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Volume 16, issue 15
Atmos. Chem. Phys., 16, 10063–10082, 2016
https://doi.org/10.5194/acp-16-10063-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Special issue: Pan-Eurasian Experiment (PEEX)

Atmos. Chem. Phys., 16, 10063–10082, 2016
https://doi.org/10.5194/acp-16-10063-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 09 Aug 2016

Research article | 09 Aug 2016

Effects of aerosol–radiation interaction on precipitation during biomass-burning season in East China

Xin Huang1,2,3, Aijun Ding1,2,3, Lixia Liu1,2, Qiang Liu1,2, Ke Ding1,2, Xiaorui Niu1,2,3, Wei Nie1,2,3, Zheng Xu1,2,3, Xuguang Chi1,2,3, Minghuai Wang1,2,3, Jianning Sun1,2,3, Weidong Guo1,2,3, and Congbin Fu1,2,3 Xin Huang et al.
  • 1Joint International Research Laboratory of Atmospheric and Earth System Sciences, Nanjing University, Nanjing, China
  • 2Institute for Climate and Global Change Research & School of Atmospheric Sciences, Nanjing University, Nanjing, 210023, China
  • 3Collaborative Innovation Center of Climate Change, Jiangsu province, China

Abstract. Biomass burning is a main source for primary carbonaceous particles in the atmosphere and acts as a crucial factor that alters Earth's energy budget and balance. It is also an important factor influencing air quality, regional climate and sustainability in the domain of Pan-Eurasian Experiment (PEEX). During the exceptionally intense agricultural fire season in mid-June 2012, accompanied by rapidly deteriorating air quality, a series of meteorological anomalies was observed, including a large decline in near-surface air temperature, spatial shifts and changes in precipitation in Jiangsu province of East China. To explore the underlying processes that link air pollution to weather modification, we conducted a numerical study with parallel simulations using the fully coupled meteorology–chemistry model WRF-Chem with a high-resolution emission inventory for agricultural fires. Evaluation of the modeling results with available ground-based measurements and satellite retrievals showed that this model was able to reproduce the magnitude and spatial variations of fire-induced air pollution. During the biomass-burning event in mid-June 2012, intensive emission of absorbing aerosols trapped a considerable part of solar radiation in the atmosphere and reduced incident radiation reaching the surface on a regional scale, followed by lowered surface sensible and latent heat fluxes. The perturbed energy balance and re-allocation gave rise to substantial adjustments in vertical temperature stratification, namely surface cooling and upper-air heating. Furthermore, an intimate link between temperature profile and small-scale processes like turbulent mixing and entrainment led to distinct changes in precipitation. On the one hand, by stabilizing the atmosphere below and reducing the surface flux, black carbon-laden plumes tended to dissipate daytime cloud and suppress the convective precipitation over Nanjing. On the other hand, heating aloft increased upper-level convective activity and then favored convergence carrying in moist air, thereby enhancing the nocturnal precipitation in the downwind areas of the biomass-burning plumes.

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We conducted a comprehensive modelling work to understand the impact of biomass burning on synoptic weather during agricultural burning season in East China. We demonstrated that the numerical model with fire emission, chemical processes, and aerosol–meteorology online coupled could reproduce the change of air temperature and precipitation induced by air pollution during this event. This study highlights the importance of including human activities in numerical-model-based weather forecast.
We conducted a comprehensive modelling work to understand the impact of biomass burning on...
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