Articles | Volume 19, issue 14
https://doi.org/10.5194/acp-19-9351-2019
https://doi.org/10.5194/acp-19-9351-2019
Research article
 | 
22 Jul 2019
Research article |  | 22 Jul 2019

Modeling of aerosol property evolution during winter haze episodes over a megacity cluster in northern China: roles of regional transport and heterogeneous reactions of SO2

Huiyun Du, Jie Li, Xueshun Chen, Zifa Wang, Yele Sun, Pingqing Fu, Jianjun Li, Jian Gao, and Ying Wei

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Cited articles

Anderson, H. R., Atkinson, R., Balbus, J., Brauer, M., Chapman, R., and Chowdhury, Z.: Outdoor Air Pollution and Health in the Developing Countries of Asia: A Comprehensive Review, Special Report 18, Health Effects Institute, Boston, MA, 2010. 
Bian, Y. X., Zhao, C. S., Ma, N., Chen, J., and Xu, W. Y.: A study of aerosol liquid water content based on hygroscopicity measurements at high relative humidity in the North China Plain, Atmos. Chem. Phys., 14, 6417–6426, https://doi.org/10.5194/acp-14-6417-2014, 2014. 
Boylan, J. W. and Russell, A. G.: PM and light extinction model performance metrics, goals, and criteria for three-dimensional air quality models, Atmos. Environ., 40, 4946–4959, https://doi.org/10.1016/j.atmosenv.2005.09.087, 2006. 
Cao J.: PM2.5 and environment, Science Press, 2014. 
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Regional transport and heterogeneous reactions play crucial roles in haze formation. Using a chemical transport model, we found that chemical transformation of SO2 along the transport pathway from source regions to Beijing was the major source of sulfate. Heterogeneous chemistry had a stronger effect under high humidity and high pollution levels. Aerosols underwent aging during transport which altered the aerosol size and the degree of aging.
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