Articles | Volume 19, issue 24
https://doi.org/10.5194/acp-19-15247-2019
https://doi.org/10.5194/acp-19-15247-2019
Research article
 | 
16 Dec 2019
Research article |  | 16 Dec 2019

Sources of organic aerosols in Europe: a modeling study using CAMx with modified volatility basis set scheme

Jianhui Jiang, Sebnem Aksoyoglu, Imad El-Haddad, Giancarlo Ciarelli, Hugo A. C. Denier van der Gon, Francesco Canonaco, Stefania Gilardoni, Marco Paglione, María Cruz Minguillón, Olivier Favez, Yunjiang Zhang, Nicolas Marchand, Liqing Hao, Annele Virtanen, Kalliopi Florou, Colin O'Dowd, Jurgita Ovadnevaite, Urs Baltensperger, and André S. H. Prévôt

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Cited articles

ACEA: Report: Vehicles in use – Europe 2017, European Automobile Manufacturers Association, available at: https://www.acea.be/statistics/article/vehicles-in-use-europe-2017 (last access: 6 December 2019), 2017. 
Ahmadov, R., McKeen, S. A., Robinson, A. L., Bahreini, R., Middlebrook, A. M., de Gouw, J. A., Meagher, J., Hsie, E. Y., Edgerton, E., Shaw, S., and Trainer, M.: A volatility basis set model for summertime secondary organic aerosols over the eastern United States in 2006, J. Geophys. Res.-Atmos, 117, D06301, https://doi.org/10.1029/2011JD016831, 2012. 
Aksoyoglu, S., Baltensperger, U., and Prévôt, A. S. H.: Contribution of ship emissions to the concentration and deposition of air pollutants in Europe, Atmos. Chem. Phys., 16, 1895-1906, https://doi.org/10.5194/acp-16-1895-2016, 2016. 
Andreani-Aksoyoglu, S. and Keller, J.: Estimates of monoterpene and isoprene emissions from the forests in switzerland, J. Atmos. Chem., 20, 71–87, https://doi.org/10.1007/bf01099919, 1995. 
Bergström, R., Denier van der Gon, H. A. C., Prévôt, A. S. H., Yttri, K. E., and Simpson, D.: Modelling of organic aerosols over Europe (2002–2007) using a volatility basis set (VBS) framework: application of different assumptions regarding the formation of secondary organic aerosol, Atmos. Chem. Phys., 12, 8499–8527, https://doi.org/10.5194/acp-12-8499-2012, 2012. 
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We use an air quality model with a modified organic aerosol (OA) module based on chamber experiments to identify the OA sources and their contributions in Europe. Comparisons with long-term measurements at nine sites in 2011 show an improvement in OA simulation. Our results suggest that the biomass burning and biogenic emissions are the dominant sources in winter and summer, respectively. Contributions of diesel and gasoline vehicles are relatively small compared to a previous study in the US.
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