Articles | Volume 19, issue 23
https://doi.org/10.5194/acp-19-14933-2019
https://doi.org/10.5194/acp-19-14933-2019
Research article
 | 
10 Dec 2019
Research article |  | 10 Dec 2019

Observations of highly oxidized molecules and particle nucleation in the atmosphere of Beijing

James Brean, Roy M. Harrison, Zongbo Shi, David C. S. Beddows, W. Joe F. Acton, C. Nicholas Hewitt, Freya A. Squires, and James Lee

Related authors

Multiple eco-regions contribute to the seasonal cycle of Antarctic aerosol size distributions
James Brean, David C. S. Beddows, Eija Asmi, Aki Virkkula, Lauriane L. J. Quéléver, Mikko Sipilä, Floortje Van Den Heuvel, Thomas Lachlan-Cope, Anna Jones, Markus Frey, Angelo Lupi, Jiyeon Park, Young Jun Yoon, Rolf Weller, Giselle L. Marincovich, Gabriela C. Mulena, Roy M. Harrison, and Manuel Dall'Osto
Atmos. Chem. Phys., 25, 1145–1162, https://doi.org/10.5194/acp-25-1145-2025,https://doi.org/10.5194/acp-25-1145-2025, 2025
Short summary
The behaviour of charged particles (ions) during new particle formation events in urban Leipzig, Germany
Alex Rowell, James Brean, David C. S. Beddows, Zongbo Shi, Avinash Kumar, Matti Rissanen, Miikka Dal Maso, Peter Mettke, Kay Weinhold, Maik Merkel, and Roy M. Harrison
Atmos. Chem. Phys., 24, 10349–10361, https://doi.org/10.5194/acp-24-10349-2024,https://doi.org/10.5194/acp-24-10349-2024, 2024
Short summary
Insights into the sources of ultrafine particle numbers at six European urban sites obtained by investigating COVID-19 lockdowns
Alex Rowell, James Brean, David C. S. Beddows, Tuukka Petäjä, Máté Vörösmarty, Imre Salma, Jarkko V. Niemi, Hanna E. Manninen, Dominik van Pinxteren, Thomas Tuch, Kay Weinhold, Zongbo Shi, and Roy M. Harrison
Atmos. Chem. Phys., 24, 9515–9531, https://doi.org/10.5194/acp-24-9515-2024,https://doi.org/10.5194/acp-24-9515-2024, 2024
Short summary
Collective geographical ecoregions and precursor sources driving Arctic new particle formation
James Brean, David C. S. Beddows, Roy M. Harrison, Congbo Song, Peter Tunved, Johan Ström, Radovan Krejci, Eyal Freud, Andreas Massling, Henrik Skov, Eija Asmi, Angelo Lupi, and Manuel Dall'Osto
Atmos. Chem. Phys., 23, 2183–2198, https://doi.org/10.5194/acp-23-2183-2023,https://doi.org/10.5194/acp-23-2183-2023, 2023
Short summary
Evaluation of isoprene nitrate chemistry in detailed chemical mechanisms
Alfred W. Mayhew, Ben H. Lee, Joel A. Thornton, Thomas J. Bannan, James Brean, James R. Hopkins, James D. Lee, Beth S. Nelson, Carl Percival, Andrew R. Rickard, Marvin D. Shaw, Peter M. Edwards, and Jaqueline F. Hamilton
Atmos. Chem. Phys., 22, 14783–14798, https://doi.org/10.5194/acp-22-14783-2022,https://doi.org/10.5194/acp-22-14783-2022, 2022
Short summary

Related subject area

Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Measurement report: Sources and meteorology influencing highly time-resolved PM2.5 trace elements at three urban sites in the extremely polluted Indo-Gangetic Plain in India
Ashutosh K. Shukla, Sachchida N. Tripathi, Shamitaksha Talukdar, Vishnu Murari, Sreenivas Gaddamidi, Manousos-Ioannis Manousakas, Vipul Lalchandani, Kuldeep Dixit, Vinayak M. Ruge, Peeyush Khare, Mayank Kumar, Vikram Singh, Neeraj Rastogi, Suresh Tiwari, Atul K. Srivastava, Dilip Ganguly, Kaspar Rudolf Daellenbach, and André S. H. Prévôt
Atmos. Chem. Phys., 25, 3765–3784, https://doi.org/10.5194/acp-25-3765-2025,https://doi.org/10.5194/acp-25-3765-2025, 2025
Short summary
Formation of highly absorptive secondary brown carbon through nighttime multiphase chemistry of biomass burning emissions
Ye Kuang, Biao Luo, Shan Huang, Junwen Liu, Weiwei Hu, Yuwen Peng, Duohong Chen, Dingli Yue, Wanyun Xu, Bin Yuan, and Min Shao
Atmos. Chem. Phys., 25, 3737–3752, https://doi.org/10.5194/acp-25-3737-2025,https://doi.org/10.5194/acp-25-3737-2025, 2025
Short summary
Measurement report: Vertically resolved atmospheric properties observed over the Southern Great Plains with the ArcticShark uncrewed aerial system
Fan Mei, Qi Zhang, Damao Zhang, Jerome D. Fast, Gourihar Kulkarni, Mikhail S. Pekour, Christopher R. Niedek, Susanne Glienke, Israel Silber, Beat Schmid, Jason M. Tomlinson, Hardeep S. Mehta, Xena Mansoura, Zezhen Cheng, Gregory W. Vandergrift, Nurun Nahar Lata, Swarup China, and Zihua Zhu
Atmos. Chem. Phys., 25, 3425–3444, https://doi.org/10.5194/acp-25-3425-2025,https://doi.org/10.5194/acp-25-3425-2025, 2025
Short summary
Non-biogenic sources are an important but overlooked contributor to aerosol isoprene-derived organosulfates during winter in northern China
Ting Yang, Yu Xu, Yu-Chen Wang, Yi-Jia Ma, Hong-Wei Xiao, Hao Xiao, and Hua-Yun Xiao
Atmos. Chem. Phys., 25, 2967–2978, https://doi.org/10.5194/acp-25-2967-2025,https://doi.org/10.5194/acp-25-2967-2025, 2025
Short summary
The critical role of aqueous-phase processes in aromatic-derived nitrogen-containing organic aerosol formation in cities with different energy consumption patterns
Yi-Jia Ma, Yu Xu, Ting Yang, Lin Gui, Hong-Wei Xiao, Hao Xiao, and Hua-Yun Xiao
Atmos. Chem. Phys., 25, 2763–2780, https://doi.org/10.5194/acp-25-2763-2025,https://doi.org/10.5194/acp-25-2763-2025, 2025
Short summary

Cited articles

Alam, A., Shi, J. P., and Harrison R. M.: Observations of new particle formation in urban air, J. Geophys. Res., 108, 4093–4107, https://doi.org/10.1029/2001JD001417, 2003. 
Atkinson, R., Aschmann, S. M., Carter, W. P. L., Winer, A. M., and Pitts, J. N.: Alkyl nitrate formation from the nitrogen oxide (NOx) air photooxidations of C2C8 n-alkanes, J. Phys. Chem., 86, 4563–4569, 1982. 
Berndt, T., Richters, S., Kaethner, R., Voigtländer, J., Stratmann, F., Sipilä, M., Kulmala, M., and Herrmann, H.: Gas-Phase Ozonolysis of Cycloalkenes: Formation of Highly Oxidized RO2 Radicals and Their Reactions with NO, NO2, SO2, and Other RO2 Radicals, J. Phys. Chem. A., 119, 10336–10348, 2015. 
Berndt, T., Richters, S., Jokinen, T., Hyttinen, N., Kurtén, T., Otkjær, R. V., Kjaergaard, H. G., Stratmann, F., Herrmann, H., Sipilä, M., Kulmala, M., and Ehn, M.: Hydroxyl radical-induced formation of highly oxidized organic compounds, Nature Comm., 7, 13677, https://doi.org/10.1038/ncomms13677, 2016. 
Download
Short summary
Measurements of highly oxidized molecules measured during a summer campaign in Beijing are presented. These molecules represent an intermediary between gas-phase chemicals from which they are formed and airborne particles which form from them. Conclusions are drawn as to the factors affecting the formation of new particles within the Beijing atmosphere.
Share
Altmetrics
Final-revised paper
Preprint