Articles | Volume 14, issue 23
Atmos. Chem. Phys., 14, 12883–12895, 2014
Atmos. Chem. Phys., 14, 12883–12895, 2014

Research article 08 Dec 2014

Research article | 08 Dec 2014

Estimating regional fluxes of CO2 and CH4 using space-borne observations of XCH4: XCO2

A. Fraser et al.

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Subject: Gases | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
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Cited articles

Bey, I., Jacob, D. J., Yantosca, R. M., Logan, J. A., Field, B., Fiore, A. M., Li, Q., Liu, H., Mickley, L. J., and Schultz, M.: Global modeling of tropospheric chemistry with assimilated meteorology: Model description and evaluation, J. Geophys. Res., 106, 23073–23096, 2001a.
Bloom, A. A., Palmer, P. I., Fraser, A., and Reay, D. S.: Seasonal variability of tropical wetland CH4 emissions: the role of the methanogen-available carbon pool, Biogeosciences, 9, 2821–2830,, 2012.
Chevallier, F., Palmer, P. I., Feng, L., Boesch, H., O'Dell, C., W., and Bousquet, P.: Toward robust and consistent regional CO2 flux estimates from in situ and spaceborne measurements of atmospheric CO2, Geophys. Res. Lett., 41, 1065–1070,, 2014.
Cogan, A. J., Boesch, H., Parker, R. J., Feng, L., Palmer, P. I., Blavier, J.-F. L., Deutscher, N. M., Macatangay, R., Notholt, J., Roehl, C., Warneke, T., and Wunch, D.: Atmospheric carbon dioxide retrieved from the Greenhouse gases Observing SATellite (GOSAT): comparison with ground-based TCCON observations and GEOS-Chem model calculations, J. Geophys. Res., 117, D21301,, 2012.
Dlugokencky, E. J., Lang, P. M., Crotwell, A., Masarie, K. A., and Crotwell, M.: Atmospheric methane dry air mole fractions from the NOAA ESRL carbon cycle cooperative global air sampling network, 1983–2012, Version: 2013-08-28, available at: (last access: September 2013), 2013.
Short summary
Satellite measurements of CO2 and CH4 can be subject to regional systematic errors that can consequently compromise their ability to infer robust flux estimates of these two gases. We develop a method to use retrieved ratios of CH4 and CO2 that are less affected by systematic error. We show that additional in situ data are needed to anchor these observed ratios so they can simultaneously infer fluxes of CO2 and CH4. We argue the ratio data will provide a more faithful description of true fluxes.
Final-revised paper