Articles | Volume 16, issue 6
https://doi.org/10.5194/acp-16-3727-2016
https://doi.org/10.5194/acp-16-3727-2016
Research article
 | 
21 Mar 2016
Research article |  | 21 Mar 2016

Simulating the formation of carbonaceous aerosol in a European Megacity (Paris) during the MEGAPOLI summer and winter campaigns

Christos Fountoukis, Athanasios G. Megaritis, Ksakousti Skyllakou, Panagiotis E. Charalampidis, Hugo A. C. Denier van der Gon, Monica Crippa, André S. H. Prévôt, Friederike Fachinger, Alfred Wiedensohler, Christodoulos Pilinis, and Spyros N. Pandis

Related authors

Spatiotemporal variation of radionuclide dispersion from nuclear power plant accidents using FLEXPART mini-ensemble modeling
Seyed Omid Nabavi, Theodoros Christoudias, Yiannis Proestos, Christos Fountoukis, Huda Al-Sulaiti, and Jos Lelieveld
Atmos. Chem. Phys., 23, 7719–7739, https://doi.org/10.5194/acp-23-7719-2023,https://doi.org/10.5194/acp-23-7719-2023, 2023
Short summary
Simulation of the size-composition distribution of atmospheric nanoparticles over Europe
David Patoulias, Christos Fountoukis, Ilona Riipinen, Ari Asmi, Markku Kulmala, and Spyros N. Pandis
Atmos. Chem. Phys., 18, 13639–13654, https://doi.org/10.5194/acp-18-13639-2018,https://doi.org/10.5194/acp-18-13639-2018, 2018
Short summary
Comparison of PMCAMx aerosol optical depth predictions over Europe with AERONET and MODIS measurements
Antigoni Panagiotopoulou, Panagiotis Charalampidis, Christos Fountoukis, Christodoulos Pilinis, and Spyros N. Pandis
Geosci. Model Dev., 9, 4257–4272, https://doi.org/10.5194/gmd-9-4257-2016,https://doi.org/10.5194/gmd-9-4257-2016, 2016
Short summary
Implementation of state-of-the-art ternary new-particle formation scheme to the regional chemical transport model PMCAMx-UF in Europe
Elham Baranizadeh, Benjamin N. Murphy, Jan Julin, Saeed Falahat, Carly L. Reddington, Antti Arola, Lars Ahlm, Santtu Mikkonen, Christos Fountoukis, David Patoulias, Andreas Minikin, Thomas Hamburger, Ari Laaksonen, Spyros N. Pandis, Hanna Vehkamäki, Kari E. J. Lehtinen, and Ilona Riipinen
Geosci. Model Dev., 9, 2741–2754, https://doi.org/10.5194/gmd-9-2741-2016,https://doi.org/10.5194/gmd-9-2741-2016, 2016
Short summary
Aerosol water parameterisation: a single parameter framework
Swen Metzger, Benedikt Steil, Mohamed Abdelkader, Klaus Klingmüller, Li Xu, Joyce E. Penner, Christos Fountoukis, Athanasios Nenes, and Jos Lelieveld
Atmos. Chem. Phys., 16, 7213–7237, https://doi.org/10.5194/acp-16-7213-2016,https://doi.org/10.5194/acp-16-7213-2016, 2016
Short summary

Related subject area

Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Opinion: The role of AerChemMIP in advancing climate and air quality research
Paul T. Griffiths, Laura J. Wilcox, Robert J. Allen, Vaishali Naik, Fiona M. O'Connor, Michael Prather, Alex Archibald, Florence Brown, Makoto Deushi, William Collins, Stephanie Fiedler, Naga Oshima, Lee T. Murray, Bjørn H. Samset, Chris Smith, Steven Turnock, Duncan Watson-Parris, and Paul J. Young
Atmos. Chem. Phys., 25, 8289–8328, https://doi.org/10.5194/acp-25-8289-2025,https://doi.org/10.5194/acp-25-8289-2025, 2025
Short summary
Uncertainties in the effects of organic aerosol coatings on polycyclic aromatic hydrocarbon concentrations and their estimated health effects
Sijia Lou, Manish Shrivastava, Alexandre Albinet, Sophie Tomaz, Deepchandra Srivastava, Olivier Favez, Huizhong Shen, and Aijun Ding
Atmos. Chem. Phys., 25, 8163–8183, https://doi.org/10.5194/acp-25-8163-2025,https://doi.org/10.5194/acp-25-8163-2025, 2025
Short summary
Source-explicit estimation of brown carbon in the polluted atmosphere over the North China Plain: implications for distribution, absorption, and the direct radiative effect
Jiamao Zhou, Jiarui Wu, Xiaoli Su, Ruonan Wang, Imad EI Haddad, Xia Li, Qian Jiang, Ting Zhang, Wenting Dai, Junji Cao, Andre S. H. Prevot, Xuexi Tie, and Guohui Li
Atmos. Chem. Phys., 25, 7563–7580, https://doi.org/10.5194/acp-25-7563-2025,https://doi.org/10.5194/acp-25-7563-2025, 2025
Short summary
Implications of reduced-complexity aerosol thermodynamics on organic aerosol mass concentration and composition over North America
Camilo Serrano Damha, Kyle Gorkowski, and Andreas Zuend
Atmos. Chem. Phys., 25, 5773–5792, https://doi.org/10.5194/acp-25-5773-2025,https://doi.org/10.5194/acp-25-5773-2025, 2025
Short summary
Trends and drivers of soluble iron deposition from East Asian dust to the Northwest Pacific: a springtime analysis (2001–2017)
Hanzheng Zhu, Yaman Liu, Man Yue, Shihui Feng, Pingqing Fu, Kan Huang, Xinyi Dong, and Minghuai Wang
Atmos. Chem. Phys., 25, 5175–5197, https://doi.org/10.5194/acp-25-5175-2025,https://doi.org/10.5194/acp-25-5175-2025, 2025
Short summary

Cited articles

Airparif: Ile-de-France gridded emission inventory 2005 (version 2008), http://www.airparif.asso.fr/ (last access: 1 October 2015), 2010.
Allan, J. D., Williams, P. I., Morgan, W. T., Martin, C. L., Flynn, M. J., Lee, J., Nemitz, E., Phillips, G. J., Gallagher, M. W., and Coe, H.: Contributions from transport, solid fuel burning and cooking to primary organic aerosols in two UK cities, Atmos. Chem. Phys., 10, 647–668, https://doi.org/10.5194/acp-10-647-2010, 2010.
Atkinson, R. and Arey, J.: Atmospheric degradation of volatile organic compounds, Chem. Rev., 103, 4605–4638, 2003.
Bergström, R., Denier van der Gon, H. A. C., Prévôt, A. S. H., Yttri, K. E., and Simpson, D.: Modelling of organic aerosols over Europe (2002–2007) using a volatility basis set (VBS) framework: application of different assumptions regarding the formation of secondary organic aerosol, Atmos. Chem. Phys., 12, 8499–8527, https://doi.org/10.5194/acp-12-8499-2012, 2012.
Download
Short summary
We use PMCAMx with high grid resolution over Paris to simulate carbonaceous aerosol during the summer and winter MEGAPOLI campaigns. PMCAMx reproduces BC observations well. Addition of cooking organic aerosol emissions of 80 mg per day per capita is needed to reproduce the corresponding observations. While the oxygenated organic aerosol predictions during the summer are encouraging a major wintertime source appears to be missing.
Share
Altmetrics
Final-revised paper
Preprint