Articles | Volume 18, issue 16
https://doi.org/10.5194/acp-18-11779-2018
https://doi.org/10.5194/acp-18-11779-2018
Research article
 | 
20 Aug 2018
Research article |  | 20 Aug 2018

Modelling studies of HOMs and their contributions to new particle formation and growth: comparison of boreal forest in Finland and a polluted environment in China

Ximeng Qi, Aijun Ding, Pontus Roldin, Zhengning Xu, Putian Zhou, Nina Sarnela, Wei Nie, Xin Huang, Anton Rusanen, Mikael Ehn, Matti P. Rissanen, Tuukka Petäjä, Markku Kulmala, and Michael Boy

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Cited articles

Boy, M., Hellmuth, O., Korhonen, H., Nilsson, E. D., ReVelle, D., Turnipseed, A., Arnold, F., and Kulmala, M.: MALTE-model to predict new aerosol formation in the lower troposphere, Atmos. Chem. Phys., 6, 4499–4517, https://doi.org/10.5194/acp-6-4499-2006, 2006. 
Boy, M., Bonn, B., Kazil, J., Lovejoy, N., Turnipseed, A., Greenberg, J., Karl, T., Mauldin, L., Kusciuch, E., Smith, J., Barsanti, K., Guenther, A., Wehner, B., Hellmuth, O., Siebert, H., Bauer, S., Wiedensohler, A., and Kulmala, M.: Relevance of Several Nucleation Theories in Different Environments, in: Nucleation and Atmospheric Aerosols: 17th International Conference, Galway, Ireland, 2007, edited by: O'Dowd, C. D. and Wagner, P. E., Springer Netherlands, Dordrecht, 87–91, 2007. 
Boy, M., Kazil, J., Lovejoy, E. R., Guenther, A., and Kulmala, M.: Relevance of ion-induced nucleation of sulfuric acid and water in the lower troposphere over the boreal forest at northern latitudes, Atmos. Res., 90, 151–158, https://doi.org/10.1016/j.atmosres.2008.01.002, 2008. 
Boy, M., Mogensen, D., Smolander, S., Zhou, L., Nieminen, T., Paasonen, P., Plass-Dülmer, C., Sipilä, M., Petäjä, T., Mauldin, L., Berresheim, H., and Kulmala, M.: Oxidation of SO2 by stabilized Criegee intermediate (sCI) radicals as a crucial source for atmospheric sulfuric acid concentrations, Atmos. Chem. Phys., 13, 3865–3879, https://doi.org/10.5194/acp-13-3865-2013, 2013. 
Carlton, A. G., Wiedinmyer, C., and Kroll, J. H.: A review of Secondary Organic Aerosol (SOA) formation from isoprene, Atmos. Chem. Phys., 9, 4987–5005, https://doi.org/10.5194/acp-9-4987-2009, 2009. 
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Short summary
In this study we simulate the HOM concentrations and discuss their roles in NPF at a remote boreal forest site in Finland and a suburban site in eastern China. We found that sulfuric acid and HOM organonitrate concentrations in the gas phase are significantly higher but other HOM monomers and dimers from monoterpene oxidation are lower in eastern China. This study highlights the need for molecular-scale measurements in improving the understanding of NPF mechanisms in polluted areas.
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