Articles | Volume 20, issue 21
https://doi.org/10.5194/acp-20-12721-2020
https://doi.org/10.5194/acp-20-12721-2020
Research article
 | 
04 Nov 2020
Research article |  | 04 Nov 2020

Size-segregated particle number and mass concentrations from different emission sources in urban Beijing

Jing Cai, Biwu Chu, Lei Yao, Chao Yan, Liine M. Heikkinen, Feixue Zheng, Chang Li, Xiaolong Fan, Shaojun Zhang, Daoyuan Yang, Yonghong Wang, Tom V. Kokkonen, Tommy Chan, Ying Zhou, Lubna Dada, Yongchun Liu, Hong He, Pauli Paasonen, Joni T. Kujansuu, Tuukka Petäjä, Claudia Mohr, Juha Kangasluoma, Federico Bianchi, Yele Sun, Philip L. Croteau, Douglas R. Worsnop, Veli-Matti Kerminen, Wei Du, Markku Kulmala, and Kaspar R. Daellenbach

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Cited articles

Abdullahi, K. L., Delgado-Saborit, J. M., and Harrison, R. M.: Emissions and indoor concentrations of particulate matter and its specific chemical components from cooking: A review, Atmos. Environ., 71, 260–294, https://doi.org/10.1016/j.atmosenv.2013.01.061, 2013. 
Beddows, D. C. S. and Harrison, R. M.: Receptor modelling of both particle composition and size distribution from a background site in London, UK – a two-step approach, Atmos. Chem. Phys., 19, 4863–4876, https://doi.org/10.5194/acp-19-4863-2019, 2019. 
Budisulistiorini, S. H., Canagaratna, M. R., Croteau, P. L., Baumann, K., Edgerton, E. S., Kollman, M. S., Ng, N. L., Verma, V., Shaw, S. L., Knipping, E. M., Worsnop, D. R., Jayne, J. T., Weber, R. J., and Surratt, J. D.: Intercomparison of an Aerosol Chemical Speciation Monitor (ACSM) with ambient fine aerosol measurements in downtown Atlanta, Georgia, Atmos. Meas. Tech., 7, 1929–1941, https://doi.org/10.5194/amt-7-1929-2014, 2014. 
Buonanno, G., Dell'Isola, M., Stabile, L., and Viola, A.: Uncertainty Budget of the SMPS–APS System in the Measurement of PM1, PM2.5, and PM10, Aerosol Sci. Tech., 43, 1130–1141, https://doi.org/10.1080/02786820903204078, 2009a. 
Buonanno, G., Morawska, L., and Stabile, L.: Particle emission factors during cooking activities, Atmos. Environ., 43, 3235–3242, https://doi.org/10.1016/j.atmosenv.2009.03.044, 2009b. 
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Short summary
By applying both OA PMF and size PMF at the same urban measurement site in Beijing, similar particle source types, including vehicular emissions, cooking emissions and secondary formation-related sources, were resolved by both frameworks and agreed well. It is also found that in the absence of new particle formation, vehicular and cooking emissions dominate the particle number concentration, while secondary particulate matter governed PM2.5 mass during spring and summer in Beijing.
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