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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
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Volume 18, issue 2
Atmos. Chem. Phys., 18, 673–689, 2018
https://doi.org/10.5194/acp-18-673-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 3.0 License.

Special issue: HD(CP)2 Observational Prototype Experiment (AMT/ACP...

Atmos. Chem. Phys., 18, 673–689, 2018
https://doi.org/10.5194/acp-18-673-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 19 Jan 2018

Research article | 19 Jan 2018

A parameterization of the heterogeneous hydrolysis of N2O5 for mass-based aerosol models: improvement of particulate nitrate prediction

Ying Chen et al.

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Status: closed
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AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment
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AR: Author's response | RR: Referee report | ED: Editor decision
AR by Ying Chen on behalf of the Authors (28 Jun 2017)  Author's response    Manuscript
ED: Referee Nomination & Report Request started (11 Jul 2017) by Herman Russchenberg
ED: Publish as is (04 Dec 2017) by Herman Russchenberg
Publications Copernicus
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Short summary
The heterogeneous hydrolysis of N2O5 on particle surfaces is crucial for the nitrogen cycle in the atmosphere. The reaction rate is determined by meteorological and particle properties, but its parameterization in previous 3-D modelling studies did not comprehensively consider these parameters. We propose a parameterization to take these into account and improve nitrate prediction; we report that the organic coating suppression on the N2O5 reaction is not as important as expected in the EU.
The heterogeneous hydrolysis of N2O5 on particle surfaces is crucial for the nitrogen cycle in...
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