Articles | Volume 16, issue 19
Atmos. Chem. Phys., 16, 12753–12765, 2016

Special issue: NETCARE (Network on Aerosols and Climate: Addressing Key Uncertainties...

Atmos. Chem. Phys., 16, 12753–12765, 2016

Research article 13 Oct 2016

Research article | 13 Oct 2016

Temporal and spectral cloud screening of polar winter aerosol optical depth (AOD): impact of homogeneous and inhomogeneous clouds and crystal layers on climatological-scale AODs

Norman T. O'Neill1, Konstantin Baibakov1,2, Sareh Hesaraki1, Liviu Ivanescu1, Randall V. Martin3, Chris Perro3, Jai P. Chaubey1, Andreas Herber4, and Thomas J. Duck3 Norman T. O'Neill et al.
  • 1Centre d'Applications et de Recherches en Télédétection, Université de Sherbrooke, Sherbrooke, Canada
  • 2National Research Council Canada, Flight Research Laboratory, Ottawa, Canada
  • 3Dept. of Physics and Atmospheric Science, Dalhousie University, Halifax, Canada
  • 4Alfred Wegener Institute for Polar and Marine Research, Bremerhaven, Germany

Abstract. We compared star-photometry-derived, polar winter aerosol optical depths (AODs), acquired at Eureka, Nunavut, Canada, and Ny-Ålesund, Svalbard, with GEOS-Chem (GC) simulations as well as ground-based lidar and CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) retrievals over a sampling period of two polar winters. The results indicate significant cloud and/or low-altitude ice crystal (LIC) contamination which is only partially corrected using temporal cloud screening. Spatially homogeneous clouds and LICs that remain after temporal cloud screening represent an inevitable systematic error in the estimation of AOD: this error was estimated to vary from 78 to 210 % at Eureka and from 2 to 157 % at Ny-Ålesund. Lidar analysis indicated that LICs appeared to have a disproportionately large influence on the homogeneous coarse-mode optical depths that escape temporal cloud screening. In principle, spectral cloud screening (to yield fine-mode or submicron AODs) reduces pre-cloud-screened AODs to the aerosol contribution if one assumes that coarse-mode (super-micron) aerosols are a minor part of the AOD. Large, low-frequency differences between these retrieved values and their GC analogue appeared to be often linked to strong, spatially extensive planetary boundary layer events whose presence at either site was inferred from CALIOP profiles. These events were either not captured or significantly underestimated by the GC simulations. High-frequency AOD variations of GC fine-mode aerosols at Ny-Ålesund were attributed to sea salt, while low-frequency GC variations at Eureka and Ny-Ålesund were attributable to sulfates. CALIOP profiles and AODs were invaluable as spatial and temporal redundancy support (or, alternatively, as insightful points of contention) for star photometry retrievals and GC estimates of AOD.

Final-revised paper