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Tropospheric inorganic bromine (BrO and Bry) shows a C-shaped profile over the tropical western Pacific Ocean, and supports previous speculation that marine convection is a source for inorganic bromine from sea salt to the upper troposphere. The Bry profile in the tropical tropopause layer (TTL) is complex, suggesting that the total Bry budget in the TTL is not closed without considering aerosol bromide. The implications for atmospheric composition and bromine sources are discussed.
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Articles | Volume 17, issue 24
Atmos. Chem. Phys., 17, 15245–15270, 2017
https://doi.org/10.5194/acp-17-15245-2017
Atmos. Chem. Phys., 17, 15245–15270, 2017
https://doi.org/10.5194/acp-17-15245-2017

Research article 22 Dec 2017

Research article | 22 Dec 2017

BrO and inferred Bry profiles over the western Pacific: relevance of inorganic bromine sources and a Bry minimum in the aged tropical tropopause layer

Theodore K. Koenig et al.

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