Articles | Volume 17, issue 24
Atmos. Chem. Phys., 17, 14987–15006, 2017

Special issue: The Saharan Aerosol Long-range Transport and Aerosol-Cloud-interaction...

Atmos. Chem. Phys., 17, 14987–15006, 2017

Research article 19 Dec 2017

Research article | 19 Dec 2017

Profiling of Saharan dust from the Caribbean to western Africa – Part 2: Shipborne lidar measurements versus forecasts

Albert Ansmann1, Franziska Rittmeister1, Ronny Engelmann1, Sara Basart2, Oriol Jorba2, Christos Spyrou3, Samuel Remy4, Annett Skupin1, Holger Baars1, Patric Seifert1, Fabian Senf1, and Thomas Kanitz5 Albert Ansmann et al.
  • 1Leibniz Institute for Tropospheric Research, Leipzig, Germany
  • 2Barcelona Supercomputing Center, Dep. of Earth Sciences, Barcelona, Spain
  • 3National and Kapodistrian University of Athens, Dep. of Physics, Athens, Greece
  • 4Laboratoire de Météorologie Dynamique, IPSL, UPMC/CNRS, Paris, France
  • 5ESTEC, Noordwijk, the Netherlands

Abstract. A unique 4-week ship cruise from Guadeloupe to Cabo Verde in April–May 2013 see part 1, Rittmeister et al. (2017) is used for an in-depth comparison of dust profiles observed with a polarization/Raman lidar aboard the German research vessel Meteor over the remote tropical Atlantic and respective dust forecasts of a regional (SKIRON) and two global atmospheric (dust) transport models (NMMB/BSC-Dust, MACC/CAMS). New options of model–observation comparisons are presented. We analyze how well the modeled fine dust (submicrometer particles) and coarse dust contributions to light extinction and mass concentration match respective lidar observations, and to what extent models, adjusted to aerosol optical thickness observations, are able to reproduce the observed layering and mixing of dust and non-dust (mostly marine) aerosol components over the remote tropical Atlantic. Based on the coherent set of dust profiles at well-defined distances from Africa (without any disturbance by anthropogenic aerosol sources over the ocean), we investigate how accurately the models handle dust removal at distances of 1500 km to more than 5000 km west of the Saharan dust source regions. It was found that (a) dust predictions are of acceptable quality for the first several days after dust emission up to 2000 km west of the African continent, (b) the removal of dust from the atmosphere is too strong for large transport paths in the global models, and (c) the simulated fine-to-coarse dust ratio (in terms of mass concentration and light extinction) is too high in the models compared to the observations. This deviation occurs initially close to the dust sources and then increases with distance from Africa and thus points to an overestimation of fine dust emission in the models.

Final-revised paper