Articles | Volume 19, issue 14
https://doi.org/10.5194/acp-19-9351-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-9351-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Modeling of aerosol property evolution during winter haze episodes over a megacity cluster in northern China: roles of regional transport and heterogeneous reactions of SO2
Huiyun Du
CORRESPONDING AUTHOR
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Jie Li
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China
Xueshun Chen
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
Zifa Wang
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China
Pingqing Fu
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
Jianjun Li
China National Environmental Monitoring Center, Beijing 100012, China
Jian Gao
Chinese Research Academy of Environmental Sciences, Beijing 100012, China
Ying Wei
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
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- A 3D study on the amplification of regional haze and particle growth by local emissions W. Du et al. 10.1038/s41612-020-00156-5
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- Optimal emission reduction scheme aimed at eliminating PM2.5 city pollution days within North China during a haze episode Z. Ye et al. 10.1016/j.apr.2023.101712
- PM2.5 and O3 pollution during 2015–2019 over 367 Chinese cities: Spatiotemporal variations, meteorological and topographical impacts S. Zhao et al. 10.1016/j.envpol.2020.114694
- Exploring the Influence of 34S Fractionation From Emission Sources and SO2 Atmospheric Oxidation on Sulfate Source Apportionment Based on Hourly Resolution δ34S‐SO2/SO42− X. Feng et al. 10.1029/2023JD038595
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- Optimal emission control plan aiming to basically eliminate PM2.5 heavy pollution in North and Northwest China in 2018 Z. Ye et al. 10.1016/j.jclepro.2024.142893
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Latest update: 08 Dec 2024
Short summary
Regional transport and heterogeneous reactions play crucial roles in haze formation. Using a chemical transport model, we found that chemical transformation of SO2 along the transport pathway from source regions to Beijing was the major source of sulfate. Heterogeneous chemistry had a stronger effect under high humidity and high pollution levels. Aerosols underwent aging during transport which altered the aerosol size and the degree of aging.
Regional transport and heterogeneous reactions play crucial roles in haze formation. Using a...
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