Articles | Volume 23, issue 21
https://doi.org/10.5194/acp-23-13911-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-13911-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
08 Nov 2023
Research article |
| 08 Nov 2023
| 08 Nov 2023
Biomass-burning smoke's properties and its interactions with marine stratocumulus clouds in WRF-CAM5 and southeastern Atlantic field campaigns
Dept. of Atmospheric and Oceanic Sciences, University of California, Los Angeles, CA 90095, USA
Pablo E. Saide
Dept. of Atmospheric and Oceanic Sciences, University of California, Los Angeles, CA 90095, USA
Institute of the Environment and Sustainability, University of California–Los Angeles, Los Angeles, CA 90095-1496, USA
Dept. of Earth and Environmental Science, University of Manchester, Manchester, M13 9PL, UK
Amie Dobracki
Dept. of Atmospheric Sciences, Rosenstiel School of Marine, Atmospheric, and Earth Science, University of Miami, Miami, FL 33149, USA
Steffen Freitag
State Agency for Nature, Environment, and Consumer Protection, 45659 Essen, North Rhine-Westphalia, Germany
Jim M. Haywood
Dept. of Mathematics and Statistics, University of Exeter, Exeter, EX4 4PY, UK
Steven G. Howell
Dept. of Oceanography, University of Hawaii Manoa, Honolulu, HI 96822, USA
Siddhant Gupta
Brookhaven National Laboratory, Upton, NY 11973, USA
Janek Uin
Brookhaven National Laboratory, Upton, NY 11973, USA
Mary Kacarab
School of Earth and Atmospheric Sciences, Georgia Institute of Technology, Atlanta, GA 30332, USA
Chongai Kuang
Brookhaven National Laboratory, Upton, NY 11973, USA
L. Ruby Leung
Pacific Northwest National Laboratory, Richland, WA 99354, USA
Athanasios Nenes
School of Architecture, Civil & Environmental Engineering, Swiss Federal Institute of Technology, 1015 Lausanne, Switzerland
Institute of Chemical Engineering Sciences, Foundation for Research and Technology Hellas, Patras, 26504, Greece
School of Earth and Atmospheric Sciences, Georgia Institute of Technology, Atlanta, GA 30332, USA
Greg M. McFarquhar
School of Meteorology, University of Oklahoma, Norman, OK 73072, USA
Cooperative Institute for Severe and High Impact Weather Research and Operations (CIWRO), University of Oklahoma, Norman, OK 73072, USA
James Podolske
NASA/Ames Research Center, Moffett Field, CA 94035, USA
Jens Redemann
School of Meteorology, University of Oklahoma, Norman, OK 73072, USA
Arthur J. Sedlacek
Brookhaven National Laboratory, Upton, NY 11973, USA
Kenneth L. Thornhill
NASA Langley Research Center, Hampton, VA 23666, USA
Jenny P. S. Wong
School of Earth and Atmospheric Sciences, Georgia Institute of Technology, Atlanta, GA 30332, USA
Robert Wood
Dept. of Atmospheric Sciences, University of Washington, Seattle, WA 98195, USA
Huihui Wu
Dept. of Earth and Environmental Science, University of Manchester, Manchester, M13 9PL, UK
Yang Zhang
Dept. of Civil and Environmental Engineering, Northeastern University, Boston, MA 02115, USA
Jianhao Zhang
Chemical Sciences Laboratory, National Oceanic and Atmospheric Administration (NOAA), Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO 80305, USA
Paquita Zuidema
Dept. of Atmospheric Sciences, Rosenstiel School of Marine, Atmospheric, and Earth Science, University of Miami, Miami, FL 33149, USA
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This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Olivia Mae Jackson, Aristeidis Voliotis, Thomas J. Bannan, Simon P. O'Meara, Gordon McFiggans, Dave Johnson, and Hugh Coe
EGUsphere, https://doi.org/10.5194/egusphere-2024-2380, https://doi.org/10.5194/egusphere-2024-2380, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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The paper details a method of measuring volatility of pesticides using chemical ionisation mass spectrometry (CIMS) to calculate vapour pressure. This was then compared to current literature values and commonly used models. The exact nature of the literature values often remain uncertain due to being hidden in industrial reports. The results show that the method used primarily matches current literature values and any difference can be explained by method differences either in the methodology.
Pamela A. Dominutti, Jean-Luc Jaffrezo, Anouk Marsal, Takoua Mhadhbi, Rhabira Elazzouzi, Camille Rak, Fabrizia Cavalli, Jean-Philippe Putaud, Aikaterini Bougiatioti, Nikolaos Mihalopoulos, Despina Paraskevopoulou, Ian S. Mudway, Athanasios Nenes, Kaspar R. Daellenbach, Catherine Banach, Steven J. Campbell, Hana Cigánková, Daniele Contini, Greg Evans, Maria Georgopoulou, Manuella Ghanem, Drew A. Glencross, Maria Rachele Guascito, Hartmut Herrmann, Saima Iram, Maja Jovanović, Milena Jovašević-Stojanović, Markus Kalberer, Ingeborg M. Kooter, Suzanne E. Paulson, Anil Patel, Esperanza Perdrix, Maria Chiara Pietrogrande, Pavel Mikuška, Jean-Jacques Sauvain, Aikaterina Seitanidi, Pourya Shahpoury, Eduardo J. S. Souza, Sarah Steimer, Svetlana Stevanovic, Guillaume Suarez, P. S. Ganesh Subramanian, Battist Utinger, Marloes F. van Os, Vishal Verma, Xing Wang, Rodney J. Weber, Yuhan Yang, Xavier Querol, Gerard Hoek, Roy M. Harrison, and Gaëlle Uzu
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2024-107, https://doi.org/10.5194/amt-2024-107, 2024
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Atmos. Chem. Phys., 24, 7983–8005, https://doi.org/10.5194/acp-24-7983-2024, https://doi.org/10.5194/acp-24-7983-2024, 2024
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The springtime southeast Atlantic atmosphere contains lots of smoke from continental fires. This smoke travels with water vapor; more smoke means more humidity. We use aircraft observations and models to describe how the values change through the season and over the region. We sort the atmosphere into different types by vertical structure and amount of smoke and humidity. Since our work shows how frequently these components coincide, it helps to better quantify heating effects over this region.
Kerry Meyer, Steven Platnick, G. Thomas Arnold, Nandana Amarasinghe, Daniel Miller, Jennifer Small-Griswold, Mikael Witte, Brian Cairns, Siddhant Gupta, Greg McFarquhar, and Joseph O'Brien
EGUsphere, https://doi.org/10.5194/egusphere-2024-2021, https://doi.org/10.5194/egusphere-2024-2021, 2024
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Alexandros Milousis, Klaus Klingmüller, Alexandra P. Tsimpidi, Jasper F. Kok, Maria Kanakidou, Athanasios Nenes, and Vlassis A. Karydis
EGUsphere, https://doi.org/10.5194/egusphere-2024-1579, https://doi.org/10.5194/egusphere-2024-1579, 2024
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Atmos. Chem. Phys., 24, 7331–7345, https://doi.org/10.5194/acp-24-7331-2024, https://doi.org/10.5194/acp-24-7331-2024, 2024
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Human activities release copious amounts of small particles called aerosols into the atmosphere. These particles change how much sunlight clouds reflect to space, an important human perturbation of the climate, whose magnitude is highly uncertain. We found that the latest climate models show a negative correlation but a positive causal relationship between aerosols and cloud water. This means we need to be very careful when we interpret observational studies that can only see correlation.
Fan Mei, Jennifer M. Comstock, Mikhail S. Pekour, Jerome D. Fast, Beat Schmid, Krista L. Gaustad, Shuaiqi Tang, Damao Zhang, John E. Shilling, Jason Tomlinson, Adam C. Varble, Jian Wang, L. Ruby Leung, Lawrence Kleinman, Scot Martin, Sebastien C. Biraud, Brian D. Ermold, and Kenneth W. Burk
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-97, https://doi.org/10.5194/essd-2024-97, 2024
Preprint under review for ESSD
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Our study explores a rich dataset from the final decade of the U.S. DOE's Gulfstream-1 (G-1) aircraft operations (2013-2018). The 236 flights cover diverse regions, including the Arctic, U.S. Southern Great Plains, U.S. West Coast, Eastern North Atlantic, Amazon Basin in Brazil, and Sierras de Córdoba range in Argentina. This airborne dataset offers unprecedented insights into atmospheric dynamics, aerosols, and clouds with a more accessible data format.
Sebastian Diez, Stuart Lacy, Hugh Coe, Josefina Urquiza, Max Priestman, Michael Flynn, Nicholas Marsden, Nicholas A. Martin, Stefan Gillott, Thomas Bannan, and Pete M. Edwards
Atmos. Meas. Tech., 17, 3809–3827, https://doi.org/10.5194/amt-17-3809-2024, https://doi.org/10.5194/amt-17-3809-2024, 2024
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In this paper we present an overview of the QUANT project, which to our knowledge is one of the largest evaluations of commercial sensors to date. The objective was to evaluate the performance of a range of commercial products and also to nourish the different applications in which these technologies can offer relevant information.
Guta Wakbulcho Abeshu, Hong-Yi Li, Mingjie Shi, and Ruby Leung
EGUsphere, https://doi.org/10.5194/egusphere-2024-1748, https://doi.org/10.5194/egusphere-2024-1748, 2024
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This study examined how water availability, climate dryness, and plant productivity interact at the catchment scale. Using various indices and statistical methods, it found a 0–2-month lag in these interactions. Strong correlations during peak productivity months were observed, with a notable hysteresis effect in vegetation response to changes in water availability and climate dryness. The findings help better understand catchment responses to climate variability.
Jianfeng Li, Andrew Geiss, Zhe Feng, L. Ruby Leung, Yun Qian, and Wenjun Cui
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-112, https://doi.org/10.5194/essd-2024-112, 2024
Preprint under review for ESSD
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We develop a high-resolution (4 km and hourly) observational derecho dataset over the United States east of the Rocky Mountains from 2004 to 2021 by using a mesoscale convective system dataset, bow echo detection based on a machine learning method, hourly gust speed measurements, and physically based identification criteria.
Tapio Schneider, L. Ruby Leung, and Robert C. J. Wills
Atmos. Chem. Phys., 24, 7041–7062, https://doi.org/10.5194/acp-24-7041-2024, https://doi.org/10.5194/acp-24-7041-2024, 2024
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Climate models are crucial for predicting climate change in detail. This paper proposes a balanced approach to improving their accuracy by combining traditional process-based methods with modern artificial intelligence (AI) techniques while maximizing the resolution to allow for ensemble simulations. The authors propose using AI to learn from both observational and simulated data while incorporating existing physical knowledge to reduce data demands and improve climate prediction reliability.
Sanja Dmitrovic, Johnathan W. Hair, Brian L. Collister, Ewan Crosbie, Marta A. Fenn, Richard A. Ferrare, David B. Harper, Chris A. Hostetler, Yongxiang Hu, John A. Reagan, Claire E. Robinson, Shane T. Seaman, Taylor J. Shingler, Kenneth L. Thornhill, Holger Vömel, Xubin Zeng, and Armin Sorooshian
Atmos. Meas. Tech., 17, 3515–3532, https://doi.org/10.5194/amt-17-3515-2024, https://doi.org/10.5194/amt-17-3515-2024, 2024
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This study introduces and evaluates a new ocean surface wind speed product from the NASA Langley Research Center (LARC) airborne High-Spectral-Resolution Lidar – Generation 2 (HSRL-2) during the NASA ACTIVATE mission. We show that HSRL-2 surface wind speed data are accurate when compared to ground-truth dropsonde measurements. Therefore, the HSRL-2 instrument is able obtain accurate, high-resolution surface wind speed data in airborne field campaigns.
Amie Dobracki, Ernie Lewis, Arthur Sedlacek III, Tyler Tatro, Maria Zawadowicz, and Paquita Zuidema
EGUsphere, https://doi.org/10.5194/egusphere-2024-1347, https://doi.org/10.5194/egusphere-2024-1347, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Biomass-burning aerosol is commonly present in the marine boundary layer of the southeast Atlantic Ocean between June and October. Our research indicates that burning conditions, aerosol transport pathways, and prolonged oxidation processes, both heterogeneous and aqueous-phase determine the chemical, microphysical, and optical properties of the boundary layer aerosol. Notably, we find that the aerosol optical properties can be estimated from the chemical properties alone.
Matthew Henry, Ewa M. Bednarz, and Jim Haywood
EGUsphere, https://doi.org/10.5194/egusphere-2024-1565, https://doi.org/10.5194/egusphere-2024-1565, 2024
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Stratospheric Aerosol Injection (SAI) refers to a climate intervention method by which aerosols are intentionally added to the stratosphere (~21 km) to increase the amount of reflected sunlight and reduce the Earth’s temperature. The climate outcomes of SAI depend on the location, amount, and timing of injection. Here, we analyse the role of the latitude of injection in different climate simulations which reduce Earth’s temperature by the same amount but have a different latitude of injection.
Ryan Eastman, Isabel L. McCoy, Hauke Schulz, and Robert Wood
Atmos. Chem. Phys., 24, 6613–6634, https://doi.org/10.5194/acp-24-6613-2024, https://doi.org/10.5194/acp-24-6613-2024, 2024
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Cloud types are determined using machine learning image classifiers applied to satellite imagery for 1 year in the North Atlantic. This survey of these cloud types shows that the climate impact of a cloud scene is, in part, a function of cloud type. Each type displays a different mix of thick and thin cloud cover, with the fraction of thin cloud cover having the strongest impact on the clouds' radiative effect. Future studies must account for differing properties and processes among cloud types.
Yilin Fang, Hoang Viet Tran, and L. Ruby Leung
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-70, https://doi.org/10.5194/gmd-2024-70, 2024
Preprint under review for GMD
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Hurricanes may worsen the water quality in the lower Mississippi River Basin (LMRB) by increasing nutrient runoff. We found that runoff parameterizations greatly affect nitrate-nitrogen runoff simulated using an Earth system land model. Our simulations predicted increased nitrogen runoff in LMRB during Hurricane Ida in 2021, but less pronounced than the observations, indicating areas for model improvement to better understand and manage nutrient runoff loss during hurricanes in the region.
Ewan Crosbie, Luke D. Ziemba, Michael A. Shook, Taylor Shingler, Johnathan W. Hair, Armin Sorooshian, Richard A. Ferrare, Brian Cairns, Yonghoon Choi, Joshua DiGangi, Glenn S. Diskin, Chris Hostetler, Simon Kirschler, Richard H. Moore, David Painemal, Claire Robinson, Shane T. Seaman, K. Lee Thornhill, Christiane Voigt, and Edward Winstead
Atmos. Chem. Phys., 24, 6123–6152, https://doi.org/10.5194/acp-24-6123-2024, https://doi.org/10.5194/acp-24-6123-2024, 2024
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Marine clouds are found to clump together in regions or lines, readily discernible from satellite images of the ocean. While clustering is also a feature of deep storm clouds, we focus on smaller cloud systems associated with fair weather and brief localized showers. Two aircraft sampled the region around these shallow systems: one incorporated measurements taken within, adjacent to, and below the clouds, while the other provided a survey from above using remote sensing techniques.
Alexei Korolev, Zhipeng Qu, Jason Milbrandt, Ivan Heckman, Mélissa Cholette, Mengistu Wolde, Cuong Nguyen, Greg McFarquhar, Paul Lawson, and Ann Fridlind
EGUsphere, https://doi.org/10.5194/egusphere-2024-1465, https://doi.org/10.5194/egusphere-2024-1465, 2024
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The phenomenon of high ice water content (HIWC) occurs in mesoscale convective systems (MCS) when a large number of small ice particles with typical sizes of a few hundred micrometers are found at high altitudes. This study presents a conceptual model of the formation of HIWC in tropical MCSs developed based on in-situ observations and numerical simulation. It was found that secondary ice production in the vicinity of the melting layer plays a key role in the formation and maintenance of HIWC.
Jerome D. Fast, Adam C. Varble, Fan Mei, Mikhail Pekour, Jason Tomlinson, Alla Zelenyuk, Art J. Sedlacek III, Maria Zawadowicz, and Louisa K. Emmons
EGUsphere, https://doi.org/10.5194/egusphere-2024-1349, https://doi.org/10.5194/egusphere-2024-1349, 2024
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Aerosol property measurements recently collected at the ground and by a research aircraft in central Argentina during the CACTI campaign exhibit large spatial and temporal variability. These measurements coupled with coincident meteorological information provide a valuable dataset needed to evaluate and improve model predictions of aerosols in a traditionally data sparse region of South America.
Michie Vianca De Vera, Larry Di Girolamo, Guangyu Zhao, Robert M. Rauber, Stephen W. Nesbitt, and Greg M. McFarquhar
Atmos. Chem. Phys., 24, 5603–5623, https://doi.org/10.5194/acp-24-5603-2024, https://doi.org/10.5194/acp-24-5603-2024, 2024
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Tropical oceanic low clouds remain a dominant source of uncertainty in cloud feedback in climate models due to their macrophysical properties (fraction, size, height, shape, distribution) being misrepresented. High-resolution satellite imagery over the Philippine oceans is used here to characterize cumulus macrophysical properties and their relationship to meteorological variables. Such information can act as a benchmark for cloud models and can improve low-cloud generation in climate models.
Fang Li, Xiang Song, Sandy P. Harrison, Jennifer R. Marlon, Zhongda Lin, L. Ruby Leung, Jörg Schwinger, Virginie Marécal, Shiyu Wang, Daniel S. Ward, Xiao Dong, Hanna Lee, Lars Nieradzik, Sam S. Rabin, and Roland Séférian
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-85, https://doi.org/10.5194/gmd-2024-85, 2024
Preprint under review for GMD
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This study provides the first comprehensive assessment of historical fire simulations from 19 CMIP6 ESMs. Most models reproduce global total, spatial pattern, seasonality, and regional historical changes well, but fail to simulate the recent decline in global burned area and underestimate the fire sensitivity to wet-dry conditions. They addressed three critical issues in CMIP5. We present targeted guidance for fire scheme development and methodologies to generate reliable fire projections.
Declan L. Finney, Alan M. Blyth, Martin Gallagher, Huihui Wu, Graeme J. Nott, Michael I. Biggerstaff, Richard G. Sonnenfeld, Martin Daily, Dan Walker, David Dufton, Keith Bower, Steven Böing, Thomas Choularton, Jonathan Crosier, James Groves, Paul R. Field, Hugh Coe, Benjamin J. Murray, Gary Lloyd, Nicholas A. Marsden, Michael Flynn, Kezhen Hu, Navaneeth M. Thamban, Paul I. Williams, Paul J. Connolly, James B. McQuaid, Joseph Robinson, Zhiqiang Cui, Ralph R. Burton, Gordon Carrie, Robert Moore, Steven J. Abel, Dave Tiddeman, and Graydon Aulich
Earth Syst. Sci. Data, 16, 2141–2163, https://doi.org/10.5194/essd-16-2141-2024, https://doi.org/10.5194/essd-16-2141-2024, 2024
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The DCMEX (Deep Convective Microphysics Experiment) project undertook an aircraft- and ground-based measurement campaign of New Mexico deep convective clouds during July–August 2022. The campaign coordinated a broad range of instrumentation measuring aerosol, cloud physics, radar signals, thermodynamics, dynamics, electric fields, and weather. The project's objectives included the utilisation of these data with satellite observations to study the anvil cloud radiative effect.
Lingcheng Li, Gautam Bisht, Dalei Hao, and L. Ruby Leung
Earth Syst. Sci. Data, 16, 2007–2032, https://doi.org/10.5194/essd-16-2007-2024, https://doi.org/10.5194/essd-16-2007-2024, 2024
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This study fills a gap to meet the emerging needs of kilometer-scale Earth system modeling by developing global 1 km land surface parameters for land use, vegetation, soil, and topography. Our demonstration simulations highlight the substantial impacts of these parameters on spatial variability and information loss in water and energy simulations. Using advanced explainable machine learning methods, we identified influential factors driving spatial variability and information loss.
Bryce E. Harrop, Jian Lu, L. Ruby Leung, William K. M. Lau, Kyu-Myong Kim, Brian Medeiros, Brian J. Soden, Gabriel A. Vecchi, Bosong Zhang, and Balwinder Singh
Geosci. Model Dev., 17, 3111–3135, https://doi.org/10.5194/gmd-17-3111-2024, https://doi.org/10.5194/gmd-17-3111-2024, 2024
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Seven new experimental setups designed to interfere with cloud radiative heating have been added to the Energy Exascale Earth System Model (E3SM). These experiments include both those that test the mean impact of cloud radiative heating and those examining its covariance with circulations. This paper documents the code changes and steps needed to run these experiments. Results corroborate prior findings for how cloud radiative heating impacts circulations and rainfall patterns.
Marios Chatziparaschos, Stelios Myriokefalitakis, Nikos Kalivitis, Nikos Daskalakis, Athanasios Nenes, María Gonçalves Ageitos, Montserrat Costa-Surós, Carlos Pérez García-Pando, Mihalis Vrekoussis, and Maria Kanakidou
EGUsphere, https://doi.org/10.5194/egusphere-2024-952, https://doi.org/10.5194/egusphere-2024-952, 2024
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We show distinct seasonal and geographical patterns in the contributions of mineral dust, marine and terrestrial biological particles to ice-nucleating particles (INP) concentrations that lead to atmospheric ice formation, a major source of uncertainty in climate predictions. Bioaerosols are the major source of INP at high temperatures, while mineral dust influences the global INP population at lower temperatures. These particles can satisfactorily reproduce INP in a climate model.
Hiren T. Jethva, Omar Torres, Richard A. Ferrare, Sharon P. Burton, Anthony L. Cook, David B. Harper, Chris A. Hostetler, Jens Redemann, Vinay Kayetha, Samuel LeBlanc, Kristina Pistone, Logan Mitchell, and Connor J. Flynn
Atmos. Meas. Tech., 17, 2335–2366, https://doi.org/10.5194/amt-17-2335-2024, https://doi.org/10.5194/amt-17-2335-2024, 2024
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We introduce a novel synergy algorithm applied to ORALCES airborne measurements of above-cloud aerosol optical depth and UV–Vis satellite observations from OMI and MODIS to retrieve spectral aerosol single-scattering albedo of lofted layers of carbonaceous smoke aerosols over clouds. The development of the proposed aerosol–cloud algorithm implies a possible synergy of CALIOP and OMI–MODIS passive sensors to deduce a global product of AOD and SSA of absorbing aerosols above clouds.
Siddhant Gupta, Dié Wang, Scott E. Giangrande, Thiago S. Biscaro, and Michael P. Jensen
Atmos. Chem. Phys., 24, 4487–4510, https://doi.org/10.5194/acp-24-4487-2024, https://doi.org/10.5194/acp-24-4487-2024, 2024
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We examine the lifecycle of isolated deep convective clouds (DCCs) in the Amazon rainforest. Weather radar echoes from the DCCs are tracked to evaluate their lifecycle. The DCC size and intensity increase, reach a peak, and then decrease over the DCC lifetime. Vertical profiles of air motion and mass transport from different seasons are examined to understand the transport of energy and momentum within DCC cores and to address the deficiencies in simulating DCCs using weather and climate models.
Pengfei Shi, L. Ruby Leung, Bin Wang, Kai Zhang, Samson M. Hagos, and Shixuan Zhang
Geosci. Model Dev., 17, 3025–3040, https://doi.org/10.5194/gmd-17-3025-2024, https://doi.org/10.5194/gmd-17-3025-2024, 2024
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Improving climate predictions have profound socio-economic impacts. This study introduces a new weakly coupled land data assimilation (WCLDA) system for a coupled climate model. We demonstrate improved simulation of soil moisture and temperature in many global regions and throughout the soil layers. Furthermore, significant improvements are also found in reproducing the time evolution of the 2012 US Midwest drought. The WCLDA system provides the groundwork for future predictability studies.
Cassidy Soloff, Taiwo Ajayi, Yonghoon Choi, Ewan C. Crosbie, Joshua P. DiGangi, Glenn S. Diskin, Marta A. Fenn, Richard A. Ferrare, Francesca Gallo, Johnathan W. Hair, Miguel Ricardo A. Hilario, Simon Kirschler, Richard H. Moore, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Christiane Voigt, Edward L. Winstead, Luke D. Ziemba, and Armin Sorooshian
EGUsphere, https://doi.org/10.5194/egusphere-2024-926, https://doi.org/10.5194/egusphere-2024-926, 2024
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Using aircraft measurements over the northwest Atlantic between the U.S. East Coast and Bermuda and trajectory modeling of continental outflow, we identify trace gas and particle properties that exhibit gradients with offshore distance and quantify these changes with high resolution measurements of concentrations as well as particle chemistry, size, and scattering properties. This work furthers our understanding of the complex interactions between continental and marine environments.
Jianhao Zhang, Yao-Sheng Chen, Takanobu Yamaguchi, and Graham Feingold
EGUsphere, https://doi.org/10.5194/egusphere-2024-1021, https://doi.org/10.5194/egusphere-2024-1021, 2024
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Quantifying cloud response to aerosol perturbations presents a major challenge to understanding the human impact on climate. Using a large number of process-resolving simulations of marine stratocumulus, we show that solar heating plays an important role in governing this response, such that a persistent negative trend is buffered by a negative feedback mechanism after sunrise. It provides implications for the dependence of cloud cooling effect on the timing of advertent aerosol perturbations.
Philip Rasch, Haruki Hirasawa, Mingxuan Wu, Sarah Doherty, Robert Wood, Hailong Wang, Andy Jones, James Haywood, and Hansi Singh
EGUsphere, https://doi.org/10.5194/egusphere-2024-1031, https://doi.org/10.5194/egusphere-2024-1031, 2024
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We introduce a protocol to compare computer climate simulations to better understand a proposed strategy intended to counter warming & climate impacts from greenhouse gas increases. The strategy slightly changes clouds in 6 ocean regions to reflect more sunlight & cool Earth. Example changes in clouds & climate are shown for 3 climate models. Clouds change differently between the models, but precipitation and surface temperature changes are similar when their cooling effects are made similar.
Yao-Sheng Chen, Jianhao Zhang, Fabian Hoffmann, Takanobu Yamaguchi, Franziska Glassmeier, Xiaoli Zhou, and Graham Feingold
EGUsphere, https://doi.org/10.5194/egusphere-2024-1033, https://doi.org/10.5194/egusphere-2024-1033, 2024
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Marine stratocumulus cloud is a type of shallow clouds that covers the vast areas of Earth's surface. They play an important role in Earth's energy balance by reflecting solar radiation back to space. We used numerical models to simulate a large number of marine stratocumuli with different characteristics. We found that how the clouds develop throughout the day is affected by the level of humidity in the air above the clouds and how closely the clouds connect to the ocean surface.
Daniele Visioni, Alan Robock, Jim Haywood, Matthew Henry, Simone Tilmes, Douglas G. MacMartin, Ben Kravitz, Sarah J. Doherty, John Moore, Chris Lennard, Shingo Watanabe, Helene Muri, Ulrike Niemeier, Olivier Boucher, Abu Syed, Temitope S. Egbebiyi, Roland Séférian, and Ilaria Quaglia
Geosci. Model Dev., 17, 2583–2596, https://doi.org/10.5194/gmd-17-2583-2024, https://doi.org/10.5194/gmd-17-2583-2024, 2024
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This paper describes a new experimental protocol for the Geoengineering Model Intercomparison Project (GeoMIP). In it, we describe the details of a new simulation of sunlight reflection using the stratospheric aerosols that climate models are supposed to run, and we explain the reasons behind each choice we made when defining the protocol.
Xiaoli Shen, David M. Bell, Hugh Coe, Naruki Hiranuma, Fabian Mahrt, Nicholas A. Marsden, Claudia Mohr, Daniel M. Murphy, Harald Saathoff, Johannes Schneider, Jacqueline Wilson, Maria A. Zawadowicz, Alla Zelenyuk, Paul J. DeMott, Ottmar Möhler, and Daniel J. Cziczo
EGUsphere, https://doi.org/10.5194/egusphere-2024-928, https://doi.org/10.5194/egusphere-2024-928, 2024
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Single particle mass spectrometer (SPMS) is commonly used to measure chemical composition and mixing state of aerosol particles. Intercomparison of SPMSs was conducted. All instruments reported similar size ranges and common spectral features. The instrument-specific detection efficiency was found to be more dependent on particle size than type. All instruments differentiated secondary organic aerosol, soot, and soil dust, but had difficulties differentiating among specific minerals and dusts.
Lingbo Li, Hong-Yi Li, Guta Abeshu, Jinyun Tang, L. Ruby Leung, Chang Liao, Zeli Tan, Hanqin Tian, Peter Thornton, and Xiaojuan Yang
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-43, https://doi.org/10.5194/essd-2024-43, 2024
Preprint under review for ESSD
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We have developed a new map that reveals how organic carbon from soil leaches into headwater streams over the contiguous United States. We use advanced artificial intelligence techniques and a massive amount of data, including observations at over 2,500 gauges and a wealth of climate and environmental information. The map is a critical step in understanding and predicting how carbon moves through our environment, hence a useful tool for tackling climate challenges.
Johannes Mülmenstädt, Andrew S. Ackerman, Ann M. Fridlind, Meng Huang, Po-Lun Ma, Naser Mahfouz, Susanne E. Bauer, Susannah M. Burrows, Matthew W. Christensen, Sudhakar Dipu, Andrew Gettelman, L. Ruby Leung, Florian Tornow, Johannes Quaas, Adam C. Varble, Hailong Wang, Kai Zhang, and Youtong Zheng
EGUsphere, https://doi.org/10.5194/egusphere-2024-778, https://doi.org/10.5194/egusphere-2024-778, 2024
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Stratocumulus clouds play a large role in Earth's climate by reflecting incoming solar energy back to space. Turbulence at stratocumulus cloud top mixes in drier, warmer air, which can lead to a reduction in cloud. This process is challenging for coarse-resolution global models to represent. We show that global models nevertheless agree well with our process understanding. Global models also think the process is less important for the climate than other lines of evidence had led us to conclude.
Jeonggyu Kim, Sungmin Park, Greg Michael McFarquhar, Anthony J. Baran, Joo Wan Cha, Kyoungmi Lee, Seoung Soo Lee, Chang Hoon Jung, Kyo-Sun Sunny Lim, and Junshik Um
EGUsphere, https://doi.org/10.5194/egusphere-2024-608, https://doi.org/10.5194/egusphere-2024-608, 2024
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In this study, we developed idealized models to represent the shapes of ice particles found in deep convective clouds and calculated their single-scattering properties. By comparing these results with in situ measurements, we discovered that a mixture of shape models provides a closer match to in situ measurements than either single-form models or aggregate models do. This finding has important implications for enhancing the simulation of single-scattering properties of deep convective clouds.
Yawen Liu, Yun Qian, Philip J. Rasch, Kai Zhang, Lai-yung Ruby Leung, Yuhang Wang, Minghuai Wang, Hailong Wang, Xin Huang, and Xiu-Qun Yang
Atmos. Chem. Phys., 24, 3115–3128, https://doi.org/10.5194/acp-24-3115-2024, https://doi.org/10.5194/acp-24-3115-2024, 2024
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Fire management has long been a challenge. Here we report that spring-peak fire activity over southern Mexico and Central America (SMCA) has a distinct quasi-biennial signal by measuring multiple fire metrics. This signal is initially driven by quasi-biennial variability in precipitation and is further amplified by positive feedback of fire–precipitation interaction at short timescales. This work highlights the importance of fire–climate interactions in shaping fires on an interannual scale.
Lucas A. McMichael, Michael J. Schmidt, Robert Wood, Peter N. Blossey, and Lekha Patel
EGUsphere, https://doi.org/10.5194/egusphere-2024-235, https://doi.org/10.5194/egusphere-2024-235, 2024
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Marine Cloud Brightening (MCB) is a climate intervention technique to potentially cool the climate. Climate models used to gauge regional climate impacts associated with MCB often assume large areas of the ocean are uniformly perturbed; However, a more realistic representation of MCB application would require information about how an injected particle plume spreads. This work aims to develop such a plume spreading model.
Alexander T. Archibald, Bablu Sinha, Maria Russo, Emily Matthews, Freya Squires, N. Luke Abraham, Stephane Bauguitte, Thomas Bannan, Thomas Bell, David Berry, Lucy Carpenter, Hugh Coe, Andrew Coward, Peter Edwards, Daniel Feltham, Dwayne Heard, Jim Hopkins, James Keeble, Elizabeth C. Kent, Brian King, Isobel R. Lawrence, James Lee, Claire R. Macintosh, Alex Megann, Ben I. Moat, Katie Read, Chris Reed, Malcolm Roberts, Reinhard Schiemann, David Schroeder, Tim Smyth, Loren Temple, Navaneeth Thamban, Lisa Whalley, Simon Williams, Huihui Wu, and Ming-Xi Yang
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2023-405, https://doi.org/10.5194/essd-2023-405, 2024
Preprint under review for ESSD
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Here we present an overview of the data generated as part of the North Atlantic Climate System Integrated Studies (ACSIS) programme which are available through dedicated repositories at the Centre for Environmental Data Analysis (CEDA, www.ceda.ac.uk) and the British Oceanographic Data Centre (BODC, bodc.ac.uk). ACSIS data cover the full North Atlantic System comprising: the North Atlantic Ocean, the atmosphere above it including its composition, Arctic Sea Ice and the Greenland Ice Sheet.
George Jordan, Florent Malavelle, Ying Chen, Amy Peace, Eliza Duncan, Daniel G. Partridge, Paul Kim, Duncan Watson-Parris, Toshihiko Takemura, David Neubauer, Gunnar Myhre, Ragnhild Skeie, Anton Laakso, and James Haywood
Atmos. Chem. Phys., 24, 1939–1960, https://doi.org/10.5194/acp-24-1939-2024, https://doi.org/10.5194/acp-24-1939-2024, 2024
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The 2014–15 Holuhraun eruption caused a huge aerosol plume in an otherwise unpolluted region, providing a chance to study how aerosol alters cloud properties. This two-part study uses observations and models to quantify this relationship’s impact on the Earth’s energy budget. Part 1 suggests the models capture the observed spatial and chemical evolution of the plume, yet no model plume is exact. Understanding these differences is key for Part 2, where changes to cloud properties are explored.
Donghui Xu, Gautam Bisht, Zeli Tan, Chang Liao, Tian Zhou, Hong-Yi Li, and L. Ruby Leung
Geosci. Model Dev., 17, 1197–1215, https://doi.org/10.5194/gmd-17-1197-2024, https://doi.org/10.5194/gmd-17-1197-2024, 2024
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We aim to disentangle the hydrological and hydraulic controls on streamflow variability in a fully coupled earth system model. We found that calibrating only one process (i.e., traditional calibration procedure) will result in unrealistic parameter values and poor performance of the water cycle, while the simulated streamflow is improved. To address this issue, we further proposed a two-step calibration procedure to reconcile the impacts from hydrological and hydraulic processes on streamflow.
Alexandros Milousis, Alexandra P. Tsimpidi, Holger Tost, Spyros N. Pandis, Athanasios Nenes, Astrid Kiendler-Scharr, and Vlassis A. Karydis
Geosci. Model Dev., 17, 1111–1131, https://doi.org/10.5194/gmd-17-1111-2024, https://doi.org/10.5194/gmd-17-1111-2024, 2024
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This study aims to evaluate the newly developed ISORROPIA-lite aerosol thermodynamic module within the EMAC model and explore discrepancies in global atmospheric simulations of aerosol composition and acidity by utilizing different aerosol phase states. Even though local differences were found in regions where the RH ranged from 20 % to 60 %, on a global scale the results are similar. Therefore, ISORROPIA-lite can be a reliable and computationally effective alternative to ISORROPIA II in EMAC.
Luis F. Millán, Matthew D. Lebsock, Ken B. Cooper, Jose V. Siles, Robert Dengler, Raquel Rodriguez Monje, Amin Nehrir, Rory A. Barton-Grimley, James E. Collins, Claire E. Robinson, Kenneth L. Thornhill, and Holger Vömel
Atmos. Meas. Tech., 17, 539–559, https://doi.org/10.5194/amt-17-539-2024, https://doi.org/10.5194/amt-17-539-2024, 2024
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In this study, we describe and validate a new technique in which three radar tones are used to estimate the water vapor inside clouds and precipitation. This instrument flew on board NASA's P-3 aircraft during the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Snowstorms (IMPACTS) campaign and the Synergies Of Active optical and Active microwave Remote Sensing Experiment (SOA2RSE) campaign.
Ou Wang, Ju Liang, Yuchen Gu, Jim M. Haywood, Ying Chen, Chenwei Fang, and Qingeng Wang
EGUsphere, https://doi.org/10.5194/egusphere-2023-2904, https://doi.org/10.5194/egusphere-2023-2904, 2024
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This study investigates the impact of stratospheric aerosol injection (SAI) on extreme precipitation in China by the late 21st century. The effects of SAI (G6sulfur) are compared with simulations from SSP5-8.5, SSP2-4.5, and G6solar. The results indicate that both G6sulfur and G6solar reduce extreme rainfall in eastern China. However, caution is advised due to potential side effects at high latitudes. Further optimization is deemed crucial for the future deployment of SAI.
Jim M. Haywood, Andy Jones, Anthony C. Jones, Paul Halloran, and Philip J. Rasch
Atmos. Chem. Phys., 23, 15305–15324, https://doi.org/10.5194/acp-23-15305-2023, https://doi.org/10.5194/acp-23-15305-2023, 2023
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The difficulties in ameliorating global warming and the associated climate change via conventional mitigation are well documented, with all climate model scenarios exceeding 1.5 °C above the preindustrial level in the near future. There is therefore a growing interest in geoengineering to reflect a greater proportion of sunlight back to space and offset some of the global warming. We use a state-of-the-art Earth-system model to investigate two of the most prominent geoengineering strategies.
Jiemei Liu, Jesper Heile Christensen, Zhuyun Ye, Shikui Dong, Camilla Geels, Jørgen Brandt, Athanasios Nenes, Yuan Yuan, and Ulas Im
EGUsphere, https://doi.org/10.5194/egusphere-2023-2615, https://doi.org/10.5194/egusphere-2023-2615, 2023
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In this study, China was chosen as an example to conduct a quantitative analysis using the Danish Eulerian Hemispheric Model (DEHM) system with meteorological input from WRF weather forecast model. It found that meteorological conditions and emission inventories contributed 46 % (65 %) and 54 % (35 %) to the variations in PM2.5 concentrations (OP), respectively, highlighting secondary aerosol formation and biomass burning as the primary contributors to PM2.5 and OP levels.
Ghislain Motos, Gabriel Freitas, Paraskevi Georgakaki, Jörg Wieder, Guangyu Li, Wenche Aas, Chris Lunder, Radovan Krejci, Julie Thérèse Pasquier, Jan Henneberger, Robert Oscar David, Christoph Ritter, Claudia Mohr, Paul Zieger, and Athanasios Nenes
Atmos. Chem. Phys., 23, 13941–13956, https://doi.org/10.5194/acp-23-13941-2023, https://doi.org/10.5194/acp-23-13941-2023, 2023
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Low-altitude clouds play a key role in regulating the climate of the Arctic, a region that suffers from climate change more than any other on the planet. We gathered meteorological and aerosol physical and chemical data over a year and utilized them for a parameterization that help us unravel the factors driving and limiting the efficiency of cloud droplet formation. We then linked this information to the sources of aerosol found during each season and to processes of cloud glaciation.
Dongyu Feng, Zeli Tan, Donghui Xu, and L. Ruby Leung
Hydrol. Earth Syst. Sci., 27, 3911–3934, https://doi.org/10.5194/hess-27-3911-2023, https://doi.org/10.5194/hess-27-3911-2023, 2023
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This study assesses the flood risks concurrently induced by river flooding and coastal storm surge along the coast of the contiguous United States using statistical and numerical models. We reveal a few hotspots of such risks, the critical spatial variabilities within a river basin and over the whole US coast, and the uncertainties of the risk assessment. We highlight the importance of weighing different risk measures to avoid underestimating or exaggerating the compound flood impacts.
Stylianos Kakavas, Spyros N. Pandis, and Athanasios Nenes
Atmos. Chem. Phys., 23, 13555–13564, https://doi.org/10.5194/acp-23-13555-2023, https://doi.org/10.5194/acp-23-13555-2023, 2023
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Water uptake from organic species in aerosol can affect the partitioning of semi-volatile inorganic compounds but are not considered in global and chemical transport models. We address this with a version of the PM-CAMx model that considers such organic water effects and use it to carry out 1-year aerosol simulations over the continental US. We show that such organic water impacts can increase dry PM1 levels by up to 2 μg m-3 when RH levels and PM1 concentrations are high.
Matthew Henry, Jim Haywood, Andy Jones, Mohit Dalvi, Alice Wells, Daniele Visioni, Ewa M. Bednarz, Douglas G. MacMartin, Walker Lee, and Mari R. Tye
Atmos. Chem. Phys., 23, 13369–13385, https://doi.org/10.5194/acp-23-13369-2023, https://doi.org/10.5194/acp-23-13369-2023, 2023
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Solar climate interventions, such as injecting sulfur in the stratosphere, may be used to offset some of the adverse impacts of global warming. We use two independently developed Earth system models to assess the uncertainties around stratospheric sulfur injections. The injection locations and amounts are optimized to maintain the same pattern of surface temperature. While both models show reduced warming, the change in rainfall patterns (even without sulfur injections) is uncertain.
Lu Zhang, Michal Segal-Rozenhaimer, Haochi Che, Caroline Dang, Junying Sun, Ye Kuang, Paola Formenti, and Steven Howell
EGUsphere, https://doi.org/10.5194/egusphere-2023-2199, https://doi.org/10.5194/egusphere-2023-2199, 2023
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Using airborne measurements over the South-East Atlantic, our study explored how aerosols—tiny atmospheric particles—interact with moisture over the ocean, especially during the biomass burning season. We noticed unique patterns in their behavior at different altitudes and introduced a predictive model for this moisture interaction. Our results aid our understanding of aerosol-moisture interactions and benefit the research of aerosol radiative effect in this climatically significant region.
Simon Kirschler, Christiane Voigt, Bruce E. Anderson, Gao Chen, Ewan C. Crosbie, Richard A. Ferrare, Valerian Hahn, Johnathan W. Hair, Stefan Kaufmann, Richard H. Moore, David Painemal, Claire E. Robinson, Kevin J. Sanchez, Amy J. Scarino, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Edward L. Winstead, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 23, 10731–10750, https://doi.org/10.5194/acp-23-10731-2023, https://doi.org/10.5194/acp-23-10731-2023, 2023
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In this study we present an overview of liquid and mixed-phase clouds and precipitation in the marine boundary layer over the western North Atlantic Ocean. We compare microphysical properties of pure liquid clouds to mixed-phase clouds and show that the initiation of the ice phase in mixed-phase clouds promotes precipitation. The observational data presented in this study are well suited for investigating the processes that give rise to liquid and mixed-phase clouds, ice, and precipitation.
Guangyu Li, Elise K. Wilbourn, Zezhen Cheng, Jörg Wieder, Allison Fagerson, Jan Henneberger, Ghislain Motos, Rita Traversi, Sarah D. Brooks, Mauro Mazzola, Swarup China, Athanasios Nenes, Ulrike Lohmann, Naruki Hiranuma, and Zamin A. Kanji
Atmos. Chem. Phys., 23, 10489–10516, https://doi.org/10.5194/acp-23-10489-2023, https://doi.org/10.5194/acp-23-10489-2023, 2023
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In this work, we present results from an Arctic field campaign (NASCENT) in Ny-Ålesund, Svalbard, on the abundance, variability, physicochemical properties, and potential sources of ice-nucleating particles (INPs) relevant for mixed-phase cloud formation. This work improves the data coverage of Arctic INPs and aerosol properties, allowing for the validation of models predicting cloud microphysical and radiative properties of mixed-phase clouds in the rapidly warming Arctic.
Anne-Claire Billault-Roux, Paraskevi Georgakaki, Josué Gehring, Louis Jaffeux, Alfons Schwarzenboeck, Pierre Coutris, Athanasios Nenes, and Alexis Berne
Atmos. Chem. Phys., 23, 10207–10234, https://doi.org/10.5194/acp-23-10207-2023, https://doi.org/10.5194/acp-23-10207-2023, 2023
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Secondary ice production plays a key role in clouds and precipitation. In this study, we analyze radar measurements from a snowfall event in the Jura Mountains. Complex signatures are observed, which reveal that ice crystals were formed through various processes. An analysis of multi-sensor data suggests that distinct ice multiplication processes were taking place. Both the methods used and the insights gained through this case study contribute to a better understanding of snowfall microphysics.
Mária Lbadaoui-Darvas, Ari Laaksonen, and Athanasios Nenes
Atmos. Chem. Phys., 23, 10057–10074, https://doi.org/10.5194/acp-23-10057-2023, https://doi.org/10.5194/acp-23-10057-2023, 2023
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Heterogeneous ice nucleation is the main ice formation mechanism in clouds. The mechanism of different freezing modes is to date unknown, which results in large model biases. Experiments do not allow for direct observation of ice nucleation at its native resolution. This work uses first principles molecular simulations to determine the mechanism of the least-understood ice nucleation mode and link it to adsorption through a novel modeling framework that unites ice and droplet formation.
Rose Marie Miller, Robert M. Rauber, Larry Di Girolamo, Matthew Rilloraza, Dongwei Fu, Greg M. McFarquhar, Stephen W. Nesbitt, Luke D. Ziemba, Sarah Woods, and Kenneth Lee Thornhill
Atmos. Chem. Phys., 23, 8959–8977, https://doi.org/10.5194/acp-23-8959-2023, https://doi.org/10.5194/acp-23-8959-2023, 2023
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The influence of human-produced aerosols on clouds remains one of the uncertainties in radiative forcing of Earth’s climate. Measurements of aerosol chemistry from sources around the Philippines illustrate the linkage between aerosol chemical composition and cloud droplet characteristics. Differences in aerosol chemical composition in the marine layer from biomass burning, industrial, ship-produced, and marine aerosols are shown to impact cloud microphysical structure just above cloud base.
Armin Sorooshian, Mikhail D. Alexandrov, Adam D. Bell, Ryan Bennett, Grace Betito, Sharon P. Burton, Megan E. Buzanowicz, Brian Cairns, Eduard V. Chemyakin, Gao Chen, Yonghoon Choi, Brian L. Collister, Anthony L. Cook, Andrea F. Corral, Ewan C. Crosbie, Bastiaan van Diedenhoven, Joshua P. DiGangi, Glenn S. Diskin, Sanja Dmitrovic, Eva-Lou Edwards, Marta A. Fenn, Richard A. Ferrare, David van Gilst, Johnathan W. Hair, David B. Harper, Miguel Ricardo A. Hilario, Chris A. Hostetler, Nathan Jester, Michael Jones, Simon Kirschler, Mary M. Kleb, John M. Kusterer, Sean Leavor, Joseph W. Lee, Hongyu Liu, Kayla McCauley, Richard H. Moore, Joseph Nied, Anthony Notari, John B. Nowak, David Painemal, Kasey E. Phillips, Claire E. Robinson, Amy Jo Scarino, Joseph S. Schlosser, Shane T. Seaman, Chellappan Seethala, Taylor J. Shingler, Michael A. Shook, Kenneth A. Sinclair, William L. Smith Jr., Douglas A. Spangenberg, Snorre A. Stamnes, Kenneth L. Thornhill, Christiane Voigt, Holger Vömel, Andrzej P. Wasilewski, Hailong Wang, Edward L. Winstead, Kira Zeider, Xubin Zeng, Bo Zhang, Luke D. Ziemba, and Paquita Zuidema
Earth Syst. Sci. Data, 15, 3419–3472, https://doi.org/10.5194/essd-15-3419-2023, https://doi.org/10.5194/essd-15-3419-2023, 2023
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The NASA Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) produced a unique dataset for research into aerosol–cloud–meteorology interactions. HU-25 Falcon and King Air aircraft conducted systematic and spatially coordinated flights over the northwest Atlantic Ocean. This paper describes the ACTIVATE flight strategy, instrument and complementary dataset products, data access and usage details, and data application notes.
Valerian Hahn, Ralf Meerkötter, Christiane Voigt, Sonja Gisinger, Daniel Sauer, Valéry Catoire, Volker Dreiling, Hugh Coe, Cyrille Flamant, Stefan Kaufmann, Jonas Kleine, Peter Knippertz, Manuel Moser, Philip Rosenberg, Hans Schlager, Alfons Schwarzenboeck, and Jonathan Taylor
Atmos. Chem. Phys., 23, 8515–8530, https://doi.org/10.5194/acp-23-8515-2023, https://doi.org/10.5194/acp-23-8515-2023, 2023
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During the DACCIWA campaign in West Africa, we found a 35 % increase in the cloud droplet concentration that formed in a polluted compared with a less polluted environment and a decrease of 17 % in effective droplet diameter. Radiative transfer simulations, based on the measured cloud properties, reveal that these low-level polluted clouds radiate only 2.6 % more energy back to space, compared with a less polluted cloud. The corresponding additional decrease in temperature is rather small.
Chenwei Fang, Jim M. Haywood, Ju Liang, Ben T. Johnson, Ying Chen, and Bin Zhu
Atmos. Chem. Phys., 23, 8341–8368, https://doi.org/10.5194/acp-23-8341-2023, https://doi.org/10.5194/acp-23-8341-2023, 2023
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The responses of Asian summer monsoon duration and intensity to air pollution mitigation are identified given the net-zero future. We show that reducing scattering aerosols makes the rainy season longer and stronger across South Asia and East Asia but that absorbing aerosol reduction has the opposite effect. Our results hint at distinct monsoon responses to emission controls that target different aerosols.
Lingcheng Li, Yilin Fang, Zhonghua Zheng, Mingjie Shi, Marcos Longo, Charles D. Koven, Jennifer A. Holm, Rosie A. Fisher, Nate G. McDowell, Jeffrey Chambers, and L. Ruby Leung
Geosci. Model Dev., 16, 4017–4040, https://doi.org/10.5194/gmd-16-4017-2023, https://doi.org/10.5194/gmd-16-4017-2023, 2023
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Accurately modeling plant coexistence in vegetation demographic models like ELM-FATES is challenging. This study proposes a repeatable method that uses machine-learning-based surrogate models to optimize plant trait parameters in ELM-FATES. Our approach significantly improves plant coexistence modeling, thus reducing errors. It has important implications for modeling ecosystem dynamics in response to climate change.
Qi Tang, Jean-Christophe Golaz, Luke P. Van Roekel, Mark A. Taylor, Wuyin Lin, Benjamin R. Hillman, Paul A. Ullrich, Andrew M. Bradley, Oksana Guba, Jonathan D. Wolfe, Tian Zhou, Kai Zhang, Xue Zheng, Yunyan Zhang, Meng Zhang, Mingxuan Wu, Hailong Wang, Cheng Tao, Balwinder Singh, Alan M. Rhoades, Yi Qin, Hong-Yi Li, Yan Feng, Yuying Zhang, Chengzhu Zhang, Charles S. Zender, Shaocheng Xie, Erika L. Roesler, Andrew F. Roberts, Azamat Mametjanov, Mathew E. Maltrud, Noel D. Keen, Robert L. Jacob, Christiane Jablonowski, Owen K. Hughes, Ryan M. Forsyth, Alan V. Di Vittorio, Peter M. Caldwell, Gautam Bisht, Renata B. McCoy, L. Ruby Leung, and David C. Bader
Geosci. Model Dev., 16, 3953–3995, https://doi.org/10.5194/gmd-16-3953-2023, https://doi.org/10.5194/gmd-16-3953-2023, 2023
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High-resolution simulations are superior to low-resolution ones in capturing regional climate changes and climate extremes. However, uniformly reducing the grid size of a global Earth system model is too computationally expensive. We provide an overview of the fully coupled regionally refined model (RRM) of E3SMv2 and document a first-of-its-kind set of climate production simulations using RRM at an economic cost. The key to this success is our innovative hybrid time step method.
Amir Yazdani, Satoshi Takahama, John K. Kodros, Marco Paglione, Mauro Masiol, Stefania Squizzato, Kalliopi Florou, Christos Kaltsonoudis, Spiro D. Jorga, Spyros N. Pandis, and Athanasios Nenes
Atmos. Chem. Phys., 23, 7461–7477, https://doi.org/10.5194/acp-23-7461-2023, https://doi.org/10.5194/acp-23-7461-2023, 2023
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Organic aerosols directly emitted from wood and pellet stove combustion are found to chemically transform (approximately 15 %–35 % by mass) under daytime aging conditions simulated in an environmental chamber. A new marker for lignin-like compounds is found to degrade at a different rate than previously identified biomass burning markers and can potentially provide indication of aging time in ambient samples.
Koichi Sakaguchi, L. Ruby Leung, Colin M. Zarzycki, Jihyeon Jang, Seth McGinnis, Bryce E. Harrop, William C. Skamarock, Andrew Gettelman, Chun Zhao, William J. Gutowski, Stephen Leak, and Linda Mearns
Geosci. Model Dev., 16, 3029–3081, https://doi.org/10.5194/gmd-16-3029-2023, https://doi.org/10.5194/gmd-16-3029-2023, 2023
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We document details of the regional climate downscaling dataset produced by a global variable-resolution model. The experiment is unique in that it follows a standard protocol designed for coordinated experiments of regional models. We found negligible influence of post-processing on statistical analysis, importance of simulation quality outside of the target region, and computational challenges that our model code faced due to rapidly changing super computer systems.
Harrison A. Parker, Joshua L. Laughner, Geoffrey C. Toon, Debra Wunch, Coleen M. Roehl, Laura T. Iraci, James R. Podolske, Kathryn McKain, Bianca C. Baier, and Paul O. Wennberg
Atmos. Meas. Tech., 16, 2601–2625, https://doi.org/10.5194/amt-16-2601-2023, https://doi.org/10.5194/amt-16-2601-2023, 2023
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We describe a retrieval algorithm for determining limited information about the vertical distribution of carbon monoxide (CO) and carbon dioxide (CO2) from total column observations from ground-based observations. Our retrieved partial column values compare well with integrated in situ data. The average error for our retrieval is 1.51 ppb (~ 2 %) for CO and 5.09 ppm (~ 1.25 %) for CO2. We anticipate that this approach will find broad application for use in carbon cycle science.
Ernesto Reyes-Villegas, Douglas Lowe, Jill S. Johnson, Kenneth S. Carslaw, Eoghan Darbyshire, Michael Flynn, James D. Allan, Hugh Coe, Ying Chen, Oliver Wild, Scott Archer-Nicholls, Alex Archibald, Siddhartha Singh, Manish Shrivastava, Rahul A. Zaveri, Vikas Singh, Gufran Beig, Ranjeet Sokhi, and Gordon McFiggans
Atmos. Chem. Phys., 23, 5763–5782, https://doi.org/10.5194/acp-23-5763-2023, https://doi.org/10.5194/acp-23-5763-2023, 2023
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Organic aerosols (OAs), their sources and their processes remain poorly understood. The volatility basis set (VBS) approach, implemented in air quality models such as WRF-Chem, can be a useful tool to describe primary OA (POA) production and aging. However, the main disadvantage is its complexity. We used a Gaussian process simulator to reproduce model results and to estimate the sources of model uncertainty. We do this by comparing the outputs with OA observations made at Delhi, India, in 2018.
Zhe Feng, Joseph Hardin, Hannah C. Barnes, Jianfeng Li, L. Ruby Leung, Adam Varble, and Zhixiao Zhang
Geosci. Model Dev., 16, 2753–2776, https://doi.org/10.5194/gmd-16-2753-2023, https://doi.org/10.5194/gmd-16-2753-2023, 2023
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PyFLEXTRKR is a flexible atmospheric feature tracking framework with specific capabilities to track convective clouds from a variety of observations and model simulations. The package has a collection of multi-object identification algorithms and has been optimized for large datasets. This paper describes the algorithms and demonstrates applications for tracking deep convective cells and mesoscale convective systems from observations and model simulations at a wide range of scales.
Joanna E. Dyson, Lisa K. Whalley, Eloise J. Slater, Robert Woodward-Massey, Chunxiang Ye, James D. Lee, Freya Squires, James R. Hopkins, Rachel E. Dunmore, Marvin Shaw, Jacqueline F. Hamilton, Alastair C. Lewis, Stephen D. Worrall, Asan Bacak, Archit Mehra, Thomas J. Bannan, Hugh Coe, Carl J. Percival, Bin Ouyang, C. Nicholas Hewitt, Roderic L. Jones, Leigh R. Crilley, Louisa J. Kramer, W. Joe F. Acton, William J. Bloss, Supattarachai Saksakulkrai, Jingsha Xu, Zongbo Shi, Roy M. Harrison, Simone Kotthaus, Sue Grimmond, Yele Sun, Weiqi Xu, Siyao Yue, Lianfang Wei, Pingqing Fu, Xinming Wang, Stephen R. Arnold, and Dwayne E. Heard
Atmos. Chem. Phys., 23, 5679–5697, https://doi.org/10.5194/acp-23-5679-2023, https://doi.org/10.5194/acp-23-5679-2023, 2023
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The hydroxyl (OH) and closely coupled hydroperoxyl (HO2) radicals are vital for their role in the removal of atmospheric pollutants. In less polluted regions, atmospheric models over-predict HO2 concentrations. In this modelling study, the impact of heterogeneous uptake of HO2 onto aerosol surfaces on radical concentrations and the ozone production regime in Beijing in the summertime is investigated, and the implications for emissions policies across China are considered.
Zeyu Xue, Paul Ullrich, and Lai-Yung Ruby Leung
Hydrol. Earth Syst. Sci., 27, 1909–1927, https://doi.org/10.5194/hess-27-1909-2023, https://doi.org/10.5194/hess-27-1909-2023, 2023
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We examine the sensitivity and robustness of conclusions drawn from the PGW method over the NEUS by conducting multiple PGW experiments and varying the perturbation spatial scales and choice of perturbed meteorological variables to provide a guideline for this increasingly popular regional modeling method. Overall, we recommend PGW experiments be performed with perturbations to temperature or the combination of temperature and wind at the gridpoint scale, depending on the research question.
Daniele Visioni, Ben Kravitz, Alan Robock, Simone Tilmes, Jim Haywood, Olivier Boucher, Mark Lawrence, Peter Irvine, Ulrike Niemeier, Lili Xia, Gabriel Chiodo, Chris Lennard, Shingo Watanabe, John C. Moore, and Helene Muri
Atmos. Chem. Phys., 23, 5149–5176, https://doi.org/10.5194/acp-23-5149-2023, https://doi.org/10.5194/acp-23-5149-2023, 2023
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Geoengineering indicates methods aiming to reduce the temperature of the planet by means of reflecting back a part of the incoming radiation before it reaches the surface or allowing more of the planetary radiation to escape into space. It aims to produce modelling experiments that are easy to reproduce and compare with different climate models, in order to understand the potential impacts of these techniques. Here we assess its past successes and failures and talk about its future.
Amie Dobracki, Paquita Zuidema, Steven G. Howell, Pablo Saide, Steffen Freitag, Allison C. Aiken, Sharon P. Burton, Arthur J. Sedlacek III, Jens Redemann, and Robert Wood
Atmos. Chem. Phys., 23, 4775–4799, https://doi.org/10.5194/acp-23-4775-2023, https://doi.org/10.5194/acp-23-4775-2023, 2023
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Southern Africa produces approximately one-third of the world’s carbon from fires. The thick smoke layer can flow westward, interacting with the southeastern Atlantic cloud deck. The net radiative impact can alter regional circulation patterns, impacting rainfall over Africa. We find that the smoke is highly absorbing of sunlight, mostly because it contains more black carbon than smoke over the Northern Hemisphere.
Emily D. Lenhardt, Lan Gao, Jens Redemann, Feng Xu, Sharon P. Burton, Brian Cairns, Ian Chang, Richard A. Ferrare, Chris A. Hostetler, Pablo E. Saide, Calvin Howes, Yohei Shinozuka, Snorre Stamnes, Mary Kacarab, Amie Dobracki, Jenny Wong, Steffen Freitag, and Athanasios Nenes
Atmos. Meas. Tech., 16, 2037–2054, https://doi.org/10.5194/amt-16-2037-2023, https://doi.org/10.5194/amt-16-2037-2023, 2023
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Small atmospheric particles, such as smoke from wildfires or pollutants from human activities, impact cloud properties, and clouds have a strong influence on climate. To better understand the distributions of these particles, we develop relationships to derive their concentrations from remote sensing measurements from an instrument called a lidar. Our method is reliable for smoke particles, and similar steps can be taken to develop relationships for other particle types.
Ian Chang, Lan Gao, Connor J. Flynn, Yohei Shinozuka, Sarah J. Doherty, Michael S. Diamond, Karla M. Longo, Gonzalo A. Ferrada, Gregory R. Carmichael, Patricia Castellanos, Arlindo M. da Silva, Pablo E. Saide, Calvin Howes, Zhixin Xue, Marc Mallet, Ravi Govindaraju, Qiaoqiao Wang, Yafang Cheng, Yan Feng, Sharon P. Burton, Richard A. Ferrare, Samuel E. LeBlanc, Meloë S. Kacenelenbogen, Kristina Pistone, Michal Segal-Rozenhaimer, Kerry G. Meyer, Ju-Mee Ryoo, Leonhard Pfister, Adeyemi A. Adebiyi, Robert Wood, Paquita Zuidema, Sundar A. Christopher, and Jens Redemann
Atmos. Chem. Phys., 23, 4283–4309, https://doi.org/10.5194/acp-23-4283-2023, https://doi.org/10.5194/acp-23-4283-2023, 2023
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Abundant aerosols are present above low-level liquid clouds over the southeastern Atlantic during late austral spring. The model simulation differences in the proportion of aerosol residing in the planetary boundary layer and in the free troposphere can greatly affect the regional aerosol radiative effects. This study examines the aerosol loading and fractional aerosol loading in the free troposphere among various models and evaluates them against measurements from the NASA ORACLES campaign.
Francesca Gallo, Janek Uin, Kevin J. Sanchez, Richard H. Moore, Jian Wang, Robert Wood, Fan Mei, Connor Flynn, Stephen Springston, Eduardo B. Azevedo, Chongai Kuang, and Allison C. Aiken
Atmos. Chem. Phys., 23, 4221–4246, https://doi.org/10.5194/acp-23-4221-2023, https://doi.org/10.5194/acp-23-4221-2023, 2023
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This study provides a summary statistic of multiday aerosol plume transport event influences on aerosol physical properties and the cloud condensation nuclei budget at the U.S. Department of Energy Atmospheric Radiation Measurement Facility in the eastern North Atlantic (ENA). An algorithm that integrates aerosol properties is developed and applied to identify multiday aerosol transport events. The influence of the aerosol plumes on aerosol populations at the ENA is successively assessed.
Alice F. Wells, Andy Jones, Martin Osborne, Lilly Damany-Pearce, Daniel G. Partridge, and James M. Haywood
Atmos. Chem. Phys., 23, 3985–4007, https://doi.org/10.5194/acp-23-3985-2023, https://doi.org/10.5194/acp-23-3985-2023, 2023
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In 2019 the Raikoke volcano erupted explosively, emitting the largest injection of SO2 into the stratosphere since 2011. Observations indicated that a large amount of volcanic ash was also injected. Previous studies have identified that volcanic ash can prolong the lifetime of stratospheric aerosol optical depth, which we explore in UKESM1. Comparisons to observations suggest that including ash in model emission schemes can improve the representation of volcanic plumes in global climate models.
Kai Krause, Folkard Wittrock, Andreas Richter, Dieter Busch, Anton Bergen, John P. Burrows, Steffen Freitag, and Olesia Halbherr
Atmos. Meas. Tech., 16, 1767–1787, https://doi.org/10.5194/amt-16-1767-2023, https://doi.org/10.5194/amt-16-1767-2023, 2023
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Inland shipping is an important source of nitrogen oxides (NOx). The amount of emitted NOx depends on the characteristics of the individual vessels and the traffic density. Ship emissions are often characterised by the amount of emitted NOx per unit of burnt fuel, and further knowledge about fuel consumption is needed to quantify the total emissions caused by ship traffic. In this study, a new approach to derive absolute emission rates (in g s−1) from onshore measurements is presented.
Ruhi S. Humphries, Melita D. Keywood, Jason P. Ward, James Harnwell, Simon P. Alexander, Andrew R. Klekociuk, Keiichiro Hara, Ian M. McRobert, Alain Protat, Joel Alroe, Luke T. Cravigan, Branka Miljevic, Zoran D. Ristovski, Robyn Schofield, Stephen R. Wilson, Connor J. Flynn, Gourihar R. Kulkarni, Gerald G. Mace, Greg M. McFarquhar, Scott D. Chambers, Alastair G. Williams, and Alan D. Griffiths
Atmos. Chem. Phys., 23, 3749–3777, https://doi.org/10.5194/acp-23-3749-2023, https://doi.org/10.5194/acp-23-3749-2023, 2023
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Observations of aerosols in pristine regions are rare but are vital to constraining the natural baseline from which climate simulations are calculated. Here we present recent seasonal observations of aerosols from the Southern Ocean and contrast them with measurements from Antarctica, Australia and regionally relevant voyages. Strong seasonal cycles persist, but striking differences occur at different latitudes. This study highlights the need for more long-term observations in remote regions.
Zhenquan Wang, Jian Yuan, Robert Wood, Yifan Chen, and Tiancheng Tong
Atmos. Chem. Phys., 23, 3247–3266, https://doi.org/10.5194/acp-23-3247-2023, https://doi.org/10.5194/acp-23-3247-2023, 2023
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This study develops a novel profile-based algorithm based on the ERA5 to estimate the inversion strength in the planetary boundary layer better than the previous inversion index, which is a key low-cloud-controlling factor. This improved measure is more effective at representing the meteorological influence on low-cloud variations. It can better constrain the meteorological influence on low clouds to better isolate cloud responses to aerosols or to estimate low cloud feedbacks in climate models.
Dalei Hao, Gautam Bisht, Karl Rittger, Timbo Stillinger, Edward Bair, Yu Gu, and L. Ruby Leung
The Cryosphere, 17, 673–697, https://doi.org/10.5194/tc-17-673-2023, https://doi.org/10.5194/tc-17-673-2023, 2023
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We comprehensively evaluated the snow simulations in E3SM land model over the western United States in terms of spatial patterns, temporal correlations, interannual variabilities, elevation gradients, and change with forest cover of snow properties and snow phenology. Our study underscores the need for diagnosing model biases and improving the model representations of snow properties and snow phenology in mountainous areas for more credible simulation and future projection of mountain snowpack.
Marios Chatziparaschos, Nikos Daskalakis, Stelios Myriokefalitakis, Nikos Kalivitis, Athanasios Nenes, María Gonçalves Ageitos, Montserrat Costa-Surós, Carlos Pérez García-Pando, Medea Zanoli, Mihalis Vrekoussis, and Maria Kanakidou
Atmos. Chem. Phys., 23, 1785–1801, https://doi.org/10.5194/acp-23-1785-2023, https://doi.org/10.5194/acp-23-1785-2023, 2023
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Ice formation is enabled by ice-nucleating particles (INP) at higher temperatures than homogeneous formation and can profoundly affect the properties of clouds. Our global model results show that K-feldspar is the most important contributor to INP concentrations globally, affecting mid-level mixed-phase clouds. However, quartz can significantly contribute and dominates the lowest and the highest altitudes of dust-derived INP, affecting mainly low-level and high-level mixed-phase clouds.
Chandan Sarangi, Yun Qian, L. Ruby Leung, Yang Zhang, Yufei Zou, and Yuhang Wang
Atmos. Chem. Phys., 23, 1769–1783, https://doi.org/10.5194/acp-23-1769-2023, https://doi.org/10.5194/acp-23-1769-2023, 2023
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We show that for air quality, the densely populated eastern US may see even larger impacts of wildfires due to long-distance smoke transport and associated positive climatic impacts, partially compensating the improvements from regulations on anthropogenic emissions. This study highlights the tension between natural and anthropogenic contributions and the non-local nature of air pollution that complicate regulatory strategies for improving future regional air quality for human health.
Ju Liang and Jim Haywood
Atmos. Chem. Phys., 23, 1687–1703, https://doi.org/10.5194/acp-23-1687-2023, https://doi.org/10.5194/acp-23-1687-2023, 2023
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The recent record-breaking flood events in China during the summer of 2021 highlight the importance of mitigating the risks from future changes in high-impact weather systems under global warming. Based on a state-of-the-art Earth system model, we demonstrate a pilot study on the responses of atmospheric rivers and extreme precipitation over East Asia to anthropogenically induced climate warming and an unconventional mitigation strategy – stratospheric aerosol injection.
Francesca Gallo, Kevin J. Sanchez, Bruce E. Anderson, Ryan Bennett, Matthew D. Brown, Ewan C. Crosbie, Chris Hostetler, Carolyn Jordan, Melissa Yang Martin, Claire E. Robinson, Lynn M. Russell, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Elizabeth B. Wiggins, Edward L. Winstead, Armin Wisthaler, Luke D. Ziemba, and Richard H. Moore
Atmos. Chem. Phys., 23, 1465–1490, https://doi.org/10.5194/acp-23-1465-2023, https://doi.org/10.5194/acp-23-1465-2023, 2023
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We integrate in situ ship- and aircraft-based measurements of aerosol, trace gases, and meteorological parameters collected during the NASA North Atlantic Aerosols and Marine Ecosystems Study (NAAMES) field campaigns in the western North Atlantic Ocean region. A comprehensive characterization of the vertical profiles of aerosol properties under different seasonal regimes is provided for improving the understanding of aerosol key processes and aerosol–cloud interactions in marine regions.
Je-Yun Chun, Robert Wood, Peter Blossey, and Sarah J. Doherty
Atmos. Chem. Phys., 23, 1345–1368, https://doi.org/10.5194/acp-23-1345-2023, https://doi.org/10.5194/acp-23-1345-2023, 2023
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We investigate the impact of injected aerosol on subtropical low marine clouds under a variety of meteorological conditions using high-resolution model simulations. This study illustrates processes perturbed by aerosol injections and their impact on cloud properties (e.g., cloud number concentration, thickness, and cover). We show that those responses are highly sensitive to background meteorological conditions, such as precipitation, and background cloud properties.
Haley M. Royer, Mira L. Pöhlker, Ovid Krüger, Edmund Blades, Peter Sealy, Nurun Nahar Lata, Zezhen Cheng, Swarup China, Andrew P. Ault, Patricia K. Quinn, Paquita Zuidema, Christopher Pöhlker, Ulrich Pöschl, Meinrat Andreae, and Cassandra J. Gaston
Atmos. Chem. Phys., 23, 981–998, https://doi.org/10.5194/acp-23-981-2023, https://doi.org/10.5194/acp-23-981-2023, 2023
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This paper presents atmospheric particle chemical composition and measurements of aerosol water uptake properties collected at Ragged Point, Barbados, during the winter of 2020. The result of this study indicates the importance of small African smoke particles for cloud droplet formation in the tropical North Atlantic and highlights the large spatial and temporal pervasiveness of smoke over the Atlantic Ocean.
Jianhao Zhang and Graham Feingold
Atmos. Chem. Phys., 23, 1073–1090, https://doi.org/10.5194/acp-23-1073-2023, https://doi.org/10.5194/acp-23-1073-2023, 2023
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Using observations from space, we show maps of potential brightness changes in marine warm clouds in response to increases in cloud droplet concentrations. The environmental and aerosol conditions in which these clouds reside covary differently in each ocean basin, leading to distinct evolutions of cloud brightness changes. This work stresses the central importance of the covariability between meteorology and aerosol for scaling up the radiative response of cloud brightness changes.
Daniele Visioni, Ewa M. Bednarz, Walker R. Lee, Ben Kravitz, Andy Jones, Jim M. Haywood, and Douglas G. MacMartin
Atmos. Chem. Phys., 23, 663–685, https://doi.org/10.5194/acp-23-663-2023, https://doi.org/10.5194/acp-23-663-2023, 2023
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The paper constitutes Part 1 of a study performing a first systematic inter-model comparison of the atmospheric responses to stratospheric sulfate aerosol injections (SAIs) at various latitudes as simulated by three state-of-the-art Earth system models. We identify similarities and differences in the modeled aerosol burden, investigate the differences in the aerosol approaches between the models, and ultimately show the differences produced in surface climate, temperature and precipitation.
Ewa M. Bednarz, Daniele Visioni, Ben Kravitz, Andy Jones, James M. Haywood, Jadwiga Richter, Douglas G. MacMartin, and Peter Braesicke
Atmos. Chem. Phys., 23, 687–709, https://doi.org/10.5194/acp-23-687-2023, https://doi.org/10.5194/acp-23-687-2023, 2023
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Building on Part 1 of this two-part study, we demonstrate the role of biases in climatological circulation and specific aspects of model microphysics in driving the differences in simulated sulfate distributions amongst three Earth system models. We then characterize the simulated changes in stratospheric and free-tropospheric temperatures, ozone, water vapor, and large-scale circulation, elucidating the role of the above aspects in the surface responses discussed in Part 1.
Dalei Hao, Gautam Bisht, Karl Rittger, Edward Bair, Cenlin He, Huilin Huang, Cheng Dang, Timbo Stillinger, Yu Gu, Hailong Wang, Yun Qian, and L. Ruby Leung
Geosci. Model Dev., 16, 75–94, https://doi.org/10.5194/gmd-16-75-2023, https://doi.org/10.5194/gmd-16-75-2023, 2023
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Snow with the highest albedo of land surface plays a vital role in Earth’s surface energy budget and water cycle. This study accounts for the impacts of snow grain shape and mixing state of light-absorbing particles with snow on snow albedo in the E3SM land model. The findings advance our understanding of the role of snow grain shape and mixing state of LAP–snow in land surface processes and offer guidance for improving snow simulations and radiative forcing estimates in Earth system models.
Pamela S. Rickly, Hongyu Guo, Pedro Campuzano-Jost, Jose L. Jimenez, Glenn M. Wolfe, Ryan Bennett, Ilann Bourgeois, John D. Crounse, Jack E. Dibb, Joshua P. DiGangi, Glenn S. Diskin, Maximilian Dollner, Emily M. Gargulinski, Samuel R. Hall, Hannah S. Halliday, Thomas F. Hanisco, Reem A. Hannun, Jin Liao, Richard Moore, Benjamin A. Nault, John B. Nowak, Jeff Peischl, Claire E. Robinson, Thomas Ryerson, Kevin J. Sanchez, Manuel Schöberl, Amber J. Soja, Jason M. St. Clair, Kenneth L. Thornhill, Kirk Ullmann, Paul O. Wennberg, Bernadett Weinzierl, Elizabeth B. Wiggins, Edward L. Winstead, and Andrew W. Rollins
Atmos. Chem. Phys., 22, 15603–15620, https://doi.org/10.5194/acp-22-15603-2022, https://doi.org/10.5194/acp-22-15603-2022, 2022
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Biomass burning sulfur dioxide (SO2) emission factors range from 0.27–1.1 g kg-1 C. Biomass burning SO2 can quickly form sulfate and organosulfur, but these pathways are dependent on liquid water content and pH. Hydroxymethanesulfonate (HMS) appears to be directly emitted from some fire sources but is not the sole contributor to the organosulfur signal. It is shown that HMS and organosulfur chemistry may be an important S(IV) reservoir with the fate dependent on the surrounding conditions.
Rachel A. Bergin, Monica Harkey, Alicia Hoffman, Richard H. Moore, Bruce Anderson, Andreas Beyersdorf, Luke Ziemba, Lee Thornhill, Edward Winstead, Tracey Holloway, and Timothy H. Bertram
Atmos. Chem. Phys., 22, 15449–15468, https://doi.org/10.5194/acp-22-15449-2022, https://doi.org/10.5194/acp-22-15449-2022, 2022
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Correctly predicting aerosol surface area concentrations is important for determining the rate of heterogeneous reactions in chemical transport models. Here, we compare aircraft measurements of aerosol surface area with a regional model. In polluted air masses, we show that the model underpredicts aerosol surface area by a factor of 2. Despite this disagreement, the representation of heterogeneous chemistry still dominates the overall uncertainty in the loss rate of molecules such as N2O5.
Ju-Mee Ryoo, Leonhard Pfister, Rei Ueyama, Paquita Zuidema, Robert Wood, Ian Chang, and Jens Redemann
Atmos. Chem. Phys., 22, 14209–14241, https://doi.org/10.5194/acp-22-14209-2022, https://doi.org/10.5194/acp-22-14209-2022, 2022
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The variability in the meteorological fields during each deployment is highly modulated at a daily to synoptic timescale. This paper, along with part 1, the climatological overview paper, provides a meteorological context for interpreting the airborne measurements gathered during the three ORACLES deployments. This study supports related studies focusing on the detailed investigation of the processes controlling stratocumulus decks, aerosol lifting, transport, and their interactions.
Paul A. Barrett, Steven J. Abel, Hugh Coe, Ian Crawford, Amie Dobracki, James Haywood, Steve Howell, Anthony Jones, Justin Langridge, Greg M. McFarquhar, Graeme J. Nott, Hannah Price, Jens Redemann, Yohei Shinozuka, Kate Szpek, Jonathan W. Taylor, Robert Wood, Huihui Wu, Paquita Zuidema, Stéphane Bauguitte, Ryan Bennett, Keith Bower, Hong Chen, Sabrina Cochrane, Michael Cotterell, Nicholas Davies, David Delene, Connor Flynn, Andrew Freedman, Steffen Freitag, Siddhant Gupta, David Noone, Timothy B. Onasch, James Podolske, Michael R. Poellot, Sebastian Schmidt, Stephen Springston, Arthur J. Sedlacek III, Jamie Trembath, Alan Vance, Maria A. Zawadowicz, and Jianhao Zhang
Atmos. Meas. Tech., 15, 6329–6371, https://doi.org/10.5194/amt-15-6329-2022, https://doi.org/10.5194/amt-15-6329-2022, 2022
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To better understand weather and climate, it is vital to go into the field and collect observations. Often measurements take place in isolation, but here we compared data from two aircraft and one ground-based site. This was done in order to understand how well measurements made on one platform compared to those made on another. Whilst this is easy to do in a controlled laboratory setting, it is more challenging in the real world, and so these comparisons are as valuable as they are rare.
Dongyu Feng, Zeli Tan, Darren Engwirda, Chang Liao, Donghui Xu, Gautam Bisht, Tian Zhou, Hong-Yi Li, and L. Ruby Leung
Hydrol. Earth Syst. Sci., 26, 5473–5491, https://doi.org/10.5194/hess-26-5473-2022, https://doi.org/10.5194/hess-26-5473-2022, 2022
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Sea level rise, storm surge and river discharge can cause coastal backwater effects in downstream sections of rivers, creating critical flood risks. This study simulates the backwater effects using a large-scale river model on a coastal-refined computational mesh. By decomposing the backwater drivers, we revealed their relative importance and long-term variations. Our analysis highlights the increasing strength of backwater effects due to sea level rise and more frequent storm surge.
Hossein Dadashazar, Andrea F. Corral, Ewan Crosbie, Sanja Dmitrovic, Simon Kirschler, Kayla McCauley, Richard Moore, Claire Robinson, Joseph S. Schlosser, Michael Shook, K. Lee Thornhill, Christiane Voigt, Edward Winstead, Luke Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 22, 13897–13913, https://doi.org/10.5194/acp-22-13897-2022, https://doi.org/10.5194/acp-22-13897-2022, 2022
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Multi-season airborne data over the northwestern Atlantic show that organic mass fraction and the relative amount of oxygenated organics within that fraction are enhanced in droplet residual particles as compared to particles below and above cloud. In-cloud aqueous processing is shown to be a potential driver of this compositional shift in cloud. This implies that aerosol–cloud interactions in the region reduce aerosol hygroscopicity due to the jump in the organic : sulfate ratio in cloud.
Yilin Fang, L. Ruby Leung, Charles D. Koven, Gautam Bisht, Matteo Detto, Yanyan Cheng, Nate McDowell, Helene Muller-Landau, S. Joseph Wright, and Jeffrey Q. Chambers
Geosci. Model Dev., 15, 7879–7901, https://doi.org/10.5194/gmd-15-7879-2022, https://doi.org/10.5194/gmd-15-7879-2022, 2022
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We develop a model that integrates an Earth system model with a three-dimensional hydrology model to explicitly resolve hillslope topography and water flow underneath the land surface to understand how local-scale hydrologic processes modulate vegetation along water availability gradients. Our coupled model can be used to improve the understanding of the diverse impact of local heterogeneity and water flux on nutrient availability and plant communities.
Ewan Crosbie, Luke D. Ziemba, Michael A. Shook, Claire E. Robinson, Edward L. Winstead, K. Lee Thornhill, Rachel A. Braun, Alexander B. MacDonald, Connor Stahl, Armin Sorooshian, Susan C. van den Heever, Joshua P. DiGangi, Glenn S. Diskin, Sarah Woods, Paola Bañaga, Matthew D. Brown, Francesca Gallo, Miguel Ricardo A. Hilario, Carolyn E. Jordan, Gabrielle R. Leung, Richard H. Moore, Kevin J. Sanchez, Taylor J. Shingler, and Elizabeth B. Wiggins
Atmos. Chem. Phys., 22, 13269–13302, https://doi.org/10.5194/acp-22-13269-2022, https://doi.org/10.5194/acp-22-13269-2022, 2022
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The linkage between cloud droplet and aerosol particle chemical composition was analyzed using samples collected in a polluted tropical marine environment. Variations in the droplet composition were related to physical and dynamical processes in clouds to assess their relative significance across three cases that spanned a range of rainfall amounts. In spite of the pollution, sea salt still remained a major contributor to the droplet composition and was preferentially enhanced in rainwater.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, Michael R. Poellot, David J. Delene, Ian Chang, Lan Gao, Feng Xu, and Jens Redemann
Atmos. Chem. Phys., 22, 12923–12943, https://doi.org/10.5194/acp-22-12923-2022, https://doi.org/10.5194/acp-22-12923-2022, 2022
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The ability of NASA’s Terra and Aqua satellites to retrieve cloud properties and estimate the changes in cloud properties due to aerosol–cloud interactions (ACI) was examined. There was good agreement between satellite retrievals and in situ measurements over the southeast Atlantic Ocean. This suggests that, combined with information on aerosol properties, satellite retrievals of cloud properties can be used to study ACI over larger domains and longer timescales in the absence of in situ data.
Youngseob Kim, Lya Lugon, Alice Maison, Thibaud Sarica, Yelva Roustan, Myrto Valari, Yang Zhang, Michel André, and Karine Sartelet
Geosci. Model Dev., 15, 7371–7396, https://doi.org/10.5194/gmd-15-7371-2022, https://doi.org/10.5194/gmd-15-7371-2022, 2022
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This paper presents the latest version of the street-network model MUNICH, v2.0. The description of MUNICH v1.0, which models gas-phase pollutants in a street network, was published in GMD in 2018. Since then, major modifications have been made to MUNICH. The comprehensive aerosol model SSH-aerosol is now coupled to MUNICH to simulate primary and secondary aerosol concentrations. New parameterisations have also been introduced. Test cases are defined to illustrate the new model functionalities.
Nicole A. June, Anna L. Hodshire, Elizabeth B. Wiggins, Edward L. Winstead, Claire E. Robinson, K. Lee Thornhill, Kevin J. Sanchez, Richard H. Moore, Demetrios Pagonis, Hongyu Guo, Pedro Campuzano-Jost, Jose L. Jimenez, Matthew M. Coggon, Jonathan M. Dean-Day, T. Paul Bui, Jeff Peischl, Robert J. Yokelson, Matthew J. Alvarado, Sonia M. Kreidenweis, Shantanu H. Jathar, and Jeffrey R. Pierce
Atmos. Chem. Phys., 22, 12803–12825, https://doi.org/10.5194/acp-22-12803-2022, https://doi.org/10.5194/acp-22-12803-2022, 2022
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The evolution of organic aerosol composition and size is uncertain due to variability within and between smoke plumes. We examine the impact of plume concentration on smoke evolution from smoke plumes sampled by the NASA DC-8 during FIREX-AQ. We find that observed organic aerosol and size distribution changes are correlated to plume aerosol mass concentrations. Additionally, coagulation explains the majority of the observed growth.
Flossie Brown, Gerd A. Folberth, Stephen Sitch, Susanne Bauer, Marijn Bauters, Pascal Boeckx, Alexander W. Cheesman, Makoto Deushi, Inês Dos Santos Vieira, Corinne Galy-Lacaux, James Haywood, James Keeble, Lina M. Mercado, Fiona M. O'Connor, Naga Oshima, Kostas Tsigaridis, and Hans Verbeeck
Atmos. Chem. Phys., 22, 12331–12352, https://doi.org/10.5194/acp-22-12331-2022, https://doi.org/10.5194/acp-22-12331-2022, 2022
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Surface ozone can decrease plant productivity and impair human health. In this study, we evaluate the change in surface ozone due to climate change over South America and Africa using Earth system models. We find that if the climate were to change according to the worst-case scenario used here, models predict that forested areas in biomass burning locations and urban populations will be at increasing risk of ozone exposure, but other areas will experience a climate benefit.
Zhipeng Qu, Alexei Korolev, Jason A. Milbrandt, Ivan Heckman, Yongjie Huang, Greg M. McFarquhar, Hugh Morrison, Mengistu Wolde, and Cuong Nguyen
Atmos. Chem. Phys., 22, 12287–12310, https://doi.org/10.5194/acp-22-12287-2022, https://doi.org/10.5194/acp-22-12287-2022, 2022
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Secondary ice production (SIP) is an important physical phenomenon that results in an increase in the cloud ice particle concentration and can have a significant impact on the evolution of clouds. Here, idealized simulations of a tropical convective system were conducted. Agreement between the simulations and observations highlights the impacts of SIP on the maintenance of tropical convection in nature and the importance of including the modelling of SIP in numerical weather prediction models.
Michael S. Diamond, Pablo E. Saide, Paquita Zuidema, Andrew S. Ackerman, Sarah J. Doherty, Ann M. Fridlind, Hamish Gordon, Calvin Howes, Jan Kazil, Takanobu Yamaguchi, Jianhao Zhang, Graham Feingold, and Robert Wood
Atmos. Chem. Phys., 22, 12113–12151, https://doi.org/10.5194/acp-22-12113-2022, https://doi.org/10.5194/acp-22-12113-2022, 2022
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Smoke from southern Africa blankets the southeast Atlantic from June-October, overlying a major transition region between overcast and scattered clouds. The smoke affects Earth's radiation budget by absorbing sunlight and changing cloud properties. We investigate these effects in regional climate and large eddy simulation models based on international field campaigns. We find that large-scale circulation changes more strongly affect cloud transitions than smoke microphysical effects in our case.
Samuel E. LeBlanc, Michal Segal-Rozenhaimer, Jens Redemann, Connor Flynn, Roy R. Johnson, Stephen E. Dunagan, Robert Dahlgren, Jhoon Kim, Myungje Choi, Arlindo da Silva, Patricia Castellanos, Qian Tan, Luke Ziemba, Kenneth Lee Thornhill, and Meloë Kacenelenbogen
Atmos. Chem. Phys., 22, 11275–11304, https://doi.org/10.5194/acp-22-11275-2022, https://doi.org/10.5194/acp-22-11275-2022, 2022
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Airborne observations of atmospheric particles and pollution over Korea during a field campaign in May–June 2016 showed that the smallest atmospheric particles are present in the lowest 2 km of the atmosphere. The aerosol size is more spatially variable than optical thickness. We show this with remote sensing (4STAR), in situ (LARGE) observations, satellite measurements (GOCI), and modeled properties (MERRA-2), and it is contrary to the current understanding.
Meng Huang, Po-Lun Ma, Nathaniel W. Chaney, Dalei Hao, Gautam Bisht, Megan D. Fowler, Vincent E. Larson, and L. Ruby Leung
Geosci. Model Dev., 15, 6371–6384, https://doi.org/10.5194/gmd-15-6371-2022, https://doi.org/10.5194/gmd-15-6371-2022, 2022
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The land surface in one grid cell may be diverse in character. This study uses an explicit way to account for that subgrid diversity in a state-of-the-art Earth system model (ESM) and explores its implications for the overlying atmosphere. We find that the shallow clouds are increased significantly with the land surface diversity. Our work highlights the importance of accurately representing the land surface and its interaction with the atmosphere in next-generation ESMs.
Yilin Fang, L. Ruby Leung, Ryan Knox, Charlie Koven, and Ben Bond-Lamberty
Geosci. Model Dev., 15, 6385–6398, https://doi.org/10.5194/gmd-15-6385-2022, https://doi.org/10.5194/gmd-15-6385-2022, 2022
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Accounting for water movement in the soil and water transport within the plant is important for plant growth in Earth system modeling. We implemented different numerical approaches for a plant hydrodynamic model and compared their impacts on the simulated aboveground biomass (AGB) at single points and globally. We found care should be taken when discretizing the number of soil layers for numerical simulations as it can significantly affect AGB if accuracy and computational costs are of concern.
Jessica Danker, Odran Sourdeval, Isabel L. McCoy, Robert Wood, and Anna Possner
Atmos. Chem. Phys., 22, 10247–10265, https://doi.org/10.5194/acp-22-10247-2022, https://doi.org/10.5194/acp-22-10247-2022, 2022
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Using spaceborne lidar-radar retrievals, we show that seasonal changes in cloud phase outweigh changes in cloud-phase statistics across cloud morphologies at given cloud-top temperatures. These results show that cloud morphology does not seem to pose a primary constraint on cloud-phase statistics in the Southern Ocean. Meanwhile, larger changes in in-cloud albedo across cloud morphologies are observed in supercooled liquid rather than mixed-phase stratocumuli.
Caroline Dang, Michal Segal-Rozenhaimer, Haochi Che, Lu Zhang, Paola Formenti, Jonathan Taylor, Amie Dobracki, Sara Purdue, Pui-Shan Wong, Athanasios Nenes, Arthur Sedlacek III, Hugh Coe, Jens Redemann, Paquita Zuidema, Steven Howell, and James Haywood
Atmos. Chem. Phys., 22, 9389–9412, https://doi.org/10.5194/acp-22-9389-2022, https://doi.org/10.5194/acp-22-9389-2022, 2022
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Transmission electron microscopy was used to analyze aged African smoke particles and how the smoke interacts with the marine atmosphere. We found that the volatility of organic aerosol increases with biomass burning plume age, that black carbon is often mixed with potassium salts and that the marine atmosphere can incorporate Na and Cl into smoke particles. Marine salts are more processed when mixed with smoke plumes, and there are interesting Cl-rich yet Na-absent marine particles.
Sol Kim, L. Ruby Leung, Bin Guan, and John C. H. Chiang
Geosci. Model Dev., 15, 5461–5480, https://doi.org/10.5194/gmd-15-5461-2022, https://doi.org/10.5194/gmd-15-5461-2022, 2022
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The Energy Exascale Earth System Model (E3SM) project is a state-of-the-science Earth system model developed by the US Department of Energy (DOE). Understanding how the water cycle behaves in this model is of particular importance to the DOE’s mission. Atmospheric rivers (ARs) – which are crucial to the global water cycle – move vast amounts of water vapor through the sky and produce rain and snow. We find that this model reliably represents atmospheric rivers around the world.
Lingcheng Li, Gautam Bisht, and L. Ruby Leung
Geosci. Model Dev., 15, 5489–5510, https://doi.org/10.5194/gmd-15-5489-2022, https://doi.org/10.5194/gmd-15-5489-2022, 2022
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Land surface heterogeneity plays a critical role in the terrestrial water, energy, and biogeochemical cycles. Our study systematically quantified the effects of four dominant heterogeneity sources on water and energy partitioning via Sobol' indices. We found that atmospheric forcing and land use land cover are the most dominant heterogeneity sources in determining spatial variability of water and energy partitioning. Our findings can help prioritize the future development of land surface models.
Lu Zhang, Michal Segal-Rozenhaimer, Haochi Che, Caroline Dang, Arthur J. Sedlacek III, Ernie R. Lewis, Amie Dobracki, Jenny P. S. Wong, Paola Formenti, Steven G. Howell, and Athanasios Nenes
Atmos. Chem. Phys., 22, 9199–9213, https://doi.org/10.5194/acp-22-9199-2022, https://doi.org/10.5194/acp-22-9199-2022, 2022
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Widespread biomass burning (BB) events occur annually in Africa and contribute ~ 1 / 3 of global BB emissions, which contain a large family of light-absorbing organics, known as brown carbon (BrC), whose absorption of incident radiation is difficult to estimate, leading to large uncertainties in the global radiative forcing estimation. This study quantifies the BrC absorption of aged BB particles and highlights the potential presence of absorbing iron oxides in this climatically important region.
Kai Zhang, Wentao Zhang, Hui Wan, Philip J. Rasch, Steven J. Ghan, Richard C. Easter, Xiangjun Shi, Yong Wang, Hailong Wang, Po-Lun Ma, Shixuan Zhang, Jian Sun, Susannah M. Burrows, Manish Shrivastava, Balwinder Singh, Yun Qian, Xiaohong Liu, Jean-Christophe Golaz, Qi Tang, Xue Zheng, Shaocheng Xie, Wuyin Lin, Yan Feng, Minghuai Wang, Jin-Ho Yoon, and L. Ruby Leung
Atmos. Chem. Phys., 22, 9129–9160, https://doi.org/10.5194/acp-22-9129-2022, https://doi.org/10.5194/acp-22-9129-2022, 2022
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Here we analyze the effective aerosol forcing simulated by E3SM version 1 using both century-long free-running and short nudged simulations. The aerosol forcing in E3SMv1 is relatively large compared to other models, mainly due to the large indirect aerosol effect. Aerosol-induced changes in liquid and ice cloud properties in E3SMv1 have a strong correlation. The aerosol forcing estimates in E3SMv1 are sensitive to the parameterization changes in both liquid and ice cloud processes.
Haochi Che, Michal Segal-Rozenhaimer, Lu Zhang, Caroline Dang, Paquita Zuidema, Arthur J. Sedlacek III, Xiaoye Zhang, and Connor Flynn
Atmos. Chem. Phys., 22, 8767–8785, https://doi.org/10.5194/acp-22-8767-2022, https://doi.org/10.5194/acp-22-8767-2022, 2022
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A 17-month in situ study on Ascension Island found low single-scattering albedo and strong absorption enhancement of the marine boundary layer aerosols during biomass burnings on the African continent, along with apparent patterns of regular monthly variability. We further discuss the characteristics and drivers behind these changes and find that biomass burning conditions in Africa may be the main factor influencing the optical properties of marine boundary aerosols.
Donghui Xu, Gautam Bisht, Khachik Sargsyan, Chang Liao, and L. Ruby Leung
Geosci. Model Dev., 15, 5021–5043, https://doi.org/10.5194/gmd-15-5021-2022, https://doi.org/10.5194/gmd-15-5021-2022, 2022
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The runoff outputs in Earth system model simulations involve high uncertainty, which needs to be constrained by parameter calibration. In this work, we used a surrogate-assisted Bayesian framework to efficiently calibrate the runoff-generation processes in the Energy Exascale Earth System Model v1 at a global scale. The model performance was improved compared to the default parameter after calibration, and the associated parametric uncertainty was significantly constrained.
Simon Kirschler, Christiane Voigt, Bruce Anderson, Ramon Campos Braga, Gao Chen, Andrea F. Corral, Ewan Crosbie, Hossein Dadashazar, Richard A. Ferrare, Valerian Hahn, Johannes Hendricks, Stefan Kaufmann, Richard Moore, Mira L. Pöhlker, Claire Robinson, Amy J. Scarino, Dominik Schollmayer, Michael A. Shook, K. Lee Thornhill, Edward Winstead, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 22, 8299–8319, https://doi.org/10.5194/acp-22-8299-2022, https://doi.org/10.5194/acp-22-8299-2022, 2022
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In this study we show that the vertical velocity dominantly impacts the cloud droplet number concentration (NC) of low-level clouds over the western North Atlantic in the winter and summer season, while the cloud condensation nuclei concentration, aerosol size distribution and chemical composition impact NC within a season. The observational data presented in this study can evaluate and improve the representation of aerosol–cloud interactions for a wide range of conditions.
Dongwei Fu, Larry Di Girolamo, Robert M. Rauber, Greg M. McFarquhar, Stephen W. Nesbitt, Jesse Loveridge, Yulan Hong, Bastiaan van Diedenhoven, Brian Cairns, Mikhail D. Alexandrov, Paul Lawson, Sarah Woods, Simone Tanelli, Sebastian Schmidt, Chris Hostetler, and Amy Jo Scarino
Atmos. Chem. Phys., 22, 8259–8285, https://doi.org/10.5194/acp-22-8259-2022, https://doi.org/10.5194/acp-22-8259-2022, 2022
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Satellite-retrieved cloud microphysics are widely used in climate research because of their central role in water and energy cycles. Here, we provide the first detailed investigation of retrieved cloud drop sizes from in situ and various satellite and airborne remote sensing techniques applied to real cumulus cloud fields. We conclude that the most widely used passive remote sensing method employed in climate research produces high biases of 6–8 µm (60 %–80 %) caused by 3-D radiative effects.
Yun Lin, Jiwen Fan, Pengfei Li, Lai-yung Ruby Leung, Paul J. DeMott, Lexie Goldberger, Jennifer Comstock, Ying Liu, Jong-Hoon Jeong, and Jason Tomlinson
Atmos. Chem. Phys., 22, 6749–6771, https://doi.org/10.5194/acp-22-6749-2022, https://doi.org/10.5194/acp-22-6749-2022, 2022
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How sea spray aerosols may affect cloud and precipitation over the region by acting as ice-nucleating particles (INPs) is unknown. We explored the effects of INPs from marine aerosols on orographic cloud and precipitation for an atmospheric river event observed during the 2015 ACAPEX field campaign. The marine INPs enhance the formation of ice and snow, leading to less shallow warm clouds but more mixed-phase and deep clouds. This work suggests models need to consider the impacts of marine INPs.
Jim M. Haywood, Andy Jones, Ben T. Johnson, and William McFarlane Smith
Atmos. Chem. Phys., 22, 6135–6150, https://doi.org/10.5194/acp-22-6135-2022, https://doi.org/10.5194/acp-22-6135-2022, 2022
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Simulations are presented investigating the influence of moderately absorbing aerosol in the stratosphere to combat the impacts of climate change. A number of detrimental impacts are noted compared to sulfate aerosol, including (i) reduced cooling efficiency, (ii) increased deficits in global precipitation, (iii) delays in the recovery of the stratospheric ozone hole, and (iv) disruption of the stratospheric circulation and the wintertime storm tracks that impact European precipitation.
Pinya Wang, Yang Yang, Huimin Li, Lei Chen, Ruijun Dang, Daokai Xue, Baojie Li, Jianping Tang, L. Ruby Leung, and Hong Liao
Atmos. Chem. Phys., 22, 4705–4719, https://doi.org/10.5194/acp-22-4705-2022, https://doi.org/10.5194/acp-22-4705-2022, 2022
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China is now suffering from both severe ozone (O3) pollution and heat events. We highlight that North China Plain is the hot spot of the co-occurrences of extremes in O3 and high temperatures in China. Such coupled extremes exhibit an increasing trend during 2014–2019 and will continue to increase until the middle of this century. And the coupled extremes impose more severe health impacts to human than O3 pollution occurring alone because of elevated O3 levels and temperatures.
Stelios Myriokefalitakis, Elisa Bergas-Massó, María Gonçalves-Ageitos, Carlos Pérez García-Pando, Twan van Noije, Philippe Le Sager, Akinori Ito, Eleni Athanasopoulou, Athanasios Nenes, Maria Kanakidou, Maarten C. Krol, and Evangelos Gerasopoulos
Geosci. Model Dev., 15, 3079–3120, https://doi.org/10.5194/gmd-15-3079-2022, https://doi.org/10.5194/gmd-15-3079-2022, 2022
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We here describe the implementation of atmospheric multiphase processes in the EC-Earth Earth system model. We provide global budgets of oxalate, sulfate, and iron-containing aerosols, along with an analysis of the links among atmospheric composition, aqueous-phase processes, and aerosol dissolution, supported by comparison to observations. This work is a first step towards an interactive calculation of the deposition of bioavailable atmospheric iron coupled to the model’s ocean component.
Simone Tilmes, Daniele Visioni, Andy Jones, James Haywood, Roland Séférian, Pierre Nabat, Olivier Boucher, Ewa Monica Bednarz, and Ulrike Niemeier
Atmos. Chem. Phys., 22, 4557–4579, https://doi.org/10.5194/acp-22-4557-2022, https://doi.org/10.5194/acp-22-4557-2022, 2022
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This study assesses the impacts of climate interventions, using stratospheric sulfate aerosol and solar dimming on stratospheric ozone, based on three Earth system models with interactive stratospheric chemistry. The climate interventions have been applied to a high emission (baseline) scenario in order to reach global surface temperatures of a medium emission scenario. We find significant increases and decreases in total column ozone, depending on regions and seasons.
Po-Lun Ma, Bryce E. Harrop, Vincent E. Larson, Richard B. Neale, Andrew Gettelman, Hugh Morrison, Hailong Wang, Kai Zhang, Stephen A. Klein, Mark D. Zelinka, Yuying Zhang, Yun Qian, Jin-Ho Yoon, Christopher R. Jones, Meng Huang, Sheng-Lun Tai, Balwinder Singh, Peter A. Bogenschutz, Xue Zheng, Wuyin Lin, Johannes Quaas, Hélène Chepfer, Michael A. Brunke, Xubin Zeng, Johannes Mülmenstädt, Samson Hagos, Zhibo Zhang, Hua Song, Xiaohong Liu, Michael S. Pritchard, Hui Wan, Jingyu Wang, Qi Tang, Peter M. Caldwell, Jiwen Fan, Larry K. Berg, Jerome D. Fast, Mark A. Taylor, Jean-Christophe Golaz, Shaocheng Xie, Philip J. Rasch, and L. Ruby Leung
Geosci. Model Dev., 15, 2881–2916, https://doi.org/10.5194/gmd-15-2881-2022, https://doi.org/10.5194/gmd-15-2881-2022, 2022
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An alternative set of parameters for E3SM Atmospheric Model version 1 has been developed based on a tuning strategy that focuses on clouds. When clouds in every regime are improved, other aspects of the model are also improved, even though they are not the direct targets for calibration. The recalibrated model shows a lower sensitivity to anthropogenic aerosols and surface warming, suggesting potential improvements to the simulated climate in the past and future.
Chenjie Yu, Dantong Liu, Kang Hu, Ping Tian, Yangzhou Wu, Delong Zhao, Huihui Wu, Dawei Hu, Wenbo Guo, Qiang Li, Mengyu Huang, Deping Ding, and James D. Allan
Atmos. Chem. Phys., 22, 4375–4391, https://doi.org/10.5194/acp-22-4375-2022, https://doi.org/10.5194/acp-22-4375-2022, 2022
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In this study, we applied a new technique to investigate the aerosol properties on both a mass and number basis and CCN abilities in Beijing suburban regions. The size-resolved aerosol chemical compositions and CCN activation measurement enable a detailed analysis of BC-containing particle hygroscopicity and its size-dependent contribution to the CCN activation. The results presented in this study will affect future models and human health studies.
Glenn M. Wolfe, Thomas F. Hanisco, Heather L. Arkinson, Donald R. Blake, Armin Wisthaler, Tomas Mikoviny, Thomas B. Ryerson, Ilana Pollack, Jeff Peischl, Paul O. Wennberg, John D. Crounse, Jason M. St. Clair, Alex Teng, L. Gregory Huey, Xiaoxi Liu, Alan Fried, Petter Weibring, Dirk Richter, James Walega, Samuel R. Hall, Kirk Ullmann, Jose L. Jimenez, Pedro Campuzano-Jost, T. Paul Bui, Glenn Diskin, James R. Podolske, Glen Sachse, and Ronald C. Cohen
Atmos. Chem. Phys., 22, 4253–4275, https://doi.org/10.5194/acp-22-4253-2022, https://doi.org/10.5194/acp-22-4253-2022, 2022
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Smoke plumes are chemically complex. This work combines airborne observations of smoke plume composition with a photochemical model to probe the production of ozone and the fate of reactive gases in the outflow of a large wildfire. Model–measurement comparisons illustrate how uncertain emissions and chemical processes propagate into simulated chemical evolution. Results provide insight into how this system responds to perturbations, which can help guide future observation and modeling efforts.
Meloë S. F. Kacenelenbogen, Qian Tan, Sharon P. Burton, Otto P. Hasekamp, Karl D. Froyd, Yohei Shinozuka, Andreas J. Beyersdorf, Luke Ziemba, Kenneth L. Thornhill, Jack E. Dibb, Taylor Shingler, Armin Sorooshian, Reed W. Espinosa, Vanderlei Martins, Jose L. Jimenez, Pedro Campuzano-Jost, Joshua P. Schwarz, Matthew S. Johnson, Jens Redemann, and Gregory L. Schuster
Atmos. Chem. Phys., 22, 3713–3742, https://doi.org/10.5194/acp-22-3713-2022, https://doi.org/10.5194/acp-22-3713-2022, 2022
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The impact of aerosols on Earth's radiation budget and human health is important and strongly depends on their composition. One desire of our scientific community is to derive the composition of the aerosol from satellite sensors. However, satellites observe aerosol optical properties (and not aerosol composition) based on remote sensing instrumentation. This study assesses how much aerosol optical properties can tell us about aerosol composition.
Sally S.-C. Wang, Yun Qian, L. Ruby Leung, and Yang Zhang
Atmos. Chem. Phys., 22, 3445–3468, https://doi.org/10.5194/acp-22-3445-2022, https://doi.org/10.5194/acp-22-3445-2022, 2022
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This study develops an interpretable machine learning (ML) model predicting monthly PM2.5 fire emission over the contiguous US at 0.25° resolution and compares the prediction skills of the ML and process-based models. The comparison facilitates attributions of model biases and better understanding of the strengths and uncertainties in the two types of models at regional scales, for informing future model development and their applications in fire emission projection.
Matthew S. Norgren, John Wood, K. Sebastian Schmidt, Bastiaan van Diedenhoven, Snorre A. Stamnes, Luke D. Ziemba, Ewan C. Crosbie, Michael A. Shook, A. Scott Kittelman, Samuel E. LeBlanc, Stephen Broccardo, Steffen Freitag, and Jeffrey S. Reid
Atmos. Meas. Tech., 15, 1373–1394, https://doi.org/10.5194/amt-15-1373-2022, https://doi.org/10.5194/amt-15-1373-2022, 2022
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A new spectral instrument (SPN-S), with the ability to partition solar radiation into direct and diffuse components, is used in airborne settings to study the optical properties of aerosols and cirrus. It is a low-cost and mechanically simple system but has higher measurement uncertainty than existing standards. This challenge is overcome by utilizing the unique measurement capabilities to develop new retrieval techniques. Validation is done with data from two NASA airborne research campaigns.
Andy Jones, Jim M. Haywood, Adam A. Scaife, Olivier Boucher, Matthew Henry, Ben Kravitz, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Roland Séférian, Simone Tilmes, and Daniele Visioni
Atmos. Chem. Phys., 22, 2999–3016, https://doi.org/10.5194/acp-22-2999-2022, https://doi.org/10.5194/acp-22-2999-2022, 2022
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Simulations by six Earth-system models of geoengineering by introducing sulfuric acid aerosols into the tropical stratosphere are compared. A robust impact on the northern wintertime North Atlantic Oscillation is found, exacerbating precipitation reduction over parts of southern Europe. In contrast, the models show no consistency with regard to impacts on the Quasi-Biennial Oscillation, although results do indicate a risk that the oscillation could become locked into a permanent westerly phase.
Jessica Slater, Hugh Coe, Gordon McFiggans, Juha Tonttila, and Sami Romakkaniemi
Atmos. Chem. Phys., 22, 2937–2953, https://doi.org/10.5194/acp-22-2937-2022, https://doi.org/10.5194/acp-22-2937-2022, 2022
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This paper shows the specific impact of black carbon (BC) on the aerosol–planetary boundary layer (PBL) feedback and its influence on a Beijing haze episode. Overall, this paper shows that strong temperature inversions prevent BC heating within the PBL from significantly increasing PBL height, while BC above the PBL suppresses PBL development significantly through the day. From this we suggest a method by which both locally and regionally emitted BC may impact urban pollution episodes.
Kevin J. Sanchez, Bo Zhang, Hongyu Liu, Matthew D. Brown, Ewan C. Crosbie, Francesca Gallo, Johnathan W. Hair, Chris A. Hostetler, Carolyn E. Jordan, Claire E. Robinson, Amy Jo Scarino, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Elizabeth B. Wiggins, Edward L. Winstead, Luke D. Ziemba, Georges Saliba, Savannah L. Lewis, Lynn M. Russell, Patricia K. Quinn, Timothy S. Bates, Jack Porter, Thomas G. Bell, Peter Gaube, Eric S. Saltzman, Michael J. Behrenfeld, and Richard H. Moore
Atmos. Chem. Phys., 22, 2795–2815, https://doi.org/10.5194/acp-22-2795-2022, https://doi.org/10.5194/acp-22-2795-2022, 2022
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Atmospheric particle concentrations impact clouds, which strongly impact the amount of sunlight reflected back into space and the overall climate. Measurements of particles over the ocean are rare and expensive to collect, so models are necessary to fill in the gaps by simulating both particle and clouds. However, some measurements are needed to test the accuracy of the models. Here, we measure changes in particles in different weather conditions, which are ideal for comparison with models.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, Michael R. Poellot, David J. Delene, Rose M. Miller, and Jennifer D. Small Griswold
Atmos. Chem. Phys., 22, 2769–2793, https://doi.org/10.5194/acp-22-2769-2022, https://doi.org/10.5194/acp-22-2769-2022, 2022
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This study evaluates the impact of biomass burning aerosols on precipitation in marine stratocumulus clouds using observations from the NASA ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) field campaign over the Southeast Atlantic. Instances of contact and separation between aerosol and cloud layers show polluted clouds have a lower precipitation rate and a lower precipitation susceptibility. This information will help improve cloud representation in Earth system models.
Guta Wakbulcho Abeshu, Hong-Yi Li, Zhenduo Zhu, Zeli Tan, and L. Ruby Leung
Earth Syst. Sci. Data, 14, 929–942, https://doi.org/10.5194/essd-14-929-2022, https://doi.org/10.5194/essd-14-929-2022, 2022
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Existing riverbed sediment particle size data are sparsely available at individual sites. We develop a continuous map of median riverbed sediment particle size over the contiguous US corresponding to millions of river segments based on the existing observations and machine learning methods. This map is useful for research in large-scale river sediment using model- and data-driven approaches, teaching environmental and earth system sciences, planning and managing floodplain zones, etc.
Yongjie Huang, Wei Wu, Greg M. McFarquhar, Ming Xue, Hugh Morrison, Jason Milbrandt, Alexei V. Korolev, Yachao Hu, Zhipeng Qu, Mengistu Wolde, Cuong Nguyen, Alfons Schwarzenboeck, and Ivan Heckman
Atmos. Chem. Phys., 22, 2365–2384, https://doi.org/10.5194/acp-22-2365-2022, https://doi.org/10.5194/acp-22-2365-2022, 2022
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Numerous small ice crystals in tropical convective storms are difficult to detect and could be potentially hazardous for commercial aircraft. Previous numerical simulations failed to reproduce this phenomenon and hypothesized that key microphysical processes are still lacking in current models to realistically simulate the phenomenon. This study uses numerical experiments to confirm the dominant role of secondary ice production in the formation of these large numbers of small ice crystals.
Paraskevi Georgakaki, Georgia Sotiropoulou, Étienne Vignon, Anne-Claire Billault-Roux, Alexis Berne, and Athanasios Nenes
Atmos. Chem. Phys., 22, 1965–1988, https://doi.org/10.5194/acp-22-1965-2022, https://doi.org/10.5194/acp-22-1965-2022, 2022
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The modelling study focuses on the importance of ice multiplication processes in orographic mixed-phase clouds, which is one of the least understood cloud types in the climate system. We show that the consideration of ice seeding and secondary ice production through ice–ice collisional breakup is essential for correct predictions of precipitation in mountainous terrain, with important implications for radiation processes.
Hong-Yi Li, Zeli Tan, Hongbo Ma, Zhenduo Zhu, Guta Wakbulcho Abeshu, Senlin Zhu, Sagy Cohen, Tian Zhou, Donghui Xu, and L. Ruby Leung
Hydrol. Earth Syst. Sci., 26, 665–688, https://doi.org/10.5194/hess-26-665-2022, https://doi.org/10.5194/hess-26-665-2022, 2022
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We introduce a new multi-process river sediment module for Earth system models. Application and validation over the contiguous US indicate a satisfactory model performance over large river systems, including those heavily regulated by reservoirs. This new sediment module enables future modeling of the transportation and transformation of carbon and nutrients carried by the fine sediment along the river–ocean continuum to close the global carbon and nutrient cycles.
Jianhao Zhang, Xiaoli Zhou, Tom Goren, and Graham Feingold
Atmos. Chem. Phys., 22, 861–880, https://doi.org/10.5194/acp-22-861-2022, https://doi.org/10.5194/acp-22-861-2022, 2022
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Oceanic liquid-form clouds are effective sunlight reflectors. Their brightness is highly sensitive to changes in the amount of aerosol particles in the atmosphere and the state of the atmosphere they reside in. This study quantifies this sensitivity using long-term satellite observations and finds an overall cloud brightening (a cooling effect) potential and an essential role of the covarying meteorological conditions in governing this sensitivity for northeastern Pacific stratocumulus.
Matthew W. Christensen, Andrew Gettelman, Jan Cermak, Guy Dagan, Michael Diamond, Alyson Douglas, Graham Feingold, Franziska Glassmeier, Tom Goren, Daniel P. Grosvenor, Edward Gryspeerdt, Ralph Kahn, Zhanqing Li, Po-Lun Ma, Florent Malavelle, Isabel L. McCoy, Daniel T. McCoy, Greg McFarquhar, Johannes Mülmenstädt, Sandip Pal, Anna Possner, Adam Povey, Johannes Quaas, Daniel Rosenfeld, Anja Schmidt, Roland Schrödner, Armin Sorooshian, Philip Stier, Velle Toll, Duncan Watson-Parris, Robert Wood, Mingxi Yang, and Tianle Yuan
Atmos. Chem. Phys., 22, 641–674, https://doi.org/10.5194/acp-22-641-2022, https://doi.org/10.5194/acp-22-641-2022, 2022
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Trace gases and aerosols (tiny airborne particles) are released from a variety of point sources around the globe. Examples include volcanoes, industrial chimneys, forest fires, and ship stacks. These sources provide opportunistic experiments with which to quantify the role of aerosols in modifying cloud properties. We review the current state of understanding on the influence of aerosol on climate built from the wide range of natural and anthropogenic laboratories investigated in recent decades.
Sabrina P. Cochrane, K. Sebastian Schmidt, Hong Chen, Peter Pilewskie, Scott Kittelman, Jens Redemann, Samuel LeBlanc, Kristina Pistone, Michal Segal Rozenhaimer, Meloë Kacenelenbogen, Yohei Shinozuka, Connor Flynn, Rich Ferrare, Sharon Burton, Chris Hostetler, Marc Mallet, and Paquita Zuidema
Atmos. Meas. Tech., 15, 61–77, https://doi.org/10.5194/amt-15-61-2022, https://doi.org/10.5194/amt-15-61-2022, 2022
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This work presents heating rates derived from aircraft observations from the 2016 and 2017 field campaigns of ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS). We separate the total heating rates into aerosol and gas (primarily water vapor) absorption and explore some of the co-variability of heating rate profiles and their primary drivers, leading to the development of a new concept: the heating rate efficiency (HRE; the heating rate per unit aerosol extinction).
Sarah J. Doherty, Pablo E. Saide, Paquita Zuidema, Yohei Shinozuka, Gonzalo A. Ferrada, Hamish Gordon, Marc Mallet, Kerry Meyer, David Painemal, Steven G. Howell, Steffen Freitag, Amie Dobracki, James R. Podolske, Sharon P. Burton, Richard A. Ferrare, Calvin Howes, Pierre Nabat, Gregory R. Carmichael, Arlindo da Silva, Kristina Pistone, Ian Chang, Lan Gao, Robert Wood, and Jens Redemann
Atmos. Chem. Phys., 22, 1–46, https://doi.org/10.5194/acp-22-1-2022, https://doi.org/10.5194/acp-22-1-2022, 2022
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Between July and October, biomass burning smoke is advected over the southeastern Atlantic Ocean, leading to climate forcing. Model calculations of forcing by this plume vary significantly in both magnitude and sign. This paper compares aerosol and cloud properties observed during three NASA ORACLES field campaigns to the same in four models. It quantifies modeled biases in properties key to aerosol direct radiative forcing and evaluates how these biases propagate to biases in forcing.
Amie Dobracki, Paquita Zuidema, Steve Howell, Pablo Saide, Steffen Freitag, Allison C. Aiken, Sharon P. Burton, Arthur J. Sedlacek III, Jens Redemann, and Robert Wood
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-1081, https://doi.org/10.5194/acp-2021-1081, 2022
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The global maximum of shortwave-absorbing aerosol above cloud occurs above the southeast Atlantic, where the biomass-burning aerosol provides a distinct aerosol radiative warming of regional climate. The smoke aerosols are unusually highly absorbing of sunlight. This study seeks to understand the cause. We conclude the aerosol is already strongly absorbing at the fire emission source, but that chemical aging, through encouraging a net loss of organic aerosol, also contributes.
Ruili Wu, Christopher W. Tessum, Yang Zhang, Chaopeng Hong, Yixuan Zheng, Xinyin Qin, Shigan Liu, and Qiang Zhang
Geosci. Model Dev., 14, 7621–7638, https://doi.org/10.5194/gmd-14-7621-2021, https://doi.org/10.5194/gmd-14-7621-2021, 2021
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Reduced-complexity air quality models are less computationally intensive and easier to use. We developed a reduced-complexity air quality Intervention Model for Air Pollution over China (InMAP-China) to rapidly predict the air quality and estimate the health impacts of emission sources in China. We believe that this work will be of great interest to a broad audience, including environmentalists in China and scientists in relevant fields at both national and local institutes.
Irini Tsiodra, Georgios Grivas, Kalliopi Tavernaraki, Aikaterini Bougiatioti, Maria Apostolaki, Despina Paraskevopoulou, Alexandra Gogou, Constantine Parinos, Konstantina Oikonomou, Maria Tsagkaraki, Pavlos Zarmpas, Athanasios Nenes, and Nikolaos Mihalopoulos
Atmos. Chem. Phys., 21, 17865–17883, https://doi.org/10.5194/acp-21-17865-2021, https://doi.org/10.5194/acp-21-17865-2021, 2021
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We analyze observations from year-long measurements at Athens, Greece. Nighttime wintertime PAH levels are 4 times higher than daytime, and wintertime values are 15 times higher than summertime. Biomass burning aerosol during wintertime pollution events is responsible for these significant wintertime enhancements and accounts for 43 % of the population exposure to PAH carcinogenic risk. Biomass burning poses additional health risks beyond those associated with the high PM levels that develop.
Claudia Tebaldi, Kalyn Dorheim, Michael Wehner, and Ruby Leung
Earth Syst. Dynam., 12, 1427–1501, https://doi.org/10.5194/esd-12-1427-2021, https://doi.org/10.5194/esd-12-1427-2021, 2021
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We address the question of how large an initial condition ensemble of climate model simulations should be if we are concerned with accurately projecting future changes in temperature and precipitation extremes. We find that for most cases (and both models considered), an ensemble of 20–25 members is sufficient for many extreme metrics, spatial scales and time horizons. This may leave computational resources to tackle other uncertainties in climate model simulations with our ensembles.
Mária Lbadaoui-Darvas, Satoshi Takahama, and Athanasios Nenes
Atmos. Chem. Phys., 21, 17687–17714, https://doi.org/10.5194/acp-21-17687-2021, https://doi.org/10.5194/acp-21-17687-2021, 2021
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Aerosol–cloud interactions constitute the most uncertain contribution to climate change. The uptake kinetics of water by aerosol is a central process of cloud droplet formation, yet its molecular-scale mechanism is unknown. We use molecular simulations to study this process for phase-separated organic particles. Our results explain the increased cloud condensation activity of such particles and can be generalized over various compositions, thus possibly serving as a basis for future models.
Kai Wang, Yang Zhang, Shaocai Yu, David C. Wong, Jonathan Pleim, Rohit Mathur, James T. Kelly, and Michelle Bell
Geosci. Model Dev., 14, 7189–7221, https://doi.org/10.5194/gmd-14-7189-2021, https://doi.org/10.5194/gmd-14-7189-2021, 2021
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The two-way coupled WRF-CMAQ model accounting for complex chemistry–meteorology feedbacks has been applied to the long-term predictions of regional meteorology and air quality over the US. The model results show superior performance and importance of chemistry–meteorology feedbacks when compared to the offline coupled WRF and CMAQ simulations, which suggests that feedbacks should be considered along with other factors in developing future model applications to inform policy making.
Steven G. Howell, Steffen Freitag, Amie Dobracki, Nikolai Smirnow, and Arthur J. Sedlacek III
Atmos. Meas. Tech., 14, 7381–7404, https://doi.org/10.5194/amt-14-7381-2021, https://doi.org/10.5194/amt-14-7381-2021, 2021
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Small particles in the air have important effects on visibility, clouds, and human health. For the ORACLES project we got a new particle sizing instrument that is fast, works over the most important particle sizes, and avoids some of the issues that plague other optical particle sizers. Unfortunately it sees some particles much smaller than they really are, likely because they heat up and evaporate. We show a crude correction and speculate why these particles heat up much more than expected.
Ju-Mee Ryoo, Leonhard Pfister, Rei Ueyama, Paquita Zuidema, Robert Wood, Ian Chang, and Jens Redemann
Atmos. Chem. Phys., 21, 16689–16707, https://doi.org/10.5194/acp-21-16689-2021, https://doi.org/10.5194/acp-21-16689-2021, 2021
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Part 1 of the meteorological overview paper highlights the anomalous meteorological characteristics during the ORACLES deployment compared to the climatological mean at monthly timescales. The upper-level wave disturbance and the associated anomalous circulation explain the weakening of AEJ-S through the reduction of the strength of the heat low over the land during August 2017. This may also help explain the anomalously low aerosol optical depth observed in the August 2017 ORACLES deployment.
Raphaela Vogel, Heike Konow, Hauke Schulz, and Paquita Zuidema
Atmos. Chem. Phys., 21, 16609–16630, https://doi.org/10.5194/acp-21-16609-2021, https://doi.org/10.5194/acp-21-16609-2021, 2021
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The shallow cumulus clouds that populate the trade-wind regions can produce substantial amounts of rain. Before reaching the surface, part of the rain can evaporate and form pools of cold air that spread at the surface as density currents. We use 10 years of data from Barbados to show that such cold pools occur on 3 out of 4 d, that cold-pool periods are 90 % cloudier relative to the average winter conditions, and that they are connected to specific patterns of mesoscale cloud organization.
Rachel Atlas, Johannes Mohrmann, Joseph Finlon, Jeremy Lu, Ian Hsiao, Robert Wood, and Minghui Diao
Atmos. Meas. Tech., 14, 7079–7101, https://doi.org/10.5194/amt-14-7079-2021, https://doi.org/10.5194/amt-14-7079-2021, 2021
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Many clouds with temperatures between 0 °C and −40 °C contain both liquid and ice particles, and the ratio of liquid to ice particles influences how the clouds interact with radiation and moderate Earth's climate. We use a machine learning method called random forest to classify images of individual cloud particles as either liquid or ice. We apply our algorithm to images captured by aircraft within clouds overlying the Southern Ocean, and we find that it outperforms two existing algorithms.
Zachary C. J. Decker, Michael A. Robinson, Kelley C. Barsanti, Ilann Bourgeois, Matthew M. Coggon, Joshua P. DiGangi, Glenn S. Diskin, Frank M. Flocke, Alessandro Franchin, Carley D. Fredrickson, Georgios I. Gkatzelis, Samuel R. Hall, Hannah Halliday, Christopher D. Holmes, L. Gregory Huey, Young Ro Lee, Jakob Lindaas, Ann M. Middlebrook, Denise D. Montzka, Richard Moore, J. Andrew Neuman, John B. Nowak, Brett B. Palm, Jeff Peischl, Felix Piel, Pamela S. Rickly, Andrew W. Rollins, Thomas B. Ryerson, Rebecca H. Schwantes, Kanako Sekimoto, Lee Thornhill, Joel A. Thornton, Geoffrey S. Tyndall, Kirk Ullmann, Paul Van Rooy, Patrick R. Veres, Carsten Warneke, Rebecca A. Washenfelder, Andrew J. Weinheimer, Elizabeth Wiggins, Edward Winstead, Armin Wisthaler, Caroline Womack, and Steven S. Brown
Atmos. Chem. Phys., 21, 16293–16317, https://doi.org/10.5194/acp-21-16293-2021, https://doi.org/10.5194/acp-21-16293-2021, 2021
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To understand air quality impacts from wildfires, we need an accurate picture of how wildfire smoke changes chemically both day and night as sunlight changes the chemistry of smoke. We present a chemical analysis of wildfire smoke as it changes from midday through the night. We use aircraft observations from the FIREX-AQ field campaign with a chemical box model. We find that even under sunlight typical
nighttimechemistry thrives and controls the fate of key smoke plume chemical processes.
Dawei Hu, M. Rami Alfarra, Kate Szpek, Justin M. Langridge, Michael I. Cotterell, Claire Belcher, Ian Rule, Zixia Liu, Chenjie Yu, Yunqi Shao, Aristeidis Voliotis, Mao Du, Brett Smith, Greg Smallwood, Prem Lobo, Dantong Liu, Jim M. Haywood, Hugh Coe, and James D. Allan
Atmos. Chem. Phys., 21, 16161–16182, https://doi.org/10.5194/acp-21-16161-2021, https://doi.org/10.5194/acp-21-16161-2021, 2021
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Here, we developed new techniques for investigating these properties in the laboratory and applied these to BC and BrC from different sources, including diesel exhaust, inverted propane flame and wood combustion. These have allowed us to quantify the changes in shape and chemical composition of different soots according to source and variables such as the moisture content of wood.
Dalei Hao, Gautam Bisht, Yu Gu, Wei-Liang Lee, Kuo-Nan Liou, and L. Ruby Leung
Geosci. Model Dev., 14, 6273–6289, https://doi.org/10.5194/gmd-14-6273-2021, https://doi.org/10.5194/gmd-14-6273-2021, 2021
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Topography exerts significant influence on the incoming solar radiation at the land surface. This study incorporated a well-validated sub-grid topographic parameterization in E3SM land model (ELM) version 1.0. The results demonstrate that sub-grid topography has non-negligible effects on surface energy budget, snow cover, and surface temperature over the Tibetan Plateau and that the ELM simulations are sensitive to season, elevation, and spatial scale.
David Painemal, Douglas Spangenberg, William L. Smith Jr., Patrick Minnis, Brian Cairns, Richard H. Moore, Ewan Crosbie, Claire Robinson, Kenneth L. Thornhill, Edward L. Winstead, and Luke Ziemba
Atmos. Meas. Tech., 14, 6633–6646, https://doi.org/10.5194/amt-14-6633-2021, https://doi.org/10.5194/amt-14-6633-2021, 2021
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Cloud properties derived from satellite sensors are critical for the global monitoring of climate. This study evaluates satellite-based cloud properties over the North Atlantic using airborne data collected during NAAMES. Satellite observations of droplet size and cloud optical depth tend to compare well with NAAMES data. The analysis indicates that the satellite pixel resolution and the specific viewing geometry need to be taken into account in research applications.
Spiro D. Jorga, Kalliopi Florou, Christos Kaltsonoudis, John K. Kodros, Christina Vasilakopoulou, Manuela Cirtog, Axel Fouqueau, Bénédicte Picquet-Varrault, Athanasios Nenes, and Spyros N. Pandis
Atmos. Chem. Phys., 21, 15337–15349, https://doi.org/10.5194/acp-21-15337-2021, https://doi.org/10.5194/acp-21-15337-2021, 2021
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We test the hypothesis that significant secondary organic aerosol production can take place even during winter nights through the oxidation of the emitted organic vapors by the nitrate radicals produced during the reaction of ozone and nitrogen oxides. Our experiments, using as a starting point the ambient air of an urban area with high biomass burning activity, demonstrate that, even with sunlight, there is 20 %–70 % additional organic aerosol formed in a few hours.
Rose M. Miller, Greg M. McFarquhar, Robert M. Rauber, Joseph R. O'Brien, Siddhant Gupta, Michal Segal-Rozenhaimer, Amie N. Dobracki, Arthur J. Sedlacek, Sharon P. Burton, Steven G. Howell, Steffen Freitag, and Caroline Dang
Atmos. Chem. Phys., 21, 14815–14831, https://doi.org/10.5194/acp-21-14815-2021, https://doi.org/10.5194/acp-21-14815-2021, 2021
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A large stratocumulus cloud deck resides off the west coast of central Africa. Biomass burning in Africa produces a large plume of aerosol that is carried by the wind over this stratocumulus cloud deck. This paper shows that particles with sizes from 0.01 to 1 mm reside within this plume. Past studies have shown that biomass burning produces such particles, but this is the first study to show that they can be transported westward, over long distances, to the Atlantic stratocumulus cloud deck.
Robert Wood
Atmos. Chem. Phys., 21, 14507–14533, https://doi.org/10.5194/acp-21-14507-2021, https://doi.org/10.5194/acp-21-14507-2021, 2021
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A simple model is described to assess the potential for increasing solar reflection by augmenting the aerosol population below marine low clouds, which increases the concentration of cloud droplets. The model is used to predict global cooling from marine cloud brightening climate intervention as a function of the quantity, size, and lifetime of salt particles injected per sprayer, the number of sprayers deployed, the cloud updraft speed, and unperturbed aerosol size distribution.
Xinxin Ye, Pargoal Arab, Ravan Ahmadov, Eric James, Georg A. Grell, Bradley Pierce, Aditya Kumar, Paul Makar, Jack Chen, Didier Davignon, Greg R. Carmichael, Gonzalo Ferrada, Jeff McQueen, Jianping Huang, Rajesh Kumar, Louisa Emmons, Farren L. Herron-Thorpe, Mark Parrington, Richard Engelen, Vincent-Henri Peuch, Arlindo da Silva, Amber Soja, Emily Gargulinski, Elizabeth Wiggins, Johnathan W. Hair, Marta Fenn, Taylor Shingler, Shobha Kondragunta, Alexei Lyapustin, Yujie Wang, Brent Holben, David M. Giles, and Pablo E. Saide
Atmos. Chem. Phys., 21, 14427–14469, https://doi.org/10.5194/acp-21-14427-2021, https://doi.org/10.5194/acp-21-14427-2021, 2021
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Wildfire smoke has crucial impacts on air quality, while uncertainties in the numerical forecasts remain significant. We present an evaluation of 12 real-time forecasting systems. Comparison of predicted smoke emissions suggests a large spread in magnitudes, with temporal patterns deviating from satellite detections. The performance for AOD and surface PM2.5 and their discrepancies highlighted the role of accurately represented spatiotemporal emission profiles in improving smoke forecasts.
Zixia Liu, Martin Osborne, Karen Anderson, Jamie D. Shutler, Andy Wilson, Justin Langridge, Steve H. L. Yim, Hugh Coe, Suresh Babu, Sreedharan K. Satheesh, Paquita Zuidema, Tao Huang, Jack C. H. Cheng, and James Haywood
Atmos. Meas. Tech., 14, 6101–6118, https://doi.org/10.5194/amt-14-6101-2021, https://doi.org/10.5194/amt-14-6101-2021, 2021
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This paper first validates the performance of an advanced aerosol observation instrument POPS against a reference instrument and examines any biases introduced by operating it on a quadcopter drone. The results show the POPS performs relatively well on the ground. The impact of the UAV rotors on the POPS is small at low wind speeds, but when operating under higher wind speeds, larger discrepancies occur. It appears that the POPS measures sub-micron aerosol particles more accurately on the UAV.
Syuichi Itahashi, Rohit Mathur, Christian Hogrefe, Sergey L. Napelenok, and Yang Zhang
Geosci. Model Dev., 14, 5751–5768, https://doi.org/10.5194/gmd-14-5751-2021, https://doi.org/10.5194/gmd-14-5751-2021, 2021
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The Community Multiscale Air Quality (CMAQ) modeling system extended for hemispheric-scale applications (H-CMAQ) incorporated the satellite-constrained degassing SO2 emissions from 50 volcanos across the Northern Hemisphere. The impact on tropospheric sulfate aerosol (SO42−) is assessed for 2010. Although the considered volcanic emissions occurred at or below the middle of free troposphere (500 hPa), SO42− enhancements of more than 10 % were detected up to the top of free troposphere (250 hPa).
Andreas Tilgner, Thomas Schaefer, Becky Alexander, Mary Barth, Jeffrey L. Collett Jr., Kathleen M. Fahey, Athanasios Nenes, Havala O. T. Pye, Hartmut Herrmann, and V. Faye McNeill
Atmos. Chem. Phys., 21, 13483–13536, https://doi.org/10.5194/acp-21-13483-2021, https://doi.org/10.5194/acp-21-13483-2021, 2021
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Feedbacks of acidity and atmospheric multiphase chemistry in deliquesced particles and clouds are crucial for the tropospheric composition, depositions, climate, and human health. This review synthesizes the current scientific knowledge on these feedbacks using both inorganic and organic aqueous-phase chemistry. Finally, this review outlines atmospheric implications and highlights the need for future investigations with respect to reducing emissions of key acid precursors in a changing world.
Ruhi S. Humphries, Melita D. Keywood, Sean Gribben, Ian M. McRobert, Jason P. Ward, Paul Selleck, Sally Taylor, James Harnwell, Connor Flynn, Gourihar R. Kulkarni, Gerald G. Mace, Alain Protat, Simon P. Alexander, and Greg McFarquhar
Atmos. Chem. Phys., 21, 12757–12782, https://doi.org/10.5194/acp-21-12757-2021, https://doi.org/10.5194/acp-21-12757-2021, 2021
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The Southern Ocean region is one of the most pristine in the world and serves as an important proxy for the pre-industrial atmosphere. Improving our understanding of the natural processes in this region is likely to result in the largest reductions in the uncertainty of climate and earth system models. In this paper we present a statistical summary of the latitudinal gradient of aerosol and cloud condensation nuclei concentrations obtained from five voyages spanning the Southern Ocean.
Bjorn Stevens, Sandrine Bony, David Farrell, Felix Ament, Alan Blyth, Christopher Fairall, Johannes Karstensen, Patricia K. Quinn, Sabrina Speich, Claudia Acquistapace, Franziska Aemisegger, Anna Lea Albright, Hugo Bellenger, Eberhard Bodenschatz, Kathy-Ann Caesar, Rebecca Chewitt-Lucas, Gijs de Boer, Julien Delanoë, Leif Denby, Florian Ewald, Benjamin Fildier, Marvin Forde, Geet George, Silke Gross, Martin Hagen, Andrea Hausold, Karen J. Heywood, Lutz Hirsch, Marek Jacob, Friedhelm Jansen, Stefan Kinne, Daniel Klocke, Tobias Kölling, Heike Konow, Marie Lothon, Wiebke Mohr, Ann Kristin Naumann, Louise Nuijens, Léa Olivier, Robert Pincus, Mira Pöhlker, Gilles Reverdin, Gregory Roberts, Sabrina Schnitt, Hauke Schulz, A. Pier Siebesma, Claudia Christine Stephan, Peter Sullivan, Ludovic Touzé-Peiffer, Jessica Vial, Raphaela Vogel, Paquita Zuidema, Nicola Alexander, Lyndon Alves, Sophian Arixi, Hamish Asmath, Gholamhossein Bagheri, Katharina Baier, Adriana Bailey, Dariusz Baranowski, Alexandre Baron, Sébastien Barrau, Paul A. Barrett, Frédéric Batier, Andreas Behrendt, Arne Bendinger, Florent Beucher, Sebastien Bigorre, Edmund Blades, Peter Blossey, Olivier Bock, Steven Böing, Pierre Bosser, Denis Bourras, Pascale Bouruet-Aubertot, Keith Bower, Pierre Branellec, Hubert Branger, Michal Brennek, Alan Brewer, Pierre-Etienne Brilouet, Björn Brügmann, Stefan A. Buehler, Elmo Burke, Ralph Burton, Radiance Calmer, Jean-Christophe Canonici, Xavier Carton, Gregory Cato Jr., Jude Andre Charles, Patrick Chazette, Yanxu Chen, Michal T. Chilinski, Thomas Choularton, Patrick Chuang, Shamal Clarke, Hugh Coe, Céline Cornet, Pierre Coutris, Fleur Couvreux, Susanne Crewell, Timothy Cronin, Zhiqiang Cui, Yannis Cuypers, Alton Daley, Gillian M. Damerell, Thibaut Dauhut, Hartwig Deneke, Jean-Philippe Desbios, Steffen Dörner, Sebastian Donner, Vincent Douet, Kyla Drushka, Marina Dütsch, André Ehrlich, Kerry Emanuel, Alexandros Emmanouilidis, Jean-Claude Etienne, Sheryl Etienne-Leblanc, Ghislain Faure, Graham Feingold, Luca Ferrero, Andreas Fix, Cyrille Flamant, Piotr Jacek Flatau, Gregory R. Foltz, Linda Forster, Iulian Furtuna, Alan Gadian, Joseph Galewsky, Martin Gallagher, Peter Gallimore, Cassandra Gaston, Chelle Gentemann, Nicolas Geyskens, Andreas Giez, John Gollop, Isabelle Gouirand, Christophe Gourbeyre, Dörte de Graaf, Geiske E. de Groot, Robert Grosz, Johannes Güttler, Manuel Gutleben, Kashawn Hall, George Harris, Kevin C. Helfer, Dean Henze, Calvert Herbert, Bruna Holanda, Antonio Ibanez-Landeta, Janet Intrieri, Suneil Iyer, Fabrice Julien, Heike Kalesse, Jan Kazil, Alexander Kellman, Abiel T. Kidane, Ulrike Kirchner, Marcus Klingebiel, Mareike Körner, Leslie Ann Kremper, Jan Kretzschmar, Ovid Krüger, Wojciech Kumala, Armin Kurz, Pierre L'Hégaret, Matthieu Labaste, Tom Lachlan-Cope, Arlene Laing, Peter Landschützer, Theresa Lang, Diego Lange, Ingo Lange, Clément Laplace, Gauke Lavik, Rémi Laxenaire, Caroline Le Bihan, Mason Leandro, Nathalie Lefevre, Marius Lena, Donald Lenschow, Qiang Li, Gary Lloyd, Sebastian Los, Niccolò Losi, Oscar Lovell, Christopher Luneau, Przemyslaw Makuch, Szymon Malinowski, Gaston Manta, Eleni Marinou, Nicholas Marsden, Sebastien Masson, Nicolas Maury, Bernhard Mayer, Margarette Mayers-Als, Christophe Mazel, Wayne McGeary, James C. McWilliams, Mario Mech, Melina Mehlmann, Agostino Niyonkuru Meroni, Theresa Mieslinger, Andreas Minikin, Peter Minnett, Gregor Möller, Yanmichel Morfa Avalos, Caroline Muller, Ionela Musat, Anna Napoli, Almuth Neuberger, Christophe Noisel, David Noone, Freja Nordsiek, Jakub L. Nowak, Lothar Oswald, Douglas J. Parker, Carolyn Peck, Renaud Person, Miriam Philippi, Albert Plueddemann, Christopher Pöhlker, Veronika Pörtge, Ulrich Pöschl, Lawrence Pologne, Michał Posyniak, Marc Prange, Estefanía Quiñones Meléndez, Jule Radtke, Karim Ramage, Jens Reimann, Lionel Renault, Klaus Reus, Ashford Reyes, Joachim Ribbe, Maximilian Ringel, Markus Ritschel, Cesar B. Rocha, Nicolas Rochetin, Johannes Röttenbacher, Callum Rollo, Haley Royer, Pauline Sadoulet, Leo Saffin, Sanola Sandiford, Irina Sandu, Michael Schäfer, Vera Schemann, Imke Schirmacher, Oliver Schlenczek, Jerome Schmidt, Marcel Schröder, Alfons Schwarzenboeck, Andrea Sealy, Christoph J. Senff, Ilya Serikov, Samkeyat Shohan, Elizabeth Siddle, Alexander Smirnov, Florian Späth, Branden Spooner, M. Katharina Stolla, Wojciech Szkółka, Simon P. de Szoeke, Stéphane Tarot, Eleni Tetoni, Elizabeth Thompson, Jim Thomson, Lorenzo Tomassini, Julien Totems, Alma Anna Ubele, Leonie Villiger, Jan von Arx, Thomas Wagner, Andi Walther, Ben Webber, Manfred Wendisch, Shanice Whitehall, Anton Wiltshire, Allison A. Wing, Martin Wirth, Jonathan Wiskandt, Kevin Wolf, Ludwig Worbes, Ethan Wright, Volker Wulfmeyer, Shanea Young, Chidong Zhang, Dongxiao Zhang, Florian Ziemen, Tobias Zinner, and Martin Zöger
Earth Syst. Sci. Data, 13, 4067–4119, https://doi.org/10.5194/essd-13-4067-2021, https://doi.org/10.5194/essd-13-4067-2021, 2021
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The EUREC4A field campaign, designed to test hypothesized mechanisms by which clouds respond to warming and benchmark next-generation Earth-system models, is presented. EUREC4A comprised roughly 5 weeks of measurements in the downstream winter trades of the North Atlantic – eastward and southeastward of Barbados. It was the first campaign that attempted to characterize the full range of processes and scales influencing trade wind clouds.
Ernesto Reyes-Villegas, Upasana Panda, Eoghan Darbyshire, James M. Cash, Rutambhara Joshi, Ben Langford, Chiara F. Di Marco, Neil J. Mullinger, Mohammed S. Alam, Leigh R. Crilley, Daniel J. Rooney, W. Joe F. Acton, Will Drysdale, Eiko Nemitz, Michael Flynn, Aristeidis Voliotis, Gordon McFiggans, Hugh Coe, James Lee, C. Nicholas Hewitt, Mathew R. Heal, Sachin S. Gunthe, Tuhin K. Mandal, Bhola R. Gurjar, Shivani, Ranu Gadi, Siddhartha Singh, Vijay Soni, and James D. Allan
Atmos. Chem. Phys., 21, 11655–11667, https://doi.org/10.5194/acp-21-11655-2021, https://doi.org/10.5194/acp-21-11655-2021, 2021
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This paper shows the first multisite online measurements of PM1 in Delhi, India, with measurements over different seasons in Old Delhi and New Delhi in 2018. Organic aerosol (OA) source apportionment was performed using positive matrix factorisation (PMF). Traffic was the main primary aerosol source for both OAs and black carbon, seen with PMF and Aethalometer model analysis, indicating that control of primary traffic exhaust emissions would make a significant reduction to Delhi air pollution.
J. Brant Dodson, Patrick C. Taylor, Richard H. Moore, David H. Bromwich, Keith M. Hines, Kenneth L. Thornhill, Chelsea A. Corr, Bruce E. Anderson, Edward L. Winstead, and Joseph R. Bennett
Atmos. Chem. Phys., 21, 11563–11580, https://doi.org/10.5194/acp-21-11563-2021, https://doi.org/10.5194/acp-21-11563-2021, 2021
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Aircraft in situ observations of low-level Beaufort Sea cloud properties and thermodynamics from the ARISE campaign are compared with the Arctic System Reanalysis (ASR) to better understand deficiencies in simulated clouds. ASR produces too little cloud water, which coincides with being too warm and dry. In addition, ASR struggles to produce cloud water even in favorable thermodynamic conditions. A random sampling experiment also shows the effects of the limited aircraft sampling on the results.
Benjamin A. Nault, Duseong S. Jo, Brian C. McDonald, Pedro Campuzano-Jost, Douglas A. Day, Weiwei Hu, Jason C. Schroder, James Allan, Donald R. Blake, Manjula R. Canagaratna, Hugh Coe, Matthew M. Coggon, Peter F. DeCarlo, Glenn S. Diskin, Rachel Dunmore, Frank Flocke, Alan Fried, Jessica B. Gilman, Georgios Gkatzelis, Jacqui F. Hamilton, Thomas F. Hanisco, Patrick L. Hayes, Daven K. Henze, Alma Hodzic, James Hopkins, Min Hu, L. Greggory Huey, B. Thomas Jobson, William C. Kuster, Alastair Lewis, Meng Li, Jin Liao, M. Omar Nawaz, Ilana B. Pollack, Jeffrey Peischl, Bernhard Rappenglück, Claire E. Reeves, Dirk Richter, James M. Roberts, Thomas B. Ryerson, Min Shao, Jacob M. Sommers, James Walega, Carsten Warneke, Petter Weibring, Glenn M. Wolfe, Dominique E. Young, Bin Yuan, Qiang Zhang, Joost A. de Gouw, and Jose L. Jimenez
Atmos. Chem. Phys., 21, 11201–11224, https://doi.org/10.5194/acp-21-11201-2021, https://doi.org/10.5194/acp-21-11201-2021, 2021
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Secondary organic aerosol (SOA) is an important aspect of poor air quality for urban regions around the world, where a large fraction of the population lives. However, there is still large uncertainty in predicting SOA in urban regions. Here, we used data from 11 urban campaigns and show that the variability in SOA production in these regions is predictable and is explained by key emissions. These results are used to estimate the premature mortality associated with SOA in urban regions.
Jianhao Zhang and Paquita Zuidema
Atmos. Chem. Phys., 21, 11179–11199, https://doi.org/10.5194/acp-21-11179-2021, https://doi.org/10.5194/acp-21-11179-2021, 2021
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The subtropical Atlantic hosts one of the planet's largest marine low cloud decks and interacts with biomass burning aerosol from approximately July through October. This study clarifies how the monthly evolution in meteorology and the biomass burning aerosol vertical structure affects the seasonal cycle in its low cloud fraction, such that the July–October evolution in low cloud cover and morphology are reinforced, when compared to scenarios with less aerosol present.
Yang Wang, Guangjie Zheng, Michael P. Jensen, Daniel A. Knopf, Alexander Laskin, Alyssa A. Matthews, David Mechem, Fan Mei, Ryan Moffet, Arthur J. Sedlacek, John E. Shilling, Stephen Springston, Amy Sullivan, Jason Tomlinson, Daniel Veghte, Rodney Weber, Robert Wood, Maria A. Zawadowicz, and Jian Wang
Atmos. Chem. Phys., 21, 11079–11098, https://doi.org/10.5194/acp-21-11079-2021, https://doi.org/10.5194/acp-21-11079-2021, 2021
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This paper reports the vertical profiles of trace gas and aerosol properties over the eastern North Atlantic, a region of persistent but diverse subtropical marine boundary layer (MBL) clouds. We examined the key processes that drive the cloud condensation nuclei (CCN) population and how it varies with season and synoptic conditions. This study helps improve the model representation of the aerosol processes in the remote MBL, reducing the simulated aerosol indirect effects.
Yongkang Xue, Tandong Yao, Aaron A. Boone, Ismaila Diallo, Ye Liu, Xubin Zeng, William K. M. Lau, Shiori Sugimoto, Qi Tang, Xiaoduo Pan, Peter J. van Oevelen, Daniel Klocke, Myung-Seo Koo, Tomonori Sato, Zhaohui Lin, Yuhei Takaya, Constantin Ardilouze, Stefano Materia, Subodh K. Saha, Retish Senan, Tetsu Nakamura, Hailan Wang, Jing Yang, Hongliang Zhang, Mei Zhao, Xin-Zhong Liang, J. David Neelin, Frederic Vitart, Xin Li, Ping Zhao, Chunxiang Shi, Weidong Guo, Jianping Tang, Miao Yu, Yun Qian, Samuel S. P. Shen, Yang Zhang, Kun Yang, Ruby Leung, Yuan Qiu, Daniele Peano, Xin Qi, Yanling Zhan, Michael A. Brunke, Sin Chan Chou, Michael Ek, Tianyi Fan, Hong Guan, Hai Lin, Shunlin Liang, Helin Wei, Shaocheng Xie, Haoran Xu, Weiping Li, Xueli Shi, Paulo Nobre, Yan Pan, Yi Qin, Jeff Dozier, Craig R. Ferguson, Gianpaolo Balsamo, Qing Bao, Jinming Feng, Jinkyu Hong, Songyou Hong, Huilin Huang, Duoying Ji, Zhenming Ji, Shichang Kang, Yanluan Lin, Weiguang Liu, Ryan Muncaster, Patricia de Rosnay, Hiroshi G. Takahashi, Guiling Wang, Shuyu Wang, Weicai Wang, Xu Zhou, and Yuejian Zhu
Geosci. Model Dev., 14, 4465–4494, https://doi.org/10.5194/gmd-14-4465-2021, https://doi.org/10.5194/gmd-14-4465-2021, 2021
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The subseasonal prediction of extreme hydroclimate events such as droughts/floods has remained stubbornly low for years. This paper presents a new international initiative which, for the first time, introduces spring land surface temperature anomalies over high mountains to improve precipitation prediction through remote effects of land–atmosphere interactions. More than 40 institutions worldwide are participating in this effort. The experimental protocol and preliminary results are presented.
Paraskevi Georgakaki, Aikaterini Bougiatioti, Jörg Wieder, Claudia Mignani, Fabiola Ramelli, Zamin A. Kanji, Jan Henneberger, Maxime Hervo, Alexis Berne, Ulrike Lohmann, and Athanasios Nenes
Atmos. Chem. Phys., 21, 10993–11012, https://doi.org/10.5194/acp-21-10993-2021, https://doi.org/10.5194/acp-21-10993-2021, 2021
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Aerosol and cloud observations coupled with a droplet activation parameterization was used to investigate the aerosol–cloud droplet link in alpine mixed-phase clouds. Predicted droplet number, Nd, agrees with observations and never exceeds a characteristic “limiting droplet number”, Ndlim, which depends solely on σw. Nd becomes velocity limited when it is within 50 % of Ndlim. Identifying when dynamical changes control Nd variability is central for understanding aerosol–cloud interactions.
Zainab Bibi, Hugh Coe, James Brooks, Paul I. Williams, Ernesto Reyes-Villegas, Michael Priestley, Carl J. Percival, and James D. Allan
Atmos. Chem. Phys., 21, 10763–10777, https://doi.org/10.5194/acp-21-10763-2021, https://doi.org/10.5194/acp-21-10763-2021, 2021
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We are presenting a new method to apportion black carbon/soot into multiple sources through the inclusion of fullerene and metal data into HR-SP-AMS factorisation. While this itself would be considered a technical development, we can present a budget of contributions to measured BC during the event studied, including the conclusion that fireworks contributed little compared to the bonfire, traffic, and domestic wood-burning emissions.
Konstantin Baibakov, Samuel LeBlanc, Keyvan Ranjbar, Norman T. O'Neill, Mengistu Wolde, Jens Redemann, Kristina Pistone, Shao-Meng Li, John Liggio, Katherine Hayden, Tak W. Chan, Michael J. Wheeler, Leonid Nichman, Connor Flynn, and Roy Johnson
Atmos. Chem. Phys., 21, 10671–10687, https://doi.org/10.5194/acp-21-10671-2021, https://doi.org/10.5194/acp-21-10671-2021, 2021
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We find that the airborne measurements of the vertical extinction due to aerosols (aerosol optical depth, AOD) obtained in the Athabasca Oil Sands Region (AOSR) can significantly exceed ground-based values. This can have an effect on estimating the AOSR radiative impact and is relevant to satellite validation based on ground-based measurements. We also show that the AOD can marginally increase as the plumes are being transported away from the source and the new particles are being formed.
Hossein Dadashazar, David Painemal, Majid Alipanah, Michael Brunke, Seethala Chellappan, Andrea F. Corral, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Claire Robinson, Amy Jo Scarino, Michael Shook, Kenneth Sinclair, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Xubin Zeng, Luke Ziemba, Paquita Zuidema, and Armin Sorooshian
Atmos. Chem. Phys., 21, 10499–10526, https://doi.org/10.5194/acp-21-10499-2021, https://doi.org/10.5194/acp-21-10499-2021, 2021
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This study investigates the seasonal cycle of cloud drop number concentration (Nd) over the western North Atlantic Ocean (WNAO) using multiple datasets. Reasons for the puzzling discrepancy between the seasonal cycles of Nd and aerosol concentration were identified. Results indicate that Nd is highest in winter (when aerosol proxy values are often lowest) due to conditions both linked to cold-air outbreaks and that promote greater droplet activation.
Robert Pincus, Chris W. Fairall, Adriana Bailey, Haonan Chen, Patrick Y. Chuang, Gijs de Boer, Graham Feingold, Dean Henze, Quinn T. Kalen, Jan Kazil, Mason Leandro, Ashley Lundry, Ken Moran, Dana A. Naeher, David Noone, Akshar J. Patel, Sergio Pezoa, Ivan PopStefanija, Elizabeth J. Thompson, James Warnecke, and Paquita Zuidema
Earth Syst. Sci. Data, 13, 3281–3296, https://doi.org/10.5194/essd-13-3281-2021, https://doi.org/10.5194/essd-13-3281-2021, 2021
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This paper describes observations taken from a research aircraft during a field experiment in the western Atlantic Ocean during January and February 2020. The plane made 11 flights, most 8-9 h long, and measured the properties of the atmosphere and ocean with a combination of direct measurements, sensors falling from the plane to profile the atmosphere and ocean, and remote sensing measurements of clouds and the ocean surface.
Georgia Sotiropoulou, Luisa Ickes, Athanasios Nenes, and Annica M. L. Ekman
Atmos. Chem. Phys., 21, 9741–9760, https://doi.org/10.5194/acp-21-9741-2021, https://doi.org/10.5194/acp-21-9741-2021, 2021
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Mixed-phase clouds are a large source of uncertainty in projections of the Arctic climate. This is partly due to the poor representation of the cloud ice formation processes. Implementing a parameterization for ice multiplication due to mechanical breakup upon collision of two ice particles in a high-resolution model improves cloud ice phase representation; however, cloud liquid remains overestimated.
Xiaoyang Chen, Yang Zhang, Kai Wang, Daniel Tong, Pius Lee, Youhua Tang, Jianping Huang, Patrick C. Campbell, Jeff Mcqueen, Havala O. T. Pye, Benjamin N. Murphy, and Daiwen Kang
Geosci. Model Dev., 14, 3969–3993, https://doi.org/10.5194/gmd-14-3969-2021, https://doi.org/10.5194/gmd-14-3969-2021, 2021
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The continuously updated National Air Quality Forecast Capability (NAQFC) provides air quality forecasts. To support the development of the next-generation NAQFC, we evaluate a prototype of GFSv15-CMAQv5.0.2. The performance and the potential improvements for the system are discussed. This study can provide a scientific basis for further development of NAQFC and help it to provide more accurate air quality forecasts to the public over the contiguous United States.
Kristina Pistone, Paquita Zuidema, Robert Wood, Michael Diamond, Arlindo M. da Silva, Gonzalo Ferrada, Pablo E. Saide, Rei Ueyama, Ju-Mee Ryoo, Leonhard Pfister, James Podolske, David Noone, Ryan Bennett, Eric Stith, Gregory Carmichael, Jens Redemann, Connor Flynn, Samuel LeBlanc, Michal Segal-Rozenhaimer, and Yohei Shinozuka
Atmos. Chem. Phys., 21, 9643–9668, https://doi.org/10.5194/acp-21-9643-2021, https://doi.org/10.5194/acp-21-9643-2021, 2021
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Using aircraft-based measurements off the Atlantic coast of Africa, we found the springtime smoke plume was strongly correlated with the amount of water vapor in the atmosphere (more smoke indicated more humidity). We see the same general feature in satellite-assimilated and free-running models. Our analysis suggests this relationship is not caused by the burning but originates due to coincident continental meteorology plus fires. This air is transported over the ocean without further mixing.
Johannes Mohrmann, Robert Wood, Tianle Yuan, Hua Song, Ryan Eastman, and Lazaros Oreopoulos
Atmos. Chem. Phys., 21, 9629–9642, https://doi.org/10.5194/acp-21-9629-2021, https://doi.org/10.5194/acp-21-9629-2021, 2021
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Observations of marine-boundary-layer conditions are composited by cloud type, based on a new classification dataset. It is found that two cloud types, representing regions of clustered and suppressed low-level clouds, occur in very similar large-scale conditions but are distinguished from each other by considering low-level circulation and surface wind fields, validating prior results from modeling.
Huihui Wu, Jonathan W. Taylor, Justin M. Langridge, Chenjie Yu, James D. Allan, Kate Szpek, Michael I. Cotterell, Paul I. Williams, Michael Flynn, Patrick Barker, Cathryn Fox, Grant Allen, James Lee, and Hugh Coe
Atmos. Chem. Phys., 21, 9417–9440, https://doi.org/10.5194/acp-21-9417-2021, https://doi.org/10.5194/acp-21-9417-2021, 2021
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Seasonal biomass burning over West Africa is a globally significant source of carbonaceous particles in the atmosphere, which have important climate impacts but are poorly constrained. We conducted in situ airborne measurements to investigate the evolution of smoke aerosol properties in this region. We observed absorption enhancement for both black carbon and brown carbon after emission, which provides new field results and constraints on aerosol parameterizations for future climate models.
Richard H. Moore, Elizabeth B. Wiggins, Adam T. Ahern, Stephen Zimmerman, Lauren Montgomery, Pedro Campuzano Jost, Claire E. Robinson, Luke D. Ziemba, Edward L. Winstead, Bruce E. Anderson, Charles A. Brock, Matthew D. Brown, Gao Chen, Ewan C. Crosbie, Hongyu Guo, Jose L. Jimenez, Carolyn E. Jordan, Ming Lyu, Benjamin A. Nault, Nicholas E. Rothfuss, Kevin J. Sanchez, Melinda Schueneman, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Nicholas L. Wagner, and Jian Wang
Atmos. Meas. Tech., 14, 4517–4542, https://doi.org/10.5194/amt-14-4517-2021, https://doi.org/10.5194/amt-14-4517-2021, 2021
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Atmospheric particles are everywhere and exist in a range of sizes, from a few nanometers to hundreds of microns. Because particle size determines the behavior of chemical and physical processes, accurately measuring particle sizes is an important and integral part of atmospheric field measurements! Here, we discuss the performance of two commonly used particle sizers and how changes in particle composition and optical properties may result in sizing uncertainties, which we quantify.
Sobhan Kumar Kompalli, Surendran Nair Suresh Babu, Krishnaswamy Krishna Moorthy, Sreedharan Krishnakumari Satheesh, Mukunda Madhab Gogoi, Vijayakumar S. Nair, Venugopalan Nair Jayachandran, Dantong Liu, Michael J. Flynn, and Hugh Coe
Atmos. Chem. Phys., 21, 9173–9199, https://doi.org/10.5194/acp-21-9173-2021, https://doi.org/10.5194/acp-21-9173-2021, 2021
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The first observations of refractory black carbon aerosol size distributions and mixing state in South Asian outflow to the northern Indian Ocean were carried out as a part of the ICARB-2018 experiment during winter. Size distributions indicated mixed sources of BC particles in the outflow, which are thickly coated. The coating thickness of BC is controlled mainly by the availability of condensable species in the outflow.
Mohanan R. Manoj, Sreedharan K. Satheesh, Krishnaswamy K. Moorthy, Jamie Trembath, and Hugh Coe
Atmos. Chem. Phys., 21, 8979–8997, https://doi.org/10.5194/acp-21-8979-2021, https://doi.org/10.5194/acp-21-8979-2021, 2021
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Vertical distributions of atmospheric aerosols across the Indo-Gangetic Plain (IGP) and their ability to form clouds have been studied based on airborne measurements during the SWAAMI field campaign. The ability of the aerosols to act as cloud-forming nuclei exhibited large spatial variation across the IGP and strong seasonality with increase in this ability with increase in altitude prior to the onset of monsoon and decrease with increase in altitude during the active phase of the monsoon.
Mario Eduardo Gavidia-Calderón, Sergio Ibarra-Espinosa, Youngseob Kim, Yang Zhang, and Maria de Fatima Andrade
Geosci. Model Dev., 14, 3251–3268, https://doi.org/10.5194/gmd-14-3251-2021, https://doi.org/10.5194/gmd-14-3251-2021, 2021
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The MUNICH model was used to calculate pollutant concentrations inside the streets of São Paulo. The VEIN emission model provided the vehicular emissions and the coordinates of the streets. We used information from an air quality station to account for pollutant concentrations over the street rooftops. Results showed that when emissions are calibrated, MUNICH satisfied the performance criteria. MUNICH can be used to evaluate the impact of traffic-related air pollution on public health.
Maria A. Zawadowicz, Kaitlyn Suski, Jiumeng Liu, Mikhail Pekour, Jerome Fast, Fan Mei, Arthur J. Sedlacek, Stephen Springston, Yang Wang, Rahul A. Zaveri, Robert Wood, Jian Wang, and John E. Shilling
Atmos. Chem. Phys., 21, 7983–8002, https://doi.org/10.5194/acp-21-7983-2021, https://doi.org/10.5194/acp-21-7983-2021, 2021
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This paper describes the results of a recent field campaign in the eastern North Atlantic, where two mass spectrometers were deployed aboard a research aircraft to measure the chemistry of aerosols and trace gases. Very clean conditions were found, dominated by local sulfate-rich acidic aerosol and very aged organics. Evidence of
long-range transport of aerosols from the continents was also identified.
Stefan Noël, Maximilian Reuter, Michael Buchwitz, Jakob Borchardt, Michael Hilker, Heinrich Bovensmann, John P. Burrows, Antonio Di Noia, Hiroshi Suto, Yukio Yoshida, Matthias Buschmann, Nicholas M. Deutscher, Dietrich G. Feist, David W. T. Griffith, Frank Hase, Rigel Kivi, Isamu Morino, Justus Notholt, Hirofumi Ohyama, Christof Petri, James R. Podolske, David F. Pollard, Mahesh Kumar Sha, Kei Shiomi, Ralf Sussmann, Yao Té, Voltaire A. Velazco, and Thorsten Warneke
Atmos. Meas. Tech., 14, 3837–3869, https://doi.org/10.5194/amt-14-3837-2021, https://doi.org/10.5194/amt-14-3837-2021, 2021
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We present the first GOSAT and GOSAT-2 XCO2 data derived with the FOCAL retrieval algorithm. Comparisons of the GOSAT-FOCAL product with other data reveal long-term agreement within about 1 ppm over 1 decade, differences in seasonal variations of about 0.5 ppm, and a mean regional bias to ground-based TCCON data of 0.56 ppm with a mean scatter of 1.89 ppm. GOSAT-2-FOCAL data are preliminary only, but first comparisons show that they compare well with the GOSAT-FOCAL results and TCCON.
Yongjie Huang, Wei Wu, Greg M. McFarquhar, Xuguang Wang, Hugh Morrison, Alexander Ryzhkov, Yachao Hu, Mengistu Wolde, Cuong Nguyen, Alfons Schwarzenboeck, Jason Milbrandt, Alexei V. Korolev, and Ivan Heckman
Atmos. Chem. Phys., 21, 6919–6944, https://doi.org/10.5194/acp-21-6919-2021, https://doi.org/10.5194/acp-21-6919-2021, 2021
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Numerous small ice crystals in the tropical convective storms are difficult to detect and could be potentially hazardous for commercial aircraft. This study evaluated the numerical models against the airborne observations and investigated the potential cloud processes that could lead to the production of these large numbers of small ice crystals. It is found that key microphysical processes are still lacking or misrepresented in current numerical models to realistically simulate the phenomenon.
Nick Schutgens, Oleg Dubovik, Otto Hasekamp, Omar Torres, Hiren Jethva, Peter J. T. Leonard, Pavel Litvinov, Jens Redemann, Yohei Shinozuka, Gerrit de Leeuw, Stefan Kinne, Thomas Popp, Michael Schulz, and Philip Stier
Atmos. Chem. Phys., 21, 6895–6917, https://doi.org/10.5194/acp-21-6895-2021, https://doi.org/10.5194/acp-21-6895-2021, 2021
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Absorptive aerosol has a potentially large impact on climate change. We evaluate and intercompare four global satellite datasets of absorptive aerosol optical depth (AAOD) and single-scattering albedo (SSA). We show that these datasets show reasonable correlations with the AErosol RObotic NETwork (AERONET) reference, although significant biases remain. In a follow-up paper we show that these observations nevertheless can be used for model evaluation.
Anna L. Hodshire, Emily Ramnarine, Ali Akherati, Matthew L. Alvarado, Delphine K. Farmer, Shantanu H. Jathar, Sonia M. Kreidenweis, Chantelle R. Lonsdale, Timothy B. Onasch, Stephen R. Springston, Jian Wang, Yang Wang, Lawrence I. Kleinman, Arthur J. Sedlacek III, and Jeffrey R. Pierce
Atmos. Chem. Phys., 21, 6839–6855, https://doi.org/10.5194/acp-21-6839-2021, https://doi.org/10.5194/acp-21-6839-2021, 2021
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Biomass burning emits particles and vapors that can impact both health and climate. Here, we investigate the role of dilution in the evolution of aerosol size and composition in observed US wildfire smoke plumes. Centers of plumes dilute more slowly than edges. We see differences in concentrations and composition between the centers and edges both in the first measurement and in subsequent measurements. Our findings support the hypothesis that plume dilution influences smoke aging.
Patricia K. Quinn, Elizabeth J. Thompson, Derek J. Coffman, Sunil Baidar, Ludovic Bariteau, Timothy S. Bates, Sebastien Bigorre, Alan Brewer, Gijs de Boer, Simon P. de Szoeke, Kyla Drushka, Gregory R. Foltz, Janet Intrieri, Suneil Iyer, Chris W. Fairall, Cassandra J. Gaston, Friedhelm Jansen, James E. Johnson, Ovid O. Krüger, Richard D. Marchbanks, Kenneth P. Moran, David Noone, Sergio Pezoa, Robert Pincus, Albert J. Plueddemann, Mira L. Pöhlker, Ulrich Pöschl, Estefania Quinones Melendez, Haley M. Royer, Malgorzata Szczodrak, Jim Thomson, Lucia M. Upchurch, Chidong Zhang, Dongxiao Zhang, and Paquita Zuidema
Earth Syst. Sci. Data, 13, 1759–1790, https://doi.org/10.5194/essd-13-1759-2021, https://doi.org/10.5194/essd-13-1759-2021, 2021
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