Articles | Volume 15, issue 18
https://doi.org/10.5194/acp-15-10777-2015
https://doi.org/10.5194/acp-15-10777-2015
Research article
 | 
28 Sep 2015
Research article |  | 28 Sep 2015

Modelling the contribution of biogenic volatile organic compounds to new particle formation in the Jülich plant atmosphere chamber

P. Roldin, L. Liao, D. Mogensen, M. Dal Maso, A. Rusanen, V.-M. Kerminen, T. F. Mentel, J. Wildt, E. Kleist, A. Kiendler-Scharr, R. Tillmann, M. Ehn, M. Kulmala, and M. Boy

Related authors

Formation and temperature dependence of highly oxygenated organic molecules (HOMs) from Δ3-carene ozonolysis
Yuanyuan Luo, Ditte Thomsen, Emil Mark Iversen, Pontus Roldin, Jane Tygesen Skønager, Linjie Li, Michael Priestley, Henrik B. Pedersen, Mattias Hallquist, Merete Bilde, Marianne Glasius, and Mikael Ehn
Atmos. Chem. Phys., 24, 9459–9473, https://doi.org/10.5194/acp-24-9459-2024,https://doi.org/10.5194/acp-24-9459-2024, 2024
Short summary
Measurement report: Black carbon properties and concentrations in southern Sweden urban and rural air – the importance of long-range transport
Erik Ahlberg, Stina Ausmeel, Lovisa Nilsson, Mårten Spanne, Julija Pauraite, Jacob Klenø Nøjgaard, Michele Bertò, Henrik Skov, Pontus Roldin, Adam Kristensson, Erik Swietlicki, and Axel Eriksson
Atmos. Chem. Phys., 23, 3051–3064, https://doi.org/10.5194/acp-23-3051-2023,https://doi.org/10.5194/acp-23-3051-2023, 2023
Short summary
Atmospherically Relevant Chemistry and Aerosol box model – ARCA box (version 1.2)
Petri Clusius, Carlton Xavier, Lukas Pichelstorfer, Putian Zhou, Tinja Olenius, Pontus Roldin, and Michael Boy
Geosci. Model Dev., 15, 7257–7286, https://doi.org/10.5194/gmd-15-7257-2022,https://doi.org/10.5194/gmd-15-7257-2022, 2022
Short summary
Secondary aerosol formation in marine Arctic environments: a model measurement comparison at Ny-Ålesund
Carlton Xavier, Metin Baykara, Robin Wollesen de Jonge, Barbara Altstädter, Petri Clusius, Ville Vakkari, Roseline Thakur, Lisa Beck, Silvia Becagli, Mirko Severi, Rita Traversi, Radovan Krejci, Peter Tunved, Mauro Mazzola, Birgit Wehner, Mikko Sipilä, Markku Kulmala, Michael Boy, and Pontus Roldin
Atmos. Chem. Phys., 22, 10023–10043, https://doi.org/10.5194/acp-22-10023-2022,https://doi.org/10.5194/acp-22-10023-2022, 2022
Short summary
Secondary aerosol formation from dimethyl sulfide – improved mechanistic understanding based on smog chamber experiments and modelling
Robin Wollesen de Jonge, Jonas Elm, Bernadette Rosati, Sigurd Christiansen, Noora Hyttinen, Dana Lüdemann, Merete Bilde, and Pontus Roldin
Atmos. Chem. Phys., 21, 9955–9976, https://doi.org/10.5194/acp-21-9955-2021,https://doi.org/10.5194/acp-21-9955-2021, 2021
Short summary

Related subject area

Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Regional variability of aerosol impacts on clouds and radiation in global kilometer-scale simulations
Ross J. Herbert, Andrew I. L. Williams, Philipp Weiss, Duncan Watson-Parris, Elisabeth Dingley, Daniel Klocke, and Philip Stier
Atmos. Chem. Phys., 25, 7789–7814, https://doi.org/10.5194/acp-25-7789-2025,https://doi.org/10.5194/acp-25-7789-2025, 2025
Short summary
A novel method to quantify the uncertainty contribution of aerosol–radiation interaction factors
Bishuo He and Chunsheng Zhao
Atmos. Chem. Phys., 25, 7765–7776, https://doi.org/10.5194/acp-25-7765-2025,https://doi.org/10.5194/acp-25-7765-2025, 2025
Short summary
Exploring the aerosol activation properties in coastal shallow convection using cloud- and particle-resolving models
Ge Yu, Yueya Wang, Zhe Wang, and Xiaoming Shi
Atmos. Chem. Phys., 25, 7527–7542, https://doi.org/10.5194/acp-25-7527-2025,https://doi.org/10.5194/acp-25-7527-2025, 2025
Short summary
Machine-learning-assisted inference of the particle charge fraction and the ion-induced nucleation rates during new particle formation events
Pan Wang, Yue Zhao, Jiandong Wang, Veli-Matti Kerminen, Jingkun Jiang, and Chenxi Li
Atmos. Chem. Phys., 25, 7431–7446, https://doi.org/10.5194/acp-25-7431-2025,https://doi.org/10.5194/acp-25-7431-2025, 2025
Short summary
Modeling CMAQ dry deposition treatment over the western Pacific: a distinct characteristic of mineral dust and anthropogenic aerosols
Steven Soon-Kai Kong, Joshua S. Fu, Neng-Huei Lin, Guey-Rong Sheu, and Wei-Syun Huang
Atmos. Chem. Phys., 25, 7245–7268, https://doi.org/10.5194/acp-25-7245-2025,https://doi.org/10.5194/acp-25-7245-2025, 2025
Short summary

Cited articles

Almeida, J., Schobesberger, S., Kürten, A., Ortega, I. K., Kupiainen-Määttä, O., Praplan, A. P., Adamov, A., Amorim, A., Bianchi, F., and Breitenlechner, M.: Molecular understanding of sulphuric acid-amine particle nucleation in the atmosphere, Nature, 502, 359–363, 2013.
Berndt, T., Stratmann, F., Sipilä, M., Vanhanen, J., Petäjä, T., Mikkilä, J., Grüner, A., Spindler, G., Lee Mauldin III, R., Curtius, J., Kulmala, M., and Heintzenberg, J.: Laboratory study on new particle formation from the reaction \chemOH + SO_2: influence of experimental conditions, H2O vapour, NH3 and the amine tert-butylamine on the overall process, Atmos. Chem. Phys., 10, 7101–7116, https://doi.org/10.5194/acp-10-7101-2010, 2010.
Bonn, B. and Moortgat, G. K.: Sesquiterpene ozonolysis: origin of atmospheric new particle formation from biogenic hydrocarbons, Geophys. Res. Lett., 30, 1585, https://doi.org/10.1029/2003GL017000, 2003.
Boy, M., Rannik, Ü., Lehtinen, K. E. J., Tarvainen, V., Hakola, H., and Kulmala, M.: Nucleation events in the continental boundary layer: long-term statistical analyses of aerosol relevant characteristics, J. Geophys. Res., 108, 4667, https://doi.org/10.1029/2003JD003838, 2003.
Boy, M., Mogensen, D., Smolander, S., Zhou, L., Nieminen, T., Paasonen, P., Plass-Dülmer, C., Sipilä, M., Petäjä, T., Mauldin, L., Berresheim, H., and Kulmala, M.: Oxidation of SO2 by stabilized Criegee intermediate (sCI) radicals as a crucial source for atmospheric sulfuric acid concentrations, Atmos. Chem. Phys., 13, 3865–3879, https://doi.org/10.5194/acp-13-3865-2013, 2013.
Short summary
We used the ADCHAM model to study new particle formation events in the JPAC chamber. The model results show that the new particles may be formed by a kinetic type of nucleation involving both sulphuric acid and organic compounds formed from OH oxidation of volatile organic compounds (VOCs). The observed particle growth may either be controlled by the condensation of semi- and low-volatililty organic compounds or by the formation of low-volatility compounds (oligomers) at the particle surface.
Share
Altmetrics
Final-revised paper
Preprint