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Atmospheric Chemistry and Physics
An interactive open-access journal of the European Geosciences Union
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- Editorial board
- Articles
- Special issues
- Highlight articles
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- Subscribe to alerts
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IF5.414
IF 5-year
5.958
5.958
CiteScore
9.7
9.7
SNIP1.517
IPP5.61
SJR2.601
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index191
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Abstracted/indexed
Volume 16, issue 13
Atmos. Chem. Phys., 16, 8609–8642, 2016
https://doi.org/10.5194/acp-16-8609-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-8609-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
Special issue: CHemistry and AeRosols Mediterranean EXperiments (ChArMEx)...
Atmos. Chem. Phys., 16, 8609–8642, 2016
https://doi.org/10.5194/acp-16-8609-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-8609-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
Research article 15 Jul 2016
Research article | 15 Jul 2016
Mediterranean intense desert dust outbreaks and their vertical structure based on remote sensing data
Antonis Gkikas et al.
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Antonis Gkikas, Emmanouil Proestakis, Vassilis Amiridis, Stelios Kazadzis, Enza Di Tomaso, Alexandra Tsekeri, Eleni Marinou, Nikos Hatzianastassiou, and Carlos Pérez García-Pando
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-222, https://doi.org/10.5194/amt-2020-222, 2020
Preprint under review for AMT
Short summary
Short summary
We present the development of the MIDAS (ModIs Dust AeroSol) dataset providing daily dust optical depth (DOD at 550 nm) at global scale and fine spatial resolution (0.1° x 0.1°) over a decade (2007-2016). It has been developed via the synergy of MODIS-Aqua and MERRA-2 data while CALIOP and AERONET retrievals are used for its assessment. MIDAS upgrades existing dust observational capabilities and it is suitable for dust climatological studies, model evaluation and data assimilation.
Christine Aebi, Julian Gröbner, Stelios Kazadzis, Laurent Vuilleumier, Antonis Gkikas, and Niklaus Kämpfer
Atmos. Meas. Tech., 13, 907–923, https://doi.org/10.5194/amt-13-907-2020, https://doi.org/10.5194/amt-13-907-2020, 2020
Short summary
Short summary
Clouds are one of the largest sources of uncertainties in climate models. The current study estimates the cloud optical thickness (COT), the effective droplet radius and the single scattering albedo of stratus–altostratus and cirrus–cirrostratus clouds in Payerne, Switzerland, by combining ground- and satellite-based measurements and radiative transfer models. The estimated values are thereafter compared with data retrieved from other methods. The mean COT is distinct for different seasons.
new blackfor smoke?
Anna Gialitaki, Alexandra Tsekeri, Vassilis Amiridis, Romain Ceolato, Lucas Paulien, Anna Kampouri, Antonis Gkikas, Stavros Solomos, Eleni Marinou, Moritz Haarig, Holger Baars, Albert Ansmann, Tatyana Lapyonok, Anton Lopatin, Oleg Dubovik, Silke Groß, Martin Wirth, and Dimitris Balis
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-22, https://doi.org/10.5194/acp-2020-22, 2020
Revised manuscript accepted for ACP
Short summary
Short summary
Smoke particles injected into the stratosphere are find to significantly depolarize the incident light while this effect is also accompanied by a strong spectral dependence. Here we utilize scattering simulations to show that this behavior can be attributed to the near-spherical shape of stratospheric smoke which can produce both the non-typical values and wavelength dependence of smoke depolarization. This was not feasible when assuming more complicated morphologies for the smoke particles.
Antonis Gkikas, Vincenzo Obiso, Carlos Pérez García-Pando, Oriol Jorba, Nikos Hatzianastassiou, Lluis Vendrell, Sara Basart, Stavros Solomos, Santiago Gassó, and José Maria Baldasano
Atmos. Chem. Phys., 18, 8757–8787, https://doi.org/10.5194/acp-18-8757-2018, https://doi.org/10.5194/acp-18-8757-2018, 2018
Short summary
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The present study investigates the direct radiative effects (DREs), induced during 20 intense Mediterranean desert dust outbreaks, based on regional short-term numerical simulations of the NMMB-MONARCH model: more specifically, (i) the DREs and their associated impacts on temperature and surface sensible and latent heat fluxes, (ii) the feedbacks on dust AOD and dust emissions, and (iii) the possible improvements in short-term forecasts (up to 84 h) of temperature and radiation.
M. B. Korras-Carraca, N. Hatzianastassiou, C. Matsoukas, A. Gkikas, and C. D. Papadimas
Atmos. Chem. Phys., 15, 13113–13132, https://doi.org/10.5194/acp-15-13113-2015, https://doi.org/10.5194/acp-15-13113-2015, 2015
M. Taylor, S. Kazadzis, A. Tsekeri, A. Gkikas, and V. Amiridis
Atmos. Meas. Tech., 7, 3151–3175, https://doi.org/10.5194/amt-7-3151-2014, https://doi.org/10.5194/amt-7-3151-2014, 2014
V. Amiridis, U. Wandinger, E. Marinou, E. Giannakaki, A. Tsekeri, S. Basart, S. Kazadzis, A. Gkikas, M. Taylor, J. Baldasano, and A. Ansmann
Atmos. Chem. Phys., 13, 12089–12106, https://doi.org/10.5194/acp-13-12089-2013, https://doi.org/10.5194/acp-13-12089-2013, 2013
A. Gkikas, N. Hatzianastassiou, N. Mihalopoulos, V. Katsoulis, S. Kazadzis, J. Pey, X. Querol, and O. Torres
Atmos. Chem. Phys., 13, 12135–12154, https://doi.org/10.5194/acp-13-12135-2013, https://doi.org/10.5194/acp-13-12135-2013, 2013
Nikolaos Papagiannopoulos, Giuseppe D'Amico, Anna Gialitaki, Nicolae Ajtai, Lucas Alados-Arboledas, Aldo Amodeo, Vassilis Amiridis, Holger Baars, Dimitris Balis, Ioannis Binietoglou, Adolfo Comerón, Davide Dionisi, Alfredo Falconieri, Patrick Fréville, Anna Kampouri, Ina Mattis, Zoran Mijić, Francisco Molero, Alex Papayannis, Gelsomina Pappalardo, Alejandro Rodríguez-Gómez, Stavros Solomos, and Lucia Mona
Atmos. Chem. Phys., 20, 10775–10789, https://doi.org/10.5194/acp-20-10775-2020, https://doi.org/10.5194/acp-20-10775-2020, 2020
Short summary
Short summary
Volcanic and desert dust particles affect human activities in manifold ways; consequently, mitigation tools are important. Their early detection and the issuance of early warnings are key elements in the initiation of operational response procedures. A methodology for the early warning of these hazards using European Aerosol Research Lidar Network (EARLINET) data is presented. The tailored product is investigated during a volcanic eruption and mineral dust advected in the eastern Mediterranean.
Dimitrios Bousiotis, Francis D. Pope, David C. Beddows, Manuel Dall’Osto, Andreas Massling, Jacob Klenø Nøjgaard, Claus Nørdstrom, Jarkko V. Niemi, Harri Portin, Tuukka Petäjä, Noemi Perez, Andrés Alastuey, Xavier Querol, Giorgos Kouvarakis, Stergios Vratolis, Konstantinos Eleftheriadis, Alfred Wiedensohler, Kay Weinhold, Maik Merkel, Thomas Tuch, and Roy M. Harrison
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-414, https://doi.org/10.5194/acp-2020-414, 2020
Preprint under review for ACP
Short summary
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Formation of new particles is a key process in the atmosphere. New Particle Formation events arising from nucleation of gaseous precursors have been analysed in extensive datasets from thirteen sites in five European countries in terms of frequency, nucleation rate and particle growth rate, with several common features and many differences identified. Although nucleation frequencies are lower at roadside sites, nucleation rates and particle growth rates are typically higher.
James Brean, David C. S. Beddows, Zongbo Shi, Brice Temime-Roussel, Nicolas Marchand, Xavier Querol, Andrés Alastuey, María Cruz Minguillón, and Roy M. Harrison
Atmos. Chem. Phys., 20, 10029–10045, https://doi.org/10.5194/acp-20-10029-2020, https://doi.org/10.5194/acp-20-10029-2020, 2020
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New particle formation is a key process influencing both local air quality and climatically active cloud condensation nuclei concentrations. This study has carried out fundamental measurements of nucleation processes in Barcelona, Spain, and concludes that a mechanism involving stabilisation of sulfuric acid clusters by low molecular weight amines is primarily responsible for new particle formation events.
Jesús Yus-Díez, Marina Ealo, Marco Pandolfi, Noemí Perez, Gloria Titos, Griša Močnik, Xavier Querol, and Andrés Alastuey
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-837, https://doi.org/10.5194/acp-2020-837, 2020
Preprint under review for ACP
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Here we describe the vertical profiles of aerosol optical properties – both extensive (scattering and absorption) and intensive (e.g. albedo and asymmetry parameter), obtained coupling ground based measurements from two sites in NE Spain with airborne measurements performed with an aircraft. We analyze different aerosol layers along the vertical profile for a regional pollution episode and a Saharan dust intrusion. The results show a change with height depending on the different measured layers.
Teruyuki Nakajima, Monica Campanelli, Huizheng Che, Victor Estellés, Hitoshi Irie, Sang-Woo Kim, Jhoon Kim, Dong Liu, Tomoaki Nishizawa, Govindan Pandithurai, Vijay Kumar Soni, Boossarasiri Thana, Nas-Urt Tugjsurn, Kazuma Aoki, Sujung Go, Makiko Hashimoto, Akiko Higurashi, Stelios Kazadzis, Pradeep Khatri, Natalia Kouremeti, Rei Kudo, Franco Marenco, Masahiro Momoi, Shantikumar S. Ningombam, Claire L. Ryder, Akihiro Uchiyama, and Akihiro Yamazaki
Atmos. Meas. Tech., 13, 4195–4218, https://doi.org/10.5194/amt-13-4195-2020, https://doi.org/10.5194/amt-13-4195-2020, 2020
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This paper overviews the progress in sky radiometer technology and the development of the network called SKYNET. It is found that the technology has produced useful on-site calibration methods, retrieval algorithms, and data analyses from sky radiometer observations of aerosol, cloud, water vapor, and ozone. The paper also discusses current issues of SKYNET to provide better information for the community.
Dimitrios Bousiotis, James Brean, Francis Pope, Manuel Dall'Osto, Xavier Querol, Andres Alastuey, Noemi Perez, Tuukka Petäjä, Andreas Massling, Jacob Klenø Nøjgaard, Claus Nørdstrom, Giorgos Kouvarakis, Stergios Vratolis, Konstantinos Eleftheriadis, Jarkko V. Niemi, Harri Portin, and Roy M. Harrison
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-555, https://doi.org/10.5194/acp-2020-555, 2020
Preprint under review for ACP
Short summary
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New Particle Formation events from 16 sites over Europe have been studied and the influence of meteorological and atmospheric composition variables has been investigated. Some variables like solar radiation intensity or temperature have a positive effect upon the occurrence of these events, while others have a negative effect, affecting different aspects such as the rate at which particles are formed or grow. This effect varies depending on the site type and magnitude of these variables.
Marc Guevara, Oriol Jorba, Carles Tena, Hugo Denier van der Gon, Jeroen Kuenen, Nellie Elguindi-Solmon, Sabine Darras, Claire Granier, and Carlos Pérez García-Pando
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2020-175, https://doi.org/10.5194/essd-2020-175, 2020
Preprint under review for ESSD
Short summary
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The temporal variability of atmospheric emissions is linked to changes in activity patterns, emission processes and meteorology. Accounting for the change in temporal emission characteristics is a key aspect for modelling the trends of air pollutants. This work presents a dataset of global and European emission temporal profiles to be used for air quality modelling purposes. The profiles were constructed considering the influences of local sociodemographic factors and climatological conditions.
Vasiliki Daskalopoulou, Sotirios A. Mallios, Zbigniew Ulanowski, George Hloupis, Anna Gialitaki, Konstantinos Tassis, and Vassilis Amiridis
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-668, https://doi.org/10.5194/acp-2020-668, 2020
Preprint under review for ACP
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This research highlights the detection of charged Saharan dust in Greece and provides indications of charge separation in the plumes through the first ever co-located ground electric field measurements and sophisticated lidar observations. We provide a robust methodology for the extraction of a fair weather proxy field, used to assess the effect of lofted dust particles to the electric field and insert a realistic modelling aspect to the charge accumulation areas within electrically active dust.
Marc Guevara, Oriol Jorba, Albert Soret, Hervé Petetin, Dene Bowdalo, Kim Serradell, Carles Tena, Hugo Denier van der Gon, Jeroen Kuenen, Vincent-Henri Peuch, and Carlos Pérez García-Pando
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-686, https://doi.org/10.5194/acp-2020-686, 2020
Preprint under review for ACP
Short summary
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Most European countries have imposed lockdowns to combat the spread of the COVID-19 pandemic. Such a socioeconomic disruption has resulted in a sudden drop of atmospheric emissions and air pollution levels. This study quantifies the daily reductions in national emissions and associated levels of nitrogen dioxide (NO2) due to the COVID-19 lockdowns in Europe, by making use of multiple open access measured activity data as well as artificial intelligence and modelling techniques.
Antonis Gkikas, Emmanouil Proestakis, Vassilis Amiridis, Stelios Kazadzis, Enza Di Tomaso, Alexandra Tsekeri, Eleni Marinou, Nikos Hatzianastassiou, and Carlos Pérez García-Pando
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-222, https://doi.org/10.5194/amt-2020-222, 2020
Preprint under review for AMT
Short summary
Short summary
We present the development of the MIDAS (ModIs Dust AeroSol) dataset providing daily dust optical depth (DOD at 550 nm) at global scale and fine spatial resolution (0.1° x 0.1°) over a decade (2007-2016). It has been developed via the synergy of MODIS-Aqua and MERRA-2 data while CALIOP and AERONET retrievals are used for its assessment. MIDAS upgrades existing dust observational capabilities and it is suitable for dust climatological studies, model evaluation and data assimilation.
Ana Moreno, Miguel Bartolomé, Juan Ignacio López-Moreno, Jorge Pey, Pablo Corella, Jordi García-Orellana, Carlos Sancho, María Leunda, Graciela Gil-Romera, Penélope González-Sampériz, Carlos Pérez-Mejías, Francisco Navarro, Jaime Otero-García, Javier Lapazaran, Esteban Alonso-González, Cristina Cid, Jerónimo López-Martínez, Belén Oliva-Urcia, Sérgio H. Faria, María José Sierra, Rocío Millán, Xavier Querol, Andrés Alastuey, and José M. García-Ruiz
The Cryosphere Discuss., https://doi.org/10.5194/tc-2020-107, https://doi.org/10.5194/tc-2020-107, 2020
Preprint under review for TC
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Our study of the chronological sequence of Monte Perdido Glacier in Central Pyrenees (Spain) reveals that, although the intense warming associated with the Roman Period or the Medieval Climate Anomaly produced important ice mass losses, it was insufficient to make this glacier disappear. By contrast, recent global warming has melted away almost 600 years of ice accumulated since the Little Ice Age, jeopardizing the survival of this and other southern European glaciers over the next few decades.
Hervé Petetin, Dene Bowdalo, Albert Soret, Marc Guevara, Oriol Jorba, Kim Serradell, and Carlos Pérez García-Pando
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-446, https://doi.org/10.5194/acp-2020-446, 2020
Revised manuscript accepted for ACP
Short summary
Short summary
To control the spread of the COVID-19 coronavirus, the Spanish Government recently implemented a strict lockdown of the population, which has strongly reduced the levels of nitrogen dioxide (NO2), one of the most critical air pollutant in Spain. This study quantifies the contribution of the lockdown on these reduced NO2 levels in Spain, taking into account the confounding effect of meteorology with artificial intelligence techniques.
Myrto Gratsea, Tim Bösch, Panos Kokkalis, Andreas Richter, Mihalis Vrekoussis, Stelios Kazadzis, Alexandra Tsekeri, Alexandros Papayannis, Maria Mylonaki, Vassilis Amiridis, Nikos Mihalopoulos, and Evangelos Gerasopoulos
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-100, https://doi.org/10.5194/amt-2020-100, 2020
Preprint under review for AMT
Marc Guevara, Carles Tena, Manuel Porquet, Oriol Jorba, and Carlos Pérez García-Pando
Geosci. Model Dev., 13, 873–903, https://doi.org/10.5194/gmd-13-873-2020, https://doi.org/10.5194/gmd-13-873-2020, 2020
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Emission inventories are a key input to numerical systems that simulate air quality. In this paper, we present an open-source tool intended for the computation of high-resolution anthropogenic emissions for air quality modelling. Emissions are estimated using detailed methods that combine local activity and emission factors along with meteorological data. Specific results are presented for Spain. Nevertheless, the model is designed so that it can be applicable to any European country or region.
Christine Aebi, Julian Gröbner, Stelios Kazadzis, Laurent Vuilleumier, Antonis Gkikas, and Niklaus Kämpfer
Atmos. Meas. Tech., 13, 907–923, https://doi.org/10.5194/amt-13-907-2020, https://doi.org/10.5194/amt-13-907-2020, 2020
Short summary
Short summary
Clouds are one of the largest sources of uncertainties in climate models. The current study estimates the cloud optical thickness (COT), the effective droplet radius and the single scattering albedo of stratus–altostratus and cirrus–cirrostratus clouds in Payerne, Switzerland, by combining ground- and satellite-based measurements and radiative transfer models. The estimated values are thereafter compared with data retrieved from other methods. The mean COT is distinct for different seasons.
Elina Giannakaki, Panos Kokkalis, Eleni Marinou, Nikolaos S. Bartsotas, Vassilis Amiridis, Albert Ansmann, and Mika Komppula
Atmos. Meas. Tech., 13, 893–905, https://doi.org/10.5194/amt-13-893-2020, https://doi.org/10.5194/amt-13-893-2020, 2020
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A new method, called ElEx, is proposed for the estimation of extinction coefficient lidar profiles using only the information provided by the elastic and polarization channels of a lidar system. The method is applicable to lidar measurements both during daytime and nighttime under well-defined aerosol mixtures. Comparisons with both Raman lidar profiles during nightime and sun photometer daytime aerosol optical depth observations demonstrate the potential of the ElEx methodology.
new blackfor smoke?
Anna Gialitaki, Alexandra Tsekeri, Vassilis Amiridis, Romain Ceolato, Lucas Paulien, Anna Kampouri, Antonis Gkikas, Stavros Solomos, Eleni Marinou, Moritz Haarig, Holger Baars, Albert Ansmann, Tatyana Lapyonok, Anton Lopatin, Oleg Dubovik, Silke Groß, Martin Wirth, and Dimitris Balis
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-22, https://doi.org/10.5194/acp-2020-22, 2020
Revised manuscript accepted for ACP
Short summary
Short summary
Smoke particles injected into the stratosphere are find to significantly depolarize the incident light while this effect is also accompanied by a strong spectral dependence. Here we utilize scattering simulations to show that this behavior can be attributed to the near-spherical shape of stratospheric smoke which can produce both the non-typical values and wavelength dependence of smoke depolarization. This was not feasible when assuming more complicated morphologies for the smoke particles.
Marco Pandolfi, Dennis Mooibroek, Philip Hopke, Dominik van Pinxteren, Xavier Querol, Hartmut Herrmann, Andrés Alastuey, Olivier Favez, Christoph Hüglin, Esperanza Perdrix, Véronique Riffault, Stéphane Sauvage, Eric van der Swaluw, Oksana Tarasova, and Augustin Colette
Atmos. Chem. Phys., 20, 409–429, https://doi.org/10.5194/acp-20-409-2020, https://doi.org/10.5194/acp-20-409-2020, 2020
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In the last scientific assessment report from the LRTAP Convention, it is stated that because non-urban sources are often major contributors to urban pollution, many cities will be unable to meet WHO guideline levels for air pollutants through local action alone. Consequently, it is very important to estimate how much the local and non-local sources contribute to urban pollution in order to design global strategies to reduce the levels of pollutants in European cities.
Holger Baars, Albert Ansmann, Kevin Ohneiser, Moritz Haarig, Ronny Engelmann, Dietrich Althausen, Ingrid Hanssen, Michael Gausa, Aleksander Pietruczuk, Artur Szkop, Iwona S. Stachlewska, Dongxiang Wang, Jens Reichardt, Annett Skupin, Ina Mattis, Thomas Trickl, Hannes Vogelmann, Francisco Navas-Guzmán, Alexander Haefele, Karen Acheson, Albert A. Ruth, Boyan Tatarov, Detlef Müller, Qiaoyun Hu, Thierry Podvin, Philippe Goloub, Igor Veselovskii, Christophe Pietras, Martial Haeffelin, Patrick Fréville, Michaël Sicard, Adolfo Comerón, Alfonso Javier Fernández García, Francisco Molero Menéndez, Carmen Córdoba-Jabonero, Juan Luis Guerrero-Rascado, Lucas Alados-Arboledas, Daniele Bortoli, Maria João Costa, Davide Dionisi, Gian Luigi Liberti, Xuan Wang, Alessia Sannino, Nikolaos Papagiannopoulos, Antonella Boselli, Lucia Mona, Giuseppe D'Amico, Salvatore Romano, Maria Rita Perrone, Livio Belegante, Doina Nicolae, Ivan Grigorov, Anna Gialitaki, Vassilis Amiridis, Ourania Soupiona, Alexandros Papayannis, Rodanthi-Elisaveth Mamouri, Argyro Nisantzi, Birgit Heese, Julian Hofer, Yoav Y. Schechner, Ulla Wandinger, and Gelsomina Pappalardo
Atmos. Chem. Phys., 19, 15183–15198, https://doi.org/10.5194/acp-19-15183-2019, https://doi.org/10.5194/acp-19-15183-2019, 2019
Michael Pikridas, Spiros Bezantakos, Griša Močnik, Christos Keleshis, Fred Brechtel, Iasonas Stavroulas, Gregoris Demetriades, Panayiota Antoniou, Panagiotis Vouterakos, Marios Argyrides, Eleni Liakakou, Luka Drinovec, Eleni Marinou, Vassilis Amiridis, Mihalis Vrekoussis, Nikolaos Mihalopoulos, and Jean Sciare
Atmos. Meas. Tech., 12, 6425–6447, https://doi.org/10.5194/amt-12-6425-2019, https://doi.org/10.5194/amt-12-6425-2019, 2019
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This work evaluates the performance of three sensors that monitor black carbon (soot). These sensors exhibit similar behavior to their rack-mounted counterparts and are therefore promising for more extended use. A reconstruction of the black carbon mass vertical distribution above Athens, Greece, is shown using drones, similar to those acquired by remote-sensing techniques. The potential of combining miniature sensors with drones for at least the lower part of the atmosphere is exhibited.
Rebecca M. Pauly, John E. Yorks, Dennis L. Hlavka, Matthew J. McGill, Vassilis Amiridis, Stephen P. Palm, Sharon D. Rodier, Mark A. Vaughan, Patrick A. Selmer, Andrew W. Kupchock, Holger Baars, and Anna Gialitaki
Atmos. Meas. Tech., 12, 6241–6258, https://doi.org/10.5194/amt-12-6241-2019, https://doi.org/10.5194/amt-12-6241-2019, 2019
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The Cloud Aerosol Transport System (CATS) demonstrated that direct calibration of 1064 nm lidar data from a spaceborne platform is possible. By normalizing the CATS signal to a modeled molecular backscatter profile the CATS data were calibrated, enabling the derivation of optical properties of clouds and aerosols. Comparisons of the calibrated signal with airborne lidar, ground-based lidar, and spaceborne lidar all show agreement within the estimated error bars of the respective instruments.
Miguel Escudero, Arjo Segers, Richard Kranenburg, Xavier Querol, Andrés Alastuey, Rafael Borge, David de la Paz, Gotzon Gangoiti, and Martijn Schaap
Atmos. Chem. Phys., 19, 14211–14232, https://doi.org/10.5194/acp-19-14211-2019, https://doi.org/10.5194/acp-19-14211-2019, 2019
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In this work we optimise LOTOS-EUROS CTM for simulating tropospheric O3 during summer in the Madrid metropolitan area, one of the largest conurbations in the Mediterranean. Comparing the outputs from five set-ups with different combinations of spatial resolution, meteorological data and vertical structure, we conclude that the model benefits from fine horizontal resolution and highly resolved vertical structure. Running optimized configuration run, we interpret O3 variability during July 2016.
Emmanouil Proestakis, Vassilis Amiridis, Eleni Marinou, Ioannis Binietoglou, Albert Ansmann, Ulla Wandinger, Julian Hofer, John Yorks, Edward Nowottnick, Abduvosit Makhmudov, Alexandros Papayannis, Aleksander Pietruczuk, Anna Gialitaki, Arnoud Apituley, Artur Szkop, Constantino Muñoz Porcar, Daniele Bortoli, Davide Dionisi, Dietrich Althausen, Dimitra Mamali, Dimitris Balis, Doina Nicolae, Eleni Tetoni, Gian Luigi Liberti, Holger Baars, Ina Mattis, Iwona Sylwia Stachlewska, Kalliopi Artemis Voudouri, Lucia Mona, Maria Mylonaki, Maria Rita Perrone, Maria João Costa, Michael Sicard, Nikolaos Papagiannopoulos, Nikolaos Siomos, Pasquale Burlizzi, Rebecca Pauly, Ronny Engelmann, Sabur Abdullaev, and Gelsomina Pappalardo
Atmos. Chem. Phys., 19, 11743–11764, https://doi.org/10.5194/acp-19-11743-2019, https://doi.org/10.5194/acp-19-11743-2019, 2019
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To increase accuracy and validate satellite-based products, comparison with ground-based reference observations is required. To do this, we present evaluation activity of EARLINET for the qualitative and quantitative assessment of NASA's CATS lidar operating aboard the International Space Station (ISS) while identified discrepancies are discussed. Better understanding CATS performance and limitations provides a valuable basis for scientific studies implementing the satellite-based lidar system.
Eleni Marinou, Matthias Tesche, Athanasios Nenes, Albert Ansmann, Jann Schrod, Dimitra Mamali, Alexandra Tsekeri, Michael Pikridas, Holger Baars, Ronny Engelmann, Kalliopi-Artemis Voudouri, Stavros Solomos, Jean Sciare, Silke Groß, Florian Ewald, and Vassilis Amiridis
Atmos. Chem. Phys., 19, 11315–11342, https://doi.org/10.5194/acp-19-11315-2019, https://doi.org/10.5194/acp-19-11315-2019, 2019
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We assess the feasibility of ground-based and spaceborne lidars to retrieve profiles of cloud-relevant aerosol concentrations and ice-nucleating particles. The retrieved profiles are in good agreement with airborne in situ measurements. Our methodology will be applied to satellite observations in the future so as to provide a global 3D product of cloud-relevant properties.
Emilio Cuevas, Pedro Miguel Romero-Campos, Natalia Kouremeti, Stelios Kazadzis, Petri Räisänen, Rosa Delia García, Africa Barreto, Carmen Guirado-Fuentes, Ramón Ramos, Carlos Toledano, Fernando Almansa, and Julian Gröbner
Atmos. Meas. Tech., 12, 4309–4337, https://doi.org/10.5194/amt-12-4309-2019, https://doi.org/10.5194/amt-12-4309-2019, 2019
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A comprehensive comparison of more than 70 000 synchronous 1 min aerosol optical depth (AOD) data from 3 Global Atmosphere Watch precision filter radiometers (GAW-PFR) and 15 Aerosol Robotic Network Cimel radiometers (AERONET-Cimel) was performed for the four
nearwavelengths (380, 440, 500 and 870 nm) in the period 2005–2015. The goal of this study is to assess whether their long term AOD data are comparable and consistent.
Jaime Benavides, Michelle Snyder, Marc Guevara, Albert Soret, Carlos Pérez García-Pando, Fulvio Amato, Xavier Querol, and Oriol Jorba
Geosci. Model Dev., 12, 2811–2835, https://doi.org/10.5194/gmd-12-2811-2019, https://doi.org/10.5194/gmd-12-2811-2019, 2019
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The NO2 annual air quality limit value is systematically exceeded in many European cities. In this context, understanding human exposure, improving policy and planning, and providing forecasts requires the development of accurate air quality models at street level. We describe CALIOPE-Urban, a system coupling an operational mesoscale air quality forecast system with an urban roadway dispersion model over Barcelona city (Spain). The methodology may be replicated for other cities in the future.
Jordi Massagué, Cristina Carnerero, Miguel Escudero, José María Baldasano, Andrés Alastuey, and Xavier Querol
Atmos. Chem. Phys., 19, 7445–7465, https://doi.org/10.5194/acp-19-7445-2019, https://doi.org/10.5194/acp-19-7445-2019, 2019
Marc Guevara, Carles Tena, Manuel Porquet, Oriol Jorba, and Carlos Pérez García-Pando
Geosci. Model Dev., 12, 1885–1907, https://doi.org/10.5194/gmd-12-1885-2019, https://doi.org/10.5194/gmd-12-1885-2019, 2019
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Atmospheric emission inventories, which describe the amounts of pollutants released into the air by different sources and for specific regions, are an essential input to numerical models that estimate air quality. This work presents the High-Elective Resolution Modelling Emission System version 3 (HERMESv3), an open-source modelling framework that allows adapting existing global and regional emission inventories to the input requirements of air quality models in a flexible and transparent way.
María Teresa Pay, Gotzon Gangoiti, Marc Guevara, Sergey Napelenok, Xavier Querol, Oriol Jorba, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 19, 5467–5494, https://doi.org/10.5194/acp-19-5467-2019, https://doi.org/10.5194/acp-19-5467-2019, 2019
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The poor diagnostic of the O3 issue over southwestern Europe prevents authorities from implementing effective mitigation plans. This work is a pioneer in identifying that imported O3 is the largest input to the ground-level O3 concentration in the Iberian Peninsula, which is largely explained by vertical mixing. This study also proves that anthropogenic emissions control the severe O3 peaks during stagnant conditions. Ad hoc local actions should complement national/European strategies.
Ville Vakkari, Antti J. Manninen, Ewan J. O'Connor, Jan H. Schween, Pieter G. van Zyl, and Eleni Marinou
Atmos. Meas. Tech., 12, 839–852, https://doi.org/10.5194/amt-12-839-2019, https://doi.org/10.5194/amt-12-839-2019, 2019
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Commercially available Doppler lidars have been proven to be efficient tools for studying winds and turbulence in the planetary boundary layer. However, in many cases low signal is still a limiting factor for utilising measurements by these devices. Here, we present a novel post-processing algorithm for Halo Stream Line Doppler lidars, which enables an improvement in sensitivity of a factor of 5 or more.
Cristina Carnerero, Noemí Pérez, Cristina Reche, Marina Ealo, Gloria Titos, Hong-Ku Lee, Hee-Ram Eun, Yong-Hee Park, Lubna Dada, Pauli Paasonen, Veli-Matti Kerminen, Enrique Mantilla, Miguel Escudero, Francisco J. Gómez-Moreno, Elisabeth Alonso-Blanco, Esther Coz, Alfonso Saiz-Lopez, Brice Temime-Roussel, Nicolas Marchand, David C. S. Beddows, Roy M. Harrison, Tuukka Petäjä, Markku Kulmala, Kang-Ho Ahn, Andrés Alastuey, and Xavier Querol
Atmos. Chem. Phys., 18, 16601–16618, https://doi.org/10.5194/acp-18-16601-2018, https://doi.org/10.5194/acp-18-16601-2018, 2018
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The vertical distribution of new particle formation events was studied using tethered balloons carrying miniaturized instrumentation. Results show that new particle formation and growth occurs only in the lower layer of the atmosphere, where aerosols are mixed due to convection, especially when the atmosphere is clean. A comparison of urban and suburban surface stations was also made, suggesting that such events may have a significant impact on ultrafine particle concentrations in a wide area.
Nikolaos Papagiannopoulos, Lucia Mona, Aldo Amodeo, Giuseppe D'Amico, Pilar Gumà Claramunt, Gelsomina Pappalardo, Lucas Alados-Arboledas, Juan Luís Guerrero-Rascado, Vassilis Amiridis, Panagiotis Kokkalis, Arnoud Apituley, Holger Baars, Anja Schwarz, Ulla Wandinger, Ioannis Binietoglou, Doina Nicolae, Daniele Bortoli, Adolfo Comerón, Alejandro Rodríguez-Gómez, Michaël Sicard, Alex Papayannis, and Matthias Wiegner
Atmos. Chem. Phys., 18, 15879–15901, https://doi.org/10.5194/acp-18-15879-2018, https://doi.org/10.5194/acp-18-15879-2018, 2018
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A stand-alone automatic method for typing observations of the European Aerosol Research Lidar Network (EARLINET) is presented. The method compares the observations to model distributions that were constructed using EARLINET pre-classified data. The algorithm’s versatility and adaptability makes it suitable for network-wide typing studies.
Carlos Toledano, Ramiro González, David Fuertes, Emilio Cuevas, Thomas F. Eck, Stelios Kazadzis, Natalia Kouremeti, Julian Gröbner, Philippe Goloub, Luc Blarel, Roberto Román, África Barreto, Alberto Berjón, Brent N. Holben, and Victoria E. Cachorro
Atmos. Chem. Phys., 18, 14555–14567, https://doi.org/10.5194/acp-18-14555-2018, https://doi.org/10.5194/acp-18-14555-2018, 2018
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Most of the ground-based radiometric networks have their reference instruments and/or calibrate them at Mauna Loa or Izaña. The suitability of these high-mountain stations for absolute radiometric calibrations is investigated with the support of 20 years of first-class Sun photometer data from the AERONET and GAW-PFR networks. We analyze the number of calibration days at each site in a climatological sense and investigate the uncertainty of the calibrations based on long-term statistics.
Marco Zanatta, Paolo Laj, Martin Gysel, Urs Baltensperger, Stergios Vratolis, Konstantinos Eleftheriadis, Yutaka Kondo, Philippe Dubuisson, Victor Winiarek, Stelios Kazadzis, Peter Tunved, and Hans-Werner Jacobi
Atmos. Chem. Phys., 18, 14037–14057, https://doi.org/10.5194/acp-18-14037-2018, https://doi.org/10.5194/acp-18-14037-2018, 2018
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The research community aims to quantify the actual contribution of soot particles to the recent Arctic warming. We discovered that mixing of soot with other components might enhance its light absorption power by 50 %. The neglection of such amplification might lead to the underestimation of radiative forcing by 0.12 W m−2. Thus a better understanding of the optical properties of soot is a crucial step for an accurate quantification of the radiative impact of soot in the Arctic atmosphere.
Kaisa Lakkala, Antti Arola, Julian Gröbner, Sergio Fabian León-Luis, Alberto Redondas, Stelios Kazadzis, Tomi Karppinen, Juha Matti Karhu, Luca Egli, Anu Heikkilä, Tapani Koskela, Antonio Serrano, and José Manuel Vilaplana
Atmos. Meas. Tech., 11, 5167–5180, https://doi.org/10.5194/amt-11-5167-2018, https://doi.org/10.5194/amt-11-5167-2018, 2018
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The performance of the cosine error correction method for correcting spectral UV measurements of the Brewer spectroradiometer was studied. The correction depends on the sky radiation distribution, which can change during one spectral scan. The results showed that the correction varied between 4 and 14 %, and that the relative differences between the reference and the Brewer diminished by 10 %. The method is applicable to other instruments as long as the required input parameters are available.
Nikolaos Siomos, Dimitris S. Balis, Kalliopi A. Voudouri, Eleni Giannakaki, Maria Filioglou, Vassilis Amiridis, Alexandros Papayannis, and Konstantinos Fragkos
Atmos. Chem. Phys., 18, 11885–11903, https://doi.org/10.5194/acp-18-11885-2018, https://doi.org/10.5194/acp-18-11885-2018, 2018
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In this study we investigate the climatological behavior of the aerosol optical properties over Thessaloniki during the years 2003–2017. For this purpose, measurements from two individual networks, the European Lidar Aerosol Network (EARLINET) and the Aerosol Robotic Network (AERONET), were deployed. The analysis implies that the EARLINET sampling schedule can be quite effective in producing data that can be applied to
climatological studies.
Larisa Sogacheva, Gerrit de Leeuw, Edith Rodriguez, Pekka Kolmonen, Aristeidis K. Georgoulias, Georgia Alexandri, Konstantinos Kourtidis, Emmanouil Proestakis, Eleni Marinou, Vassilis Amiridis, Yong Xue, and Ronald J. van der A
Atmos. Chem. Phys., 18, 11389–11407, https://doi.org/10.5194/acp-18-11389-2018, https://doi.org/10.5194/acp-18-11389-2018, 2018
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Using AATSR ADV (1995–2011) and MODIS C6.1 (2000–2017) annual and seasonal aerosol optical depth (AOD) aggregates, we obtained information regarding the occurrence of aerosols and their spatial and temporal variation over China. We specifically focused on regional differences in annual and seasonal AOD behavior for selected regions. AOD dataset comparisons, validation results and AOD tendencies during the overlapping period (2000–2011) are discussed.
Angela Benedetti, Jeffrey S. Reid, Peter Knippertz, John H. Marsham, Francesca Di Giuseppe, Samuel Rémy, Sara Basart, Olivier Boucher, Ian M. Brooks, Laurent Menut, Lucia Mona, Paolo Laj, Gelsomina Pappalardo, Alfred Wiedensohler, Alexander Baklanov, Malcolm Brooks, Peter R. Colarco, Emilio Cuevas, Arlindo da Silva, Jeronimo Escribano, Johannes Flemming, Nicolas Huneeus, Oriol Jorba, Stelios Kazadzis, Stefan Kinne, Thomas Popp, Patricia K. Quinn, Thomas T. Sekiyama, Taichu Tanaka, and Enric Terradellas
Atmos. Chem. Phys., 18, 10615–10643, https://doi.org/10.5194/acp-18-10615-2018, https://doi.org/10.5194/acp-18-10615-2018, 2018
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Numerical prediction of aerosol particle properties has become an important activity at many research and operational weather centers. This development is due to growing interest from a diverse set of stakeholders, such as air quality regulatory bodies, aviation authorities, solar energy plant managers, climate service providers, and health professionals. This paper describes the advances in the field and sets out requirements for observations for the sustainability of these activities.
Marta G. Vivanco, Mark R. Theobald, Héctor García-Gómez, Juan Luis Garrido, Marje Prank, Wenche Aas, Mario Adani, Ummugulsum Alyuz, Camilla Andersson, Roberto Bellasio, Bertrand Bessagnet, Roberto Bianconi, Johannes Bieser, Jørgen Brandt, Gino Briganti, Andrea Cappelletti, Gabriele Curci, Jesper H. Christensen, Augustin Colette, Florian Couvidat, Cornelis Cuvelier, Massimo D'Isidoro, Johannes Flemming, Andrea Fraser, Camilla Geels, Kaj M. Hansen, Christian Hogrefe, Ulas Im, Oriol Jorba, Nutthida Kitwiroon, Astrid Manders, Mihaela Mircea, Noelia Otero, Maria-Teresa Pay, Luca Pozzoli, Efisio Solazzo, Svetlana Tsyro, Alper Unal, Peter Wind, and Stefano Galmarini
Atmos. Chem. Phys., 18, 10199–10218, https://doi.org/10.5194/acp-18-10199-2018, https://doi.org/10.5194/acp-18-10199-2018, 2018
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European wet and dry atmospheric deposition of N and S estimated by 14 air quality models was found to vary substantially. An ensemble of models meeting acceptability criteria was used to estimate the exceedances of the critical loads for N in habitats within the Natura 2000 network, as well as their lower and upper limits. Scenarios with 20 % emission reductions in different regions of the world showed that European emissions are responsible for most of the N and S deposition in Europe.
Antonis Gkikas, Vincenzo Obiso, Carlos Pérez García-Pando, Oriol Jorba, Nikos Hatzianastassiou, Lluis Vendrell, Sara Basart, Stavros Solomos, Santiago Gassó, and José Maria Baldasano
Atmos. Chem. Phys., 18, 8757–8787, https://doi.org/10.5194/acp-18-8757-2018, https://doi.org/10.5194/acp-18-8757-2018, 2018
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The present study investigates the direct radiative effects (DREs), induced during 20 intense Mediterranean desert dust outbreaks, based on regional short-term numerical simulations of the NMMB-MONARCH model: more specifically, (i) the DREs and their associated impacts on temperature and surface sensible and latent heat fluxes, (ii) the feedbacks on dust AOD and dust emissions, and (iii) the possible improvements in short-term forecasts (up to 84 h) of temperature and radiation.
Aristeidis K. Georgoulias, Athanasios Tsikerdekis, Vassilis Amiridis, Eleni Marinou, Angela Benedetti, Prodromos Zanis, Georgia Alexandri, Lucia Mona, Konstantinos A. Kourtidis, and Jos Lelieveld
Atmos. Chem. Phys., 18, 8601–8620, https://doi.org/10.5194/acp-18-8601-2018, https://doi.org/10.5194/acp-18-8601-2018, 2018
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In this work, the MACC reanalysis dust product is evaluated over Europe, Northern Africa and the Middle East using the EARLINET-optimized CALIOP/CALIPSO pure dust satellite-based product LIVAS (2007–2012). As dust plays a determinant role in processes related to weather and climate, human healt, and the economy, it is obvious that adequately simulating the amount of dust and its optical properties is essential. Our results could be used as a reference in future climate model evaluations.
Dimitra Mamali, Eleni Marinou, Jean Sciare, Michael Pikridas, Panagiotis Kokkalis, Michael Kottas, Ioannis Binietoglou, Alexandra Tsekeri, Christos Keleshis, Ronny Engelmann, Holger Baars, Albert Ansmann, Vassilis Amiridis, Herman Russchenberg, and George Biskos
Atmos. Meas. Tech., 11, 2897–2910, https://doi.org/10.5194/amt-11-2897-2018, https://doi.org/10.5194/amt-11-2897-2018, 2018
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The paper's scope is to evaluate the performance of in situ atmospheric aerosol instrumentation on board unmanned aerial vehicles (UAVs) and the performance of algorithms used to calculate the aerosol mass from remote sensing instruments by comparing the two independent techniques to each other. Our results indicate that UAV-based aerosol measurements (using specific in situ and remote sensing instrumentation) can provide reliable ways to determine the aerosol mass throughout the atmosphere.
Xavier Querol, Andrés Alastuey, Gotzon Gangoiti, Noemí Perez, Hong K. Lee, Heeram R. Eun, Yonghee Park, Enrique Mantilla, Miguel Escudero, Gloria Titos, Lucio Alonso, Brice Temime-Roussel, Nicolas Marchand, Juan R. Moreta, M. Arantxa Revuelta, Pedro Salvador, Begoña Artíñano, Saúl García dos Santos, Mónica Anguas, Alberto Notario, Alfonso Saiz-Lopez, Roy M. Harrison, Millán Millán, and Kang-Ho Ahn
Atmos. Chem. Phys., 18, 6511–6533, https://doi.org/10.5194/acp-18-6511-2018, https://doi.org/10.5194/acp-18-6511-2018, 2018
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We show the main drivers of high O3 episodes in and around Madrid. High levels of ultrafine particles (UFPs) are evidenced, but we demonstrate that most O3 arises from the fumigation of high atmospheric layers, whereas UFPs are generated inside the PBL. O3 contributions from the fumigation of the vertical recirculation of regional air masses, hemispheric transport, and horizontally from direct urban plume transport are shown. Complexity arises from the need to quantify them to abate surface O3.
Javier López-Solano, Alberto Redondas, Thomas Carlund, Juan J. Rodriguez-Franco, Henri Diémoz, Sergio F. León-Luis, Bentorey Hernández-Cruz, Carmen Guirado-Fuentes, Natalia Kouremeti, Julian Gröbner, Stelios Kazadzis, Virgilio Carreño, Alberto Berjón, Daniel Santana-Díaz, Manuel Rodríguez-Valido, Veerle De Bock, Juan R. Moreta, John Rimmer, Andrew R. D. Smedley, Lamine Boulkelia, Nis Jepsen, Paul Eriksen, Alkiviadis F. Bais, Vadim Shirotov, José M. Vilaplana, Keith M. Wilson, and Tomi Karppinen
Atmos. Chem. Phys., 18, 3885–3902, https://doi.org/10.5194/acp-18-3885-2018, https://doi.org/10.5194/acp-18-3885-2018, 2018
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The European Brewer Network (EUBREWNET, COST Action ES1207) is comprised of close to 50 instruments and currently provides near-real-time ozone and UV data. Aerosols also play key role in the Earth–atmosphere system and introduce a large uncertainty into our understanding of climate change. In this work we describe and validate a method to incorporate the measurement of aerosols in EUBREWNET. We find that this Brewer network can provide reliable aerosol data across Europe in the UV range.
Stelios Kazadzis, Natalia Kouremeti, Henri Diémoz, Julian Gröbner, Bruce W. Forgan, Monica Campanelli, Victor Estellés, Kathleen Lantz, Joseph Michalsky, Thomas Carlund, Emilio Cuevas, Carlos Toledano, Ralf Becker, Stephan Nyeki, Panagiotis G. Kosmopoulos, Viktar Tatsiankou, Laurent Vuilleumier, Frederick M. Denn, Nozomu Ohkawara, Osamu Ijima, Philippe Goloub, Panagiotis I. Raptis, Michael Milner, Klaus Behrens, Africa Barreto, Giovanni Martucci, Emiel Hall, James Wendell, Bryan E. Fabbri, and Christoph Wehrli
Atmos. Chem. Phys., 18, 3185–3201, https://doi.org/10.5194/acp-18-3185-2018, https://doi.org/10.5194/acp-18-3185-2018, 2018
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Aerosol optical depth measured from ground-based sun photometers is the most important parameter for studying the changes in the Earth's radiation balance due to aerosols. Representatives for various sun photometer types belonging to individual institutions or international aerosol networks gather every 5 years, for 3 weeks, in Davos, Switzerland, in order to compare their aeorosol optical depth retrievals. This work presents the results of the latest (fourth) filter radiometer intercomparison.
Panagiotis-Ioannis Raptis, Stelios Kazadzis, Julian Gröbner, Natalia Kouremeti, Lionel Doppler, Ralf Becker, and Constantinos Helmis
Atmos. Meas. Tech., 11, 1143–1157, https://doi.org/10.5194/amt-11-1143-2018, https://doi.org/10.5194/amt-11-1143-2018, 2018
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The purpose of this work is to retrieve integrated water vapour using spectral measurements from Precision Solar Spectroradiometer (PSR). Two different approaches were developed one using single-channel direct sun irradiance measurements, and the second one integrating at a certain spectral region. The results of the spectral approach are closer to the retrievals of non-photometric techniques (GPS, microwave radiometer and radiosondes), suggesting this method provide more accurate IWV product.
Panagiotis G. Kosmopoulos, Stelios Kazadzis, Michael Taylor, Panagiotis I. Raptis, Iphigenia Keramitsoglou, Chris Kiranoudis, and Alkiviadis F. Bais
Atmos. Meas. Tech., 11, 907–924, https://doi.org/10.5194/amt-11-907-2018, https://doi.org/10.5194/amt-11-907-2018, 2018
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Continuous monitoring of solar energy from space is critical for its efficient exploitation and distribution. For this reason we developed neural-network- and function-based real-time models, which are capable of producing massive radiation outputs in high spectral, spatial and temporal resolution. The models' performance against ground-based measurements revealed a dependence on input quality and resolution, and an overall accuracy under cloudless and high solar energy potential conditions.
Lev D. Labzovskii, Alexandros Papayannis, Ioannis Binietoglou, Robert F. Banks, Jose M. Baldasano, Florica Toanca, Chris G. Tzanis, and John Christodoulakis
Ann. Geophys., 36, 213–229, https://doi.org/10.5194/angeo-36-213-2018, https://doi.org/10.5194/angeo-36-213-2018, 2018
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This study aims to evaluate synergetic methods for relative humidity vertical profiling based on lidar–radiometer and lidar–simulation combinations. We demonstrate the effectiveness of combined lidar-based methods for relative humidity profiling in comparison with radiometer observations or WRF simulations and assess temperature-related uncertainties in resulting relative humidity profiles. All results are acquired during the HygrA-CD campaign in Athens (Greece) in 2014.
Gerrit de Leeuw, Larisa Sogacheva, Edith Rodriguez, Konstantinos Kourtidis, Aristeidis K. Georgoulias, Georgia Alexandri, Vassilis Amiridis, Emmanouil Proestakis, Eleni Marinou, Yong Xue, and Ronald van der A
Atmos. Chem. Phys., 18, 1573–1592, https://doi.org/10.5194/acp-18-1573-2018, https://doi.org/10.5194/acp-18-1573-2018, 2018
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The complementary use of two sensors, ATSR and MODIS, to provide aerosol information over two decades (1995–2015) is described. To this end, the AOD retrieved from both instruments had to be compared, showing that ATSR slightly underestimates and MODIS overestimates by a similar amount. Results show the increase of aerosols over the years, with an indication of the onset of a decrease in recent years. The AOD spatial distribution shows seasonal variations across China.
Stelios Kazadzis, Natalia Kouremeti, Stephan Nyeki, Julian Gröbner, and Christoph Wehrli
Geosci. Instrum. Method. Data Syst., 7, 39–53, https://doi.org/10.5194/gi-7-39-2018, https://doi.org/10.5194/gi-7-39-2018, 2018
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The World Optical Depth Research Calibration Center (WORCC) has been established after the recommendations of WMO for calibration of aerosol optical depth (AOD) -related sun photometers. WORCC is mandated to initiate homogenization activities among different AOD networks and to run a network (GAW-PFR) of sun photometers. To calibrate such instruments aiming at low measurement uncertainties the quality assurance, quality control and a basic hierarchy have to be defined and followed.
Emmanouil Proestakis, Vassilis Amiridis, Eleni Marinou, Aristeidis K. Georgoulias, Stavros Solomos, Stelios Kazadzis, Julien Chimot, Huizheng Che, Georgia Alexandri, Ioannis Binietoglou, Vasiliki Daskalopoulou, Konstantinos A. Kourtidis, Gerrit de Leeuw, and Ronald J. van der A
Atmos. Chem. Phys., 18, 1337–1362, https://doi.org/10.5194/acp-18-1337-2018, https://doi.org/10.5194/acp-18-1337-2018, 2018
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We provide a 3-D climatology of desert dust aerosols over South and East Asia, based on 9 years of CALIPSO observations and an EARLINET methodology. The results provide the horizontal, vertical and seasonal distribution of dust aerosols over SE Asia along with the change in dust transport pathways. The dataset is unique for its potential applications, including evaluation and assimilation activities in atmospheric simulations and the estimation of the climatic impact of dust aerosols.
Marina Ealo, Andrés Alastuey, Noemí Pérez, Anna Ripoll, Xavier Querol, and Marco Pandolfi
Atmos. Chem. Phys., 18, 1149–1169, https://doi.org/10.5194/acp-18-1149-2018, https://doi.org/10.5194/acp-18-1149-2018, 2018
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This study aims to quantify the mass scattering and absorption efficiencies of different aerosol sources at urban (Barcelona), regional (Montseny) and remote (Montsec) background sites in the NW Mediterranean by analysing a source apportionment, first to PM10 and then to scattering and absorption coefficients. With this approach we addressed both the effect that aerosol sources have on air quality and their potential effect on light extinction.
Alexandra Tsekeri, Anton Lopatin, Vassilis Amiridis, Eleni Marinou, Julia Igloffstein, Nikolaos Siomos, Stavros Solomos, Panagiotis Kokkalis, Ronny Engelmann, Holger Baars, Myrto Gratsea, Panagiotis I. Raptis, Ioannis Binietoglou, Nikolaos Mihalopoulos, Nikolaos Kalivitis, Giorgos Kouvarakis, Nikolaos Bartsotas, George Kallos, Sara Basart, Dirk Schuettemeyer, Ulla Wandinger, Albert Ansmann, Anatoli P. Chaikovsky, and Oleg Dubovik
Atmos. Meas. Tech., 10, 4995–5016, https://doi.org/10.5194/amt-10-4995-2017, https://doi.org/10.5194/amt-10-4995-2017, 2017
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The Generalized Aerosol Retrieval from Radiometer and Lidar Combined data algorithm (GARRLiC) and the LIdar-Radiometer Inversion Code (LIRIC) provide the opportunity to study the aerosol vertical distribution by combining ground-based lidar and sun-photometric measurements. Here, we utilize the capabilities of both algorithms for the characterization of Saharan dust and marine particles, along with their mixtures, in the south-eastern Mediterranean.
Albert Ansmann, Franziska Rittmeister, Ronny Engelmann, Sara Basart, Oriol Jorba, Christos Spyrou, Samuel Remy, Annett Skupin, Holger Baars, Patric Seifert, Fabian Senf, and Thomas Kanitz
Atmos. Chem. Phys., 17, 14987–15006, https://doi.org/10.5194/acp-17-14987-2017, https://doi.org/10.5194/acp-17-14987-2017, 2017
Moritz Haarig, Albert Ansmann, Dietrich Althausen, André Klepel, Silke Groß, Volker Freudenthaler, Carlos Toledano, Rodanthi-Elisavet Mamouri, David A. Farrell, Damien A. Prescod, Eleni Marinou, Sharon P. Burton, Josef Gasteiger, Ronny Engelmann, and Holger Baars
Atmos. Chem. Phys., 17, 10767–10794, https://doi.org/10.5194/acp-17-10767-2017, https://doi.org/10.5194/acp-17-10767-2017, 2017
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Our measurements performed with a lidar on Barbados give a vertical profile of Saharan dust, which was transported over 5000 km across the Atlantic. The new triple-wavelength depolarization technique reveals more information about the shape and size of dust, which will improve our understanding of the aging process of dust in the atmosphere and its representation in dust models. Changing properties of dust particles influence the solar radiation and the cloud properties and thus our climate.
Panagiotis G. Kosmopoulos, Stelios Kazadzis, Michael Taylor, Eleni Athanasopoulou, Orestis Speyer, Panagiotis I. Raptis, Eleni Marinou, Emmanouil Proestakis, Stavros Solomos, Evangelos Gerasopoulos, Vassilis Amiridis, Alkiviadis Bais, and Charalabos Kontoes
Atmos. Meas. Tech., 10, 2435–2453, https://doi.org/10.5194/amt-10-2435-2017, https://doi.org/10.5194/amt-10-2435-2017, 2017
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We study the impact of dust on solar energy using remote sensing data in conjunction with synergistic modelling and forecasting techniques. Under high aerosol loads, we found great solar energy losses of the order of 80 and 50% for concentrated solar power and photovoltaic installations, respectively. The 1-day forecast presented an overall accuracy within 10% in direct comparison to the real conditions under high energy potential, optimising the efficient energy planning and policies.
Nikolaos Siomos, Dimitris S. Balis, Anastasia Poupkou, Natalia Liora, Spyridon Dimopoulos, Dimitris Melas, Eleni Giannakaki, Maria Filioglou, Sara Basart, and Anatoli Chaikovsky
Atmos. Chem. Phys., 17, 7003–7023, https://doi.org/10.5194/acp-17-7003-2017, https://doi.org/10.5194/acp-17-7003-2017, 2017
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This study presents an evaluation of an air quality model using aerosol measurements from radiometric and lidar data at Thessaloniki, Greece. The aerosol mass concentration profiles of CAMx are compared against the fine and coarse mode aerosol concentration profiles retrieved by the Lidar-Radiometer Inversion Code (LIRIC). The CAMx model and the LIRIC algorithm results were compared in terms of mean mass concentration profiles, center of mass and integrated mass concentration.
Eleni Marinou, Vassilis Amiridis, Ioannis Binietoglou, Athanasios Tsikerdekis, Stavros Solomos, Emannouil Proestakis, Dimitra Konsta, Nikolaos Papagiannopoulos, Alexandra Tsekeri, Georgia Vlastou, Prodromos Zanis, Dimitrios Balis, Ulla Wandinger, and Albert Ansmann
Atmos. Chem. Phys., 17, 5893–5919, https://doi.org/10.5194/acp-17-5893-2017, https://doi.org/10.5194/acp-17-5893-2017, 2017
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We provide a 3D multiyear analysis on the evolution of Saharan dust over Europe, using a dust product retrieved from the CALIPSO satellite and using EARLINET methods. The results reveal for the first time the 9-year 3D seasonal patterns of dust over its transport paths from the Sahara towards the Mediterranean. The dataset is unique with respect to its potential applications, including the evaluation of dust models and the estimation of ice nuclei concentration profiles from space.
Jann Schrod, Daniel Weber, Jaqueline Drücke, Christos Keleshis, Michael Pikridas, Martin Ebert, Bojan Cvetković, Slobodan Nickovic, Eleni Marinou, Holger Baars, Albert Ansmann, Mihalis Vrekoussis, Nikos Mihalopoulos, Jean Sciare, Joachim Curtius, and Heinz G. Bingemer
Atmos. Chem. Phys., 17, 4817–4835, https://doi.org/10.5194/acp-17-4817-2017, https://doi.org/10.5194/acp-17-4817-2017, 2017
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In this paper we present data of ice-nucleating particles (INPs) from a 1-month campaign in the Eastern Mediterranean using unmanned aircraft systems (UASs, drones) and offline sampling with subsequent laboratory analysis. To our knowledge, this is the first time INPs were measured onboard a UAS. We find that INP concentrations were 1 magnitude higher aloft than at the ground, highlighting that surface-based measurement of INP may only be of limited significance for the situation at cloud level.
Stavros Solomos, Albert Ansmann, Rodanthi-Elisavet Mamouri, Ioannis Binietoglou, Platon Patlakas, Eleni Marinou, and Vassilis Amiridis
Atmos. Chem. Phys., 17, 4063–4079, https://doi.org/10.5194/acp-17-4063-2017, https://doi.org/10.5194/acp-17-4063-2017, 2017
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An extreme dust storm affected Middle East and the Eastern Mediterranean in September 2015. This event was produced by a combination of meteorological and land-use properties. Analysis with remote sensing observations and modeling simulations reveals (i) transport of warm moist air from the Red and Arabian seas, (ii) formation of a thermal low over Syria, (iii) convective outflows and haboob formation (i.e. propagating dust walls), and (iv) changes in land-use and dust erodibility due to war.
Alejandro Marti, Arnau Folch, Oriol Jorba, and Zavisa Janjic
Atmos. Chem. Phys., 17, 4005–4030, https://doi.org/10.5194/acp-17-4005-2017, https://doi.org/10.5194/acp-17-4005-2017, 2017
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We describe and evaluate NMMB-MONARCH-ASH, a novel online multi-scale meteorological and transport model developed at the BSC-CNS capable of forecasting the dispersal and deposition of volcanic ash. The forecast skills of the model have been validated and they improve on those from traditional operational offline (decoupled) models. The results support the use of online coupled models to aid civil aviation and emergency management during a crisis such as the 2010 eruption of Eyjafjallajökull.
Evangelia Diapouli, Manousos I. Manousakas, Stergios Vratolis, Vasiliki Vasilatou, Stella Pateraki, Kyriaki A. Bairachtari, Xavier Querol, Fulvio Amato, Andrés Alastuey, Angeliki A. Karanasiou, Franco Lucarelli, Silvia Nava, Giulia Calzolai, Vorne L. Gianelle, Cristina Colombi, Célia Alves, Danilo Custódio, Casimiro Pio, Christos Spyrou, George B. Kallos, and Konstantinos Eleftheriadis
Atmos. Chem. Phys., 17, 3673–3685, https://doi.org/10.5194/acp-17-3673-2017, https://doi.org/10.5194/acp-17-3673-2017, 2017
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This study examined the contribution of two natural sources (long-range transport of African dust and sea salt) to the airborne particulate matter concentrations, in 5 southern European cities (Porto, Barcelona, Milan, Florence, Athens). The results demonstrated that natural sources are often expressed with high-intensity events, leading even to exceedances of the EU air quality standards. This effect was more pronounced in the case of African dust intrusions in the eastern Mediterranean area.
Enza Di Tomaso, Nick A. J. Schutgens, Oriol Jorba, and Carlos Pérez García-Pando
Geosci. Model Dev., 10, 1107–1129, https://doi.org/10.5194/gmd-10-1107-2017, https://doi.org/10.5194/gmd-10-1107-2017, 2017
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A data assimilation capability has been built for a chemical weather prediction system, with a focus on mineral dust. Before this work, dust was produced uniquely from model estimated emissions. As emissions are recognized as a major factor limiting the accuracy of dust modelling, satellite observations have been used to improve the description of the atmospheric dust load, with a significant impact on dust forecast from assimilating observations particularly relevant for dust applications.
Thomas Carlund, Natalia Kouremeti, Stelios Kazadzis, and Julian Gröbner
Atmos. Meas. Tech., 10, 905–923, https://doi.org/10.5194/amt-10-905-2017, https://doi.org/10.5194/amt-10-905-2017, 2017
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Aerosols play an important role in atmospheric processes. Aerosol optical depth is the most common measure of columnar aerosol load. We present a sunphotometer called UVPFR that is able to measure aerosol optical depth in the ultraviolet range, including the calibration, characterization and validation of the instrument/measurements. The instrument will serve as a reference on the intercalibration of Brewer spectrophotometers that are also able to measure aerosol optical depth in the UV region.
Julien Chimot, J. Pepijn Veefkind, Tim Vlemmix, Johan F. de Haan, Vassilis Amiridis, Emmanouil Proestakis, Eleni Marinou, and Pieternel F. Levelt
Atmos. Meas. Tech., 10, 783–809, https://doi.org/10.5194/amt-10-783-2017, https://doi.org/10.5194/amt-10-783-2017, 2017
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We have developed artificial neural network algorithms to retrieve aerosol layer height from satellite OMI observations of the 477 nm O2–O2 spectral band. Based on 3-year (2005–2007) cloud-free scenes over north-east Asia, the results show uncertainties of 260–800 m when aerosol optical thickness is larger than 1. These algorithms also enable aerosol optical thickness retrievals by exploring the OMI continuum reflectance. These results may be used for future trace gas retrievals from TROPOMI.
Xavier Querol, Gotzon Gangoiti, Enrique Mantilla, Andrés Alastuey, Maria Cruz Minguillón, Fulvio Amato, Cristina Reche, Mar Viana, Teresa Moreno, Angeliki Karanasiou, Ioar Rivas, Noemí Pérez, Anna Ripoll, Mariola Brines, Marina Ealo, Marco Pandolfi, Hong-Ku Lee, Hee-Ram Eun, Yong-Hee Park, Miguel Escudero, David Beddows, Roy M. Harrison, Amelie Bertrand, Nicolas Marchand, Andrei Lyasota, Bernat Codina, Miriam Olid, Mireia Udina, Bernat Jiménez-Esteve, María R. Soler, Lucio Alonso, Millán Millán, and Kang-Ho Ahn
Atmos. Chem. Phys., 17, 2817–2838, https://doi.org/10.5194/acp-17-2817-2017, https://doi.org/10.5194/acp-17-2817-2017, 2017
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High summer O3 episodes in NE Spain were analysed. We evidence the relevance of local emission of precursors in meteorological scenarios of vertical air mass recirculations, when transboundary contributions are also significant. Forecasting these scenarios and sensitivity analysis of possible O3 precursors drop are key for potential abatement strategies. However, this is a very difficult task due to the complexity of scenarios, the external contributions, and the complex O3 production reactions.
Alba Badia, Oriol Jorba, Apostolos Voulgarakis, Donald Dabdub, Carlos Pérez García-Pando, Andreas Hilboll, María Gonçalves, and Zavisa Janjic
Geosci. Model Dev., 10, 609–638, https://doi.org/10.5194/gmd-10-609-2017, https://doi.org/10.5194/gmd-10-609-2017, 2017
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This paper presents a comprehensive description and benchmark evaluation of the tropospheric gas-phase chemistry component of the Multiscale Online Nonhydrostatic AtmospheRe CHemistry model (NMMB-MONARCH), an online chemical weather prediction system conceived for both the regional and global scales. We provide an extensive evaluation of a global annual cycle simulation using a variety of background surface stations, ozonesondes, aircraft data and satellite observations.
Athanasios Tsikerdekis, Prodromos Zanis, Allison L. Steiner, Fabien Solmon, Vassilis Amiridis, Eleni Marinou, Eleni Katragkou, Theodoros Karacostas, and Gilles Foret
Atmos. Chem. Phys., 17, 769–791, https://doi.org/10.5194/acp-17-769-2017, https://doi.org/10.5194/acp-17-769-2017, 2017
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Dust is the most abundant aerosol in the atmosphere, considerably affecting Earth's climate. We use a new dust size discretization that improves the physical representation of dust in a regional climate model. This study is among the first studies evaluating the vertical profile of simulated dust with a pure dust product. The new dust size discretization increases dust optical depth by 10 % over the desert and Mediterranean. Consequently, the dust SW and LW radiative forcing is enhanced by 10 %.
Alexandra Tsekeri, Vassilis Amiridis, Franco Marenco, Athanasios Nenes, Eleni Marinou, Stavros Solomos, Phil Rosenberg, Jamie Trembath, Graeme J. Nott, James Allan, Michael Le Breton, Asan Bacak, Hugh Coe, Carl Percival, and Nikolaos Mihalopoulos
Atmos. Meas. Tech., 10, 83–107, https://doi.org/10.5194/amt-10-83-2017, https://doi.org/10.5194/amt-10-83-2017, 2017
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The In situ/Remote sensing aerosol Retrieval Algorithm (IRRA) provides vertical profiles of aerosol optical, microphysical and hygroscopic properties from airborne in situ and remote sensing measurements. The algorithm is highly advantageous for aerosol characterization in humid conditions, employing the ISORROPIA II model for acquiring the particle hygroscopic growth. IRRA can find valuable applications in aerosol–cloud interaction schemes and in validation of active space-borne sensors.
Ioannis Kioutsioukis, Ulas Im, Efisio Solazzo, Roberto Bianconi, Alba Badia, Alessandra Balzarini, Rocío Baró, Roberto Bellasio, Dominik Brunner, Charles Chemel, Gabriele Curci, Hugo Denier van der Gon, Johannes Flemming, Renate Forkel, Lea Giordano, Pedro Jiménez-Guerrero, Marcus Hirtl, Oriol Jorba, Astrid Manders-Groot, Lucy Neal, Juan L. Pérez, Guidio Pirovano, Roberto San Jose, Nicholas Savage, Wolfram Schroder, Ranjeet S. Sokhi, Dimiter Syrakov, Paolo Tuccella, Johannes Werhahn, Ralf Wolke, Christian Hogrefe, and Stefano Galmarini
Atmos. Chem. Phys., 16, 15629–15652, https://doi.org/10.5194/acp-16-15629-2016, https://doi.org/10.5194/acp-16-15629-2016, 2016
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Four ensemble methods are applied to two annual AQMEII datasets and their performance is compared for O3, NO2 and PM10. The goal of the study is to quantify to what extent we can extract predictable signals from an ensemble with superior skill at each station over the single models and the ensemble mean. The promotion of the right amount of accuracy and diversity within the ensemble results in an average additional skill of up to 31 % compared to using the full ensemble in an unconditional way.
Stelios Kazadzis, Panagiotis Raptis, Natalia Kouremeti, Vassilis Amiridis, Antti Arola, Evangelos Gerasopoulos, and Gregory L. Schuster
Atmos. Meas. Tech., 9, 5997–6011, https://doi.org/10.5194/amt-9-5997-2016, https://doi.org/10.5194/amt-9-5997-2016, 2016
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Aerosols play an important role in the Earth's climate. One of the main aerosol properties is the single scattering albedo which is a measure of the aerosol absorption. In this work we have presented a method to retrieve this aerosol property in the ultraviolet and we presented the results for measurements at the urban environment of Athens, Greece. We show that the spectral dependence of the aerosol absorption in the VIS–IR and the UV range depends on the aerosol composition and type.
Aristeidis K. Georgoulias, Georgia Alexandri, Konstantinos A. Kourtidis, Jos Lelieveld, Prodromos Zanis, Ulrich Pöschl, Robert Levy, Vassilis Amiridis, Eleni Marinou, and Athanasios Tsikerdekis
Atmos. Chem. Phys., 16, 13853–13884, https://doi.org/10.5194/acp-16-13853-2016, https://doi.org/10.5194/acp-16-13853-2016, 2016
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In this work, single pixel observations from MODIS Terra and Aqua are analyzed together with data from other satellite sensors, reanalysis projects and a chemistry–aerosol-transport model to study the spatiotemporal variability of different aerosol types. The results are in accordance with previous works and are a good reference for future studies in the area focusing on aerosols, clouds, radiation and the effects of particle pollution on human health.
Bertrand Bessagnet, Guido Pirovano, Mihaela Mircea, Cornelius Cuvelier, Armin Aulinger, Giuseppe Calori, Giancarlo Ciarelli, Astrid Manders, Rainer Stern, Svetlana Tsyro, Marta García Vivanco, Philippe Thunis, Maria-Teresa Pay, Augustin Colette, Florian Couvidat, Frédérik Meleux, Laurence Rouïl, Anthony Ung, Sebnem Aksoyoglu, José María Baldasano, Johannes Bieser, Gino Briganti, Andrea Cappelletti, Massimo D'Isidoro, Sandro Finardi, Richard Kranenburg, Camillo Silibello, Claudio Carnevale, Wenche Aas, Jean-Charles Dupont, Hilde Fagerli, Lucia Gonzalez, Laurent Menut, André S. H. Prévôt, Pete Roberts, and Les White
Atmos. Chem. Phys., 16, 12667–12701, https://doi.org/10.5194/acp-16-12667-2016, https://doi.org/10.5194/acp-16-12667-2016, 2016
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The EURODELTA III exercise allows a very comprehensive intercomparison and evaluation of air quality models' performance. On average, the models provide a rather good picture of the particulate matter (PM) concentrations over Europe even if the highest concentrations are underestimated. The meteorology is responsible for model discrepancies, while the lack of emissions, particularly in winter, is mentioned as the main reason for the underestimations of PM.
Marina Ealo, Andrés Alastuey, Anna Ripoll, Noemí Pérez, María Cruz Minguillón, Xavier Querol, and Marco Pandolfi
Atmos. Chem. Phys., 16, 12567–12586, https://doi.org/10.5194/acp-16-12567-2016, https://doi.org/10.5194/acp-16-12567-2016, 2016
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The present work demonstrates the potential of in situ aerosol optical measurements, from both nephelometer and aethalometer instruments, for detecting specific air pollution scenarios in near real time. Given the high sensitivity of the intensive aerosol optical properties to characterize atmospheric aerosols, these parameters were calibrated in order to detect Saharan dust and biomass burning events at regional (Montseny) and continental (Montsec) environments in the NW Mediterranean.
Marco Pandolfi, Andrés Alastuey, Noemi Pérez, Cristina Reche, Iria Castro, Victor Shatalov, and Xavier Querol
Atmos. Chem. Phys., 16, 11787–11805, https://doi.org/10.5194/acp-16-11787-2016, https://doi.org/10.5194/acp-16-11787-2016, 2016
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The ambient concentration of many air pollutants in Europe has decreased in these last decades thanks to the effectiveness of the pollution control measures implemented at European or regional/local levels. In this work we studied the trends of the concentrations of many different pollutants during the period 2004–2014, reporting on the type of trend, magnitude of the trend, and its statistical significance. Data from two twin sites in NE Spain (regional and urban background) were used.
María José Granados-Muñoz, Francisco Navas-Guzmán, Juan Luis Guerrero-Rascado, Juan Antonio Bravo-Aranda, Ioannis Binietoglou, Sergio Nepomuceno Pereira, Sara Basart, José María Baldasano, Livio Belegante, Anatoli Chaikovsky, Adolfo Comerón, Giuseppe D'Amico, Oleg Dubovik, Luka Ilic, Panos Kokkalis, Constantino Muñoz-Porcar, Slobodan Nickovic, Doina Nicolae, Francisco José Olmo, Alexander Papayannis, Gelsomina Pappalardo, Alejandro Rodríguez, Kerstin Schepanski, Michaël Sicard, Ana Vukovic, Ulla Wandinger, François Dulac, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 16, 7043–7066, https://doi.org/10.5194/acp-16-7043-2016, https://doi.org/10.5194/acp-16-7043-2016, 2016
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This study provides a detailed overview of the Mediterranean region regarding aerosol microphysical properties during the ChArMEx/EMEP campaign in July 2012. An in-depth analysis of the horizontal, vertical, and temporal dimensions is performed using LIRIC, proving the algorithm's ability in automated retrieval of microphysical property profiles within a network. A validation of four dust models is included, obtaining fair good agreement, especially for the vertical distribution of the aerosol.
Mariola Brines, Manuel Dall'Osto, Fulvio Amato, María Cruz Minguillón, Angeliki Karanasiou, Andrés Alastuey, and Xavier Querol
Atmos. Chem. Phys., 16, 6785–6804, https://doi.org/10.5194/acp-16-6785-2016, https://doi.org/10.5194/acp-16-6785-2016, 2016
Andrés Alastuey, Xavier Querol, Wenche Aas, Franco Lucarelli, Noemí Pérez, Teresa Moreno, Fabrizia Cavalli, Hans Areskoug, Violeta Balan, Maria Catrambone, Darius Ceburnis, José C. Cerro, Sébastien Conil, Lusine Gevorgyan, Christoph Hueglin, Kornelia Imre, Jean-Luc Jaffrezo, Sarah R. Leeson, Nikolaos Mihalopoulos, Marta Mitosinkova, Colin D. O'Dowd, Jorge Pey, Jean-Philippe Putaud, Véronique Riffault, Anna Ripoll, Jean Sciare, Karine Sellegri, Gerald Spindler, and Karl Espen Yttri
Atmos. Chem. Phys., 16, 6107–6129, https://doi.org/10.5194/acp-16-6107-2016, https://doi.org/10.5194/acp-16-6107-2016, 2016
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Mineral dust content in PM10 was analysed at 20 regional background sites across Europe. Higher dust loadings were observed at most sites in summer, with the most elevated concentrations in the southern- and easternmost countries, due to external and regional sources. Saharan dust outbreaks impacted western and central European in summer and eastern Mediterranean sites in winter. The spatial distribution of some metals reveals the influence of specific anthropogenic sources on a regional scale.
Henri Diémoz, Kostas Eleftheratos, Stelios Kazadzis, Vassilis Amiridis, and Christos S. Zerefos
Atmos. Meas. Tech., 9, 1871–1888, https://doi.org/10.5194/amt-9-1871-2016, https://doi.org/10.5194/amt-9-1871-2016, 2016
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A new algorithm allowed to retrieve aerosol optical depths from a Brewer spectrophotometer in Athens with excellent agreement with AERONET. The instrument radiometric stability and the performances of in situ Langley extrapolations as a way to track it are investigated. Potential sources of error and recommendations to operators are reported. MkIV Brewers represent a great source of information about aerosols in the past decades and a promising worldwide network for coordinated AOD measurements.
Holger Baars, Thomas Kanitz, Ronny Engelmann, Dietrich Althausen, Birgit Heese, Mika Komppula, Jana Preißler, Matthias Tesche, Albert Ansmann, Ulla Wandinger, Jae-Hyun Lim, Joon Young Ahn, Iwona S. Stachlewska, Vassilis Amiridis, Eleni Marinou, Patric Seifert, Julian Hofer, Annett Skupin, Florian Schneider, Stephanie Bohlmann, Andreas Foth, Sebastian Bley, Anne Pfüller, Eleni Giannakaki, Heikki Lihavainen, Yrjö Viisanen, Rakesh Kumar Hooda, Sérgio Nepomuceno Pereira, Daniele Bortoli, Frank Wagner, Ina Mattis, Lucja Janicka, Krzysztof M. Markowicz, Peggy Achtert, Paulo Artaxo, Theotonio Pauliquevis, Rodrigo A. F. Souza, Ved Prakesh Sharma, Pieter Gideon van Zyl, Johan Paul Beukes, Junying Sun, Erich G. Rohwer, Ruru Deng, Rodanthi-Elisavet Mamouri, and Felix Zamorano
Atmos. Chem. Phys., 16, 5111–5137, https://doi.org/10.5194/acp-16-5111-2016, https://doi.org/10.5194/acp-16-5111-2016, 2016
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The findings from more than 10 years of global aerosol lidar measurements with Polly systems are summarized, and a data set of optical properties for specific aerosol types is given. An automated data retrieval algorithm for continuous Polly lidar observations is presented and discussed by means of a Saharan dust advection event in Leipzig, Germany. Finally, a statistic on the vertical aerosol distribution including the seasonal variability at PollyNET locations around the globe is presented.
Ronny Engelmann, Thomas Kanitz, Holger Baars, Birgit Heese, Dietrich Althausen, Annett Skupin, Ulla Wandinger, Mika Komppula, Iwona S. Stachlewska, Vassilis Amiridis, Eleni Marinou, Ina Mattis, Holger Linné, and Albert Ansmann
Atmos. Meas. Tech., 9, 1767–1784, https://doi.org/10.5194/amt-9-1767-2016, https://doi.org/10.5194/amt-9-1767-2016, 2016
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The atmospheric science community demands for autonomous and quality-assured vertically resolved measurements of aerosol and cloud properties. For this purpose, a portable lidar called Polly
was developed at TROPOS in 2003. This lidar type was continuously improved with gained experience from EARLINET, worldwide field campaigns, and institute collaborations within the last 10 years. We present recent changes to the setup of our portable multiwavelength Raman and polarization lidar PollyXT.
E. Cuevas, Á. J. Gómez-Peláez, S. Rodríguez, E. Terradellas, S. Basart, R. D. García, O. E. García, and S. Alonso-Pérez
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-287, https://doi.org/10.5194/acp-2016-287, 2016
Revised manuscript not accepted
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We revise the North African Dipole Intensity (NAFDI) index, and explain and quantify its relationship with the Saharan Heat Low (SHL) and mid-latitude Rossby waves. An analysis of aerosol optical depth anomalies over Northern Africa is performed for each phase of NAFDI/SHL. A comprehensive top-down conceptual model is introduced to explain the relationships between the NAFDI, the SHL and the mid-latitude Rossby waves and their impact in dust mobilization and transport in Northern Africa.
N. Huneeus, S. Basart, S. Fiedler, J.-J. Morcrette, A. Benedetti, J. Mulcahy, E. Terradellas, C. Pérez García-Pando, G. Pejanovic, S. Nickovic, P. Arsenovic, M. Schulz, E. Cuevas, J. M. Baldasano, J. Pey, S. Remy, and B. Cvetkovic
Atmos. Chem. Phys., 16, 4967–4986, https://doi.org/10.5194/acp-16-4967-2016, https://doi.org/10.5194/acp-16-4967-2016, 2016
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Five dust models are evaluated regarding their performance in predicting an intense Saharan dust outbreak affecting western and northern Europe (NE). Models predict the onset and evolution of the event for all analysed lead times. On average, differences among the models are larger than differences in lead times for each model. The models tend to underestimate the long-range transport towards NE. This is partly due to difficulties in simulating the vertical dust distribution and horizontal wind.
Anatoli Chaikovsky, Oleg Dubovik, Brent Holben, Andrey Bril, Philippe Goloub, Didier Tanré, Gelsomina Pappalardo, Ulla Wandinger, Ludmila Chaikovskaya, Sergey Denisov, Jan Grudo, Anton Lopatin, Yana Karol, Tatsiana Lapyonok, Vassilis Amiridis, Albert Ansmann, Arnoud Apituley, Lucas Allados-Arboledas, Ioannis Binietoglou, Antonella Boselli, Giuseppe D'Amico, Volker Freudenthaler, David Giles, María José Granados-Muñoz, Panayotis Kokkalis, Doina Nicolae, Sergey Oshchepkov, Alex Papayannis, Maria Rita Perrone, Alexander Pietruczuk, Francesc Rocadenbosch, Michaël Sicard, Ilya Slutsker, Camelia Talianu, Ferdinando De Tomasi, Alexandra Tsekeri, Janet Wagner, and Xuan Wang
Atmos. Meas. Tech., 9, 1181–1205, https://doi.org/10.5194/amt-9-1181-2016, https://doi.org/10.5194/amt-9-1181-2016, 2016
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This paper presents a detailed description of LIRIC (LIdar-Radiometer Inversion Code) algorithm for simultaneous processing of coincident lidar and radiometric observations for the retrieval of the aerosol concentrations. As the lidar/radiometric input data we use measurements from European Aerosol Research Lidar Network (EARLINET) lidars and collocated sun-photometers of Aerosol Robotic Network (AERONET). The LIRIC software package was implemented and tested at a number of EARLINET stations.
Fulvio Amato, Andrés Alastuey, Angeliki Karanasiou, Franco Lucarelli, Silvia Nava, Giulia Calzolai, Mirko Severi, Silvia Becagli, Vorne L. Gianelle, Cristina Colombi, Celia Alves, Danilo Custódio, Teresa Nunes, Mario Cerqueira, Casimiro Pio, Konstantinos Eleftheriadis, Evangelia Diapouli, Cristina Reche, María Cruz Minguillón, Manousos-Ioannis Manousakas, Thomas Maggos, Stergios Vratolis, Roy M. Harrison, and Xavier Querol
Atmos. Chem. Phys., 16, 3289–3309, https://doi.org/10.5194/acp-16-3289-2016, https://doi.org/10.5194/acp-16-3289-2016, 2016
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Harmonized source apportionment of atmospheric particulate matter (PM10 and PM2.5) at 5 EU cities (Barcelona, Florence, Milan, Athens and Porto) reveals that vehicle exhaust (excluding nitrate) plus non-exhaust contributes 16–32 % to PM10 and 15–36 % to PM2.5. Secondary PM represents 37–82 % of PM2.5. Biomass burning varies from < 2 to 24 % of PM10, depending on the residential heating fuel. Other sources are local dust (7–19 % of PM10), industries (4–11 % of PM10), shipping, sea salt and Saharan dust.
Nikolaos Papagiannopoulos, Lucia Mona, Lucas Alados-Arboledas, Vassilis Amiridis, Holger Baars, Ioannis Binietoglou, Daniele Bortoli, Giuseppe D'Amico, Aldo Giunta, Juan Luis Guerrero-Rascado, Anja Schwarz, Sergio Pereira, Nicola Spinelli, Ulla Wandinger, Xuan Wang, and Gelsomina Pappalardo
Atmos. Chem. Phys., 16, 2341–2357, https://doi.org/10.5194/acp-16-2341-2016, https://doi.org/10.5194/acp-16-2341-2016, 2016
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Satellite-derived products must undergo data evaluation with reference data sets in order to identify any possible reasons of discrepancy or to assess their representativity. In that direction, data coming from CALIPSO satellite were compared with observations from the ground. We identified a CALIPSO underestimation that could be linked to an assumption in the satellites' algorithms. The proposed correction improves the performance and could enhance aerosol modeling.
A. S. Fonseca, N. Talbot, J. Schwarz, J. Ondráček, V. Ždímal, J. Kozáková, M. Viana, A. Karanasiou, X. Querol, A. Alastuey, T. V. Vu, J. M. Delgado-Saborit, and R. M. Harrison
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2015-1016, https://doi.org/10.5194/acp-2015-1016, 2016
Revised manuscript not accepted
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This work assessed the performance of 4 cascade impactors, by means of two intercomparison exercises in 2 European locations. The comparability between the different types of impactors assessed was dependent on particle size and on impactor design characteristics. Particle processes such as particle bounce, dissociation of semi volatiles in the coarser stages and/or particle shrinkage were identified as the main causes for the differences observed in particle mass across size fractions.
M. B. Korras-Carraca, N. Hatzianastassiou, C. Matsoukas, A. Gkikas, and C. D. Papadimas
Atmos. Chem. Phys., 15, 13113–13132, https://doi.org/10.5194/acp-15-13113-2015, https://doi.org/10.5194/acp-15-13113-2015, 2015
M. Sicard, G. D'Amico, A. Comerón, L. Mona, L. Alados-Arboledas, A. Amodeo, H. Baars, J. M. Baldasano, L. Belegante, I. Binietoglou, J. A. Bravo-Aranda, A. J. Fernández, P. Fréville, D. García-Vizcaíno, A. Giunta, M. J. Granados-Muñoz, J. L. Guerrero-Rascado, D. Hadjimitsis, A. Haefele, M. Hervo, M. Iarlori, P. Kokkalis, D. Lange, R. E. Mamouri, I. Mattis, F. Molero, N. Montoux, A. Muñoz, C. Muñoz Porcar, F. Navas-Guzmán, D. Nicolae, A. Nisantzi, N. Papagiannopoulos, A. Papayannis, S. Pereira, J. Preißler, M. Pujadas, V. Rizi, F. Rocadenbosch, K. Sellegri, V. Simeonov, G. Tsaknakis, F. Wagner, and G. Pappalardo
Atmos. Meas. Tech., 8, 4587–4613, https://doi.org/10.5194/amt-8-4587-2015, https://doi.org/10.5194/amt-8-4587-2015, 2015
Short summary
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In the framework of the ACTRIS summer 2012 measurement campaign (8 June–17 July 2012), EARLINET organized and performed a controlled exercise of feasibility to demonstrate its potential to perform operational, coordinated measurements and deliver products in near-real time. The paper describes the measurement protocol and discusses the delivery of real-time and near-real-time lidar-derived products.
I. Binietoglou, S. Basart, L. Alados-Arboledas, V. Amiridis, A. Argyrouli, H. Baars, J. M. Baldasano, D. Balis, L. Belegante, J. A. Bravo-Aranda, P. Burlizzi, V. Carrasco, A. Chaikovsky, A. Comerón, G. D'Amico, M. Filioglou, M. J. Granados-Muñoz, J. L. Guerrero-Rascado, L. Ilic, P. Kokkalis, A. Maurizi, L. Mona, F. Monti, C. Muñoz-Porcar, D. Nicolae, A. Papayannis, G. Pappalardo, G. Pejanovic, S. N. Pereira, M. R. Perrone, A. Pietruczuk, M. Posyniak, F. Rocadenbosch, A. Rodríguez-Gómez, M. Sicard, N. Siomos, A. Szkop, E. Terradellas, A. Tsekeri, A. Vukovic, U. Wandinger, and J. Wagner
Atmos. Meas. Tech., 8, 3577–3600, https://doi.org/10.5194/amt-8-3577-2015, https://doi.org/10.5194/amt-8-3577-2015, 2015
S. Rodríguez, E. Cuevas, J. M. Prospero, A. Alastuey, X. Querol, J. López-Solano, M. I. García, and S. Alonso-Pérez
Atmos. Chem. Phys., 15, 7471–7486, https://doi.org/10.5194/acp-15-7471-2015, https://doi.org/10.5194/acp-15-7471-2015, 2015
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Long-term 28-year variability of Saharan dust export to the Atlantic is correlated with large-scale meteorology in North Africa, particularly with the intensity of the Saharan high to tropical low dipole-like pattern, the so-called North African Dipole. Variability in the dipole intensity is connected with winds, monsoon rain band and latitudinal shifts of the Saharan air layer. Variability in the dipole intensity suggests connections with ENSO and the Sahel drought.
V. Amiridis, E. Marinou, A. Tsekeri, U. Wandinger, A. Schwarz, E. Giannakaki, R. Mamouri, P. Kokkalis, I. Binietoglou, S. Solomos, T. Herekakis, S. Kazadzis, E. Gerasopoulos, E. Proestakis, M. Kottas, D. Balis, A. Papayannis, C. Kontoes, K. Kourtidis, N. Papagiannopoulos, L. Mona, G. Pappalardo, O. Le Rille, and A. Ansmann
Atmos. Chem. Phys., 15, 7127–7153, https://doi.org/10.5194/acp-15-7127-2015, https://doi.org/10.5194/acp-15-7127-2015, 2015
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LIVAS is a 3-D multi-wavelength global aerosol and cloud optical database optimized for future space-based lidar end-to-end simulations of realistic atmospheric scenarios as well as retrieval algorithm testing activities. The global database is based on CALIPSO observations at 532nm, while for the conversion at 355nm EARLINET data are utilized.
M. C. Minguillón, A. Ripoll, N. Pérez, A. S. H. Prévôt, F. Canonaco, X. Querol, and A. Alastuey
Atmos. Chem. Phys., 15, 6379–6391, https://doi.org/10.5194/acp-15-6379-2015, https://doi.org/10.5194/acp-15-6379-2015, 2015
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The study focuses on the aerosol variations found in the regional background of the western Mediterranean basin and their relation with atmospheric conditions and scenarios. An Aerosol Chemical Speciation Monitor (ACSM) was deployed for 1 year and the results were validated with co-located PM1 measurements. The organic sources were investigated and the local secondary organic aerosol (SOA) formation was estimated.
M. Brines, M. Dall'Osto, D. C. S. Beddows, R. M. Harrison, F. Gómez-Moreno, L. Núñez, B. Artíñano, F. Costabile, G. P. Gobbi, F. Salimi, L. Morawska, C. Sioutas, and X. Querol
Atmos. Chem. Phys., 15, 5929–5945, https://doi.org/10.5194/acp-15-5929-2015, https://doi.org/10.5194/acp-15-5929-2015, 2015
E. Cuevas, C. Camino, A. Benedetti, S. Basart, E. Terradellas, J. M. Baldasano, J. J. Morcrette, B. Marticorena, P. Goloub, A. Mortier, A. Berjón, Y. Hernández, M. Gil-Ojeda, and M. Schulz
Atmos. Chem. Phys., 15, 3991–4024, https://doi.org/10.5194/acp-15-3991-2015, https://doi.org/10.5194/acp-15-3991-2015, 2015
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Atmospheric mineral dust from a MACC-II short reanalysis (2007-2008) has been evaluated over northern Africa and the Middle East using satellite aerosol products, AERONET data, in situ PM10 concentrations, and extinction vertical profiles. The MACC-II AOD spatial and temporal variability shows good agreement with satellite sensors and AERONET. We find a good agreement in averaged extinction vertical profiles between MACC-II and lidars. MACC correctly reproduces daily to interannual PM10.
A. Ripoll, M. C. Minguillón, J. Pey, J. L. Jimenez, D. A. Day, Y. Sosedova, F. Canonaco, A. S. H. Prévôt, X. Querol, and A. Alastuey
Atmos. Chem. Phys., 15, 2935–2951, https://doi.org/10.5194/acp-15-2935-2015, https://doi.org/10.5194/acp-15-2935-2015, 2015
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Real-time measurements of inorganic (sulfate, nitrate, ammonium, chloride and black carbon (BC)) and organic submicron aerosols from a continental background site (Montsec, MSC, 1570m a.s.l.) in the western Mediterranean Basin (WMB) were conducted for 10 months (July 2011 - April 2012) with an aerosol chemical speciation monitor (ACSM). The ACSM was co-located with other online and offline PM1 measurements. Analyses of the hourly, diurnal, and seasonal variations are presented here.
A. Ripoll, M. C. Minguillón, J. Pey, N. Pérez, X. Querol, and A. Alastuey
Atmos. Chem. Phys., 15, 1129–1145, https://doi.org/10.5194/acp-15-1129-2015, https://doi.org/10.5194/acp-15-1129-2015, 2015
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Short summary
The complete chemical compositions of atmospheric particulate matter (PM1 and PM10) from a continental (Montsec, 1570 m a.s.l.) and a regional (Montseny, 720 m a.s.l) background site in the western Mediterranean Basin were jointly studied for the first time over a relatively long-term period (January 2010-March 2013). Results revealed a) a high relevance of African dust transport and regional dust resuspension; b) low biomass burning contribution; and c) high organic matter contribution.
W. R. Sessions, J. S. Reid, A. Benedetti, P. R. Colarco, A. da Silva, S. Lu, T. Sekiyama, T. Y. Tanaka, J. M. Baldasano, S. Basart, M. E. Brooks, T. F. Eck, M. Iredell, J. A. Hansen, O. C. Jorba, H.-M. H. Juang, P. Lynch, J.-J. Morcrette, S. Moorthi, J. Mulcahy, Y. Pradhan, M. Razinger, C. B. Sampson, J. Wang, and D. L. Westphal
Atmos. Chem. Phys., 15, 335–362, https://doi.org/10.5194/acp-15-335-2015, https://doi.org/10.5194/acp-15-335-2015, 2015
Short summary
F. Marenco, V. Amiridis, E. Marinou, A. Tsekeri, and J. Pelon
Atmos. Chem. Phys., 14, 11871–11881, https://doi.org/10.5194/acp-14-11871-2014, https://doi.org/10.5194/acp-14-11871-2014, 2014
C. Guirado, E. Cuevas, V. E. Cachorro, C. Toledano, S. Alonso-Pérez, J. J. Bustos, S. Basart, P. M. Romero, C. Camino, M. Mimouni, L. Zeudmi, P. Goloub, J. M. Baldasano, and A. M. de Frutos
Atmos. Chem. Phys., 14, 11753–11773, https://doi.org/10.5194/acp-14-11753-2014, https://doi.org/10.5194/acp-14-11753-2014, 2014
Short summary
Short summary
Tamanrasset, in the heart of the Sahara, is a key site for aerosol research. The analysis of more than 2 years (2006-2009) of AERONET and KCICLO-corrected sun photometer measurements shows that atmospheric aerosols at Tamanrasset are modulated by the Convective Boundary Layer leading to pure Saharan dust conditions (April-September) and very clear sky conditions (November-February). Dust potential sources and anthropogenic fine aerosols arriving at Tamanrasset are also identified.
M. Taylor, S. Kazadzis, A. Tsekeri, A. Gkikas, and V. Amiridis
Atmos. Meas. Tech., 7, 3151–3175, https://doi.org/10.5194/amt-7-3151-2014, https://doi.org/10.5194/amt-7-3151-2014, 2014
M. T. Pay, F. Martínez, M. Guevara, and J. M. Baldasano
Geosci. Model Dev., 7, 1979–1999, https://doi.org/10.5194/gmd-7-1979-2014, https://doi.org/10.5194/gmd-7-1979-2014, 2014
L. Mona, N. Papagiannopoulos, S. Basart, J. Baldasano, I. Binietoglou, C. Cornacchia, and G. Pappalardo
Atmos. Chem. Phys., 14, 8781–8793, https://doi.org/10.5194/acp-14-8781-2014, https://doi.org/10.5194/acp-14-8781-2014, 2014
G. Pappalardo, A. Amodeo, A. Apituley, A. Comeron, V. Freudenthaler, H. Linné, A. Ansmann, J. Bösenberg, G. D'Amico, I. Mattis, L. Mona, U. Wandinger, V. Amiridis, L. Alados-Arboledas, D. Nicolae, and M. Wiegner
Atmos. Meas. Tech., 7, 2389–2409, https://doi.org/10.5194/amt-7-2389-2014, https://doi.org/10.5194/amt-7-2389-2014, 2014
S. Kazadzis, I. Veselovskii, V. Amiridis, J. Gröbner, A. Suvorina, S. Nyeki, E. Gerasopoulos, N. Kouremeti, M. Taylor, A. Tsekeri, and C. Wehrli
Atmos. Meas. Tech., 7, 2013–2025, https://doi.org/10.5194/amt-7-2013-2014, https://doi.org/10.5194/amt-7-2013-2014, 2014
P. Salvador, S. Alonso-Pérez, J. Pey, B. Artíñano, J. J. de Bustos, A. Alastuey, and X. Querol
Atmos. Chem. Phys., 14, 6759–6775, https://doi.org/10.5194/acp-14-6759-2014, https://doi.org/10.5194/acp-14-6759-2014, 2014
M. Pandolfi, A. Ripoll, X. Querol, and A. Alastuey
Atmos. Chem. Phys., 14, 6443–6460, https://doi.org/10.5194/acp-14-6443-2014, https://doi.org/10.5194/acp-14-6443-2014, 2014
M. Viana, I. Rivas, X. Querol, A. Alastuey, J. Sunyer, M. Álvarez-Pedrerol, L. Bouso, and C. Sioutas
Atmos. Chem. Phys., 14, 4459–4472, https://doi.org/10.5194/acp-14-4459-2014, https://doi.org/10.5194/acp-14-4459-2014, 2014
A. Ripoll, J. Pey, M. C. Minguillón, N. Pérez, M. Pandolfi, X. Querol, and A. Alastuey
Atmos. Chem. Phys., 14, 4279–4295, https://doi.org/10.5194/acp-14-4279-2014, https://doi.org/10.5194/acp-14-4279-2014, 2014
F. Amato, A. Alastuey, J. de la Rosa, Y. Gonzalez Castanedo, A. M. Sánchez de la Campa, M. Pandolfi, A. Lozano, J. Contreras González, and X. Querol
Atmos. Chem. Phys., 14, 3533–3544, https://doi.org/10.5194/acp-14-3533-2014, https://doi.org/10.5194/acp-14-3533-2014, 2014
M. Taylor, S. Kazadzis, and E. Gerasopoulos
Atmos. Meas. Tech., 7, 839–858, https://doi.org/10.5194/amt-7-839-2014, https://doi.org/10.5194/amt-7-839-2014, 2014
M. Brines, M. Dall'Osto, D.C.S. Beddows, R. M. Harrison, and X. Querol
Atmos. Chem. Phys., 14, 2973–2986, https://doi.org/10.5194/acp-14-2973-2014, https://doi.org/10.5194/acp-14-2973-2014, 2014
C. S. Zerefos, P. Tetsis, A. Kazantzidis, V. Amiridis, S. C. Zerefos, J. Luterbacher, K. Eleftheratos, E. Gerasopoulos, S. Kazadzis, and A. Papayannis
Atmos. Chem. Phys., 14, 2987–3015, https://doi.org/10.5194/acp-14-2987-2014, https://doi.org/10.5194/acp-14-2987-2014, 2014
A. Baklanov, K. Schlünzen, P. Suppan, J. Baldasano, D. Brunner, S. Aksoyoglu, G. Carmichael, J. Douros, J. Flemming, R. Forkel, S. Galmarini, M. Gauss, G. Grell, M. Hirtl, S. Joffre, O. Jorba, E. Kaas, M. Kaasik, G. Kallos, X. Kong, U. Korsholm, A. Kurganskiy, J. Kushta, U. Lohmann, A. Mahura, A. Manders-Groot, A. Maurizi, N. Moussiopoulos, S. T. Rao, N. Savage, C. Seigneur, R. S. Sokhi, E. Solazzo, S. Solomos, B. Sørensen, G. Tsegas, E. Vignati, B. Vogel, and Y. Zhang
Atmos. Chem. Phys., 14, 317–398, https://doi.org/10.5194/acp-14-317-2014, https://doi.org/10.5194/acp-14-317-2014, 2014
V. Amiridis, U. Wandinger, E. Marinou, E. Giannakaki, A. Tsekeri, S. Basart, S. Kazadzis, A. Gkikas, M. Taylor, J. Baldasano, and A. Ansmann
Atmos. Chem. Phys., 13, 12089–12106, https://doi.org/10.5194/acp-13-12089-2013, https://doi.org/10.5194/acp-13-12089-2013, 2013
A. Gkikas, N. Hatzianastassiou, N. Mihalopoulos, V. Katsoulis, S. Kazadzis, J. Pey, X. Querol, and O. Torres
Atmos. Chem. Phys., 13, 12135–12154, https://doi.org/10.5194/acp-13-12135-2013, https://doi.org/10.5194/acp-13-12135-2013, 2013
M. Spada, O. Jorba, C. Pérez García-Pando, Z. Janjic, and J. M. Baldasano
Atmos. Chem. Phys., 13, 11735–11755, https://doi.org/10.5194/acp-13-11735-2013, https://doi.org/10.5194/acp-13-11735-2013, 2013
M. Alier, B. L. van Drooge, M. Dall'Osto, X. Querol, J. O. Grimalt, and R. Tauler
Atmos. Chem. Phys., 13, 10353–10371, https://doi.org/10.5194/acp-13-10353-2013, https://doi.org/10.5194/acp-13-10353-2013, 2013
M. Dall'Osto, X. Querol, A. Alastuey, M. C. Minguillon, M. Alier, F. Amato, M. Brines, M. Cusack, J. O. Grimalt, A. Karanasiou, T. Moreno, M. Pandolfi, J. Pey, C. Reche, A. Ripoll, R. Tauler, B. L. Van Drooge, M. Viana, R. M. Harrison, J. Gietl, D. Beddows, W. Bloss, C. O'Dowd, D. Ceburnis, G. Martucci, N. L. Ng, D. Worsnop, J. Wenger, E. Mc Gillicuddy, J. Sodeau, R. Healy, F. Lucarelli, S. Nava, J. L. Jimenez, F. Gomez Moreno, B. Artinano, A. S. H. Prévôt, L. Pfaffenberger, S. Frey, F. Wilsenack, D. Casabona, P. Jiménez-Guerrero, D. Gross, and N. Cots
Atmos. Chem. Phys., 13, 8991–9019, https://doi.org/10.5194/acp-13-8991-2013, https://doi.org/10.5194/acp-13-8991-2013, 2013
V. Pappas, N. Hatzianastassiou, C. Papadimas, C. Matsoukas, S. Kinne, and I. Vardavas
Atmos. Chem. Phys., 13, 8381–8399, https://doi.org/10.5194/acp-13-8381-2013, https://doi.org/10.5194/acp-13-8381-2013, 2013
G. P. Gobbi, F. Angelini, F. Barnaba, F. Costabile, J. M. Baldasano, S. Basart, R. Sozzi, and A. Bolignano
Atmos. Chem. Phys., 13, 7395–7404, https://doi.org/10.5194/acp-13-7395-2013, https://doi.org/10.5194/acp-13-7395-2013, 2013
X. Querol, A. Alastuey, M. Viana, T. Moreno, C. Reche, M. C. Minguillón, A. Ripoll, M. Pandolfi, F. Amato, A. Karanasiou, N. Pérez, J. Pey, M. Cusack, R. Vázquez, F. Plana, M. Dall'Osto, J. de la Rosa, A. Sánchez de la Campa, R. Fernández-Camacho, S. Rodríguez, C. Pio, L. Alados-Arboledas, G. Titos, B. Artíñano, P. Salvador, S. García Dos Santos, and R. Fernández Patier
Atmos. Chem. Phys., 13, 6185–6206, https://doi.org/10.5194/acp-13-6185-2013, https://doi.org/10.5194/acp-13-6185-2013, 2013
M. Cusack, N. Pérez, J. Pey, A. Alastuey, and X. Querol
Atmos. Chem. Phys., 13, 5173–5187, https://doi.org/10.5194/acp-13-5173-2013, https://doi.org/10.5194/acp-13-5173-2013, 2013
M. Pandolfi, G. Martucci, X. Querol, A. Alastuey, F. Wilsenack, S. Frey, C. D. O'Dowd, and M. Dall'Osto
Atmos. Chem. Phys., 13, 4983–4996, https://doi.org/10.5194/acp-13-4983-2013, https://doi.org/10.5194/acp-13-4983-2013, 2013
M. Dall'Osto, X. Querol, F. Amato, A. Karanasiou, F. Lucarelli, S. Nava, G. Calzolai, and M. Chiari
Atmos. Chem. Phys., 13, 4375–4392, https://doi.org/10.5194/acp-13-4375-2013, https://doi.org/10.5194/acp-13-4375-2013, 2013
A. V. Lindfors, N. Kouremeti, A. Arola, S. Kazadzis, A. F. Bais, and A. Laaksonen
Atmos. Chem. Phys., 13, 3733–3741, https://doi.org/10.5194/acp-13-3733-2013, https://doi.org/10.5194/acp-13-3733-2013, 2013
C. A. Randles, S. Kinne, G. Myhre, M. Schulz, P. Stier, J. Fischer, L. Doppler, E. Highwood, C. Ryder, B. Harris, J. Huttunen, Y. Ma, R. T. Pinker, B. Mayer, D. Neubauer, R. Hitzenberger, L. Oreopoulos, D. Lee, G. Pitari, G. Di Genova, J. Quaas, F. G. Rose, S. Kato, S. T. Rumbold, I. Vardavas, N. Hatzianastassiou, C. Matsoukas, H. Yu, F. Zhang, H. Zhang, and P. Lu
Atmos. Chem. Phys., 13, 2347–2379, https://doi.org/10.5194/acp-13-2347-2013, https://doi.org/10.5194/acp-13-2347-2013, 2013
J. Pey, X. Querol, A. Alastuey, F. Forastiere, and M. Stafoggia
Atmos. Chem. Phys., 13, 1395–1410, https://doi.org/10.5194/acp-13-1395-2013, https://doi.org/10.5194/acp-13-1395-2013, 2013
M. Dall'Osto, X. Querol, A. Alastuey, C. O'Dowd, R. M. Harrison, J. Wenger, and F. J. Gómez-Moreno
Atmos. Chem. Phys., 13, 741–759, https://doi.org/10.5194/acp-13-741-2013, https://doi.org/10.5194/acp-13-741-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Aerosol solar radiative forcing near the Taklimakan Desert based on radiative transfer and regional meteorological simulations during the Dust Aerosol Observation-Kashi campaign
An EARLINET early warning system for atmospheric aerosol aviation hazards
Optical properties of Central Asian aerosol relevant for spaceborne lidar applications and aerosol typing at 355 and 532 nm
Optical and geometrical aerosol particle properties over the United Arab Emirates
Determination and climatology of the diurnal cycle of the atmospheric mixing layer height over Beijing 2013–2018: lidar measurements and implications for air pollution
Site representativity of AERONET and GAW remotely sensed aerosol optical thickness and absorbing aerosol optical thickness observations
Reducing uncertainties in satellite estimates of aerosol–cloud interactions over the subtropical ocean by integrating vertically resolved aerosol observations
Remote sensing of two exceptional winter aerosol pollution events and representativeness of ground-based measurements
Comparison of south-east Atlantic aerosol direct radiative effect over clouds from SCIAMACHY, POLDER and OMI–MODIS
Radiative effects of long-range-transported Saharan air layers as determined from airborne lidar measurements
The mechanisms and seasonal differences of the impact of aerosols on daytime surface urban heat island effect
An observational study of the effects of aerosols on diurnal variation of heavy rainfall and associated clouds over Beijing–Tianjin–Hebei
Long-term profiling of aerosol light extinction, particle mass, cloud condensation nuclei, and ice-nucleating particle concentration over Dushanbe, Tajikistan, in Central Asia
Satellite mapping of PM2.5 episodes in the wintertime San Joaquin Valley: a “static” model using column water vapor
Improved 1 km resolution PM2.5 estimates across China using enhanced space–time extremely randomized trees
Merging regional and global aerosol optical depth records from major available satellite products
An AeroCom/AeroSat study: Intercomparison of Satellite AOD Datasets for Aerosol Model Evaluation
Satellite observations of aerosols and clouds over southern China from 2006 to 2015: analysis of changes and possible interaction mechanisms
Interannual variability and trends of combustion aerosol and dust in major continental outflows revealed by MODIS retrievals and CAM5 simulations during 2003–2017
Technical note: A simple method for retrieval of dust aerosol optical depth with polarized reflectance over oceans
How should we aggregate data? Methods accounting for the numerical distributions, with an assessment of aerosol optical depth
Constraining global aerosol emissions using POLDER/PARASOL satellite remote sensing observations
Detection and characterization of birch pollen in the atmosphere using a multiwavelength Raman polarization lidar and Hirst-type pollen sampler in Finland
Different strategies to retrieve aerosol properties at night-time with the GRASP algorithm
Two-dimensional mineral dust radiative effect calculations from CALIPSO observations over Europe
Investigation of CATS aerosol products and application toward global diurnal variation of aerosols
EARLINET evaluation of the CATS Level 2 aerosol backscatter coefficient product
Characterization of aerosol hygroscopicity using Raman lidar measurements at the EARLINET station of Payerne
Satellite inference of water vapour and above-cloud aerosol combined effect on radiative budget and cloud-top processes in the southeastern Atlantic Ocean
Retrieval of ice-nucleating particle concentrations from lidar observations and comparison with UAV in situ measurements
Comparison of two automated aerosol typing methods and their application to an EARLINET station
Cloud macro-physical properties in Saharan-dust-laden and dust-free North Atlantic trade wind regimes: a lidar case study
Evaluating the relative importance of northern African mineral dust sources using remote sensing
Large contribution of meteorological factors to inter-decadal changes in regional aerosol optical depth
The remote sensing of radiative forcing by light-absorbing particles (LAPs) in seasonal snow over northeastern China
Observation of absorbing aerosols above clouds over the south-east Atlantic Ocean from the geostationary satellite SEVIRI – Part 1: Method description and sensitivity
Aerosol properties and their influences on low warm clouds during the Two-Column Aerosol Project
Is positive correlation between cloud droplet effective radius and aerosol optical depth over land due to retrieval artifacts or real physical processes?
Evaluation and comparison of multiangle implementation of the atmospheric correction algorithm, Dark Target, and Deep Blue aerosol products over China
Long-term aerosol optical hygroscopicity study at the ACTRIS SIRTA observatory: synergy between ceilometer and in situ measurements
Intercomparison in spatial distributions and temporal trends derived from multi-source satellite aerosol products
Effects of air pollution control policies on PM2.5 pollution improvement in China from 2005 to 2017: a satellite-based perspective
A 10-year characterization of the Saharan Air Layer lidar ratio in the subtropical North Atlantic
Analysis of sulfate aerosols over Austria: a case study
Vertical aerosol distribution in the southern hemispheric midlatitudes as observed with lidar in Punta Arenas, Chile (53.2° S and 70.9° W), during ALPACA
Transport of aerosols over the French Riviera – link between ground-based lidar and spaceborne observations
Saharan dust and biomass burning aerosols during ex-hurricane Ophelia: observations from the new UK lidar and sun-photometer network
Multi-satellite retrieval of single scattering albedo using the OMI–MODIS algorithm
Remote sensing of aerosol properties from multi-wavelength and multi-pixel information over the ocean
Biomass-burning smoke heights over the Amazon observed from space
Li Li, Zhengqiang Li, Wenyuan Chang, Yang Ou, Philippe Goloub, Chengzhe Li, Kaitao Li, Qiaoyun Hu, Jianping Wang, and Manfred Wendisch
Atmos. Chem. Phys., 20, 10845–10864, https://doi.org/10.5194/acp-20-10845-2020, https://doi.org/10.5194/acp-20-10845-2020, 2020
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Dust Aerosol Observation-Kashi (DAO-K) campaign was conducted near the Taklimakan Desert in April 2019 to obtain comprehensive aerosol, atmosphere, and surface parameters. Estimations of aerosol solar radiative forcing by a radiative transfer (RT) model were improved based on the measured aerosol parameters, additionally considering atmospheric profiles and diurnal variations of surface albedo. RT simulations agree well with simultaneous irradiance observations, even in dust-polluted conditions.
Nikolaos Papagiannopoulos, Giuseppe D'Amico, Anna Gialitaki, Nicolae Ajtai, Lucas Alados-Arboledas, Aldo Amodeo, Vassilis Amiridis, Holger Baars, Dimitris Balis, Ioannis Binietoglou, Adolfo Comerón, Davide Dionisi, Alfredo Falconieri, Patrick Fréville, Anna Kampouri, Ina Mattis, Zoran Mijić, Francisco Molero, Alex Papayannis, Gelsomina Pappalardo, Alejandro Rodríguez-Gómez, Stavros Solomos, and Lucia Mona
Atmos. Chem. Phys., 20, 10775–10789, https://doi.org/10.5194/acp-20-10775-2020, https://doi.org/10.5194/acp-20-10775-2020, 2020
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Volcanic and desert dust particles affect human activities in manifold ways; consequently, mitigation tools are important. Their early detection and the issuance of early warnings are key elements in the initiation of operational response procedures. A methodology for the early warning of these hazards using European Aerosol Research Lidar Network (EARLINET) data is presented. The tailored product is investigated during a volcanic eruption and mineral dust advected in the eastern Mediterranean.
Julian Hofer, Albert Ansmann, Dietrich Althausen, Ronny Engelmann, Holger Baars, Khanneh Wadinga Fomba, Ulla Wandinger, Sabur F. Abdullaev, and Abduvosit N. Makhmudov
Atmos. Chem. Phys., 20, 9265–9280, https://doi.org/10.5194/acp-20-9265-2020, https://doi.org/10.5194/acp-20-9265-2020, 2020
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For the first time, a dense data set of particle extinction-to-backscatter ratios (lidar ratios), depolarization ratios, and backscatter- and extinction-related Ångström exponents for a Central Asian site are presented. The observations were performed with a continuously running multiwavelength polarization Raman lidar at Dushanbe, Tajikistan, during an 18-month campaign. The found optical properties reflect the large range of occurring aerosol mixtures.
Maria Filioglou, Elina Giannakaki, John Backman, Jutta Kesti, Anne Hirsikko, Ronny Engelmann, Ewan O'Connor, Jari T. T. Leskinen, Xiaoxia Shang, Hannele Korhonen, Heikki Lihavainen, Sami Romakkaniemi, and Mika Komppula
Atmos. Chem. Phys., 20, 8909–8922, https://doi.org/10.5194/acp-20-8909-2020, https://doi.org/10.5194/acp-20-8909-2020, 2020
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Dust optical properties are region-dependent. Saharan, Asian, and Arabian dusts do not pose similar optical properties in terms of lidar ratios; thus, a universal lidar ratio for dust particles will lead to biases. The present study analyses observations over the United Arab Emirates, quantifying the optical and geometrical extents of the aerosol layers in the area, providing at the same time the Arabian dust properties along with chemical analysis of dust samples collected in the region.
Haofei Wang, Zhengqiang Li, Yang Lv, Ying Zhang, Hua Xu, Jianping Guo, and Philippe Goloub
Atmos. Chem. Phys., 20, 8839–8854, https://doi.org/10.5194/acp-20-8839-2020, https://doi.org/10.5194/acp-20-8839-2020, 2020
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Lidar shows good performance in calculating the convective layer height in the daytime and the residual layer height at night, as well as having the potential to describe the stable layer height at night. The MLH seasonal change in Beijing indicates that it is low in winter and autumn and high in spring and summer. From 2014 to 2018, the magnitude of the diurnal cycle of MLH increased year by year. MLH from lidar shows better accuracy than a radiosonde when calculating surface pollution.
Nick A. J. Schutgens
Atmos. Chem. Phys., 20, 7473–7488, https://doi.org/10.5194/acp-20-7473-2020, https://doi.org/10.5194/acp-20-7473-2020, 2020
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Aerosols are tiny particles in the air that affect human health and climate. To study these particles, measurement networks across the world are used. Each site, however, can only observe the air directly above it, so how representative is this measurement for the wider environment? The sites of a well-known remote sensing network (AERONET) are examined and ranked according to their representativity. This should benefit researchers using this measurement network.
David Painemal, Fu-Lung Chang, Richard Ferrare, Sharon Burton, Zhujun Li, William L. Smith Jr., Patrick Minnis, Yan Feng, and Marian Clayton
Atmos. Chem. Phys., 20, 7167–7177, https://doi.org/10.5194/acp-20-7167-2020, https://doi.org/10.5194/acp-20-7167-2020, 2020
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Aerosol–cloud interactions (ACIs) are the most uncertain aspect of anthropogenic forcing. Although satellites provide the observational dataset for the global ACI quantification, retrievals are limited to vertically integrated quantities (e.g., aerosol optical depth – AOD), which are typically used as an aerosol proxy. This study demonstrates that matching vertically resolved aerosol from CALIOP at the cloud-layer height with satellite cloud retrievals reduces uncertainties in ACI estimates.
Alexandre Baron, Patrick Chazette, and Julien Totems
Atmos. Chem. Phys., 20, 6749–6768, https://doi.org/10.5194/acp-20-6749-2020, https://doi.org/10.5194/acp-20-6749-2020, 2020
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Two major winter aerosol pollution events have been sampled over the Paris area. They correspond to weather conditions with a high-pressure system. We show that during such events the ground-based particle matter content can be related to lidar-derived aerosol extinction coefficient within the atmospheric planetary boundary layer. This opens a new horizon for the monitoring of intense pollution events from space-borne active sensors.
Martin de Graaf, Ruben Schulte, Fanny Peers, Fabien Waquet, L. Gijsbert Tilstra, and Piet Stammes
Atmos. Chem. Phys., 20, 6707–6723, https://doi.org/10.5194/acp-20-6707-2020, https://doi.org/10.5194/acp-20-6707-2020, 2020
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The radiative effect from smoke by wildfires has been found to be much stronger than models predict. The effect is complex; smoke generally cools the climate system by reflecting sunlight but strongly warms the system when it is found over a bright cloud deck. In this paper three different satellite datasets are compared and all three confirm the strong warming of African smoke over the cloud deck in the south-east Atlantic. The intercomparison reduces the uncertainties in the observations.
Manuel Gutleben, Silke Groß, Martin Wirth, and Bernhard Mayer
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-420, https://doi.org/10.5194/acp-2020-420, 2020
Revised manuscript accepted for ACP
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Airborne lidar measurements in the vicinity of Barbados are used to investigate radiative effects of long-range-transported Saharan air layers. Derived atmospheric heating rates indicate that observed enhanced water vapor concentrations inside these layers are the main drivers for dust vertical mixing inside the layers. Additionally, they may play a major role for the suppression of subjacent convective cloud development.
Wenchao Han, Zhanqing Li, Fang Wu, Yuwei Zhang, Jianping Guo, Tianning Su, Maureen Cribb, Jiwen Fan, Tianmeng Chen, Jing Wei, and Seoung-Soo Lee
Atmos. Chem. Phys., 20, 6479–6493, https://doi.org/10.5194/acp-20-6479-2020, https://doi.org/10.5194/acp-20-6479-2020, 2020
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Observational data and model simulation were used to analyze the daytime urban heat island intensity (UHII) under polluted and clean conditions in China. We found that aerosols reduce the UHII in summer but increase the UHII in winter. Two mechanisms, the aerosol radiative effect (ARE) and the aerosol dynamic effect (ADE), behave differently in summer and winter. In summer, the UHII is mainly affected by the ARE, and the ADE is weak, and the opposite is the case in winter.
Siyuan Zhou, Jing Yang, Wei-Chyung Wang, Chuanfeng Zhao, Daoyi Gong, and Peijun Shi
Atmos. Chem. Phys., 20, 5211–5229, https://doi.org/10.5194/acp-20-5211-2020, https://doi.org/10.5194/acp-20-5211-2020, 2020
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Aerosol–cloud–precipitation interaction is a challenging problem in regional climate. Our study contrasted the observed diurnal variation of heavy rainfall and associated clouds over Beijing–Tianjin–Hebei between clean and polluted days during the 2002–2012 summers. We found the heavy rainfall under pollution has earlier start time, earlier peak time and longer duration, and further found the absorbing aerosols and scattering aerosols play different roles in the heavy rainfall diurnal variation.
Julian Hofer, Albert Ansmann, Dietrich Althausen, Ronny Engelmann, Holger Baars, Sabur F. Abdullaev, and Abduvosit N. Makhmudov
Atmos. Chem. Phys., 20, 4695–4711, https://doi.org/10.5194/acp-20-4695-2020, https://doi.org/10.5194/acp-20-4695-2020, 2020
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For the first time, continuous, vertically resolved long-term aerosol measurements were conducted with a state-of-the-art multiwavelength lidar over a Central Asian site. Such observations are urgently required in efforts to predict future climate and environmental conditions and to support spaceborne remote sensing (ground truth activities).
Robert B. Chatfield, Meytar Sorek-Hamer, Robert F. Esswein, and Alexei Lyapustin
Atmos. Chem. Phys., 20, 4379–4397, https://doi.org/10.5194/acp-20-4379-2020, https://doi.org/10.5194/acp-20-4379-2020, 2020
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There is a great need to define health-affecting pollution by small particles as “respirable aerosol”. The wintertime San Joaquin Valley experiences severe episodes that need full maps. A few air pollution monitors are set out by agencies in such regions. Satellite data on haziness and daily calibration using the monitors map out improved pollution estimates for the winter of 2012–2013. These show patterns of valuable empirical information about sources, transport, and cleanout of pollution.
Jing Wei, Zhanqing Li, Maureen Cribb, Wei Huang, Wenhao Xue, Lin Sun, Jianping Guo, Yiran Peng, Jing Li, Alexei Lyapustin, Lei Liu, Hao Wu, and Yimeng Song
Atmos. Chem. Phys., 20, 3273–3289, https://doi.org/10.5194/acp-20-3273-2020, https://doi.org/10.5194/acp-20-3273-2020, 2020
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This study introduced an enhanced space–time extremely randomized trees (STET) approach to improve the 1 km resolution ground-level PM2.5 estimates across China using the remote sensing technology. The STET model shows high accuracy and strong predictive power and appears to outperform most models reported by previous studies. Thus, it is of great importance for future air pollution studies at medium- or small-scale areas and will be applied to generate the historical PM2.5 dataset across China.
Larisa Sogacheva, Thomas Popp, Andrew M. Sayer, Oleg Dubovik, Michael J. Garay, Andreas Heckel, N. Christina Hsu, Hiren Jethva, Ralph A. Kahn, Pekka Kolmonen, Miriam Kosmale, Gerrit de Leeuw, Robert C. Levy, Pavel Litvinov, Alexei Lyapustin, Peter North, Omar Torres, and Antti Arola
Atmos. Chem. Phys., 20, 2031–2056, https://doi.org/10.5194/acp-20-2031-2020, https://doi.org/10.5194/acp-20-2031-2020, 2020
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The typical lifetime of a single satellite platform is on the order of 5–15 years; thus, for climate studies the usage of multiple satellite sensors should be considered.
Here we introduce and evaluate a monthly AOD merged product and AOD global and regional time series for the period 1995–2017 created from 12 individual satellite AOD products, which provide a long-term perspective on AOD changes over different regions of the globe.
Nick Schutgens, Andrew M. Sayer, Andreas Heckel, Christina Hsu, Hiren Jethva, Gerrit de Leeuw, Peter J. T. Leonard, Robert C. Levy, Antti Lipponen, Alexei Lyapustin, Peter North, Thomas Popp, Caroline Poulson, Virginia Sawyer, Larisa Sogacheva, Gareth Thomas, Omar Torres, Yujie Wang, Stefan Kinne, Michael Schulz, and Philip Stier
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2019-1193, https://doi.org/10.5194/acp-2019-1193, 2020
Revised manuscript accepted for ACP
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We intercompare 14 different datasets of satellite observations of aerosol. Such meaaurements are challenging but also provide the best opportunity to globally observe an atmospheric component strongly related to air pollution and climate change. Our study shows that most datasets perform similarly well on a global scale but that locally errors can be quite different. We develop a technique to estimate satellite errors everywhere, even in the absence of surface reference data.
Nikos Benas, Jan Fokke Meirink, Karl-Göran Karlsson, Martin Stengel, and Piet Stammes
Atmos. Chem. Phys., 20, 457–474, https://doi.org/10.5194/acp-20-457-2020, https://doi.org/10.5194/acp-20-457-2020, 2020
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In this study we analyse aerosol and cloud changes over southern China from 2006 to 2015 and investigate their possible interaction mechanisms. Results show decreasing aerosol loads and increasing liquid cloud cover in late autumn. Further analysis based on various satellite data sets shows consistency with the aerosol semi-direct effect, whereby less absorbing aerosols in the cloud layer would lead to an overall decrease in the evaporation of cloud droplets, thus increasing cloud amount.
Hongbin Yu, Yang Yang, Hailong Wang, Qian Tan, Mian Chin, Robert C. Levy, Lorraine A. Remer, Steven J. Smith, Tianle Yuan, and Yingxi Shi
Atmos. Chem. Phys., 20, 139–161, https://doi.org/10.5194/acp-20-139-2020, https://doi.org/10.5194/acp-20-139-2020, 2020
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Emissions and long-range transport of mineral dust and
combustion-related aerosol from burning fossil fuels and biomass vary from year to year, driven by the evolution of the economy and changes in meteorological conditions and environmental regulations. This study offers both satellite and model perspectives on interannual variability and possible trends in combustion aerosol and dust in major continental outflow regions over the past 15 years (2003–2017).
Wenbo Sun, Yongxiang Hu, Rosemary R. Baize, Gorden Videen, Sungsoo S. Kim, Young-Jun Choi, Kyungin Kang, Chae Kyung Sim, Minsup Jeong, Ali Omar, Snorre A. Stamnes, David G. MacDonnell, and Evgenij Zubko
Atmos. Chem. Phys., 19, 15583–15586, https://doi.org/10.5194/acp-19-15583-2019, https://doi.org/10.5194/acp-19-15583-2019, 2019
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Dusts have a significant impact on climate and environment. Detecting dust using satellite instruments is generally conducted by measuring at multiple observation angles due to the uncertainty of the surface reflection. This report shows that the degree of polarization of reflected light can be used for retrieving the optical depth of dust at backscatter angles only, regardless of surface conditions. This simple method is suitable for surveying dust aerosols over oceans with low-cost satellites.
Andrew M. Sayer and Kirk D. Knobelspiesse
Atmos. Chem. Phys., 19, 15023–15048, https://doi.org/10.5194/acp-19-15023-2019, https://doi.org/10.5194/acp-19-15023-2019, 2019
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Data about the Earth are routinely obtained from satellite observations, model simulations, and ground-based or other measurements. These are at different space and timescales, and it is common to average them to reduce gaps and increase ease of use. The question of how the data should be averaged depends on the underlying distribution of the quantity. This study presents a method for determining how to appropriately aggregate data and applies it to data sets about atmospheric aerosol levels.
Cheng Chen, Oleg Dubovik, Daven K. Henze, Mian Chin, Tatyana Lapyonok, Gregory L. Schuster, Fabrice Ducos, David Fuertes, Pavel Litvinov, Lei Li, Anton Lopatin, Qiaoyun Hu, and Benjamin Torres
Atmos. Chem. Phys., 19, 14585–14606, https://doi.org/10.5194/acp-19-14585-2019, https://doi.org/10.5194/acp-19-14585-2019, 2019
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Global BC, OC and DD aerosol emissions are inverted from POLDER/PARASOL observations for the year 2010 based on the GEOS-Chem inverse modeling framework. The retrieved emissions are 18.4 Tg yr−1 BC, 109.9 Tg yr−1 OC and 731.6 Tg yr−1 DD, which indicate an increase of 166.7 % for BC and 184.0 % for OC, while a decrease of 42.4 % for DD with respect to GEOS-Chem a priori emission inventories is seen. Global annul mean AOD and AAOD resulting from retrieved emissions are 0.119 and 0.0071 at 550 nm.
Stephanie Bohlmann, Xiaoxia Shang, Elina Giannakaki, Maria Filioglou, Annika Saarto, Sami Romakkaniemi, and Mika Komppula
Atmos. Chem. Phys., 19, 14559–14569, https://doi.org/10.5194/acp-19-14559-2019, https://doi.org/10.5194/acp-19-14559-2019, 2019
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Measurements of the multiwavelength Raman polarization lidar PollyXT have been combined with measurements of pollen type and concentration using a traditional pollen sampler at the rural forest site in Vehmasmäki, Finland. High particle depolarization ratios were observed during an intense pollination event of birch pollen occasionally mixed with spruce pollen. Our observations illustrate the potential of the particle depolarization ratio to track pollen grains in the atmosphere.
Jose Antonio Benavent-Oltra, Roberto Román, Juan Andrés Casquero-Vera, Daniel Pérez-Ramírez, Hassan Lyamani, Pablo Ortiz-Amezcua, Andrés Esteban Bedoya-Velásquez, Gregori de Arruda Moreira, África Barreto, Anton Lopatin, David Fuertes, Milagros Herrera, Benjamin Torres, Oleg Dubovik, Juan Luis Guerrero-Rascado, Philippe Goloub, Francisco Jose Olmo-Reyes, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 19, 14149–14171, https://doi.org/10.5194/acp-19-14149-2019, https://doi.org/10.5194/acp-19-14149-2019, 2019
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In this paper, we use the GRASP algorithm combining different
remote-sensing measurements to obtain the aerosol vertical and column properties, both during the day and at night-time. The column properties are compared with AERONET products, and the vertical properties retrieved by GRASP are compared with in situ measurements at high-altitude stations. As an originality, we proposed three new schemes to retrieve the night-time aerosol properties.
Maria José Granados-Muñoz, Michaël Sicard, Nikolaos Papagiannopoulos, Rubén Barragán, Juan Antonio Bravo-Aranda, and Doina Nicolae
Atmos. Chem. Phys., 19, 13157–13173, https://doi.org/10.5194/acp-19-13157-2019, https://doi.org/10.5194/acp-19-13157-2019, 2019
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The use of satellite data is of great interest for the determination of aerosol radiative forcing at regional or even global scales, as previous studies in the literature are predominantly only valid locally. A methodology to retrieve 2-D dust radiative effects with large spatial and temporal coverage based on combined satellite data from CALIPSO, MODIS and CERES is presented and evaluated against well-established methods based on ground-based lidar measurements, obtaining quite good results.
Logan Lee, Jianglong Zhang, Jeffrey S. Reid, and John E. Yorks
Atmos. Chem. Phys., 19, 12687–12707, https://doi.org/10.5194/acp-19-12687-2019, https://doi.org/10.5194/acp-19-12687-2019, 2019
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The study of the diurnal variation of aerosol optical depth (AOD) and aerosol vertical distribution is necessary for the monitoring and modeling of aerosol particles for various air pollution, visibility and climate-related studies. Upon evaluating 1064 nm AOD and aerosol extinction profiles from the Cloud-Aerosol Transport System (CATS) level 2 aerosol product, we studied the diurnal variation of AOD and aerosol extinction profiles on both regional and global scales.
Emmanouil Proestakis, Vassilis Amiridis, Eleni Marinou, Ioannis Binietoglou, Albert Ansmann, Ulla Wandinger, Julian Hofer, John Yorks, Edward Nowottnick, Abduvosit Makhmudov, Alexandros Papayannis, Aleksander Pietruczuk, Anna Gialitaki, Arnoud Apituley, Artur Szkop, Constantino Muñoz Porcar, Daniele Bortoli, Davide Dionisi, Dietrich Althausen, Dimitra Mamali, Dimitris Balis, Doina Nicolae, Eleni Tetoni, Gian Luigi Liberti, Holger Baars, Ina Mattis, Iwona Sylwia Stachlewska, Kalliopi Artemis Voudouri, Lucia Mona, Maria Mylonaki, Maria Rita Perrone, Maria João Costa, Michael Sicard, Nikolaos Papagiannopoulos, Nikolaos Siomos, Pasquale Burlizzi, Rebecca Pauly, Ronny Engelmann, Sabur Abdullaev, and Gelsomina Pappalardo
Atmos. Chem. Phys., 19, 11743–11764, https://doi.org/10.5194/acp-19-11743-2019, https://doi.org/10.5194/acp-19-11743-2019, 2019
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To increase accuracy and validate satellite-based products, comparison with ground-based reference observations is required. To do this, we present evaluation activity of EARLINET for the qualitative and quantitative assessment of NASA's CATS lidar operating aboard the International Space Station (ISS) while identified discrepancies are discussed. Better understanding CATS performance and limitations provides a valuable basis for scientific studies implementing the satellite-based lidar system.
Francisco Navas-Guzmán, Giovanni Martucci, Martine Collaud Coen, María José Granados-Muñoz, Maxime Hervo, Michael Sicard, and Alexander Haefele
Atmos. Chem. Phys., 19, 11651–11668, https://doi.org/10.5194/acp-19-11651-2019, https://doi.org/10.5194/acp-19-11651-2019, 2019
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The present study demonstrates the capability of a Raman lidar to monitor aerosol hygroscopic processes. The results showed a higher hygroscopicity and wavelength dependency for smoke particles than for mineral dust. The higher sensitivity of the shortest wavelength to hygroscopic growth found for smoke particles was qualitatively reproduced using Mie simulations. The impact of aerosol hygroscopicity on the Earth's radiative balance has been evaluated using a radiative transfer model.
Lucia T. Deaconu, Nicolas Ferlay, Fabien Waquet, Fanny Peers, François Thieuleux, and Philippe Goloub
Atmos. Chem. Phys., 19, 11613–11634, https://doi.org/10.5194/acp-19-11613-2019, https://doi.org/10.5194/acp-19-11613-2019, 2019
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We analyse and quantify the effect of above-cloud aerosol (AAC) loading on the underlying cloud properties in the South Atlantic Ocean. We use a synergy of remote sensing retrievals collocated with ERA-Interim meteorological profiles. The results show that for larger loads of AACs, clouds are optically thicker, with an increase in liquid water path by 20 g m−2 and lower cloud-top altitudes. We also observe a strong covariation between the aerosol plume and the presence of water vapour.
Eleni Marinou, Matthias Tesche, Athanasios Nenes, Albert Ansmann, Jann Schrod, Dimitra Mamali, Alexandra Tsekeri, Michael Pikridas, Holger Baars, Ronny Engelmann, Kalliopi-Artemis Voudouri, Stavros Solomos, Jean Sciare, Silke Groß, Florian Ewald, and Vassilis Amiridis
Atmos. Chem. Phys., 19, 11315–11342, https://doi.org/10.5194/acp-19-11315-2019, https://doi.org/10.5194/acp-19-11315-2019, 2019
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We assess the feasibility of ground-based and spaceborne lidars to retrieve profiles of cloud-relevant aerosol concentrations and ice-nucleating particles. The retrieved profiles are in good agreement with airborne in situ measurements. Our methodology will be applied to satellite observations in the future so as to provide a global 3D product of cloud-relevant properties.
Kalliopi Artemis Voudouri, Nikolaos Siomos, Konstantinos Michailidis, Nikolaos Papagiannopoulos, Lucia Mona, Carmela Cornacchia, Doina Nicolae, and Dimitris Balis
Atmos. Chem. Phys., 19, 10961–10980, https://doi.org/10.5194/acp-19-10961-2019, https://doi.org/10.5194/acp-19-10961-2019, 2019
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In this study, a first attempt at comparing and evaluating two classification tools developed within EARLINET that provide near-real-time aerosol typing information for the lidar profiles of Thessaloniki is presented. Our aim is (i) to check the performance of both supervised learning techniques in their low-resolution mode and (ii) to investigate the reasons for typing agreement and disagreement with respect to the uncertainties and the threshold criteria applied.
Manuel Gutleben, Silke Groß, and Martin Wirth
Atmos. Chem. Phys., 19, 10659–10673, https://doi.org/10.5194/acp-19-10659-2019, https://doi.org/10.5194/acp-19-10659-2019, 2019
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This study concentrates on airborne lidar measurements conducted during the NARVAL field experiments over the western subtropical North Atlantic Ocean to study differences between shallow marine cloud macro-physical properties (i.e. cloud fraction, cloud top height, cloud length, cloud gap length) in Saharan-dust-laden and dust-free trade wind regions. Cloud top heights, cloud fractions and cloud lengths are found to be lower and smaller in Saharan-dust-laden compared to dust-free regions.
Natalie L. Bakker, Nick A. Drake, and Charlie S. Bristow
Atmos. Chem. Phys., 19, 10525–10535, https://doi.org/10.5194/acp-19-10525-2019, https://doi.org/10.5194/acp-19-10525-2019, 2019
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Northern African mineral dust provides the Amazon Basin with essential nutrients, although the process is still poorly understood. In our study, we utilise high-resolution satellite data to analyse northern African dust sources of the 2015–2017 winter dust seasons. We find that the majority of dust is emitted from palaeolake and palaeoriver systems. Specifically, palaeorivers have been mostly overlooked to date. Furthermore, we find that dune fields do not produce much dust.
Huizheng Che, Ke Gui, Xiangao Xia, Yaqiang Wang, Brent N. Holben, Philippe Goloub, Emilio Cuevas-Agulló, Hong Wang, Yu Zheng, Hujia Zhao, and Xiaoye Zhang
Atmos. Chem. Phys., 19, 10497–10523, https://doi.org/10.5194/acp-19-10497-2019, https://doi.org/10.5194/acp-19-10497-2019, 2019
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A comprehensive assessment of the global and regional AOD trends over the past 37 years (1980–2016) is presented. AOD observations from both AERONET and CARSNET were used for the first time to assess the performance of the MERRA-2 AOD dataset on a global scale. Based on statistical models, we found the meteorological parameters explained a larger proportion of the regional AOD variability (20.4 %–2.8 %) when compared with emission factors (0 %%–56 %).
Wei Pu, Jiecan Cui, Tenglong Shi, Xuelei Zhang, Cenlin He, and Xin Wang
Atmos. Chem. Phys., 19, 9949–9968, https://doi.org/10.5194/acp-19-9949-2019, https://doi.org/10.5194/acp-19-9949-2019, 2019
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LAPs (light-absorbing particles) deposited on snow can decrease snow albedo and increase the absorption of solar radiation. Radiative forcing by LAPs will affect the regional hydrological cycle and climate. We use MODIS observations to retrieve the radiative forcing by LAPs in snow across northeastern China (NEC). The results of radiative forcing present distinct spatial variability. We find that the biases are negatively correlated with LAP concentrations and range from
~ 5 % to ~ 350 %.
Fanny Peers, Peter Francis, Cathryn Fox, Steven J. Abel, Kate Szpek, Michael I. Cotterell, Nicholas W. Davies, Justin M. Langridge, Kerry G. Meyer, Steven E. Platnick, and Jim M. Haywood
Atmos. Chem. Phys., 19, 9595–9611, https://doi.org/10.5194/acp-19-9595-2019, https://doi.org/10.5194/acp-19-9595-2019, 2019
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The measurements from the geostationary satellite MSG/SEVIRI are used to retrieve the cloud and above-cloud aerosol properties over the South Atlantic. The technique relies on the spectral contrast and the magnitude of the signal in the visible to shortwave infrared region as well as the atmospheric correction based on forecasted water vapour profiles. The sensitivity analysis and the stability of the retrieval over time show great potential of the high-temporal-resolution observations.
Jianjun Liu and Zhanqing Li
Atmos. Chem. Phys., 19, 9515–9529, https://doi.org/10.5194/acp-19-9515-2019, https://doi.org/10.5194/acp-19-9515-2019, 2019
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This study uses the data collected during the TCAP field campaign to investigate the aerosol properties and the influence of aerosol loading and composition on low-warm-cloud development and microphysical properties. The results indicated that the aerosols significantly weaken the dependence of cloud development on thermodynamic conditions. Aerosol first indirect effects estimated for aerosols with a low mass of organics were larger than those for aerosols with a high mass of organics.
Hailing Jia, Xiaoyan Ma, Johannes Quaas, Yan Yin, and Tom Qiu
Atmos. Chem. Phys., 19, 8879–8896, https://doi.org/10.5194/acp-19-8879-2019, https://doi.org/10.5194/acp-19-8879-2019, 2019
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We systematically assess how and to what extent satellite retrieval biases may affect correlations, as well as explore the underlying physical mechanisms. It is noted that the retrieval biases of both cloud and aerosol can result in a serious overestimation of the slope of CER–AI. Positive correlations more likely to occur in the case of drier cloud top and stronger turbulence in clouds, implying entrainment mixing might be a possible physical interpretation for such a positive CER–AI slope.
Ning Liu, Bin Zou, Huihui Feng, Wei Wang, Yuqi Tang, and Yu Liang
Atmos. Chem. Phys., 19, 8243–8268, https://doi.org/10.5194/acp-19-8243-2019, https://doi.org/10.5194/acp-19-8243-2019, 2019
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The systematic validation and comparison of MAIAC, DT, and DB AOD products across China from 2000 to 2017 is presented. In this process, the overall accuracy, land type dependence, view geometry dependence, spatiotemporal retrieval accuracy, spatial variation pattern, and spatiotemporal completeness of the three products are analyzed in detail. In general, MAIAC achieves higher accuracy than DT and DB, but DT and DB may perform better than MAIAC under some specific land cover types or seasons.
Andrés Esteban Bedoya-Velásquez, Gloria Titos, Juan Antonio Bravo-Aranda, Martial Haeffelin, Olivier Favez, Jean-Eudes Petit, Juan Andrés Casquero-Vera, Francisco José Olmo-Reyes, Elena Montilla-Rosero, Carlos D. Hoyos, Lucas Alados-Arboledas, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 19, 7883–7896, https://doi.org/10.5194/acp-19-7883-2019, https://doi.org/10.5194/acp-19-7883-2019, 2019
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This study is related to the first time hygroscopic enhancement factors retrieved directly for ambient aerosols using remote sensing techniques are combined with online chemical composition in situ measurements to evaluate the role of the different aerosol species in aerosol hygroscopicity at ACTRIS SIRTA observatory. The results showed 8 cases that fulfilled strict criteria over 107 cases identified in this study.
Jing Wei, Yiran Peng, Rashed Mahmood, Lin Sun, and Jianping Guo
Atmos. Chem. Phys., 19, 7183–7207, https://doi.org/10.5194/acp-19-7183-2019, https://doi.org/10.5194/acp-19-7183-2019, 2019
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This study evaluates the suitability of 11 satellite-derived aerosol products in describing the spatio-temporal variations over the world. Our results show similar global patterns among these products but noticeable spatial heterogeneity and numerical differences over land regions. In general, MODIS products perform best at reflecting the spatial distributions and capturing the temporal trends of aerosol. This study help readers select a suitable aerosol dataset for their studies.
Zongwei Ma, Riyang Liu, Yang Liu, and Jun Bi
Atmos. Chem. Phys., 19, 6861–6877, https://doi.org/10.5194/acp-19-6861-2019, https://doi.org/10.5194/acp-19-6861-2019, 2019
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This paper reviewed the air pollution control policies in China from 2005 to 2017. Then we gave an overall evaluation of the effects of these policies on PM2.5 pollution improvement in China from the perspective of satellite remote sensing. This paper can provide reference for future policy making of air pollution control in China.
Alberto Berjón, Africa Barreto, Yballa Hernández, Margarita Yela, Carlos Toledano, and Emilio Cuevas
Atmos. Chem. Phys., 19, 6331–6349, https://doi.org/10.5194/acp-19-6331-2019, https://doi.org/10.5194/acp-19-6331-2019, 2019
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Lidar ratio is a key parameter for the aerosol characterization using satellite remote-sensing platforms as CALIOP. However, there are important differences in the values reported in the bibliography. The geographic characteristics of the IARC observatories location and a 10-year data series allow us to make a unique study of the mineral dust in the Saharan air layer. We report lidar ratios at 523 nm of 49 ± 6 sr and 50 ± 11 sr obtained by two different methods.
Camelia Talianu and Petra Seibert
Atmos. Chem. Phys., 19, 6235–6250, https://doi.org/10.5194/acp-19-6235-2019, https://doi.org/10.5194/acp-19-6235-2019, 2019
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The episode of elevated sulfate aerosols over eastern Austria during 1–6 April 2014 is analyzed using in situ measurements, EARLINET lidar measurements, CAMS reanalysis data, and backward simulations with the FLEXPART Lagrangian dispersion model. It was found that the lowest layers came from central Europe, while at higher levels, sources in NW Africa and the eastern US contributed. The methodology can be used as a tool to relate in situ and EARLINET measurements.
Andreas Foth, Thomas Kanitz, Ronny Engelmann, Holger Baars, Martin Radenz, Patric Seifert, Boris Barja, Michael Fromm, Heike Kalesse, and Albert Ansmann
Atmos. Chem. Phys., 19, 6217–6233, https://doi.org/10.5194/acp-19-6217-2019, https://doi.org/10.5194/acp-19-6217-2019, 2019
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In this study, we present the vertical aerosol distribution in the pristine region of the southern tip of South America determined by ground-based and spaceborne lidar observations. Most aerosol load is contained within the planetary boundary layer up to about 1200 m. The free troposphere is characterized by a very low aerosol concentration but a frequent occurrence of clouds. Lofted aerosol layers were rarely observed and, when present, were characterized by very low optical thicknesses.
Patrick Chazette, Julien Totems, and Xiaoxia Shang
Atmos. Chem. Phys., 19, 3885–3904, https://doi.org/10.5194/acp-19-3885-2019, https://doi.org/10.5194/acp-19-3885-2019, 2019
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Using a backscatter N2-Raman lidar deployed on the western part of the French Riviera, we investigate the vertical aerosol structure below 5 km. By coupling these observations with spaceborne instruments and trajectory modeling, we highlight plumes of particulate pollutants moving towards the French Riviera. This pollution, mainly due to traffic and petrochemical activities, originates from the Spanish coast (Costa Blanca and Costa Brava–Daurada) and mixes with local emissions.
Martin Osborne, Florent F. Malavelle, Mariana Adam, Joelle Buxmann, Jaqueline Sugier, Franco Marenco, and Jim Haywood
Atmos. Chem. Phys., 19, 3557–3578, https://doi.org/10.5194/acp-19-3557-2019, https://doi.org/10.5194/acp-19-3557-2019, 2019
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In this paper we present an analysis of the unusual
red skyevent that occurred over the UK on 15 and 16 October 2017. We use measurements from the Met Office operational lidar and sun-photometer network, as well as other data and model output, to show that the event was caused by the passage of ex-hurricane Ophelia which transported unusual amounts of dust from the Sahara to the UK as well as smoke from forest fires in Portugal.
Kruthika Eswaran, Sreedharan Krishnakumari Satheesh, and Jayaraman Srinivasan
Atmos. Chem. Phys., 19, 3307–3324, https://doi.org/10.5194/acp-19-3307-2019, https://doi.org/10.5194/acp-19-3307-2019, 2019
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Multiple satellite retrieval algorithms are used to counter problems, such as cloud contamination, faced by sensors with large pixel sizes. This work uses one such algorithm to retrieve a parameter (single scattering albedo) over the oceans. It was found that the joint algorithm performed better than the original when aerosols were present near the surface. Discrepancy between the measurements was seen when elevated aerosols were present which might not have been detected by cruise instruments.
Chong Shi, Makiko Hashimoto, and Teruyuki Nakajima
Atmos. Chem. Phys., 19, 2461–2475, https://doi.org/10.5194/acp-19-2461-2019, https://doi.org/10.5194/acp-19-2461-2019, 2019
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This paper presents a new technique for retrieving aerosol optical properties using multi-wavelength and multi-pixel information over the ocean. Different from the traditional satellite aerosol retrievals conducted pixel by pixel, we derive the aerosol optical properties of multiple pixels simultaneously by adding a smoothness constraint on the spatial variation of aerosols and oceanic substances. The technique asserts that the multi-pixel scheme is conducive to aerosol retrieval over the ocean.
Laura Gonzalez-Alonso, Maria Val Martin, and Ralph A. Kahn
Atmos. Chem. Phys., 19, 1685–1702, https://doi.org/10.5194/acp-19-1685-2019, https://doi.org/10.5194/acp-19-1685-2019, 2019
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The vertical distribution of fire smoke and factors that control its rise had not yet been quantified across the Amazon. We developed a satellite-based long record of smoke plume heights. We find that smoke heights are driven by many factors: vegetation, seasonality, time of day, fire intensity, and atmospheric and drought conditions. Also, drought increases fire pollution, with implications for air quality. Policies to control fires may be crucial in the future as more droughts are projected.
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Basart, S., Pérez, C., Cuevas, E., Baldasano, J. M., and Gobbi, G. P.: Aerosol characterization in Northern Africa, Northeastern Atlantic, Mediterranean Basin and Middle East from direct-sun AERONET observations, Atmos. Chem. Phys., 9, 8265–8282, https://doi.org/10.5194/acp-9-8265-2009, 2009.
Basart, S., Pay, M. T., Jorba, O., Pérez, C., Jiménez-Guerrero, P., Schulz, M., and Baldasano, J. M.: Aerosols in the CALIOPE air quality modelling system: evaluation and analysis of PM levels, optical depths and chemical composition over Europe, Atmos. Chem. Phys., 12, 3363–3392, https://doi.org/10.5194/acp-12-3363-2012, 2012.
Ben-Ami, Y., Koren, I., and Altaratz, O.: Patterns of North African dust transport over the Atlantic: winter vs. summer, based on CALIPSO first year data, Atmos. Chem. Phys., 9, 7867–7875, https://doi.org/10.5194/acp-9-7867-2009, 2009.
Ben-Ami, Y., Koren, I., Rudich, Y., Artaxo, P., Martin, S. T., and Andreae, M. O.: Transport of North African dust from the Bodélé depression to the Amazon Basin: a case study, Atmos. Chem. Phys., 10, 7533–7544, https://doi.org/10.5194/acp-10-7533-2010, 2010.
Bègue, N., Tulet, P., Chaboureau, J. P., Roberts, G., Gomes, L., and Mallet, M.: Long-range transport of Saharan dust over north-western Europe during EUCAARI 2008 campaign: Evolution of dust optical properties by scavenging, J. Geophys. Res., 117, D17201, https://doi.org/10.1029/2012JD017611, 2012.
Berthier, S., Chazette, P., Couvert, P., Pelon, J., Dulac, F., Thieuleux, F., Moulin, C., and Pain, T.: Desert dust aerosol columnar properties over ocean and continental Africa from Lidar in-Space Technology Experiment (LITE) and Meteosat synergy. J. Geophys. Res., 111, D21202, https://doi.org/10.1029/2005JD006999, 2006.
Bhartia, P. K.: OMI/Aura TOMS-Like Ozone, Aerosol Index, Cloud Radiance Fraction Daily L3 Global 1.0 × 1.0 deg, version 003, NASA Goddard Space Flight Center, https://doi.org/10.5067/Aura/OMI/DATA3001, 2013.
Bollasina, M. A., Ming, Y., and Ramaswamy, V.: Anthropogenic Aerosols and the Weakening of the South Asian Summer Monsoon, Science, 334, 502–505, https://doi.org/10.1126/science.1204994, 2011.
Bösenberg, J., Matthias, V., Amodeo, A., Amoiridis, V., Ansmann, A., Baldasano, J. M., Balin, I., Balis, D., Böckmann, C., Boselli, A., Carlsson, G., Chaikovsky, A., Chourdakis, G., Comerón, A., De Tomasi, F., Eixmann, R., Freudenthaler, V., Giehl, H., Grigorov, I., Hågård, A., Iarlori, M., Kirsche, A., Kolarov, G., Komguem, L., Kreipl, S., Kumpf, W., Larchevêque, G., Linné, H., Matthey, R., Mattis, I., Mekler, A., Mironova, I., Mitev, V., Mona, L., Müller, D., Music, S., Nickovic, S., Pandolfi,M., Papayannis, A., Pappalardo, G., Pelon, J., Pérez, C., Perrone, R. M., Persson, R., Resendes, D. P., Rizi, V., Rocadenbosch, F., Rodrigues, J. A., Sauvage, L., Schneidenbach, L., Schumacher, R., Shcherbakov, V., Simeonov, V., Sobolewski, P., Spinelli, N., Stachlewska, I., Stoyanov, D., Trickl, T., Tsaknakis, G., Vaughan, G., Wandinger, U., Wang, X., Wiegner, M., Zavrtanik, M., and Zerefos, C.: A European aerosol research lidar network to establish an aerosol climatology, MPI-Rep. 317, Max-Planck Inst. für Meteorol., Hamburg, Germany, available at: http://www.mpimet.mpg.de/fileadmin/publikationen/Reports/max_scirep_348.pdf (last acce3ss: 28 May 2016), 2003.
Burton, S. P., Ferrare, R. A., Vaughan, M. A., Omar, A. H., Rogers, R. R., Hostetler, C. A., and Hair, J. W.: Aerosol classification from airborne HSRL and comparisons with the CALIPSO vertical feature mask, Atmos. Meas. Tech., 6, 1397–1412, https://doi.org/10.5194/amt-6-1397-2013, 2013.
Cachorro, V. E., Vergaz, R., de Frutos, A. M., Vilaplana, J. M., Henriques, D., Laulainen, N., and Toledano, C.: Study of desert dust events over the southwestern Iberian Peninsula in year 2000: two case studies, Ann. Geophys., 24, 1493–1510, https://doi.org/10.5194/angeo-24-1493-2006, 2006.
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Eck, T. F., Holben, B. N., Reid, J. S., Dubovik, O., Smirnov, A., O'Neill, N. T., Slutsker, I., and Kinne, S.: Wavelength dependence of optical depth of biomass burning, urban and desert dust aerosols, J. Geophys. Res., 104, 31333–31350, https://doi.org/10.1029/1999JD900923, 1999.
Eguchi, K., Uno, I., Yumimoto, K., Takemura, T., Shimizu, A., Sugimoto, N., and Liu, Z.: Trans-pacific dust transport: integrated analysis of NASA/CALIPSO and a global aerosol transport model, Atmos. Chem. Phys., 9, 3137–3145, https://doi.org/10.5194/acp-9-3137-2009, 2009.
Escudero, M., Querol, X., Pey, J., Alastuey, A., Pérez, N., Ferreira, F., Alonso, S., Rodríguez, S., and Cuevas, E.: A methodology for the quantification of the net African dust load in air quality monitoring networks, Atmos. Environ., 41, 5516–5524, https://doi.org/10.1016/j.atmosenv.2007.04.047, 2007.
Fotiadi, A., Hatzianastassiou, N., Drakakis, E., Matsoukas, C., Pavlakis, K. G., Hatzidimitriou, D., Gerasopoulos, E., Mihalopoulos, N., and Vardavas, I.: Aerosol physical and optical properties in the Eastern Mediterranean Basin, Crete, from Aerosol Robotic Network data, Atmos. Chem. Phys., 6, 5399–5413, https://doi.org/10.5194/acp-6-5399-2006, 2006.
Ginoux, P., Prospero, J. M., Gill, T. E., Hsu, N. C., and Zhao, M.: Global-scale attribution of anthropogenic and natural dust sources and their emission rates based on MODIS Deep Blue aerosol products, Rev. Geophys., 50, RG3005, https://doi.org/10.1029/2012rg000388, 2012.
Gkikas, A., Hatzianastassiou, N., and Mihalopoulos, N.: Aerosol events in the broader Mediterranean basin based on 7-year (2000–2007) MODIS C005 data, Ann. Geophys., 27, 3509–3522, https://doi.org/10.5194/angeo-27-3509-2009, 2009.
Gkikas, A., Hatzianastassiou, N., Mihalopoulos, N., Katsoulis, V., Kazadzis, S., Pey, J., Querol, X., and Torres, O.: The regime of intense desert dust episodes in the Mediterranean based on contemporary satellite observations and ground measurements, Atmos. Chem. Phys., 13, 12135–12154, https://doi.org/10.5194/acp-13-12135-2013, 2013.
Gkikas, A., Houssos, E. E., Lolis, C. J., Bartzokas, A., Mihalopoulos, N., and Hatzianastassiou, N.: Atmospheric circulation evolution related to desert-dust episodes over the Mediterranean, Q. J. Roy. Meteor. Soc., 141, 1634–1645, https://doi.org/10.1002/qj.2466, 2015.
Gkikas, A., Hatzianastassiou, N., Mihalopoulos, N., and Torres, O.: Characterization of aerosols episodes in the greater Mediterranean Sea area from satellite observations (2000–2007), Atmos. Environ., 128, 286–304, https://doi.org/10.1016/j.atmosenv.2015.11.056, 2016.
Gobbi, G. P., Barnaba, F., Giorgi, R., and Santacasa, A.: Altitude-resolved properties of a Saharan dust event over the Mediterranean, Atmos. Environ., 34, 5119–5127, https://doi.org/10.1016/S1352-2310(00)00194-1, 2000.
Gobbi, G. P., Kaufman, Y. J., Koren, I., and Eck, T. F.: Classification of aerosol properties derived from AERONET direct sun data, Atmos. Chem. Phys., 7, 453–458, https://doi.org/10.5194/acp-7-453-2007, 2007.
Gobbi, G. P., Angelini, F., Barnaba, F., Costabile, F., Baldasano, J. M., Basart, S., Sozzi, R., and Bolignano, A.: Changes in particulate matter physical properties during Saharan advections over Rome (Italy): a four-year study, 2001–2004, Atmos. Chem. Phys., 13, 7395–7404, https://doi.org/10.5194/acp-13-7395-2013, 2013.
Hamonou, E., Chazette, P., Balis, D., Dulac, F., Schneider, X., Galani, E., Ancellet, G., and Papayannis, A.: Characterization of the vertical structure of Saharan dust export to the Mediterranean basin, J. Geophys. Res., 104, 22257–22270, https://doi.org/10.1029/1999JD900257, 1999.
Hara, Y., Yumimoto, K., Uno, I., Shimizu, A., Sugimoto, N., Liu, Z., and Winker, D. M.: Asian dust outflow in the PBL and free atmosphere retrieved by NASA CALIPSO and an assimilated dust transport model, Atmos. Chem. Phys., 9, 1227–1239, https://doi.org/10.5194/acp-9-1227-2009, 2009.
Hatzianastassiou, N., Gkikas, A., Mihalopoulos, N., Torres, O., and Katsoulis, B. D.: Natural versus anthropogenic aerosols in the eastern Mediterranean basin derived from multiyear TOMS and MODIS satellite data, J. Geophys. Res., 114, D24202, https://doi.org/10.1029/2009JD011982, 2009.
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Heinold, B., Tegen, I., Schepanski, K., and Hellmuth, O.: Dust Radiative feedback on Saharan boundary layer dynamics and dust mobilization, Geophys. Res. Lett., 35, L20817, https://doi.org/10.1029/2008GL035319, 2008.
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Short summary
This study presents the 3-D structures of intense Mediterranean desert dust outbreaks, over the period Mar 2000–Feb 2013. The desert dust (DD) episodes are identified through an objective and dynamic algorithm, which utilizes satellite retrievals (MODIS, TOMS and OMI) as inputs. The performance of the satellite algorithm is evaluated vs. AERONET and PM10 data. The geometrical characteristics of the identified DD episodes are analyzed using the collocated CALIOP profiles as a complementary tool.
This study presents the 3-D structures of intense Mediterranean desert dust outbreaks, over the...
Atmospheric Chemistry and Physics
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