- About
- Editorial board
- Articles
- Special issues
- Highlight articles
- Manuscript tracking
- Subscribe to alerts
- Peer review
- For authors
- For reviewers
- EGU publications
Journal cover
Journal topic
Atmospheric Chemistry and Physics
An interactive open-access journal of the European Geosciences Union
Journal topic
- About
- Editorial board
- Articles
- Special issues
- Highlight articles
- Manuscript tracking
- Subscribe to alerts
- Peer review
- For authors
- For reviewers
- EGU publications
Journal metrics
IF5.414
IF 5-year
5.958
5.958
CiteScore
9.7
9.7
SNIP1.517
IPP5.61
SJR2.601
Scimago H
index191
index191
h5-index89
Abstracted/indexed
Abstracted/indexed
Volume 17, issue 12
Atmos. Chem. Phys., 17, 7703–7719, 2017
https://doi.org/10.5194/acp-17-7703-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-7703-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 17, 7703–7719, 2017
https://doi.org/10.5194/acp-17-7703-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-7703-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
Research article 26 Jun 2017
Research article | 26 Jun 2017
Effects of mixing on resolved and unresolved scales on stratospheric age of air
Simone Dietmüller et al.
Related authors
Petr Šácha, Roland Eichinger, Hella Garny, Petr Pišoft, Simone Dietmüller, Laura de la Torre, David A. Plummer, Patrick Jöckel, Olaf Morgenstern, Guang Zeng, Neal Butchart, and Juan A. Añel
Atmos. Chem. Phys., 19, 7627–7647, https://doi.org/10.5194/acp-19-7627-2019, https://doi.org/10.5194/acp-19-7627-2019, 2019
Short summary
Short summary
Climate models robustly project a Brewer–Dobson circulation (BDC) acceleration in the course of climate change. Analyzing mean age of stratospheric air (AoA) from a subset of climate projection simulations, we find a remarkable agreement in simulating the largest AoA trends in the extratropical stratosphere. This is shown to be related with the upward shift of the circulation, resulting in a so-called stratospheric shrinkage, which could be one of the so-far-omitted BDC acceleration drivers.
Roland Eichinger, Simone Dietmüller, Hella Garny, Petr Šácha, Thomas Birner, Harald Bönisch, Giovanni Pitari, Daniele Visioni, Andrea Stenke, Eugene Rozanov, Laura Revell, David A. Plummer, Patrick Jöckel, Luke Oman, Makoto Deushi, Douglas E. Kinnison, Rolando Garcia, Olaf Morgenstern, Guang Zeng, Kane Adam Stone, and Robyn Schofield
Atmos. Chem. Phys., 19, 921–940, https://doi.org/10.5194/acp-19-921-2019, https://doi.org/10.5194/acp-19-921-2019, 2019
Short summary
Short summary
To shed more light upon the changes in stratospheric circulation in the 21st century, climate projection simulations of 10 state-of-the-art global climate models, spanning from 1960 to 2100, are analyzed. The study shows that in addition to changes in transport, mixing also plays an important role in stratospheric circulation and that the properties of mixing vary over time. Furthermore, the influence of mixing is quantified and a dynamical framework is provided to understand the changes.
Simone Dietmüller, Roland Eichinger, Hella Garny, Thomas Birner, Harald Boenisch, Giovanni Pitari, Eva Mancini, Daniele Visioni, Andrea Stenke, Laura Revell, Eugene Rozanov, David A. Plummer, John Scinocca, Patrick Jöckel, Luke Oman, Makoto Deushi, Shibata Kiyotaka, Douglas E. Kinnison, Rolando Garcia, Olaf Morgenstern, Guang Zeng, Kane Adam Stone, and Robyn Schofield
Atmos. Chem. Phys., 18, 6699–6720, https://doi.org/10.5194/acp-18-6699-2018, https://doi.org/10.5194/acp-18-6699-2018, 2018
Simone Dietmüller, Patrick Jöckel, Holger Tost, Markus Kunze, Catrin Gellhorn, Sabine Brinkop, Christine Frömming, Michael Ponater, Benedikt Steil, Axel Lauer, and Johannes Hendricks
Geosci. Model Dev., 9, 2209–2222, https://doi.org/10.5194/gmd-9-2209-2016, https://doi.org/10.5194/gmd-9-2209-2016, 2016
Short summary
Short summary
Four new radiation related submodels (RAD, AEROPT, CLOUDOPT, and ORBIT) are available within the MESSy framework now. They are largely based on the original radiation scheme of ECHAM5. RAD simulates radiative transfer, AEROPT calculates aerosol optical properties, CLOUDOPT calculates cloud optical properties, and ORBIT is responsible for Earth orbit calculations. Multiple diagnostic calls of the radiation routine are possible, so radiative forcing can be calculated during the model simulation.
Chaim Israel Garfinkel, Ohad Harari, Shlomi Ziskin, Jian Rao, Olaf Morgenstern, Guang Zeng, Simone Tilmes, Doug Kinnison, Fiona M. O'Connor, Neal Butchart, Makoto Deushi, Patrick Jöckel, and Andrea Pozzer
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-801, https://doi.org/10.5194/acp-2020-801, 2020
Preprint under review for ACP
Short summary
Short summary
Water vapor is the dominant greenhouse gas in the atmosphere, and the dominant mode of variability in the ocean-atmosphere system is El Nino. The connection between El Nino and water vapor above ~17km is unclear, with single model studies reaching a range of conclusions. This study examines this connection in 12 different models. While there are substantial differences among the models, all models appear to capture the fundamental physical processes correctly.
Arseniy Karagodin-Doyennel, Eugene Rozanov, Ales Kuchar, William Ball, Pavle Arsenovic, Ellis Remsberg, Patrick Jöckel, Markus Kunze, David A. Plummer, Andrea Stenke, Daniel Marsh, Doug Kinnison, and Thomas Peter
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-793, https://doi.org/10.5194/acp-2020-793, 2020
Preprint under review for ACP
Short summary
Short summary
1) The solar signal in the mesospheric H2O and CO was extracted from the CCMI-1 model simulations and satellite observations using MLR analysis.
2) MLR analysis shows a pronounced and statistically robust solar signal in both H2O and CO.
3) The model results show a general agreement with observations reproducing a negative/positive solar signal in H2O/CO.
4) The pattern of the solar signal rather varies among the considered models, reflecting some differences in the model set-up.
Marc von Hobe, Felix Ploeger, Paul Konopka, Corinna Kloss, Alexey Ulanowski, Vladimir Yushkov, Fabrizio Ravegnani, C. Michael Volk, Laura L. Pan, Shawn B. Honomichl, Simone Tilmes, Douglas E. Kinnison, Rolando R. Garcia, and Jonathon S. Wright
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-891, https://doi.org/10.5194/acp-2020-891, 2020
Preprint under review for ACP
Short summary
Short summary
The Asian summer monsoon (ASM) is known to foster transport of polluted tropospheric air into the stratosphere. To test and amend our picture of ASM vertical transport, we analyze distributions of airborne trace gas observations up to 20 km altitude near the main ASM vertical conduit south of the Himalayas. We also show that a new high resolution version of the global chemistry climate model WACCM is able to reproduce the observations well.
Matt Amos, Paul J. Young, J. Scott Hosking, Jean-François Lamarque, N. Luke Abraham, Hideharu Akiyoshi, Alexander T. Archibald, Slimane Bekki, Makoto Deushi, Patrick Jöckel, Douglas Kinnison, Ole Kirner, Markus Kunze, Marion Marchand, David A. Plummer, David Saint-Martin, Kengo Sudo, Simone Tilmes, and Yousuke Yamashita
Atmos. Chem. Phys., 20, 9961–9977, https://doi.org/10.5194/acp-20-9961-2020, https://doi.org/10.5194/acp-20-9961-2020, 2020
Short summary
Short summary
We present an updated projection of Antarctic ozone hole recovery using an ensemble of chemistry–climate models. To do so, we employ a method, more advanced and skilful than the current multi-model mean standard, which is applicable to other ensemble analyses. It calculates the performance and similarity of the models, which we then use to weight the model. Calculating model similarity allows us to account for models which are constructed from similar components.
Johannes C. Laube, Emma C. Leedham Elvidge, Karina E. Adcock, Bianca Baier, Carl A. M. Brenninkmeijer, Huilin Chen, Elise S. Droste, Jens-Uwe Grooß, Pauli Heikkinen, Andrew J. Hind, Rigel Kivi, Alexander Lojko, Stephen A. Montzka, David E. Oram, Steve Randall, Thomas Röckmann, William T. Sturges, Colm Sweeney, Max Thomas, Elinor Tuffnell, and Felix Ploeger
Atmos. Chem. Phys., 20, 9771–9782, https://doi.org/10.5194/acp-20-9771-2020, https://doi.org/10.5194/acp-20-9771-2020, 2020
Short summary
Short summary
We demonstrate that AirCore technology, which is based on small low-cost balloons, can provide access to trace gas measurements such as CFCs at ultra-low abundances. This is a new way to quantify ozone-depleting, and related, substances in the stratosphere, which is largely inaccessible to aircraft. We show two potential uses: (a) tracking the stratospheric circulation, which is predicted to change, and (b) assessing three common meteorological reanalyses driving a global stratospheric model.
Christine Frömming, Volker Grewe, Sabine Brinkop, Patrick Jöckel, Amund S. Haslerud, Simon Rosanka, Jesper van Manen, and Sigrun Matthes
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-529, https://doi.org/10.5194/acp-2020-529, 2020
Preprint under review for ACP
Short summary
Short summary
We investigate the influence of different weather situations on non-CO2 aviation climate impact to identify systematic weather related sensitivities. If aircraft avoid most sensitive areas, climate impact might be reduced. Enhanced significance is found for emission in relation to high pressure systems, jet stream, polar night, tropopause altitude. The results represent a comprehensive dataset for studies aiming at weather dependent flight trajectory optimization reducing total climate impact.
Corinna Kloss, Gwenaël Berthet, Pasquale Sellitto, Felix Ploeger, Ghassan Taha, Mariam Tidiga, Maxim Eremenko, Adriana Bossolasco, Fabrice Jégou, Jean-Baptiste Renard, and Bernard Legras
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-701, https://doi.org/10.5194/acp-2020-701, 2020
Preprint under review for ACP
Short summary
Short summary
The year 2019 was particularly rich for the stratospheric aerosol layer due to two volcanic eruptions (at Raikoke and Ulawun) and wild fire events. With satellite observations and models, we describe the exceptionally complex situation following the Raikoke eruption. The respective plume overwhelmed the northern hemispheric stratosphere in terms of aerosol load and climate impact for the past decade.
Marius Hauck, Harald Bönisch, Peter Hoor, Timo Keber, Felix Ploeger, Tanja J. Schuck, and Andreas Engel
Atmos. Chem. Phys., 20, 8763–8785, https://doi.org/10.5194/acp-20-8763-2020, https://doi.org/10.5194/acp-20-8763-2020, 2020
Short summary
Short summary
This study features an extended inversion method that includes transport across the extratropical tropopause to derive age spectra in the lowermost stratosphere from in situ trace gas measurements. The refined method is validated in a model setup and applied to data gained with the HALO research aircraft. Results are congruent with the findings of previous studies so that the method provides a promising toolset for the analysis of stratospheric dynamics based on observations in the future.
Frauke Fritsch, Hella Garny, Andreas Engel, Harald Bönisch, and Roland Eichinger
Atmos. Chem. Phys., 20, 8709–8725, https://doi.org/10.5194/acp-20-8709-2020, https://doi.org/10.5194/acp-20-8709-2020, 2020
Short summary
Short summary
We test two methods to derive age of air as a diagnostic of the Brewer–Dobson circulation from non-linear increasing trace gases such as SF6 using a chemistry-climate model and observations. Both the model and the observations show systematic variation of the age of air trend dependent on the chosen assumptions that are required when deriving age of air from measurements. This provides insight into the differences in age of air trends of observations and models.
Patrick E. Sheese, Kaley A. Walker, Chris D. Boone, Doug A. Degenstein, Felicia Kolonjari, David Plummer, Douglas E. Kinnison, Patrick Jöckel, and Thomas von Clarmann
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-207, https://doi.org/10.5194/amt-2020-207, 2020
Preprint under review for AMT
Edward J. Charlesworth, Ann-Kristin Dugstad, Frauke Fritsch, Patrick Jöckel, and Felix Plöger
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-458, https://doi.org/10.5194/acp-2020-458, 2020
Preprint under review for ACP
Short summary
Short summary
Modeling the stratosphere requires models with good representations of chemical transport. To do this, nearly all models divide the atmosphere into boxes. This creates some unwanted problems. However, the only other option is to divide the atmosphere into balloons, and this method is very complicated. Here, we use a model which uses this balloon-like method to estimate the impacts of this method on chemical transport. We find significant differences in sensitive regions of the stratosphere.
Mariano Mertens, Astrid Kerkweg, Volker Grewe, Patrick Jöckel, and Robert Sausen
Atmos. Chem. Phys., 20, 7843–7873, https://doi.org/10.5194/acp-20-7843-2020, https://doi.org/10.5194/acp-20-7843-2020, 2020
Short summary
Short summary
We investigate the contribution of land transport emissions to ozone and ozone precursors in Europe and Germany. Our results show that land transport emissions are one of the most important contributors to reactive nitrogen in Europe. The contribution to ozone is in the range of 8 % to 16 % and varies strongly for different seasons. The hots-pots with the largest ozone concentrations are the Po Valley, while the largest concentration to reactive nitrogen is located mainly in western Europe.
Daniele Visioni, Giovanni Pitari, Vincenzo Rizi, Marco Iarlori, Irene Cionni, Ilaria Quaglia, Hideharu Akiyoshi, Slimane Bekki, Neal Butchart, Martin Chipperfield, Makoto Deushi, Sandip S. Dhomse, Rolando Garcia, Patrick Joeckel, Douglas Kinnison, Jean-François Lamarque, Marion Marchand, Martine Michou, Olaf Morgenstern, Tatsuya Nagashima, Fiona M. O'Connor, Luke D. Oman, David Plummer, Eugene Rozanov, David Saint-Martin, Robyn Schofield, John Scinocca, Andrea Stenke, Kane Stone, Kengo Sudo, Taichu Y. Tanaka, Simone Tilmes, Holger Tost, Yousuke Yamashita, and Guang Zeng
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-525, https://doi.org/10.5194/acp-2020-525, 2020
Preprint under review for ACP
Short summary
Short summary
In this work we analyse the trend in ozone profiles taken at L'Aquila (Italy, 42.4° N) for seventeen years, between 2000 and 2016 and compare them against already available measured ozone trends. We try to understand and explain the observed trends at various heights in light of the simulations from seventeen different model, highlighting the contribution of changes in circulation and chemical ozone loss during this time period.
Laura Stecher, Franziska Winterstein, Martin Dameris, Patrick Jöckel, Michael Ponater, and Markus Kunze
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-519, https://doi.org/10.5194/acp-2020-519, 2020
Preprint under review for ACP
Short summary
Short summary
This study investigates the impact of strongly increased atmospheric methane mixing ratios on the Earth's climate. An interactive model system including atmospheric dynamics, chemistry, and a mixed layer ocean model is used to analyse the effect of doubled and fivefold methane mixing ratios. We assess feedbacks on atmospheric chemistry and changes in the stratospheric circulation, focusing on the impact of tropospheric warming, and their relevance for the model's climate sensitivity.
Franziska Winterstein and Patrick Jöckel
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-137, https://doi.org/10.5194/gmd-2020-137, 2020
Preprint under review for GMD
Short summary
Short summary
Atmospheric methane is currently a hot topic in climate research, among others due to its chemically active nature. We introduce a simplified approach to simulate methane chemistry in climate models to enable extensive sensitivity studies by reducing computational cost, but including the crucial feedback of methane on stratospheric water vapor. We further provide options to simulate isotopes in methane and to generate output for an inverse optimization technique.
Marta Abalos, Clara Orbe, Douglas E. Kinnison, David Plummer, Luke D. Oman, Patrick Jöckel, Olaf Morgenstern, Rolando R. Garcia, Guang Zeng, Kane A. Stone, and Martin Dameris
Atmos. Chem. Phys., 20, 6883–6901, https://doi.org/10.5194/acp-20-6883-2020, https://doi.org/10.5194/acp-20-6883-2020, 2020
Short summary
Short summary
A set of state-of-the art chemistry–climate models is used to examine future changes in downward transport from the stratosphere, a key contributor to tropospheric ozone. The acceleration of the stratospheric circulation results in increased stratosphere-to-troposphere transport. In the subtropics, downward advection into the troposphere is enhanced due to climate change. At higher latitudes, the ozone reservoir above the tropopause is enlarged due to the stronger circulation and ozone recovery.
Alina Fiehn, Julian Kostinek, Maximilian Eckl, Theresa Klausner, Michał Gałkowski, Jinxuan Chen, Christoph Gerbig, Thomas Röckmann, Hossein Maazallahi, Martina Schmidt, Piotr Korbeń, Jarosław Nȩcki, Pawel Jagoda, Norman Wildmann, Christian Mallaun, Rostyslav Bun, Anna-Leah Nickl, Patrick Jöckel, Andreas Fix, and Anke Roiger
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-282, https://doi.org/10.5194/acp-2020-282, 2020
Revised manuscript accepted for ACP
Short summary
Short summary
A severe reduction of greenhouse gas emissions is necessary to fulfill the Paris Agreement. We use aircraft- and ground-based in situ observations of trace gases and wind speed from two flights over the Upper Silesian Coal Basin, Poland, for independent emission estimation. The derived methane emission estimates are within the range of emission inventories, carbon dioxide estimates are in the lower range and carbon monoxide emission estimates are slightly higher than emission inventory values.
Peter H. Zimmermann, Carl A. M. Brenninkmeijer, Andrea Pozzer, Patrick Jöckel, Franziska Winterstein, Andreas Zahn, Sander Houweling, and Jos Lelieveld
Atmos. Chem. Phys., 20, 5787–5809, https://doi.org/10.5194/acp-20-5787-2020, https://doi.org/10.5194/acp-20-5787-2020, 2020
Short summary
Short summary
The atmospheric abundance of the greenhouse gas methane is determined by interacting emission sources and sinks in a dynamic global environment. In this study, its global budget from 1997 to 2016 is simulated with a general circulation model using emission estimates of 11 source categories. The model results are evaluated against 17 ground station and 320 intercontinental flight observation series. Deviations are used to re-scale the emission quantities with the aim of matching observations.
Yuanhong Zhao, Marielle Saunois, Philippe Bousquet, Xin Lin, Antoine Berchet, Michaela I. Hegglin, Josep G. Canadell, Robert B. Jackson, Makoto Deushi, Patrick Jöckel, Douglas Kinnison, Ole Kirner, Sarah Strode, Simone Tilmes, Edward J. Dlugokencky, and Bo Zheng
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-308, https://doi.org/10.5194/acp-2020-308, 2020
Revised manuscript accepted for ACP
Short summary
Short summary
Decadal trends and variations in the OH are critical for understanding the atmospheric CH4 evolution. We quantify the impacts of OH trends and variations on the CH4 budget by conducting CH4 inversions on decadal-scale with an ensemble of OH fields. We find the negative OH anomalies due to enhanced fires can reduce the optimized CH4 emissions by up to 10 Tg yr−1 during El Niño years, and the positive OH trend from 1986 to 2010 results in ~ 23 Tg yr−1 additional increase in optimized CH4 emissions.
Anna-Leah Nickl, Mariano Mertens, Anke Roiger, Andreas Fix, Axel Amediek, Alina Fiehn, Christoph Gerbig, Michal Galkowski, Astrid Kerkweg, Theresa Klausner, Maximilian Eckl, and Patrick Jöckel
Geosci. Model Dev., 13, 1925–1943, https://doi.org/10.5194/gmd-13-1925-2020, https://doi.org/10.5194/gmd-13-1925-2020, 2020
Short summary
Short summary
Based on the global and regional chemistry–climate model system MECO(n), we implemented a forecast system to support the planning of measurement campaign research flights with chemical weather forecasts. We applied this system for the first time to provide 6 d forecasts in support of the CoMet 1.0
campaign targeting methane emitted from coal mining ventilation shafts in the Upper Silesian Coal Basin in Poland. We describe the new forecast system and evaluate its forecast skill.
Dan Li, Bärbel Vogel, Rolf Müller, Jianchun Bian, Gebhard Günther, Felix Ploeger, Qian Li, Jinqiang Zhang, Zhixuan Bai, Holger Vömel, and Martin Riese
Atmos. Chem. Phys., 20, 4133–4152, https://doi.org/10.5194/acp-20-4133-2020, https://doi.org/10.5194/acp-20-4133-2020, 2020
Short summary
Short summary
Low ozone and low water vapour signatures in the UTLS were investigated using balloon-borne measurements and trajectory calculations. The results show that deep convection in tropical cyclones over the western Pacific transports boundary air parcels with low ozone into the tropopause region. Subsequently, these air parcels are dehydrated when passing the lowest temperature region (< 190 K) during quasi-horizontal advection.
Timo Keber, Harald Bönisch, Carl Hartick, Marius Hauck, Fides Lefrancois, Florian Obersteiner, Akima Ringsdorf, Nils Schohl, Tanja Schuck, Ryan Hossaini, Phoebe Graf, Patrick Jöckel, and Andreas Engel
Atmos. Chem. Phys., 20, 4105–4132, https://doi.org/10.5194/acp-20-4105-2020, https://doi.org/10.5194/acp-20-4105-2020, 2020
Short summary
Short summary
In this paper we summarize observations of short-lived halocarbons in the tropopause region. We show that, especially during winter, the levels of short-lived bromine gases at the extratropical tropopause are higher than at the tropical tropopause. We discuss the impact of the distributions on stratospheric bromine levels and compare our observations to two models with four different emission scenarios.
Clara Orbe, David A. Plummer, Darryn W. Waugh, Huang Yang, Patrick Jöckel, Douglas E. Kinnison, Beatrice Josse, Virginie Marecal, Makoto Deushi, Nathan Luke Abraham, Alexander T. Archibald, Martyn P. Chipperfield, Sandip Dhomse, Wuhu Feng, and Slimane Bekki
Atmos. Chem. Phys., 20, 3809–3840, https://doi.org/10.5194/acp-20-3809-2020, https://doi.org/10.5194/acp-20-3809-2020, 2020
Short summary
Short summary
Atmospheric composition is strongly influenced by global-scale winds that are not always properly simulated in computer models. A common approach to correct for this bias is to relax or
nudgeto the observed winds. Here we systematically evaluate how well this technique performs across a large suite of chemistry–climate models in terms of its ability to reproduce key aspects of both the tropospheric and stratospheric circulations.
Markus Kilian, Sabine Brinkop, and Patrick Jöckel
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-147, https://doi.org/10.5194/acp-2020-147, 2020
Revised manuscript accepted for ACP
Short summary
Short summary
After the volcanic eruption of Mt. Pinatubo in 1991, ozone is decreased in the tropics and increased in the mid-latitudes and polar regions for one year. The change in the ozone column is solely a result of the volcanic heating, followed by an ozone decrease in the higher latitudes. This is caused by the volcanic aerosol, which changes the heterogeneous chemistry and thus the catalytic ozone loss cycles. Vertical transport of water vapour is enhanced by volcanic heating and increases methane.
Julie M. Nicely, Bryan N. Duncan, Thomas F. Hanisco, Glenn M. Wolfe, Ross J. Salawitch, Makoto Deushi, Amund S. Haslerud, Patrick Jöckel, Béatrice Josse, Douglas E. Kinnison, Andrew Klekociuk, Michael E. Manyin, Virginie Marécal, Olaf Morgenstern, Lee T. Murray, Gunnar Myhre, Luke D. Oman, Giovanni Pitari, Andrea Pozzer, Ilaria Quaglia, Laura E. Revell, Eugene Rozanov, Andrea Stenke, Kane Stone, Susan Strahan, Simone Tilmes, Holger Tost, Daniel M. Westervelt, and Guang Zeng
Atmos. Chem. Phys., 20, 1341–1361, https://doi.org/10.5194/acp-20-1341-2020, https://doi.org/10.5194/acp-20-1341-2020, 2020
Short summary
Short summary
Differences in methane lifetime among global models are large and poorly understood. We use a neural network method and simulations from the Chemistry Climate Model Initiative to quantify the factors influencing methane lifetime spread among models and variations over time. UV photolysis, tropospheric ozone, and nitrogen oxides drive large model differences, while the same factors plus specific humidity contribute to a decreasing trend in methane lifetime between 1980 and 2015.
Mariano Mertens, Astrid Kerkweg, Volker Grewe, Patrick Jöckel, and Robert Sausen
Geosci. Model Dev., 13, 363–383, https://doi.org/10.5194/gmd-13-363-2020, https://doi.org/10.5194/gmd-13-363-2020, 2020
Short summary
Short summary
This study investigates if ozone source apportionment results using a tagged tracer approach depend on the resolutions of the applied model and/or emission inventory. For this we apply a global to regional atmospheric chemistry model, which allows us to compare the results on global and regional scales. Our results show that differences on the continental scale (e.g. Europe) are rather small (10 %); on the regional scale, however, differences of up to 30 % were found.
Le Kuai, Kevin W. Bowman, Kazuyuki Miyazaki, Makoto Deushi, Laura Revell, Eugene Rozanov, Fabien Paulot, Sarah Strode, Andrew Conley, Jean-François Lamarque, Patrick Jöckel, David A. Plummer, Luke D. Oman, Helen Worden, Susan Kulawik, David Paynter, Andrea Stenke, and Markus Kunze
Atmos. Chem. Phys., 20, 281–301, https://doi.org/10.5194/acp-20-281-2020, https://doi.org/10.5194/acp-20-281-2020, 2020
Short summary
Short summary
The tropospheric ozone increase from pre-industrial to the present day leads to a radiative forcing. The top-of-atmosphere outgoing fluxes at the ozone band are controlled by ozone, water vapor, and temperature. We demonstrate a method to attribute the models’ flux biases to these key players using satellite-constrained instantaneous radiative kernels. The largest spread between models is found in the tropics, mainly driven by ozone and then water vapor.
Xiaolu Yan, Paul Konopka, Felix Ploeger, Aurélien Podglajen, Jonathon S. Wright, Rolf Müller, and Martin Riese
Atmos. Chem. Phys., 19, 15629–15649, https://doi.org/10.5194/acp-19-15629-2019, https://doi.org/10.5194/acp-19-15629-2019, 2019
Short summary
Short summary
The Asian and North American summer monsoons (ASM and NASM) have considerable influence on stratospheric chemistry and physics. More air mass is transported from the monsoon regions to the tropical stratosphere when the tracers are released clearly below the tropopause than when they are released close to the tropopause. Results for different altitudes of air origin reveal two transport pathways (monsoon and tropical) from the upper troposphere over the monsoon regions to the tropical pipe.
Hella Garny, Roland Walz, Matthias Nützel, and Thomas Birner
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2019-330, https://doi.org/10.5194/gmd-2019-330, 2019
Revised manuscript accepted for GMD
Short summary
Short summary
Numerical models of Earth's climate system have been gaining more and more complexity over the last decades. Therefore, it is important to establish simplified models to improve process understanding. In our study, we present and document the development of a new simplified model set-up within the framework of a complex climate model system that uses the same routines to calculate atmospheric dynamics as the complex model, but is simplified in the representation of clouds and radiation.
Hiroshi Yamashita, Feijia Yin, Volker Grewe, Patrick Jöckel, Sigrun Matthes, Bastian Kern, Katrin Dahlmann, and Christine Frömming
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2019-331, https://doi.org/10.5194/gmd-2019-331, 2019
Revised manuscript accepted for GMD
Short summary
Short summary
This paper describes the updated submodel AirTraf 2.0 which simulates global air traffic in the ECHAM/MESSy Atmospheric Chemistry (EMAC) model. Nine aircraft routing options have been integrated, including contrail avoidance, minimum economic costs, and minimum climate impact. Example simulations reveal characteristics of various routing options on air traffic performances. The consistency of the AirTraf simulations is also verified with literature data.
Martin Dameris, Patrick Jöckel, and Matthias Nützel
Atmos. Chem. Phys., 19, 13759–13771, https://doi.org/10.5194/acp-19-13759-2019, https://doi.org/10.5194/acp-19-13759-2019, 2019
Short summary
Short summary
A chemistry–climate model (CCM) study is performed, investigating the consequences of a constant CFC-11 surface mixing ratio for stratospheric ozone in the future. The total column ozone is particularly affected in both polar regions in winter and spring. It turns out that the calculated ozone changes, especially in the upper stratosphere, are smaller than expected. In this attitudinal region the additional ozone depletion due to the catalysis by reactive chlorine is partly compensated for.
Yuanhong Zhao, Marielle Saunois, Philippe Bousquet, Xin Lin, Antoine Berchet, Michaela I. Hegglin, Josep G. Canadell, Robert B. Jackson, Didier A. Hauglustaine, Sophie Szopa, Ann R. Stavert, Nathan Luke Abraham, Alex T. Archibald, Slimane Bekki, Makoto Deushi, Patrick Jöckel, Béatrice Josse, Douglas Kinnison, Ole Kirner, Virginie Marécal, Fiona M. O'Connor, David A. Plummer, Laura E. Revell, Eugene Rozanov, Andrea Stenke, Sarah Strode, Simone Tilmes, Edward J. Dlugokencky, and Bo Zheng
Atmos. Chem. Phys., 19, 13701–13723, https://doi.org/10.5194/acp-19-13701-2019, https://doi.org/10.5194/acp-19-13701-2019, 2019
Short summary
Short summary
The role of hydroxyl radical changes in methane trends is debated, hindering our understanding of the methane cycle. This study quantifies how uncertainties in the hydroxyl radical may influence methane abundance in the atmosphere based on the inter-model comparison of hydroxyl radical fields and model simulations of CH4 abundance with different hydroxyl radical scenarios during 2000–2016. We show that hydroxyl radical changes could contribute up to 54 % of model-simulated methane biases.
Corinna Kloss, Gwenaël Berthet, Pasquale Sellitto, Felix Ploeger, Silvia Bucci, Sergey Khaykin, Fabrice Jégou, Ghassan Taha, Larry W. Thomason, Brice Barret, Eric Le Flochmoen, Marc von Hobe, Adriana Bossolasco, Nelson Bègue, and Bernard Legras
Atmos. Chem. Phys., 19, 13547–13567, https://doi.org/10.5194/acp-19-13547-2019, https://doi.org/10.5194/acp-19-13547-2019, 2019
Short summary
Short summary
With satellite measurements and transport models, we show that a plume resulting from strong Canadian fires in July/August 2017 was not only distributed throughout the northern/higher latitudes, but also reached the faraway tropics, aided by the circulation of Asian monsoon anticyclone. The regional climate impact in the wider Asian monsoon area in September exceeds the impact of the Asian tropopause aerosol layer by a factor of ~ 3 and compares to that of an advected moderate volcanic eruption.
Andreas Luther, Ralph Kleinschek, Leon Scheidweiler, Sara Defratyka, Mila Stanisavljevic, Andreas Forstmaier, Alexandru Dandocsi, Sebastian Wolff, Darko Dubravica, Norman Wildmann, Julian Kostinek, Patrick Jöckel, Anna-Leah Nickl, Theresa Klausner, Frank Hase, Matthias Frey, Jia Chen, Florian Dietrich, Jarosław Nȩcki, Justyna Swolkień, Andreas Fix, Anke Roiger, and André Butz
Atmos. Meas. Tech., 12, 5217–5230, https://doi.org/10.5194/amt-12-5217-2019, https://doi.org/10.5194/amt-12-5217-2019, 2019
Short summary
Short summary
Methane ventilated from hard coal mines in the Upper Silesian
Coal Basin in Poland is measured with a mobile Fourier transform spectrometer EM27/SUN. The instrument was mounted on a truck driving in stop-and-go patterns downwind of the methane sources. The emissions are estimated with the cross-sectional flux method. Calculated emissions are in broad agreement with the E-PRTR database. Wind-related errors on the methane estimates dominate the error budget and typically amount to 20 %.
Andreas Chrysanthou, Amanda C. Maycock, Martyn P. Chipperfield, Sandip Dhomse, Hella Garny, Douglas Kinnison, Hideharu Akiyoshi, Makoto Deushi, Rolando R. Garcia, Patrick Jöckel, Oliver Kirner, Giovanni Pitari, David A. Plummer, Laura Revell, Eugene Rozanov, Andrea Stenke, Taichu Y. Tanaka, Daniele Visioni, and Yousuke Yamashita
Atmos. Chem. Phys., 19, 11559–11586, https://doi.org/10.5194/acp-19-11559-2019, https://doi.org/10.5194/acp-19-11559-2019, 2019
Short summary
Short summary
We perform the first multi-model comparison of the impact of nudged meteorology on the stratospheric residual circulation (RC) in chemistry–climate models. Nudging meteorology does not constrain the mean strength of RC compared to free-running simulations, and despite the lack of agreement in the mean circulation, nudging tightly constrains the inter-annual variability in the tropical upward mass flux in the lower stratosphere. In summary, nudging strongly affects the representation of RC.
Kévin Lamy, Thierry Portafaix, Béatrice Josse, Colette Brogniez, Sophie Godin-Beekmann, Hassan Bencherif, Laura Revell, Hideharu Akiyoshi, Slimane Bekki, Michaela I. Hegglin, Patrick Jöckel, Oliver Kirner, Ben Liley, Virginie Marecal, Olaf Morgenstern, Andrea Stenke, Guang Zeng, N. Luke Abraham, Alexander T. Archibald, Neil Butchart, Martyn P. Chipperfield, Glauco Di Genova, Makoto Deushi, Sandip S. Dhomse, Rong-Ming Hu, Douglas Kinnison, Michael Kotkamp, Richard McKenzie, Martine Michou, Fiona M. O'Connor, Luke D. Oman, Giovanni Pitari, David A. Plummer, John A. Pyle, Eugene Rozanov, David Saint-Martin, Kengo Sudo, Taichu Y. Tanaka, Daniele Visioni, and Kohei Yoshida
Atmos. Chem. Phys., 19, 10087–10110, https://doi.org/10.5194/acp-19-10087-2019, https://doi.org/10.5194/acp-19-10087-2019, 2019
Short summary
Short summary
In this study, we simulate the ultraviolet radiation evolution during the 21st century on Earth's surface using the output from several numerical models which participated in the Chemistry-Climate Model Initiative. We present four possible futures which depend on greenhouse gases emissions. The role of ozone-depleting substances, greenhouse gases and aerosols are investigated. Our results emphasize the important role of aerosols for future ultraviolet radiation in the Northern Hemisphere.
Ohad Harari, Chaim I. Garfinkel, Shlomi Ziskin Ziv, Olaf Morgenstern, Guang Zeng, Simone Tilmes, Douglas Kinnison, Makoto Deushi, Patrick Jöckel, Andrea Pozzer, Fiona M. O'Connor, and Sean Davis
Atmos. Chem. Phys., 19, 9253–9268, https://doi.org/10.5194/acp-19-9253-2019, https://doi.org/10.5194/acp-19-9253-2019, 2019
Short summary
Short summary
Ozone depletion in the Antarctic has been shown to influence surface conditions, but the effects of ozone depletion in the Arctic on surface climate are unclear. We show that Arctic ozone does influence surface climate in both polar regions and tropical regions, though the proximate cause of these surface impacts is not yet clear.
Matthias Nützel, Aurélien Podglajen, Hella Garny, and Felix Ploeger
Atmos. Chem. Phys., 19, 8947–8966, https://doi.org/10.5194/acp-19-8947-2019, https://doi.org/10.5194/acp-19-8947-2019, 2019
Short summary
Short summary
We investigate the transport pathways of water vapour from the upper troposphere in the Asian monsoon region to the stratosphere. In the employed chemistry-transport model we use a tagging method, such that the impact of different source regions on the stratospheric water vapour budget can be quantified. A key finding is that the Asian monsoon (compared to other source regions) is very efficient in transporting air masses and water vapour to the tropical and extratropical stratosphere.
Paul Konopka, Mengchu Tao, Felix Ploeger, Mohamadou Diallo, and Martin Riese
Geosci. Model Dev., 12, 2441–2462, https://doi.org/10.5194/gmd-12-2441-2019, https://doi.org/10.5194/gmd-12-2441-2019, 2019
Short summary
Short summary
CLaMS is a Lagrangian transport model suitable for simulating atmospheric transport and chemistry. The novel approach of CLaMS is its description of atmospheric mixing. Whereas the common approach is to minimize the numerical diffusion ever present in the modeling of transport, CLaMS is a first attempt to apply this
undesirable disturbing effectto parametrize the true physical mixing. In this paper, we show how this concept works both in the stratosphere and in the troposphere.
Petr Šácha, Roland Eichinger, Hella Garny, Petr Pišoft, Simone Dietmüller, Laura de la Torre, David A. Plummer, Patrick Jöckel, Olaf Morgenstern, Guang Zeng, Neal Butchart, and Juan A. Añel
Atmos. Chem. Phys., 19, 7627–7647, https://doi.org/10.5194/acp-19-7627-2019, https://doi.org/10.5194/acp-19-7627-2019, 2019
Short summary
Short summary
Climate models robustly project a Brewer–Dobson circulation (BDC) acceleration in the course of climate change. Analyzing mean age of stratospheric air (AoA) from a subset of climate projection simulations, we find a remarkable agreement in simulating the largest AoA trends in the extratropical stratosphere. This is shown to be related with the upward shift of the circulation, resulting in a so-called stratospheric shrinkage, which could be one of the so-far-omitted BDC acceleration drivers.
Franziska Winterstein, Fabian Tanalski, Patrick Jöckel, Martin Dameris, and Michael Ponater
Atmos. Chem. Phys., 19, 7151–7163, https://doi.org/10.5194/acp-19-7151-2019, https://doi.org/10.5194/acp-19-7151-2019, 2019
Short summary
Short summary
The atmospheric concentrations of the anthropogenic greenhouse gas methane are predicted to rise in the future. In this paper we investigate how very strong methane concentrations will impact the atmosphere. We analyse two experiments, one with doubled and one with quintupled methane concentrations and focus on the rapid atmospheric changes before the ocean adjusts to the induced
forcing. In particular these are changes in temperature, ozone, the hydroxyl radical and stratospheric water vapour.
Sabine Brinkop and Patrick Jöckel
Geosci. Model Dev., 12, 1991–2008, https://doi.org/10.5194/gmd-12-1991-2019, https://doi.org/10.5194/gmd-12-1991-2019, 2019
Short summary
Short summary
We have extended ATTILA (Atmospheric Tracer Transport in a LAgrangian model), a Lagrangian tracer transport scheme which is online coupled to the global ECHAM/MESSy Atmospheric Chemistry (EMAC) model, with a combination of newly developed and modified physical routines and new diagnostic and infrastructure submodels. The results show an improvement of the tracer transport into and within the stratosphere due to the newly implemented diabatic vertical velocity.
Mengchu Tao, Paul Konopka, Felix Ploeger, Xiaolu Yan, Jonathon S. Wright, Mohamadou Diallo, Stephan Fueglistaler, and Martin Riese
Atmos. Chem. Phys., 19, 6509–6534, https://doi.org/10.5194/acp-19-6509-2019, https://doi.org/10.5194/acp-19-6509-2019, 2019
Short summary
Short summary
This paper examines the annual and interannual variations as well as long-term trend of modeled stratospheric water vapor with a Lagrangian chemical transport model driven by ERA-I, MERRA-2 and JRA-55. We find reasonable consistency among the annual cycle, QBO and the variabilities induced by ENSO and volcanic aerosols. The main discrepancies are linked to the differences in reanalysis upwelling rates in the lower stratosphere. The trends are sensitive to the reanalyses that drives the model.
Felix Ploeger, Bernard Legras, Edward Charlesworth, Xiaolu Yan, Mohamadou Diallo, Paul Konopka, Thomas Birner, Mengchu Tao, Andreas Engel, and Martin Riese
Atmos. Chem. Phys., 19, 6085–6105, https://doi.org/10.5194/acp-19-6085-2019, https://doi.org/10.5194/acp-19-6085-2019, 2019
Short summary
Short summary
We analyse the change in the circulation of the middle atmosphere based on current generation meteorological reanalysis data sets. We find that long-term changes from 1989 to 2015 are similar for the chosen reanalyses, mainly resembling the forced response in climate model simulations to climate change. For shorter periods circulation changes are less robust, and the representation of decadal variability appears to be a major uncertainty for modelling the circulation of the middle atmosphere.
Huang Yang, Darryn W. Waugh, Clara Orbe, Guang Zeng, Olaf Morgenstern, Douglas E. Kinnison, Jean-Francois Lamarque, Simone Tilmes, David A. Plummer, Patrick Jöckel, Susan E. Strahan, Kane A. Stone, and Robyn Schofield
Atmos. Chem. Phys., 19, 5511–5528, https://doi.org/10.5194/acp-19-5511-2019, https://doi.org/10.5194/acp-19-5511-2019, 2019
Short summary
Short summary
We evaluate the performance of a suite of models in simulating the large-scale transport from the northern midlatitudes to the Arctic using a CO-like idealized tracer. We find a large multi-model spread of the Arctic concentration of this CO-like tracer that is well correlated with the differences in the location of the midlatitude jet as well as the northern Hadley Cell edge. Our results suggest the Hadley Cell is key and zonal-mean transport by surface meridional flow needs better constraint.
Marius Hauck, Frauke Fritsch, Hella Garny, and Andreas Engel
Atmos. Chem. Phys., 19, 5269–5291, https://doi.org/10.5194/acp-19-5269-2019, https://doi.org/10.5194/acp-19-5269-2019, 2019
Short summary
Short summary
The paper presents a modified method to invert mixing ratios of chemically active tracers into stratospheric age spectra. It features an imposed seasonal cycle to include transport seasonality into the spectra. An idealized set of tracers from a model is used as proof of concept and results are in good agreement with the model reference, except for the lowermost stratosphere. Applicability is studied with focus on number of tracers and error tolerance, providing a starting point for future work.
Rolf Sander, Andreas Baumgaertner, David Cabrera-Perez, Franziska Frank, Sergey Gromov, Jens-Uwe Grooß, Hartwig Harder, Vincent Huijnen, Patrick Jöckel, Vlassis A. Karydis, Kyle E. Niemeyer, Andrea Pozzer, Hella Riede, Martin G. Schultz, Domenico Taraborrelli, and Sebastian Tauer
Geosci. Model Dev., 12, 1365–1385, https://doi.org/10.5194/gmd-12-1365-2019, https://doi.org/10.5194/gmd-12-1365-2019, 2019
Short summary
Short summary
We present the atmospheric chemistry box model CAABA/MECCA which
now includes a number of new features: skeletal mechanism
reduction, the MOM chemical mechanism for volatile organic
compounds, an option to include reactions from the Master
Chemical Mechanism (MCM) and other chemical mechanisms, updated
isotope tagging, improved and new photolysis modules, and the new
feature of coexisting multiple chemistry mechanisms.
CAABA/MECCA is a community model published under the GPL.
Ryan S. Williams, Michaela I. Hegglin, Brian J. Kerridge, Patrick Jöckel, Barry G. Latter, and David A. Plummer
Atmos. Chem. Phys., 19, 3589–3620, https://doi.org/10.5194/acp-19-3589-2019, https://doi.org/10.5194/acp-19-3589-2019, 2019
Short summary
Short summary
Tropospheric ozone has important implications for air quality and climate change but is poorly understood at a regional and seasonal level. Analysis of model simulations indicates that downward transport of ozone from the stratosphere has a larger influence than previously thought (as much as ~50 % even near the surface). Recent estimated changes in tropospheric ozone (1980–89 to 2001–10) are generally positive, with substantial attribution from the stratosphere identified over some regions.
Aurélien Podglajen and Felix Ploeger
Atmos. Chem. Phys., 19, 1767–1783, https://doi.org/10.5194/acp-19-1767-2019, https://doi.org/10.5194/acp-19-1767-2019, 2019
Short summary
Short summary
The age spectrum (distribution of transit times) provides a compact description of transport from the surface to a given point in the atmosphere. It also determines the surface-emitted tracer content of an air parcel. We propose a method to invert this relation in order to retrieve age spectra from tracer concentrations and demonstrate its feasibility in idealized and model setups. Applied to observations, the approach might help to better constrain atmospheric transport timescales.
J. Christopher Kaiser, Johannes Hendricks, Mattia Righi, Patrick Jöckel, Holger Tost, Konrad Kandler, Bernadett Weinzierl, Daniel Sauer, Katharina Heimerl, Joshua P. Schwarz, Anne E. Perring, and Thomas Popp
Geosci. Model Dev., 12, 541–579, https://doi.org/10.5194/gmd-12-541-2019, https://doi.org/10.5194/gmd-12-541-2019, 2019
Short summary
Short summary
The implementation of the aerosol microphysics submodel MADE3 into the global atmospheric chemistry model EMAC is described and evaluated against an extensive pool of observational data, focusing on aerosol mass and number concentrations, size distributions, composition, and optical properties. EMAC (MADE3) is able to reproduce main aerosol properties reasonably well, in line with the performance of other global aerosol models.
Roland Eichinger, Simone Dietmüller, Hella Garny, Petr Šácha, Thomas Birner, Harald Bönisch, Giovanni Pitari, Daniele Visioni, Andrea Stenke, Eugene Rozanov, Laura Revell, David A. Plummer, Patrick Jöckel, Luke Oman, Makoto Deushi, Douglas E. Kinnison, Rolando Garcia, Olaf Morgenstern, Guang Zeng, Kane Adam Stone, and Robyn Schofield
Atmos. Chem. Phys., 19, 921–940, https://doi.org/10.5194/acp-19-921-2019, https://doi.org/10.5194/acp-19-921-2019, 2019
Short summary
Short summary
To shed more light upon the changes in stratospheric circulation in the 21st century, climate projection simulations of 10 state-of-the-art global climate models, spanning from 1960 to 2100, are analyzed. The study shows that in addition to changes in transport, mixing also plays an important role in stratospheric circulation and that the properties of mixing vary over time. Furthermore, the influence of mixing is quantified and a dynamical framework is provided to understand the changes.
Mohamadou Diallo, Paul Konopka, Michelle L. Santee, Rolf Müller, Mengchu Tao, Kaley A. Walker, Bernard Legras, Martin Riese, Manfred Ern, and Felix Ploeger
Atmos. Chem. Phys., 19, 425–446, https://doi.org/10.5194/acp-19-425-2019, https://doi.org/10.5194/acp-19-425-2019, 2019
Short summary
Short summary
This paper assesses the structural changes in the shallow and transition branches of the BDC induced by El Nino using the Lagrangian model simulations driven by ERAi and JRA-55 combined with MLS observations. We found a clear evidence of a weakening of the transition branch due to an upward shift in the dissipation height of the planetary and gravity waves and a strengthening of the shallow branch due to enhanced GW breaking in the tropics–subtropics and PW breaking at high latitudes.
Laura E. Revell, Andrea Stenke, Fiona Tummon, Aryeh Feinberg, Eugene Rozanov, Thomas Peter, N. Luke Abraham, Hideharu Akiyoshi, Alexander T. Archibald, Neal Butchart, Makoto Deushi, Patrick Jöckel, Douglas Kinnison, Martine Michou, Olaf Morgenstern, Fiona M. O'Connor, Luke D. Oman, Giovanni Pitari, David A. Plummer, Robyn Schofield, Kane Stone, Simone Tilmes, Daniele Visioni, Yousuke Yamashita, and Guang Zeng
Atmos. Chem. Phys., 18, 16155–16172, https://doi.org/10.5194/acp-18-16155-2018, https://doi.org/10.5194/acp-18-16155-2018, 2018
Short summary
Short summary
Global models such as those participating in the Chemistry-Climate Model Initiative (CCMI) consistently simulate biases in tropospheric ozone compared with observations. We performed an advanced statistical analysis with one of the CCMI models to understand the cause of the bias. We found that emissions of ozone precursor gases are the dominant driver of the bias, implying either that the emissions are too large, or that the way in which the model handles emissions needs to be improved.
Mohamadou Diallo, Martin Riese, Thomas Birner, Paul Konopka, Rolf Müller, Michaela I. Hegglin, Michelle L. Santee, Mark Baldwin, Bernard Legras, and Felix Ploeger
Atmos. Chem. Phys., 18, 13055–13073, https://doi.org/10.5194/acp-18-13055-2018, https://doi.org/10.5194/acp-18-13055-2018, 2018
Short summary
Short summary
The unprecedented timing of an El Niño event aligned with the disrupted QBO in 2015–2016 caused a perturbation to the stratospheric circulation, affecting trace gases. This paper resolves the puzzling response of the lower stratospheric water vapor by showing that the QBO disruption reversed the lower stratosphere moistening triggered by the alignment of the El Niño event with a westerly QBO in early boreal winter.
Amanda C. Maycock, Katja Matthes, Susann Tegtmeier, Hauke Schmidt, Rémi Thiéblemont, Lon Hood, Hideharu Akiyoshi, Slimane Bekki, Makoto Deushi, Patrick Jöckel, Oliver Kirner, Markus Kunze, Marion Marchand, Daniel R. Marsh, Martine Michou, David Plummer, Laura E. Revell, Eugene Rozanov, Andrea Stenke, Yousuke Yamashita, and Kohei Yoshida
Atmos. Chem. Phys., 18, 11323–11343, https://doi.org/10.5194/acp-18-11323-2018, https://doi.org/10.5194/acp-18-11323-2018, 2018
Short summary
Short summary
The 11-year solar cycle is an important driver of climate variability. Changes in incoming solar ultraviolet radiation affect atmospheric ozone, which in turn influences atmospheric temperatures. Constraining the impact of the solar cycle on ozone is therefore important for understanding climate variability. This study examines the representation of the solar influence on ozone in numerical models used to simulate past and future climate. We highlight important differences among model datasets.
Blanca Ayarzagüena, Lorenzo M. Polvani, Ulrike Langematz, Hideharu Akiyoshi, Slimane Bekki, Neal Butchart, Martin Dameris, Makoto Deushi, Steven C. Hardiman, Patrick Jöckel, Andrew Klekociuk, Marion Marchand, Martine Michou, Olaf Morgenstern, Fiona M. O'Connor, Luke D. Oman, David A. Plummer, Laura Revell, Eugene Rozanov, David Saint-Martin, John Scinocca, Andrea Stenke, Kane Stone, Yousuke Yamashita, Kohei Yoshida, and Guang Zeng
Atmos. Chem. Phys., 18, 11277–11287, https://doi.org/10.5194/acp-18-11277-2018, https://doi.org/10.5194/acp-18-11277-2018, 2018
Short summary
Short summary
Stratospheric sudden warmings (SSWs) are natural major disruptions of the polar stratospheric circulation that also affect surface weather. In the literature there are conflicting claims as to whether SSWs will change in the future. The confusion comes from studies using different models and methods. Here we settle the question by analysing 12 models with a consistent methodology, to show that no robust changes in frequency and other features are expected over the 21st century.
Franziska Frank, Patrick Jöckel, Sergey Gromov, and Martin Dameris
Atmos. Chem. Phys., 18, 9955–9973, https://doi.org/10.5194/acp-18-9955-2018, https://doi.org/10.5194/acp-18-9955-2018, 2018
Short summary
Short summary
It is frequently assumed that one methane molecule produces two water molecules. Applying various modeling concepts, we find that the yield of water from methane is vertically not constantly 2. In the upper stratosphere and lower mesosphere, transport of intermediate H2 molecules even led to a yield greater than 2. We conclude that for a realistic chemical source of stratospheric water vapor, one must also take other sources (H2), intermediates and the chemical removal of water into account.
Sergey Gromov, Carl A. M. Brenninkmeijer, and Patrick Jöckel
Atmos. Chem. Phys., 18, 9831–9843, https://doi.org/10.5194/acp-18-9831-2018, https://doi.org/10.5194/acp-18-9831-2018, 2018
Short summary
Short summary
Using the observational data on 13C (CO) and 13C (CH4) from the extra-tropical Southern Hemisphere (ETSH) and EMAC model we (1) provide an independent, observation-based evaluation of Cl atom concentration variations in the ETSH throughout 1994–2000, (2) show that the role of tropospheric Cl as a sink of CH4 is seriously overestimated in the literature, (3) demonstrate that the 13C/12C ratio of CO is a sensitive indicator for the isotopic composition of reacted CH4 and therefore for its sources.
Liubov Poshyvailo, Rolf Müller, Paul Konopka, Gebhard Günther, Martin Riese, Aurélien Podglajen, and Felix Ploeger
Atmos. Chem. Phys., 18, 8505–8527, https://doi.org/10.5194/acp-18-8505-2018, https://doi.org/10.5194/acp-18-8505-2018, 2018
Short summary
Short summary
Water vapour (H2O) in the UTLS is a key player for global radiation, which is critical for predictions of future climate change. We investigate the effects of current uncertainties in tropopause temperature, horizontal transport and small-scale mixing on simulated H2O, using the Chemical Lagrangian Model of the Stratosphere. Our sensitivity studies provide new insights into the leading processes controlling stratospheric H2O, important for assessing and improving climate model projections.
Sandip S. Dhomse, Douglas Kinnison, Martyn P. Chipperfield, Ross J. Salawitch, Irene Cionni, Michaela I. Hegglin, N. Luke Abraham, Hideharu Akiyoshi, Alex T. Archibald, Ewa M. Bednarz, Slimane Bekki, Peter Braesicke, Neal Butchart, Martin Dameris, Makoto Deushi, Stacey Frith, Steven C. Hardiman, Birgit Hassler, Larry W. Horowitz, Rong-Ming Hu, Patrick Jöckel, Beatrice Josse, Oliver Kirner, Stefanie Kremser, Ulrike Langematz, Jared Lewis, Marion Marchand, Meiyun Lin, Eva Mancini, Virginie Marécal, Martine Michou, Olaf Morgenstern, Fiona M. O'Connor, Luke Oman, Giovanni Pitari, David A. Plummer, John A. Pyle, Laura E. Revell, Eugene Rozanov, Robyn Schofield, Andrea Stenke, Kane Stone, Kengo Sudo, Simone Tilmes, Daniele Visioni, Yousuke Yamashita, and Guang Zeng
Atmos. Chem. Phys., 18, 8409–8438, https://doi.org/10.5194/acp-18-8409-2018, https://doi.org/10.5194/acp-18-8409-2018, 2018
Short summary
Short summary
We analyse simulations from the Chemistry-Climate Model Initiative (CCMI) to estimate the return dates of the stratospheric ozone layer from depletion by anthropogenic chlorine and bromine. The simulations from 20 models project that global column ozone will return to 1980 values in 2047 (uncertainty range 2042–2052). Return dates in other regions vary depending on factors related to climate change and importance of chlorine and bromine. Column ozone in the tropics may continue to decline.
Stefan Lossow, Dale F. Hurst, Karen H. Rosenlof, Gabriele P. Stiller, Thomas von Clarmann, Sabine Brinkop, Martin Dameris, Patrick Jöckel, Doug E. Kinnison, Johannes Plieninger, David A. Plummer, Felix Ploeger, William G. Read, Ellis E. Remsberg, James M. Russell, and Mengchu Tao
Atmos. Chem. Phys., 18, 8331–8351, https://doi.org/10.5194/acp-18-8331-2018, https://doi.org/10.5194/acp-18-8331-2018, 2018
Short summary
Short summary
Trend estimates of lower stratospheric H2O derived from the FPH observations at Boulder and a merged zonal mean satellite data set clearly differ for the time period from the late 1980s to 2010. We investigate if a sampling bias between Boulder and the zonal mean around the Boulder latitude can explain these trend discrepancies. Typically they are small and not sufficient to explain the trend discrepancies in the observational database.
Xiaolu Yan, Paul Konopka, Felix Ploeger, Mengchu Tao, Rolf Müller, Michelle L. Santee, Jianchun Bian, and Martin Riese
Atmos. Chem. Phys., 18, 8079–8096, https://doi.org/10.5194/acp-18-8079-2018, https://doi.org/10.5194/acp-18-8079-2018, 2018
Short summary
Short summary
Many works investigate the impact of ENSO on the troposphere. However, only a few works check the impact of ENSO at higher altitudes.
Here, we analyse the impact of ENSO on the vicinity of the tropopause using reanalysis, satellite, in situ and model data. We find that ENSO shows the strongest signal in winter, but its impact can last until early the next summer. The ENSO anomaly is insignificant in late summer. Our study can help to understand the atmosphere propagation after ENSO.
Stefanie Meul, Ulrike Langematz, Philipp Kröger, Sophie Oberländer-Hayn, and Patrick Jöckel
Atmos. Chem. Phys., 18, 7721–7738, https://doi.org/10.5194/acp-18-7721-2018, https://doi.org/10.5194/acp-18-7721-2018, 2018
Short summary
Short summary
Using a chemistry--climate model future changes in the stratosphere-to-troposphere ozone mass flux, their drivers, and the future distribution of stratospheric ozone in the troposphere are investigated. In an extreme greenhouse gas (GHG) scenario, the global influx of stratospheric ozone into the troposphere is projected to grow between 2000 and 2100 by 53%. The increase is due to the recovery of stratospheric ozone owing to declining halogens and GHG induced circulation and temperature changes.
Clara Orbe, Huang Yang, Darryn W. Waugh, Guang Zeng, Olaf Morgenstern, Douglas E. Kinnison, Jean-Francois Lamarque, Simone Tilmes, David A. Plummer, John F. Scinocca, Beatrice Josse, Virginie Marecal, Patrick Jöckel, Luke D. Oman, Susan E. Strahan, Makoto Deushi, Taichu Y. Tanaka, Kohei Yoshida, Hideharu Akiyoshi, Yousuke Yamashita, Andreas Stenke, Laura Revell, Timofei Sukhodolov, Eugene Rozanov, Giovanni Pitari, Daniele Visioni, Kane A. Stone, Robyn Schofield, and Antara Banerjee
Atmos. Chem. Phys., 18, 7217–7235, https://doi.org/10.5194/acp-18-7217-2018, https://doi.org/10.5194/acp-18-7217-2018, 2018
Short summary
Short summary
In this study we compare a few atmospheric transport properties among several numerical models that are used to study the influence of atmospheric chemistry on climate. We show that there are large differences among models in terms of the timescales that connect the Northern Hemisphere midlatitudes, where greenhouse gases and ozone-depleting substances are emitted, to the Southern Hemisphere. Our results may have important implications for how models represent atmospheric composition.
Simone Dietmüller, Roland Eichinger, Hella Garny, Thomas Birner, Harald Boenisch, Giovanni Pitari, Eva Mancini, Daniele Visioni, Andrea Stenke, Laura Revell, Eugene Rozanov, David A. Plummer, John Scinocca, Patrick Jöckel, Luke Oman, Makoto Deushi, Shibata Kiyotaka, Douglas E. Kinnison, Rolando Garcia, Olaf Morgenstern, Guang Zeng, Kane Adam Stone, and Robyn Schofield
Atmos. Chem. Phys., 18, 6699–6720, https://doi.org/10.5194/acp-18-6699-2018, https://doi.org/10.5194/acp-18-6699-2018, 2018
Jens Krause, Peter Hoor, Andreas Engel, Felix Plöger, Jens-Uwe Grooß, Harald Bönisch, Timo Keber, Björn-Martin Sinnhuber, Wolfgang Woiwode, and Hermann Oelhaf
Atmos. Chem. Phys., 18, 6057–6073, https://doi.org/10.5194/acp-18-6057-2018, https://doi.org/10.5194/acp-18-6057-2018, 2018
Short summary
Short summary
We present tracer measurements of CO and N2O measured during the POLSTRACC aircraft campaign in winter 2015–2016. We found enhanced CO values relative to N2O in the polar lower stratosphere in addition to the ageing of this region during winter. By using model simulations it was possible to link this enhancement to an increased mixing of the tropical tropopause. We thus conclude that the polar lower stratosphere in late winter is strongly influenced by quasi-isentropic mixing from the tropics.
Klaus-Dirk Gottschaldt, Hans Schlager, Robert Baumann, Duy Sinh Cai, Veronika Eyring, Phoebe Graf, Volker Grewe, Patrick Jöckel, Tina Jurkat-Witschas, Christiane Voigt, Andreas Zahn, and Helmut Ziereis
Atmos. Chem. Phys., 18, 5655–5675, https://doi.org/10.5194/acp-18-5655-2018, https://doi.org/10.5194/acp-18-5655-2018, 2018
Short summary
Short summary
This study places aircraft trace gas measurements from within the Asian summer monsoon anticyclone into the context of regional, intra- and interannual variability. We find that the processes reflected in the measurements are present throughout multiple simulated monsoon seasons. Dynamical instabilities, photochemical ozone production, lightning and entrainments from the lower troposphere and from the tropopause region determine the distinct composition of the anticyclone and its outflow.
Mariano Mertens, Volker Grewe, Vanessa S. Rieger, and Patrick Jöckel
Atmos. Chem. Phys., 18, 5567–5588, https://doi.org/10.5194/acp-18-5567-2018, https://doi.org/10.5194/acp-18-5567-2018, 2018
Short summary
Short summary
We quantified the contribution of land transport and shipping emissions to tropospheric ozone using a global chemistry–climate model. Our results indicate a contribution to ground-level ozone from land transport emissions of up to 18 % in North America and Southern Europe as well as a contribution from shipping emissions of up to 30 % in the Pacific. Our estimates of the radiative ozone forcing due to land transport and shipping emissions are 92 mW m−2 and 62 mW m−2, respectively.
Astrid Kerkweg, Christiane Hofmann, Patrick Jöckel, Mariano Mertens, and Gregor Pante
Geosci. Model Dev., 11, 1059–1076, https://doi.org/10.5194/gmd-11-1059-2018, https://doi.org/10.5194/gmd-11-1059-2018, 2018
Short summary
Short summary
As part of the model documentation of the MECO(n) system, this article documents the basics of the Multi-Model-Driver expansion (MMD v2.0) to two-way coupling and the newly developed generic MESSy submodel GRID (v1.0), which is used by MMD v2.0 for the generalised definition of arbitrary grids and for the
transformation of data between them.
Andreas Engel, Harald Bönisch, Jennifer Ostermöller, Martyn P. Chipperfield, Sandip Dhomse, and Patrick Jöckel
Atmos. Chem. Phys., 18, 601–619, https://doi.org/10.5194/acp-18-601-2018, https://doi.org/10.5194/acp-18-601-2018, 2018
Short summary
Short summary
We present a new method to derive equivalent effective stratospheric chlorine (EESC), which is based on an improved formulation of the propagation of trends of species with chemical loss from the troposphere to the stratosphere. EESC calculated with the new method shows much better agreement with model-derived ESC. Based on this new formulation, we expect the halogen impact on midlatitude stratospheric ozone to return to 1980 values about 10 years later, then using the current formulation.
Tilman Hüneke, Oliver-Alex Aderhold, Jannik Bounin, Marcel Dorf, Eric Gentry, Katja Grossmann, Jens-Uwe Grooß, Peter Hoor, Patrick Jöckel, Mareike Kenntner, Marvin Knapp, Matthias Knecht, Dominique Lörks, Sabrina Ludmann, Sigrun Matthes, Rasmus Raecke, Marcel Reichert, Jannis Weimar, Bodo Werner, Andreas Zahn, Helmut Ziereis, and Klaus Pfeilsticker
Atmos. Meas. Tech., 10, 4209–4234, https://doi.org/10.5194/amt-10-4209-2017, https://doi.org/10.5194/amt-10-4209-2017, 2017
Short summary
Short summary
This paper describes a novel instrument for the aircraft-borne remote sensing of trace gases and liquid and solid water. Until recently, such measurements could only be evaluated under clear-sky conditions. We present a characterization and error assessment of the novel "scaling method", which allows for the retrieval of absolute trace gas concentrations under all sky conditions, significantly expanding the applicability of such measurements to study atmospheric photochemistry.
Stefan Lossow, Hella Garny, and Patrick Jöckel
Atmos. Chem. Phys., 17, 11521–11539, https://doi.org/10.5194/acp-17-11521-2017, https://doi.org/10.5194/acp-17-11521-2017, 2017
Stefanie Falk, Björn-Martin Sinnhuber, Gisèle Krysztofiak, Patrick Jöckel, Phoebe Graf, and Sinikka T. Lennartz
Atmos. Chem. Phys., 17, 11313–11329, https://doi.org/10.5194/acp-17-11313-2017, https://doi.org/10.5194/acp-17-11313-2017, 2017
Short summary
Short summary
Brominated very short-lived source gases (VSLS) contribute significantly to the tropospheric and stratospheric bromine loading. We find an increase of future ocean–atmosphere flux of brominated VSLS of 8–10 % compared to present day. A decrease in the tropospheric mixing ratios of VSLS and an increase in the lower stratosphere are attributed to changes in atmospheric chemistry and transport. Bromine impact on stratospheric ozone at the end of the 21st century is reduced compared to present day.
Gabriele P. Stiller, Federico Fierli, Felix Ploeger, Chiara Cagnazzo, Bernd Funke, Florian J. Haenel, Thomas Reddmann, Martin Riese, and Thomas von Clarmann
Atmos. Chem. Phys., 17, 11177–11192, https://doi.org/10.5194/acp-17-11177-2017, https://doi.org/10.5194/acp-17-11177-2017, 2017
Short summary
Short summary
The discrepancy between modelled and observed 25-year trends of the strength of the stratospheric Brewer–Dobson circulation (BDC) is still not resolved. With our paper we trace the observed hemispheric dipole structure of age of air trends back to natural variability in shorter-term (decadal) time frames. Beyond this we demonstrate that after correction for the decadal natural variability the remaining trend for the first decade of the 21st century is consistent with model simulations.
Sergey Gromov, Carl A. M. Brenninkmeijer, and Patrick Jöckel
Atmos. Chem. Phys., 17, 8525–8552, https://doi.org/10.5194/acp-17-8525-2017, https://doi.org/10.5194/acp-17-8525-2017, 2017
Short summary
Short summary
We revisit the proxies/uncertainties for the 13C/12C ratios of emissions of reactive C into the atmosphere. Our main findings are (i) a factor of 2 less uncertain estimate of tropospheric CO surface sources δ13C, (ii) a confirmed disagreement between the bottom-up and top-down 13CO-inclusive emission estimates, and (iii) a novel estimate of the δ13C signatures of a range of NMHCs/VOCs to be used in modelling studies. Results are based on the EMAC model emission set-up evaluated for 2000.
Volker Grewe, Eleni Tsati, Mariano Mertens, Christine Frömming, and Patrick Jöckel
Geosci. Model Dev., 10, 2615–2633, https://doi.org/10.5194/gmd-10-2615-2017, https://doi.org/10.5194/gmd-10-2615-2017, 2017
Short summary
Short summary
We present a diagnostics, implemented in an Earth system model, which keeps track of the contribution of source categories (mainly emission sectors) to various concentrations (O3 and HOx). For the first time, it takes into account chemically competing effects, e.g., the competition between ozone precursors in the production of ozone. We show that the results are in-line with results from other tagging schemes and provide plausibility checks for OH and HO2, which have not previously been tagged.
Felix Ploeger, Paul Konopka, Kaley Walker, and Martin Riese
Atmos. Chem. Phys., 17, 7055–7066, https://doi.org/10.5194/acp-17-7055-2017, https://doi.org/10.5194/acp-17-7055-2017, 2017
Short summary
Short summary
Pollution transport from the surface to the stratosphere within the Asian summer monsoon circulation may cause harmful effects on stratospheric chemistry and climate. We investigate air mass transport from the monsoon anticyclone into the stratosphere, combining model simulations with satellite trace gas measurements. We show evidence for two transport pathways from the monsoon: (i) into the tropical stratosphere and (ii) into the Northern Hemisphere extratropical lower stratosphere.
Klaus-D. Gottschaldt, Hans Schlager, Robert Baumann, Heiko Bozem, Veronika Eyring, Peter Hoor, Patrick Jöckel, Tina Jurkat, Christiane Voigt, Andreas Zahn, and Helmut Ziereis
Atmos. Chem. Phys., 17, 6091–6111, https://doi.org/10.5194/acp-17-6091-2017, https://doi.org/10.5194/acp-17-6091-2017, 2017
Short summary
Short summary
We present upper-tropospheric trace gas measurements in the Asian summer monsoon anticyclone, obtained with the HALO research aircraft in September 2012. The anticyclone is one of the largest atmospheric features on Earth, but many aspects of it are not well understood. With the help of model simulations we find that entrainments from the tropopause region and the lower troposphere, combined with photochemistry and dynamical instabilities, can explain the observations.
Jennifer Ostermöller, Harald Bönisch, Patrick Jöckel, and Andreas Engel
Atmos. Chem. Phys., 17, 3785–3797, https://doi.org/10.5194/acp-17-3785-2017, https://doi.org/10.5194/acp-17-3785-2017, 2017
Short summary
Short summary
We analysed the temporal evolution of fractional release factors (FRFs) from EMAC model simulations for several halocarbons and nitrous oxide. The current formulation of FRFs yields values that depend on the tropospheric trend of the species. This is a problematic issue for the application of FRF in the calculation of steady-state quantities (e.g. ODP). Including a loss term in the calculation, we develop a new formulation of FRF and find that the time dependence can almost be compensated.
Olaf Morgenstern, Michaela I. Hegglin, Eugene Rozanov, Fiona M. O'Connor, N. Luke Abraham, Hideharu Akiyoshi, Alexander T. Archibald, Slimane Bekki, Neal Butchart, Martyn P. Chipperfield, Makoto Deushi, Sandip S. Dhomse, Rolando R. Garcia, Steven C. Hardiman, Larry W. Horowitz, Patrick Jöckel, Beatrice Josse, Douglas Kinnison, Meiyun Lin, Eva Mancini, Michael E. Manyin, Marion Marchand, Virginie Marécal, Martine Michou, Luke D. Oman, Giovanni Pitari, David A. Plummer, Laura E. Revell, David Saint-Martin, Robyn Schofield, Andrea Stenke, Kane Stone, Kengo Sudo, Taichu Y. Tanaka, Simone Tilmes, Yousuke Yamashita, Kohei Yoshida, and Guang Zeng
Geosci. Model Dev., 10, 639–671, https://doi.org/10.5194/gmd-10-639-2017, https://doi.org/10.5194/gmd-10-639-2017, 2017
Short summary
Short summary
We present a review of the make-up of 20 models participating in the Chemistry–Climate Model Initiative (CCMI). In comparison to earlier such activities, most of these models comprise a whole-atmosphere chemistry, and several of them include an interactive ocean module. This makes them suitable for studying the interactions of tropospheric air quality, stratospheric ozone, and climate. The paper lays the foundation for other studies using the CCMI simulations for scientific analysis.
Chaitri Roy, Suvarna Fadnavis, Rolf Müller, D. C. Ayantika, Felix Ploeger, and Alexandru Rap
Atmos. Chem. Phys., 17, 1297–1311, https://doi.org/10.5194/acp-17-1297-2017, https://doi.org/10.5194/acp-17-1297-2017, 2017
Short summary
Short summary
In the monsoon season, Asian NOx emissions are rapidly transported to the UTLS and can impact ozone in the UTLS. From chemistry–climate model simulations, we show that increasing Asian NOx emissions have enhanced ozone radiative forcing over Southeast Asia, which leads to significant warming over the Tibetan Plateau and increase precipitation over India. However, a further increase in NOx emissions elicited negative precipitation due to reversal of monsoon Hadley circulation.
Matthias Nützel, Martin Dameris, and Hella Garny
Atmos. Chem. Phys., 16, 14755–14774, https://doi.org/10.5194/acp-16-14755-2016, https://doi.org/10.5194/acp-16-14755-2016, 2016
Short summary
Short summary
Using seven reanalyses, we study the movement and drivers of the upper tropospheric–lower stratospheric anticyclone (AC) that forms during the Asian summer monsoon and is debated to be an important pathway for air masses to the stratosphere. We find that the distribution of the AC's centre position, and especially the so-called bimodality, largely depends on the reanalysis. Furthermore, we can connect shifts of the AC to precipitation and convection anomalies over India and the western Pacific.
Duy Cai, Martin Dameris, Hella Garny, Felix Bunzel, Patrick Jöckel, and Phoebe Graf
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-870, https://doi.org/10.5194/acp-2016-870, 2016
Revised manuscript not accepted
Short summary
Short summary
Reliable information on weather and climate are of increasing interest for economy, politics and society.
In particular decadal timescales become more and more important. This study focuses on stratospheric processes relevant for the dynamical variability on intra decadal timescale. We apply a so called power spectra analysis. With this method and further analyses we could determine a minimum vertical resolution for numerical models, which is required to capture these processes.
Bastian Kern and Patrick Jöckel
Geosci. Model Dev., 9, 3639–3654, https://doi.org/10.5194/gmd-9-3639-2016, https://doi.org/10.5194/gmd-9-3639-2016, 2016
Short summary
Short summary
Input and output of large data limit the performance of numerical models on supercomputers. We present an interface for the calculation of online diagnostics in a weather and climate model. These diagnostics are calculated online during the simulation instead of as subsequent post-processing. Depending on the diagnostic, we can reduce the amount of model output.
Mariano Mertens, Astrid Kerkweg, Patrick Jöckel, Holger Tost, and Christiane Hofmann
Geosci. Model Dev., 9, 3545–3567, https://doi.org/10.5194/gmd-9-3545-2016, https://doi.org/10.5194/gmd-9-3545-2016, 2016
Short summary
Short summary
This fourth part in a series of publications describing the newly developed regional chemistry–climate system MECO(n) is dedicated to the evaluation of MECO(n) with respect to tropospheric gas-phase chemistry. For this, a simulation incorporating two regional instances, one over Europe with 50 km resolution and one over Germany with 12 km resolution, is conducted. The model results are compared with satellite, ground-based and aircraft in situ observations.
Sergey M. Khaykin, Jean-Pierre Pommereau, Emmanuel D. Riviere, Gerhard Held, Felix Ploeger, Melanie Ghysels, Nadir Amarouche, Jean-Paul Vernier, Frank G. Wienhold, and Dmitry Ionov
Atmos. Chem. Phys., 16, 12273–12286, https://doi.org/10.5194/acp-16-12273-2016, https://doi.org/10.5194/acp-16-12273-2016, 2016
Short summary
Short summary
The study makes use of a series of field experiments conducted in Brazil and aimed at studying the processes controlling the composition of the tropical lower stratosphere. High-resolution balloon-borne measurements together with global-coverage satellite observations and weather radar acquisitions are analysed using trajectory and transport modelling in order to evaluate the contribution of different transport pathways to the stratospheric water budget.
Hiroshi Yamashita, Volker Grewe, Patrick Jöckel, Florian Linke, Martin Schaefer, and Daisuke Sasaki
Geosci. Model Dev., 9, 3363–3392, https://doi.org/10.5194/gmd-9-3363-2016, https://doi.org/10.5194/gmd-9-3363-2016, 2016
Short summary
Short summary
This study introduces AirTraf v1.0 for climate impact evaluations, which performs global air traffic simulations in the ECHAM5/MESSy Atmospheric Chemistry model. AirTraf simulations were demonstrated with great circle and flight time routing options for a specific winter day, assuming an Airbus A330 aircraft. The results confirmed that AirTraf simulates the air traffic properly for the two options. Calculated flight time, fuel consumption and NOx emission index are comparable to reference data.
Felix Ploeger and Thomas Birner
Atmos. Chem. Phys., 16, 10195–10213, https://doi.org/10.5194/acp-16-10195-2016, https://doi.org/10.5194/acp-16-10195-2016, 2016
Short summary
Short summary
We investigate the aging of air in the stratosphere caused by transport due to Brewer's circulation, using the Boundary Impulse Evolving Response (BIER) method. The age spectra show multiple peaks caused by the seasonal and inter-annual variations of transport. The modal age is controlled by the residual circulation in the tropics and winter hemisphere extratropics and by mixing in the summer hemisphere. Analysis of the full age spectrum is strongly recommended for model inter-comparisons.
Jörn Ungermann, Mandfred Ern, Martin Kaufmann, Rolf Müller, Reinhold Spang, Felix Ploeger, Bärbel Vogel, and Martin Riese
Atmos. Chem. Phys., 16, 8389–8403, https://doi.org/10.5194/acp-16-8389-2016, https://doi.org/10.5194/acp-16-8389-2016, 2016
Short summary
Short summary
This paper presents an analysis of temperature and the trace gases PAN and O3 in
the Asian Summer Monsoon (ASM) region. The positive PAN anomaly consisting of
polluted air is confined vertically within the main ASM anticyclone, whereas a
recently shed eddy exhibits enhanced PAN VMRs for 1 to 2 km above the thermal
tropopause. This implies that eddy shedding provides a very rapid horizontal
transport pathway of Asian pollution into the extratropical lowermost
stratosphere.
Sabine Brinkop, Martin Dameris, Patrick Jöckel, Hella Garny, Stefan Lossow, and Gabriele Stiller
Atmos. Chem. Phys., 16, 8125–8140, https://doi.org/10.5194/acp-16-8125-2016, https://doi.org/10.5194/acp-16-8125-2016, 2016
Short summary
Short summary
This study investigates the water vapour decline in the stratosphere beginning in the year 2000 and other similarly strong stratospheric water vapour reductions. The driving forces are tropical sea surface temperature (SST) changes due to coincidence with a preceding ENSO event and supported by the west to east change of the QBO.
There are indications that both SSTs and the specific dynamical state of the atmosphere contribute to the long period of low water vapour values from 2001 to 2006.
Steffen Beirle, Christoph Hörmann, Patrick Jöckel, Song Liu, Marloes Penning de Vries, Andrea Pozzer, Holger Sihler, Pieter Valks, and Thomas Wagner
Atmos. Meas. Tech., 9, 2753–2779, https://doi.org/10.5194/amt-9-2753-2016, https://doi.org/10.5194/amt-9-2753-2016, 2016
Simone Dietmüller, Patrick Jöckel, Holger Tost, Markus Kunze, Catrin Gellhorn, Sabine Brinkop, Christine Frömming, Michael Ponater, Benedikt Steil, Axel Lauer, and Johannes Hendricks
Geosci. Model Dev., 9, 2209–2222, https://doi.org/10.5194/gmd-9-2209-2016, https://doi.org/10.5194/gmd-9-2209-2016, 2016
Short summary
Short summary
Four new radiation related submodels (RAD, AEROPT, CLOUDOPT, and ORBIT) are available within the MESSy framework now. They are largely based on the original radiation scheme of ECHAM5. RAD simulates radiative transfer, AEROPT calculates aerosol optical properties, CLOUDOPT calculates cloud optical properties, and ORBIT is responsible for Earth orbit calculations. Multiple diagnostic calls of the radiation routine are possible, so radiative forcing can be calculated during the model simulation.
Michael Löffler, Sabine Brinkop, and Patrick Jöckel
Atmos. Chem. Phys., 16, 6547–6562, https://doi.org/10.5194/acp-16-6547-2016, https://doi.org/10.5194/acp-16-6547-2016, 2016
Short summary
Short summary
After the two major volcanic eruptions of El Chichón in Mexico in 1982 and Mount Pinatubo on the Philippines in 1991, stratospheric water vapour is significantly increased. This results from increased stratospheric heating rates due to volcanic aerosol and the subsequent changes in stratospheric and tropopause temperatures in the tropics. The tropical vertical advection and the South Asian summer monsoon are identified as important sources for the additional water vapour in the stratosphere.
Charlotte Marinke Hoppe, Felix Ploeger, Paul Konopka, and Rolf Müller
Atmos. Chem. Phys., 16, 6223–6239, https://doi.org/10.5194/acp-16-6223-2016, https://doi.org/10.5194/acp-16-6223-2016, 2016
Patrick Jöckel, Holger Tost, Andrea Pozzer, Markus Kunze, Oliver Kirner, Carl A. M. Brenninkmeijer, Sabine Brinkop, Duy S. Cai, Christoph Dyroff, Johannes Eckstein, Franziska Frank, Hella Garny, Klaus-Dirk Gottschaldt, Phoebe Graf, Volker Grewe, Astrid Kerkweg, Bastian Kern, Sigrun Matthes, Mariano Mertens, Stefanie Meul, Marco Neumaier, Matthias Nützel, Sophie Oberländer-Hayn, Roland Ruhnke, Theresa Runde, Rolf Sander, Dieter Scharffe, and Andreas Zahn
Geosci. Model Dev., 9, 1153–1200, https://doi.org/10.5194/gmd-9-1153-2016, https://doi.org/10.5194/gmd-9-1153-2016, 2016
Short summary
Short summary
With an advanced numerical global chemistry climate model (CCM) we performed several detailed
combined hind-cast and projection simulations of the period 1950 to 2100 to assess the
past, present, and potential future dynamical and chemical state of the Earth atmosphere.
The manuscript documents the model and the various applied model set-ups and provides
a first evaluation of the simulation results from a global perspective as a quality check of the data.
Hella Garny and William J. Randel
Atmos. Chem. Phys., 16, 2703–2718, https://doi.org/10.5194/acp-16-2703-2016, https://doi.org/10.5194/acp-16-2703-2016, 2016
Short summary
Short summary
We investigate the fate of air that originates in the monsoon region in the upper troposphere, where it was transported to by convection. We find that almost half of the air parcels released in the monsoon region in the upper troposphere reach the stratosphere within 60 days, and most ascend to the tropical lower stratosphere. This suggests that trace gases, including pollutants, that are transported into the stratosphere via the Asian monsoon are in a position to enter the deep stratosphere.
A. J. G. Baumgaertner, P. Jöckel, A. Kerkweg, R. Sander, and H. Tost
Geosci. Model Dev., 9, 125–135, https://doi.org/10.5194/gmd-9-125-2016, https://doi.org/10.5194/gmd-9-125-2016, 2016
Short summary
Short summary
The Community Earth System Model (CESM1) is connected to the the Modular Earth Submodel System (MESSy) as a new base model. This allows MESSy users the option to utilize either the state-of-the art spectral element atmosphere dynamical core or the finite volume core of CESM1. Additionally, this makes several other component models available to MESSy users.
Christiane Hofmann, Astrid Kerkweg, Peter Hoor, and Patrick Jöckel
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2015-949, https://doi.org/10.5194/acp-2015-949, 2016
Revised manuscript not accepted
Short summary
Short summary
Ozone enhancements at the surface, caused by descending stratospheric air masses along deep tropopause folds, can be reproduced using the model system MECO(n). It is shown that stratosphere-troposphere-exchange (STE) in the vicinity of a tropopause fold occurs in regions of turbulence and diabatic processes. The efficiency of mixing is quantified, showing that almost all of the air masses originating in the tropopause fold are transported into the troposphere during the following two days.
F. Ploeger, C. Gottschling, S. Griessbach, J.-U. Grooß, G. Guenther, P. Konopka, R. Müller, M. Riese, F. Stroh, M. Tao, J. Ungermann, B. Vogel, and M. von Hobe
Atmos. Chem. Phys., 15, 13145–13159, https://doi.org/10.5194/acp-15-13145-2015, https://doi.org/10.5194/acp-15-13145-2015, 2015
Short summary
Short summary
The Asian summer monsoon provides an important pathway of tropospheric source gases and pollution into the lower stratosphere. This transport is characterized by deep convection and steady upwelling, combined with confinement inside a large-scale anticyclonic circulation in the upper troposphere and lower stratosphere. In this paper, we show that a barrier to horizontal transport in the monsoon can be determined from a local maximum in the gradient of potential vorticity.
A. Kerkweg and P. Jöckel
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmdd-8-8607-2015, https://doi.org/10.5194/gmdd-8-8607-2015, 2015
Revised manuscript not accepted
M. Tao, P. Konopka, F. Ploeger, J.-U. Grooß, R. Müller, C. M. Volk, K. A. Walker, and M. Riese
Atmos. Chem. Phys., 15, 8695–8715, https://doi.org/10.5194/acp-15-8695-2015, https://doi.org/10.5194/acp-15-8695-2015, 2015
Short summary
Short summary
A remarkable major stratospheric sudden warming during the boreal winter 2008/09 is studied with the Chemical Lagrangian Model of the Stratosphere (CLaMS). We investigate how mixing triggered by this event correlates the wave forcing and how transport and mixing affect the composition of the whole stratosphere in the Northern Hemisphere, by using the tracer-tracer correlation technique.
H. Fischer, A. Pozzer, T. Schmitt, P. Jöckel, T. Klippel, D. Taraborrelli, and J. Lelieveld
Atmos. Chem. Phys., 15, 6971–6980, https://doi.org/10.5194/acp-15-6971-2015, https://doi.org/10.5194/acp-15-6971-2015, 2015
R. Eichinger, P. Jöckel, and S. Lossow
Atmos. Chem. Phys., 15, 7003–7015, https://doi.org/10.5194/acp-15-7003-2015, https://doi.org/10.5194/acp-15-7003-2015, 2015
L. E. Revell, F. Tummon, A. Stenke, T. Sukhodolov, A. Coulon, E. Rozanov, H. Garny, V. Grewe, and T. Peter
Atmos. Chem. Phys., 15, 5887–5902, https://doi.org/10.5194/acp-15-5887-2015, https://doi.org/10.5194/acp-15-5887-2015, 2015
Short summary
Short summary
We have examined the effects of ozone precursor emissions and climate change on the tropospheric ozone budget. Under RCP 6.0, ozone in the future is governed primarily by changes in nitrogen oxides (NOx). Methane is also important, and induces an increase in tropospheric ozone that is approximately one-third of that caused by NOx. This study highlights the critical role that emission policies globally have to play in determining tropospheric ozone evolution through the 21st century.
R. Eichinger, P. Jöckel, S. Brinkop, M. Werner, and S. Lossow
Atmos. Chem. Phys., 15, 5537–5555, https://doi.org/10.5194/acp-15-5537-2015, https://doi.org/10.5194/acp-15-5537-2015, 2015
M. Righi, V. Eyring, K.-D. Gottschaldt, C. Klinger, F. Frank, P. Jöckel, and I. Cionni
Geosci. Model Dev., 8, 733–768, https://doi.org/10.5194/gmd-8-733-2015, https://doi.org/10.5194/gmd-8-733-2015, 2015
R. Pommrich, R. Müller, J.-U. Grooß, P. Konopka, F. Ploeger, B. Vogel, M. Tao, C. M. Hoppe, G. Günther, N. Spelten, L. Hoffmann, H.-C. Pumphrey, S. Viciani, F. D'Amato, C. M. Volk, P. Hoor, H. Schlager, and M. Riese
Geosci. Model Dev., 7, 2895–2916, https://doi.org/10.5194/gmd-7-2895-2014, https://doi.org/10.5194/gmd-7-2895-2014, 2014
Short summary
Short summary
A version of the chemical transport model CLaMS is presented, which features a simplified (numerically inexpensive) chemistry scheme. The model results using this version of CLaMS show a good representation of anomaly fields of CO, CH4, N2O, and CFC-11 in the lower stratosphere. CO measurements of three instruments (COLD, HAGAR, and Falcon-CO) in the lower tropical stratosphere (during the campaign TROCCINOX in 2005) have been compared and show a good agreement within the error bars.
R. Sander, P. Jöckel, O. Kirner, A. T. Kunert, J. Landgraf, and A. Pozzer
Geosci. Model Dev., 7, 2653–2662, https://doi.org/10.5194/gmd-7-2653-2014, https://doi.org/10.5194/gmd-7-2653-2014, 2014
C. M. Hoppe, L. Hoffmann, P. Konopka, J.-U. Grooß, F. Ploeger, G. Günther, P. Jöckel, and R. Müller
Geosci. Model Dev., 7, 2639–2651, https://doi.org/10.5194/gmd-7-2639-2014, https://doi.org/10.5194/gmd-7-2639-2014, 2014
P. Valks, N. Hao, S. Gimeno Garcia, D. Loyola, M. Dameris, P. Jöckel, and A. Delcloo
Atmos. Meas. Tech., 7, 2513–2530, https://doi.org/10.5194/amt-7-2513-2014, https://doi.org/10.5194/amt-7-2513-2014, 2014
R. Eichinger and P. Jöckel
Geosci. Model Dev., 7, 1573–1582, https://doi.org/10.5194/gmd-7-1573-2014, https://doi.org/10.5194/gmd-7-1573-2014, 2014
M. Riese, H. Oelhaf, P. Preusse, J. Blank, M. Ern, F. Friedl-Vallon, H. Fischer, T. Guggenmoser, M. Höpfner, P. Hoor, M. Kaufmann, J. Orphal, F. Plöger, R. Spang, O. Suminska-Ebersoldt, J. Ungermann, B. Vogel, and W. Woiwode
Atmos. Meas. Tech., 7, 1915–1928, https://doi.org/10.5194/amt-7-1915-2014, https://doi.org/10.5194/amt-7-1915-2014, 2014
S. Meul, U. Langematz, S. Oberländer, H. Garny, and P. Jöckel
Atmos. Chem. Phys., 14, 2959–2971, https://doi.org/10.5194/acp-14-2959-2014, https://doi.org/10.5194/acp-14-2959-2014, 2014
C. Liu, S. Beirle, T. Butler, P. Hoor, C. Frankenberg, P. Jöckel, M. Penning de Vries, U. Platt, A. Pozzer, M. G. Lawrence, J. Lelieveld, H. Tost, and T. Wagner
Atmos. Chem. Phys., 14, 1717–1732, https://doi.org/10.5194/acp-14-1717-2014, https://doi.org/10.5194/acp-14-1717-2014, 2014
V. Grewe, C. Frömming, S. Matthes, S. Brinkop, M. Ponater, S. Dietmüller, P. Jöckel, H. Garny, E. Tsati, K. Dahlmann, O. A. Søvde, J. Fuglestvedt, T. K. Berntsen, K. P. Shine, E. A. Irvine, T. Champougny, and P. Hullah
Geosci. Model Dev., 7, 175–201, https://doi.org/10.5194/gmd-7-175-2014, https://doi.org/10.5194/gmd-7-175-2014, 2014
M. Abalos, F. Ploeger, P. Konopka, W. J. Randel, and E. Serrano
Atmos. Chem. Phys., 13, 10787–10794, https://doi.org/10.5194/acp-13-10787-2013, https://doi.org/10.5194/acp-13-10787-2013, 2013
E. Regelin, H. Harder, M. Martinez, D. Kubistin, C. Tatum Ernest, H. Bozem, T. Klippel, Z. Hosaynali-Beygi, H. Fischer, R. Sander, P. Jöckel, R. Königstedt, and J. Lelieveld
Atmos. Chem. Phys., 13, 10703–10720, https://doi.org/10.5194/acp-13-10703-2013, https://doi.org/10.5194/acp-13-10703-2013, 2013
H. Garny, G. E. Bodeker, D. Smale, M. Dameris, and V. Grewe
Atmos. Chem. Phys., 13, 7279–7300, https://doi.org/10.5194/acp-13-7279-2013, https://doi.org/10.5194/acp-13-7279-2013, 2013
K. Gottschaldt, C. Voigt, P. Jöckel, M. Righi, R. Deckert, and S. Dietmüller
Atmos. Chem. Phys., 13, 3003–3025, https://doi.org/10.5194/acp-13-3003-2013, https://doi.org/10.5194/acp-13-3003-2013, 2013
Related subject area
Subject: Dynamics | Research Activity: Atmospheric Modelling | Altitude Range: Stratosphere | Science Focus: Physics (physical properties and processes)
The effect of interactive ozone chemistry on weak and strong stratospheric polar vortex events
Lagrangian gravity wave spectra in the lower stratosphere of current (re)analyses
Representation of the equatorial stratopause semiannual oscillation in global atmospheric reanalyses
A convolution of observational and model data to estimate age of air spectra in the northern hemispheric lower stratosphere
Sensitivity of age of air trends to the derivation method for non-linear increasing inert SF6
Adding value to extended-range forecasts in northern Europe by statistical post-processing using stratospheric observations
Propagation of gravity waves and its effects on pseudomomentum flux in a sudden stratospheric warming event
Future trends in stratosphere-to-troposphere transport in CCMI models
Simulating age of air and the distribution of SF6 in the stratosphere with the SILAM model
A tropospheric pathway of the stratospheric quasi-biennial oscillation (QBO) impact on the boreal winter polar vortex
Quantifying climate feedbacks in the middle atmosphere using WACCM
Temperature and tropopause characteristics from reanalyses data in the tropical tropopause layer
Deep convective influence on the UTLS composition in the Asian Monsoon Anticyclone region: 2017 StratoClim campaign results
The efficiency of transport into the stratosphere via the Asian and North American summer monsoon circulations
Evidence of small-scale quasi-isentropic mixing in ridges of extratropical baroclinic waves
The effect of atmospheric nudging on the stratospheric residual circulation in chemistry–climate models
On the representation of major stratospheric warmings in reanalyses
Influence of Arctic stratospheric ozone on surface climate in CCMI models
Quantification of water vapour transport from the Asian monsoon to the stratosphere
Extratropical age of air trends and causative factors in climate projection simulations
Composite analysis of the tropopause inversion layer in extratropical baroclinic waves
Lagrangian simulations of the transport of young air masses to the top of the Asian monsoon anticyclone and into the tropical pipe
Deriving stratospheric age of air spectra using an idealized set of chemically active trace gases
The global diabatic circulation of the stratosphere as a metric for the Brewer–Dobson circulation
The importance of interactive chemistry for stratosphere–troposphere coupling
From ERA-Interim to ERA5: the considerable impact of ECMWF's next-generation reanalysis on Lagrangian transport simulations
On the value of reanalyses prior to 1979 for dynamical studies of stratosphere–troposphere coupling
The influence of mixing on the stratospheric age of air changes in the 21st century
Structural changes in the shallow and transition branch of the Brewer–Dobson circulation induced by El Niño
Quantifying the variability of the annular modes: reanalysis uncertainty vs. sampling uncertainty
Response of Arctic ozone to sudden stratospheric warmings
Long-range transport of volcanic aerosol from the 2010 Merapi tropical eruption to Antarctica
Comparison of mean age of air in five reanalyses using the BASCOE transport model
Detection of a climatological short break in the polar night jet in early winter and its relation to cooling over Siberia
No robust evidence of future changes in major stratospheric sudden warmings: a multi-model assessment from CCMI
Sensitivities of modelled water vapour in the lower stratosphere: temperature uncertainty, effects of horizontal transport and small-scale mixing
Surface impacts of the Quasi Biennial Oscillation
Bifurcation of potential vorticity gradients across the Southern Hemisphere stratospheric polar vortex
El Niño Southern Oscillation influence on the Asian summer monsoon anticyclone
A comparison of the momentum budget in reanalysis datasets during sudden stratospheric warming events
A novel method for the extraction of local gravity wave parameters from gridded three-dimensional data: description, validation, and application
Quantifying the effect of mixing on the mean age of air in CCMVal-2 and CCMI-1 models
Radiative effects of ozone waves on the Northern Hemisphere polar vortex and its modulation by the QBO
Nonlinear response of tropical lower-stratospheric temperature and water vapor to ENSO
Extraction of wind and temperature information from hybrid 4D-Var assimilation of stratospheric ozone using NAVGEM
Representation of solar tides in the stratosphere and lower mesosphere in state-of-the-art reanalyses and in satellite observations
Climatology and interannual variability of dynamic variables in multiple reanalyses evaluated by the SPARC Reanalysis Intercomparison Project (S-RIP)
The evolution of zonally asymmetric austral ozone in a chemistry–climate model
Reanalysis comparisons of upper tropospheric–lower stratospheric jets and multiple tropopauses
Comparison of large-scale dynamical variability in the extratropical stratosphere among the JRA-55 family data sets: impacts of assimilation of observational data in JRA-55 reanalysis data
Jessica Oehrlein, Gabriel Chiodo, and Lorenzo M. Polvani
Atmos. Chem. Phys., 20, 10531–10544, https://doi.org/10.5194/acp-20-10531-2020, https://doi.org/10.5194/acp-20-10531-2020, 2020
Short summary
Short summary
Winter winds in the stratosphere 10–50 km above the surface impact climate at the surface. Prior studies suggest that this interaction between the stratosphere and the surface is affected by ozone. We compare two ways of including ozone in computer simulations of climate. One method is more realistic but more expensive. We find that the method of including ozone in simulations affects the surface climate when the stratospheric winds are unusually weak but not when they are unusually strong.
Aurélien Podglajen, Albert Hertzog, Riwal Plougonven, and Bernard Legras
Atmos. Chem. Phys., 20, 9331–9350, https://doi.org/10.5194/acp-20-9331-2020, https://doi.org/10.5194/acp-20-9331-2020, 2020
Short summary
Short summary
Thanks to the increase in resolution, numerical weather prediction models resolve a growing fraction of the gravity wave (GW) spectrum. Here, we assess the representation of Lagrangian GW fluctuations by comparing trajectories in the models to long-duration balloon observations. Most characteristics of the observed GW spectrum, such as near-inertial oscillations, are qualitatively present. However, the variability remains underestimated, emphasizing the continuous need for GW parameterizations.
Yoshio Kawatani, Toshihiko Hirooka, Kevin Hamilton, Anne K. Smith, and Masatomo Fujiwara
Atmos. Chem. Phys., 20, 9115–9133, https://doi.org/10.5194/acp-20-9115-2020, https://doi.org/10.5194/acp-20-9115-2020, 2020
Short summary
Short summary
This paper reports on a project to compare the representation of the semiannual oscillation (SAO) among six major global atmospheric reanalyses and with recent satellite observations. The differences among the zonal mean zonal wind as represented by the various reanalyses display a prominent equatorial maximum that increases with height. It is shown that assimilation of satellite temperature measurements is crucial for the realistic representation of the tropical upper stratospheric circulation.
Marius Hauck, Harald Bönisch, Peter Hoor, Timo Keber, Felix Ploeger, Tanja J. Schuck, and Andreas Engel
Atmos. Chem. Phys., 20, 8763–8785, https://doi.org/10.5194/acp-20-8763-2020, https://doi.org/10.5194/acp-20-8763-2020, 2020
Short summary
Short summary
This study features an extended inversion method that includes transport across the extratropical tropopause to derive age spectra in the lowermost stratosphere from in situ trace gas measurements. The refined method is validated in a model setup and applied to data gained with the HALO research aircraft. Results are congruent with the findings of previous studies so that the method provides a promising toolset for the analysis of stratospheric dynamics based on observations in the future.
Frauke Fritsch, Hella Garny, Andreas Engel, Harald Bönisch, and Roland Eichinger
Atmos. Chem. Phys., 20, 8709–8725, https://doi.org/10.5194/acp-20-8709-2020, https://doi.org/10.5194/acp-20-8709-2020, 2020
Short summary
Short summary
We test two methods to derive age of air as a diagnostic of the Brewer–Dobson circulation from non-linear increasing trace gases such as SF6 using a chemistry-climate model and observations. Both the model and the observations show systematic variation of the age of air trend dependent on the chosen assumptions that are required when deriving age of air from measurements. This provides insight into the differences in age of air trends of observations and models.
Natalia Korhonen, Otto Hyvärinen, Matti Kämäräinen, David S. Richardson, Heikki Järvinen, and Hilppa Gregow
Atmos. Chem. Phys., 20, 8441–8451, https://doi.org/10.5194/acp-20-8441-2020, https://doi.org/10.5194/acp-20-8441-2020, 2020
Short summary
Short summary
Reanalysis data of the strength of the polar vortex is applied in the post-processing of the European Centre for Medium-Range Weather Forecasts (ECMWF) winter surface temperature forecasts for weeks 3–4 and 5–6 over northern Europe. In this way, the skill scores of these forecasts are slightly improved. It is also found that, in cases where the polar vortex was weak at the start of the forecast, the mean skill scores of these forecasts were higher than average.
In-Sun Song, Changsup Lee, Hye-Yeong Chun, Jeong-Han Kim, Geonhwa Jee, Byeong-Gwon Song, and Julio T. Bacmeister
Atmos. Chem. Phys., 20, 7617–7644, https://doi.org/10.5194/acp-20-7617-2020, https://doi.org/10.5194/acp-20-7617-2020, 2020
Short summary
Short summary
A modeling study on the effects of propagation of atmospheric gravity waves is carried out for the 2009 sudden stratospheric warming (SSW) event. It is found that gravity-wave-induced momentum fluxes are significantly affected by horizontal refraction and the Earth's curvature effects. Gravity wave convergence and effects of ray geometry also have some impact. In the evolution of the SSW, significantly enhanced momentum fluxes are likely to change nonlocally nearby large-scale vortex structures.
Marta Abalos, Clara Orbe, Douglas E. Kinnison, David Plummer, Luke D. Oman, Patrick Jöckel, Olaf Morgenstern, Rolando R. Garcia, Guang Zeng, Kane A. Stone, and Martin Dameris
Atmos. Chem. Phys., 20, 6883–6901, https://doi.org/10.5194/acp-20-6883-2020, https://doi.org/10.5194/acp-20-6883-2020, 2020
Short summary
Short summary
A set of state-of-the art chemistry–climate models is used to examine future changes in downward transport from the stratosphere, a key contributor to tropospheric ozone. The acceleration of the stratospheric circulation results in increased stratosphere-to-troposphere transport. In the subtropics, downward advection into the troposphere is enhanced due to climate change. At higher latitudes, the ozone reservoir above the tropopause is enlarged due to the stronger circulation and ozone recovery.
Rostislav Kouznetsov, Mikhail Sofiev, Julius Vira, and Gabriele Stiller
Atmos. Chem. Phys., 20, 5837–5859, https://doi.org/10.5194/acp-20-5837-2020, https://doi.org/10.5194/acp-20-5837-2020, 2020
Short summary
Short summary
Estimates of the age of stratospheric air (AoA), its distribution, and trends, obtained by different experimental methods, differ among each other. AoA derived form MIPAS satellite observations, the richest observational dataset on sulfur hexafluoride (SF6) in the stratosphere, are a clear outlier. With multi-decade simulations of AoA and SF6 in the stratosphere, we show that the origin of the discrepancy is in a methodology of deriving AoA from observations rather than in observational data.
Koji Yamazaki, Tetsu Nakamura, Jinro Ukita, and Kazuhira Hoshi
Atmos. Chem. Phys., 20, 5111–5127, https://doi.org/10.5194/acp-20-5111-2020, https://doi.org/10.5194/acp-20-5111-2020, 2020
Short summary
Short summary
It has been well known that the stratospheric quasi-biennial oscillation (QBO) affects the winter Arctic polar vortex. This relation has been explained through stratospheric processes. We show that a tropospheric process also plays a role, especially in early winter, based on data analysis and numerical simulations. The QBO modifies tropical convection, which affects planetary waves in the midlatitude troposphere, then modulating vertical propagation and the polar vortex.
Maartje Sanne Kuilman, Qiong Zhang, Ming Cai, and Qin Wen
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2019-1169, https://doi.org/10.5194/acp-2019-1169, 2020
Revised manuscript accepted for ACP
Short summary
Short summary
In this study, we quantify the temperature changes in the middle atmosphere due to different feedback processes using a relative new method. We have found that the change due to the increase in CO2 alone, without feedbacks, would be approximately −9 K in the stratosphere and mesosphere. The combined effect of the different feedbacks causes the atmosphere to cool less. The ozone feedback is the most important feedback process, while the cloud, water vapour and albedo are only of minor importance.
Susann Tegtmeier, James Anstey, Sean Davis, Rossana Dragani, Yayoi Harada, Ioana Ivanciu, Robin Pilch Kedzierski, Kirstin Krüger, Bernard Legras, Craig Long, James S. Wang, Krzysztof Wargan, and Jonathon S. Wright
Atmos. Chem. Phys., 20, 753–770, https://doi.org/10.5194/acp-20-753-2020, https://doi.org/10.5194/acp-20-753-2020, 2020
Short summary
Short summary
The tropical tropopause layer is an important atmospheric region right in between the troposphere and the stratosphere. We evaluate the representation of this layer in reanalyses data sets, which create a complete picture of the state of Earth's atmosphere using atmospheric modeling and available observations. The recent reanalyses show realistic temperatures in the tropical tropopause layer. However, where the temperature is lowest, the so-called cold point, the reanalyses are too cold.
Silvia Bucci, Bernard Legras, Pasquale Sellitto, Francesco D'Amato, Silvia Viciani, Alessio Montori, Antonio Chiarugi, Fabrizio Ravegnani, Alexey Ulanovsky, Francesco Cairo, and Fred Stroh
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2019-1053, https://doi.org/10.5194/acp-2019-1053, 2020
Revised manuscript accepted for ACP
Short summary
Short summary
The paper presents and evaluates a transport analysis method to study the convective injection of air in the upper troposphere–lower stratosphere of the Asian monsoon anticyclone region. The approach is thereby used to analyse the trace gas data collected during the StratoClim aircraft campaign. The results showed that fresh convective air can be fastly injected at a high level of the atmosphere (above 17 km) with potential impacts on the stratospheric chemistry of the northern hemisphere.
Xiaolu Yan, Paul Konopka, Felix Ploeger, Aurélien Podglajen, Jonathon S. Wright, Rolf Müller, and Martin Riese
Atmos. Chem. Phys., 19, 15629–15649, https://doi.org/10.5194/acp-19-15629-2019, https://doi.org/10.5194/acp-19-15629-2019, 2019
Short summary
Short summary
The Asian and North American summer monsoons (ASM and NASM) have considerable influence on stratospheric chemistry and physics. More air mass is transported from the monsoon regions to the tropical stratosphere when the tracers are released clearly below the tropopause than when they are released close to the tropopause. Results for different altitudes of air origin reveal two transport pathways (monsoon and tropical) from the upper troposphere over the monsoon regions to the tropical pipe.
Daniel Kunkel, Peter Hoor, Thorsten Kaluza, Jörn Ungermann, Björn Kluschat, Andreas Giez, Hans-Christoph Lachnitt, Martin Kaufmann, and Martin Riese
Atmos. Chem. Phys., 19, 12607–12630, https://doi.org/10.5194/acp-19-12607-2019, https://doi.org/10.5194/acp-19-12607-2019, 2019
Short summary
Short summary
In this study we present a mixing process around the tropopause in extratropical baroclinic waves. We analyze airborne data from a flight during the WISE campaign in autumn 2017 over the North Atlantic. We use idealized experiments to study the mixing process. Although the process occurs on a small geographical scale, it might be of importance due to its relation to a frequent feature of the extratropical UTLS. The process is relevant for STE but is not fully included in climatologies.
Andreas Chrysanthou, Amanda C. Maycock, Martyn P. Chipperfield, Sandip Dhomse, Hella Garny, Douglas Kinnison, Hideharu Akiyoshi, Makoto Deushi, Rolando R. Garcia, Patrick Jöckel, Oliver Kirner, Giovanni Pitari, David A. Plummer, Laura Revell, Eugene Rozanov, Andrea Stenke, Taichu Y. Tanaka, Daniele Visioni, and Yousuke Yamashita
Atmos. Chem. Phys., 19, 11559–11586, https://doi.org/10.5194/acp-19-11559-2019, https://doi.org/10.5194/acp-19-11559-2019, 2019
Short summary
Short summary
We perform the first multi-model comparison of the impact of nudged meteorology on the stratospheric residual circulation (RC) in chemistry–climate models. Nudging meteorology does not constrain the mean strength of RC compared to free-running simulations, and despite the lack of agreement in the mean circulation, nudging tightly constrains the inter-annual variability in the tropical upward mass flux in the lower stratosphere. In summary, nudging strongly affects the representation of RC.
Blanca Ayarzagüena, Froila M. Palmeiro, David Barriopedro, Natalia Calvo, Ulrike Langematz, and Kiyotaka Shibata
Atmos. Chem. Phys., 19, 9469–9484, https://doi.org/10.5194/acp-19-9469-2019, https://doi.org/10.5194/acp-19-9469-2019, 2019
Short summary
Short summary
Sudden stratospheric warmings (SSWs) are abrupt rises in the wintertime polar stratosphere that also affect the troposphere. Their study is hampered by the limited observations in the stratosphere and mostly relies on reanalyses, i.e., models that include observations. Here we compare the representation of SSWs by the most used reanalyses. SSW results are consistent across reanalyses but some differences are found, in particular before the satellite era.
Ohad Harari, Chaim I. Garfinkel, Shlomi Ziskin Ziv, Olaf Morgenstern, Guang Zeng, Simone Tilmes, Douglas Kinnison, Makoto Deushi, Patrick Jöckel, Andrea Pozzer, Fiona M. O'Connor, and Sean Davis
Atmos. Chem. Phys., 19, 9253–9268, https://doi.org/10.5194/acp-19-9253-2019, https://doi.org/10.5194/acp-19-9253-2019, 2019
Short summary
Short summary
Ozone depletion in the Antarctic has been shown to influence surface conditions, but the effects of ozone depletion in the Arctic on surface climate are unclear. We show that Arctic ozone does influence surface climate in both polar regions and tropical regions, though the proximate cause of these surface impacts is not yet clear.
Matthias Nützel, Aurélien Podglajen, Hella Garny, and Felix Ploeger
Atmos. Chem. Phys., 19, 8947–8966, https://doi.org/10.5194/acp-19-8947-2019, https://doi.org/10.5194/acp-19-8947-2019, 2019
Short summary
Short summary
We investigate the transport pathways of water vapour from the upper troposphere in the Asian monsoon region to the stratosphere. In the employed chemistry-transport model we use a tagging method, such that the impact of different source regions on the stratospheric water vapour budget can be quantified. A key finding is that the Asian monsoon (compared to other source regions) is very efficient in transporting air masses and water vapour to the tropical and extratropical stratosphere.
Petr Šácha, Roland Eichinger, Hella Garny, Petr Pišoft, Simone Dietmüller, Laura de la Torre, David A. Plummer, Patrick Jöckel, Olaf Morgenstern, Guang Zeng, Neal Butchart, and Juan A. Añel
Atmos. Chem. Phys., 19, 7627–7647, https://doi.org/10.5194/acp-19-7627-2019, https://doi.org/10.5194/acp-19-7627-2019, 2019
Short summary
Short summary
Climate models robustly project a Brewer–Dobson circulation (BDC) acceleration in the course of climate change. Analyzing mean age of stratospheric air (AoA) from a subset of climate projection simulations, we find a remarkable agreement in simulating the largest AoA trends in the extratropical stratosphere. This is shown to be related with the upward shift of the circulation, resulting in a so-called stratospheric shrinkage, which could be one of the so-far-omitted BDC acceleration drivers.
Thorsten Kaluza, Daniel Kunkel, and Peter Hoor
Atmos. Chem. Phys., 19, 6621–6636, https://doi.org/10.5194/acp-19-6621-2019, https://doi.org/10.5194/acp-19-6621-2019, 2019
Short summary
Short summary
We present a comprehensive mean evolution of the tropopause inversion layer in mid-latitudes, an atmospheric feature that is located in the region that separates the well-mixed troposphere and the stably stratified stratosphere. We counter-intuitively find this region, which is expected to stabilise atmospheric flow, to exhibit favourable conditions for turbulent exchange between troposphere and stratosphere. This is an important result concerning the overall assessment of exchange processes.
Bärbel Vogel, Rolf Müller, Gebhard Günther, Reinhold Spang, Sreeharsha Hanumanthu, Dan Li, Martin Riese, and Gabriele P. Stiller
Atmos. Chem. Phys., 19, 6007–6034, https://doi.org/10.5194/acp-19-6007-2019, https://doi.org/10.5194/acp-19-6007-2019, 2019
Short summary
Short summary
We identified the transport pathways of air masses from the region of the Asian monsoon (e.g. pollution and greenhouse gases caused by increasing population and growing industries in Asia) into the lower stratosphere. Even small changes of the chemical composition of the lower stratosphere have an impact on surface climate (e.g. surface temperatures). Therefore, it is important to identify transport pathways to the stratosphere to allow potential environmental risks to be assessed.
Marius Hauck, Frauke Fritsch, Hella Garny, and Andreas Engel
Atmos. Chem. Phys., 19, 5269–5291, https://doi.org/10.5194/acp-19-5269-2019, https://doi.org/10.5194/acp-19-5269-2019, 2019
Short summary
Short summary
The paper presents a modified method to invert mixing ratios of chemically active tracers into stratospheric age spectra. It features an imposed seasonal cycle to include transport seasonality into the spectra. An idealized set of tracers from a model is used as proof of concept and results are in good agreement with the model reference, except for the lowermost stratosphere. Applicability is studied with focus on number of tracers and error tolerance, providing a starting point for future work.
Marianna Linz, Marta Abalos, Anne Sasha Glanville, Douglas E. Kinnison, Alison Ming, and Jessica L. Neu
Atmos. Chem. Phys., 19, 5069–5090, https://doi.org/10.5194/acp-19-5069-2019, https://doi.org/10.5194/acp-19-5069-2019, 2019
Short summary
Short summary
The stratospheric circulation is important for transporting ozone and water vapor, and models of the stratosphere differ. The metrics used to compare models are inconsistent between studies and cannot be calculated from observational data. In this paper, we explore a metric for the circulation that can be calculated from observations and examine how it relates to the more commonly used metrics. We find substantial differences in the upper and lower stratosphere depending on the choice of metric.
Sabine Haase and Katja Matthes
Atmos. Chem. Phys., 19, 3417–3432, https://doi.org/10.5194/acp-19-3417-2019, https://doi.org/10.5194/acp-19-3417-2019, 2019
Short summary
Short summary
The Antarctic ozone hole influences surface climate in the Southern Hemisphere. Recent studies have shown that stratospheric ozone depletion in the Arctic can also affect the surface. We evaluate the importance of the direct and indirect representation of ozone variability in a climate model for this surface response. We show that allowing feedbacks between ozone chemistry, radiation, and dynamics enhances and prolongs the surface response to Northern Hemisphere spring ozone depletion.
Lars Hoffmann, Gebhard Günther, Dan Li, Olaf Stein, Xue Wu, Sabine Griessbach, Yi Heng, Paul Konopka, Rolf Müller, Bärbel Vogel, and Jonathon S. Wright
Atmos. Chem. Phys., 19, 3097–3124, https://doi.org/10.5194/acp-19-3097-2019, https://doi.org/10.5194/acp-19-3097-2019, 2019
Short summary
Short summary
ECMWF's new ERA5 reanalysis provides higher spatiotemporal resolution, yielding an improved representation of meso- and synoptic-scale features of the atmosphere. We assessed the impact of this challenging new data set on Lagrangian trajectory calculations for the free troposphere and stratosphere. Key findings are considerable transport deviations between the ERA5 and ERA-Interim simulations as well as significantly improved conservation of potential temperature in the stratosphere for ERA5.
Peter Hitchcock
Atmos. Chem. Phys., 19, 2749–2764, https://doi.org/10.5194/acp-19-2749-2019, https://doi.org/10.5194/acp-19-2749-2019, 2019
Short summary
Short summary
Studies of the dynamics of stratosphere–troposphere coupling benefit from long observational records in order to distinguish common dynamical features from unrelated atmospheric variability. On the basis of a comparison between a range of reanalysis products, this study argues that the period from 1958 to 1979 is of significant value in the Northern Hemisphere for this purpose, despite the lack of global satellite records.
Roland Eichinger, Simone Dietmüller, Hella Garny, Petr Šácha, Thomas Birner, Harald Bönisch, Giovanni Pitari, Daniele Visioni, Andrea Stenke, Eugene Rozanov, Laura Revell, David A. Plummer, Patrick Jöckel, Luke Oman, Makoto Deushi, Douglas E. Kinnison, Rolando Garcia, Olaf Morgenstern, Guang Zeng, Kane Adam Stone, and Robyn Schofield
Atmos. Chem. Phys., 19, 921–940, https://doi.org/10.5194/acp-19-921-2019, https://doi.org/10.5194/acp-19-921-2019, 2019
Short summary
Short summary
To shed more light upon the changes in stratospheric circulation in the 21st century, climate projection simulations of 10 state-of-the-art global climate models, spanning from 1960 to 2100, are analyzed. The study shows that in addition to changes in transport, mixing also plays an important role in stratospheric circulation and that the properties of mixing vary over time. Furthermore, the influence of mixing is quantified and a dynamical framework is provided to understand the changes.
Mohamadou Diallo, Paul Konopka, Michelle L. Santee, Rolf Müller, Mengchu Tao, Kaley A. Walker, Bernard Legras, Martin Riese, Manfred Ern, and Felix Ploeger
Atmos. Chem. Phys., 19, 425–446, https://doi.org/10.5194/acp-19-425-2019, https://doi.org/10.5194/acp-19-425-2019, 2019
Short summary
Short summary
This paper assesses the structural changes in the shallow and transition branches of the BDC induced by El Nino using the Lagrangian model simulations driven by ERAi and JRA-55 combined with MLS observations. We found a clear evidence of a weakening of the transition branch due to an upward shift in the dissipation height of the planetary and gravity waves and a strengthening of the shallow branch due to enhanced GW breaking in the tropics–subtropics and PW breaking at high latitudes.
Edwin P. Gerber and Patrick Martineau
Atmos. Chem. Phys., 18, 17099–17117, https://doi.org/10.5194/acp-18-17099-2018, https://doi.org/10.5194/acp-18-17099-2018, 2018
Short summary
Short summary
The annular modes characterize the variability of the extratropical circulation. We show that they are extremely consistent across all reanalyses during the satellite era (1979 onward). Consequently, uncertainty in the annual cycle of variability of the tropospheric jet streams and their coupling with the stratospheric polar vortices is dominated by sampling uncertainty. Pre-satellite reanalysis of the Northern Hemisphere appears to be of high quality and can help reduce this uncertainty.
Alvaro de la Cámara, Marta Abalos, Peter Hitchcock, Natalia Calvo, and Rolando R. Garcia
Atmos. Chem. Phys., 18, 16499–16513, https://doi.org/10.5194/acp-18-16499-2018, https://doi.org/10.5194/acp-18-16499-2018, 2018
Short summary
Short summary
Long chemistry–climate runs are used to investigate the changes that sudden stratospheric warmings (extreme and fast disruptions of the wintertime stratospheric polar vortex) induce on Arctic ozone. Ozone increases rapidly during the onset of the events, driven by deep changes in the stratospheric transport circulation. These anomalies decay slowly, particularly in the lower stratosphere where they can last up to 2 months. Irreversible mixing makes an important contribution to this behavior.
Xue Wu, Sabine Griessbach, and Lars Hoffmann
Atmos. Chem. Phys., 18, 15859–15877, https://doi.org/10.5194/acp-18-15859-2018, https://doi.org/10.5194/acp-18-15859-2018, 2018
Short summary
Short summary
Volcanic aerosol is an important source of sulfur for Antarctica, where local sources of sulfur are rare. Midlatitude and high-latitude volcanism can directly influence the aerosol budget of the polar stratosphere, but tropical volcanic eruptions can also enhance polar aerosols by transport. Our study investigates pathway and transport processes of volcanic aerosol from the tropics to the lower stratosphere over Antarctica by combining Lagrangian transport simulation and satellite observations.
Simon Chabrillat, Corinne Vigouroux, Yves Christophe, Andreas Engel, Quentin Errera, Daniele Minganti, Beatriz M. Monge-Sanz, Arjo Segers, and Emmanuel Mahieu
Atmos. Chem. Phys., 18, 14715–14735, https://doi.org/10.5194/acp-18-14715-2018, https://doi.org/10.5194/acp-18-14715-2018, 2018
Short summary
Short summary
Mean age of stratospheric air is computed for the period 1989–2015 with a kinematic transport model which uses surface pressure and wind fields from five reanalyses: ERA-I, MERRA-2, MERRA, CFSR, JRA-55. The spread between the resulting datasets is as large as in climate model intercomparisons; the age trends have large disagreement and depend strongly on the considered period. We highlight the need for similar studies using diabatic transport models which also use temperature and heating rates.
Yuta Ando, Koji Yamazaki, Yoshihiro Tachibana, Masayo Ogi, and Jinro Ukita
Atmos. Chem. Phys., 18, 12639–12661, https://doi.org/10.5194/acp-18-12639-2018, https://doi.org/10.5194/acp-18-12639-2018, 2018
Short summary
Short summary
We found the climatological strong stratospheric westerly circumpolar wind stops increasing temporarily during November, when the upward propagation of large-scale atmospheric waves from the troposphere increases. The propagation of atmospheric waves, which is strongest over Siberia, is related to strengthening of the low pressure. Longitudinally asymmetric forcing by land–sea heating contrasts caused by their different heat capacities might cause the strengthening of the low pressure.
Blanca Ayarzagüena, Lorenzo M. Polvani, Ulrike Langematz, Hideharu Akiyoshi, Slimane Bekki, Neal Butchart, Martin Dameris, Makoto Deushi, Steven C. Hardiman, Patrick Jöckel, Andrew Klekociuk, Marion Marchand, Martine Michou, Olaf Morgenstern, Fiona M. O'Connor, Luke D. Oman, David A. Plummer, Laura Revell, Eugene Rozanov, David Saint-Martin, John Scinocca, Andrea Stenke, Kane Stone, Yousuke Yamashita, Kohei Yoshida, and Guang Zeng
Atmos. Chem. Phys., 18, 11277–11287, https://doi.org/10.5194/acp-18-11277-2018, https://doi.org/10.5194/acp-18-11277-2018, 2018
Short summary
Short summary
Stratospheric sudden warmings (SSWs) are natural major disruptions of the polar stratospheric circulation that also affect surface weather. In the literature there are conflicting claims as to whether SSWs will change in the future. The confusion comes from studies using different models and methods. Here we settle the question by analysing 12 models with a consistent methodology, to show that no robust changes in frequency and other features are expected over the 21st century.
Liubov Poshyvailo, Rolf Müller, Paul Konopka, Gebhard Günther, Martin Riese, Aurélien Podglajen, and Felix Ploeger
Atmos. Chem. Phys., 18, 8505–8527, https://doi.org/10.5194/acp-18-8505-2018, https://doi.org/10.5194/acp-18-8505-2018, 2018
Short summary
Short summary
Water vapour (H2O) in the UTLS is a key player for global radiation, which is critical for predictions of future climate change. We investigate the effects of current uncertainties in tropopause temperature, horizontal transport and small-scale mixing on simulated H2O, using the Chemical Lagrangian Model of the Stratosphere. Our sensitivity studies provide new insights into the leading processes controlling stratospheric H2O, important for assessing and improving climate model projections.
Lesley J. Gray, James A. Anstey, Yoshio Kawatani, Hua Lu, Scott Osprey, and Verena Schenzinger
Atmos. Chem. Phys., 18, 8227–8247, https://doi.org/10.5194/acp-18-8227-2018, https://doi.org/10.5194/acp-18-8227-2018, 2018
Short summary
Short summary
A major phenomenon in the stratosphere is the Quasi Biennial Oscillation (QBO). Although a feature of the equatorial stratosphere, its influence extends to surface weather at both equatorial and mid latitudes. Improved knowledge of mechanisms of influence should help to improve weather forecasts. In this paper, QBO impacts at the surface are characterized and dominant mechanisms explored. Three pathways are identified, referred to as the tropical, subtropical and polar routes.
Jonathan Conway, Greg Bodeker, and Chris Cameron
Atmos. Chem. Phys., 18, 8065–8077, https://doi.org/10.5194/acp-18-8065-2018, https://doi.org/10.5194/acp-18-8065-2018, 2018
Short summary
Short summary
Strong westerly winds occur in the stratosphere during winter and spring. These winds, the polar vortex, limit how much air is mixed between mid- and high-latitudes. We present a new view of the polar vortex mixing barrier in the Southern Hemisphere, revealing a frequent double-walled barrier with two distinct regions of weak mixing. This double-walled structure is expected to alter the spatial and temporal variation of trace gas concentrations (e.g. ozone) across the polar vortex.
Xiaolu Yan, Paul Konopka, Felix Ploeger, Mengchu Tao, Rolf Müller, Michelle L. Santee, Jianchun Bian, and Martin Riese
Atmos. Chem. Phys., 18, 8079–8096, https://doi.org/10.5194/acp-18-8079-2018, https://doi.org/10.5194/acp-18-8079-2018, 2018
Short summary
Short summary
Many works investigate the impact of ENSO on the troposphere. However, only a few works check the impact of ENSO at higher altitudes.
Here, we analyse the impact of ENSO on the vicinity of the tropopause using reanalysis, satellite, in situ and model data. We find that ENSO shows the strongest signal in winter, but its impact can last until early the next summer. The ENSO anomaly is insignificant in late summer. Our study can help to understand the atmosphere propagation after ENSO.
Patrick Martineau, Seok-Woo Son, Masakazu Taguchi, and Amy H. Butler
Atmos. Chem. Phys., 18, 7169–7187, https://doi.org/10.5194/acp-18-7169-2018, https://doi.org/10.5194/acp-18-7169-2018, 2018
Short summary
Short summary
This study evaluates the agreement between eight reanalysis datasets by comparing zonal-mean zonal winds and the forcing terms of the zonal-mean momentum equation during sudden stratospheric warming events. Results show that the spread between datasets increases exponentially with height and is largest during the most intense sudden stratospheric warming events. The largest uncertainties arise from differences in the mean meridional circulation and horizontal fluxes of momentum by eddies.
Lena Schoon and Christoph Zülicke
Atmos. Chem. Phys., 18, 6971–6983, https://doi.org/10.5194/acp-18-6971-2018, https://doi.org/10.5194/acp-18-6971-2018, 2018
Short summary
Short summary
Different kinds of waves are the subject of intense research because they are suspected to steer several different atmospheric phenomena.
To analyse the effects of waves, wave packet characteristics have to be known. We introduce a new tool to study wave packets locally:
Unified Wave Diagnostics (UWaDi). To show the advantages of UWaDi, a sudden stratospheric warming period in 2016 is analysed for different
background wind conditions, revealing gravity waves emitted from a jet exit region.
Simone Dietmüller, Roland Eichinger, Hella Garny, Thomas Birner, Harald Boenisch, Giovanni Pitari, Eva Mancini, Daniele Visioni, Andrea Stenke, Laura Revell, Eugene Rozanov, David A. Plummer, John Scinocca, Patrick Jöckel, Luke Oman, Makoto Deushi, Shibata Kiyotaka, Douglas E. Kinnison, Rolando Garcia, Olaf Morgenstern, Guang Zeng, Kane Adam Stone, and Robyn Schofield
Atmos. Chem. Phys., 18, 6699–6720, https://doi.org/10.5194/acp-18-6699-2018, https://doi.org/10.5194/acp-18-6699-2018, 2018
Vered Silverman, Nili Harnik, Katja Matthes, Sandro W. Lubis, and Sebastian Wahl
Atmos. Chem. Phys., 18, 6637–6659, https://doi.org/10.5194/acp-18-6637-2018, https://doi.org/10.5194/acp-18-6637-2018, 2018
Short summary
Short summary
This study provides a quantified and mechanistic understanding of the radiative effects of ozone waves on the NH stratosphere. In particular, we find these effects to influence the seasonal evolution of the midlatitude QBO signal (Holton–Tan effect), which is important for getting realistic dynamical interactions in climate models. We also provide a synoptic view on the evolution of the seasonal development of the Holton–Tan effect by looking at the life cycle of upward-propagating waves.
Chaim I. Garfinkel, Amit Gordon, Luke D. Oman, Feng Li, Sean Davis, and Steven Pawson
Atmos. Chem. Phys., 18, 4597–4615, https://doi.org/10.5194/acp-18-4597-2018, https://doi.org/10.5194/acp-18-4597-2018, 2018
Short summary
Short summary
The impact of El Niño in the lower stratosphere is nonlinear in spring. While moderate El Niño events lead to cooling in this region,
strong El Niño events appear to lead to warming, and hence the water vapor response is nonlinear too. The net effect is that strong
El Nino events, such as in 1997/1998 and 2015/2016, lead to qualitatively different water vapor impacts as compared to moderate
El Nino events.
Douglas R. Allen, Karl W. Hoppel, and David D. Kuhl
Atmos. Chem. Phys., 18, 2999–3026, https://doi.org/10.5194/acp-18-2999-2018, https://doi.org/10.5194/acp-18-2999-2018, 2018
Short summary
Short summary
This study examines whether ozone data in the stratosphere (10–50 km altitude) can be used to benefit weather forecasts. The approach involves creating simulated ozone data and assimilating these into the US Navy's global weather model. Key findings are that assimilation of dense and accurate ozone data markedly benefits winds and temperature. However, the benefit is small when realistic ozone data are assimilated along with currently available microwave and infrared sounding measurements.
Takatoshi Sakazaki, Masatomo Fujiwara, and Masato Shiotani
Atmos. Chem. Phys., 18, 1437–1456, https://doi.org/10.5194/acp-18-1437-2018, https://doi.org/10.5194/acp-18-1437-2018, 2018
Short summary
Short summary
Atmospheric solar tides in the stratosphere and lower mesosphere are examined using temperature data from five reanalyses and satellite measurements. The reanalyses agree reasonably well with each other and with the satellite observations, but the agreement among the reanalyses is weaker in the mesosphere. The assimilation of satellite data improves the representation of tides in the reanalyses, while long-term changes are mostly artificial and driven by changes in the input data employed.
Craig S. Long, Masatomo Fujiwara, Sean Davis, Daniel M. Mitchell, and Corwin J. Wright
Atmos. Chem. Phys., 17, 14593–14629, https://doi.org/10.5194/acp-17-14593-2017, https://doi.org/10.5194/acp-17-14593-2017, 2017
Short summary
Short summary
As part of the SPARC Reanalysis Intercomparison Project, we evaluate the temperature and wind structure of all the recent and past reanalyses with 2.5-degree monthly zonal mean data sets from 1979–2014. There is a distinct change in the temperature structure in the stratosphere in 1998. Zonal winds are in greater agreement than temperatures. All reanalyses have issues analysing the tropical stratospheric winds. Caution is advised for using reanalysis temperatures for trend detection.
Fraser Dennison, Adrian McDonald, and Olaf Morgenstern
Atmos. Chem. Phys., 17, 14075–14084, https://doi.org/10.5194/acp-17-14075-2017, https://doi.org/10.5194/acp-17-14075-2017, 2017
Short summary
Short summary
The Antarctic ozone is not centred directly over the pole. In this research we examine how the position and shape of the ozone hole changes using a chemistry–climate model. As ozone becomes increasingly depleted during the late 20th century the centre of the ozone hole moves toward the west and becomes more circular. As the ozone hole recovers over the course of the 21st century the ozone hole moves back towards the east.
Gloria L. Manney, Michaela I. Hegglin, Zachary D. Lawrence, Krzysztof Wargan, Luis F. Millán, Michael J. Schwartz, Michelle L. Santee, Alyn Lambert, Steven Pawson, Brian W. Knosp, Ryan A. Fuller, and William H. Daffer
Atmos. Chem. Phys., 17, 11541–11566, https://doi.org/10.5194/acp-17-11541-2017, https://doi.org/10.5194/acp-17-11541-2017, 2017
Short summary
Short summary
The upper tropospheric–lower stratospheric (UTLS) jet stream and multiple tropopause distributions are compared among five state-of-the-art reanalyses. The reanalyses show very similar global distributions of UTLS jets, reflecting their overall high quality; slightly larger differences are seen in tropopause characteristics. Regional and seasonal differences, albeit small, may have implications for using these reanalyses for quantitative dynamical and transport studies focusing on the UTLS.
Masakazu Taguchi
Atmos. Chem. Phys., 17, 11193–11207, https://doi.org/10.5194/acp-17-11193-2017, https://doi.org/10.5194/acp-17-11193-2017, 2017
Short summary
Short summary
This study explores dynamical variability of the polar vortex in the stratosphere among the Japanese 55-year Reanalysis family data. Results show that the assimilation of conventional (surface and balloon) observations increases the dynamical variability as the vortex in the model is more quiescent without the assimilation. The assimilation of satellite data in addition to the conventional data strengthens and/or advances some vortex weakening events, although the impacts appear in various ways.
Cited articles
Abalos, M., Randel, W. J., Kinnison, D. E., and Serrano, E.: Quantifying tracer transport in the tropical lower stratosphere using WACCM, Atmos. Chem. Phys., 13, 10591–10607, https://doi.org/10.5194/acp-13-10591-2013, 2013.
Abalos, M., Legras, B., Ploeger, F., and Randel, W. J.: Evaluating the advective Brewer–Dobson circulation in three reanalyses for the period 1979–2012, J. Geophys. Res.-Atmos., 120, 7534–7554, 2015.
Andrews, A., Boering, K., Daube, B., Wofsy, S., Loewenstein, M., Jost, H., Podolske, J., Webster, C., Herman, R., Scott, D. C., Flesch, G. J., Moyer, E. J., Elkins, J. W., Dutton, G. S., Hurst, D. F., Moore, F. L., Ray, E. A., Romashkin, P. A., and Strahan, S. E.: Mean ages of stratospheric air derived from in situ observations of CO2, CH4, and N2O, J. Geophys. Res.-Atmos., 106, 32295–32314, 2001.
Andrews, D. G., Holton, J. R., and Leovy, C. B.: Middle atmosphere dynamics, vol. 40, Academic press, San Diego, California, USA, 1987.
Birner, T. and Bönisch, H.: Residual circulation trajectories and transit times into the extratropical lowermost stratosphere, Atmos. Chem. Phys., 11, 817–827, https://doi.org/10.5194/acp-11-817-2011, 2011.
Brinkop, S. and Roeckner, E.: Sensitivity of a general circulation model to parameterizations of cloud–turbulence interactions in the atmospheric boundary layer, Tellus A, 47, 197–220, 1995.
Butchart, N.: The Brewer–Dobson circulation, Rev. Geophys., 52, 157–184, https://doi.org/10.1002/2013RG000448, 2014.
Butchart, N., Cionni, I., Eyring, V., Shepherd, T., Waugh, D., Akiyoshi, H., Austin, J., Brühl, C., Chipperfield, M., Cordero, E., Dameris, M., Deckert, R., Dhomse, S., Frith, S. M., Garcia, R. R., Gettelman, A., Giorgetta, M. A., Kinnison, D. E., Li, F., Mancini, E., McLandress, C., Pawson, S., Pitari, G., Plummer, D. A., Rozanov, E., Sassi, F., Scinocca, J. F., Shibata, K., Steil, B., and Tian, W.: Chemistry-climate model simulations of twenty-first century stratospheric climate and circulation changes, J. Climate, 23, 5349–5374, 2010.
Dee, D., Uppala, S., Simmons, A., Berrisford, P., Poli, P., Kobayashi, S., Andrae, U., Balmaseda, M., Balsamo, G., Bauer, P., Bechtold, P., Beljaars, A. C. M., van de Berg, L., Bidlot, J., Bormann, N., Delsol, C., Dragani, R., Fuentes, M., Geer, A. J., Haimberger, L., Healy, S. B., Hersbach, H., Hólm, E. V., Isaksen, L., Kallberg, P., Köhler, M., Matricardi, M., McNally, A. P., Monge-Sanz, B. M., Morcrette, J.-J., Park, B.-K., Peubey, C., de Rosnay, P., Tavolato, C., Thépaut, J.-N., and Vitart, F.: The ERA-Interim reanalysis: Configuration and performance of the data assimilation system, Q. J. Roy. Meteor. Soc., 137, 553–597, 2011.
Diallo, M., Legras, B., and Chédin, A.: Age of stratospheric air in the ERA-Interim, Atmos. Chem. Phys., 12, 12133–12154, https://doi.org/10.5194/acp-12-12133-2012, 2012.
Eluszkiewicz, J., Hemler, R. S., Mahlman, J. D., Bruhwiler, L., and Takacs, L. L.: Sensitivity of age-of-air calculations to the choice of advection scheme, J. Atmos. Sci., 57, 3185–3201, 2000.
Engel, A., Möbius, T., Bönisch, H., Schmidt, U., Heinz, R., Levin, I., Atlas, E., Aoki, S., Nakazawa, T., Sugawara, S., Moore, F., Hurst, D., Elkins, J., Schauffler, S., Andrews, A., and Boering, A.: Age of stratospheric air unchanged within uncertainties over the past 30 years, Nat. Geosci., 2, 28–31, 2009.
Eyring, V., Butchart, N., Waugh, D. W., Akiyoshi, H., Austin, J., Bekki, S., Bodeker, G. E., Boville, B. A., Brühl, C., Chipperfield, M. P., Cordero, E., Dameris, M., Deushi, M., Fioletov, V. E., Frith, S. M., Garcia, R. R., Gettelman, A., Giorgetta, M. A., Grewe, V., Jourdain, L., Kinnison, D. E., Mancini, E., Manzini, E., Marchand, M., Marsh, D. R., Nagashima, T., Newman, P. A., Nielsen, J. E., Pawson, S., Pitari, G., Plummer, D. A., Rozanov, E., Schraner, M., Shepherd, T. G., Shibata, K., Stolarski, R. S., Struthers, H., Tian, W., and Yoshiki, M.: Assessment of temperature, trace species, and ozone in chemistry-climate model simulations of the recent past, J. Geophys. Res.-Atmos., 111, D22308, https://doi.org/10.1029/2006JD007327, 2006.
Eyring, V., Lamarque, J.-F., Hess, P., Arfeuille, F., Bowman, K., Chipperfield, M., Duncan, B., Fiore, A., Gettelman, A., Giorgetta, M., Granier, C., Hegglin, M., Kinnison, D., Kunze, M., Langematz, U., Luo, B., Martin, R., Matthes, K., Newman, P., Peter, T., Robock, A., Ryerson, A., Saiz-Lopez, A., Salawitch, R., Schultz, M., Shepherd, T., Shindell, D., Stähelin, J., Tegtmeier, S., Thomason, L., Tilmes, S., Vernier, J.-P., Waugh, D., and Young, P.: Overview of IGAC/SPARC Chemistry-Climate Model Initiative (CCMI) Community Simulations in Support of Upcoming Ozone and Climate Assessments, SPARC newsletter, SPARC Office, Zurich, Switzerland, 48–66, 2013.
Garcia, R. R. and Randel, W. J.: Acceleration of the Brewer–Dobson circulation due to increases in greenhouse gases, J. Atmos. Sci., 65, 2731–2739, 2008.
Garcia, R. R., Randel, W. J., and Kinnison, D. E.: On the determination of age of air trends from atmospheric trace species, J. Atmos. Sci., 68, 139–154, 2011.
Garny, H., Birner, T., Bönisch, H., and Bunzel, F.: The effects of mixing on age of air, J. Geophys. Res.-Atmos., 119, 7015–7034, 2014.
Hall, T. M. and Plumb, R. A.: Age as a diagnostic of stratospheric transport, J. Geophys. Res.-Atmos., 99, 1059–1070, 1994.
Hall, T. M., Waugh, D. W., Boering, K. A., and Plumb, R. A.: Evaluation of transport in stratospheric models, J. Geophys. Res.-Atmos., 104, 18815–18839, 1999.
Hoppe, C. M., Hoffmann, L., Konopka, P., Grooß, J.-U., Ploeger, F., Günther, G., Jöckel, P., and Müller, R.: The implementation of the CLaMS Lagrangian transport core into the chemistry climate model EMAC 2.40.1: application on age of air and transport of long-lived trace species, Geosci. Model Dev., 7, 2639–2651, https://doi.org/10.5194/gmd-7-2639-2014, 2014.
Hoppe, C. M., Ploeger, F., Konopka, P., and Müller, R.: Kinematic and diabatic vertical velocity climatologies from a chemistry climate model, Atmos. Chem. Phys., 16, 6223–6239, https://doi.org/10.5194/acp-16-6223-2016, 2016.
Jöckel, P., Kerkweg, A., Buchholz-Dietsch, J., Tost, H., Sander, R., and Pozzer, A.: Technical Note: Coupling of chemical processes with the Modular Earth Submodel System (MESSy) submodel TRACER, Atmos. Chem. Phys., 8, 1677–1687, https://doi.org/10.5194/acp-8-1677-2008, 2008.
Jöckel, P., Kerkweg, A., Pozzer, A., Sander, R., Tost, H., Riede, H., Baumgaertner, A., Gromov, S., and Kern, B.: Development cycle 2 of the Modular Earth Submodel System (MESSy2), Geosci. Model Dev., 3, 717–752, https://doi.org/10.5194/gmd-3-717-2010, 2010.
Jöckel, P., Tost, H., Pozzer, A., Kunze, M., Kirner, O., Brenninkmeijer, C. A. M., Brinkop, S., Cai, D. S., Dyroff, C., Eckstein, J., Frank, F., Garny, H., Gottschaldt, K.-D., Graf, P., Grewe, V., Kerkweg, A., Kern, B., Matthes, S., Mertens, M., Meul, S., Neumaier, M., Nützel, M., Oberländer-Hayn, S., Ruhnke, R., Runde, T., Sander, R., Scharffe, D., and Zahn, A.: Earth System Chemistry integrated Modelling (ESCiMo) with the Modular Earth Submodel System (MESSy) version 2.51, Geosci. Model Dev., 9, 1153–1200, https://doi.org/10.5194/gmd-9-1153-2016, 2016.
Konopka, P., Steinhorst, H.-M., Grooß, J.-U., Günther, G., Müller, R., Elkins, J. W., Jost, H.-J., Richard, E., Schmidt, U., Toon, G., and McKenna, D. S.: Mixing and ozone loss in the 1999–2000 Arctic vortex: Simulations with the three-dimensional Chemical Lagrangian Model of the Stratosphere (CLaMS), J. Geophys. Res.-Atmos., 109, D02315, https://doi.org/10.1029/2003JD003792, 2004.
Lauritzen, P. H., Mirin, A. A., Truesdale, J., Raeder, K., Anderson, J. L., Bacmeister, J., and Neale, R. B.: Implementation of new diffusion/filtering operators in the CAM-FV dynamical core, Int. J. High Perform. C., 26, 63–73, https://doi.org/10.1177/1094342011410088, 2011.
Lin, S.-J.: A vertically Lagrangian finite-volume dynamical core for global models, Mon. Weather Rev., 132, 2293–2307, 2004.
Lin, S. J. and Rood, R. B.: Multidimensional flux-form semi-Lagrangian transport schemes, Mon. Weather Rev., 124, 2046–2070, 1996.
Mahowald, N. M., Plumb, R. A., Rasch, P. J., del Corral, J., Sassi, F., and Heres, W.: Stratospheric transport in a three-dimensional isentropic coordinate model, J. Geophys. Res.-Atmos., 107, ACH 3-1–ACH 3-14, https://doi.org/10.1029/2001JD001313, 2002.
Monge-Sanz, B., Chipperfield, M., Dee, D., Simmons, A., and Uppala, S.: Improvements in the stratospheric transport achieved by a chemistry transport model with ECMWF (re) analyses: Identifying effects and remaining challenges, Q. J. Roy. Meteor. Soc., 139, 654–673, 2013.
Neu, J. L. and Plumb, R. A.: Age of air in a leaky pipe model of stratospheric transport, J. Geophys. Res.-Atmos., 104, 19243–19255, 1999.
Ploeger, F., Abalos, M., Birner, T., Konopka, P., Legras, B., Müller, R., and Riese, M.: Quantifying the effects of mixing and residual circulation on trends of stratospheric mean age of air, Geophys. Res. Lett., 42, 2047–2054, https://doi.org/10.1002/2014GL062927, 2015a.
Ploeger, F., Riese, M., Haenel, F., Konopka, P., Müller, R., and Stiller, G.: Variability of stratospheric mean age of air and of the local effects of residual circulation and eddy mixing, J. Geophys. Res.-Atmos., 120, 716–733, https://doi.org/10.1002/2014JD022468, 2015b.
Plumb, R.: Stratospheric transport, J. Meteorol. Soc. Jpn., 80, 793–809, 2002.
Pommrich, R., Müller, R., Grooß, J.-U., Konopka, P., Ploeger, F., Vogel, B., Tao, M., Hoppe, C. M., Günther, G., Spelten, N., Hoffmann, L., Pumphrey, H.-C., Viciani, S., D'Amato, F., Volk, C. M., Hoor, P., Schlager, H., and Riese, M.: Tropical troposphere to stratosphere transport of carbon monoxide and long-lived trace species in the Chemical Lagrangian Model of the Stratosphere (CLaMS), Geosci. Model Dev., 7, 2895–2916, https://doi.org/10.5194/gmd-7-2895-2014, 2014.
Ray, E. A., Moore, F. L., Rosenlof, K. H., Davis, S. M., Sweeney, C., Tans, P., Wang, T., Elkins, J. W., Bönisch, H., Engel, A., Sugawara, S., Nakazawa, T., and Aoki, S.: Improving stratospheric transport trend analysis based on SF6 and CO2 measurements, J. Geophys. Res.-Atmos., 119, 14110–14128, https://doi.org/10.1002/2014JD021802, 2014.
Righi, M., Eyring, V., Gottschaldt, K.-D., Klinger, C., Frank, F., Jöckel, P., and Cionni, I.: Quantitative evaluation of ozone and selected climate parameters in a set of EMAC simulations, Geosci. Model Dev., 8, 733–768, https://doi.org/10.5194/gmd-8-733-2015, 2015.
Roeckner, E., Brokopf, R., Esch, M., Giorgetta, M., Hagemann, S., Kornblueh, L., Manzini, E., Schlese, U., and Schulzweida, U.: Sensitivity of simulated climate to horizontal and vertical resolution in the ECHAM5 atmosphere model, J. Climate, 19, 3771–3791, 2006.
Shepherd, T. G.: Transport in the middle atmosphere, J. Meteorol. Soc. Jpn., 85, 165–191, 2007.
SPARC CCMVal: SPARC Report No 5 (2010) Chemistry-Climate Model Validation, WCRP-132, WMO/TD-No. 1526, available at: http://www.atmosp.physics.utoronto.ca/SPARC (last access: 20 May 2017), 2010.
Stiller, G. P., von Clarmann, T., Haenel, F., Funke, B., Glatthor, N., Grabowski, U., Kellmann, S., Kiefer, M., Linden, A., Lossow, S., and López-Puertas, M.: Observed temporal evolution of global mean age of stratospheric air for the 2002 to 2010 period, Atmos. Chem. Phys., 12, 3311–3331, https://doi.org/10.5194/acp-12-3311-2012, 2012.
Thompson, D. W. and Solomon, S.: Interpretation of recent Southern Hemisphere climate change, Science, 296, 895–899, 2002.
Waugh, D. and Hall, T.: Age of stratospheric air: Theory, observations, and models, Rev. Geophys., 40, 1010, https://doi.org/10.1029/2000RG000101, 2002.
Atmospheric Chemistry and Physics
An interactive open-access journal of the European Geosciences Union
All site content, except where otherwise noted, is licensed under the Creative Commons Attribution 4.0 License.