Articles | Volume 19, issue 14
https://doi.org/10.5194/acp-19-9351-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-9351-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
22 Jul 2019
Research article |
| 22 Jul 2019
| 22 Jul 2019
Modeling of aerosol property evolution during winter haze episodes over a megacity cluster in northern China: roles of regional transport and heterogeneous reactions of SO2
Huiyun Du
CORRESPONDING AUTHOR
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Jie Li
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China
Xueshun Chen
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
Zifa Wang
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China
Pingqing Fu
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
Jianjun Li
China National Environmental Monitoring Center, Beijing 100012, China
Jian Gao
Chinese Research Academy of Environmental Sciences, Beijing 100012, China
Ying Wei
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Viewed
Total article views: 3,192 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 27 Nov 2018)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 2,117 | 1,004 | 71 | 3,192 | 303 | 81 | 88 |
- HTML: 2,117
- PDF: 1,004
- XML: 71
- Total: 3,192
- Supplement: 303
- BibTeX: 81
- EndNote: 88
Total article views: 2,367 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 22 Jul 2019)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 1,608 | 693 | 66 | 2,367 | 169 | 77 | 81 |
- HTML: 1,608
- PDF: 693
- XML: 66
- Total: 2,367
- Supplement: 169
- BibTeX: 77
- EndNote: 81
Total article views: 825 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 27 Nov 2018)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 509 | 311 | 5 | 825 | 134 | 4 | 7 |
- HTML: 509
- PDF: 311
- XML: 5
- Total: 825
- Supplement: 134
- BibTeX: 4
- EndNote: 7
Viewed (geographical distribution)
Total article views: 3,192 (including HTML, PDF, and XML)
Thereof 2,971 with geography defined
and 221 with unknown origin.
Total article views: 2,367 (including HTML, PDF, and XML)
Thereof 2,226 with geography defined
and 141 with unknown origin.
Total article views: 825 (including HTML, PDF, and XML)
Thereof 745 with geography defined
and 80 with unknown origin.
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
Cited
35 citations as recorded by crossref.
- Enhanced mixing state of black carbon with nitrate in single particles during haze periods in Zhengzhou, China Q. Zhou et al. 10.1016/j.jes.2021.03.031
- High-resolution Simulation Dataset of Hourly PM2.5 Chemical Composition in China (CAQRA-aerosol) from 2013 to 2020 L. Kong et al. 10.1007/s00376-024-4046-5
- Global–regional nested simulation of particle number concentration by combing microphysical processes with an evolving organic aerosol module X. Chen et al. 10.5194/acp-21-9343-2021
- Regional transport dominates air pollution events in all seasons in Beijing in 2020 Z. Zhang et al. 10.1016/j.atmosenv.2024.120395
- Rapid transition in winter aerosol composition in Beijing from 2014 to 2017: response to clean air actions H. Li et al. 10.5194/acp-19-11485-2019
- Annual nonmethane hydrocarbon trends in Beijing from 2000 to 2019 D. Yao et al. 10.1016/j.jes.2021.04.017
- Size-resolved characterization of organic aerosol in the North China Plain: new insights from high resolution spectral analysis W. Xu et al. 10.1039/D1EA00025J
- Meteorological mechanisms of regional PM2.5 and O3 transport in the North China Plain driven by the East Asian monsoon S. Liu et al. 10.1016/j.apr.2022.101638
- The effect of cross-regional transport on ozone and particulate matter pollution in China: A review of methodology and current knowledge K. Qu et al. 10.1016/j.scitotenv.2024.174196
- Persistent residential burning-related primary organic particles during wintertime hazes in North China: insights into their aging and optical changes L. Liu et al. 10.5194/acp-21-2251-2021
- Measurement report: On the contribution of long-distance transport to the secondary aerosol formation and aging H. Zhong et al. 10.5194/acp-22-9513-2022
- Effects of Regional Transport on Haze in the North China Plain: Transport of Precursors or Secondary Inorganic Aerosols H. Du et al. 10.1029/2020GL087461
- Aerosol Evolution and Influencing Factor Analysis during Haze Periods in the Guanzhong Area of China Based on Multi-Source Data Y. Zhong et al. 10.3390/atmos13121975
- Simultaneous measurements of urban and rural particles in Beijing – Part 2: Case studies of haze events and regional transport Y. Chen et al. 10.5194/acp-20-9249-2020
- A 3D study on the amplification of regional haze and particle growth by local emissions W. Du et al. 10.1038/s41612-020-00156-5
- Characteristics and similarity relations of turbulence dispersion parameters under heavy haze conditions L. Liu et al. 10.1016/j.apr.2020.11.014
- Evaluation and Bias Correction of the Secondary Inorganic Aerosol Modeling over North China Plain in Autumn and Winter Q. Wu et al. 10.3390/atmos12050578
- Cross-boundary transport and source apportionment for PM2.5 in a typical industrial city in the Hebei Province, China: A modeling study X. Liu et al. 10.1016/j.jes.2021.03.008
- Modeling of polycyclic aromatic hydrocarbons (PAHs) from global to regional scales: model development (IAP-AACM_PAH v1.0) and investigation of health risks in 2013 and 2018 in China Z. Wu et al. 10.5194/gmd-17-8885-2024
- Optimal emission reduction scheme aimed at eliminating PM2.5 city pollution days within North China during a haze episode Z. Ye et al. 10.1016/j.apr.2023.101712
- PM2.5 and O3 pollution during 2015–2019 over 367 Chinese cities: Spatiotemporal variations, meteorological and topographical impacts S. Zhao et al. 10.1016/j.envpol.2020.114694
- Exploring the Influence of 34S Fractionation From Emission Sources and SO2 Atmospheric Oxidation on Sulfate Source Apportionment Based on Hourly Resolution δ34S‐SO2/SO42− X. Feng et al. 10.1029/2023JD038595
- Assessment of the effect of meteorological and emission variations on winter PM2.5 over the North China Plain in the three-year action plan against air pollution in 2018–2020 H. Du et al. 10.1016/j.atmosres.2022.106395
- Source apportionment and regional transport of PM2.5 during haze episodes in Beijing combined with multiple models L. Lv et al. 10.1016/j.atmosres.2021.105957
- Unexpected high contribution of in-cloud wet scavenging to nitrogen deposition induced by pumping effect of typhoon landfall in China Q. Tan et al. 10.1088/2515-7620/acb90b
- Increasing impacts of the relative contributions of regional transport on air pollution in Beijing: Observational evidence Q. Tan et al. 10.1016/j.envpol.2021.118407
- Optimal emission control plan aiming to basically eliminate PM2.5 heavy pollution in North and Northwest China in 2018 Z. Ye et al. 10.1016/j.jclepro.2024.142893
- Characteristics and sources of PM2.5 with focus on two severe pollution events in a coastal city of Qingdao, China Y. Gao et al. 10.1016/j.chemosphere.2020.125861
- Development of a city-level surface ozone forecasting system using deep learning techniques and air quality model: Application in eastern China Q. Li et al. 10.1016/j.atmosenv.2024.120865
- Variability of turbulence dispersion characteristics during heavy haze process: A case study in Beijing L. Liu et al. 10.1016/j.jes.2021.10.034
- Insights into air pollution chemistry and sulphate formation from nitrous acid (HONO) measurements during haze events in Beijing W. Bloss et al. 10.1039/D0FD00100G
- Sources of PM2.5 and its responses to emission reduction strategies in the Central Plains Economic Region in China: Implications for the impacts of COVID-19 H. Du et al. 10.1016/j.envpol.2021.117783
- Hydroxymethanesulfonate formation as a significant pathway of transformation of SO2 H. Zhang et al. 10.1016/j.atmosenv.2022.119474
- Development of a coupled aerosol lidar data quality assurance and control scheme with Monte Carlo analysis and bilateral filtering H. Wang et al. 10.1016/j.scitotenv.2020.138844
- Introduction to the special issue “In-depth study of air pollution sources and processes within Beijing and its surrounding region (APHH-Beijing)” Z. Shi et al. 10.5194/acp-19-7519-2019
34 citations as recorded by crossref.
- Enhanced mixing state of black carbon with nitrate in single particles during haze periods in Zhengzhou, China Q. Zhou et al. 10.1016/j.jes.2021.03.031
- High-resolution Simulation Dataset of Hourly PM2.5 Chemical Composition in China (CAQRA-aerosol) from 2013 to 2020 L. Kong et al. 10.1007/s00376-024-4046-5
- Global–regional nested simulation of particle number concentration by combing microphysical processes with an evolving organic aerosol module X. Chen et al. 10.5194/acp-21-9343-2021
- Regional transport dominates air pollution events in all seasons in Beijing in 2020 Z. Zhang et al. 10.1016/j.atmosenv.2024.120395
- Rapid transition in winter aerosol composition in Beijing from 2014 to 2017: response to clean air actions H. Li et al. 10.5194/acp-19-11485-2019
- Annual nonmethane hydrocarbon trends in Beijing from 2000 to 2019 D. Yao et al. 10.1016/j.jes.2021.04.017
- Size-resolved characterization of organic aerosol in the North China Plain: new insights from high resolution spectral analysis W. Xu et al. 10.1039/D1EA00025J
- Meteorological mechanisms of regional PM2.5 and O3 transport in the North China Plain driven by the East Asian monsoon S. Liu et al. 10.1016/j.apr.2022.101638
- The effect of cross-regional transport on ozone and particulate matter pollution in China: A review of methodology and current knowledge K. Qu et al. 10.1016/j.scitotenv.2024.174196
- Persistent residential burning-related primary organic particles during wintertime hazes in North China: insights into their aging and optical changes L. Liu et al. 10.5194/acp-21-2251-2021
- Measurement report: On the contribution of long-distance transport to the secondary aerosol formation and aging H. Zhong et al. 10.5194/acp-22-9513-2022
- Effects of Regional Transport on Haze in the North China Plain: Transport of Precursors or Secondary Inorganic Aerosols H. Du et al. 10.1029/2020GL087461
- Aerosol Evolution and Influencing Factor Analysis during Haze Periods in the Guanzhong Area of China Based on Multi-Source Data Y. Zhong et al. 10.3390/atmos13121975
- Simultaneous measurements of urban and rural particles in Beijing – Part 2: Case studies of haze events and regional transport Y. Chen et al. 10.5194/acp-20-9249-2020
- A 3D study on the amplification of regional haze and particle growth by local emissions W. Du et al. 10.1038/s41612-020-00156-5
- Characteristics and similarity relations of turbulence dispersion parameters under heavy haze conditions L. Liu et al. 10.1016/j.apr.2020.11.014
- Evaluation and Bias Correction of the Secondary Inorganic Aerosol Modeling over North China Plain in Autumn and Winter Q. Wu et al. 10.3390/atmos12050578
- Cross-boundary transport and source apportionment for PM2.5 in a typical industrial city in the Hebei Province, China: A modeling study X. Liu et al. 10.1016/j.jes.2021.03.008
- Modeling of polycyclic aromatic hydrocarbons (PAHs) from global to regional scales: model development (IAP-AACM_PAH v1.0) and investigation of health risks in 2013 and 2018 in China Z. Wu et al. 10.5194/gmd-17-8885-2024
- Optimal emission reduction scheme aimed at eliminating PM2.5 city pollution days within North China during a haze episode Z. Ye et al. 10.1016/j.apr.2023.101712
- PM2.5 and O3 pollution during 2015–2019 over 367 Chinese cities: Spatiotemporal variations, meteorological and topographical impacts S. Zhao et al. 10.1016/j.envpol.2020.114694
- Exploring the Influence of 34S Fractionation From Emission Sources and SO2 Atmospheric Oxidation on Sulfate Source Apportionment Based on Hourly Resolution δ34S‐SO2/SO42− X. Feng et al. 10.1029/2023JD038595
- Assessment of the effect of meteorological and emission variations on winter PM2.5 over the North China Plain in the three-year action plan against air pollution in 2018–2020 H. Du et al. 10.1016/j.atmosres.2022.106395
- Source apportionment and regional transport of PM2.5 during haze episodes in Beijing combined with multiple models L. Lv et al. 10.1016/j.atmosres.2021.105957
- Unexpected high contribution of in-cloud wet scavenging to nitrogen deposition induced by pumping effect of typhoon landfall in China Q. Tan et al. 10.1088/2515-7620/acb90b
- Increasing impacts of the relative contributions of regional transport on air pollution in Beijing: Observational evidence Q. Tan et al. 10.1016/j.envpol.2021.118407
- Optimal emission control plan aiming to basically eliminate PM2.5 heavy pollution in North and Northwest China in 2018 Z. Ye et al. 10.1016/j.jclepro.2024.142893
- Characteristics and sources of PM2.5 with focus on two severe pollution events in a coastal city of Qingdao, China Y. Gao et al. 10.1016/j.chemosphere.2020.125861
- Development of a city-level surface ozone forecasting system using deep learning techniques and air quality model: Application in eastern China Q. Li et al. 10.1016/j.atmosenv.2024.120865
- Variability of turbulence dispersion characteristics during heavy haze process: A case study in Beijing L. Liu et al. 10.1016/j.jes.2021.10.034
- Insights into air pollution chemistry and sulphate formation from nitrous acid (HONO) measurements during haze events in Beijing W. Bloss et al. 10.1039/D0FD00100G
- Sources of PM2.5 and its responses to emission reduction strategies in the Central Plains Economic Region in China: Implications for the impacts of COVID-19 H. Du et al. 10.1016/j.envpol.2021.117783
- Hydroxymethanesulfonate formation as a significant pathway of transformation of SO2 H. Zhang et al. 10.1016/j.atmosenv.2022.119474
- Development of a coupled aerosol lidar data quality assurance and control scheme with Monte Carlo analysis and bilateral filtering H. Wang et al. 10.1016/j.scitotenv.2020.138844
Latest update: 30 Mar 2025
Short summary
Regional transport and heterogeneous reactions play crucial roles in haze formation. Using a chemical transport model, we found that chemical transformation of SO2 along the transport pathway from source regions to Beijing was the major source of sulfate. Heterogeneous chemistry had a stronger effect under high humidity and high pollution levels. Aerosols underwent aging during transport which altered the aerosol size and the degree of aging.
Regional transport and heterogeneous reactions play crucial roles in haze formation. Using a...
Altmetrics
Final-revised paper
Preprint