Articles | Volume 18, issue 16
https://doi.org/10.5194/acp-18-11779-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-18-11779-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
20 Aug 2018
Research article |
| 20 Aug 2018
| 20 Aug 2018
Modelling studies of HOMs and their contributions to new particle formation and growth: comparison of boreal forest in Finland and a polluted environment in China
Ximeng Qi
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing
University, Nanjing, 210023, China
Collaborative Innovation Center
of Climate Change, Nanjing, 210023, China
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, P.O. Box 64, 00014 University of
Helsinki, Helsinki, Finland
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing
University, Nanjing, 210023, China
Collaborative Innovation Center
of Climate Change, Nanjing, 210023, China
Pontus Roldin
Division of Nuclear
Physics, Lund University, P.O. Box 118, 22100 Lund, Sweden
Zhengning Xu
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing
University, Nanjing, 210023, China
Collaborative Innovation Center
of Climate Change, Nanjing, 210023, China
Putian Zhou
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, P.O. Box 64, 00014 University of
Helsinki, Helsinki, Finland
Nina Sarnela
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, P.O. Box 64, 00014 University of
Helsinki, Helsinki, Finland
Wei Nie
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing
University, Nanjing, 210023, China
Collaborative Innovation Center
of Climate Change, Nanjing, 210023, China
Xin Huang
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing
University, Nanjing, 210023, China
Collaborative Innovation Center
of Climate Change, Nanjing, 210023, China
Anton Rusanen
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, P.O. Box 64, 00014 University of
Helsinki, Helsinki, Finland
Mikael Ehn
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, P.O. Box 64, 00014 University of
Helsinki, Helsinki, Finland
Matti P. Rissanen
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, P.O. Box 64, 00014 University of
Helsinki, Helsinki, Finland
Tuukka Petäjä
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, P.O. Box 64, 00014 University of
Helsinki, Helsinki, Finland
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing
University, Nanjing, 210023, China
Markku Kulmala
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, P.O. Box 64, 00014 University of
Helsinki, Helsinki, Finland
Michael Boy
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, P.O. Box 64, 00014 University of
Helsinki, Helsinki, Finland
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- The neglected autoxidation pathways for the formation of highly oxygenated organic molecules (HOMs) and the nucleation of the HOMs generated by limonene S. Wang et al. 10.1016/j.atmosenv.2023.119727
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- Organic Peroxides in Aerosol: Key Reactive Intermediates for Multiphase Processes in the Atmosphere S. Wang et al. 10.1021/acs.chemrev.2c00430
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- Structures and reactivity of peroxy radicals and dimeric products revealed by online tandem mass spectrometry S. Tomaz et al. 10.1038/s41467-020-20532-2
- Impacts of Mixed Gaseous and Particulate Pollutants on Secondary Particle Formation during Ozonolysis of Butyl Vinyl Ether P. Zhang et al. 10.1021/acs.est.9b07650
- Chemistry of new particle formation and growth events during wintertime in suburban area of Beijing: Insights from highly polluted atmosphere S. Yang et al. 10.1016/j.atmosres.2021.105553
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- Direct measurement of new particle formation based on tethered airship around the top of the planetary boundary layer in eastern China X. Qi et al. 10.1016/j.atmosenv.2019.04.024
- Vigorous New Particle Formation Above Polluted Boundary Layer in the North China Plain S. Lai et al. 10.1029/2022GL100301
- A kinetic partitioning method for simulating the condensation mass flux of organic vapors in a wide volatility range Y. Li et al. 10.1016/j.jaerosci.2024.106400
30 citations as recorded by crossref.
- New particle formation and its CCN enhancement in the Yangtze River Delta under the control of continental and marine air masses X. Fang et al. 10.1016/j.atmosenv.2021.118400
- Enhancement of Atmospheric Nucleation by Highly Oxygenated Organic Molecules: A Density Functional Theory Study F. Zhao et al. 10.1021/acs.jpca.9b03142
- Spatial Inhomogeneity of New Particle Formation in the Urban and Mountainous Atmospheres of the North China Plain during the 2022 Winter Olympics D. Shang et al. 10.3390/atmos14091395
- Response of organic aerosol characteristics to emission reduction in Yangtze River Delta region J. Wang et al. 10.1007/s11783-023-1714-0
- Insights into the chemistry of aerosol growth in Beijing: Implication of fine particle episode formation during wintertime S. Yang et al. 10.1016/j.chemosphere.2021.129776
- The neglected autoxidation pathways for the formation of highly oxygenated organic molecules (HOMs) and the nucleation of the HOMs generated by limonene S. Wang et al. 10.1016/j.atmosenv.2023.119727
- Comprehensive simulations of new particle formation events in Beijing with a cluster dynamics–multicomponent sectional model C. Li et al. 10.5194/acp-23-6879-2023
- Secondary reactions of aromatics-derived oxygenated organic molecules lead to plentiful highly oxygenated organic molecules within an intraday OH exposure Y. Wang et al. 10.5194/acp-24-7961-2024
- Observations of highly oxidized molecules and particle nucleation in the atmosphere of Beijing J. Brean et al. 10.5194/acp-19-14933-2019
- Measurement report: Contribution of atmospheric new particle formation to ultrafine particle concentration, cloud condensation nuclei, and radiative forcing – results from 5-year observations in central Europe J. Sun et al. 10.5194/acp-24-10667-2024
- Secondary aerosol formation in winter haze over the Beijing-Tianjin-Hebei Region, China D. Shang et al. 10.1007/s11783-020-1326-x
- Opinion: The strength of long-term comprehensive observations to meet multiple grand challenges in different environments and in the atmosphere M. Kulmala et al. 10.5194/acp-23-14949-2023
- Atmospheric new particle formation in China B. Chu et al. 10.5194/acp-19-115-2019
- New particle formation (NPF) events in China urban clusters given by sever composite pollution background Q. Zhang et al. 10.1016/j.chemosphere.2020.127842
- Nontrivial Impact of Relative Humidity on Organic New Particle Formation from Ozonolysis of cis-3-Hexenyl Acetate A. Flueckiger et al. 10.3390/air1040017
- Organic Peroxides in Aerosol: Key Reactive Intermediates for Multiphase Processes in the Atmosphere S. Wang et al. 10.1021/acs.chemrev.2c00430
- Atmospheric and ecosystem big data providing key contributions in reaching United Nations’ Sustainable Development Goals M. Kulmala et al. 10.1080/20964471.2021.1936943
- Aerosol mass yields of selected biogenic volatile organic compounds – a theoretical study with nearly explicit gas-phase chemistry C. Xavier et al. 10.5194/acp-19-13741-2019
- Theoretical study of the formation and nucleation mechanism of highly oxygenated multi-functional organic compounds produced by α-pinene X. Shi et al. 10.1016/j.scitotenv.2021.146422
- Measurement report: New particle formation characteristics at an urban and a mountain station in northern China Y. Zhou et al. 10.5194/acp-21-17885-2021
- New particle formation induced by anthropogenic–biogenic interactions on the southeastern Tibetan Plateau S. Lai et al. 10.5194/acp-24-2535-2024
- Structures and reactivity of peroxy radicals and dimeric products revealed by online tandem mass spectrometry S. Tomaz et al. 10.1038/s41467-020-20532-2
- Impacts of Mixed Gaseous and Particulate Pollutants on Secondary Particle Formation during Ozonolysis of Butyl Vinyl Ether P. Zhang et al. 10.1021/acs.est.9b07650
- Chemistry of new particle formation and growth events during wintertime in suburban area of Beijing: Insights from highly polluted atmosphere S. Yang et al. 10.1016/j.atmosres.2021.105553
- The striking effect of vertical mixing in the planetary boundary layer on new particle formation in the Yangtze River Delta S. Lai et al. 10.1016/j.scitotenv.2022.154607
- Atmospheric oxidation of (E)-β-farnesene initiated by hydroxyl radical: New formation mechanism of HOMs S. Zhang et al. 10.1016/j.jece.2023.110654
- Aerosol characteristics at the Southern Great Plains site during the HI-SCALE campaign J. Liu et al. 10.5194/acp-21-5101-2021
- Direct measurement of new particle formation based on tethered airship around the top of the planetary boundary layer in eastern China X. Qi et al. 10.1016/j.atmosenv.2019.04.024
- Vigorous New Particle Formation Above Polluted Boundary Layer in the North China Plain S. Lai et al. 10.1029/2022GL100301
- A kinetic partitioning method for simulating the condensation mass flux of organic vapors in a wide volatility range Y. Li et al. 10.1016/j.jaerosci.2024.106400
Latest update: 20 Nov 2024
Short summary
In this study we simulate the HOM concentrations and discuss their roles in NPF at a remote boreal forest site in Finland and a suburban site in eastern China. We found that sulfuric acid and HOM organonitrate concentrations in the gas phase are significantly higher but other HOM monomers and dimers from monoterpene oxidation are lower in eastern China. This study highlights the need for molecular-scale measurements in improving the understanding of NPF mechanisms in polluted areas.
In this study we simulate the HOM concentrations and discuss their roles in NPF at a remote...
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