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Volume 18, issue 2
Atmos. Chem. Phys., 18, 673–689, 2018
https://doi.org/10.5194/acp-18-673-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 3.0 License.

Special issue: HD(CP)2 Observational Prototype Experiment (AMT/ACP...

Atmos. Chem. Phys., 18, 673–689, 2018
https://doi.org/10.5194/acp-18-673-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 19 Jan 2018

Research article | 19 Jan 2018

A parameterization of the heterogeneous hydrolysis of N2O5 for mass-based aerosol models: improvement of particulate nitrate prediction

Ying Chen et al.

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Cited articles

Anttila, T., Kiendler-Scharr, A., Tillmann, R., and Mentel, T. F.: On the Reactive Uptake of Gaseous Compounds by Organic-Coated Aqueous Aerosols:? Theoretical Analysis and Application to the Heterogeneous Hydrolysis of N2O5, J. Phys. Chem. A, 110, 10435–10443, https://doi.org/10.1021/jp062403c, 2006.
Archer-Nicholls, S., Lowe, D., Utembe, S., Allan, J., Zaveri, R. A., Fast, J. D., Hodnebrog, Ø., Denier van der Gon, H., and McFiggans, G.: Gaseous chemistry and aerosol mechanism developments for version 3.5.1 of the online regional model, WRF-Chem, Geosci. Model Dev., 7, 2557–2579, https://doi.org/10.5194/gmd-7-2557-2014, 2014.
Backes, A. M., Aulinger, A., Bieser, J., Matthias, V., and Quante, M.: Ammonia emissions in Europe, part II: How ammonia emission abatement strategies affect secondary aerosols, Atmos. Environ., 126, 153–161, https://doi.org/10.1016/j.atmosenv.2015.11.039, 2016.
Badger, C. L., Griffiths, P. T., George, I., Abbatt, J. P. D., and Cox, R. A.: Reactive Uptake of N2O5 by Aerosol Particles Containing Mixtures of Humic Acid and Ammonium Sulfate, J. Phys. Chem. A, 110, 6986–6994, https://doi.org/10.1021/jp0562678, 2006.
Baldauf, M., Seifert, A., Förstner, J., Majewski, D., Raschendorfer, M., and Reinhardt, T.: Operational Convective-Scale Numerical Weather Prediction with the COSMO Model: Description and Sensitivities, Mon. Weather Rev., 139, 3887–3905, https://doi.org/10.1175/mwr-d-10-05013.1, 2011.
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The heterogeneous hydrolysis of N2O5 on particle surfaces is crucial for the nitrogen cycle in the atmosphere. The reaction rate is determined by meteorological and particle properties, but its parameterization in previous 3-D modelling studies did not comprehensively consider these parameters. We propose a parameterization to take these into account and improve nitrate prediction; we report that the organic coating suppression on the N2O5 reaction is not as important as expected in the EU.
The heterogeneous hydrolysis of N2O5 on particle surfaces is crucial for the nitrogen cycle in...
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