Articles | Volume 19, issue 23
https://doi.org/10.5194/acp-19-14703-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-14703-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
05 Dec 2019
Research article |
| 05 Dec 2019
| 05 Dec 2019
Predominance of secondary organic aerosol to particle-bound reactive oxygen species activity in fine ambient aerosol
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
now at: Graduate School of Global Environmental Studies, Kyoto
University, Kyoto, 606-8501, Japan
Miriam Elser
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
now at: Automotive Powertrain Technologies, Empa, 8600
Dübendorf, Switzerland
Ru-Jin Huang
CORRESPONDING AUTHOR
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Institute of Earth Environment, Chinese Academy of Sciences, Xi'an,
710061, China
Manuel Krapf
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Roman Fröhlich
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Deepika Bhattu
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Giulia Stefenelli
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Peter Zotter
Bioenergy Research Group, Engineering and Architecture, Lucerne
University of Applied Sciences and Arts, 6048 Horw, Switzerland
Emily A. Bruns
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Simone M. Pieber
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
now at: Laboratory for Air Pollution / Environmental Technology, Empa,
8600 Dübendorf, Switzerland
Haiyan Ni
Institute of Earth Environment, Chinese Academy of Sciences, Xi'an,
710061, China
Qiyuan Wang
Institute of Earth Environment, Chinese Academy of Sciences, Xi'an,
710061, China
Yichen Wang
Institute of Earth Environment, Chinese Academy of Sciences, Xi'an,
710061, China
Yaqing Zhou
Institute of Earth Environment, Chinese Academy of Sciences, Xi'an,
710061, China
Chunying Chen
CAS Key Laboratory for Biological Effects of Nanomaterials and
Nanosafety, National Center for Nanoscience and Technology, Beijing, 100191,
China
Mao Xiao
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Jay G. Slowik
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Samuel Brown
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Institute for Atmospheric and Climate Science, ETH, 8092 Zurich,
Switzerland
Laure-Estelle Cassagnes
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Kaspar R. Daellenbach
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
now at: Institute for Atmospheric and Earth System Research,
Faculty of Science, University of Helsinki, 00014, Helsinki, Finland
Thomas Nussbaumer
Bioenergy Research Group, Engineering and Architecture, Lucerne
University of Applied Sciences and Arts, 6048 Horw, Switzerland
Marianne Geiser
Institute of Anatomy, University of Bern, 3012 Bern, Switzerland
André S. H. Prévôt
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Imad El-Haddad
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Junji Cao
Institute of Earth Environment, Chinese Academy of Sciences, Xi'an,
710061, China
Urs Baltensperger
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
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- Multiphase Reactions between Secondary Organic Aerosol and Sulfur Dioxide: Kinetics and Contributions to Sulfate Formation and Aerosol Aging M. Yao et al. 10.1021/acs.estlett.9b00657
33 citations as recorded by crossref.
- Effect of Renewable Fuels and Intake O2 Concentration on Diesel Engine Emission Characteristics and Reactive Oxygen Species (ROS) Formation L. Gren et al. 10.3390/atmos11060641
- Dynamic Wood Smoke Aerosol Toxicity during Oxidative Atmospheric Aging S. Wang et al. 10.1021/acs.est.2c05929
- Source apportionment of oxidative potential: What we know so far S. Stevanovic et al. 10.2298/TSCI221107111S
- Aqueous-phase chemistry of atmospheric phenolic compounds: A critical review of laboratory studies F. Li et al. 10.1016/j.scitotenv.2022.158895
- Highly time-resolved chemical speciation and source apportionment of organic aerosol components in Delhi, India, using extractive electrospray ionization mass spectrometry V. Kumar et al. 10.5194/acp-22-7739-2022
- Substantial contribution of transported emissions to organic aerosol in Beijing K. Daellenbach et al. 10.1038/s41561-024-01493-3
- Kinetics and impacting factors of HO2 uptake onto submicron atmospheric aerosols during the 2019 Air QUAlity Study (AQUAS) in Yokohama, Japan J. Zhou et al. 10.5194/acp-21-12243-2021
- Pathogenic Mechanisms of Secondary Organic Aerosols T. Déméautis et al. 10.1021/acs.chemrestox.1c00353
- Brown Carbon in Primary and Aged Coal Combustion Emission H. Ni et al. 10.1021/acs.est.0c08084
- Source apportionment of atmospheric PM10 oxidative potential: synthesis of 15 year-round urban datasets in France S. Weber et al. 10.5194/acp-21-11353-2021
- Aging Effects on the Toxicity Alteration of Different Types of Organic Aerosols: A Review R. Lei et al. 10.1007/s40726-023-00272-9
- Reaction Rate Coefficient of OH Radicals with d9-Butanol as a Function of Temperature A. Allani et al. 10.1021/acsomega.1c01942
- Aged and Obscured Wildfire Smoke Associated with Downwind Health Risks T. Joo et al. 10.1021/acs.estlett.4c00785
- Disparities in particulate matter (PM10) origins and oxidative potential at a city scale (Grenoble, France) – Part 2: Sources of PM10 oxidative potential using multiple linear regression analysis and the predictive applicability of multilayer perceptron neural network analysis L. Borlaza et al. 10.5194/acp-21-9719-2021
- Secondary organic aerosol formed by condensing anthropogenic vapours over China’s megacities W. Nie et al. 10.1038/s41561-022-00922-5
- Sulfate Formation by Photosensitization in Mixed Incense Burning–Sodium Chloride Particles: Effects of RH, Light Intensity, and Aerosol Aging R. Tang et al. 10.1021/acs.est.3c02225
- Production of Peroxy Radicals from the Photochemical Reaction of Fatty Acids at the Air–Water Interface N. Hayeck et al. 10.1021/acsearthspacechem.0c00048
- Real-time quantification of the total HO2 reactivity of ambient air and HO2 uptake kinetics onto ambient aerosols in Kyoto (Japan) J. Zhou et al. 10.1016/j.atmosenv.2019.117189
- Organic Peroxides in Aerosol: Key Reactive Intermediates for Multiphase Processes in the Atmosphere S. Wang et al. 10.1021/acs.chemrev.2c00430
- Are reactive oxygen species (ROS) a suitable metric to predict toxicity of carbonaceous aerosol particles? Z. Zhang et al. 10.5194/acp-22-1793-2022
- Environmentally persistent free radicals in indoor particulate matter, dust, and on surfaces A. Filippi et al. 10.1039/D1EA00075F
- Development and Validation of the Particle into Nitroxide Quencher System with BPEAnit Probe for High-Sensitivity Reactive Oxygen Species Detection in Atmospheric Monitoring R. Wang et al. 10.3390/s25041129
- Specific differences and responses to reductions for premature mortality attributable to ambient PM2.5 in China Y. Li et al. 10.1016/j.scitotenv.2020.140643
- Oxidative potential associated with water-soluble components of PM2.5 in Beijing: The important role of anthropogenic organic aerosols Q. Yu et al. 10.1016/j.jhazmat.2022.128839
- Disentangling fine particles (PM2.5) composition in Hanoi, Vietnam: Emission sources and oxidative potential P. Dominutti et al. 10.1016/j.scitotenv.2024.171466
- Contributions of acidic ions in secondary aerosol to PM2.5 bioreactivity in an urban area V. Laiman et al. 10.1016/j.atmosenv.2022.119001
- Inter-continental variability in the relationship of oxidative potential and cytotoxicity with PM2.5 mass S. Salana et al. 10.1038/s41467-024-49649-4
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- Particle-bound reactive oxygen species in cooking emissions: Aging effects and cytotoxicity L. Lu et al. 10.1016/j.atmosenv.2023.120309
- Predominance of secondary organic aerosol to particle-bound reactive oxygen species activity in fine ambient aerosol J. Zhou et al. 10.5194/acp-19-14703-2019
- Online monitoring of volatile organic compounds emitted from human bronchial epithelial cells as markers for oxidative stress L. Cassagnes et al. 10.1088/1752-7163/abc055
- Mortality Attributable to Ambient Air Pollution: A Review of Global Estimates A. Pozzer et al. 10.1029/2022GH000711
Latest update: 08 Jul 2025
Short summary
Reactive oxygen species (ROS) are believed to contribute to the adverse health effects of aerosols. We measured particle-bound ROS (PB-ROS) with an online instrument in two distinct environments, i.e., Beijing (China) and Bern (Switzerland). In both cities these exogenic ROS are predominantly related to secondary organic aerosol (SOA). PB-ROS content in SOA from various anthropogenic emission sources tested in the laboratory was comparable to that in the ambient measurements.
Reactive oxygen species (ROS) are believed to contribute to the adverse health effects of...
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