Articles | Volume 19, issue 23
https://doi.org/10.5194/acp-19-14933-2019
https://doi.org/10.5194/acp-19-14933-2019
Research article
 | 
10 Dec 2019
Research article |  | 10 Dec 2019

Observations of highly oxidized molecules and particle nucleation in the atmosphere of Beijing

James Brean, Roy M. Harrison, Zongbo Shi, David C. S. Beddows, W. Joe F. Acton, C. Nicholas Hewitt, Freya A. Squires, and James Lee

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Cited articles

Alam, A., Shi, J. P., and Harrison R. M.: Observations of new particle formation in urban air, J. Geophys. Res., 108, 4093–4107, https://doi.org/10.1029/2001JD001417, 2003. 
Atkinson, R., Aschmann, S. M., Carter, W. P. L., Winer, A. M., and Pitts, J. N.: Alkyl nitrate formation from the nitrogen oxide (NOx) air photooxidations of C2C8 n-alkanes, J. Phys. Chem., 86, 4563–4569, 1982. 
Berndt, T., Richters, S., Kaethner, R., Voigtländer, J., Stratmann, F., Sipilä, M., Kulmala, M., and Herrmann, H.: Gas-Phase Ozonolysis of Cycloalkenes: Formation of Highly Oxidized RO2 Radicals and Their Reactions with NO, NO2, SO2, and Other RO2 Radicals, J. Phys. Chem. A., 119, 10336–10348, 2015. 
Berndt, T., Richters, S., Jokinen, T., Hyttinen, N., Kurtén, T., Otkjær, R. V., Kjaergaard, H. G., Stratmann, F., Herrmann, H., Sipilä, M., Kulmala, M., and Ehn, M.: Hydroxyl radical-induced formation of highly oxidized organic compounds, Nature Comm., 7, 13677, https://doi.org/10.1038/ncomms13677, 2016. 
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Short summary
Measurements of highly oxidized molecules measured during a summer campaign in Beijing are presented. These molecules represent an intermediary between gas-phase chemicals from which they are formed and airborne particles which form from them. Conclusions are drawn as to the factors affecting the formation of new particles within the Beijing atmosphere.
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