Articles | Volume 19, issue 23
https://doi.org/10.5194/acp-19-14933-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-14933-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
10 Dec 2019
Research article |
| 10 Dec 2019
| 10 Dec 2019
Observations of highly oxidized molecules and particle nucleation in the atmosphere of Beijing
James Brean
Division of Environmental Health and Risk Management, School of Geography, Earth and Environmental Sciences, University of Birmingham, Edgbaston, Birmingham B15 2TT, UK
Division of Environmental Health and Risk Management, School of Geography, Earth and Environmental Sciences, University of Birmingham, Edgbaston, Birmingham B15 2TT, UK
also at: Department of Environmental Sciences/Center of Excellence in Environmental Studies, King Abdulaziz University, P.O. Box 80203, Jeddah,
21589, Saudi Arabia
Zongbo Shi
Division of Environmental Health and Risk Management, School of Geography, Earth and Environmental Sciences, University of Birmingham, Edgbaston, Birmingham B15 2TT, UK
David C. S. Beddows
Division of Environmental Health and Risk Management, School of Geography, Earth and Environmental Sciences, University of Birmingham, Edgbaston, Birmingham B15 2TT, UK
W. Joe F. Acton
Lancaster Environment Centre, Lancaster University, Lancaster LA1 4YQ, UK
C. Nicholas Hewitt
Lancaster Environment Centre, Lancaster University, Lancaster LA1 4YQ, UK
Freya A. Squires
National Centre for Atmospheric Science, Wolfson Atmospheric Chemistry Laboratories, University of York, York YO10 5DD, UK
James Lee
National Centre for Atmospheric Science, Wolfson Atmospheric Chemistry Laboratories, University of York, York YO10 5DD, UK
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- A phenomenology of new particle formation (NPF) at 13 European sites D. Bousiotis et al. 10.5194/acp-21-11905-2021
- Evaluating the sensitivity of radical chemistry and ozone formation to ambient VOCs and NOx in Beijing L. Whalley et al. 10.5194/acp-21-2125-2021
- The striking effect of vertical mixing in the planetary boundary layer on new particle formation in the Yangtze River Delta S. Lai et al. 10.1016/j.scitotenv.2022.154607
- Influence of anthropogenic emissions on the composition of highly oxygenated organic molecules in Helsinki: a street canyon and urban background station comparison M. Okuljar et al. 10.5194/acp-23-12965-2023
- Seasonal variation in oxygenated organic molecules in urban Beijing and their contribution to secondary organic aerosol Y. Guo et al. 10.5194/acp-22-10077-2022
- Resolving Atmospheric Oxygenated Organic Molecules in Urban Beijing Using Online Ultrahigh-Resolution Chemical Ionization Mass Spectrometry Y. Yuan et al. 10.1021/acs.est.4c04214
- Using highly time-resolved online mass spectrometry to examine biogenic and anthropogenic contributions to organic aerosol in Beijing A. Mehra et al. 10.1039/D0FD00080A
- Road Traffic Emissions Lead to Much Enhanced New Particle Formation through Increased Growth Rates J. Brean et al. 10.1021/acs.est.3c10526
- Enigma of Urban Gaseous Oxygenated Organic Molecules: Precursor Type, Role of NOx, and Degree of Oxygenation L. Tian et al. 10.1021/acs.est.2c05047
- Oxygenated products formed from OH-initiated reactions of trimethylbenzene: autoxidation and accretion Y. Wang et al. 10.5194/acp-20-9563-2020
- Low-NO atmospheric oxidation pathways in a polluted megacity M. Newland et al. 10.5194/acp-21-1613-2021
- Hydrolysis reactivity reveals significant seasonal variation in the composition of organic peroxides in ambient PM2.5 Y. Dai et al. 10.1016/j.scitotenv.2024.172143
- Particle-Bound Highly Oxidized Organic Molecules Derived from Aromatic Hydrocarbons in an Urban Atmosphere M. Zhu et al. 10.1021/acs.estlett.2c00841
- Estimates of Future New Particle Formation under Different Emission Scenarios in Beijing J. Brean et al. 10.1021/acs.est.2c08348
- Field Detection of Highly Oxygenated Organic Molecules in Shanghai by Chemical Ionization–Orbitrap Y. Zhang et al. 10.1021/acs.est.1c08346
- Effect of wet flue gas desulfurization on the concentrations and component profiles of condensable particulate matter from ultralow emission coal-fired power plants C. Yuan et al. 10.1016/j.apr.2022.101376
- Nighttime reactions of a series of unsaturated alcohols with NO3•: Kinetics, products and mechanisms study Y. Xu et al. 10.1016/j.jes.2024.03.043
- Contribution of Atmospheric Oxygenated Organic Compounds to Particle Growth in an Urban Environment X. Qiao et al. 10.1021/acs.est.1c02095
- On the influence of VOCs on new particle growth in a Continental-Mediterranean region F. Gómez-Moreno et al. 10.1088/2515-7620/acacf0
- Large differences of highly oxygenated organic molecules (HOMs) and low-volatile species in secondary organic aerosols (SOAs) formed from ozonolysis of β-pinene and limonene D. Liu et al. 10.5194/acp-23-8383-2023
- Investigating three patterns of new particles growing to the size of cloud condensation nuclei in Beijing's urban atmosphere L. Ma et al. 10.5194/acp-21-183-2021
- Molecular Characterization of Oxygenated Organic Molecules and Their Dominating Roles in Particle Growth in Hong Kong P. Zheng et al. 10.1021/acs.est.2c09252
- Molecular insights into new particle formation in Barcelona, Spain J. Brean et al. 10.5194/acp-20-10029-2020
- Molecular Composition of Oxygenated Organic Molecules and Their Contributions to Organic Aerosol in Beijing Y. Wang et al. 10.1021/acs.est.1c05191
- An aldehyde as a rapid source of secondary aerosol precursors: theoretical and experimental study of hexanal autoxidation S. Barua et al. 10.5194/acp-23-10517-2023
- Photolysis of nitrophenols in gas phase and aqueous environment: a potential daytime source for atmospheric nitrous acid (HONO) S. Guo & H. Li 10.1039/D2EA00053A
- Structures and reactivity of peroxy radicals and dimeric products revealed by online tandem mass spectrometry S. Tomaz et al. 10.1038/s41467-020-20532-2
- Open ocean and coastal new particle formation from sulfuric acid and amines around the Antarctic Peninsula J. Brean et al. 10.1038/s41561-021-00751-y
- Airborne particulate matter R. Harrison 10.1098/rsta.2019.0319
30 citations as recorded by crossref.
- Emission of organic components and distribution characteristics of PAHs in condensable particulate matter from coal-fired power and industrial plants Y. Wu et al. 10.1016/j.joei.2021.04.011
- A phenomenology of new particle formation (NPF) at 13 European sites D. Bousiotis et al. 10.5194/acp-21-11905-2021
- Evaluating the sensitivity of radical chemistry and ozone formation to ambient VOCs and NOx in Beijing L. Whalley et al. 10.5194/acp-21-2125-2021
- The striking effect of vertical mixing in the planetary boundary layer on new particle formation in the Yangtze River Delta S. Lai et al. 10.1016/j.scitotenv.2022.154607
- Influence of anthropogenic emissions on the composition of highly oxygenated organic molecules in Helsinki: a street canyon and urban background station comparison M. Okuljar et al. 10.5194/acp-23-12965-2023
- Seasonal variation in oxygenated organic molecules in urban Beijing and their contribution to secondary organic aerosol Y. Guo et al. 10.5194/acp-22-10077-2022
- Resolving Atmospheric Oxygenated Organic Molecules in Urban Beijing Using Online Ultrahigh-Resolution Chemical Ionization Mass Spectrometry Y. Yuan et al. 10.1021/acs.est.4c04214
- Using highly time-resolved online mass spectrometry to examine biogenic and anthropogenic contributions to organic aerosol in Beijing A. Mehra et al. 10.1039/D0FD00080A
- Road Traffic Emissions Lead to Much Enhanced New Particle Formation through Increased Growth Rates J. Brean et al. 10.1021/acs.est.3c10526
- Enigma of Urban Gaseous Oxygenated Organic Molecules: Precursor Type, Role of NOx, and Degree of Oxygenation L. Tian et al. 10.1021/acs.est.2c05047
- Oxygenated products formed from OH-initiated reactions of trimethylbenzene: autoxidation and accretion Y. Wang et al. 10.5194/acp-20-9563-2020
- Low-NO atmospheric oxidation pathways in a polluted megacity M. Newland et al. 10.5194/acp-21-1613-2021
- Hydrolysis reactivity reveals significant seasonal variation in the composition of organic peroxides in ambient PM2.5 Y. Dai et al. 10.1016/j.scitotenv.2024.172143
- Particle-Bound Highly Oxidized Organic Molecules Derived from Aromatic Hydrocarbons in an Urban Atmosphere M. Zhu et al. 10.1021/acs.estlett.2c00841
- Estimates of Future New Particle Formation under Different Emission Scenarios in Beijing J. Brean et al. 10.1021/acs.est.2c08348
- Field Detection of Highly Oxygenated Organic Molecules in Shanghai by Chemical Ionization–Orbitrap Y. Zhang et al. 10.1021/acs.est.1c08346
- Effect of wet flue gas desulfurization on the concentrations and component profiles of condensable particulate matter from ultralow emission coal-fired power plants C. Yuan et al. 10.1016/j.apr.2022.101376
- Nighttime reactions of a series of unsaturated alcohols with NO3•: Kinetics, products and mechanisms study Y. Xu et al. 10.1016/j.jes.2024.03.043
- Contribution of Atmospheric Oxygenated Organic Compounds to Particle Growth in an Urban Environment X. Qiao et al. 10.1021/acs.est.1c02095
- On the influence of VOCs on new particle growth in a Continental-Mediterranean region F. Gómez-Moreno et al. 10.1088/2515-7620/acacf0
- Large differences of highly oxygenated organic molecules (HOMs) and low-volatile species in secondary organic aerosols (SOAs) formed from ozonolysis of β-pinene and limonene D. Liu et al. 10.5194/acp-23-8383-2023
- Investigating three patterns of new particles growing to the size of cloud condensation nuclei in Beijing's urban atmosphere L. Ma et al. 10.5194/acp-21-183-2021
- Molecular Characterization of Oxygenated Organic Molecules and Their Dominating Roles in Particle Growth in Hong Kong P. Zheng et al. 10.1021/acs.est.2c09252
- Molecular insights into new particle formation in Barcelona, Spain J. Brean et al. 10.5194/acp-20-10029-2020
- Molecular Composition of Oxygenated Organic Molecules and Their Contributions to Organic Aerosol in Beijing Y. Wang et al. 10.1021/acs.est.1c05191
- An aldehyde as a rapid source of secondary aerosol precursors: theoretical and experimental study of hexanal autoxidation S. Barua et al. 10.5194/acp-23-10517-2023
- Photolysis of nitrophenols in gas phase and aqueous environment: a potential daytime source for atmospheric nitrous acid (HONO) S. Guo & H. Li 10.1039/D2EA00053A
- Structures and reactivity of peroxy radicals and dimeric products revealed by online tandem mass spectrometry S. Tomaz et al. 10.1038/s41467-020-20532-2
- Open ocean and coastal new particle formation from sulfuric acid and amines around the Antarctic Peninsula J. Brean et al. 10.1038/s41561-021-00751-y
- Airborne particulate matter R. Harrison 10.1098/rsta.2019.0319
Latest update: 06 Jul 2025
Short summary
Measurements of highly oxidized molecules measured during a summer campaign in Beijing are presented. These molecules represent an intermediary between gas-phase chemicals from which they are formed and airborne particles which form from them. Conclusions are drawn as to the factors affecting the formation of new particles within the Beijing atmosphere.
Measurements of highly oxidized molecules measured during a summer campaign in Beijing are...
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