Articles | Volume 19, issue 23
https://doi.org/10.5194/acp-19-14703-2019
https://doi.org/10.5194/acp-19-14703-2019
Research article
 | 
05 Dec 2019
Research article |  | 05 Dec 2019

Predominance of secondary organic aerosol to particle-bound reactive oxygen species activity in fine ambient aerosol

Jun Zhou, Miriam Elser, Ru-Jin Huang, Manuel Krapf, Roman Fröhlich, Deepika Bhattu, Giulia Stefenelli, Peter Zotter, Emily A. Bruns, Simone M. Pieber, Haiyan Ni, Qiyuan Wang, Yichen Wang, Yaqing Zhou, Chunying Chen, Mao Xiao, Jay G. Slowik, Samuel Brown, Laure-Estelle Cassagnes, Kaspar R. Daellenbach, Thomas Nussbaumer, Marianne Geiser, André S. H. Prévôt, Imad El-Haddad, Junji Cao, Urs Baltensperger, and Josef Dommen

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Cited articles

Adams, K., Greenbaum, D. S., Shaikh, R., van Erp, A. M., and Russell, A. G.: Particulate matter components, sources, and health: Systematic approaches to testing effects, J. Air Waste Manag. Assoc., 65, 544–558, https://doi.org/10.1080/10962247.2014.1001884, 2015. 
Arashiro, M., Lin, Y.-H., Sexton, K. G., Zhang, Z., Jaspers, I., Fry, R. C., Vizuete, W. G., Gold, A., and Surratt, J. D.: In vitro exposure to isoprene-derived secondary organic aerosol by direct deposition and its effects on COX-2 and IL-8 gene expression, Atmos. Chem. Phys., 16, 14079–14090, https://doi.org/10.5194/acp-16-14079-2016, 2016. 
Arashiro, M., Lin, Y.-H., Zhang, Z., Sexton, K. G., Gold, A., Jaspers, I., Fry, R. C., and Surratt, J. D.: Effect of secondary organic aerosol from isoprene-derived hydroxyhydroperoxides on the expression of oxidative stress response genes in human bronchial epithelial cells, Environ. Science: Proc. Imp., 20, 332–339, https://doi.org/10.1039/C7EM00439G, 2018. 
Badali, K. M., Zhou, S., Aljawhary, D., Antiñolo, M., Chen, W. J., Lok, A., Mungall, E., Wong, J. P. S., Zhao, R., and Abbatt, J. P. D.: Formation of hydroxyl radicals from photolysis of secondary organic aerosol material, Atmos. Chem. Phys., 15, 7831–7840, https://doi.org/10.5194/acp-15-7831-2015, 2015. 
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Reactive oxygen species (ROS) are believed to contribute to the adverse health effects of aerosols. We measured particle-bound ROS (PB-ROS) with an online instrument in two distinct environments, i.e., Beijing (China) and Bern (Switzerland). In both cities these exogenic ROS are predominantly related to secondary organic aerosol (SOA). PB-ROS content in SOA from various anthropogenic emission sources tested in the laboratory was comparable to that in the ambient measurements.
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