kristensson, Nikos Kalivitis, Iasonas Stavroulas, Samara Carbone, Anne Jefferson, Minsu Park, Patrick Schlag, Yoko Iwamoto, Pasi Aalto, Mikko Äijälä, Nicolas Bukowiecki, Mikael Ehn, Göran Frank, Roman Fröhlich, Arnoud Frumau, Erik Herrmann, Hartmut Herrmann, Rupert Holzinger, Gerard Kos, Markku Kulmala, Nikolaos Mihalopoulos, Athanasios Nenes, Colin O'Dowd, Tuukka Petäjä, David Picard, Christopher Pöhlker, Ulrich Pöschl, Laurent Poulain, André Stephan Henry Prévôt, Erik Swietlicki, Meinrat O. Andreae, Paulo Artaxo, Alfred Wiedensohler, John Ogren, Atsushi Matsuki, Seong Soo Yum, Frank Stratmann, Urs Baltensperger, and Martin Gysel
Atmos. Chem. Phys., 18, 2853–2881, https://doi.org/10.5194/acp-18-2853-2018, https://doi.org/10.5194/acp-18-2853-2018, 2018
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Collocated long-term observations of cloud condensation nuclei (CCN) number concentrations, particle number size distributions and chemical composition from 12 sites are synthesized. Observations cover coastal environments, the Arctic, the Mediterranean, the boreal and rain forest, high alpine and continental background sites, and Monsoon-influenced areas. We interpret regional and seasonal variability. CCN concentrations are predicted with the κ–Köhler model and compared to the measurements.
Sebastian Düsing, Birgit Wehner, Patric Seifert, Albert Ansmann, Holger Baars, Florian Ditas, Silvia Henning, Nan Ma, Laurent Poulain, Holger Siebert, Alfred Wiedensohler, and Andreas Macke
Atmos. Chem. Phys., 18, 1263–1290, https://doi.org/10.5194/acp-18-1263-2018, https://doi.org/10.5194/acp-18-1263-2018, 2018
Meinrat O. Andreae, Armin Afchine, Rachel Albrecht, Bruna Amorim Holanda, Paulo Artaxo, Henrique M. J. Barbosa, Stephan Borrmann, Micael A. Cecchini, Anja Costa, Maximilian Dollner, Daniel Fütterer, Emma Järvinen, Tina Jurkat, Thomas Klimach, Tobias Konemann, Christoph Knote, Martina Krämer, Trismono Krisna, Luiz A. T. Machado, Stephan Mertes, Andreas Minikin, Christopher Pöhlker, Mira L. Pöhlker, Ulrich Pöschl, Daniel Rosenfeld, Daniel Sauer, Hans Schlager, Martin Schnaiter, Johannes Schneider, Christiane Schulz, Antonio Spanu, Vinicius B. Sperling, Christiane Voigt, Adrian Walser, Jian Wang, Bernadett Weinzierl, Manfred Wendisch, and Helmut Ziereis
Atmos. Chem. Phys., 18, 921–961, https://doi.org/10.5194/acp-18-921-2018, https://doi.org/10.5194/acp-18-921-2018, 2018
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We made airborne measurements of aerosol particle concentrations and properties over the Amazon Basin. We found extremely high concentrations of very small particles in the region between 8 and 14 km altitude all across the basin, which had been recently formed by gas-to-particle conversion at these altitudes. This makes the upper troposphere a very important source region of atmospheric particles with significant implications for the Earth's climate system.
Hannah Meusel, Alexandra Tamm, Uwe Kuhn, Dianming Wu, Anna Lena Leifke, Sabine Fiedler, Nina Ruckteschler, Petya Yordanova, Naama Lang-Yona, Mira Pöhlker, Jos Lelieveld, Thorsten Hoffmann, Ulrich Pöschl, Hang Su, Bettina Weber, and Yafang Cheng
Atmos. Chem. Phys., 18, 799–813, https://doi.org/10.5194/acp-18-799-2018, https://doi.org/10.5194/acp-18-799-2018, 2018
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The photolysis of nitrous acid (HONO) forms the OH radical. However, not all sources are known. Recent studies showed that HONO can be emitted from soil but they did not evaluate the importance to the HONO budget. In this work HONO emissions from 43 soil and biological soil crust samples from Cyprus were measured in a dynamic chamber and extrapolated to the real atmosphere. A large fraction of the local missing source (published earlier; Meusel et al., 2016) could be assigned to soil emissions.
Joel Brito, Evelyn Freney, Pamela Dominutti, Agnes Borbon, Sophie L. Haslett, Anneke M. Batenburg, Aurelie Colomb, Regis Dupuy, Cyrielle Denjean, Frederic Burnet, Thierry Bourriane, Adrien Deroubaix, Karine Sellegri, Stephan Borrmann, Hugh Coe, Cyrille Flamant, Peter Knippertz, and Alfons Schwarzenboeck
Atmos. Chem. Phys., 18, 757–772, https://doi.org/10.5194/acp-18-757-2018, https://doi.org/10.5194/acp-18-757-2018, 2018
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This work focuses on sources of submicron aerosol particles over southern West Africa (SWA). Results have shown that isoprene, a gas-phase compound of biogenic origin, is responsible for roughly 25 % of the organic aerosol (OA) loading, under most background or urban plumes alike. This fraction represents a lower estimate from the biogenic contribution in this fairly polluted region. This work sheds light upon the role of anthropogenic and biogenic emissions on the pollution burden over SWA.
Jessie M. Creamean, Maximilian Maahn, Gijs de Boer, Allison McComiskey, Arthur J. Sedlacek, and Yan Feng
Atmos. Chem. Phys., 18, 555–570, https://doi.org/10.5194/acp-18-555-2018, https://doi.org/10.5194/acp-18-555-2018, 2018
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We report on airborne observations from the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) program's Fifth Airborne Carbon Measurements (ACME-V) campaign along the North Slope of Alaska during the summer of 2015. We show how local oil extraction activities, 2015's central Alaskan wildfires, and, to a lesser extent, long-range transport introduce aerosols and trace gases higher in concentration than previously reported in Arctic haze measurements to the North Slope.
Volker Freudenthaler, Holger Linné, Anatoli Chaikovski, Dieter Rabus, and Silke Groß
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2017-395, https://doi.org/10.5194/amt-2017-395, 2018
Revised manuscript has not been submitted
Romy Heller, Christiane Voigt, Stuart Beaton, Andreas Dörnbrack, Andreas Giez, Stefan Kaufmann, Christian Mallaun, Hans Schlager, Johannes Wagner, Kate Young, and Markus Rapp
Atmos. Chem. Phys., 17, 14853–14869, https://doi.org/10.5194/acp-17-14853-2017, https://doi.org/10.5194/acp-17-14853-2017, 2017
Micael A. Cecchini, Luiz A. T. Machado, Manfred Wendisch, Anja Costa, Martina Krämer, Meinrat O. Andreae, Armin Afchine, Rachel I. Albrecht, Paulo Artaxo, Stephan Borrmann, Daniel Fütterer, Thomas Klimach, Christoph Mahnke, Scot T. Martin, Andreas Minikin, Sergej Molleker, Lianet H. Pardo, Christopher Pöhlker, Mira L. Pöhlker, Ulrich Pöschl, Daniel Rosenfeld, and Bernadett Weinzierl
Atmos. Chem. Phys., 17, 14727–14746, https://doi.org/10.5194/acp-17-14727-2017, https://doi.org/10.5194/acp-17-14727-2017, 2017
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This study introduces and explores the concept of gamma phase space. This space is able to represent all possible variations in the cloud droplet size distributions (DSDs). The methodology was applied to recent in situ aircraft measurements over the Amazon. It is shown that the phase space is able to represent several processes occurring in the clouds in a simple manner. The consequences for cloud studies, modeling, and the representation of the transition from warm to mixed phase are discussed.
Maximilian Maahn, Gijs de Boer, Jessie M. Creamean, Graham Feingold, Greg M. McFarquhar, Wei Wu, and Fan Mei
Atmos. Chem. Phys., 17, 14709–14726, https://doi.org/10.5194/acp-17-14709-2017, https://doi.org/10.5194/acp-17-14709-2017, 2017
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Liquid-containing clouds are a key component of the Arctic climate system and their radiative properties depend strongly on cloud drop sizes. Here, we investigate how cloud drop sizes are modified in the presence of local emissions from industrial facilities at the North Slope of Alaska using aircraft in situ observations. We show that near local anthropogenic sources, the concentrations of black carbon and condensation nuclei are enhanced and cloud drop sizes are reduced.
Ramon Campos Braga, Daniel Rosenfeld, Ralf Weigel, Tina Jurkat, Meinrat O. Andreae, Manfred Wendisch, Ulrich Pöschl, Christiane Voigt, Christoph Mahnke, Stephan Borrmann, Rachel I. Albrecht, Sergej Molleker, Daniel A. Vila, Luiz A. T. Machado, and Lucas Grulich
Atmos. Chem. Phys., 17, 14433–14456, https://doi.org/10.5194/acp-17-14433-2017, https://doi.org/10.5194/acp-17-14433-2017, 2017
Rintaro Okamura, Hironobu Iwabuchi, and K. Sebastian Schmidt
Atmos. Meas. Tech., 10, 4747–4759, https://doi.org/10.5194/amt-10-4747-2017, https://doi.org/10.5194/amt-10-4747-2017, 2017
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Three-dimensional (3-D) radiative transfer effects are a major source of retrieval errors in satellite-based optical remote sensing of clouds. Multi-pixel, multispectral approaches based on deep learning are proposed for retrieval of cloud optical thickness and droplet effective radius. A feasibility test shows that proposed retrieval methods are effective to obtain accurate cloud properties. Use of the convolutional neural network is effective to reduce 3-D radiative transfer effects.
Alexandra Gossart, Niels Souverijns, Irina V. Gorodetskaya, Stef Lhermitte, Jan T. M. Lenaerts, Jan H. Schween, Alexander Mangold, Quentin Laffineur, and Nicole P. M. van Lipzig
The Cryosphere, 11, 2755–2772, https://doi.org/10.5194/tc-11-2755-2017, https://doi.org/10.5194/tc-11-2755-2017, 2017
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Blowing snow plays an important role on local surface mass balance of Antarctica. We present here the blowing snow detection algorithm, to retrieve blowing snow occurrence from the attenuated backscatter signal of ceilometers set up at two station. There is a good correspondence in detection of heavy blowing snow by the algorithm and the visual observations performed at Neumayer station. Moreover, most of the blowing snow occurs during events bringing precipitation from the coast inland.
Tim Carlsen, Gerit Birnbaum, André Ehrlich, Johannes Freitag, Georg Heygster, Larysa Istomina, Sepp Kipfstuhl, Anaïs Orsi, Michael Schäfer, and Manfred Wendisch
The Cryosphere, 11, 2727–2741, https://doi.org/10.5194/tc-11-2727-2017, https://doi.org/10.5194/tc-11-2727-2017, 2017
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The optical size of snow grains (ropt) affects the reflectivity of snow surfaces and thus the local surface energy budget in particular in polar regions. The temporal evolution of ropt retrieved from ground-based, airborne, and spaceborne remote sensing could reproduce optical in situ measurements for a 2-month period in central Antarctica (2013/14). The presented validation study provided a unique testbed for retrievals of ropt under Antarctic conditions where in situ data are scarce.
Ulrich Schumann and Bernhard Mayer
Atmos. Chem. Phys., 17, 13833–13848, https://doi.org/10.5194/acp-17-13833-2017, https://doi.org/10.5194/acp-17-13833-2017, 2017
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It is generally assumed that a positive radiative forcing of the atmosphere implies a warming of the Earth surface. This assumption is valid for well-mixed greenhouse gases but is not guaranteed for disturbances which cause a vertically variable radiative heating rate profile with warming in the upper troposphere and cooling near the surface. This conceptual study shows that the warming induced by contrail cirrus prevails only for fast vertical heat exchange by mixing within the troposphere.
Franziska Köllner, Johannes Schneider, Megan D. Willis, Thomas Klimach, Frank Helleis, Heiko Bozem, Daniel Kunkel, Peter Hoor, Julia Burkart, W. Richard Leaitch, Amir A. Aliabadi, Jonathan P. D. Abbatt, Andreas B. Herber, and Stephan Borrmann
Atmos. Chem. Phys., 17, 13747–13766, https://doi.org/10.5194/acp-17-13747-2017, https://doi.org/10.5194/acp-17-13747-2017, 2017
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We conducted aircraft-based single particle chemical composition measurements in the Canadian high Arctic during summer. Our results provide evidence for a marine-biogenic influence on secondary formation of particulate trimethylamine in the Arctic boundary layer. Understanding emission sources and further processes controlling aerosol number concentration and chemical composition in the pristine Arctic summer is crucial for modeling future climate in the area.
Fabian Jakub and Bernhard Mayer
Atmos. Chem. Phys., 17, 13317–13327, https://doi.org/10.5194/acp-17-13317-2017, https://doi.org/10.5194/acp-17-13317-2017, 2017
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The formation of shallow cumulus cloud streets was historically attributed primarily to dynamics. Here, we focus on the interaction between radiatively induced surface heterogeneities and the resulting patterns in the flow. Our results suggest that solar radiative heating has the potential to organize clouds perpendicular to the sun's incidence angle.
Douglas B. Collins, Julia Burkart, Rachel Y.-W. Chang, Martine Lizotte, Aude Boivin-Rioux, Marjolaine Blais, Emma L. Mungall, Matthew Boyer, Victoria E. Irish, Guillaume Massé, Daniel Kunkel, Jean-Éric Tremblay, Tim Papakyriakou, Allan K. Bertram, Heiko Bozem, Michel Gosselin, Maurice Levasseur, and Jonathan P. D. Abbatt
Atmos. Chem. Phys., 17, 13119–13138, https://doi.org/10.5194/acp-17-13119-2017, https://doi.org/10.5194/acp-17-13119-2017, 2017
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The sources of aerosol particles and their growth to sizes large enough to act as cloud droplet seeds is of major importance to climate since clouds exert substantial control over the atmospheric energy balance. Using ship-board measurements from two summers in the Canadian Arctic, aerosol formation events were related to co-sampled atmospheric and oceanic parameters, providing insight into factors that drive particle formation and motivating further study of ocean–atmosphere interactions.
Guillaume Mioche, Olivier Jourdan, Julien Delanoë, Christophe Gourbeyre, Guy Febvre, Régis Dupuy, Marie Monier, Frédéric Szczap, Alfons Schwarzenboeck, and Jean-François Gayet
Atmos. Chem. Phys., 17, 12845–12869, https://doi.org/10.5194/acp-17-12845-2017, https://doi.org/10.5194/acp-17-12845-2017, 2017
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This paper is a study about the mixed-phase clouds frequently occurring in the Arctic region. It is based on airborne measurements and highlights the microphysical properties of these particular clouds composed of liquid droplets at cloud top and ice crystals below precipitating down to the surface. This work may help to improve the representation of the mixed-phase clouds in numerical prediction models as well as the retrieval of their properties from remote sensing observations.
Katharina Schütze, James Charles Wilson, Stephan Weinbruch, Nathalie Benker, Martin Ebert, Gebhard Günther, Ralf Weigel, and Stephan Borrmann
Atmos. Chem. Phys., 17, 12475–12493, https://doi.org/10.5194/acp-17-12475-2017, https://doi.org/10.5194/acp-17-12475-2017, 2017
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Stratospheric particles were collected in the polar stratosphere in winter 1999/2000. Besides the well-studied volatile particles from that region, the main findings of this study are stable carbonaceous particles in the sub-micrometer size range. In addition to carbon, many particles show the elements Si, Fe, Cr and Ni to a minor amount. Based on exclusion, carbonaceous material from IDPs and residues from meteoric ablation and fragmentation remain as the most probable sources.
Anja Costa, Jessica Meyer, Armin Afchine, Anna Luebke, Gebhard Günther, James R. Dorsey, Martin W. Gallagher, Andre Ehrlich, Manfred Wendisch, Darrel Baumgardner, Heike Wex, and Martina Krämer
Atmos. Chem. Phys., 17, 12219–12238, https://doi.org/10.5194/acp-17-12219-2017, https://doi.org/10.5194/acp-17-12219-2017, 2017
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The paper presents 38 h of in situ cloud spectrometer observations of microphysical cloud properties in the Arctic, midlatitudes and tropics. The clouds are classified via particle concentrations, size distributions, and – as a novelty – small particle aspherical fractions. Cloud-type profiles are given for different temperatures and locations. The results confine regions where different cloud transformation processes occurred and emphasise the importance of small particle shape detection.
Jun-Wei Xu, Randall V. Martin, Andrew Morrow, Sangeeta Sharma, Lin Huang, W. Richard Leaitch, Julia Burkart, Hannes Schulz, Marco Zanatta, Megan D. Willis, Daven K. Henze, Colin J. Lee, Andreas B. Herber, and Jonathan P. D. Abbatt
Atmos. Chem. Phys., 17, 11971–11989, https://doi.org/10.5194/acp-17-11971-2017, https://doi.org/10.5194/acp-17-11971-2017, 2017
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We interpret a series of recent airborne and ground-based measurements with the GEOS-Chem model and its adjoint to attribute the sources of Arctic BC. Anthropogenic emissions in eastern and southern Asia make the largest contribution to Arctic BC. Gas flaring emissions from oilfields in western Siberia and from the Tarim oilfield in western China could have striking impacts on Arctic BC loadings.
Heiko Bozem, Andrea Pozzer, Hartwig Harder, Monica Martinez, Jonathan Williams, Jos Lelieveld, and Horst Fischer
Atmos. Chem. Phys., 17, 11835–11848, https://doi.org/10.5194/acp-17-11835-2017, https://doi.org/10.5194/acp-17-11835-2017, 2017
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We present a case study of deep convection over Germany in July 2007 within the framework of the HOOVER II project. Airborne in situ measurements within the in- and outflow regions of an isolated thunderstorm provide a unique data set to study the influence of deep convection on the transport efficiency of soluble and insoluble trace gases. Despite their high solubility HCHO and H2O2 show enhanced concentrations in the outflow presumably due to degassing from cloud droplets during freezing.
Ryan Thalman, Suzane S. de Sá, Brett B. Palm, Henrique M. J. Barbosa, Mira L. Pöhlker, M. Lizabeth Alexander, Joel Brito, Samara Carbone, Paulo Castillo, Douglas A. Day, Chongai Kuang, Antonio Manzi, Nga Lee Ng, Arthur J. Sedlacek III, Rodrigo Souza, Stephen Springston, Thomas Watson, Christopher Pöhlker, Ulrich Pöschl, Meinrat O. Andreae, Paulo Artaxo, Jose L. Jimenez, Scot T. Martin, and Jian Wang
Atmos. Chem. Phys., 17, 11779–11801, https://doi.org/10.5194/acp-17-11779-2017, https://doi.org/10.5194/acp-17-11779-2017, 2017
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Particle hygroscopicity, mixing state, and the hygroscopicity of organic components were characterized in central Amazonia for 1 year; their seasonal and diel variations were driven by a combination of primary emissions, photochemical oxidation, and boundary layer development. The relationship between the hygroscopicity of organic components and their oxidation level was examined, and the results help to reconcile the differences among the relationships observed in previous studies.
Monika Burkert-Kohn, Heike Wex, André Welti, Susan Hartmann, Sarah Grawe, Lisa Hellner, Paul Herenz, James D. Atkinson, Frank Stratmann, and Zamin A. Kanji
Atmos. Chem. Phys., 17, 11683–11705, https://doi.org/10.5194/acp-17-11683-2017, https://doi.org/10.5194/acp-17-11683-2017, 2017
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Several instruments can investigate properties of ice-nucleating particles (INPs), which are crucial to understanding ice cloud formation. We intercompare four online ice nucleation counters and reasonable agreement is found when the same ice nucleation mode is tested. A variable scaling factor was necessary to reconcile condensation freezing results with immersion freezing. Factors related to instrumental setup and aerosol generation are discussed to explain observed differences.
Marcus Klingebiel, André Ehrlich, Fanny Finger, Timo Röschenthaler, Suad Jakirlić, Matthias Voigt, Stefan Müller, Rolf Maser, Manfred Wendisch, Peter Hoor, Peter Spichtinger, and Stephan Borrmann
Atmos. Meas. Tech., 10, 3485–3498, https://doi.org/10.5194/amt-10-3485-2017, https://doi.org/10.5194/amt-10-3485-2017, 2017
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Microphysical and radiation measurements were collected with the unique AIRcraft TOwed Sensor Shuttle (AIRTOSS) – Learjet tandem platform. It is a combination of a Learjet 35A research aircraft and an instrumented aerodynamic bird, which can be detached from and retracted back to the aircraft during flight.
AIRTOSS and Learjet are equipped with radiative, cloud microphysical, trace gas,
and meteorological instruments to study cirrus clouds.
Jean-Christophe Raut, Louis Marelle, Jerome D. Fast, Jennie L. Thomas, Bernadett Weinzierl, Katharine S. Law, Larry K. Berg, Anke Roiger, Richard C. Easter, Katharina Heimerl, Tatsuo Onishi, Julien Delanoë, and Hans Schlager
Atmos. Chem. Phys., 17, 10969–10995, https://doi.org/10.5194/acp-17-10969-2017, https://doi.org/10.5194/acp-17-10969-2017, 2017
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We study the cross-polar transport of plumes from Siberian fires to the Arctic in summer, both in terms of transport pathways and efficiency of deposition processes. Those plumes containing soot may originate from anthropogenic and biomass burning sources in mid-latitude regions and may impact the Arctic climate by depositing on snow and ice surfaces. We evaluate the role of the respective source contributions, investigate the transport of plumes and treat pathway-dependent removal of particles.
Eivind G. Wærsted, Martial Haeffelin, Jean-Charles Dupont, Julien Delanoë, and Philippe Dubuisson
Atmos. Chem. Phys., 17, 10811–10835, https://doi.org/10.5194/acp-17-10811-2017, https://doi.org/10.5194/acp-17-10811-2017, 2017
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Heating and cooling of fog layers by solar and terrestrial radiation influence the fog life cycle. We quantify these radiative impacts on fog liquid water using detailed cloud radar observations of seven fog events as well as sensitivity studies. We find that the impact of radiation is affected mainly by fog optical thickness, atmospheric humidity and the presence of clouds above the fog. Observing these quantities in real time can therefore be useful for forecasting fog dissipation.
Moritz Haarig, Albert Ansmann, Dietrich Althausen, André Klepel, Silke Groß, Volker Freudenthaler, Carlos Toledano, Rodanthi-Elisavet Mamouri, David A. Farrell, Damien A. Prescod, Eleni Marinou, Sharon P. Burton, Josef Gasteiger, Ronny Engelmann, and Holger Baars
Atmos. Chem. Phys., 17, 10767–10794, https://doi.org/10.5194/acp-17-10767-2017, https://doi.org/10.5194/acp-17-10767-2017, 2017
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Our measurements performed with a lidar on Barbados give a vertical profile of Saharan dust, which was transported over 5000 km across the Atlantic. The new triple-wavelength depolarization technique reveals more information about the shape and size of dust, which will improve our understanding of the aging process of dust in the atmosphere and its representation in dust models. Changing properties of dust particles influence the solar radiation and the cloud properties and thus our climate.
Heiko Bozem, Tim M. Butler, Mark G. Lawrence, Hartwig Harder, Monica Martinez, Dagmar Kubistin, Jos Lelieveld, and Horst Fischer
Atmos. Chem. Phys., 17, 10565–10582, https://doi.org/10.5194/acp-17-10565-2017, https://doi.org/10.5194/acp-17-10565-2017, 2017
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We present airborne measurements and model simulations in the tropics and mid-latitudes during GABRIEL and HOOVER, respectively. Based only on in situ data net ozone formation/destruction tendencies (NOPR) are calculated and compared to a 3-D chemistry transport model. The NOPR is positive in the continental boundary layer and the upper troposphere above 6 km. In the marine boundary layer and the middle troposphere ozone destruction prevails. Fresh convection shows strong net ozone formation.
Leonid Nichman, Emma Järvinen, James Dorsey, Paul Connolly, Jonathan Duplissy, Claudia Fuchs, Karoliina Ignatius, Kamalika Sengupta, Frank Stratmann, Ottmar Möhler, Martin Schnaiter, and Martin Gallagher
Atmos. Meas. Tech., 10, 3231–3248, https://doi.org/10.5194/amt-10-3231-2017, https://doi.org/10.5194/amt-10-3231-2017, 2017
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Optical probes are frequently used for the detection of cloud particles. The detected microphysical properties may affect particle growth and accretion mechanisms and the light scattering properties of cirrus clouds. In the CLOUD chamber study at CERN, we compared four optical measurement techniques. We show that shape derivation alone is not sufficient to determine the phase of the small cloud particles. None of the instruments were able to unambiguously determine the phase of small particles.
André Ehrlich, Eike Bierwirth, Larysa Istomina, and Manfred Wendisch
Atmos. Meas. Tech., 10, 3215–3230, https://doi.org/10.5194/amt-10-3215-2017, https://doi.org/10.5194/amt-10-3215-2017, 2017
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In the Arctic, uncertainties in passive solar remote sensing of cloud properties arise from uncertainties in the assumed spectral surface albedo, mainly determined by the generally unknown effective snow grain size. Therefore, a retrieval method is presented that simultaneously derives liquid water cloud and snow surface parameters, including cloud optical thickness, droplet effective radius, and effective snow grain size. Airborne measurements were used to test the retrieval procedure.
Stefan Metzger, David Durden, Cove Sturtevant, Hongyan Luo, Natchaya Pingintha-Durden, Torsten Sachs, Andrei Serafimovich, Jörg Hartmann, Jiahong Li, Ke Xu, and Ankur R. Desai
Geosci. Model Dev., 10, 3189–3206, https://doi.org/10.5194/gmd-10-3189-2017, https://doi.org/10.5194/gmd-10-3189-2017, 2017
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We apply the
development and systems operationssoftware development model to create the eddy4R–Docker open-source, flexible, and modular eddy-covariance data processing environment. Test applications to aircraft and tower data, as well as a software cross validation demonstrate its efficiency and consistency. Key improvements in accessibility, extensibility, and reproducibility build the foundation for deploying complex scientific algorithms in an effective and scalable manner.
Micael A. Cecchini, Luiz A. T. Machado, Meinrat O. Andreae, Scot T. Martin, Rachel I. Albrecht, Paulo Artaxo, Henrique M. J. Barbosa, Stephan Borrmann, Daniel Fütterer, Tina Jurkat, Christoph Mahnke, Andreas Minikin, Sergej Molleker, Mira L. Pöhlker, Ulrich Pöschl, Daniel Rosenfeld, Christiane Voigt, Bernadett Weinzierl, and Manfred Wendisch
Atmos. Chem. Phys., 17, 10037–10050, https://doi.org/10.5194/acp-17-10037-2017, https://doi.org/10.5194/acp-17-10037-2017, 2017
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We study the effects of aerosol particles and updraft speed on the warm phase of Amazonian clouds. We expand the sensitivity analysis usually found in the literature by concomitantly considering cloud evolution and the effects on droplet size distribution (DSD) shape. The quantitative results show that particle concentration is the primary driver for the vertical profiles of effective diameter and droplet concentration in the warm phase of Amazonian convective clouds.
Alexander Jost, Miklós Szakáll, Karoline Diehl, Subir K. Mitra, and Stephan Borrmann
Atmos. Chem. Phys., 17, 9717–9732, https://doi.org/10.5194/acp-17-9717-2017, https://doi.org/10.5194/acp-17-9717-2017, 2017
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During riming of graupel and hail, soluble chemical trace constituents contained in the liquid droplets could be retained while freezing onto the glaciated particle, or released back to the air potentially at other altitudes as retained. Quantification of retention constitutes a major uncertainty in numerical models for atmospheric chemistry and improvements hinge upon experimental determination of retention for carboxylic acids, aldehydes, SO2, H2O2, NH2, and others, as presented in this paper.
Jorge Saturno, Christopher Pöhlker, Dario Massabò, Joel Brito, Samara Carbone, Yafang Cheng, Xuguang Chi, Florian Ditas, Isabella Hrabě de Angelis, Daniel Morán-Zuloaga, Mira L. Pöhlker, Luciana V. Rizzo, David Walter, Qiaoqiao Wang, Paulo Artaxo, Paolo Prati, and Meinrat O. Andreae
Atmos. Meas. Tech., 10, 2837–2850, https://doi.org/10.5194/amt-10-2837-2017, https://doi.org/10.5194/amt-10-2837-2017, 2017
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Different Aethalometer correction schemes were compared to a multi-wavelength absorption reference measurement. One of the correction schemes was found to artificially increase the short-wavelength absorption coefficients. It was found that accounting for aerosol scattering properties in the correction is crucial to retrieve the proper absorption Ångström exponent (AAE). We found that the raw AAE of uncompensated Aethalometer attenuation significantly correlates with a measured reference AAE.
Lena Frey, Frida A.-M. Bender, and Gunilla Svensson
Atmos. Chem. Phys., 17, 9145–9162, https://doi.org/10.5194/acp-17-9145-2017, https://doi.org/10.5194/acp-17-9145-2017, 2017
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In this study, the cloud albedo effect in climate models is investigated, separating the influence of anthropogenic sulfate and non-sulfate aerosols. Cloud albedo changes induced by added anthropogenic aerosols are found to be determined by changes in the cloud water content rather than model sensitivity to monthly aerosol variations. The results also indicate that the background aerosol is the main driver for a cloud brightening effect on the month-to-month scale.
Evelyn Jäkel, Manfred Wendisch, Trismono C. Krisna, Florian Ewald, Tobias Kölling, Tina Jurkat, Christiane Voigt, Micael A. Cecchini, Luiz A. T. Machado, Armin Afchine, Anja Costa, Martina Krämer, Meinrat O. Andreae, Ulrich Pöschl, Daniel Rosenfeld, and Tianle Yuan
Atmos. Chem. Phys., 17, 9049–9066, https://doi.org/10.5194/acp-17-9049-2017, https://doi.org/10.5194/acp-17-9049-2017, 2017
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Vertical profiles of the cloud particle phase state in tropical deep convective clouds (DCCs) were investigated using airborne imaging spectrometer measurements during the ACRIDICON-CHUVA campaign, which was conducted over the Brazilian rainforest in September 2014. A phase discrimination retrieval was applied to observations of clouds formed in different aerosol conditions. The profiles were compared to in situ and satellite measurements.
Georgios Tsagkogeorgas, Pontus Roldin, Jonathan Duplissy, Linda Rondo, Jasmin Tröstl, Jay G. Slowik, Sebastian Ehrhart, Alessandro Franchin, Andreas Kürten, Antonio Amorim, Federico Bianchi, Jasper Kirkby, Tuukka Petäjä, Urs Baltensperger, Michael Boy, Joachim Curtius, Richard C. Flagan, Markku Kulmala, Neil M. Donahue, and Frank Stratmann
Atmos. Chem. Phys., 17, 8923–8938, https://doi.org/10.5194/acp-17-8923-2017, https://doi.org/10.5194/acp-17-8923-2017, 2017
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The H2SO4 vapour pressure plays key role in Earth's and Venus' atmospheres. In regions where RH is low and stabilising bases are scarce, H2SO4 can evaporate from particles; however the H2SO4 vapour pressure at low RH is uncertain. To address this, we measured H2SO4 evaporation versus T and RH in the CLOUD chamber and constrained the equilibrium constants for dissociation and dehydration of H2SO4. This study is important for nucleation, particle growth and H2SO4 formation occurring in atmosphere.
Roya Ghahreman, Ann-Lise Norman, Betty Croft, Randall V. Martin, Jeffrey R. Pierce, Julia Burkart, Ofelia Rempillo, Heiko Bozem, Daniel Kunkel, Jennie L. Thomas, Amir A. Aliabadi, Gregory R. Wentworth, Maurice Levasseur, Ralf M. Staebler, Sangeeta Sharma, and W. Richard Leaitch
Atmos. Chem. Phys., 17, 8757–8770, https://doi.org/10.5194/acp-17-8757-2017, https://doi.org/10.5194/acp-17-8757-2017, 2017
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We present spring and summertime vertical profile measurements of Arctic dimethyl sulfide (DMS), together with model simulations to consider what these profiles indicate about DMS sources and lifetimes in the Arctic. Our results highlight the role of local open water as the source of DMS(g) during July 2014 and the influence of long-range transport of DMS(g) from further afield in the Arctic during April 2015.
Linda Forster, Meinhard Seefeldner, Matthias Wiegner, and Bernhard Mayer
Atmos. Meas. Tech., 10, 2499–2516, https://doi.org/10.5194/amt-10-2499-2017, https://doi.org/10.5194/amt-10-2499-2017, 2017
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Halo displays are produced by scattering of sunlight by smooth, hexagonal ice crystals. Consequently, the presence of a halo should contain information on particle shape. This study presents HaloCam, a novel sun-tracking camera system, and an automated detection algorithm to collect and evaluate long-term halo observations. Two-year HaloCam observations revealed that about 25 % of the detected cirrus clouds occurred together with a 22° halo indicating the presence of smooth, hexagonal crystals.
Gunnar Spreen, Ron Kwok, Dimitris Menemenlis, and An T. Nguyen
The Cryosphere, 11, 1553–1573, https://doi.org/10.5194/tc-11-1553-2017, https://doi.org/10.5194/tc-11-1553-2017, 2017
Andrea Mues, Maheswar Rupakheti, Christoph Münkel, Axel Lauer, Heiko Bozem, Peter Hoor, Tim Butler, and Mark G. Lawrence
Atmos. Chem. Phys., 17, 8157–8176, https://doi.org/10.5194/acp-17-8157-2017, https://doi.org/10.5194/acp-17-8157-2017, 2017
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Ceilometer measurements taken in the Kathmandu Valley, Nepal, were used to study the temporal and spatial evolution of the mixing layer height in the valley. This provides important information on the vertical structure of the atmosphere and can thus also help to understand the mixing of air pollutants (e.g. black carbon) in the valley. The seasonal and diurnal cycles of the mixing layer were found to be highly dependent on meteorology and mainly anticorrelated to black carbon concentrations.
Ramon Campos Braga, Daniel Rosenfeld, Ralf Weigel, Tina Jurkat, Meinrat O. Andreae, Manfred Wendisch, Mira L. Pöhlker, Thomas Klimach, Ulrich Pöschl, Christopher Pöhlker, Christiane Voigt, Christoph Mahnke, Stephan Borrmann, Rachel I. Albrecht, Sergej Molleker, Daniel A. Vila, Luiz A. T. Machado, and Paulo Artaxo
Atmos. Chem. Phys., 17, 7365–7386, https://doi.org/10.5194/acp-17-7365-2017, https://doi.org/10.5194/acp-17-7365-2017, 2017
Rieke Heinze, Christopher Moseley, Lennart Nils Böske, Shravan Kumar Muppa, Vera Maurer, Siegfried Raasch, and Bjorn Stevens
Atmos. Chem. Phys., 17, 7083–7109, https://doi.org/10.5194/acp-17-7083-2017, https://doi.org/10.5194/acp-17-7083-2017, 2017
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High-resolution multi-week simulations of a measurement campaign are evaluated with respect to mean boundary layer quantities and turbulence statistics. Two models are used in a semi-idealized setup through forcing, with output from a coarser-scale model to account for the larger-scale conditions. The boundary layer depth is in principal agreement with observations. Turbulence statistics like variance profiles agree satisfactorily with measurements.
Elena Shevnina, Ekaterina Kourzeneva, Viktor Kovalenko, and Timo Vihma
Hydrol. Earth Syst. Sci., 21, 2559–2578, https://doi.org/10.5194/hess-21-2559-2017, https://doi.org/10.5194/hess-21-2559-2017, 2017
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This paper presents the probabilistic approach to evaluate design floods in a changing climate, adapted in this case to the northern territories. For the Russian Arctic, the regions are delineated, where it is suggested to correct engineering hydrological calculations to account for climate change. An example of the calculation of a maximal discharge of 1 % exceedance probability for the Nadym River at Nadym is provided.
Harald Sodemann, Franziska Aemisegger, Stephan Pfahl, Mark Bitter, Ulrich Corsmeier, Thomas Feuerle, Pascal Graf, Rolf Hankers, Gregor Hsiao, Helmut Schulz, Andreas Wieser, and Heini Wernli
Atmos. Chem. Phys., 17, 6125–6151, https://doi.org/10.5194/acp-17-6125-2017, https://doi.org/10.5194/acp-17-6125-2017, 2017
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We report here the first survey of stable water isotope composition over the Mediterranean sea made from aircraft. The stable isotope composition of the atmospheric water vapour changed in response to evaporation conditions at the sea surface, elevation, and airmass transport history. Our data set will be valuable for testing how water is transported in weather prediction and climate models and for understanding processes in the Mediterranean water cycle.
Klaus-D. Gottschaldt, Hans Schlager, Robert Baumann, Heiko Bozem, Veronika Eyring, Peter Hoor, Patrick Jöckel, Tina Jurkat, Christiane Voigt, Andreas Zahn, and Helmut Ziereis
Atmos. Chem. Phys., 17, 6091–6111, https://doi.org/10.5194/acp-17-6091-2017, https://doi.org/10.5194/acp-17-6091-2017, 2017
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We present upper-tropospheric trace gas measurements in the Asian summer monsoon anticyclone, obtained with the HALO research aircraft in September 2012. The anticyclone is one of the largest atmospheric features on Earth, but many aspects of it are not well understood. With the help of model simulations we find that entrainments from the tropopause region and the lower troposphere, combined with photochemistry and dynamical instabilities, can explain the observations.
Claudia Acquistapace, Stefan Kneifel, Ulrich Löhnert, Pavlos Kollias, Maximilian Maahn, and Matthias Bauer-Pfundstein
Atmos. Meas. Tech., 10, 1783–1802, https://doi.org/10.5194/amt-10-1783-2017, https://doi.org/10.5194/amt-10-1783-2017, 2017
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The goal of the paper is to understand what the optimal cloud radar settings for drizzle detection are. The number of cloud radars in the world has increased in the last 10 years and it is important to develop strategies to derive optimal settings which can be applied to all radar systems. The study is part of broader research focused on better understanding the microphysical process of drizzle growth using ground-based observations.
Katrina M. Macdonald, Sangeeta Sharma, Desiree Toom, Alina Chivulescu, Sarah Hanna, Allan K. Bertram, Andrew Platt, Mike Elsasser, Lin Huang, David Tarasick, Nathan Chellman, Joseph R. McConnell, Heiko Bozem, Daniel Kunkel, Ying Duan Lei, Greg J. Evans, and Jonathan P. D. Abbatt
Atmos. Chem. Phys., 17, 5775–5788, https://doi.org/10.5194/acp-17-5775-2017, https://doi.org/10.5194/acp-17-5775-2017, 2017
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Rapid climate changes within the Arctic have highlighted existing uncertainties in the transport of contaminants to Arctic snow. Fresh snow samples collected frequently through the winter season were analyzed for major constituents creating a unique record of Arctic snow. Comparison with simultaneous atmospheric measurements provides insight into the driving processes in the transfer of contaminants from air to snow. The relative importance of deposition mechanisms over the season is proposed.
Benedikt Urbanek, Silke Groß, Andreas Schäfler, and Martin Wirth
Atmos. Meas. Tech., 10, 1653–1664, https://doi.org/10.5194/amt-10-1653-2017, https://doi.org/10.5194/amt-10-1653-2017, 2017
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Cirrus evolution from nucleation to cloud breakup can be investigated with a novel classification scheme based on airborne lidar data. Applying it to a case study from the ML-CIRRUS campaign, we investigate the impact of large-scale dynamics and small-scale gravity lee waves on the detailed spatial distribution of evolution stages in individual clouds. Our scheme may help to gain more insights in optical and radiative properties of cirrus under various formation and life cycle conditions.
Julia Burkart, Megan D. Willis, Heiko Bozem, Jennie L. Thomas, Kathy Law, Peter Hoor, Amir A. Aliabadi, Franziska Köllner, Johannes Schneider, Andreas Herber, Jonathan P. D. Abbatt, and W. Richard Leaitch
Atmos. Chem. Phys., 17, 5515–5535, https://doi.org/10.5194/acp-17-5515-2017, https://doi.org/10.5194/acp-17-5515-2017, 2017
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Our aircraft study for the first time systematically investigates aerosol size distributions, including ultrafine particles (5–20 nm in diameter), in the Arctic summertime atmosphere. We find that ultrafine particles occur very frequently in the boundary layer and not aloft, suggesting a surface source of these particles. Understanding aerosol properties and sources is crucial to predict climate and especially important in the Arctic as this region responds extremely fast to climate change.
Carolin Klinger, Bernhard Mayer, Fabian Jakub, Tobias Zinner, Seung-Bu Park, and Pierre Gentine
Atmos. Chem. Phys., 17, 5477–5500, https://doi.org/10.5194/acp-17-5477-2017, https://doi.org/10.5194/acp-17-5477-2017, 2017
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Radiation is driving weather and climate. Yet, the effect of radiation on clouds is not fully understood and often only poorly represented in models. Better understanding and better parameterizations of the radiation–cloud interaction are therefore essential. Using our newly developed fast
neighboring column approximationfor 3-D thermal heating and cooling rates, we show that thermal radiation changes cloud circulation and causes organization and a deepening of the clouds.
Johannes R. W. Fachinger, Stéphane J. Gallavardin, Frank Helleis, Friederike Fachinger, Frank Drewnick, and Stephan Borrmann
Atmos. Meas. Tech., 10, 1623–1637, https://doi.org/10.5194/amt-10-1623-2017, https://doi.org/10.5194/amt-10-1623-2017, 2017
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The design of an ion trap aerosol mass spectrometer was improved, allowing for the instrument's first field deployment. Detection limits were found to be sufficiently low for ambient measurements. Via MS-MS measurements the instrument is capable of differentiating ion fragments of different elemental compositions, but also fragments which only differ in their molecular structures. This could allow for e.g. the differentiation between sugars and carboxylic acids by MS–MS studies on m/z 60 and 73.
Andreas Macke, Patric Seifert, Holger Baars, Christian Barthlott, Christoph Beekmans, Andreas Behrendt, Birger Bohn, Matthias Brueck, Johannes Bühl, Susanne Crewell, Thomas Damian, Hartwig Deneke, Sebastian Düsing, Andreas Foth, Paolo Di Girolamo, Eva Hammann, Rieke Heinze, Anne Hirsikko, John Kalisch, Norbert Kalthoff, Stefan Kinne, Martin Kohler, Ulrich Löhnert, Bomidi Lakshmi Madhavan, Vera Maurer, Shravan Kumar Muppa, Jan Schween, Ilya Serikov, Holger Siebert, Clemens Simmer, Florian Späth, Sandra Steinke, Katja Träumner, Silke Trömel, Birgit Wehner, Andreas Wieser, Volker Wulfmeyer, and Xinxin Xie
Atmos. Chem. Phys., 17, 4887–4914, https://doi.org/10.5194/acp-17-4887-2017, https://doi.org/10.5194/acp-17-4887-2017, 2017
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This article provides an overview of the instrumental setup and the main results obtained during the two HD(CP)2 Observational Prototype Experiments HOPE-Jülich and HOPE-Melpitz conducted in Germany in April–May and Sept 2013, respectively. Goal of the field experiments was to provide high-resolution observational datasets for both, improving the understaning of boundary layer and cloud processes, as well as for the evaluation of the new ICON model that is run at 156 m horizontal resolution.
Kevin Wolf, André Ehrlich, Tilman Hüneke, Klaus Pfeilsticker, Frank Werner, Martin Wirth, and Manfred Wendisch
Atmos. Chem. Phys., 17, 4283–4303, https://doi.org/10.5194/acp-17-4283-2017, https://doi.org/10.5194/acp-17-4283-2017, 2017
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The potential of airborne radiance measurements in the sideward and nadir directions for cirrus remote sensing is investigated. Therefore radiative transfer simulations were used and the sensitivity of upward radiance with respect to optical thickness, effective radius, surface albedo, wavelength and viewing angle was studied. It was shown that sideward observations lead to more accurate retrieval results. Investigating a case study of ML-CIRRUS, these findings are confirmed.
Paul Vallelonga, Niccolo Maffezzoli, Andrew D. Moy, Mark A. J. Curran, Tessa R. Vance, Ross Edwards, Gwyn Hughes, Emily Barker, Gunnar Spreen, Alfonso Saiz-Lopez, J. Pablo Corella, Carlos A. Cuevas, and Andrea Spolaor
Clim. Past, 13, 171–184, https://doi.org/10.5194/cp-13-171-2017, https://doi.org/10.5194/cp-13-171-2017, 2017
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We present a study of bromine, iodine and sodium in an ice core from Law Dome, in coastal East Antarctica. We find that bromine and iodine variability at Law Dome is correlated to changes in the area of sea ice along the Law Dome coast as observed by satellite since the early 1970s. These findings are in agreement with a previous study based on MSA and confirm a long-term trend of sea ice decrease for this sector of Antarctica over the 20th century.
Michael Schäfer, Eike Bierwirth, André Ehrlich, Evelyn Jäkel, Frank Werner, and Manfred Wendisch
Atmos. Chem. Phys., 17, 2359–2372, https://doi.org/10.5194/acp-17-2359-2017, https://doi.org/10.5194/acp-17-2359-2017, 2017
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Cloud optical thickness fields, retrieved from solar spectral radiance measurements, are used to investigate the directional structure of horizontal cloud inhomogeneities with scalar one-dimensional inhomogeneity parameters, two-dimensional auto-correlation functions, and two-dimensional Fourier analysis. The investigations reveal that it is not sufficient to quantify horizontal cloud inhomogeneities by one-dimensional inhomogeneity parameters; two-dimensional parameters are necessary.
Ulrich Schumann, Christoph Kiemle, Hans Schlager, Ralf Weigel, Stephan Borrmann, Francesco D'Amato, Martina Krämer, Renaud Matthey, Alain Protat, Christiane Voigt, and C. Michael Volk
Atmos. Chem. Phys., 17, 2311–2346, https://doi.org/10.5194/acp-17-2311-2017, https://doi.org/10.5194/acp-17-2311-2017, 2017
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A long-lived (1 h) contrail and overshooting convection were observed in the tropics, near Darwin, Australia. The data are used to study the contrail life cycle at low temperatures and cirrus from deep overturning convection in the lower tropical stratosphere. Airborne in situ, lidar, profiler, radar, and satellite data, as well as a photo, are used to distinguish contrail cirrus from convective cirrus and to study the origin of the observed ice and aerosol, up to 2.3 km above the tropopause.
Tobias Sirch, Luca Bugliaro, Tobias Zinner, Matthias Möhrlein, and Margarita Vazquez-Navarro
Atmos. Meas. Tech., 10, 409–429, https://doi.org/10.5194/amt-10-409-2017, https://doi.org/10.5194/amt-10-409-2017, 2017
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A novel approach for the nowcasting of clouds and direct normal irradiance (DNI) based on the geostationary satellite MSG is presented. The basis of the algorithm is an optical flow method to derive cloud motion vectors for low and high level clouds separately. DNI is calculated from the forecasted optical thickness of the clouds. Validation against MSG observations shows good performance: compared to persistence an improvement of forecast horizon by a factor of 2 is reached for 2 h forecasts.
Bjorn Stevens, Stephanie Fiedler, Stefan Kinne, Karsten Peters, Sebastian Rast, Jobst Müsse, Steven J. Smith, and Thorsten Mauritsen
Geosci. Model Dev., 10, 433–452, https://doi.org/10.5194/gmd-10-433-2017, https://doi.org/10.5194/gmd-10-433-2017, 2017
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A simple analytic description of aerosol optical properties and their main effects on clouds is developed and described. The analytic description is easy to use and easy to modify and should aid experimentation to help understand how aerosol radiative and cloud interactions effect climate and circulation. The climatology is recommended for adoption by models participating in the sixth phase of the Coupled Model Intercomparison Project.
Johannes Schneider, Stephan Mertes, Dominik van Pinxteren, Hartmut Herrmann, and Stephan Borrmann
Atmos. Chem. Phys., 17, 1571–1593, https://doi.org/10.5194/acp-17-1571-2017, https://doi.org/10.5194/acp-17-1571-2017, 2017
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We analyzed the composition of cloud droplet residuals and of aerosol particles sampled on a mountaintop site. The data show that about 85 % of the submicron aerosol mass partitions into the cloud phase, and that the uptake of soluble compounds (nitric acid, ammonia, and organic gases) from the gas phase into the cloud droplets is very effective. This will lead to a redistribution of these compounds among the aerosol particles and thereby to a more uniform aerosol after cloud evaporation.
Mark J. Webb, Timothy Andrews, Alejandro Bodas-Salcedo, Sandrine Bony, Christopher S. Bretherton, Robin Chadwick, Hélène Chepfer, Hervé Douville, Peter Good, Jennifer E. Kay, Stephen A. Klein, Roger Marchand, Brian Medeiros, A. Pier Siebesma, Christopher B. Skinner, Bjorn Stevens, George Tselioudis, Yoko Tsushima, and Masahiro Watanabe
Geosci. Model Dev., 10, 359–384, https://doi.org/10.5194/gmd-10-359-2017, https://doi.org/10.5194/gmd-10-359-2017, 2017
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The Cloud Feedback Model Intercomparison Project (CFMIP) aims to improve understanding of cloud-climate feedback mechanisms and evaluation of cloud processes and cloud feedbacks in climate models. CFMIP also aims to improve understanding of circulation, regional-scale precipitation and non-linear changes. CFMIP is contributing to the 6th phase of the Coupled Model Intercomparison Project (CMIP6) by coordinating a hierarchy of targeted experiments with cloud-related model outputs.
Susan Schmidt, Johannes Schneider, Thomas Klimach, Stephan Mertes, Ludwig Paul Schenk, Piotr Kupiszewski, Joachim Curtius, and Stephan Borrmann
Atmos. Chem. Phys., 17, 575–594, https://doi.org/10.5194/acp-17-575-2017, https://doi.org/10.5194/acp-17-575-2017, 2017
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Ice formation in clouds is an important process in the formation of precipitation, especially at midlatitudes, but the exact properties of the aerosol particles that initiate freezing is not fully understood. We analysed residual particles from ice crystals sampled from mixed phase clouds. The results show that the residues contain a larger relative amount of soil dust and minerals, but also particles from industrial emissions and lead-containing particles, than the out-of-cloud aerosol.
Ulrich Schumann, Robert Baumann, Darrel Baumgardner, Sarah T. Bedka, David P. Duda, Volker Freudenthaler, Jean-Francois Gayet, Andrew J. Heymsfield, Patrick Minnis, Markus Quante, Ehrhard Raschke, Hans Schlager, Margarita Vázquez-Navarro, Christiane Voigt, and Zhien Wang
Atmos. Chem. Phys., 17, 403–438, https://doi.org/10.5194/acp-17-403-2017, https://doi.org/10.5194/acp-17-403-2017, 2017
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The initially linear clouds often seen behind aircraft are known as contrails. Contrails are prototype cirrus clouds forming under well-known conditions, but with less certain life cycle and climate effects. This paper collects contrail data from a large set of measurements and compares them among each other and with models. The observations show consistent contrail properties over a wide range of aircraft and atmosphere conditions. The dataset is available for further research.
Josef Gasteiger, Silke Groß, Daniel Sauer, Moritz Haarig, Albert Ansmann, and Bernadett Weinzierl
Atmos. Chem. Phys., 17, 297–311, https://doi.org/10.5194/acp-17-297-2017, https://doi.org/10.5194/acp-17-297-2017, 2017
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To study aerosol transport in the Saharan Air Layer (SAL) from Africa to the Caribbean, we combine advanced optical models of Saharan aerosols with Stokes settling and two hypotheses about the occurrence of vertical mixing. By testing our hypotheses with lidar and in situ profiles measured near the top of the transported SAL, we find strong evidence that vertical mixing occurs in the SAL over the Atlantic with significant consequences for size distribution of the transported Saharan aerosols.
Mira L. Pöhlker, Christopher Pöhlker, Florian Ditas, Thomas Klimach, Isabella Hrabe de Angelis, Alessandro Araújo, Joel Brito, Samara Carbone, Yafang Cheng, Xuguang Chi, Reiner Ditz, Sachin S. Gunthe, Jürgen Kesselmeier, Tobias Könemann, Jošt V. Lavrič, Scot T. Martin, Eugene Mikhailov, Daniel Moran-Zuloaga, Diana Rose, Jorge Saturno, Hang Su, Ryan Thalman, David Walter, Jian Wang, Stefan Wolff, Henrique M. J. Barbosa, Paulo Artaxo, Meinrat O. Andreae, and Ulrich Pöschl
Atmos. Chem. Phys., 16, 15709–15740, https://doi.org/10.5194/acp-16-15709-2016, https://doi.org/10.5194/acp-16-15709-2016, 2016
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The paper presents a systematic characterization of cloud condensation nuclei (CCN) concentration in the central Amazonian atmosphere. Our results show that the CCN population in this globally important ecosystem follows a pollution-related seasonal cycle, in which it mainly depends on changes in total aerosol size distribution and to a minor extent in the aerosol chemical composition. Our results allow an efficient modeling and prediction of the CCN population based on a novel approach.
Quentin Libois, Liviu Ivanescu, Jean-Pierre Blanchet, Hannes Schulz, Heiko Bozem, W. Richard Leaitch, Julia Burkart, Jonathan P. D. Abbatt, Andreas B. Herber, Amir A. Aliabadi, and Éric Girard
Atmos. Chem. Phys., 16, 15689–15707, https://doi.org/10.5194/acp-16-15689-2016, https://doi.org/10.5194/acp-16-15689-2016, 2016
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The first airborne measurements performed with the FIRR are presented. Vertical profiles of upwelling spectral radiance in the far-infrared are measured in the Arctic atmosphere for the first time. They show the impact of the temperature inversion on the radiative budget of the atmosphere, especially in the far-infrared. The presence of ice clouds also significantly alters the far-infrared budget, highlighting the critical interplay between water vapour and clouds in this very dry region.
Christiane Voigt, Andreas Dörnbrack, Martin Wirth, Silke M. Groß, Robert Baumann, Benedikt Ehard, Michael C. Pitts, Lamont R. Poole, Björn-Martin Sinnhuber, and Hermann Oelhaf
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-1082, https://doi.org/10.5194/acp-2016-1082, 2016
Revised manuscript not accepted
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The letter describes unprecedented observations of widespread and persistent polar stratospheric ice clouds (ice PSCs) in the exceptionally cold Arctic stratospheric winter 2015/16. The unique observations are of global relevance because trends in Arctic ozone loss and in polar temperatures are highly uncertain. The new observations at cold conditions serve to enhance our knowledge on ice PSC formation, Arctic ozone loss and polar stratrospheric temperatures in a changing climate.
Bärbel Vogel, Gebhard Günther, Rolf Müller, Jens-Uwe Grooß, Armin Afchine, Heiko Bozem, Peter Hoor, Martina Krämer, Stefan Müller, Martin Riese, Christian Rolf, Nicole Spelten, Gabriele P. Stiller, Jörn Ungermann, and Andreas Zahn
Atmos. Chem. Phys., 16, 15301–15325, https://doi.org/10.5194/acp-16-15301-2016, https://doi.org/10.5194/acp-16-15301-2016, 2016
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The identification of transport pathways from the Asian monsoon anticyclone into the lower stratosphere is unclear. Global simulations with the CLaMS model demonstrate that source regions in Asia and in the Pacific Ocean have a significant impact on the chemical composition of the lower stratosphere of the Northern Hemisphere by flooding the extratropical lower stratosphere with young moist air masses. Two main horizontal transport pathways from the Asian monsoon anticyclone are identified.
Caroline Struckmeier, Frank Drewnick, Friederike Fachinger, Gian Paolo Gobbi, and Stephan Borrmann
Atmos. Chem. Phys., 16, 15277–15299, https://doi.org/10.5194/acp-16-15277-2016, https://doi.org/10.5194/acp-16-15277-2016, 2016
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The characteristics of ambient aerosol during two seasons (spring/autumn) and at two locations (suburban/urban) in Rome were investigated. We distinguished regionally advected and locally produced organic aerosols, including from cooking, traffic and biomass burning, but also from locally emitted cigarette smoke, for which we propose a new marker peak for identification in aerosol mass spectra. The impact of Saharan dust advection events on local aerosol concentration was studied.
Carolina Cavazos Guerra, Axel Lauer, Andreas B. Herber, Tim M. Butler, Annette Rinke, and Klaus Dethloff
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-942, https://doi.org/10.5194/acp-2016-942, 2016
Revised manuscript has not been submitted
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Accurate description of the Arctic atmosphere is a challenge for the modelling comunity. We evaluate the performance of the Weather Research and Forecast model (WRF) in the Eurasian Arctic and analyse the implications of data to initialise the model and a land surface scheme. The results show that biases can be related to the quality of data used and in the case of black carbon concentrations, to emission data. More long term measurements are need for model Validation in the area.
Hanna K. Lappalainen, Veli-Matti Kerminen, Tuukka Petäjä, Theo Kurten, Aleksander Baklanov, Anatoly Shvidenko, Jaana Bäck, Timo Vihma, Pavel Alekseychik, Meinrat O. Andreae, Stephen R. Arnold, Mikhail Arshinov, Eija Asmi, Boris Belan, Leonid Bobylev, Sergey Chalov, Yafang Cheng, Natalia Chubarova, Gerrit de Leeuw, Aijun Ding, Sergey Dobrolyubov, Sergei Dubtsov, Egor Dyukarev, Nikolai Elansky, Kostas Eleftheriadis, Igor Esau, Nikolay Filatov, Mikhail Flint, Congbin Fu, Olga Glezer, Aleksander Gliko, Martin Heimann, Albert A. M. Holtslag, Urmas Hõrrak, Juha Janhunen, Sirkku Juhola, Leena Järvi, Heikki Järvinen, Anna Kanukhina, Pavel Konstantinov, Vladimir Kotlyakov, Antti-Jussi Kieloaho, Alexander S. Komarov, Joni Kujansuu, Ilmo Kukkonen, Ella-Maria Duplissy, Ari Laaksonen, Tuomas Laurila, Heikki Lihavainen, Alexander Lisitzin, Alexsander Mahura, Alexander Makshtas, Evgeny Mareev, Stephany Mazon, Dmitry Matishov, Vladimir Melnikov, Eugene Mikhailov, Dmitri Moisseev, Robert Nigmatulin, Steffen M. Noe, Anne Ojala, Mari Pihlatie, Olga Popovicheva, Jukka Pumpanen, Tatjana Regerand, Irina Repina, Aleksei Shcherbinin, Vladimir Shevchenko, Mikko Sipilä, Andrey Skorokhod, Dominick V. Spracklen, Hang Su, Dmitry A. Subetto, Junying Sun, Arkady Y. Terzhevik, Yuri Timofeyev, Yuliya Troitskaya, Veli-Pekka Tynkkynen, Viacheslav I. Kharuk, Nina Zaytseva, Jiahua Zhang, Yrjö Viisanen, Timo Vesala, Pertti Hari, Hans Christen Hansson, Gennady G. Matvienko, Nikolai S. Kasimov, Huadong Guo, Valery Bondur, Sergej Zilitinkevich, and Markku Kulmala
Atmos. Chem. Phys., 16, 14421–14461, https://doi.org/10.5194/acp-16-14421-2016, https://doi.org/10.5194/acp-16-14421-2016, 2016
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After kick off in 2012, the Pan-Eurasian Experiment (PEEX) program has expanded fast and today the multi-disciplinary research community covers ca. 80 institutes and a network of ca. 500 scientists from Europe, Russia, and China. Here we introduce scientific topics relevant in this context. This is one of the first multi-disciplinary overviews crossing scientific boundaries, from atmospheric sciences to socio-economics and social sciences.
Heike Wex, Katrin Dieckmann, Greg C. Roberts, Thomas Conrath, Miguel A. Izaguirre, Susan Hartmann, Paul Herenz, Michael Schäfer, Florian Ditas, Tina Schmeissner, Silvia Henning, Birgit Wehner, Holger Siebert, and Frank Stratmann
Atmos. Chem. Phys., 16, 14107–14130, https://doi.org/10.5194/acp-16-14107-2016, https://doi.org/10.5194/acp-16-14107-2016, 2016
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Aerosol arriving in the eastern Caribbean after passing the Atlantic is characterized, based on ground-based and airborne measurements. We describe the repetitive occurrence of three different types of air masses and relate them to their origin from either Africa or the Atlantic and also draw conclusions about the particle composition. The length of the data series is unprecedented. By a comparison with other studies, we also suggest that the organic fraction in the aerosol depends on season.
Matthew Toohey, Bjorn Stevens, Hauke Schmidt, and Claudia Timmreck
Geosci. Model Dev., 9, 4049–4070, https://doi.org/10.5194/gmd-9-4049-2016, https://doi.org/10.5194/gmd-9-4049-2016, 2016
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Stratospheric sulfate aerosols from volcanic eruptions have a significant impact on the Earth's climate. The Easy Volcanic Aerosol (EVA) volcanic forcing generator provides a tool whereby the optical properties of volcanic aerosols can be included in climate model simulations in a self-consistent, complete, and flexible manner. EVA is based on satellite observations of the 1991 Pinatubo eruption but can be applied to any real or hypothetical eruption of interest.
Sarah Grawe, Stefanie Augustin-Bauditz, Susan Hartmann, Lisa Hellner, Jan B. C. Pettersson, Andrea Prager, Frank Stratmann, and Heike Wex
Atmos. Chem. Phys., 16, 13911–13928, https://doi.org/10.5194/acp-16-13911-2016, https://doi.org/10.5194/acp-16-13911-2016, 2016
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In this study the freezing behavior of ash particles immersed in supercooled cloud droplets was investigated. It was found that ash from coal burning initiates freezing well above the limit for homogeneous ice nucleation and may contribute to cloud glaciation and precipitation formation on a regional scale. Furthermore, the experimental results were influenced by a change in sample preparation and/or particle generation which must be accounted for when comparing to previous studies.
Shi Song, K. Sebastian Schmidt, Peter Pilewskie, Michael D. King, Andrew K. Heidinger, Andi Walther, Hironobu Iwabuchi, Gala Wind, and Odele M. Coddington
Atmos. Chem. Phys., 16, 13791–13806, https://doi.org/10.5194/acp-16-13791-2016, https://doi.org/10.5194/acp-16-13791-2016, 2016
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The radiative effects of spatially complex cloud fields are notoriously difficult to estimate and are afflicted with errors up to ±50 % of the incident solar radiation. We find that horizontal photon transport, the leading cause for these three-dimensional effects, manifests itself through a spectral fingerprint – a new observable that holds promise for reducing the errors associated with spatial complexity by moving the problem to the spectral dimension.
Bernd Schalge, Jehan Rihani, Gabriele Baroni, Daniel Erdal, Gernot Geppert, Vincent Haefliger, Barbara Haese, Pablo Saavedra, Insa Neuweiler, Harrie-Jan Hendricks Franssen, Felix Ament, Sabine Attinger, Olaf A. Cirpka, Stefan Kollet, Harald Kunstmann, Harry Vereecken, and Clemens Simmer
Hydrol. Earth Syst. Sci. Discuss., https://doi.org/10.5194/hess-2016-557, https://doi.org/10.5194/hess-2016-557, 2016
Manuscript not accepted for further review
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In this work we show how we used a coupled atmosphere-land surface-subsurface model at highest possible resolution to create a testbed for data assimilation. The model was able to capture all important processes and interactions between the compartments as well as showing realistic statistical behavior. This proves that using a model as a virtual truth is possible and it will enable us to develop data assimilation methods where states and parameters are updated across compartment.
Gavin J. Phillips, Jim Thieser, Mingjin Tang, Nicolas Sobanski, Gerhard Schuster, Johannes Fachinger, Frank Drewnick, Stephan Borrmann, Heinz Bingemer, Jos Lelieveld, and John N. Crowley
Atmos. Chem. Phys., 16, 13231–13249, https://doi.org/10.5194/acp-16-13231-2016, https://doi.org/10.5194/acp-16-13231-2016, 2016
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We use trace gas measurements (N2O5, ClNO2, NO3) and particle properties (surface area, nitrate content etc.) to derive uptake coefficients (the probability of removal from the gas-phase on a per-collision basis) for the interaction of N2O5 with ambient aerosol and also the efficiency of formation of ClNO2. The uptake coefficients show high variability but are reasonably well captured by parameterisations based on laboratory measurements.
Manuel Gutleben, Silke Gross, Martin Wirth, and Andreas Schäfler
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2016-333, https://doi.org/10.5194/amt-2016-333, 2016
Revised manuscript not accepted
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Shallow marine cumulus convection over the Atlantic ocean is studied with observations by airborne and spaceborne lidar instruments. Cloud top height as well as cloud length and cloud gap length distributions are calculated by use of a newly developed algorithm. The distribution of cloud top heights during wintertime measurements shows a two-layer structure. However, significant differences in cloud top height distributions compared to summertime measurements are found.
Hang Su, Yafang Cheng, Nan Ma, Zhibin Wang, Xiaoxiang Wang, Mira L. Pöhlker, Björn Nillius, Alfred Wiedensohler, and Ulrich Pöschl
Atmos. Meas. Tech., 9, 5183–5192, https://doi.org/10.5194/amt-9-5183-2016, https://doi.org/10.5194/amt-9-5183-2016, 2016
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In cloud condensation nuclei (CCN) measurements, the supersaturation scan is often time-consuming and limits the temporal resolution of CCN measurements. Here we present a new concept, termed the broad supersaturation scanning (BS2) method, in which a range of supersaturation is simultaneously scanned, resulting in fast measurements of CCN activity.
Ralf Weigel, Peter Spichtinger, Christoph Mahnke, Marcus Klingebiel, Armin Afchine, Andreas Petzold, Martina Krämer, Anja Costa, Sergej Molleker, Philipp Reutter, Miklós Szakáll, Max Port, Lucas Grulich, Tina Jurkat, Andreas Minikin, and Stephan Borrmann
Atmos. Meas. Tech., 9, 5135–5162, https://doi.org/10.5194/amt-9-5135-2016, https://doi.org/10.5194/amt-9-5135-2016, 2016
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The subject of our study concerns measurements with optical array probes (OAPs) on fast-flying aircraft such as the G550 (HALO or HIAPER). At up to Mach 0.7 the effect of air compression upstream of underwing-mounted instruments and particles' inertia need consideration for determining ambient particle concentrations. Compared to conventional practices the introduced correction procedure eliminates ambiguities and exhibits consistency over flight speeds between 50 and 250 m s−.
Norman T. O'Neill, Konstantin Baibakov, Sareh Hesaraki, Liviu Ivanescu, Randall V. Martin, Chris Perro, Jai P. Chaubey, Andreas Herber, and Thomas J. Duck
Atmos. Chem. Phys., 16, 12753–12765, https://doi.org/10.5194/acp-16-12753-2016, https://doi.org/10.5194/acp-16-12753-2016, 2016
Luca Ferrero, David Cappelletti, Maurizio Busetto, Mauro Mazzola, Angelo Lupi, Christian Lanconelli, Silvia Becagli, Rita Traversi, Laura Caiazzo, Fabio Giardi, Beatrice Moroni, Stefano Crocchianti, Martin Fierz, Griša Močnik, Giorgia Sangiorgi, Maria G. Perrone, Marion Maturilli, Vito Vitale, Roberto Udisti, and Ezio Bolzacchini
Atmos. Chem. Phys., 16, 12601–12629, https://doi.org/10.5194/acp-16-12601-2016, https://doi.org/10.5194/acp-16-12601-2016, 2016
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This study reports results from systematic vertical aerosol profiles measured in the Arctic using a tethered balloon platform. The collected data allowed for finding common rules of aerosol behavior along height and seasons. Transport events, secondary aerosol formation and ship impact are examples of the issues investigated along height. The importance of these issues is related to their climatic implications in reference to the aerosol direct and indirect effects in the Arctic atmosphere.
Ying Chen, Yafang Cheng, Nan Ma, Ralf Wolke, Stephan Nordmann, Stephanie Schüttauf, Liang Ran, Birgit Wehner, Wolfram Birmili, Hugo A. C. Denier van der Gon, Qing Mu, Stefan Barthel, Gerald Spindler, Bastian Stieger, Konrad Müller, Guang-Jie Zheng, Ulrich Pöschl, Hang Su, and Alfred Wiedensohler
Atmos. Chem. Phys., 16, 12081–12097, https://doi.org/10.5194/acp-16-12081-2016, https://doi.org/10.5194/acp-16-12081-2016, 2016
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Sea salt aerosol (SSA) is important for primary and secondary aerosols on a global scale. During 10–20 September 2013, the SSA mass concentration was overestimated by a factor of 8–20 over central Europe by WRF-Chem model, stem from the uncertainty of its emission scheme. This could facilitate the coarse-mode nitrate formation (~ 140 % but inhibit the fine-mode nitrate formation (~−20 %). A special long-range transport mechanism could broaden this influence of SSA to a larger downwind region.
Robert Pincus, Piers M. Forster, and Bjorn Stevens
Geosci. Model Dev., 9, 3447–3460, https://doi.org/10.5194/gmd-9-3447-2016, https://doi.org/10.5194/gmd-9-3447-2016, 2016
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This paper describes an experimental protocol to understand the changes in energy balance (the "radiative forcing") that arise due to changes in atmospheric composition and why this value is not the same across climate models. The protocol includes a way to determine the total forcing to which each model is subjected, experiments designed at teasing out why certain errors occur, and experiments to identify any robust signals caused by atmospheric particles from human activities.
Valery Shcherbakov, Olivier Jourdan, Christiane Voigt, Jean-Francois Gayet, Aurélien Chauvigne, Alfons Schwarzenboeck, Andreas Minikin, Marcus Klingebiel, Ralf Weigel, Stephan Borrmann, Tina Jurkat, Stefan Kaufmann, Romy Schlage, Christophe Gourbeyre, Guy Febvre, Tatyana Lapyonok, Wiebke Frey, Sergej Molleker, and Bernadett Weinzierl
Atmos. Chem. Phys., 16, 11883–11897, https://doi.org/10.5194/acp-16-11883-2016, https://doi.org/10.5194/acp-16-11883-2016, 2016
Tobias Zinner, Petra Hausmann, Florian Ewald, Luca Bugliaro, Claudia Emde, and Bernhard Mayer
Atmos. Meas. Tech., 9, 4615–4632, https://doi.org/10.5194/amt-9-4615-2016, https://doi.org/10.5194/amt-9-4615-2016, 2016
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A new retrieval of optical thickness and effective particle size of ice clouds over a wide range of optical thickness from transmittance measurements is presented. A visible range spectral slope is used to resolve the transmittance optical thickness ambiguity. Retrieval sensitivity to ice crystal habit, aerosol, albedo, sensor accuracy and lookup table interpolation is presented as well as an application of the method and comparison to satellite products for 2 days.
Silke Groß, Josef Gasteiger, Volker Freudenthaler, Thomas Müller, Daniel Sauer, Carlos Toledano, and Albert Ansmann
Atmos. Chem. Phys., 16, 11535–11546, https://doi.org/10.5194/acp-16-11535-2016, https://doi.org/10.5194/acp-16-11535-2016, 2016
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Dual-wavelength depolarization sensitive Raman lidar measurements were used to characterize the optical properties of the dust loaded convective boundary layer over the Caribbean. Furthermore we derived the dust volume fraction and dust mass concentration within the convective boundary layer.
W. Richard Leaitch, Alexei Korolev, Amir A. Aliabadi, Julia Burkart, Megan D. Willis, Jonathan P. D. Abbatt, Heiko Bozem, Peter Hoor, Franziska Köllner, Johannes Schneider, Andreas Herber, Christian Konrad, and Ralf Brauner
Atmos. Chem. Phys., 16, 11107–11124, https://doi.org/10.5194/acp-16-11107-2016, https://doi.org/10.5194/acp-16-11107-2016, 2016
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Thought to be mostly unimportant for summertime Arctic liquid-water clouds, airborne observations show that atmospheric aerosol particles 50 nm in diameter or smaller and most likely from natural sources are often involved in cloud formation in the pristine Arctic summer. The result expands the reference for aerosol forcing of climate. Further, for extremely low droplet concentrations, no evidence is found for a connection between cloud liquid water and aerosol particle concentrations.
Stefan Müller, Peter Hoor, Heiko Bozem, Ellen Gute, Bärbel Vogel, Andreas Zahn, Harald Bönisch, Timo Keber, Martina Krämer, Christian Rolf, Martin Riese, Hans Schlager, and Andreas Engel
Atmos. Chem. Phys., 16, 10573–10589, https://doi.org/10.5194/acp-16-10573-2016, https://doi.org/10.5194/acp-16-10573-2016, 2016
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In situ airborne measurements performed during TACTS/ESMVal 2012 were analysed to investigate the chemical compostion of the upper troposphere and lower stratosphere. N2O, CO and O3 data show an increase in tropospherically affected air masses within the extratropical stratosphere from August to September 2012, which originate from the Asian monsoon region. Thus, the Asian monsoon anticyclone significantly affected the chemical composition of the extratropical stratosphere during summer 2012.
María Barrera-Verdejo, Susanne Crewell, Ulrich Löhnert, Emiliano Orlandi, and Paolo Di Girolamo
Atmos. Meas. Tech., 9, 4013–4028, https://doi.org/10.5194/amt-9-4013-2016, https://doi.org/10.5194/amt-9-4013-2016, 2016
Wolfgang Woiwode, Michael Höpfner, Lei Bi, Michael C. Pitts, Lamont R. Poole, Hermann Oelhaf, Sergej Molleker, Stephan Borrmann, Marcus Klingebiel, Gennady Belyaev, Andreas Ebersoldt, Sabine Griessbach, Jens-Uwe Grooß, Thomas Gulde, Martina Krämer, Guido Maucher, Christof Piesch, Christian Rolf, Christian Sartorius, Reinhold Spang, and Johannes Orphal
Atmos. Chem. Phys., 16, 9505–9532, https://doi.org/10.5194/acp-16-9505-2016, https://doi.org/10.5194/acp-16-9505-2016, 2016
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The analysis of spectral signatures of a polar stratospheric cloud in airborne infrared remote sensing observations in the Arctic in combination with further collocated measurements supports the view that the observed cloud consisted of highly aspherical nitric acid trihydrate particles. A characteristic "shoulder-like" spectral signature may be exploited for identification of large, highly aspherical nitric acid trihydrate particles involved in denitrification of the polar winter stratosphere.
Alexander Lemburg, Martin Claussen, and Felix Ament
Clim. Past Discuss., https://doi.org/10.5194/cp-2016-68, https://doi.org/10.5194/cp-2016-68, 2016
Manuscript not accepted for further review
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The deforestation of Easter Island several hundred years ago might have influenced its local near-surface climate. With a series of numerical model experiments we investigate the impact of deforestation on precipitation and near-surface climate. We find that a deforested Easter Island appears to be significantly less resistant to drought than a forested island and thus, deforestation has probably exacerbated the effects of past climate drought spells on Easter Island's socio-ecological systems.
Martin Ebert, Ralf Weigel, Konrad Kandler, Gebhard Günther, Sergej Molleker, Jens-Uwe Grooß, Bärbel Vogel, Stephan Weinbruch, and Stephan Borrmann
Atmos. Chem. Phys., 16, 8405–8421, https://doi.org/10.5194/acp-16-8405-2016, https://doi.org/10.5194/acp-16-8405-2016, 2016
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Stratospheric aerosol particles were collected within the arctic vortex in late winter. The chemical composition of refractory particles were analyzed by scanning electron microscopy. More than 750 refractory particles with diameters above 500 nm were found consisting of silicates, Fe- and Ca-rich particles and metal mixtures. The detection of refractory particles in the late winter polar stratosphere has strong implications for the formation of polar stratospheric clouds and ozone depletion.
Natalia Babkovskaia, Ullar Rannik, Vaughan Phillips, Holger Siebert, Birgit Wehner, and Michael Boy
Atmos. Chem. Phys., 16, 7889–7898, https://doi.org/10.5194/acp-16-7889-2016, https://doi.org/10.5194/acp-16-7889-2016, 2016
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Turbulence, aerosol growth and microphysics of hydrometeors in clouds are intimately coupled. A new modelling approach was applied to quantify this linkage. We study the interaction in the cloud area under transient, high supersaturation conditions, using direct numerical simulations. Analysing the effect of aerosol dynamics on the turbulent kinetic energy and on vertical velocity, we conclude that the presence of aerosol has an effect on vertical motion and tends to reduce downward velocity.
Amir A. Aliabadi, Jennie L. Thomas, Andreas B. Herber, Ralf M. Staebler, W. Richard Leaitch, Hannes Schulz, Kathy S. Law, Louis Marelle, Julia Burkart, Megan D. Willis, Heiko Bozem, Peter M. Hoor, Franziska Köllner, Johannes Schneider, Maurice Levasseur, and Jonathan P. D. Abbatt
Atmos. Chem. Phys., 16, 7899–7916, https://doi.org/10.5194/acp-16-7899-2016, https://doi.org/10.5194/acp-16-7899-2016, 2016
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For the first time, ship emissions of an ice-breaker, the Amundsen, is characterized while breaking ice in the Canadian Arctic using the plume intercepts by the Polar 6 aircraft. The study is novel, estimating lower plume expansion rates over the stable Arctic marine boundary layer and different emissions factors for oxides of nitrogen, black carbon, and carbon monoxide, compared to plume intercept studies in mid latitudes. These results can inform policy making and emission inventory datasets.
Fanny Finger, Frank Werner, Marcus Klingebiel, André Ehrlich, Evelyn Jäkel, Matthias Voigt, Stephan Borrmann, Peter Spichtinger, and Manfred Wendisch
Atmos. Chem. Phys., 16, 7681–7693, https://doi.org/10.5194/acp-16-7681-2016, https://doi.org/10.5194/acp-16-7681-2016, 2016
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Solar spectra of optical layer properties of cirrus have been derived from the first truly collocated airborne radiation measurements using an aircraft and a towed sensor platform. The measured layer properties differ slightly due to horizontal cirrus inhomogeneities and the influence of low-level water clouds. Applying a 1-D radiative transfer model sensitivity studies were performed. It was found that if a low-level cloud is not considered, the solar cooling of the cirrus is strongly overestimated.
Megan D. Willis, Julia Burkart, Jennie L. Thomas, Franziska Köllner, Johannes Schneider, Heiko Bozem, Peter M. Hoor, Amir A. Aliabadi, Hannes Schulz, Andreas B. Herber, W. Richard Leaitch, and Jonathan P. D. Abbatt
Atmos. Chem. Phys., 16, 7663–7679, https://doi.org/10.5194/acp-16-7663-2016, https://doi.org/10.5194/acp-16-7663-2016, 2016
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We present a case study focused on an aerosol growth event observed in the Canadian High Arctic during summer. Using measurements of aerosol chemical and physical properties we find evidence for aerosol growth into cloud condensation nuclei-active sizes, through marine-influenced secondary organic aerosol formation. Understanding the mechanisms that control the formation and growth of aerosol is crucial for our ability to predict cloud properties, and therefore radiative balance and climate.
Veronika Eyring, Sandrine Bony, Gerald A. Meehl, Catherine A. Senior, Bjorn Stevens, Ronald J. Stouffer, and Karl E. Taylor
Geosci. Model Dev., 9, 1937–1958, https://doi.org/10.5194/gmd-9-1937-2016, https://doi.org/10.5194/gmd-9-1937-2016, 2016
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The objective of CMIP is to better understand past, present, and future climate change in a multi-model context. CMIP's increasing importance and scope is a tremendous success story, but the need to address an ever-expanding range of scientific questions arising from more and more research communities has made it necessary to revise the organization of CMIP. In response to these challenges, we have adopted a more federated structure for the sixth phase of CMIP (i.e. CMIP6) and subsequent phases.
Florian Berkes, Peter Hoor, Heiko Bozem, Daniel Kunkel, Michael Sprenger, and Stephan Henne
Atmos. Chem. Phys., 16, 6011–6025, https://doi.org/10.5194/acp-16-6011-2016, https://doi.org/10.5194/acp-16-6011-2016, 2016
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We presented airborne measurements of CO2 and O3 across the entrainment zone over a semi-remote environment in southwestern Germany in late summer 2011 .
For the first time CO2 and O3 were used as tracer to identify mixing through this transport barrier. We demonstrated that the tracer--tracer correlation of CO2 and O3 is a powerful tool to identify entrainment and mixing.
Anna E. Luebke, Armin Afchine, Anja Costa, Jens-Uwe Grooß, Jessica Meyer, Christian Rolf, Nicole Spelten, Linnea M. Avallone, Darrel Baumgardner, and Martina Krämer
Atmos. Chem. Phys., 16, 5793–5809, https://doi.org/10.5194/acp-16-5793-2016, https://doi.org/10.5194/acp-16-5793-2016, 2016
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In this study, we present observational evidence to show that two distinct types of cirrus clouds exist – in situ origin and liquid origin cirrus. These two types differ by their formation mechanism and other properties. Airborne, in-cloud measurements of cloud ice water content (IWC), ice crystal concentration (Nice), and ice crystal size from the 2014 ML-CIRRUS campaign provide cloud samples that have been divided and analyzed according to their origin type.
Florian Ewald, Tobias Kölling, Andreas Baumgartner, Tobias Zinner, and Bernhard Mayer
Atmos. Meas. Tech., 9, 2015–2042, https://doi.org/10.5194/amt-9-2015-2016, https://doi.org/10.5194/amt-9-2015-2016, 2016
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The new spectrometer of the Munich Aerosol Cloud Scanner (specMACS) is a
multipurpose hyperspectral cloud and sky imager which is designated, but not limited, to investigations of cloud-aerosol interactions in Earth's atmosphere. This paper describes the specMACS instrument's hardware and software design and
characterizes the instrument performance. Initial measurements of cloud sides are presented which demonstrate the wide applicability of the instrument.
Stefanie Augustin-Bauditz, Heike Wex, Cyrielle Denjean, Susan Hartmann, Johannes Schneider, Susann Schmidt, Martin Ebert, and Frank Stratmann
Atmos. Chem. Phys., 16, 5531–5543, https://doi.org/10.5194/acp-16-5531-2016, https://doi.org/10.5194/acp-16-5531-2016, 2016
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In this study, we mixed a pure mineral dust sample with ice active biological material and quantified the immersion freezing behavior of the resulting particles utilizing the Leipzig Aerosol Cloud Interaction Simulator (LACIS). Furthermore, we used different methods to investigate the mixing state of our generated aerosol.
We found that internally mixed particles, containing ice active biological material, follow the ice nucleation behavior observed for the pure biological particles.
Tina Jurkat, Stefan Kaufmann, Christiane Voigt, Dominik Schäuble, Philipp Jeßberger, and Helmut Ziereis
Atmos. Meas. Tech., 9, 1907–1923, https://doi.org/10.5194/amt-9-1907-2016, https://doi.org/10.5194/amt-9-1907-2016, 2016
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The paper details novel mass spectrometric measurements with AIMS-TG aboard the new German research aircraft HALO. The measurements comprise a wide range of tracers with characteristic source regions. Using these tracers, stratospheric and tropospheric air in the UTLS is tagged. The instrument is equipped with a new discharge ionization source, an in-flight calibration and improved transmission of adhesive gases like HNO3 and HCl. AIMS was built to characterize transport and mixing in the UTLS.
Martin Schnaiter, Emma Järvinen, Paul Vochezer, Ahmed Abdelmonem, Robert Wagner, Olivier Jourdan, Guillaume Mioche, Valery N. Shcherbakov, Carl G. Schmitt, Ugo Tricoli, Zbigniew Ulanowski, and Andrew J. Heymsfield
Atmos. Chem. Phys., 16, 5091–5110, https://doi.org/10.5194/acp-16-5091-2016, https://doi.org/10.5194/acp-16-5091-2016, 2016
Marion Maturilli and Christoph Ritter
Earth Syst. Sci. Data, 8, 159–164, https://doi.org/10.5194/essd-8-159-2016, https://doi.org/10.5194/essd-8-159-2016, 2016
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The total solar eclipse over Ny-Ålesund (78.9° N, 11.9° E), Svalbard, on 20 March 2015 has been followed by various sensors. Here, we present the surface radiation measurements in the context of the meteorological observations, providing basic data for further studies on e.g. radiative transfer or micrometeorology.
S. T. Martin, P. Artaxo, L. A. T. Machado, A. O. Manzi, R. A. F. Souza, C. Schumacher, J. Wang, M. O. Andreae, H. M. J. Barbosa, J. Fan, G. Fisch, A. H. Goldstein, A. Guenther, J. L. Jimenez, U. Pöschl, M. A. Silva Dias, J. N. Smith, and M. Wendisch
Atmos. Chem. Phys., 16, 4785–4797, https://doi.org/10.5194/acp-16-4785-2016, https://doi.org/10.5194/acp-16-4785-2016, 2016
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The Observations and Modeling of the Green Ocean Amazon (GoAmazon2014/5) Experiment took place in central Amazonia throughout 2014 and 2015. The experiment focused on the complex links among vegetation, atmospheric chemistry, and aerosol production on the one hand and their connections to aerosols, clouds, and precipitation on the other, especially when altered by urban pollution. This article serves as an introduction to the special issue of publications presenting findings of this experiment.
Fabian Jakub and Bernhard Mayer
Geosci. Model Dev., 9, 1413–1422, https://doi.org/10.5194/gmd-9-1413-2016, https://doi.org/10.5194/gmd-9-1413-2016, 2016
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Radiative heating or cooling plays a vital role in the evolution and lifecycle of clouds. Due to the immense computational cost of 3-D radiative transfer, today's atmospheric models usually employ crude 1-D approximations which neglect any horizontal energy transport whatsoever and may introduce non-negligible errors. This paper documents the implementation and runtime characteristics of the new TenStream solver that enables us to study 3-D effects on large domains and extended periods of time.
Martina Krämer, Christian Rolf, Anna Luebke, Armin Afchine, Nicole Spelten, Anja Costa, Jessica Meyer, Martin Zöger, Jessica Smith, Robert L. Herman, Bernhard Buchholz, Volker Ebert, Darrel Baumgardner, Stephan Borrmann, Marcus Klingebiel, and Linnea Avallone
Atmos. Chem. Phys., 16, 3463–3483, https://doi.org/10.5194/acp-16-3463-2016, https://doi.org/10.5194/acp-16-3463-2016, 2016
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A guide to cirrus clouds is compiled from extensive model simulations and aircraft observations. Two types of cirrus are found: rather thin in situ cirrus that form directly as ice and thicker liquid origin cirrus consisting of uplifted frozen liquid drops. Over Europe, thinner in situ and liquid origin cirrus occur often together with frontal systems, while over the US and the Tropics, thick liquid origin cirrus formed in large convective systems are detected more frequently.
Dominik van Pinxteren, Khanneh Wadinga Fomba, Stephan Mertes, Konrad Müller, Gerald Spindler, Johannes Schneider, Taehyoung Lee, Jeffrey L. Collett, and Hartmut Herrmann
Atmos. Chem. Phys., 16, 3185–3205, https://doi.org/10.5194/acp-16-3185-2016, https://doi.org/10.5194/acp-16-3185-2016, 2016
Ulla Wandinger, Volker Freudenthaler, Holger Baars, Aldo Amodeo, Ronny Engelmann, Ina Mattis, Silke Groß, Gelsomina Pappalardo, Aldo Giunta, Giuseppe D'Amico, Anatoli Chaikovsky, Fiodor Osipenko, Alexander Slesar, Doina Nicolae, Livio Belegante, Camelia Talianu, Ilya Serikov, Holger Linné, Friedhelm Jansen, Arnoud Apituley, Keith M. Wilson, Martin de Graaf, Thomas Trickl, Helmut Giehl, Mariana Adam, Adolfo Comerón, Constantino Muñoz-Porcar, Francesc Rocadenbosch, Michaël Sicard, Sergio Tomás, Diego Lange, Dhiraj Kumar, Manuel Pujadas, Francisco Molero, Alfonso J. Fernández, Lucas Alados-Arboledas, Juan Antonio Bravo-Aranda, Francisco Navas-Guzmán, Juan Luis Guerrero-Rascado, María José Granados-Muñoz, Jana Preißler, Frank Wagner, Michael Gausa, Ivan Grigorov, Dimitar Stoyanov, Marco Iarlori, Vincenco Rizi, Nicola Spinelli, Antonella Boselli, Xuan Wang, Teresa Lo Feudo, Maria Rita Perrone, Ferdinando De Tomasi, and Pasquale Burlizzi
Atmos. Meas. Tech., 9, 1001–1023, https://doi.org/10.5194/amt-9-1001-2016, https://doi.org/10.5194/amt-9-1001-2016, 2016
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We introduce the quality-assurance efforts of the European Aerosol Research Lidar Network (EARLINET) at instrument level. Within several campaigns, 21 EARLINET systems from 18 EARLINET stations were intercompared. A comprehensive strategy for campaign setup and data evaluation was established. The intercomparisons have reinforced our confidence in the EARLINET data quality and allowed us to draw conclusions on necessary system improvements and to identify major challenges for our future work.
T. Krumpen, R. Gerdes, C. Haas, S. Hendricks, A. Herber, V. Selyuzhenok, L. Smedsrud, and G. Spreen
The Cryosphere, 10, 523–534, https://doi.org/10.5194/tc-10-523-2016, https://doi.org/10.5194/tc-10-523-2016, 2016
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We present an extensive data set of ground-based and airborne electromagnetic ice thickness measurements covering Fram Strait in summer between 2001 and 2012. An investigation of back trajectories of surveyed sea ice using satellite-based sea ice motion data allows us to examine the connection between thickness variability, ice age and source area. In addition, we determine across and along strait gradients in ice thickness and associated volume fluxes.
Stefan Kaufmann, Christiane Voigt, Tina Jurkat, Troy Thornberry, David W. Fahey, Ru-Shan Gao, Romy Schlage, Dominik Schäuble, and Martin Zöger
Atmos. Meas. Tech., 9, 939–953, https://doi.org/10.5194/amt-9-939-2016, https://doi.org/10.5194/amt-9-939-2016, 2016
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We present the development of a new airborne mass spectrometer AIMS-H2O for the fast and accurate measurement of water vapor in the upper troposphere and lower stratosphere. The high accuracy needed for e.g. quantification of atmospheric water vapor transport processes or cloud formation is achieved by an in-flight calibration of the instrument. AIMS-H2O is deployed on the DLR research aircraft HALO and Falcon where it covers a range of water vapor mixing ratios from 1 to 500 ppmv.
Ying Chen, Ya-Fang Cheng, Stephan Nordmann, Wolfram Birmili, Hugo A. C. Denier van der Gon, Nan Ma, Ralf Wolke, Birgit Wehner, Jia Sun, Gerald Spindler, Qing Mu, Ulrich Pöschl, Hang Su, and Alfred Wiedensohler
Atmos. Chem. Phys., 16, 1823–1835, https://doi.org/10.5194/acp-16-1823-2016, https://doi.org/10.5194/acp-16-1823-2016, 2016
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We evaluated the EC point sources in Germany with high-resolution simulation by WRF-Chem, and find out that point sources contribute too much EC in the coarse mode aerosol mass. The area emissions in Eastern Europe and Russia also allocate too much EC emission in coarse mode in the EUCAARI EC emission inventory. Because of the shorter life time of coarse mode EC, about 20–40 % less EC can be transported to Melpitz from Eastern Europe. Size segregation information is important for EC inventories.
P. Hari, T. Petäjä, J. Bäck, V.-M. Kerminen, H. K. Lappalainen, T. Vihma, T. Laurila, Y. Viisanen, T. Vesala, and M. Kulmala
Atmos. Chem. Phys., 16, 1017–1028, https://doi.org/10.5194/acp-16-1017-2016, https://doi.org/10.5194/acp-16-1017-2016, 2016
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This manuscript introduces a conceptual design of a global, hierarchical observation network which provides tools and increased understanding to tackle the inter-connected environmental and societal challenges that we will face in the coming decades. Each ecosystem type on the globe has its own characteristic features that need to be taken into consideration. The hierarchical network is able to tackle problems related to large spatial scales, heterogeneity of ecosystems and their complexity.
A. Spolaor, T. Opel, J. R. McConnell, O. J. Maselli, G. Spreen, C. Varin, T. Kirchgeorg, D. Fritzsche, A. Saiz-Lopez, and P. Vallelonga
The Cryosphere, 10, 245–256, https://doi.org/10.5194/tc-10-245-2016, https://doi.org/10.5194/tc-10-245-2016, 2016
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The role of sea ice in the Earth climate system is still under debate, although it is known to influence albedo, ocean circulation, and atmosphere-ocean heat and gas exchange. Here we present a reconstruction of 1950 to 1998 AD sea ice in the Laptev Sea based on the Akademii Nauk ice core (Severnaya Zemlya, Russian Arctic) and halogen measurements. The results suggest a connection between bromine and sea ice, as well as a connection between iodine concentration in snow and summer sea ice.
A. Roth, J. Schneider, T. Klimach, S. Mertes, D. van Pinxteren, H. Herrmann, and S. Borrmann
Atmos. Chem. Phys., 16, 505–524, https://doi.org/10.5194/acp-16-505-2016, https://doi.org/10.5194/acp-16-505-2016, 2016
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This paper reports on single-particle measurements of ambient aerosol particles and cloud residues sampled from orographic clouds on a mountain site in central Germany.
The results show that soot particles can get efficiently activated in cloud droplets when they are mixed with or coated by sulfate and nitrate. Cloud processing leads to addition of nitrate and sulfate to the particles, thereby increasing the hygroscopicity of these particles when they remain in the air after cloud evaporation.
R. Pirazzini, P. Räisänen, T. Vihma, M. Johansson, and E.-M. Tastula
The Cryosphere, 9, 2357–2381, https://doi.org/10.5194/tc-9-2357-2015, https://doi.org/10.5194/tc-9-2357-2015, 2015
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We illustrate a method to measure the size distribution of a snow particle metric from macro photos of snow particles. This snow particle metric corresponds well to the optically equivalent effective radius. Our results evidence the impact of grain shape on albedo, indicate that more than just one particle metric distribution is needed to characterize the snow scattering properties at all optical wavelengths, and suggest an impact of surface roughness on the shortwave infrared albedo.
E. Jäkel, B. Mey, R. Levy, X. Gu, T. Yu, Z. Li, D. Althausen, B. Heese, and M. Wendisch
Atmos. Meas. Tech., 8, 5237–5249, https://doi.org/10.5194/amt-8-5237-2015, https://doi.org/10.5194/amt-8-5237-2015, 2015
Z. Jurányi, H. Burtscher, M. Loepfe, M. Nenkov, and E. Weingartner
Atmos. Meas. Tech., 8, 5213–5222, https://doi.org/10.5194/amt-8-5213-2015, https://doi.org/10.5194/amt-8-5213-2015, 2015
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Volcanic eruption can be a serious security risk for airplanes. We develop a new aerosol sensor for the reliable detection of volcanic ash on airplanes. We introduce here the laboratory prototype of this instrument, which is able to distinguish between water droplets and volcanic ash particles by measuring the scattered light at two distinct wavelengths simultaneously. The different optical behaviour of volcanic ash and water at these wavelengths makes this differentiation possible.
A. Lammert and F. Ament
Earth Syst. Sci. Data, 7, 311–317, https://doi.org/10.5194/essd-7-311-2015, https://doi.org/10.5194/essd-7-311-2015, 2015
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The paper presents long-term measurements of turbulent fluxes at the research platform FINO2 in the Baltic Sea. The platform was equipped at two heights (6.8 and 13.8m) for the observation of wind, temperature, humidity and CO2 over a time period of 1.5 years. The paper shows the measured quantities as well as the turbulent fluxes, latent and sensible heat, momentum and CO2 flux. In contrast to the constant-flux layer approach, we found differences in the CO2 fluxes between 6.8 and 13.8m.
M. Paramonov, V.-M. Kerminen, M. Gysel, P. P. Aalto, M. O. Andreae, E. Asmi, U. Baltensperger, A. Bougiatioti, D. Brus, G. P. Frank, N. Good, S. S. Gunthe, L. Hao, M. Irwin, A. Jaatinen, Z. Jurányi, S. M. King, A. Kortelainen, A. Kristensson, H. Lihavainen, M. Kulmala, U. Lohmann, S. T. Martin, G. McFiggans, N. Mihalopoulos, A. Nenes, C. D. O'Dowd, J. Ovadnevaite, T. Petäjä, U. Pöschl, G. C. Roberts, D. Rose, B. Svenningsson, E. Swietlicki, E. Weingartner, J. Whitehead, A. Wiedensohler, C. Wittbom, and B. Sierau
Atmos. Chem. Phys., 15, 12211–12229, https://doi.org/10.5194/acp-15-12211-2015, https://doi.org/10.5194/acp-15-12211-2015, 2015
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The research paper presents the first comprehensive overview of field measurements with the CCN Counter performed at a large number of locations around the world within the EUCAARI framework. The paper sheds light on the CCN number concentrations and activated fractions around the world and their dependence on the water vapour supersaturation ratio, the dependence of aerosol hygroscopicity on particle size, and seasonal and diurnal variation of CCN activation and hygroscopic properties.
B. Wehner, F. Werner, F. Ditas, R. A. Shaw, M. Kulmala, and H. Siebert
Atmos. Chem. Phys., 15, 11701–11711, https://doi.org/10.5194/acp-15-11701-2015, https://doi.org/10.5194/acp-15-11701-2015, 2015
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During the CARRIBA campaign on Barbados, 91 cases with increased aerosol particle number concentrations near clouds were detected from helicopter-borne measurements. Most of these cases are correlated with enhanced irradiance in the ultraviolet range. The events have a mean length of 100m, corresponding to a lifetime of 300s, meaning a growth of several nm/h. Such high values cannot be explained by sulfuric acid alone; thus extremely low volatility organic compounds are probably involved here.
S. Groß, V. Freudenthaler, K. Schepanski, C. Toledano, A. Schäfler, A. Ansmann, and B. Weinzierl
Atmos. Chem. Phys., 15, 11067–11080, https://doi.org/10.5194/acp-15-11067-2015, https://doi.org/10.5194/acp-15-11067-2015, 2015
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In June and July 2013 dual-wavelength lidar measurements were performed in Barbados to study long-range transported Saharan dust across the Atlantic Ocean and investigate transport-induced changes. The focus of our measurements is the intensive optical properties, the lidar ratio and the particle linear depolarization ratio. While the lidar ratio shows no differences compared to the values of fresh Saharan dust, the particle linear depolarization ratio shows slight differences.
M. O. Andreae, O. C. Acevedo, A. Araùjo, P. Artaxo, C. G. G. Barbosa, H. M. J. Barbosa, J. Brito, S. Carbone, X. Chi, B. B. L. Cintra, N. F. da Silva, N. L. Dias, C. Q. Dias-Júnior, F. Ditas, R. Ditz, A. F. L. Godoi, R. H. M. Godoi, M. Heimann, T. Hoffmann, J. Kesselmeier, T. Könemann, M. L. Krüger, J. V. Lavric, A. O. Manzi, A. P. Lopes, D. L. Martins, E. F. Mikhailov, D. Moran-Zuloaga, B. W. Nelson, A. C. Nölscher, D. Santos Nogueira, M. T. F. Piedade, C. Pöhlker, U. Pöschl, C. A. Quesada, L. V. Rizzo, C.-U. Ro, N. Ruckteschler, L. D. A. Sá, M. de Oliveira Sá, C. B. Sales, R. M. N. dos Santos, J. Saturno, J. Schöngart, M. Sörgel, C. M. de Souza, R. A. F. de Souza, H. Su, N. Targhetta, J. Tóta, I. Trebs, S. Trumbore, A. van Eijck, D. Walter, Z. Wang, B. Weber, J. Williams, J. Winderlich, F. Wittmann, S. Wolff, and A. M. Yáñez-Serrano
Atmos. Chem. Phys., 15, 10723–10776, https://doi.org/10.5194/acp-15-10723-2015, https://doi.org/10.5194/acp-15-10723-2015, 2015
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This paper describes the Amazon Tall Tower Observatory (ATTO), a new atmosphere-biosphere observatory located in the remote Amazon Basin. It presents results from ecosystem ecology, meteorology, trace gas, and aerosol measurements collected at the ATTO site during the first 3 years of operation.
K. Baibakov, N. T. O'Neill, L. Ivanescu, T. J. Duck, C. Perro, A. Herber, K.-H. Schulz, and O. Schrems
Atmos. Meas. Tech., 8, 3789–3809, https://doi.org/10.5194/amt-8-3789-2015, https://doi.org/10.5194/amt-8-3789-2015, 2015
F. Drewnick, J.-M. Diesch, P. Faber, and S. Borrmann
Atmos. Meas. Tech., 8, 3811–3830, https://doi.org/10.5194/amt-8-3811-2015, https://doi.org/10.5194/amt-8-3811-2015, 2015
A. Ehrlich and M. Wendisch
Atmos. Meas. Tech., 8, 3671–3684, https://doi.org/10.5194/amt-8-3671-2015, https://doi.org/10.5194/amt-8-3671-2015, 2015
M. Beekmann, A. S. H. Prévôt, F. Drewnick, J. Sciare, S. N. Pandis, H. A. C. Denier van der Gon, M. Crippa, F. Freutel, L. Poulain, V. Ghersi, E. Rodriguez, S. Beirle, P. Zotter, S.-L. von der Weiden-Reinmüller, M. Bressi, C. Fountoukis, H. Petetin, S. Szidat, J. Schneider, A. Rosso, I. El Haddad, A. Megaritis, Q. J. Zhang, V. Michoud, J. G. Slowik, S. Moukhtar, P. Kolmonen, A. Stohl, S. Eckhardt, A. Borbon, V. Gros, N. Marchand, J. L. Jaffrezo, A. Schwarzenboeck, A. Colomb, A. Wiedensohler, S. Borrmann, M. Lawrence, A. Baklanov, and U. Baltensperger
Atmos. Chem. Phys., 15, 9577–9591, https://doi.org/10.5194/acp-15-9577-2015, https://doi.org/10.5194/acp-15-9577-2015, 2015
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A detailed characterization of air quality in the Paris (France) agglomeration, a megacity, during two summer and winter intensive campaigns and from additional 1-year observations, revealed that about 70% of the fine particulate matter (PM) at urban background is transported into the megacity from upwind regions. Unexpectedly, a major part of organic PM is of modern origin (woodburning and cooking activities, secondary formation from biogenic VOC).
N. Hanrieder, S. Wilbert, R. Pitz-Paal, C. Emde, J. Gasteiger, B. Mayer, and J. Polo
Atmos. Meas. Tech., 8, 3467–3480, https://doi.org/10.5194/amt-8-3467-2015, https://doi.org/10.5194/amt-8-3467-2015, 2015
S. Eckhardt, B. Quennehen, D. J. L. Olivié, T. K. Berntsen, R. Cherian, J. H. Christensen, W. Collins, S. Crepinsek, N. Daskalakis, M. Flanner, A. Herber, C. Heyes, Ø. Hodnebrog, L. Huang, M. Kanakidou, Z. Klimont, J. Langner, K. S. Law, M. T. Lund, R. Mahmood, A. Massling, S. Myriokefalitakis, I. E. Nielsen, J. K. Nøjgaard, J. Quaas, P. K. Quinn, J.-C. Raut, S. T. Rumbold, M. Schulz, S. Sharma, R. B. Skeie, H. Skov, T. Uttal, K. von Salzen, and A. Stohl
Atmos. Chem. Phys., 15, 9413–9433, https://doi.org/10.5194/acp-15-9413-2015, https://doi.org/10.5194/acp-15-9413-2015, 2015
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The concentrations of sulfate, black carbon and other aerosols in the Arctic are characterized by high values in late winter and spring (so-called Arctic Haze) and low values in summer. Models have long been struggling to capture this seasonality. In this study, we evaluate sulfate and BC concentrations from different updated models and emissions against a comprehensive pan-Arctic measurement data set. We find that the models improved but still struggle to get the maximum concentrations.
C. Rolf, A. Afchine, H. Bozem, B. Buchholz, V. Ebert, T. Guggenmoser, P. Hoor, P. Konopka, E. Kretschmer, S. Müller, H. Schlager, N. Spelten, O. Sumińska-Ebersoldt, J. Ungermann, A. Zahn, and M. Krämer
Atmos. Chem. Phys., 15, 9143–9158, https://doi.org/10.5194/acp-15-9143-2015, https://doi.org/10.5194/acp-15-9143-2015, 2015
H. Siebert, R. A. Shaw, J. Ditas, T. Schmeissner, S. P. Malinowski, E. Bodenschatz, and H. Xu
Atmos. Meas. Tech., 8, 3219–3228, https://doi.org/10.5194/amt-8-3219-2015, https://doi.org/10.5194/amt-8-3219-2015, 2015
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We report results from simultaneous, high-resolution and collocated measurements of cloud microphysical and turbulence properties during several warm cloud events at the Umweltforschungsstation Schneefernerhaus (UFS) on Zugspitze in the German Alps. The data gathered were found to be representative of observations made with similar instrumentation in free clouds.
S. Risius, H. Xu, F. Di Lorenzo, H. Xi, H. Siebert, R. A. Shaw, and E. Bodenschatz
Atmos. Meas. Tech., 8, 3209–3218, https://doi.org/10.5194/amt-8-3209-2015, https://doi.org/10.5194/amt-8-3209-2015, 2015
E. F. Mikhailov, G. N. Mironov, C. Pöhlker, X. Chi, M. L. Krüger, M. Shiraiwa, J.-D. Förster, U. Pöschl, S. S. Vlasenko, T. I. Ryshkevich, M. Weigand, A. L. D. Kilcoyne, and M. O. Andreae
Atmos. Chem. Phys., 15, 8847–8869, https://doi.org/10.5194/acp-15-8847-2015, https://doi.org/10.5194/acp-15-8847-2015, 2015
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Our manuscript describes the hygroscopic properties of accumulation- and coarse-mode aerosol particles sampled at the ZOTTO in central Siberia (61º N, 89º E). The hygroscopic growth measurements were supplemented with chemical analyses of the samples. In addition, the microstructure and chemical composition of aerosol particles were analyzed by x-ray micro-spectroscopy (STXM-NEXAFS) and transmission electron microscopy (TEM).
P. Kupiszewski, E. Weingartner, P. Vochezer, M. Schnaiter, A. Bigi, M. Gysel, B. Rosati, E. Toprak, S. Mertes, and U. Baltensperger
Atmos. Meas. Tech., 8, 3087–3106, https://doi.org/10.5194/amt-8-3087-2015, https://doi.org/10.5194/amt-8-3087-2015, 2015
C. L. Ryder, J. B. McQuaid, C. Flamant, P. D. Rosenberg, R. Washington, H. E. Brindley, E. J. Highwood, J. H. Marsham, D. J. Parker, M. C. Todd, J. R. Banks, J. K. Brooke, S. Engelstaedter, V. Estelles, P. Formenti, L. Garcia-Carreras, C. Kocha, F. Marenco, H. Sodemann, C. J. T. Allen, A. Bourdon, M. Bart, C. Cavazos-Guerra, S. Chevaillier, J. Crosier, E. Darbyshire, A. R. Dean, J. R. Dorsey, J. Kent, D. O'Sullivan, K. Schepanski, K. Szpek, J. Trembath, and A. Woolley
Atmos. Chem. Phys., 15, 8479–8520, https://doi.org/10.5194/acp-15-8479-2015, https://doi.org/10.5194/acp-15-8479-2015, 2015
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Measurements of the Saharan atmosphere and of atmospheric mineral dust are lacking but are vital to our understanding of the climate of this region and their impacts further afield. Novel observations were made by the Fennec climate programme during June 2011 and 2012 using ground-based, remote sensing and airborne platforms. Here we describe the airborne observations and the contributions they have made to furthering our understanding of the Saharan climate system.
M. Schäfer, E. Bierwirth, A. Ehrlich, E. Jäkel, and M. Wendisch
Atmos. Chem. Phys., 15, 8147–8163, https://doi.org/10.5194/acp-15-8147-2015, https://doi.org/10.5194/acp-15-8147-2015, 2015
F. Chouza, O. Reitebuch, S. Groß, S. Rahm, V. Freudenthaler, C. Toledano, and B. Weinzierl
Atmos. Meas. Tech., 8, 2909–2926, https://doi.org/10.5194/amt-8-2909-2015, https://doi.org/10.5194/amt-8-2909-2015, 2015
C. Merker, G. Peters, M. Clemens, K. Lengfeld, and F. Ament
Atmos. Meas. Tech., 8, 2521–2530, https://doi.org/10.5194/amt-8-2521-2015, https://doi.org/10.5194/amt-8-2521-2015, 2015
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The theory of an approach for absolute radar calibration with respect to reflectivity and without a previously calibrated reference device is laid out and validated. The method requires a network of two horizontally oriented radars operating within a frequency range strongly attenuated by liquid water and a radar allowing for drop size distribution measurements with height (e.g. micro rain radar). The analysis by means of synthetic data shows potential for future practical application.
F. Ewald, C. Winkler, and T. Zinner
Atmos. Meas. Tech., 8, 2491–2508, https://doi.org/10.5194/amt-8-2491-2015, https://doi.org/10.5194/amt-8-2491-2015, 2015
J. Ungermann, J. Blank, M. Dick, A. Ebersoldt, F. Friedl-Vallon, A. Giez, T. Guggenmoser, M. Höpfner, T. Jurkat, M. Kaufmann, S. Kaufmann, A. Kleinert, M. Krämer, T. Latzko, H. Oelhaf, F. Olchewski, P. Preusse, C. Rolf, J. Schillings, O. Suminska-Ebersoldt, V. Tan, N. Thomas, C. Voigt, A. Zahn, M. Zöger, and M. Riese
Atmos. Meas. Tech., 8, 2473–2489, https://doi.org/10.5194/amt-8-2473-2015, https://doi.org/10.5194/amt-8-2473-2015, 2015
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The GLORIA sounder is an airborne infrared limb-imager combining a two-dimensional infrared detector with a Fourier transform spectrometer. It was operated aboard the new German Gulfstream G550 research aircraft HALO during the TACTS and ESMVAL campaigns in summer 2012. This paper describes the retrieval of temperature, as well as H2O, HNO3, and O3 cross sections from GLORIA dynamics mode spectra. A high correlation is achieved between the remote sensing and the in situ trace gas measurements.
M. Barrera-Verdejo, S. Crewell, U. Löhnert, E. Orlandi, and P. Di Girolamo
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amtd-8-5467-2015, https://doi.org/10.5194/amtd-8-5467-2015, 2015
Revised manuscript not accepted
A. Worringen, K. Kandler, N. Benker, T. Dirsch, S. Mertes, L. Schenk, U. Kästner, F. Frank, B. Nillius, U. Bundke, D. Rose, J. Curtius, P. Kupiszewski, E. Weingartner, P. Vochezer, J. Schneider, S. Schmidt, S. Weinbruch, and M. Ebert
Atmos. Chem. Phys., 15, 4161–4178, https://doi.org/10.5194/acp-15-4161-2015, https://doi.org/10.5194/acp-15-4161-2015, 2015
B. Altstädter, A. Platis, B. Wehner, A. Scholtz, N. Wildmann, M. Hermann, R. Käthner, H. Baars, J. Bange, and A. Lampert
Atmos. Meas. Tech., 8, 1627–1639, https://doi.org/10.5194/amt-8-1627-2015, https://doi.org/10.5194/amt-8-1627-2015, 2015
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The unmanned research aircraft Carolo P360 "ALADINA" is a flexible tool for investigating the horizontal and vertical distribution of freshly formed particles in the atmospheric boundary layer (ABL) combined with measurements of turbulent fluxes derived by fast meteorological sensors. First results of a feasibility study show, among others, events of particle bursts in an internal
layer of the ABL. Comparisons with ground-based instruments and a lidar present the reliability of the new system.
A. K. Vance, S. J. Abel, R. J. Cotton, and A. M. Woolley
Atmos. Meas. Tech., 8, 1617–1625, https://doi.org/10.5194/amt-8-1617-2015, https://doi.org/10.5194/amt-8-1617-2015, 2015
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Comparisons on the FAAM BAe 146-301 aircraft show good agreement between chilled mirror hygrometers and a WVSS-II fed from a modified Rosemount inlet (wvssR) in coud-free conditions, but a WVSS-II fed from the standard flush inlet (wvssF) over-reads, except at higher humidities. Case studies in cloudy conditions show that wvssF is immune to liquid water and ice, whilst wvssR is susceptible to both. Both WVSS-II inlets respond much more rapidly than the chilled mirror devices, especially wvssF.
L. K. Whalley, D. Stone, I. J. George, S. Mertes, D. van Pinxteren, A. Tilgner, H. Herrmann, M. J. Evans, and D. E. Heard
Atmos. Chem. Phys., 15, 3289–3301, https://doi.org/10.5194/acp-15-3289-2015, https://doi.org/10.5194/acp-15-3289-2015, 2015
S. Steinke, S. Eikenberg, U. Löhnert, G. Dick, D. Klocke, P. Di Girolamo, and S. Crewell
Atmos. Chem. Phys., 15, 2675–2692, https://doi.org/10.5194/acp-15-2675-2015, https://doi.org/10.5194/acp-15-2675-2015, 2015
B. C. Kindel, P. Pilewskie, K. S. Schmidt, T. Thornberry, A. Rollins, and T. Bui
Atmos. Meas. Tech., 8, 1147–1156, https://doi.org/10.5194/amt-8-1147-2015, https://doi.org/10.5194/amt-8-1147-2015, 2015
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Measurements of upper tropospheric-lower stratospheric water vapor amounts in the tropics were made using the 1400 and 1900nm water vapor bands present in airborne solar spectral irradiance data. These were validated with radiative transfer modeling using in situ profiles of water vapor, temperature, and pressure. An approach to extending these types of measurements from aircraft altitudes to the top of the atmosphere to infer stratospheric water vapor amount is outlined.
G. Mioche, O. Jourdan, M. Ceccaldi, and J. Delanoë
Atmos. Chem. Phys., 15, 2445–2461, https://doi.org/10.5194/acp-15-2445-2015, https://doi.org/10.5194/acp-15-2445-2015, 2015
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The study presents a characterization of the vertical, spatial and seasonal variability of Arctic clouds and mixed-phase clouds (MPCs) over the entire Arctic region. MPC properties in the region of the Svalbard archipelago (78°N, 15°E) are also investigated. The occurrence frequency of clouds and MPCs are determined from CALIPSO/CLOUDSAT measurements processed with the DARDAR retrieval algorithm which allows for a reliable cloud thermodynamic phase classification.
S. Schmidt, J. Schneider, T. Klimach, S. Mertes, L. P. Schenk, J. Curtius, P. Kupiszewski, E. Hammer, P. Vochezer, G. Lloyd, M. Ebert, K. Kandler, S. Weinbruch, and S. Borrmann
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-15-4677-2015, https://doi.org/10.5194/acpd-15-4677-2015, 2015
Revised manuscript not accepted
I. V. Gorodetskaya, S. Kneifel, M. Maahn, K. Van Tricht, W. Thiery, J. H. Schween, A. Mangold, S. Crewell, and N. P. M. Van Lipzig
The Cryosphere, 9, 285–304, https://doi.org/10.5194/tc-9-285-2015, https://doi.org/10.5194/tc-9-285-2015, 2015
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Our paper presents a new cloud-precipitation-meteorological observatory established in the escarpment zone of Dronning Maud Land, East Antarctica. The site is characterised by bimodal cloud occurrence (clear sky or overcast) with liquid-containing clouds occurring 20% of the cloudy periods. Local surface mass balance strongly depends on rare intense snowfall events. A substantial part of the accumulated snow is removed by surface and drifting snow sublimation and wind-driven snow erosion.
M. Klingebiel, A. de Lozar, S. Molleker, R. Weigel, A. Roth, L. Schmidt, J. Meyer, A. Ehrlich, R. Neuber, M. Wendisch, and S. Borrmann
Atmos. Chem. Phys., 15, 617–631, https://doi.org/10.5194/acp-15-617-2015, https://doi.org/10.5194/acp-15-617-2015, 2015
M. Mech, E. Orlandi, S. Crewell, F. Ament, L. Hirsch, M. Hagen, G. Peters, and B. Stevens
Atmos. Meas. Tech., 7, 4539–4553, https://doi.org/10.5194/amt-7-4539-2014, https://doi.org/10.5194/amt-7-4539-2014, 2014
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Here the High Altitude and LOng range research aircraft Microwave Package (HAMP) is introduced. The package consists
of three passive radiometer modules with 26 channels between 22
and 183 GHz and a 36 GHz Doppler cloud radar. The manuscript
describes the instrument specifications, the installation in the aircraft, and the operation. Furthermore, results from simulation
and retrieval studies, as well as measurements from a first test
campaign, are shown.
R. Döscher, T. Vihma, and E. Maksimovich
Atmos. Chem. Phys., 14, 13571–13600, https://doi.org/10.5194/acp-14-13571-2014, https://doi.org/10.5194/acp-14-13571-2014, 2014
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The article reviews progress in understanding of the Arctic sea ice decline. Processes are revisited from an atmospheric, ocean and sea ice perspective. There is strong evidence for decisive atmospheric drivers of sea ice change. Large-scale ocean influences on the Arctic Ocean hydrology and circulation are highly evident. Ocean heat fluxes are clearly impacting the ice margins. Little indication exists for a direct decisive influence of the warming ocean on the central Arctic sea ice cover.
W. Frey, S. Borrmann, F. Fierli, R. Weigel, V. Mitev, R. Matthey, F. Ravegnani, N. M. Sitnikov, A. Ulanovsky, and F. Cairo
Atmos. Chem. Phys., 14, 13223–13240, https://doi.org/10.5194/acp-14-13223-2014, https://doi.org/10.5194/acp-14-13223-2014, 2014
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This study presents in situ cloud microphysical observations obtained during a double flight in a Hector thunderstorm during the SCOUT-O3 campaign from Darwin, Northern Australia, in 2005. The measurements show a change of the micophysics with the storm's evolution. The clouds in the dissipating stage possess a high potential for affecting the humidity in the tropical tropopause layer.
K. Lengfeld, M. Clemens, H. Münster, and F. Ament
Atmos. Meas. Tech., 7, 4151–4166, https://doi.org/10.5194/amt-7-4151-2014, https://doi.org/10.5194/amt-7-4151-2014, 2014
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This publication intends to prove that a network of low-cost local area weather radars with a time resolution of 30s and range resolution of 60m is a reliable and scientifically valuable comple-ment to nationwide radar networks, especially in urban areas. The advantages of high temporal resolution and multiple coverage in overlapping areas are proven to enhance the quality of pre-cipitation estimates. Long-term comparison with C-band radar confirms very good accordance with POD>90% and FAR<10%.
B. H. Samset, G. Myhre, A. Herber, Y. Kondo, S.-M. Li, N. Moteki, M. Koike, N. Oshima, J. P. Schwarz, Y. Balkanski, S. E. Bauer, N. Bellouin, T. K. Berntsen, H. Bian, M. Chin, T. Diehl, R. C. Easter, S. J. Ghan, T. Iversen, A. Kirkevåg, J.-F. Lamarque, G. Lin, X. Liu, J. E. Penner, M. Schulz, Ø. Seland, R. B. Skeie, P. Stier, T. Takemura, K. Tsigaridis, and K. Zhang
Atmos. Chem. Phys., 14, 12465–12477, https://doi.org/10.5194/acp-14-12465-2014, https://doi.org/10.5194/acp-14-12465-2014, 2014
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Far from black carbon (BC) emission sources, present climate models are unable to reproduce flight measurements. By comparing recent models with data, we find that the atmospheric lifetime of BC may be overestimated in models. By adjusting modeled BC concentrations to measurements in remote regions - over oceans and at high altitudes - we arrive at a reduced estimate for BC radiative forcing over the industrial era.
K. Diehl, M. Debertshäuser, O. Eppers, H. Schmithüsen, S. K. Mitra, and S. Borrmann
Atmos. Chem. Phys., 14, 12343–12355, https://doi.org/10.5194/acp-14-12343-2014, https://doi.org/10.5194/acp-14-12343-2014, 2014
J. H. Schween, A. Hirsikko, U. Löhnert, and S. Crewell
Atmos. Meas. Tech., 7, 3685–3704, https://doi.org/10.5194/amt-7-3685-2014, https://doi.org/10.5194/amt-7-3685-2014, 2014
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Two different methods for the determination of the mixing layer height (MLH) are investigated with a one-year data set from central Europe: (i) based on a significant gradient of backscatter and (ii) on the vertical velocity. The aerosol-based method shows significant over-estimation in the morning hours when the ML grows into the residual layer and late afternoon hours when turbulent mixing decays. This results in systematic over-estimation of average characteristcs as e.g. maximum MLH.
W. Woiwode, J.-U. Grooß, H. Oelhaf, S. Molleker, S. Borrmann, A. Ebersoldt, W. Frey, T. Gulde, S. Khaykin, G. Maucher, C. Piesch, and J. Orphal
Atmos. Chem. Phys., 14, 11525–11544, https://doi.org/10.5194/acp-14-11525-2014, https://doi.org/10.5194/acp-14-11525-2014, 2014
E. Fontaine, A. Schwarzenboeck, J. Delanoë, W. Wobrock, D. Leroy, R. Dupuy, C. Gourbeyre, and A. Protat
Atmos. Chem. Phys., 14, 11367–11392, https://doi.org/10.5194/acp-14-11367-2014, https://doi.org/10.5194/acp-14-11367-2014, 2014
L. P. Schenk, S. Mertes, U. Kästner, F. Frank, B. Nillius, U. Bundke, D. Rose, S. Schmidt, J. Schneider, A. Worringen, K. Kandler, N. Bukowiecki, M. Ebert, J. Curtius, and F. Stratmann
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amtd-7-10585-2014, https://doi.org/10.5194/amtd-7-10585-2014, 2014
Revised manuscript has not been submitted
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A pumped counterflow virtual impactor (PCVI) was set up to separate ice nucleating particle (INP) counter produced ice particles that had been activated to ice from non-activated aerosol particles. The released INP were characterized with regard to their physico-chemical properties. A successful separation (PCVI) of INP for water-subsaturated conditions is proven. First results of INP properties are presented which were gained during a campaign at the high altitude research station Jungfraujoch.
S. Molleker, S. Borrmann, H. Schlager, B. Luo, W. Frey, M. Klingebiel, R. Weigel, M. Ebert, V. Mitev, R. Matthey, W. Woiwode, H. Oelhaf, A. Dörnbrack, G. Stratmann, J.-U. Grooß, G. Günther, B. Vogel, R. Müller, M. Krämer, J. Meyer, and F. Cairo
Atmos. Chem. Phys., 14, 10785–10801, https://doi.org/10.5194/acp-14-10785-2014, https://doi.org/10.5194/acp-14-10785-2014, 2014
W. Ait-Helal, A. Borbon, S. Sauvage, J. A. de Gouw, A. Colomb, V. Gros, F. Freutel, M. Crippa, C. Afif, U. Baltensperger, M. Beekmann, J.-F. Doussin, R. Durand-Jolibois, I. Fronval, N. Grand, T. Leonardis, M. Lopez, V. Michoud, K. Miet, S. Perrier, A. S. H. Prévôt, J. Schneider, G. Siour, P. Zapf, and N. Locoge
Atmos. Chem. Phys., 14, 10439–10464, https://doi.org/10.5194/acp-14-10439-2014, https://doi.org/10.5194/acp-14-10439-2014, 2014
A. Tetzlaff, C. Lüpkes, G. Birnbaum, J. Hartmann, T. Nygård, and T. Vihma
The Cryosphere, 8, 1757–1762, https://doi.org/10.5194/tc-8-1757-2014, https://doi.org/10.5194/tc-8-1757-2014, 2014
S. J. Abel, R. J. Cotton, P. A. Barrett, and A. K. Vance
Atmos. Meas. Tech., 7, 3007–3022, https://doi.org/10.5194/amt-7-3007-2014, https://doi.org/10.5194/amt-7-3007-2014, 2014
T. Vihma, R. Pirazzini, I. Fer, I. A. Renfrew, J. Sedlar, M. Tjernström, C. Lüpkes, T. Nygård, D. Notz, J. Weiss, D. Marsan, B. Cheng, G. Birnbaum, S. Gerland, D. Chechin, and J. C. Gascard
Atmos. Chem. Phys., 14, 9403–9450, https://doi.org/10.5194/acp-14-9403-2014, https://doi.org/10.5194/acp-14-9403-2014, 2014
H. Bozem, H. Fischer, C. Gurk, C. L. Schiller, U. Parchatka, R. Koenigstedt, A. Stickler, M. Martinez, H. Harder, D. Kubistin, J. Williams, G. Eerdekens, and J. Lelieveld
Atmos. Chem. Phys., 14, 8917–8931, https://doi.org/10.5194/acp-14-8917-2014, https://doi.org/10.5194/acp-14-8917-2014, 2014
S. Groß, M. Wirth, A. Schäfler, A. Fix, S. Kaufmann, and C. Voigt
Atmos. Meas. Tech., 7, 2745–2755, https://doi.org/10.5194/amt-7-2745-2014, https://doi.org/10.5194/amt-7-2745-2014, 2014
I. Välisuo, T. Vihma, and J. C. King
The Cryosphere, 8, 1519–1538, https://doi.org/10.5194/tc-8-1519-2014, https://doi.org/10.5194/tc-8-1519-2014, 2014
M. L. Krüger, S. Mertes, T. Klimach, Y. F. Cheng, H. Su, J. Schneider, M. O. Andreae, U. Pöschl, and D. Rose
Atmos. Meas. Tech., 7, 2615–2629, https://doi.org/10.5194/amt-7-2615-2014, https://doi.org/10.5194/amt-7-2615-2014, 2014
S. Henning, K. Dieckmann, K. Ignatius, M. Schäfer, P. Zedler, E. Harris, B. Sinha, D. van Pinxteren, S. Mertes, W. Birmili, M. Merkel, Z. Wu, A. Wiedensohler, H. Wex, H. Herrmann, and F. Stratmann
Atmos. Chem. Phys., 14, 7859–7868, https://doi.org/10.5194/acp-14-7859-2014, https://doi.org/10.5194/acp-14-7859-2014, 2014
N. Rastak, S. Silvergren, P. Zieger, U. Wideqvist, J. Ström, B. Svenningsson, M. Maturilli, M. Tesche, A. M. L. Ekman, P. Tunved, and I. Riipinen
Atmos. Chem. Phys., 14, 7445–7460, https://doi.org/10.5194/acp-14-7445-2014, https://doi.org/10.5194/acp-14-7445-2014, 2014
A. Winschall, S. Pfahl, H. Sodemann, and H. Wernli
Atmos. Chem. Phys., 14, 6605–6619, https://doi.org/10.5194/acp-14-6605-2014, https://doi.org/10.5194/acp-14-6605-2014, 2014
F. Dahlkötter, M. Gysel, D. Sauer, A. Minikin, R. Baumann, P. Seifert, A. Ansmann, M. Fromm, C. Voigt, and B. Weinzierl
Atmos. Chem. Phys., 14, 6111–6137, https://doi.org/10.5194/acp-14-6111-2014, https://doi.org/10.5194/acp-14-6111-2014, 2014
A. Kreuter, R. Buras, B. Mayer, A. Webb, R. Kift, A. Bais, N. Kouremeti, and M. Blumthaler
Atmos. Chem. Phys., 14, 5989–6002, https://doi.org/10.5194/acp-14-5989-2014, https://doi.org/10.5194/acp-14-5989-2014, 2014
M. Mielke, N. S. Zinoviev, K. Dethloff, A. Rinke, V. J. Kustov, A. P. Makshtas, V. T. Sokolov, R. Neuber, M. Maturilli, D. Klaus, D. Handorf, and J. Graeser
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-14-11855-2014, https://doi.org/10.5194/acpd-14-11855-2014, 2014
Revised manuscript has not been submitted
J.-L. Bonne, V. Masson-Delmotte, O. Cattani, M. Delmotte, C. Risi, H. Sodemann, and H. C. Steen-Larsen
Atmos. Chem. Phys., 14, 4419–4439, https://doi.org/10.5194/acp-14-4419-2014, https://doi.org/10.5194/acp-14-4419-2014, 2014
K. Van Tricht, I. V. Gorodetskaya, S. Lhermitte, D. D. Turner, J. H. Schween, and N. P. M. Van Lipzig
Atmos. Meas. Tech., 7, 1153–1167, https://doi.org/10.5194/amt-7-1153-2014, https://doi.org/10.5194/amt-7-1153-2014, 2014
E. Harris, B. Sinha, D. van Pinxteren, J. Schneider, L. Poulain, J. Collett, B. D'Anna, B. Fahlbusch, S. Foley, K. W. Fomba, C. George, T. Gnauk, S. Henning, T. Lee, S. Mertes, A. Roth, F. Stratmann, S. Borrmann, P. Hoppe, and H. Herrmann
Atmos. Chem. Phys., 14, 4219–4235, https://doi.org/10.5194/acp-14-4219-2014, https://doi.org/10.5194/acp-14-4219-2014, 2014
F. Aemisegger, S. Pfahl, H. Sodemann, I. Lehner, S. I. Seneviratne, and H. Wernli
Atmos. Chem. Phys., 14, 4029–4054, https://doi.org/10.5194/acp-14-4029-2014, https://doi.org/10.5194/acp-14-4029-2014, 2014
S. Pfahl and H. Sodemann
Clim. Past, 10, 771–781, https://doi.org/10.5194/cp-10-771-2014, https://doi.org/10.5194/cp-10-771-2014, 2014
B. Reinhardt, R. Buras, L. Bugliaro, S. Wilbert, and B. Mayer
Atmos. Meas. Tech., 7, 823–838, https://doi.org/10.5194/amt-7-823-2014, https://doi.org/10.5194/amt-7-823-2014, 2014
C. Fricke, A. Ehrlich, E. Jäkel, B. Bohn, M. Wirth, and M. Wendisch
Atmos. Chem. Phys., 14, 1943–1958, https://doi.org/10.5194/acp-14-1943-2014, https://doi.org/10.5194/acp-14-1943-2014, 2014
T. Nygård, T. Valkonen, and T. Vihma
Atmos. Chem. Phys., 14, 1959–1971, https://doi.org/10.5194/acp-14-1959-2014, https://doi.org/10.5194/acp-14-1959-2014, 2014
C. Jouan, J. Pelon, E. Girard, G. Ancellet, J. P. Blanchet, and J. Delanoë
Atmos. Chem. Phys., 14, 1205–1224, https://doi.org/10.5194/acp-14-1205-2014, https://doi.org/10.5194/acp-14-1205-2014, 2014
E. Hammer, N. Bukowiecki, M. Gysel, Z. Jurányi, C. R. Hoyle, R. Vogt, U. Baltensperger, and E. Weingartner
Atmos. Chem. Phys., 14, 1123–1139, https://doi.org/10.5194/acp-14-1123-2014, https://doi.org/10.5194/acp-14-1123-2014, 2014
J.-F. Gayet, V. Shcherbakov, L. Bugliaro, A. Protat, J. Delanoë, J. Pelon, and A. Garnier
Atmos. Chem. Phys., 14, 899–912, https://doi.org/10.5194/acp-14-899-2014, https://doi.org/10.5194/acp-14-899-2014, 2014
P. Jeßberger, C. Voigt, U. Schumann, I. Sölch, H. Schlager, S. Kaufmann, A. Petzold, D. Schäuble, and J.-F. Gayet
Atmos. Chem. Phys., 13, 11965–11984, https://doi.org/10.5194/acp-13-11965-2013, https://doi.org/10.5194/acp-13-11965-2013, 2013
D. Rose, S. S. Gunthe, Z. Jurányi, M. Gysel, G. P. Frank, J. Schneider, J. Curtius, and U. Pöschl
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-13-32575-2013, https://doi.org/10.5194/acpd-13-32575-2013, 2013
Revised manuscript has not been submitted
R. Fröhlich, M. J. Cubison, J. G. Slowik, N. Bukowiecki, A. S. H. Prévôt, U. Baltensperger, J. Schneider, J. R. Kimmel, M. Gonin, U. Rohner, D. R. Worsnop, and J. T. Jayne
Atmos. Meas. Tech., 6, 3225–3241, https://doi.org/10.5194/amt-6-3225-2013, https://doi.org/10.5194/amt-6-3225-2013, 2013
F. Freutel, F. Drewnick, J. Schneider, T. Klimach, and S. Borrmann
Atmos. Meas. Tech., 6, 3131–3145, https://doi.org/10.5194/amt-6-3131-2013, https://doi.org/10.5194/amt-6-3131-2013, 2013
C. E. Chung, H. Cha, T. Vihma, P. Räisänen, and D. Decremer
Atmos. Chem. Phys., 13, 11209–11219, https://doi.org/10.5194/acp-13-11209-2013, https://doi.org/10.5194/acp-13-11209-2013, 2013
L. Jakobson, T. Vihma, E. Jakobson, T. Palo, A. Männik, and J. Jaagus
Atmos. Chem. Phys., 13, 11089–11099, https://doi.org/10.5194/acp-13-11089-2013, https://doi.org/10.5194/acp-13-11089-2013, 2013
E. Regelin, H. Harder, M. Martinez, D. Kubistin, C. Tatum Ernest, H. Bozem, T. Klippel, Z. Hosaynali-Beygi, H. Fischer, R. Sander, P. Jöckel, R. Königstedt, and J. Lelieveld
Atmos. Chem. Phys., 13, 10703–10720, https://doi.org/10.5194/acp-13-10703-2013, https://doi.org/10.5194/acp-13-10703-2013, 2013
G. Maschwitz, U. Löhnert, S. Crewell, T. Rose, and D. D. Turner
Atmos. Meas. Tech., 6, 2641–2658, https://doi.org/10.5194/amt-6-2641-2013, https://doi.org/10.5194/amt-6-2641-2013, 2013
H. Siebert, M. Beals, J. Bethke, E. Bierwirth, T. Conrath, K. Dieckmann, F. Ditas, A. Ehrlich, D. Farrell, S. Hartmann, M. A. Izaguirre, J. Katzwinkel, L. Nuijens, G. Roberts, M. Schäfer, R. A. Shaw, T. Schmeissner, I. Serikov, B. Stevens, F. Stratmann, B. Wehner, M. Wendisch, F. Werner, and H. Wex
Atmos. Chem. Phys., 13, 10061–10077, https://doi.org/10.5194/acp-13-10061-2013, https://doi.org/10.5194/acp-13-10061-2013, 2013
M. von Hobe, S. Bekki, S. Borrmann, F. Cairo, F. D'Amato, G. Di Donfrancesco, A. Dörnbrack, A. Ebersoldt, M. Ebert, C. Emde, I. Engel, M. Ern, W. Frey, S. Genco, S. Griessbach, J.-U. Grooß, T. Gulde, G. Günther, E. Hösen, L. Hoffmann, V. Homonnai, C. R. Hoyle, I. S. A. Isaksen, D. R. Jackson, I. M. Jánosi, R. L. Jones, K. Kandler, C. Kalicinsky, A. Keil, S. M. Khaykin, F. Khosrawi, R. Kivi, J. Kuttippurath, J. C. Laube, F. Lefèvre, R. Lehmann, S. Ludmann, B. P. Luo, M. Marchand, J. Meyer, V. Mitev, S. Molleker, R. Müller, H. Oelhaf, F. Olschewski, Y. Orsolini, T. Peter, K. Pfeilsticker, C. Piesch, M. C. Pitts, L. R. Poole, F. D. Pope, F. Ravegnani, M. Rex, M. Riese, T. Röckmann, B. Rognerud, A. Roiger, C. Rolf, M. L. Santee, M. Scheibe, C. Schiller, H. Schlager, M. Siciliani de Cumis, N. Sitnikov, O. A. Søvde, R. Spang, N. Spelten, F. Stordal, O. Sumińska-Ebersoldt, A. Ulanovski, J. Ungermann, S. Viciani, C. M. Volk, M. vom Scheidt, P. von der Gathen, K. Walker, T. Wegner, R. Weigel, S. Weinbruch, G. Wetzel, F. G. Wienhold, I. Wohltmann, W. Woiwode, I. A. K. Young, V. Yushkov, B. Zobrist, and F. Stroh
Atmos. Chem. Phys., 13, 9233–9268, https://doi.org/10.5194/acp-13-9233-2013, https://doi.org/10.5194/acp-13-9233-2013, 2013
J. Schmale, J. Schneider, E. Nemitz, Y. S. Tang, U. Dragosits, T. D. Blackall, P. N. Trathan, G. J. Phillips, M. Sutton, and C. F. Braban
Atmos. Chem. Phys., 13, 8669–8694, https://doi.org/10.5194/acp-13-8669-2013, https://doi.org/10.5194/acp-13-8669-2013, 2013
D. Merk and T. Zinner
Atmos. Meas. Tech., 6, 1903–1918, https://doi.org/10.5194/amt-6-1903-2013, https://doi.org/10.5194/amt-6-1903-2013, 2013
M. Schäfer, E. Bierwirth, A. Ehrlich, F. Heyner, and M. Wendisch
Atmos. Meas. Tech., 6, 1855–1868, https://doi.org/10.5194/amt-6-1855-2013, https://doi.org/10.5194/amt-6-1855-2013, 2013
A. E. Luebke, L. M. Avallone, C. Schiller, J. Meyer, C. Rolf, and M. Krämer
Atmos. Chem. Phys., 13, 6447–6459, https://doi.org/10.5194/acp-13-6447-2013, https://doi.org/10.5194/acp-13-6447-2013, 2013
Z. Jurányi, T. Tritscher, M. Gysel, M. Laborde, L. Gomes, G. Roberts, U. Baltensperger, and E. Weingartner
Atmos. Chem. Phys., 13, 6431–6446, https://doi.org/10.5194/acp-13-6431-2013, https://doi.org/10.5194/acp-13-6431-2013, 2013
J. A. Seabrook, J. A. Whiteway, L. H. Gray, R. Staebler, and A. Herber
Atmos. Chem. Phys., 13, 6023–6029, https://doi.org/10.5194/acp-13-6023-2013, https://doi.org/10.5194/acp-13-6023-2013, 2013
T. Zinner, C. Forster, E. de Coning, and H.-D. Betz
Atmos. Meas. Tech., 6, 1567–1583, https://doi.org/10.5194/amt-6-1567-2013, https://doi.org/10.5194/amt-6-1567-2013, 2013
M. D. Andrés-Hernández, D. Kartal, J. N. Crowley, V. Sinha, E. Regelin, M. Martínez-Harder, V. Nenakhov, J. Williams, H. Harder, H. Bozem, W. Song, J. Thieser, M. J. Tang, Z. Hosaynali Beigi, and J. P. Burrows
Atmos. Chem. Phys., 13, 5731–5749, https://doi.org/10.5194/acp-13-5731-2013, https://doi.org/10.5194/acp-13-5731-2013, 2013
M. Laborde, M. Crippa, T. Tritscher, Z. Jurányi, P. F. Decarlo, B. Temime-Roussel, N. Marchand, S. Eckhardt, A. Stohl, U. Baltensperger, A. S. H. Prévôt, E. Weingartner, and M. Gysel
Atmos. Chem. Phys., 13, 5831–5856, https://doi.org/10.5194/acp-13-5831-2013, https://doi.org/10.5194/acp-13-5831-2013, 2013
Q. J. Zhang, M. Beekmann, F. Drewnick, F. Freutel, J. Schneider, M. Crippa, A. S. H. Prevot, U. Baltensperger, L. Poulain, A. Wiedensohler, J. Sciare, V. Gros, A. Borbon, A. Colomb, V. Michoud, J.-F. Doussin, H. A. C. Denier van der Gon, M. Haeffelin, J.-C. Dupont, G. Siour, H. Petetin, B. Bessagnet, S. N. Pandis, A. Hodzic, O. Sanchez, C. Honoré, and O. Perrussel
Atmos. Chem. Phys., 13, 5767–5790, https://doi.org/10.5194/acp-13-5767-2013, https://doi.org/10.5194/acp-13-5767-2013, 2013
T. D. Thornberry, A. W. Rollins, R. S. Gao, L. A. Watts, S. J. Ciciora, R. J. McLaughlin, C. Voigt, B. Hall, and D. W. Fahey
Atmos. Meas. Tech., 6, 1461–1475, https://doi.org/10.5194/amt-6-1461-2013, https://doi.org/10.5194/amt-6-1461-2013, 2013
H. C. Steen-Larsen, S. J. Johnsen, V. Masson-Delmotte, B. Stenni, C. Risi, H. Sodemann, D. Balslev-Clausen, T. Blunier, D. Dahl-Jensen, M. D. Ellehøj, S. Falourd, A. Grindsted, V. Gkinis, J. Jouzel, T. Popp, S. Sheldon, S. B. Simonsen, J. Sjolte, J. P. Steffensen, P. Sperlich, A. E. Sveinbjörnsdóttir, B. M. Vinther, and J. W. C. White
Atmos. Chem. Phys., 13, 4815–4828, https://doi.org/10.5194/acp-13-4815-2013, https://doi.org/10.5194/acp-13-4815-2013, 2013
E. Bierwirth, A. Ehrlich, M. Wendisch, J.-F. Gayet, C. Gourbeyre, R. Dupuy, A. Herber, R. Neuber, and A. Lampert
Atmos. Meas. Tech., 6, 1189–1200, https://doi.org/10.5194/amt-6-1189-2013, https://doi.org/10.5194/amt-6-1189-2013, 2013
V. Meunier, U. Löhnert, P. Kollias, and S. Crewell
Atmos. Meas. Tech., 6, 1171–1187, https://doi.org/10.5194/amt-6-1171-2013, https://doi.org/10.5194/amt-6-1171-2013, 2013
G. Pappalardo, L. Mona, G. D'Amico, U. Wandinger, M. Adam, A. Amodeo, A. Ansmann, A. Apituley, L. Alados Arboledas, D. Balis, A. Boselli, J. A. Bravo-Aranda, A. Chaikovsky, A. Comeron, J. Cuesta, F. De Tomasi, V. Freudenthaler, M. Gausa, E. Giannakaki, H. Giehl, A. Giunta, I. Grigorov, S. Groß, M. Haeffelin, A. Hiebsch, M. Iarlori, D. Lange, H. Linné, F. Madonna, I. Mattis, R.-E. Mamouri, M. A. P. McAuliffe, V. Mitev, F. Molero, F. Navas-Guzman, D. Nicolae, A. Papayannis, M. R. Perrone, C. Pietras, A. Pietruczuk, G. Pisani, J. Preißler, M. Pujadas, V. Rizi, A. A. Ruth, J. Schmidt, F. Schnell, P. Seifert, I. Serikov, M. Sicard, V. Simeonov, N. Spinelli, K. Stebel, M. Tesche, T. Trickl, X. Wang, F. Wagner, M. Wiegner, and K. M. Wilson
Atmos. Chem. Phys., 13, 4429–4450, https://doi.org/10.5194/acp-13-4429-2013, https://doi.org/10.5194/acp-13-4429-2013, 2013
M. Maturilli, A. Herber, and G. König-Langlo
Earth Syst. Sci. Data, 5, 155–163, https://doi.org/10.5194/essd-5-155-2013, https://doi.org/10.5194/essd-5-155-2013, 2013
K. Gottschaldt, C. Voigt, P. Jöckel, M. Righi, R. Deckert, and S. Dietmüller
Atmos. Chem. Phys., 13, 3003–3025, https://doi.org/10.5194/acp-13-3003-2013, https://doi.org/10.5194/acp-13-3003-2013, 2013
A. Kylling, R. Buras, S. Eckhardt, C. Emde, B. Mayer, and A. Stohl
Atmos. Meas. Tech., 6, 649–660, https://doi.org/10.5194/amt-6-649-2013, https://doi.org/10.5194/amt-6-649-2013, 2013
S. Groß, M. Esselborn, B. Weinzierl, M. Wirth, A. Fix, and A. Petzold
Atmos. Chem. Phys., 13, 2487–2505, https://doi.org/10.5194/acp-13-2487-2013, https://doi.org/10.5194/acp-13-2487-2013, 2013
S. Groß, M. Esselborn, F. Abicht, M. Wirth, A. Fix, and A. Minikin
Atmos. Chem. Phys., 13, 2435–2444, https://doi.org/10.5194/acp-13-2435-2013, https://doi.org/10.5194/acp-13-2435-2013, 2013
E. Jäkel, J. Walter, and M. Wendisch
Atmos. Meas. Tech., 6, 539–547, https://doi.org/10.5194/amt-6-539-2013, https://doi.org/10.5194/amt-6-539-2013, 2013
E. Jäkel, M. Wendisch, and B. Mayer
Atmos. Meas. Tech., 6, 527–537, https://doi.org/10.5194/amt-6-527-2013, https://doi.org/10.5194/amt-6-527-2013, 2013
M. Frosch, M. Bilde, A. Nenes, A. P. Praplan, Z. Jurányi, J. Dommen, M. Gysel, E. Weingartner, and U. Baltensperger
Atmos. Chem. Phys., 13, 2283–2297, https://doi.org/10.5194/acp-13-2283-2013, https://doi.org/10.5194/acp-13-2283-2013, 2013
F. Ewald, L. Bugliaro, H. Mannstein, and B. Mayer
Atmos. Meas. Tech., 6, 309–322, https://doi.org/10.5194/amt-6-309-2013, https://doi.org/10.5194/amt-6-309-2013, 2013
A. Tetzlaff, L. Kaleschke, C. Lüpkes, F. Ament, and T. Vihma
The Cryosphere, 7, 153–166, https://doi.org/10.5194/tc-7-153-2013, https://doi.org/10.5194/tc-7-153-2013, 2013
M. Crippa, P. F. DeCarlo, J. G. Slowik, C. Mohr, M. F. Heringa, R. Chirico, L. Poulain, F. Freutel, J. Sciare, J. Cozic, C. F. Di Marco, M. Elsasser, J. B. Nicolas, N. Marchand, E. Abidi, A. Wiedensohler, F. Drewnick, J. Schneider, S. Borrmann, E. Nemitz, R. Zimmermann, J.-L. Jaffrezo, A. S. H. Prévôt, and U. Baltensperger
Atmos. Chem. Phys., 13, 961–981, https://doi.org/10.5194/acp-13-961-2013, https://doi.org/10.5194/acp-13-961-2013, 2013
F. Freutel, J. Schneider, F. Drewnick, S.-L. von der Weiden-Reinmüller, M. Crippa, A. S. H. Prévôt, U. Baltensperger, L. Poulain, A. Wiedensohler, J. Sciare, R. Sarda-Estève, J. F. Burkhart, S. Eckhardt, A. Stohl, V. Gros, A. Colomb, V. Michoud, J. F. Doussin, A. Borbon, M. Haeffelin, Y. Morille, M. Beekmann, and S. Borrmann
Atmos. Chem. Phys., 13, 933–959, https://doi.org/10.5194/acp-13-933-2013, https://doi.org/10.5194/acp-13-933-2013, 2013
C. L. Ryder, E. J. Highwood, P. D. Rosenberg, J. Trembath, J. K. Brooke, M. Bart, A. Dean, J. Crosier, J. Dorsey, H. Brindley, J. Banks, J. H. Marsham, J. B. McQuaid, H. Sodemann, and R. Washington
Atmos. Chem. Phys., 13, 303–325, https://doi.org/10.5194/acp-13-303-2013, https://doi.org/10.5194/acp-13-303-2013, 2013
Related subject area
Subject: Dynamics | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Evidence of tropospheric uplift into the stratosphere via the tropical western Pacific cold trap
Identification and characterization of foehn events in Beijing and their impact on air-pollution episodes
Impact of Convectively Coupled Tropical Waves on the composition and vertical structure of the atmosphere above Cabo Verde in September 2021 during the CADDIWA campaign
Impact of boundary layer stability on urban park cooling effect intensity
Investigation of non-equilibrium turbulence decay in the atmospheric boundary layer using Doppler lidar measurements
Measurement report: The promotion of the low-level jet and thermal effects on the development of the deep convective boundary layer at the southern edge of the Taklimakan Desert
Estimating scalar turbulent fluxes with slow-response sensors in the stable atmospheric boundary layer
Contrasting extremely warm and long-lasting cold air anomalies in the North Atlantic sector of the Arctic during the HALO-(𝒜 𝒞)3 campaign
Air–sea interactions in stable atmospheric conditions: lessons from the desert semi-enclosed Gulf of Eilat (Aqaba)
An overview of the vertical structure of the atmospheric boundary layer in the central Arctic during MOSAiC
Evaluation of methods to determine the surface mixing layer height of the atmospheric boundary layer in the central Arctic during polar night and transition to polar day in cloudless and cloudy conditions
The role of a low-level jet for stirring the stable atmospheric surface layer in the Arctic
Detection of dilution due to turbulent mixing vs. precipitation scavenging effects on biomass burning aerosol concentrations using stable water isotope ratios during ORACLES
Modulation of the intraseasonal variability in early summer precipitation in eastern China by the Quasi-Biennial Oscillation and the Madden–Julian Oscillation
Thermodynamic and kinematic drivers of atmospheric boundary layer stability in the central Arctic during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC)
Occurrence frequency of subcritical Richardson numbers assessed by global high-resolution radiosonde and ERA5 reanalysis
The characteristics of atmospheric boundary layer height over the Arctic Ocean during MOSAiC
Turbulent structure of the Arctic boundary layer in early summer driven by stability, wind shear and cloud-top radiative cooling: ACLOUD airborne observations
Dependency of vertical velocity variance on meteorological conditions in the convective boundary layer
Triggering effects of large topography and boundary layer turbulence on convection over the Tibetan Plateau
A change in the relation between the Subtropical Indian Ocean Dipole and the South Atlantic Ocean Dipole indices in the past four decades
Characterising the dynamic movement of thunderstorms using very low- and low-frequency (VLF/LF) total lightning data over the Pearl River Delta region
Evolution of turbulent kinetic energy during the entire sandstorm process
Seasonal updraft speeds change cloud droplet number concentrations in low-level clouds over the western North Atlantic
The effect of ice supersaturation and thin cirrus on lapse rates in the upper troposphere
Momentum fluxes from airborne wind measurements in three cumulus cases over land
Orographically induced spontaneous imbalance within the jet causing a large-scale gravity wave event
Exploring the elevated water vapor signal associated with the free tropospheric biomass burning plume over the southeast Atlantic Ocean
Opinion: Gigacity – a source of problems or the new way to sustainable development
The thermodynamic structures of the planetary boundary layer dominated by synoptic circulations and the regular effect on air pollution in Beijing
Turbulent and boundary layer characteristics during VOCALS-REx
A foehn-induced haze front in Beijing: observations and implications
Airborne measurements and large-eddy simulations of small-scale gravity waves at the tropopause inversion layer over Scandinavia
Observational analysis of the daily cycle of the planetary boundary layer in the central Amazon during a non-El Niño year and El Niño year (GoAmazon project 2014/5)
Planetary boundary layer evolution over the Amazon rainforest in episodes of deep moist convection at the Amazon Tall Tower Observatory
Dominant patterns of summer ozone pollution in eastern China and associated atmospheric circulations
What controls the formation of nocturnal low-level stratus clouds over southern West Africa during the monsoon season?
Recent trends in climate variability at the local scale using 40 years of observations: the case of the Paris region of France
Nocturnal boundary layer turbulence regimes analysis during the BLLAST campaign
Low-level stratiform clouds and dynamical features observed within the southern West African monsoon
Residual layer ozone, mixing, and the nocturnal jet in California's San Joaquin Valley
From weak to intense downslope winds: origin, interaction with boundary-layer turbulence and impact on CO2 variability
On the fine vertical structure of the low troposphere over the coastal margins of East Antarctica
Spatial and temporal variability of turbulence dissipation rate in complex terrain
Characterizing wind gusts in complex terrain
Long-term trends of instability and associated parameters over the Indian region obtained using a radiosonde network
Implication of tropical lower stratospheric cooling in recent trends in tropical circulation and deep convective activity
The observed diurnal cycle of low-level stratus clouds over southern West Africa: a case study
Nocturnal low-level clouds in the atmospheric boundary layer over southern West Africa: an observation-based analysis of conditions and processes
Characteristics and evolution of diurnal foehn events in the Dead Sea valley
Xiaoyu Sun, Katrin Müller, Mathias Palm, Christoph Ritter, Denghui Ji, Tim Balthasar Röpke, and Justus Notholt
Atmos. Chem. Phys., 25, 6881–6902, https://doi.org/10.5194/acp-25-6881-2025, https://doi.org/10.5194/acp-25-6881-2025, 2025
Short summary
Short summary
We studied how air moves from the lower atmosphere to the stratosphere over the tropical western Pacific. Using observations and air tracking, we found that, in winter, air ascends and cold temperatures freeze water out, drying it before it enters the stratosphere. In summer, air tends to sink after cloud formation. This process affects water vapor amounts in the stratosphere, influencing the greenhouse effect and climate.
Ju Li, Jingjiang Zhang, Mengxin Bai, Jie Su, Qingchun Li, and Xingcan Jia
EGUsphere, https://doi.org/10.5194/egusphere-2024-2684, https://doi.org/10.5194/egusphere-2024-2684, 2025
Short summary
Short summary
This research examines foehn events in Beijing using weather station data from 2015 to 2020. We found an average of 56.5 foehn days annually, primarily in winter. These winds can raise temperatures significantly and are associated with air-pollution levels. Strong foehn winds tend to reduce pollution, while weaker winds may increase it. Our study highlights the impact of foehn events on air quality, providing valuable insights for urban planning and environmental management.
Tanguy Jonville, Maurus Borne, Cyrille Flamant, Juan Cuesta, Olivier Bock, Pierre Bosser, Christophe Lavaysse, Andreas Fink, and Peter Knippertz
EGUsphere, https://doi.org/10.5194/egusphere-2024-3606, https://doi.org/10.5194/egusphere-2024-3606, 2025
Short summary
Short summary
Tropical waves structure the atmosphere. Four types of tropical waves (ER, Kelvin, MRG-TD1, and MRG-TD2) are studied using filters, satellite measurements, and in situ data from the Clouds-Atmosphere Dynamics-Dust Interaction in West Africa (CADDIWA) campaign held in September 2021 in Cabo Verde. ER waves impact temperature and humidity above 2500 m, MRG-TD1 around 3500 m, and MRG-TD2 around 2000 m. Interactions between these waves favor tropical cyclone formation.
Martial Haeffelin, Jean-François Ribaud, Jonnathan Céspedes, Jean-Charles Dupont, Aude Lemonsu, Valéry Masson, Tim Nagel, and Simone Kotthaus
Atmos. Chem. Phys., 24, 14101–14122, https://doi.org/10.5194/acp-24-14101-2024, https://doi.org/10.5194/acp-24-14101-2024, 2024
Short summary
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This study highlights how the state of the urban atmospheric boundary layer impacts urban park cooling effect intensity at night. Under summertime heat wave conditions, the urban atmosphere becomes stable at night, which inhibits turbulent motions. Under those specific conditions, urban parks and woods cool much more efficiently than the surrounding built-up neighbourhoods in the evening and through the night, providing cooler air temperatures by 4 to 6° C depending on park size.
Maciej Karasewicz, Marta Wacławczyk, Pablo Ortiz-Amezcua, Łucja Janicka, Patryk Poczta, Camilla Kassar Borges, and Iwona S. Stachlewska
Atmos. Chem. Phys., 24, 13231–13251, https://doi.org/10.5194/acp-24-13231-2024, https://doi.org/10.5194/acp-24-13231-2024, 2024
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This work concerns analysis of turbulence in the atmospheric boundary layer shortly before sunset. Based on a large set of measurements at a rural and an urban site, we analyze how turbulence properties change in time during rapid decay of convection. We explain the observations using recent theories of non-equilibrium turbulence. The presence of non-equilibrium suggests that classical parametrization schemes fail to predict turbulence statistics shortly before sunset.
Lian Su, Chunsong Lu, Jinlong Yuan, Xiaofei Wang, Qing He, and Haiyun Xia
Atmos. Chem. Phys., 24, 10947–10963, https://doi.org/10.5194/acp-24-10947-2024, https://doi.org/10.5194/acp-24-10947-2024, 2024
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The cold downhill airflow of the Tibetan Plateau leading to the low-level jet weakens the height and intensity of the inversion layer, which reduces the energy demand for the broken inversion layer. The low-level jet causes dust aerosols to accumulate near the ground. The material conditions for the development of the desert atmospheric boundary layer can be quickly transformed into thermal conditions.
Mohammad Allouche, Vladislav I. Sevostianov, Einara Zahn, Mark A. Zondlo, Nelson Luís Dias, Gabriel G. Katul, Jose D. Fuentes, and Elie Bou-Zeid
Atmos. Chem. Phys., 24, 9697–9711, https://doi.org/10.5194/acp-24-9697-2024, https://doi.org/10.5194/acp-24-9697-2024, 2024
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The significance of surface–atmosphere exchanges of aerosol species to atmospheric composition is underscored by their rising concentrations that are modulating the Earth's climate and having detrimental consequences for human health and the environment. Estimating these exchanges, using field measurements, and offering alternative models are the aims here. Limitations in measuring some species misrepresent their actual exchanges, so our proposed models serve to better quantify them.
Andreas Walbröl, Janosch Michaelis, Sebastian Becker, Henning Dorff, Kerstin Ebell, Irina Gorodetskaya, Bernd Heinold, Benjamin Kirbus, Melanie Lauer, Nina Maherndl, Marion Maturilli, Johanna Mayer, Hanno Müller, Roel A. J. Neggers, Fiona M. Paulus, Johannes Röttenbacher, Janna E. Rückert, Imke Schirmacher, Nils Slättberg, André Ehrlich, Manfred Wendisch, and Susanne Crewell
Atmos. Chem. Phys., 24, 8007–8029, https://doi.org/10.5194/acp-24-8007-2024, https://doi.org/10.5194/acp-24-8007-2024, 2024
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To support the interpretation of the data collected during the HALO-(AC)3 campaign, which took place in the North Atlantic sector of the Arctic from 7 March to 12 April 2022, we analyze how unusual the weather and sea ice conditions were with respect to the long-term climatology. From observations and ERA5 reanalysis, we found record-breaking warm air intrusions and a large variety of marine cold air outbreaks. Sea ice concentration was mostly within the climatological interquartile range.
Shai Abir, Hamish A. McGowan, Yonatan Shaked, Hezi Gildor, Efrat Morin, and Nadav G. Lensky
Atmos. Chem. Phys., 24, 6177–6195, https://doi.org/10.5194/acp-24-6177-2024, https://doi.org/10.5194/acp-24-6177-2024, 2024
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Understanding air–sea heat exchange is vital for studying ocean dynamics. Eddy covariance measurements over the Gulf of Eilat revealed a 3.22 m yr-1 evaporation rate, which is inconsistent with bulk formulae estimations in stable atmospheric conditions, requiring bulk formulae to be revisited in these environments. The surface fluxes have a net cooling effect on the gulf water on an annual mean (-79 W m-2), balanced by a strong exchange flux between the Red Sea and the Gulf of Eilat.
Gina C. Jozef, John J. Cassano, Sandro Dahlke, Mckenzie Dice, Christopher J. Cox, and Gijs de Boer
Atmos. Chem. Phys., 24, 1429–1450, https://doi.org/10.5194/acp-24-1429-2024, https://doi.org/10.5194/acp-24-1429-2024, 2024
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Observations collected during MOSAiC were used to identify the range in vertical structure and stability of the central Arctic lower atmosphere through a self-organizing map analysis. Characteristics of wind features (such as low-level jets) and atmospheric moisture features (such as clouds) were analyzed in the context of the varying vertical structure and stability. Thus, the results of this paper give an overview of the thermodynamic and kinematic features of the central Arctic atmosphere.
Elisa F. Akansu, Sandro Dahlke, Holger Siebert, and Manfred Wendisch
Atmos. Chem. Phys., 23, 15473–15489, https://doi.org/10.5194/acp-23-15473-2023, https://doi.org/10.5194/acp-23-15473-2023, 2023
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The height of the mixing layer is an important measure of the surface-level distribution of energy or other substances. The experimental determination of this height is associated with large uncertainties, particularly under stable conditions that we often find during the polar night or in the presence of clouds. We present a reference method using turbulence measurements on a tethered balloon, which allows us to evaluate approaches based on radiosondes or surface observations.
Ulrike Egerer, Holger Siebert, Olaf Hellmuth, and Lise Lotte Sørensen
Atmos. Chem. Phys., 23, 15365–15373, https://doi.org/10.5194/acp-23-15365-2023, https://doi.org/10.5194/acp-23-15365-2023, 2023
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Low-level jets (LLJs) are strong winds near the surface and occur frequently in the Arctic in stable conditions. Using tethered-balloon profile measurements in Greenland, we analyze a multi-hour period with an LLJ that later weakens and finally collapses. Increased shear-induced turbulence at the LLJ bounds mostly does not reach the ground until the LLJ collapses. Our findings support the hypothesis that a passive tracer can be advected with an LLJ and mixed down when the LLJ collapses.
Dean Henze, David Noone, and Darin Toohey
Atmos. Chem. Phys., 23, 15269–15288, https://doi.org/10.5194/acp-23-15269-2023, https://doi.org/10.5194/acp-23-15269-2023, 2023
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The interaction between biomass burning aerosols and clouds remains challenging to accurately determine from observations. This is in part because of difficulties distinguishing aerosol differences due to precipitation versus dilution processes from the observations. This study addresses the challenge by utilizing atmospheric heavy water isotope ratios to constrain mixing versus precipitation processes during a field campaign (ORACLES) and in turn explain observed aerosol concentrations.
Zefan Ju, Jian Rao, Yue Wang, Junfeng Yang, and Qian Lu
Atmos. Chem. Phys., 23, 14903–14918, https://doi.org/10.5194/acp-23-14903-2023, https://doi.org/10.5194/acp-23-14903-2023, 2023
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In the paper, we explored the impact of the Madden–Julian Oscillation (MJO) and the Quasi-Biennial Oscillation (QBO) on East China summer rainfall variability. It is novel to find that the combined impact of MJO and QBO is not maximized when the QBO and MJO are in phase to enhance (or suppress) the tropical convection.
Gina C. Jozef, John J. Cassano, Sandro Dahlke, Mckenzie Dice, Christopher J. Cox, and Gijs de Boer
Atmos. Chem. Phys., 23, 13087–13106, https://doi.org/10.5194/acp-23-13087-2023, https://doi.org/10.5194/acp-23-13087-2023, 2023
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Observations from the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) were used to determine the frequency of occurrence of various central Arctic lower atmospheric stability regimes and how the stability regimes transition between each other. Wind and radiation observations were analyzed in the context of stability regime and season to reveal the relationships between Arctic atmospheric stability and mechanically and radiatively driven turbulent forcings.
Jia Shao, Jian Zhang, Wuke Wang, Shaodong Zhang, Tao Yu, and Wenjun Dong
Atmos. Chem. Phys., 23, 12589–12607, https://doi.org/10.5194/acp-23-12589-2023, https://doi.org/10.5194/acp-23-12589-2023, 2023
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Kelvin–Helmholtz instability (KHI) is indicated by the critical value of the Richardson (Ri) number, which is usually predicted to be 1/4. Compared to high-resolution radiosondes, the threshold value of Ri could be approximated as 1 rather than 1/4 when using ERA5-based Ri as a proxy for KHI. The occurrence frequency of subcritical Ri exhibits significant seasonal cycles over all climate zones and is closely associated with gravity waves and background flows.
Shijie Peng, Qinghua Yang, Matthew D. Shupe, Xingya Xi, Bo Han, Dake Chen, Sandro Dahlke, and Changwei Liu
Atmos. Chem. Phys., 23, 8683–8703, https://doi.org/10.5194/acp-23-8683-2023, https://doi.org/10.5194/acp-23-8683-2023, 2023
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Due to a lack of observations, the structure of the Arctic atmospheric boundary layer (ABL) remains to be further explored. By analyzing a year-round radiosonde dataset collected over the Arctic sea-ice surface, we found the annual cycle of the ABL height (ABLH) is primarily controlled by the evolution of ABL thermal structure, and the surface conditions also show a high correlation with ABLH variation. In addition, the Arctic ABLH is found to be decreased in summer compared with 20 years ago.
Dmitry G. Chechin, Christof Lüpkes, Jörg Hartmann, André Ehrlich, and Manfred Wendisch
Atmos. Chem. Phys., 23, 4685–4707, https://doi.org/10.5194/acp-23-4685-2023, https://doi.org/10.5194/acp-23-4685-2023, 2023
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Clouds represent a very important component of the Arctic climate system, as they strongly reduce the amount of heat lost to space from the sea ice surface. Properties of clouds, as well as their persistence, strongly depend on the complex interaction of such small-scale properties as phase transitions, radiative transfer and turbulence. In this study we use airborne observations to learn more about the effect of clouds and radiative cooling on turbulence in comparison with other factors.
Noviana Dewani, Mirjana Sakradzija, Linda Schlemmer, Ronny Leinweber, and Juerg Schmidli
Atmos. Chem. Phys., 23, 4045–4058, https://doi.org/10.5194/acp-23-4045-2023, https://doi.org/10.5194/acp-23-4045-2023, 2023
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A high daily variability of the normalized vertical velocity variance profiles in the convective boundary layer is observed using Doppler lidar data during the FESSTVaL campaign 2020–2021. The dependency of the normalized vertical velocity variance on several meteorological parameters explains that the moisture processes in the boundary layer contribute to the remaining variability. The finding suggests that a new vertical velocity scale that takes moist processes into account has to be defined.
Xiangde Xu, Yi Tang, Yinjun Wang, Hongshen Zhang, Ruixia Liu, and Mingyu Zhou
Atmos. Chem. Phys., 23, 3299–3309, https://doi.org/10.5194/acp-23-3299-2023, https://doi.org/10.5194/acp-23-3299-2023, 2023
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The vertical motion over the Tibetan Plateau (TP) is associated with the anomalous convective activities. The diurnal variations and formation mechanisms of low clouds over the TP, Rocky Mountains and low-elevation regions are analyzed. We further discuss whether there exists a
high-efficiencytriggering mechanism for convection over the TP and whether there is an association among low air density and strong turbulence and ubiquitous popcorn-like cumulus clouds.
Lejiang Yu, Shiyuan Zhong, Timo Vihma, Cuijuan Sui, and Bo Sun
Atmos. Chem. Phys., 23, 345–353, https://doi.org/10.5194/acp-23-345-2023, https://doi.org/10.5194/acp-23-345-2023, 2023
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Previous studies have noted a significant relationship between the Subtropical Indian Ocean Dipole and the South Atlantic Ocean Dipole indices, but little is known about the stability of their relationship. We found a significant positive correlation between the two indices prior to the year 2000 but an insignificant correlation afterwards.
Si Cheng, Jianguo Wang, Li Cai, Mi Zhou, Rui Su, Yijun Huang, and Quanxin Li
Atmos. Chem. Phys., 22, 10045–10059, https://doi.org/10.5194/acp-22-10045-2022, https://doi.org/10.5194/acp-22-10045-2022, 2022
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This paper helps to improve the recognition of severe thunderstorms in advance by giving a general understanding of how long the storm lasts, how fast the cluster moves and how much area the storm affects via information about the kinematic features of thunderstorms, which are the duration, valid area, the velocity, the direction and the farthest distance, and ideally to establish a foundation for future research that may contribute to the development of a new or improved prediction paradigm.
Hongyou Liu, Yanxiong Shi, and Xiaojing Zheng
Atmos. Chem. Phys., 22, 8787–8803, https://doi.org/10.5194/acp-22-8787-2022, https://doi.org/10.5194/acp-22-8787-2022, 2022
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The sandstorm, which is a common natural disaster, is mechanically characterized by a particle-laden flow experiencing wall turbulence. This work investigates a real sandstorm that was measured at the Qingtu Lake Observation Array through a lens of wall-turbulent flow dynamics. A non-stationary signal processing method is proposed based on the time-varying mean and adaptive segmented stationary method, and the evolution of turbulent kinetic energy during the entire sandstorm process is revealed.
Simon Kirschler, Christiane Voigt, Bruce Anderson, Ramon Campos Braga, Gao Chen, Andrea F. Corral, Ewan Crosbie, Hossein Dadashazar, Richard A. Ferrare, Valerian Hahn, Johannes Hendricks, Stefan Kaufmann, Richard Moore, Mira L. Pöhlker, Claire Robinson, Amy J. Scarino, Dominik Schollmayer, Michael A. Shook, K. Lee Thornhill, Edward Winstead, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 22, 8299–8319, https://doi.org/10.5194/acp-22-8299-2022, https://doi.org/10.5194/acp-22-8299-2022, 2022
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In this study we show that the vertical velocity dominantly impacts the cloud droplet number concentration (NC) of low-level clouds over the western North Atlantic in the winter and summer season, while the cloud condensation nuclei concentration, aerosol size distribution and chemical composition impact NC within a season. The observational data presented in this study can evaluate and improve the representation of aerosol–cloud interactions for a wide range of conditions.
Klaus Gierens, Lena Wilhelm, Sina Hofer, and Susanne Rohs
Atmos. Chem. Phys., 22, 7699–7712, https://doi.org/10.5194/acp-22-7699-2022, https://doi.org/10.5194/acp-22-7699-2022, 2022
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We are interested in the prediction of condensation trails, in particular strong ones. For this we need a good forecast of temperature and humidity in the levels where aircraft cruise. Unfortunately, the humidity forecast is quite difficult for these levels, in particular the ice supersaturation, which is needed for long-lasting contrails. We are thus seeking proxy variables that help distinguish situations where strong contrails can form, for instance the lapse rate.
Ada Mariska Koning, Louise Nuijens, Christian Mallaun, Benjamin Witschas, and Christian Lemmerz
Atmos. Chem. Phys., 22, 7373–7388, https://doi.org/10.5194/acp-22-7373-2022, https://doi.org/10.5194/acp-22-7373-2022, 2022
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Wind measurements from the mixed layer to cloud tops are scarce, causing a lack of knowledge on wind mixing between and within these layers. We use airborne observations of wind profiles and local wind at high frequency to study wind transport in cloud fields. A case with thick clouds had its maximum transport in the cloud layer, caused by eddies > 700 m, which was not expected from turbulence theory. In other cases large eddies undid transport of smaller eddies resulting in no net transport.
Markus Geldenhuys, Peter Preusse, Isabell Krisch, Christoph Zülicke, Jörn Ungermann, Manfred Ern, Felix Friedl-Vallon, and Martin Riese
Atmos. Chem. Phys., 21, 10393–10412, https://doi.org/10.5194/acp-21-10393-2021, https://doi.org/10.5194/acp-21-10393-2021, 2021
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A large-scale gravity wave (GW) was observed spanning the whole of Greenland. The GWs proposed in this paper come from a new jet–topography mechanism. The topography compresses the flow and triggers a change in u- and
v-wind components. The jet becomes out of geostrophic balance and sheds energy in the form of GWs to restore the balance. This topography–jet interaction was not previously considered by the community, rendering the impact of the gravity waves largely unaccounted for.
Kristina Pistone, Paquita Zuidema, Robert Wood, Michael Diamond, Arlindo M. da Silva, Gonzalo Ferrada, Pablo E. Saide, Rei Ueyama, Ju-Mee Ryoo, Leonhard Pfister, James Podolske, David Noone, Ryan Bennett, Eric Stith, Gregory Carmichael, Jens Redemann, Connor Flynn, Samuel LeBlanc, Michal Segal-Rozenhaimer, and Yohei Shinozuka
Atmos. Chem. Phys., 21, 9643–9668, https://doi.org/10.5194/acp-21-9643-2021, https://doi.org/10.5194/acp-21-9643-2021, 2021
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Using aircraft-based measurements off the Atlantic coast of Africa, we found the springtime smoke plume was strongly correlated with the amount of water vapor in the atmosphere (more smoke indicated more humidity). We see the same general feature in satellite-assimilated and free-running models. Our analysis suggests this relationship is not caused by the burning but originates due to coincident continental meteorology plus fires. This air is transported over the ocean without further mixing.
Markku Kulmala, Tom V. Kokkonen, Juha Pekkanen, Sami Paatero, Tuukka Petäjä, Veli-Matti Kerminen, and Aijun Ding
Atmos. Chem. Phys., 21, 8313–8322, https://doi.org/10.5194/acp-21-8313-2021, https://doi.org/10.5194/acp-21-8313-2021, 2021
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The eastern part of China as a whole is practically a gigacity with 650 million inhabitants. The gigacity, with its emissions, processes in the pollution cocktail and numerous feedbacks and interactions, has a crucial and big impact on regional air quality and on global climate. A large-scale research and innovation program is needed to meet the interlinked grand challenges in this gigacity and to serve as a platform for finding pathways for sustainable development of the globe.
Yunyan Jiang, Jinyuan Xin, Ying Wang, Guiqian Tang, Yuxin Zhao, Danjie Jia, Dandan Zhao, Meng Wang, Lindong Dai, Lili Wang, Tianxue Wen, and Fangkun Wu
Atmos. Chem. Phys., 21, 6111–6128, https://doi.org/10.5194/acp-21-6111-2021, https://doi.org/10.5194/acp-21-6111-2021, 2021
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Multiscale-circulation coupling affects pollution by changing the planetary boundary layer (PBL) structure. The multilayer PBL under cyclonic circulation has no diurnal variation; the temperature inversion and zero-speed zone can reach 600–900 m with strong mountain winds. The monolayer PBL under southwestern circulation can reach 2000 m; the inversion is lower than nocturnal PBL (400 m) with strong ambient winds. The zonal winds' vertical shear produces the inversion under western circulation.
Dillon S. Dodson and Jennifer D. Small Griswold
Atmos. Chem. Phys., 21, 1937–1961, https://doi.org/10.5194/acp-21-1937-2021, https://doi.org/10.5194/acp-21-1937-2021, 2021
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The results here reinforce findings from previous in situ studies of the marine boundary layer. It is found that turbulence is maximized in the middle of the stratocumulus layer from latent heating effects. Precipitation acts to increase turbulence in the sub-cloud layer, while acting to stabilize the entire boundary layer after the evaporation of precipitation in the sub-cloud has stopped. A negative correlation is present between the boundary layer height and turbulence.
Ju Li, Zhaobin Sun, Donald H. Lenschow, Mingyu Zhou, Youjun Dou, Zhigang Cheng, Yaoting Wang, and Qingchun Li
Atmos. Chem. Phys., 20, 15793–15809, https://doi.org/10.5194/acp-20-15793-2020, https://doi.org/10.5194/acp-20-15793-2020, 2020
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We analyzed a haze front event involving warm–dry downslope flow in December 2015 in Beijing, China. The haze front was formed by the collision between a clean warm–dry air mass flowing from a nearby mountainous region and a polluted cold–wet air mass over an urban area. We found that the polluted air advanced toward the clean air, resulting in a severe air pollution event. Our study highlights the need to further investigate the warm–dry downslope and its impacts on air pollution.
Sonja Gisinger, Johannes Wagner, and Benjamin Witschas
Atmos. Chem. Phys., 20, 10091–10109, https://doi.org/10.5194/acp-20-10091-2020, https://doi.org/10.5194/acp-20-10091-2020, 2020
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Gravity waves are an important coupling mechanism in the atmosphere. Measurements by two research aircraft during a mountain wave event over Scandinavia in 2016 revealed changes of the horizontal scales in the vertical velocity field and of momentum fluxes in the vicinity of the tropopause inversion. Idealized simulations revealed the presence of interfacial waves. They are found downstream of the mountain peaks, meaning that they horizontally transport momentum/energy away from their source.
Rayonil G. Carneiro and Gilberto Fisch
Atmos. Chem. Phys., 20, 5547–5558, https://doi.org/10.5194/acp-20-5547-2020, https://doi.org/10.5194/acp-20-5547-2020, 2020
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The objective of this study was to conduct observational evaluations of the daily cycle of the height of the planetary boundary layer from data that were measured and/or estimated using instruments such as a radiosonde, sodar, ceilometer, wind profiler, lidar and microwave radiometer installed in the central Amazon during 2014 (considered a typical year) and 2015 during which an intense El Niño–Southern Oscillation (ENSO) event predominated during the GoAmazon experiment.
Maurício I. Oliveira, Otávio C. Acevedo, Matthias Sörgel, Ernani L. Nascimento, Antonio O. Manzi, Pablo E. S. Oliveira, Daiane V. Brondani, Anywhere Tsokankunku, and Meinrat O. Andreae
Atmos. Chem. Phys., 20, 15–27, https://doi.org/10.5194/acp-20-15-2020, https://doi.org/10.5194/acp-20-15-2020, 2020
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In this study, data collected during four deep convection events at the 80 m tower from the Amazon Tall Tower Observatory are analyzed. It provides a unique view on how such events affect the local boundary layer and how it recovers after their passage. Quantities analyzed include mean wind speed, virtual potential temperature, turbulent kinetic energy, sensible, and latent heat fluxes. A conceptual model for boundary layer structure along the passage of deep convection events is proposed.
Zhicong Yin, Bufan Cao, and Huijun Wang
Atmos. Chem. Phys., 19, 13933–13943, https://doi.org/10.5194/acp-19-13933-2019, https://doi.org/10.5194/acp-19-13933-2019, 2019
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Ozone occurs both in the stratosphere and at ground level. Surface ozone is a man-made air pollutant and has harmful effects on people and the environment. Two dominant patterns of summer ozone pollution were determined. The most dominant pattern in 2017 and 2018 was different from that in previous years. The findings of this study help us to understand the features of surface ozone pollution in eastern China and their relationships with large-scale atmospheric circulations.
Karmen Babić, Norbert Kalthoff, Bianca Adler, Julian F. Quinting, Fabienne Lohou, Cheikh Dione, and Marie Lothon
Atmos. Chem. Phys., 19, 13489–13506, https://doi.org/10.5194/acp-19-13489-2019, https://doi.org/10.5194/acp-19-13489-2019, 2019
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This study investigates differences in atmospheric conditions between nights with and without low-level stratus clouds (LLCs) over southern West Africa. We use high-quality observations collected during 2016 summer monsoon season and the ERA5 reanalysis data set. Our results show that the formation of LLCs depends on the interplay between the onset time and strength of the nocturnal low-level jet, horizontal cold-air advection, and the overall moisture level in the whole region.
Justine Ringard, Marjolaine Chiriaco, Sophie Bastin, and Florence Habets
Atmos. Chem. Phys., 19, 13129–13155, https://doi.org/10.5194/acp-19-13129-2019, https://doi.org/10.5194/acp-19-13129-2019, 2019
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This study characterizes the changes observed at Paris urban scale and attempts to identify the surface–atmosphere feedbacks likely to explain the trends observed as a function of the different configurations of large-scale dynamics. This article is interested in several atmospheric parameters and their possible retroactions. Finally, to study urban environments, the analysis at the local scale is essential because it is very poorly represented in the model.
Jesús Yus-Díez, Mireia Udina, Maria Rosa Soler, Marie Lothon, Erik Nilsson, Joan Bech, and Jielun Sun
Atmos. Chem. Phys., 19, 9495–9514, https://doi.org/10.5194/acp-19-9495-2019, https://doi.org/10.5194/acp-19-9495-2019, 2019
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This study helps improve the understanding of the turbulence description and the interactions occurring in the lower part of the boundary layer. It is carried out at an orographically influenced site close to the Pyrenees to explore the hockey-stick transition (HOST) theory. HOST is seen to be strongly dependent on both the meteorological conditions and the orographic features. Examples of intermittent turbulence events that lead to transitions between the turbulence regimes are also identified.
Cheikh Dione, Fabienne Lohou, Marie Lothon, Bianca Adler, Karmen Babić, Norbert Kalthoff, Xabier Pedruzo-Bagazgoitia, Yannick Bezombes, and Omar Gabella
Atmos. Chem. Phys., 19, 8979–8997, https://doi.org/10.5194/acp-19-8979-2019, https://doi.org/10.5194/acp-19-8979-2019, 2019
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Low atmospheric dynamics and low-level cloud (LLC) macrophysical properties are analyzed using in situ and remote sensing data collected from 20 June to 30 July at Savè, Benin, during the DACCIWA field campaign in 2016. We find that the low-level jet (LLJ), LLCs, monsoon flow, and maritime inflow reveal a day-to-day variability. LLCs form at the same level as the jet core height. The cloud base height is stationary at night and remains below the jet. The cloud top height is found above the jet.
Dani J. Caputi, Ian Faloona, Justin Trousdell, Jeanelle Smoot, Nicholas Falk, and Stephen Conley
Atmos. Chem. Phys., 19, 4721–4740, https://doi.org/10.5194/acp-19-4721-2019, https://doi.org/10.5194/acp-19-4721-2019, 2019
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This paper covers the importance of understanding ozone pollution in California’s southern San Joaquin Valley from the perspective of meteorological conditions that occur overnight. Our main finding is that stronger winds aloft allow ozone to be depleted overnight, leading to less ozone the following day. This finding has the potential to greatly improve ozone forecasts in the San Joaquin Valley. This study is primarily conducted with aircraft observations.
Jon Ander Arrillaga, Carlos Yagüe, Carlos Román-Cascón, Mariano Sastre, Maria Antonia Jiménez, Gregorio Maqueda, and Jordi Vilà-Guerau de Arellano
Atmos. Chem. Phys., 19, 4615–4635, https://doi.org/10.5194/acp-19-4615-2019, https://doi.org/10.5194/acp-19-4615-2019, 2019
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Thermally driven downslope winds develop in mountainous areas under a weak large-scale forcing and clear skies. In this work, we find that their onset time and intensity are closely connected with both the large-scale wind and soil moisture. We also show how the distinct downslope intensities shape the turbulent and thermal features of the nocturnal atmosphere. The analysis concludes that the downslope–turbulence interaction and the horizontal transport explain the important CO2 variability.
Étienne Vignon, Olivier Traullé, and Alexis Berne
Atmos. Chem. Phys., 19, 4659–4683, https://doi.org/10.5194/acp-19-4659-2019, https://doi.org/10.5194/acp-19-4659-2019, 2019
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The future sea-level rise will depend on how much the Antarctic ice sheet gain – via precipitation – or loose mass. The simulation of precipitation by numerical models used for projections depends on the representation of the atmospheric circulation over and around Antarctica. Using daily measurements from balloon soundings at nine Antarctic stations, this study characterizes the structure of the atmosphere over the Antarctic coast and its representation in atmospheric simulations.
Nicola Bodini, Julie K. Lundquist, Raghavendra Krishnamurthy, Mikhail Pekour, Larry K. Berg, and Aditya Choukulkar
Atmos. Chem. Phys., 19, 4367–4382, https://doi.org/10.5194/acp-19-4367-2019, https://doi.org/10.5194/acp-19-4367-2019, 2019
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To improve the parameterization of the turbulence dissipation rate (ε) in numerical weather prediction models, we have assessed its temporal and spatial variability at various scales in the Columbia River Gorge during the WFIP2 field experiment. The turbulence dissipation rate shows large spatial variability, even at the microscale, with larger values in sites located downwind of complex orographic structures or in wind farm wakes. Distinct diurnal and seasonal cycles in ε have also been found.
Frederick Letson, Rebecca J. Barthelmie, Weifei Hu, and Sara C. Pryor
Atmos. Chem. Phys., 19, 3797–3819, https://doi.org/10.5194/acp-19-3797-2019, https://doi.org/10.5194/acp-19-3797-2019, 2019
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Wind gusts are a key driver of aerodynamic loading, and common approximations used to describe wind gust behavior may not be appropriate in complex terrain at heights relevant to wind turbines and other structures. High-resolution observations from sonic anemometers and vertically pointing Doppler lidars collected in the Perdigão experiment are analyzed to provide a foundation for improved wind gust characterization in complex terrain.
Rohit Chakraborty, Madineni Venkat Ratnam, and Shaik Ghouse Basha
Atmos. Chem. Phys., 19, 3687–3705, https://doi.org/10.5194/acp-19-3687-2019, https://doi.org/10.5194/acp-19-3687-2019, 2019
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Intense convective phenomena are a common climatic feature in the Indian tropical region which occur during the pre-monsoon to post-monsoon seasons (April–October) and are generally accompanied by intense thunderstorms, lightning, and wind gusts with heavy rainfall. Here we show long-term trends of the parameters related to convection and instability obtained from 27 radiosonde stations across six subdivisions over the Indian region during the period 1980–2016.
Kunihiko Kodera, Nawo Eguchi, Rei Ueyama, Yuhji Kuroda, Chiaki Kobayashi, Beatriz M. Funatsu, and Chantal Claud
Atmos. Chem. Phys., 19, 2655–2669, https://doi.org/10.5194/acp-19-2655-2019, https://doi.org/10.5194/acp-19-2655-2019, 2019
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The recent cooling of the equatorial eastern Pacific Ocean occurred in conjunction with enhanced cross-equatorial southerlies associated with a strengthening of the boreal summer Hadley circulation. A combination of land surface warming and reduced static stability in the tropical tropopause layer due to stratospheric cooling is suggested to have caused the increase in the deep ascending branch of the Hadley circulation and related recent decadal change in the tropical troposphere and ocean.
Karmen Babić, Bianca Adler, Norbert Kalthoff, Hendrik Andersen, Cheikh Dione, Fabienne Lohou, Marie Lothon, and Xabier Pedruzo-Bagazgoitia
Atmos. Chem. Phys., 19, 1281–1299, https://doi.org/10.5194/acp-19-1281-2019, https://doi.org/10.5194/acp-19-1281-2019, 2019
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The first detailed observational analysis of the complete diurnal cycle of low-level clouds (LLC) and associated atmospheric processes over southern West Africa is performed using the data gathered within the DACCIWA (Dynamics-Aerosol-Chemistry-Cloud-Interactions in West Africa) ground-based campaign. We find cooling related to the horizontal advection, which occurs in connection with the inflow of cool maritime air mass and a prominent low-level jet, to have the dominant role in LLC formation.
Bianca Adler, Karmen Babić, Norbert Kalthoff, Fabienne Lohou, Marie Lothon, Cheikh Dione, Xabier Pedruzo-Bagazgoitia, and Hendrik Andersen
Atmos. Chem. Phys., 19, 663–681, https://doi.org/10.5194/acp-19-663-2019, https://doi.org/10.5194/acp-19-663-2019, 2019
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This study deals with nocturnal stratiform low-level clouds that frequently form in the atmospheric boundary layer over southern West Africa. We use observational data from 11 nights to characterize the clouds and intranight variability of boundary layer conditions as well as to assess the physical processes relevant for cloud formation. We find that cooling is crucial to reach saturation and a large part of the cooling is related to horizontal advection of cool air from the Gulf of Guinea.
Jutta Vüllers, Georg J. Mayr, Ulrich Corsmeier, and Christoph Kottmeier
Atmos. Chem. Phys., 18, 18169–18186, https://doi.org/10.5194/acp-18-18169-2018, https://doi.org/10.5194/acp-18-18169-2018, 2018
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This paper investigates frequently occurring foehn at the Dead Sea, which strongly impacts the local climatic conditions, in particular temperature and humidity, as well as evaporation from the Dead Sea, the aerosol load, and visibility. A statistical classification exposes two types of foehn and first-time, high-resolution measurements reveal trigger mechanisms and relevant characteristics, such as wind velocities, affected air layers, and resulting phenomena such as hydraulic jumps and rotors.
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de Roode, S. R., Frederikse, T., Siebesma, A. P., Ackerman, A. S., Chylik, J., Field, P. R., Fricke, J., Gryschka, M., Hill, A., Honnert, R., Krueger, S. K., Lac, C., Lesage, A. T., and Tomassini, L.: Turbulent Transport in the Gray Zone: A Large Eddy Model Intercomparison Study of the CONSTRAIN Cold Air Outbreak Case, J. Adv. Model. Earth Sy., 11, 597–623, https://doi.org/10.1029/2018MS001443, 2019. a
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Short summary
The Arctic is warming faster than the rest of the globe. Warm-air intrusions (WAIs) into the Arctic may play an important role in explaining this phenomenon. Cold-air outbreaks (CAOs) out of the Arctic may link the Arctic climate changes to mid-latitude weather. In our article, we describe how to observe air mass transformations during CAOs and WAIs using three research aircraft instrumented with state-of-the-art remote-sensing and in situ measurement devices.
The Arctic is warming faster than the rest of the globe. Warm-air intrusions (WAIs) into the...
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