Articles | Volume 15, issue 18
https://doi.org/10.5194/acp-15-10777-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Special issue:
https://doi.org/10.5194/acp-15-10777-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Modelling the contribution of biogenic volatile organic compounds to new particle formation in the Jülich plant atmosphere chamber
Division of Nuclear Physics, Lund University, P.O. Box 118, 221 00 Lund, Sweden
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
L. Liao
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
D. Mogensen
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
M. Dal Maso
Department of Physics, Tampere University of Technology, P.O. Box 692, 33101 Tampere, Finland
A. Rusanen
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
V.-M. Kerminen
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
T. F. Mentel
Institute for Energy- and Climate Research (IEK-8), Forschungszentrum Jülich, 52425 Jülich, Germany
J. Wildt
Institute of Biogeosciences (IBG-2), Forschungszentrum Jülich, 52425 Jülich, Germany
E. Kleist
Institute of Biogeosciences (IBG-2), Forschungszentrum Jülich, 52425 Jülich, Germany
A. Kiendler-Scharr
Institute for Energy- and Climate Research (IEK-8), Forschungszentrum Jülich, 52425 Jülich, Germany
R. Tillmann
Institute for Energy- and Climate Research (IEK-8), Forschungszentrum Jülich, 52425 Jülich, Germany
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
M. Kulmala
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
M. Boy
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
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Short summary
We used the ADCHAM model to study new particle formation events in the JPAC chamber. The model results show that the new particles may be formed by a kinetic type of nucleation involving both sulphuric acid and organic compounds formed from OH oxidation of volatile organic compounds (VOCs). The observed particle growth may either be controlled by the condensation of semi- and low-volatililty organic compounds or by the formation of low-volatility compounds (oligomers) at the particle surface.
We used the ADCHAM model to study new particle formation events in the JPAC chamber. The model...
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