Articles | Volume 20, issue 6
https://doi.org/10.5194/acp-20-3645-2020
https://doi.org/10.5194/acp-20-3645-2020
Research article
 | 
26 Mar 2020
Research article |  | 26 Mar 2020

Characterising mass-resolved mixing state of black carbon in Beijing using a morphology-independent measurement method

Chenjie Yu, Dantong Liu, Kurtis Broda, Rutambhara Joshi, Jason Olfert, Yele Sun, Pingqing Fu, Hugh Coe, and James D. Allan

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Cited articles

Adachi, K., Moteki, N., Kondo, Y., and Igarashi, Y.: Mixing states of light-absorbing particles measured using a transmission electron microscope and a single-particle soot photometer in Tokyo, Japan, J. Geophys. Res.-Atmos., 121, 9153–9164, https://doi.org/10.1002/2016jd025153, 2016. 
Bond, T. C. and Bergstrom, R. W.: Light Absorption by Carbonaceous Particles: An Investigative Review, Aerosol Sci. Tech., 40, 27–67, https://doi.org/10.1080/02786820500421521, 2006. 
Bondy, A. L., Bonanno, D., Moffet, R. C., Wang, B., Laskin, A., and Ault, A. P.: The diverse chemical mixing state of aerosol particles in the southeastern United States, Atmos. Chem. Phys., 18, 12595–12612, https://doi.org/10.5194/acp-18-12595-2018, 2018. 
Broda, K. N., Olfert, J. S., Irwin, M., Schill, G. P., McMeeking, G. R., Schnitzler, E. G., and Jäger, W.: A novel inversion method to determine the mass distribution of non-refractory coatings on refractory black carbon using a centrifugal particle mass analyzer and single particle soot photometer, Aerosol Sci. Tech., 52, 567–578, https://doi.org/10.1080/02786826.2018.1433812, 2018. 
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Short summary
This study presents the first atmospheric application of a new morphology-independent measurement for the quantification of the mixing state of rBC-containing particles in urban Beijing as part of the UK–China APHH campaign. An inversion method has been applied for better quantification of rBC mixing state. The mass-resolved rBC mixing state information presented here has implications for detailed models of BC, its optical properties and its atmospheric life cycle.
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