Articles | Volume 17, issue 21
https://doi.org/10.5194/acp-17-13361-2017
https://doi.org/10.5194/acp-17-13361-2017
Research article
 | 
10 Nov 2017
Research article |  | 10 Nov 2017

Estimation of atmospheric particle formation rates through an analytical formula: validation and application in Hyytiälä and Puijo, Finland

Elham Baranizadeh, Tuomo Nieminen, Taina Yli-Juuti, Markku Kulmala, Tuukka Petäjä, Ari Leskinen, Mika Komppula, Ari Laaksonen, and Kari E. J. Lehtinen

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Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
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Cited articles

Aalto, P., Hämeri, K., Becker, E., Weber, R., Salm, J., Mäkelä, J., Hoell, C., O'dowd, C., Hansson, H.-C., Väkevä, M., Koponen, I., Buzorius, G., and Kulmala, M.: Physical characterization of aerosol particles during nucleation events, Tellus B, 53, 344–358, https://doi.org/10.3402/tellusb.v53i4.17127, 2001.
Berndt, T., Sipilä, M., Stratmann, F., Petäjä, T., Vanhanen, J., Mikkilä, J., Patokoski, J., Taipale, R., Mauldin III, R. L., and Kulmala, M.: Enhancement of atmospheric H2SO4 ∕ H2O nucleation: organic oxidation products versus amines, Atmos. Chem. Phys., 14, 751–764, https://doi.org/10.5194/acp-14-751-2014, 2014.
Dal Maso, M., Kulmala, M., Riipinen, I., Wagner, R., Hussein, T., Aalto, P. P., and Lehtinen, K. E. J.: Formation and growth of fresh atmospheric aerosols: eight years of aerosol size distribution data from SMEAR II, Hyytiälä, Finland, Boreal Environ. Res., 10, 323–336, 2005.
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Short summary
Extrapolation of the particle formation rates from one measured larger size (e.g., 7 nm) to smaller sizes (e.g., 3 nm) based on simplified growth-scavenging dynamics works fairly well to estimate mean daily formation rates, but it fails to predict the time evolution of the particle population. This points to the challenges in predicting atmospheric nucleation rates for locations where the particle growth and loss rates are size- and time-dependent.
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