Articles | Volume 15, issue 18
https://doi.org/10.5194/acp-15-10777-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Special issue:
https://doi.org/10.5194/acp-15-10777-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
28 Sep 2015
Research article |
| 28 Sep 2015
Modelling the contribution of biogenic volatile organic compounds to new particle formation in the Jülich plant atmosphere chamber
Division of Nuclear Physics, Lund University, P.O. Box 118, 221 00 Lund, Sweden
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
L. Liao
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
D. Mogensen
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
M. Dal Maso
Department of Physics, Tampere University of Technology, P.O. Box 692, 33101 Tampere, Finland
A. Rusanen
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
V.-M. Kerminen
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
T. F. Mentel
Institute for Energy- and Climate Research (IEK-8), Forschungszentrum Jülich, 52425 Jülich, Germany
J. Wildt
Institute of Biogeosciences (IBG-2), Forschungszentrum Jülich, 52425 Jülich, Germany
E. Kleist
Institute of Biogeosciences (IBG-2), Forschungszentrum Jülich, 52425 Jülich, Germany
A. Kiendler-Scharr
Institute for Energy- and Climate Research (IEK-8), Forschungszentrum Jülich, 52425 Jülich, Germany
R. Tillmann
Institute for Energy- and Climate Research (IEK-8), Forschungszentrum Jülich, 52425 Jülich, Germany
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
M. Kulmala
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
M. Boy
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
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Cited
17 citations as recorded by crossref.
- Recent advances in understanding secondary organic aerosol: Implications for global climate forcing M. Shrivastava et al. 10.1002/2016RG000540
- The Silk Road agenda of the Pan-Eurasian Experiment (PEEX) program H. Lappalainen et al. 10.1080/20964471.2018.1437704
- PyCHAM (v2.1.1): a Python box model for simulating aerosol chambers S. O'Meara et al. 10.5194/gmd-14-675-2021
- Ambient measurements of monoterpenes near Cannabis cultivation facilities in Denver, Colorado C. Wang et al. 10.1016/j.atmosenv.2020.117510
- Modelling studies of HOMs and their contributions to new particle formation and growth: comparison of boreal forest in Finland and a polluted environment in China X. Qi et al. 10.5194/acp-18-11779-2018
- Large Discrepancy in the Formation of Secondary Organic Aerosols from Structurally Similar Monoterpenes D. Thomsen et al. 10.1021/acsearthspacechem.0c00332
- Molecular Chirality and Cloud Activation Potentials of Dimeric α-Pinene Oxidation Products A. Bellcross et al. 10.1021/jacs.1c07509
- Indoor simulations reveal differences among plant species in capturing particulate matter J. Chen et al. 10.1371/journal.pone.0177539
- Modeling the role of highly oxidized multifunctional organic molecules for the growth of new particles over the boreal forest region E. Öström et al. 10.5194/acp-17-8887-2017
- A chamber study of the influence of boreal BVOC emissions and sulfuric acid on nanoparticle formation rates at ambient concentrations M. Dal Maso et al. 10.5194/acp-16-1955-2016
- Application of smog chambers in atmospheric process studies B. Chu et al. 10.1093/nsr/nwab103
- Evaporation of sulfate aerosols at low relative humidity G. Tsagkogeorgas et al. 10.5194/acp-17-8923-2017
- Interactions between the atmosphere, cryosphere, and ecosystems at northern high latitudes M. Boy et al. 10.5194/acp-19-2015-2019
- The role of highly oxygenated organic molecules in the Boreal aerosol-cloud-climate system P. Roldin et al. 10.1038/s41467-019-12338-8
- Atmospheric clusters to nanoparticles: Recent progress and challenges in closing the gap in chemical composition J. Smith et al. 10.1016/j.jaerosci.2020.105733
- Comparison of Geometrical Layouts for a Multi-Box Aerosol Model from a Single-Chamber Dispersion Study A. Jensen et al. 10.3390/environments5050052
- A chamber study of the influence of boreal BVOC emissions and sulphuric acid on nanoparticle formation rates at ambient concentrations M. Dal Maso et al. 10.5194/acpd-14-31319-2014
16 citations as recorded by crossref.
- Recent advances in understanding secondary organic aerosol: Implications for global climate forcing M. Shrivastava et al. 10.1002/2016RG000540
- The Silk Road agenda of the Pan-Eurasian Experiment (PEEX) program H. Lappalainen et al. 10.1080/20964471.2018.1437704
- PyCHAM (v2.1.1): a Python box model for simulating aerosol chambers S. O'Meara et al. 10.5194/gmd-14-675-2021
- Ambient measurements of monoterpenes near Cannabis cultivation facilities in Denver, Colorado C. Wang et al. 10.1016/j.atmosenv.2020.117510
- Modelling studies of HOMs and their contributions to new particle formation and growth: comparison of boreal forest in Finland and a polluted environment in China X. Qi et al. 10.5194/acp-18-11779-2018
- Large Discrepancy in the Formation of Secondary Organic Aerosols from Structurally Similar Monoterpenes D. Thomsen et al. 10.1021/acsearthspacechem.0c00332
- Molecular Chirality and Cloud Activation Potentials of Dimeric α-Pinene Oxidation Products A. Bellcross et al. 10.1021/jacs.1c07509
- Indoor simulations reveal differences among plant species in capturing particulate matter J. Chen et al. 10.1371/journal.pone.0177539
- Modeling the role of highly oxidized multifunctional organic molecules for the growth of new particles over the boreal forest region E. Öström et al. 10.5194/acp-17-8887-2017
- A chamber study of the influence of boreal BVOC emissions and sulfuric acid on nanoparticle formation rates at ambient concentrations M. Dal Maso et al. 10.5194/acp-16-1955-2016
- Application of smog chambers in atmospheric process studies B. Chu et al. 10.1093/nsr/nwab103
- Evaporation of sulfate aerosols at low relative humidity G. Tsagkogeorgas et al. 10.5194/acp-17-8923-2017
- Interactions between the atmosphere, cryosphere, and ecosystems at northern high latitudes M. Boy et al. 10.5194/acp-19-2015-2019
- The role of highly oxygenated organic molecules in the Boreal aerosol-cloud-climate system P. Roldin et al. 10.1038/s41467-019-12338-8
- Atmospheric clusters to nanoparticles: Recent progress and challenges in closing the gap in chemical composition J. Smith et al. 10.1016/j.jaerosci.2020.105733
- Comparison of Geometrical Layouts for a Multi-Box Aerosol Model from a Single-Chamber Dispersion Study A. Jensen et al. 10.3390/environments5050052
Saved (final revised paper)
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Latest update: 27 May 2023
Short summary
We used the ADCHAM model to study new particle formation events in the JPAC chamber. The model results show that the new particles may be formed by a kinetic type of nucleation involving both sulphuric acid and organic compounds formed from OH oxidation of volatile organic compounds (VOCs). The observed particle growth may either be controlled by the condensation of semi- and low-volatililty organic compounds or by the formation of low-volatility compounds (oligomers) at the particle surface.
We used the ADCHAM model to study new particle formation events in the JPAC chamber. The model...
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