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An interactive open-access journal of the European Geosciences Union
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Volume 16, issue 11
Atmos. Chem. Phys., 16, 6735–6756, 2016
https://doi.org/10.5194/acp-16-6735-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-6735-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 16, 6735–6756, 2016
https://doi.org/10.5194/acp-16-6735-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-6735-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
Research article 03 Jun 2016
Research article | 03 Jun 2016
Analysis of the potential of near-ground measurements of CO2 and CH4 in London, UK, for the monitoring of city-scale emissions using an atmospheric transport model
Alex Boon et al.
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Alkuin Maximilian Koenig, Olivier Magand, Paolo Laj, Marcos Andrade, Isabel Moreno, Fernando Velarde, Grover Salvatierra, René Gutierrez, Luis Blacutt, Diego Aliaga, Thomas Reichler, Karine Sellegri, Olivier Laurent, Michel Ramonet, and Aurélien Dommergue
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-988, https://doi.org/10.5194/acp-2020-988, 2020
Preprint under review for ACP
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The environmental cycling of atmospheric mercury, a harmful global contaminant, is still not sufficiently constrained, partly due to missing data in remote regions. Here, we address this issue by presenting 20 months of atmospheric mercury measurements, sampled in the Bolivian Andes. We observe a significant seasonal pattern, whose key features we explore. Moreover, we deduce ratios to constrain South American biomass burning mercury emissions and the mercury uptake by the Amazon rainforest.
Guillaume Monteil, Grégoire Broquet, Marko Scholze, Matthew Lang, Ute Karstens, Christoph Gerbig, Frank-Thomas Koch, Naomi E. Smith, Rona L. Thompson, Ingrid T. Luijkx, Emily White, Antoon Meesters, Philippe Ciais, Anita L. Ganesan, Alistair Manning, Michael Mischurow, Wouter Peters, Philippe Peylin, Jerôme Tarniewicz, Matt Rigby, Christian Rödenbeck, Alex Vermeulen, and Evie M. Walton
Atmos. Chem. Phys., 20, 12063–12091, https://doi.org/10.5194/acp-20-12063-2020, https://doi.org/10.5194/acp-20-12063-2020, 2020
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The paper presents the first results from the EUROCOM project, a regional atmospheric inversion intercomparison exercise involving six European research groups. It aims to produce an estimate of the net carbon flux between the European terrestrial ecosystems and the atmosphere for the period 2006–2015, based on constraints provided by observed CO2 concentrations and using inverse modelling techniques. The use of six different models enables us to investigate the robustness of the results.
Yidi Xu, Philippe Ciais, Le Yu, Wei Li, Xiuzhi Chen, Haicheng Zhang, Chao Yue, Kasturi Kanniah, Arthur P. Cracknell, and Peng Gong
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-252, https://doi.org/10.5194/gmd-2020-252, 2020
Preprint under review for GMD
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In this study, we implemented the specific morphology, phenology and harvest process of oil palm in the global land surface model ORCHIDEE-MICT. The improved model generally reproduces the leaf area index, biomass density and fruit yield during the life cycle with observations. This explicit representation of oil palm in global land surface model offers a useful tool for understanding the ecological processes of oil palm growth and assessing the environmental impacts of oil palm plantations.
Bowen Cao, Le Yu, Victoria Naipal, Philippe Ciais, Wei Li, Yuanyuan Zhao, Wei Wei, Die Chen, Zhuang Liu, and Peng Gong
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2020-157, https://doi.org/10.5194/essd-2020-157, 2020
Preprint under review for ESSD
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In this study, the first 30 m resolution terrace map of China was developed through supervised pixel-based classification using multi-source, multi-temporal data based on the Google Earth Engine platform. The classification performed well with an overall accuracy of 94 %. The terrace mapping algorithm can be used to map large-scale terraces in other regions globally, and the terrace map will be valuable for studies on soil erosion, carbon cycle, and ecosystem services assessments.
Yuan Zhang, Olivier Boucher, Philippe Ciais, Laurent Li, and Nicolas Bellouin
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-267, https://doi.org/10.5194/gmd-2020-267, 2020
Preprint under review for GMD
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We investigated different methods to reconstruct spatio-temporal distribution of the fraction of diffuse radiation (Fdf) to qualtify the aerosol impacts on GPP using ORCHIDEE_DF land surface model. We find that climatologically-averaging methods which dampens the variability of Fdf can cause significant bias in the modeled diffuse radiation impacts on GPP. Better methods to do the reconstruction of Fdf are recommended.
Rui Guo, Jiaoyue Wang, Longfei Bing, Dan Tong, Philippe Ciais, Steven J. Davis, Robbie M. Andrew, Fengming Xi, and Zhu Liu
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2020-275, https://doi.org/10.5194/essd-2020-275, 2020
Preprint under review for ESSD
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Using a life-cycle approach, we estimated the CO2 process emission as well as uptake of cement materials produced/consumed in 1930–2019. 21 Gt of CO2, about 52 % of the total process emission, had been abated through cement carbonation. China contributed the greatest to the cumulative uptake of more than 6 Gt (~30 % of the world total) while ~65 % of the total uptake was attributed to mortar of more than 12 Gt. Cement CO2 uptake makes up a considerable part of human carbon budget.
Pierre Friedlingstein, Michael O'Sullivan, Matthew W. Jones, Robbie M. Andrew, Judith Hauck, Are Olsen, Glen P. Peters, Wouter Peters, Julia Pongratz, Stephen Sitch, Corinne Le Quéré, Josep G. Canadell, Philippe Ciais, Robert B. Jackson, Simone Alin, Luiz E. O. C. Aragão, Almut Arneth, Vivek Arora, Nicholas R. Bates, Meike Becker, Alice Benoit-Cattin, Henry C. Bittig, Laurent Bopp, Selma Bultan, Naveen Chandra, Frédéric Chevallier, Louise P. Chini, Wiley Evans, Liesbeth Florentie, Piers M. Forster, Thomas Gasser, Marion Gehlen, Dennis Gilfillan, Thanos Gkritzalis, Luke Gregor, Nicolas Gruber, Ian Harris, Kerstin Hartung, Vanessa Haverd, Richard A. Houghton, Tatiana Ilyina, Atul K. Jain, Emilie Joetzjer, Koji Kadono, Etsushi Kato, Vassilis Kitidis, Jan Ivar Korsbakken, Peter Landschützer, Nathalie Lefèvre, Andrew Lenton, Sebastien Lienert, Zhu Liu, Danica Lombardozzi, Gregg Marland, Nicolas Metzl, David R Munro, Julia E. M. S. Nabel, Shin-Ichiro Nakaoka, Yosuke Niwa, Kevin O'Brien, Tsuneo Ono, Paul I. Palmer, Denis Pierrot, Benjamin Poulter, Laure Resplandy, Eddy Robertson, Christian Rödenbeck, Jörg Schwinger, Roland Séférian, Ingunn Skjelvan, Adam J. P. Smith, Adrienne J. Sutton, Toste Tanhua, Pieter P. Tans, Hanqin Tian, Bronte Tilbrook, Guido van der Werf, Nicolas Vuichard, Anthony P. Walker, Rik Wanninkhof, Andrew J. Watson, David Willis, Andrew J. Wiltshire, Wenping Yuan, Xu Yue, and Sönke Zaehle
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2020-286, https://doi.org/10.5194/essd-2020-286, 2020
Revised manuscript under review for ESSD
Ingeborg Levin, Ute Karstens, Markus Eritt, Fabian Maier, Sabrina Arnold, Daniel Rzesanke, Samuel Hammer, Michel Ramonet, Gabriela Vítková, Sebastien Conil, Michal Heliasz, Dagmar Kubistin, and Matthias Lindauer
Atmos. Chem. Phys., 20, 11161–11180, https://doi.org/10.5194/acp-20-11161-2020, https://doi.org/10.5194/acp-20-11161-2020, 2020
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Based on observations and Stochastic Time-Inverted Lagrangian Transport (STILT) footprint modelling, a sampling strategy has been developed for tall tower stations of the Integrated Carbon Observation System (ICOS) research infrastructure atmospheric station network. This strategy allows independent quality control of in situ measurements, provides representative coverage of the influence area of the sites, and is capable of automated targeted sampling of fossil fuel CO2 emission hotspots.
Philippe Ciais, Ana Bastos, Frédéric Chevallier, Ronny Lauerwald, Ben Poulter, Pep Canadell, Gustaf Hugelius, Robert B. Jackson, Atul Jain, Matthew Jones, Masayuki Kondo, Ingrid Luijkx, Prabir K. Patra, Wouter Peters, Julia Pongratz, A. M. Roxanna Petrescu, Shilong Piao, Chunjing Qiu, Celso Von Randow, Pierre Regnier, Marielle Saunois, Robert Scholes, Anatoli Shvidenko, Hanqin Tian, Hui Yang, Xuhui Wang, and Bo Zheng
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-259, https://doi.org/10.5194/gmd-2020-259, 2020
Preprint under review for GMD
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The phase-2 of the Regional Carbon Cycle Assessment and Processes (RECCAP) will provide updated quantification and process understanding of CO2, CH4 and N2O emissions and sinks for ten regions of the globe. In this manuscript, we provide definitions, review different methods and make recommendations to the RECCAP community for estimating different components of the total land-atmosphere carbon exchange for each region in a consistent and complete approach.
Thomas Gasser, Léa Crepin, Yann Quilcaille, Richard A. Houghton, Philippe Ciais, and Michael Obersteiner
Biogeosciences, 17, 4075–4101, https://doi.org/10.5194/bg-17-4075-2020, https://doi.org/10.5194/bg-17-4075-2020, 2020
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We combine several lines of evidence to provide a robust estimate of historical CO2 emissions from land use change. Our novel approach leads to reduced uncertainty and identifies key remaining sources of uncertainty and discrepancy.
We also quantify the carbon removal by natural ecosystems that would have occurred if these ecosystems had not been destroyed (mostly via deforestation). Over the last decade, this foregone carbon sink amounted to about 50 % of the actual emissions.
Yuanhong Zhao, Marielle Saunois, Philippe Bousquet, Xin Lin, Antoine Berchet, Michaela I. Hegglin, Josep G. Canadell, Robert B. Jackson, Edward J. Dlugokencky, Ray L. Langenfelds, Michel Ramonet, Doug Worthy, and Bo Zheng
Atmos. Chem. Phys., 20, 9525–9546, https://doi.org/10.5194/acp-20-9525-2020, https://doi.org/10.5194/acp-20-9525-2020, 2020
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The hydroxyl radical (OH), which is the dominant sink of methane (CH4), plays a key role in closing the global methane budget. This study quantifies how uncertainties in the hydroxyl radical can influence top-down estimates of CH4 emissions based on 4D Bayesian inversions with different OH fields and the same surface observations. We show that uncertainties in CH4 emissions driven by different OH fields are comparable to the uncertainties given by current bottom-up and top-down estimations.
Yan Sun, Daniel S. Goll, Jinfeng Chang, Philippe Ciais, Betrand Guenet, Julian Helfenstein, Yuanyuan Huang, Ronny Lauerwald, Fabienne Maignan, Victoria Naipal, Yilong Wang, Hui Yang, and Haicheng Zhang
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-93, https://doi.org/10.5194/gmd-2020-93, 2020
Preprint under review for GMD
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We evaluated the performance of nutrient enabled version land surface model ORCHIDEE-CNP v 1.2 against remote-sensing, ground-based measurement networks and ecological databases. We find that the simulated carbon, nitrogen and phosphorus fluxes among different spatial scales are generally in good agreement with data-driven estimates. However, the recent carbon sink in the Northern Hemisphere is substantially underestimated. Potential causes, as well as model development priorities are discussed.
Xianfeng Liu, Xiaoming Feng, Philippe Ciais, and Bojie Fu
Hydrol. Earth Syst. Sci., 24, 3663–3676, https://doi.org/10.5194/hess-24-3663-2020, https://doi.org/10.5194/hess-24-3663-2020, 2020
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Freshwater availability is crucial for sustainable development across the Asian and eastern European regions. Our results indicate widespread decline in terrestrial water storage (TWS) over the region during 2002–2017, primarily due to the intensive over-extraction of groundwater and warmth-induced surface water loss. The findings provide insights into changes in TWS and its components over the Asian and eastern European regions, where there is growing demand for food grains and water supplies.
Bo Zheng, Frédéric Chevallier, Philippe Ciais, Grégoire Broquet, Yilong Wang, Jinghui Lian, and Yuanhong Zhao
Atmos. Chem. Phys., 20, 8501–8510, https://doi.org/10.5194/acp-20-8501-2020, https://doi.org/10.5194/acp-20-8501-2020, 2020
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The Paris Climate Agreement requires all parties to report CO2 emissions regularly. Given the self-reporting nature of this system, it is critical to evaluate the emission reports with independent observation systems. Here we present the direct observations of city CO2 plumes from space and the quantification of CO2 emissions from these observations over the largest emitter country China. The emissions from 46 hot-spot regions representing 13 % of China's total emissions can be well constrained.
Marielle Saunois, Ann R. Stavert, Ben Poulter, Philippe Bousquet, Josep G. Canadell, Robert B. Jackson, Peter A. Raymond, Edward J. Dlugokencky, Sander Houweling, Prabir K. Patra, Philippe Ciais, Vivek K. Arora, David Bastviken, Peter Bergamaschi, Donald R. Blake, Gordon Brailsford, Lori Bruhwiler, Kimberly M. Carlson, Mark Carrol, Simona Castaldi, Naveen Chandra, Cyril Crevoisier, Patrick M. Crill, Kristofer Covey, Charles L. Curry, Giuseppe Etiope, Christian Frankenberg, Nicola Gedney, Michaela I. Hegglin, Lena Höglund-Isaksson, Gustaf Hugelius, Misa Ishizawa, Akihiko Ito, Greet Janssens-Maenhout, Katherine M. Jensen, Fortunat Joos, Thomas Kleinen, Paul B. Krummel, Ray L. Langenfelds, Goulven G. Laruelle, Licheng Liu, Toshinobu Machida, Shamil Maksyutov, Kyle C. McDonald, Joe McNorton, Paul A. Miller, Joe R. Melton, Isamu Morino, Jurek Müller, Fabiola Murguia-Flores, Vaishali Naik, Yosuke Niwa, Sergio Noce, Simon O'Doherty, Robert J. Parker, Changhui Peng, Shushi Peng, Glen P. Peters, Catherine Prigent, Ronald Prinn, Michel Ramonet, Pierre Regnier, William J. Riley, Judith A. Rosentreter, Arjo Segers, Isobel J. Simpson, Hao Shi, Steven J. Smith, L. Paul Steele, Brett F. Thornton, Hanqin Tian, Yasunori Tohjima, Francesco N. Tubiello, Aki Tsuruta, Nicolas Viovy, Apostolos Voulgarakis, Thomas S. Weber, Michiel van Weele, Guido R. van der Werf, Ray F. Weiss, Doug Worthy, Debra Wunch, Yi Yin, Yukio Yoshida, Wenxin Zhang, Zhen Zhang, Yuanhong Zhao, Bo Zheng, Qing Zhu, Qiuan Zhu, and Qianlai Zhuang
Earth Syst. Sci. Data, 12, 1561–1623, https://doi.org/10.5194/essd-12-1561-2020, https://doi.org/10.5194/essd-12-1561-2020, 2020
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Understanding and quantifying the global methane (CH4) budget is important for assessing realistic pathways to mitigate climate change. We have established a consortium of multidisciplinary scientists under the umbrella of the Global Carbon Project to synthesize and stimulate new research aimed at improving and regularly updating the global methane budget. This is the second version of the review dedicated to the decadal methane budget, integrating results of top-down and bottom-up estimates.
Camille Yver-Kwok, Carole Philippon, Peter Bergamaschi, Tobias Biermann, Francescopiero Calzolari, Huilin Chen, Sébastien Conil, Paolo Cristofanelli, Marc Delmotte, Juha Hatakka, Michal Heliasz, Ove Hermansen, Kateřina Komínková, Dagmar Kubistin, Nicolas Kumps, Olivier Laurent, Tuomas Laurila, Irene Lehner, Janne Levula, Matthias Lindauer, Morgan Lopez, Ivan Mammarella, Giovanni Manca, Per Marklund, Jean-Marc Metzger, Meelis Mölder, Stephen M. Platt, Michel Ramonet, Leonard Rivier, Bert Scheeren, Mahesh Kumar Sha, Paul Smith, Martin Steinbacher, Gabriela Vítková, and Simon Wyss
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-213, https://doi.org/10.5194/amt-2020-213, 2020
Revised manuscript under review for AMT
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The Integrated Carbon Observation System (ICOS) is a pan-European research infrastructure which provides harmonized and high precision scientific data on the carbon cycle and the greenhouse gas (GHG) budget. All stations have to undergo a rigorous assessment before being labeled, i.e. receiving approval to join the network. In this paper, we present the labeling process for the ICOS atmospheric network through the 23 stations that have been labeled between November 2017 and November 2019.
Yi Yin, Frederic Chevallier, Philippe Ciais, Philippe Bousquet, Marielle Saunois, Bo Zheng, John Worden, A. Anthony Bloom, Robert Parker, Daniel Jacob, Edward J. Dlugokencky, and Christian Frankenberg
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-649, https://doi.org/10.5194/acp-2020-649, 2020
Preprint under review for ACP
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The growth of methane, the second most important anthropogenic greenhouse gas after carbon dioxide, has been accelerating in the atmosphere in recent years. Using an ensemble of multi-tracer atmospheric inversions constrained by surface or satellite observations, we show that global methane emissions increased by nearly 1 % per year over 2010–2017, with leading contributions from the tropics and East Asia.
Jinghui Lian, François-Marie Bréon, Grégoire Broquet, Bo Zheng, Michel Ramonet, and Philippe Ciais
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-540, https://doi.org/10.5194/acp-2020-540, 2020
Preprint under review for ACP
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Currently there is a growing interest in monitoring city-scale CO2 emissions based on atmospheric CO2 measurements, atmospheric transport modeling and inversion technique. We analyze the various sources of uncertainty that impact the atmospheric CO2 modeling and that may compromise the potential of this method for the monitoring of CO2 emission over Paris. Results suggest selection criteria for the assimilation of CO2 measurements into the inversion system that aims at retrieving city emissions.
Robert J. Parker, Alex Webb, Hartmut Boesch, Peter Somkuti, Rocio Barrio Guillo, Antonio Di Noia, Nikoleta Kalaitzi, Jasdeep Anand, Peter Bergamaschi, Frederic Chevallier, Paul I. Palmer, Liang Feng, Nicholas M. Deutscher, Dietrich G. Feist, David W. T. Griffith, Frank Hase, Rigel Kivi, Isamu Morino, Justus Notholt, Young-Suk Oh, Hirofumi Ohyama, Christof Petri, David F. Pollard, Coleen Roehl, Mahesh K. Sha, Kei Shiomi, Kimberly Strong, Ralf Sussmann, Yao Te, Voltaire A. Velazco, Thorsten Warneke, Paul O. Wennberg, and Debra Wunch
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2020-114, https://doi.org/10.5194/essd-2020-114, 2020
Revised manuscript accepted for ESSD
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This work presents the latest release of the University of Leicester GOSAT methane data and acts as the definitive description of this dataset. We detail the processing, validation and evaluation involved in producing this data and highlight its many applications. With now over a decade of global atmospheric methane observations, this dataset has helped, and will continue to help, us better understand the global methane budget and investigate how it may respond to a future changing climate.
Franz Slemr, Lynwill Martin, Casper Labuschagne, Thumeka Mkololo, Hélène Angot, Olivier Magand, Aurélien Dommergue, Philippe Garat, Michel Ramonet, and Johannes Bieser
Atmos. Chem. Phys., 20, 7683–7692, https://doi.org/10.5194/acp-20-7683-2020, https://doi.org/10.5194/acp-20-7683-2020, 2020
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Monitoring of atmospheric mercury (Hg) concentrations is an important part of the effectiveness evaluation of the Minamata Convention on Hg. Hg concentrations in 2012–2017 at Cape Point, South Africa, and at Amsterdam Island in the remote Indian Ocean are comparable, and no trend or a slightly downward trend was observed at both stations. Over the 2007–2017 period an upward trend was observed at CPT which was driven mainly by the 2007–2014 data. The trend and its change are discussed.
Jean-Luc Baray, Laurent Deguillaume, Aurélie Colomb, Karine Sellegri, Evelyn Freney, Clémence Rose, Joël Van Baelen, Jean-Marc Pichon, David Picard, Patrick Fréville, Laëtitia Bouvier, Mickaël Ribeiro, Pierre Amato, Sandra Banson, Angelica Bianco, Agnès Borbon, Lauréline Bourcier, Yannick Bras, Marcello Brigante, Philippe Cacault, Aurélien Chauvigné, Tiffany Charbouillot, Nadine Chaumerliac, Anne-Marie Delort, Marc Delmotte, Régis Dupuy, Antoine Farah, Guy Febvre, Andrea Flossmann, Christophe Gourbeyre, Claude Hervier, Maxime Hervo, Nathalie Huret, Muriel Joly, Victor Kazan, Morgan Lopez, Gilles Mailhot, Angela Marinoni, Olivier Masson, Nadège Montoux, Marius Parazols, Frédéric Peyrin, Yves Pointin, Michel Ramonet, Manon Rocco, Martine Sancelme, Stéphane Sauvage, Martina Schmidt, Emmanuel Tison, Mickaël Vaïtilingom, Paolo Villani, Miao Wang, Camille Yver-Kwok, and Paolo Laj
Atmos. Meas. Tech., 13, 3413–3445, https://doi.org/10.5194/amt-13-3413-2020, https://doi.org/10.5194/amt-13-3413-2020, 2020
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CO-PDD (Cézeaux-Aulnat-Opme-puy de Dôme) is a fully instrumented platform for atmospheric research. The four sites located at different altitudes from 330 to 1465 m around Clermont-Ferrand (France) host in situ and remote sensing instruments to measure atmospheric composition, including long-term trends and variability, to study interconnected processes (microphysical, chemical, biological, chemical, and dynamical) and to provide a reference point for climate models.
Bruno Ringeval, Christoph Müller, Thomas A.M. Pugh, Nathaniel D. Mueller, Philippe Ciais, Christian Folberth, Wenfeng Liu, Philippe Debaeke, and Sylvain Pellerin
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-113, https://doi.org/10.5194/gmd-2020-113, 2020
Preprint under review for GMD
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We assess how and why Global Gridded Crop Models (GGCMs) differ in their simulation of potential yield. We build an emulator of GGCMs based on generic formalism, and fit its parameters against aboveground biomass and yield at harvest simulated by 8 GGCMs. Despite huge differences between GGCMs, we show that the calibration of few key parameters allows the emulator to reproduce the GGCM simulations. Our simple but mechanistic model would help to improve the global simulation of potential yield.
Pramod Kumar, Grégoire Broquet, Camille Yver-Kwok, Olivier Laurent, Susan Gichuki, Christopher Caldow, Ford Cropley, Thomas Lauvaux, Michel Ramonet, Guillaume Berthe, Frédéric Martin, Olivier Duclaux, Catherine Juery, Caroline Bouchet, and Philippe Ciais
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-226, https://doi.org/10.5194/amt-2020-226, 2020
Preprint under review for AMT
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This study presents a simple atmospheric inversion modeling framework for the localization and quantification of unknown CH4 and CO2 emissions from point sources based on near-surface mobile concentration measurements and a Gaussian plume dispersion model. It is applied for the estimate of a series of brief controlled releases of CH4 and CO2 with a wide range of rates during the TOTAL's TADI-2018 experiment. Results indicate a 20–30 % average error on the estimate of the release rates.
Leslie David, Francois-Marie Bréon, and Frédéric Chevallier
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-177, https://doi.org/10.5194/amt-2020-177, 2020
Revised manuscript under review for AMT
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This paper shows that a Neural Network approach can be used to process spaceborne observations from the OCO-2 satellite and retrieve both the surface pressure and the atmospheric CO2 content. The accuracy evaluation indicates that the retrievals have an accuracy that is at least as good as those of the operational approach that relies on complex algorithms and that is very computer intensive. The approach is therefore a very promising alternative for the processing of CO2-monitoring missions.
Diego Santaren, Grégoire Broquet, François-Marie Bréon, Frédéric Chevallier, Denis Siméoni, and Philippe Ciais
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-138, https://doi.org/10.5194/amt-2020-138, 2020
Revised manuscript under review for AMT
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Atmospheric transport inversions with synthetic data are used to assess the potential of new satellite observations of atmospheric CO2 to monitor anthropogenic emissions from regions, cities and large industrial plants. The analysis, applied to a large ensemble of sources in Western Europe, shows a strong dependence of the results to different characteristics of the spaceborne instrument, to the source emission budgets and spreads, and to the wind conditions.
Claudia Grossi, Scott D. Chambers, Olivier Llido, Felix R. Vogel, Victor Kazan, Alessandro Capuana, Sylvester Werczynski, Roger Curcoll, Marc Delmotte, Arturo Vargas, Josep-Anton Morguí, Ingeborg Levin, and Michel Ramonet
Atmos. Meas. Tech., 13, 2241–2255, https://doi.org/10.5194/amt-13-2241-2020, https://doi.org/10.5194/amt-13-2241-2020, 2020
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The sustainable support of radon metrology at the environmental level offers new scientific possibilities for the quantification of greenhouse gas (GHG) emissions and the determination of their source terms as well as for the identification of radioactive sources for the assessment of radiation exposure. This study helps to harmonize the techniques commonly used for atmospheric radon and radon progeny activity concentration measurements.
Wei Min Hao, Matthew C. Reeves, L. Scott Baggett, Yves Balkanski, Philippe Ciais, Bryce L. Nordgren, Alexander Petkov, Rachel E. Corley, Florent Mouillot, Shawn P. Urbanski, and Chao Yue
Biogeosciences Discuss., https://doi.org/10.5194/bg-2020-139, https://doi.org/10.5194/bg-2020-139, 2020
Preprint under review for BG
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1) We examined the trends of spatial and temporal distribution of the area burned in northern Eurasia from 2002 to 2016.
2) The annual area burned in this region declined by 53 % during the 15-year period.
3) Grassland fires in Kazakhstan dominated the fire activity, comprising 47 % of the area burned but accounting for 84 % of the decline.
4) Wetter climate and the increase of grazing livestock in Kazakhstan are the major factors contributing to the decline of the area burned.
Ana Maria Roxana Petrescu, Glen P. Peters, Greet Janssens-Maenhout, Philippe Ciais, Francesco N. Tubiello, Giacomo Grassi, Gert-Jan Nabuurs, Adrian Leip, Gema Carmona-Garcia, Wilfried Winiwarter, Lena Höglund-Isaksson, Dirk Günther, Efisio Solazzo, Anja Kiesow, Ana Bastos, Julia Pongratz, Julia E. M. S. Nabel, Giulia Conchedda, Roberto Pilli, Robbie M. Andrew, Mart-Jan Schelhaas, and Albertus J. Dolman
Earth Syst. Sci. Data, 12, 961–1001, https://doi.org/10.5194/essd-12-961-2020, https://doi.org/10.5194/essd-12-961-2020, 2020
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This study is topical and provides a state-of-the-art scientific overview of data availability from bottom-up GHG anthropogenic emissions from agriculture, forestry and other land use (AFOLU) in the EU28. The data integrate recent AFOLU emission inventories with ecosystem data and land carbon models, aiming at reconciling GHG budgets with official country-level UNFCCC inventories. We provide comprehensive emission assessments in support to policy, facilitating real-time verification procedures.
Yidi Xu, Le Yu, Wei Li, Philippe Ciais, Yuqi Cheng, and Peng Gong
Earth Syst. Sci. Data, 12, 847–867, https://doi.org/10.5194/essd-12-847-2020, https://doi.org/10.5194/essd-12-847-2020, 2020
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The first annual oil palm area dataset (AOPD) for Malaysia and Indonesia from 2001 to 2016 was produced by integrating multiple satellite datasets and a change-detection algorithm (BFAST). This dataset reveals that oil palm plantations have expanded from 5.69 to 19.05 M ha in the two countries during the past 16 years. The AOPD is useful in understanding the deforestation process in Southeast Asia and may serve as land-use change inputs in dynamic global vegetation models.
Zun Yin, Catherine Ottlé, Philippe Ciais, Feng Zhou, Xuhui Wang, Polcher Jan, Patrice Dumas, Shushi Peng, Laurent Li, Xudong Zhou, and Shilong Piao
Hydrol. Earth Syst. Sci. Discuss., https://doi.org/10.5194/hess-2020-7, https://doi.org/10.5194/hess-2020-7, 2020
Preprint under review for HESS
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We improved the irrigation module in a land surface model and developed a dam operation model in aim to investigate how these human activities affect the discharge of the Yellow River in China. The results show that the irrigation mainly result in the decrease of the discharge. The dam operations, however, mainly affect the river discharge fluctuations. By considering only two operation rules: flood control and base flow guarantee, our dam model can sustainably improve the simulation accuracy.
Didier G. Leibovici, Shaun Quegan, Edward Comyn-Platt, Garry Hayman, Maria Val Martin, Mathieu Guimberteau, Arsène Druel, Dan Zhu, and Philippe Ciais
Biogeosciences, 17, 1821–1844, https://doi.org/10.5194/bg-17-1821-2020, https://doi.org/10.5194/bg-17-1821-2020, 2020
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Analysing the impact of environmental changes due to climate change, e.g. geographical spread of climate-sensitive infections (CSIs) and agriculture crop modelling, may require land surface modelling (LSM) to predict future land surface conditions. There are multiple LSMs to choose from. The paper proposes a multivariate spatio-temporal data science method to understand the inherent uncertainties in four LSMs and the variations between them in Nordic areas for the net primary production.
Wei Li, Philippe Ciais, Elke Stehfest, Detlef van Vuuren, Alexander Popp, Almut Arneth, Fulvio Di Fulvio, Jonathan Doelman, Florian Humpenöder, Anna B. Harper, Taejin Park, David Makowski, Petr Havlik, Michael Obersteiner, Jingmeng Wang, Andreas Krause, and Wenfeng Liu
Earth Syst. Sci. Data, 12, 789–804, https://doi.org/10.5194/essd-12-789-2020, https://doi.org/10.5194/essd-12-789-2020, 2020
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We generated spatially explicit bioenergy crop yields based on field measurements with climate, soil condition and remote-sensing variables as explanatory variables and the machine-learning method. We further compared our yield maps with the maps from three integrated assessment models (IAMs; IMAGE, MAgPIE and GLOBIOM) and found that the median yields in our maps are > 50 % higher than those in the IAM maps.
Antoine Berchet, Isabelle Pison, Patrick M. Crill, Brett Thornton, Philippe Bousquet, Thibaud Thonat, Thomas Hocking, Joël Thanwerdas, Jean-Daniel Paris, and Marielle Saunois
Atmos. Chem. Phys., 20, 3987–3998, https://doi.org/10.5194/acp-20-3987-2020, https://doi.org/10.5194/acp-20-3987-2020, 2020
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Methane isotopes in the atmosphere can help us differentiate between emission processes. A large variety of natural and anthropogenic emission types are active in the Arctic and are unsatisfactorily understood and documented up to now. A ship-based campaign was carried out in summer 2014, providing a unique dataset of isotopic measurements in the Arctic Ocean. Using a chemistry-transport model, we link these measurements to circumpolar emissions and retrieve information about their signature.
Hong Xuan Do, Fang Zhao, Seth Westra, Michael Leonard, Lukas Gudmundsson, Julien Eric Stanislas Boulange, Jinfeng Chang, Philippe Ciais, Dieter Gerten, Simon N. Gosling, Hannes Müller Schmied, Tobias Stacke, Camelia-Eliza Telteu, and Yoshihide Wada
Hydrol. Earth Syst. Sci., 24, 1543–1564, https://doi.org/10.5194/hess-24-1543-2020, https://doi.org/10.5194/hess-24-1543-2020, 2020
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We presented a global comparison between observed and simulated trends in a flood index over the 1971–2005 period using the Global Streamflow Indices and Metadata archive and six global hydrological models available through The Inter-Sectoral Impact Model Intercomparison Project. Streamflow simulations over 2006–2099 period robustly project high flood hazard in several regions. These high-flood-risk areas, however, are under-sampled by the current global streamflow databases.
Shamil Maksyutov, Tomohiro Oda, Makoto Saito, Rajesh Janardanan, Dmitry Belikov, Johannes W. Kaiser, Ruslan Zhuravlev, Alexander Ganshin, Vinu K. Valsala, Arlyn Andrews, Lukasz Chmura, Edward Dlugokencky, László Haszpra, Ray L. Langenfelds, Toshinobu Machida, Takakiyo Nakazawa, Michel Ramonet, Colm Sweeney, and Douglas Worthy
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-251, https://doi.org/10.5194/acp-2020-251, 2020
Revised manuscript under review for ACP
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In order to improve the top-down estimation of the anthropogenic greenhouse gas emissions, a high-resolution inverse modeling technique was developed for applications to global transport modeling of carbon dioxide and other greenhouse gases. A coupled Eulerian-Lagrangian transport model and its adjoint are combined with surface fluxes at 0.1-degree resolution to provide high-resolution forward simulation and inverse modeling of surface fluxes accounting for signals from emission hotspots.
Victoria Naipal, Ronny Lauerwald, Philippe Ciais, Bertrand Guenet, and Yilong Wang
Geosci. Model Dev., 13, 1201–1222, https://doi.org/10.5194/gmd-13-1201-2020, https://doi.org/10.5194/gmd-13-1201-2020, 2020
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In this study we present the Carbon Erosion DYNAMics model (CE-DYNAM) that links sediment dynamics resulting from water erosion with the soil carbon cycle along a cascade of hillslopes, floodplains, and rivers. The model can simulate the removal of soil and carbon from eroding areas and their destination at regional scale. We calibrated and validated the model for the Rhine catchment, and we show that soil erosion is a potential large net carbon sink over the period 1850–2005.
Martin Jung, Christopher Schwalm, Mirco Migliavacca, Sophia Walther, Gustau Camps-Valls, Sujan Koirala, Peter Anthoni, Simon Besnard, Paul Bodesheim, Nuno Carvalhais, Frédéric Chevallier, Fabian Gans, Daniel S. Goll, Vanessa Haverd, Philipp Köhler, Kazuhito Ichii, Atul K. Jain, Junzhi Liu, Danica Lombardozzi, Julia E. M. S. Nabel, Jacob A. Nelson, Michael O'Sullivan, Martijn Pallandt, Dario Papale, Wouter Peters, Julia Pongratz, Christian Rödenbeck, Stephen Sitch, Gianluca Tramontana, Anthony Walker, Ulrich Weber, and Markus Reichstein
Biogeosciences, 17, 1343–1365, https://doi.org/10.5194/bg-17-1343-2020, https://doi.org/10.5194/bg-17-1343-2020, 2020
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We test the approach of producing global gridded carbon fluxes based on combining machine learning with local measurements, remote sensing and climate data. We show that we can reproduce seasonal variations in carbon assimilated by plants via photosynthesis and in ecosystem net carbon balance. The ecosystem’s mean carbon balance and carbon flux trends require cautious interpretation. The analysis paves the way for future improvements of the data-driven assessment of carbon fluxes.
Adam Hastie, Ronny Lauerwald, Philippe Ciais, Fabrice Papa, and Pierre Regnier
Earth Syst. Dynam. Discuss., https://doi.org/10.5194/esd-2020-3, https://doi.org/10.5194/esd-2020-3, 2020
Preprint under review for ESD
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We used a model of the Congo basin to investigate the transfer of carbon (C) from land (vegetation and soils) to inland waters. We find that leaching of C to inland waters, emissions of CO2 from the water surface, and the export of C to the coast have all increased over the last century, driven by increasing atmospheric CO2 levels and climate change. We predict that these trends will continue through the 21st century with potential implications for pH levels and the ecology of the Congo River.
Simon P. K. Bowring, Ronny Lauerwald, Bertrand Guenet, Dan Zhu, Matthieu Guimberteau, Pierre Regnier, Ardalan Tootchi, Agnès Ducharne, and Philippe Ciais
Geosci. Model Dev., 13, 507–520, https://doi.org/10.5194/gmd-13-507-2020, https://doi.org/10.5194/gmd-13-507-2020, 2020
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In this second part of the study, we performed simulations of the carbon and water budget of the Lena catchment with the land surface model ORCHIDEE MICT-LEAK, enabled to simulate dissolved organic carbon (DOC) production in soils and its transport and fate in high-latitude inland waters. We compare simulations using this model to existing data sources to show that it is capable of reproducing dissolved carbon fluxes of potentially great importance for the future of the global permafrost.
Yilong Wang, Grégoire Broquet, François-Marie Bréon, Franck Lespinas, Michael Buchwitz, Maximilian Reuter, Yasjka Meijer, Armin Loescher, Greet Janssens‑Maenhout, Bo Zheng, and Philippe Ciais
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2019-326, https://doi.org/10.5194/gmd-2019-326, 2020
Revised manuscript accepted for GMD
Gerrit Kuhlmann, Grégoire Broquet, Julia Marshall, Valentin Clément, Armin Löscher, Yasjka Meijer, and Dominik Brunner
Atmos. Meas. Tech., 12, 6695–6719, https://doi.org/10.5194/amt-12-6695-2019, https://doi.org/10.5194/amt-12-6695-2019, 2019
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The Copernicus Anthropogenic CO2 Monitoring (CO2M) mission is a proposed constellation of imaging satellites with a CO2 instrument as main payload and optionally instruments for NO2, CO and aerosols. This study demonstrates the huge benefit of an NO2 instrument for detecting city plumes and weak point sources. Its main advantages are the higher signal-to-noise ratio and the lower sensitivity to clouds that significantly increases the number of observations available for quantifying CO2 emission.
Sébastien Conil, Julie Helle, Laurent Langrene, Olivier Laurent, Marc Delmotte, and Michel Ramonet
Atmos. Meas. Tech., 12, 6361–6383, https://doi.org/10.5194/amt-12-6361-2019, https://doi.org/10.5194/amt-12-6361-2019, 2019
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Continuous measurements of greenhouse gases using high-precision spectrometers started in 2011 on a tall tower with three sampling inlets at 10 m, 50 m and 120 m above the ground at the OPE station, in the eastern part of France. The measurement strategy for carbon dioxide (CO2), methane (CH4) and carbon monoxide (CO) follows the ICOS recommendations. Over the 2011–2018 period, the CO2 and CH4 data show trends with annual growth rates of 2.4 ppm yr−1 and 8.8 ppb yr−1 at the 120 m level.
Pierre Friedlingstein, Matthew W. Jones, Michael O'Sullivan, Robbie M. Andrew, Judith Hauck, Glen P. Peters, Wouter Peters, Julia Pongratz, Stephen Sitch, Corinne Le Quéré, Dorothee C. E. Bakker, Josep G. Canadell, Philippe Ciais, Robert B. Jackson, Peter Anthoni, Leticia Barbero, Ana Bastos, Vladislav Bastrikov, Meike Becker, Laurent Bopp, Erik Buitenhuis, Naveen Chandra, Frédéric Chevallier, Louise P. Chini, Kim I. Currie, Richard A. Feely, Marion Gehlen, Dennis Gilfillan, Thanos Gkritzalis, Daniel S. Goll, Nicolas Gruber, Sören Gutekunst, Ian Harris, Vanessa Haverd, Richard A. Houghton, George Hurtt, Tatiana Ilyina, Atul K. Jain, Emilie Joetzjer, Jed O. Kaplan, Etsushi Kato, Kees Klein Goldewijk, Jan Ivar Korsbakken, Peter Landschützer, Siv K. Lauvset, Nathalie Lefèvre, Andrew Lenton, Sebastian Lienert, Danica Lombardozzi, Gregg Marland, Patrick C. McGuire, Joe R. Melton, Nicolas Metzl, David R. Munro, Julia E. M. S. Nabel, Shin-Ichiro Nakaoka, Craig Neill, Abdirahman M. Omar, Tsuneo Ono, Anna Peregon, Denis Pierrot, Benjamin Poulter, Gregor Rehder, Laure Resplandy, Eddy Robertson, Christian Rödenbeck, Roland Séférian, Jörg Schwinger, Naomi Smith, Pieter P. Tans, Hanqin Tian, Bronte Tilbrook, Francesco N. Tubiello, Guido R. van der Werf, Andrew J. Wiltshire, and Sönke Zaehle
Earth Syst. Sci. Data, 11, 1783–1838, https://doi.org/10.5194/essd-11-1783-2019, https://doi.org/10.5194/essd-11-1783-2019, 2019
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The Global Carbon Budget 2019 describes the data sets and methodology used to quantify the emissions of carbon dioxide and their partitioning among the atmosphere, land, and ocean. These living data are updated every year to provide the highest transparency and traceability in the reporting of CO2, the key driver of climate change.
Frédéric Chevallier, Marine Remaud, Christopher W. O'Dell, David Baker, Philippe Peylin, and Anne Cozic
Atmos. Chem. Phys., 19, 14233–14251, https://doi.org/10.5194/acp-19-14233-2019, https://doi.org/10.5194/acp-19-14233-2019, 2019
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We present a way to rate the CO2 flux estimates made from inversion of a global atmospheric transport model. Our approach relies on accurate aircraft measurements in the free troposphere. It shows that some satellite soundings can now provide inversion results that are, despite their uncertainty, comparable in credibility to traditional inversions using the accurate but sparse surface network and that these inversions are, therefore, complementary for studies of the global carbon budget.
Minqiang Zhou, Bavo Langerock, Mahesh Kumar Sha, Nicolas Kumps, Christian Hermans, Christof Petri, Thorsten Warneke, Huilin Chen, Jean-Marc Metzger, Rigel Kivi, Pauli Heikkinen, Michel Ramonet, and Martine De Mazière
Atmos. Meas. Tech., 12, 6125–6141, https://doi.org/10.5194/amt-12-6125-2019, https://doi.org/10.5194/amt-12-6125-2019, 2019
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In this study, CH4 vertical profile is retrieved by SFIT4 code from FTIR NIR spectra based on six sites during 2016–2017. The degree of freedom for signal of the SFIT4NIR retrieval is about 2.4, with two distinct species of information in the troposphere and in the stratosphere. By comparison against other measurements, e.g. TCCON standard products, satellite observations and AirCore measurements, the uncertainties of the SFIT4NIR total column and partial columns are estimated and discussed.
Peter J. Rayner, Anna M. Michalak, and Frédéric Chevallier
Atmos. Chem. Phys., 19, 13911–13932, https://doi.org/10.5194/acp-19-13911-2019, https://doi.org/10.5194/acp-19-13911-2019, 2019
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This paper describes the methods for combining models and data to understand how nutrients and pollutants move through natural systems. The methods are analogous to the process of weather forecasting in which previous information is combined with new observations and a model to improve our knowledge of the internal state of the physical system. The methods appear highly diverse but the paper shows that they are all examples of a single underlying formalism.
Jinghui Lian, François-Marie Bréon, Grégoire Broquet, T. Scott Zaccheo, Jeremy Dobler, Michel Ramonet, Johannes Staufer, Diego Santaren, Irène Xueref-Remy, and Philippe Ciais
Atmos. Chem. Phys., 19, 13809–13825, https://doi.org/10.5194/acp-19-13809-2019, https://doi.org/10.5194/acp-19-13809-2019, 2019
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CO2 emissions within urban areas impact nearby and downwind concentrations. A different system, based on bi-wavelength laser measurements, has been deployed over Paris. It samples CO2 concentrations along horizontal lines, between a transceiver and a reflector. In this paper, we analyze the measurements provided by this system, together with the more classical in situ sampling and high-resolution modeling. We focus on the temporal and spatial variability of atmospheric CO2 concentrations.
Minqiang Zhou, Bavo Langerock, Corinne Vigouroux, Mahesh Kumar Sha, Christian Hermans, Jean-Marc Metzger, Huilin Chen, Michel Ramonet, Rigel Kivi, Pauli Heikkinen, Dan Smale, David F. Pollard, Nicholas Jones, Voltaire A. Velazco, Omaira E. García, Matthias Schneider, Mathias Palm, Thorsten Warneke, and Martine De Mazière
Atmos. Meas. Tech., 12, 5979–5995, https://doi.org/10.5194/amt-12-5979-2019, https://doi.org/10.5194/amt-12-5979-2019, 2019
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The differences between the TCCON and NDACC XCO measurements are investigated and discussed based on six NDACC–TCCON sites (Ny-Ålesund, Bremen, Izaña, Saint-Denis, Wollongong and Lauder) using data over the period 2007–2017. The smoothing errors from both TCCON and NDACC measurements are estimated. In addition, the scaling factor of the TCCON XCO data is reassessed by comparing with the AirCore measurements at Sodankylä and Orléans.
Joël Thanwerdas, Marielle Saunois, Antoine Berchet, Isabelle Pison, Didier Hauglustaine, Michel Ramonet, Cyril Crevoisier, Bianca Baier, Colm Sweeney, and Philippe Bousquet
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2019-925, https://doi.org/10.5194/acp-2019-925, 2019
Revised manuscript not accepted
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Oxidation by the hydroxyl radical (OH) is the dominant atmospheric sink for methane, contributing to approximately 90 % of the total methane loss. Chemical losses by reaction with atomic oxygen (O1D) and chlorine radicals (Cl) in the stratosphere are other sinks, contributing about 3 % to the total methane destruction. We assess here the impact of atomic Cl on atmospheric methane mixing ratios, methane atmospheric loss and atmospheric isotopic δ13C-CH4 values.
Ana Bastos, Philippe Ciais, Frédéric Chevallier, Christian Rödenbeck, Ashley P. Ballantyne, Fabienne Maignan, Yi Yin, Marcos Fernández-Martínez, Pierre Friedlingstein, Josep Peñuelas, Shilong L. Piao, Stephen Sitch, William K. Smith, Xuhui Wang, Zaichun Zhu, Vanessa Haverd, Etsushi Kato, Atul K. Jain, Sebastian Lienert, Danica Lombardozzi, Julia E. M. S. Nabel, Philippe Peylin, Benjamin Poulter, and Dan Zhu
Atmos. Chem. Phys., 19, 12361–12375, https://doi.org/10.5194/acp-19-12361-2019, https://doi.org/10.5194/acp-19-12361-2019, 2019
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Here we show that land-surface models improved their ability to simulate the increase in the amplitude of seasonal CO2-cycle exchange (SCANBP) by ecosystems compared to estimates by two atmospheric inversions. We find a dominant role of vegetation growth over boreal Eurasia to the observed increase in SCANBP, strongly driven by CO2 fertilization, and an overall negative effect of temperature on SCANBP. Biases can be explained by the sensitivity of simulated microbial respiration to temperature.
Thibaud Thonat, Marielle Saunois, Isabelle Pison, Antoine Berchet, Thomas Hocking, Brett F. Thornton, Patrick M. Crill, and Philippe Bousquet
Atmos. Chem. Phys., 19, 12141–12161, https://doi.org/10.5194/acp-19-12141-2019, https://doi.org/10.5194/acp-19-12141-2019, 2019
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This paper discusses the methane isotopic signals that could be detected at instrumental surface sites in the northern high latitudes using a 3–D chemistry transport model. Isotopic signals may be used in atmospheric inverse systems to better characterize methane emissions and changes. We show that depending on the source magnitude and the location of the site, detecting isotopic signals of specific individual sources may be challenging for the new generation of methane isotope instruments.
Bo Zheng, Frederic Chevallier, Yi Yin, Philippe Ciais, Audrey Fortems-Cheiney, Merritt N. Deeter, Robert J. Parker, Yilong Wang, Helen M. Worden, and Yuanhong Zhao
Earth Syst. Sci. Data, 11, 1411–1436, https://doi.org/10.5194/essd-11-1411-2019, https://doi.org/10.5194/essd-11-1411-2019, 2019
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We use a multi-species atmospheric Bayesian inversion approach to attribute satellite-observed atmospheric carbon monoxide (CO) variations to its sources and sinks in order to achieve a full closure of the global CO budget during 2000–2017. We identify a declining trend in the global CO budget since 2000, driven by reduced anthropogenic emissions in the US, Europe, and China, as well as by reduced biomass burning emissions globally, especially in equatorial Africa.
Audrey Fortems-Cheiney, Isabelle Pison, Gaelle Dufour, Grégoire Broquet, Antoine Berchet, Elise Potier, Adriana Coman, Guillaume Siour, and Lorenzo Costantino
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2019-186, https://doi.org/10.5194/gmd-2019-186, 2019
Revised manuscript under review for GMD
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Up-to-date and accurate emission inventories for air pollutants are essential for understanding their role in the formation of tropospheric ozone and particulate matter, for anticipating pollution peaks and for identifying the key drivers that could help mitigate their emissions. Complementarily with bottom-up inventories, the system described here aims at updating and improving the knowledge on the high spatio-temporal variability of emissions of air pollutant and their precursors.
Bruno Ringeval, Marko Kvakić, Laurent Augusto, Philippe Ciais, Daniel Goll, Nathaniel D. Mueller, Christoph Müller, Thomas Nesme, Nicolas Vuichard, Xuhui Wang, and Sylvain Pellerin
Biogeosciences Discuss., https://doi.org/10.5194/bg-2019-298, https://doi.org/10.5194/bg-2019-298, 2019
Preprint withdrawn
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Crossed fertilization additions lead to the definition of nutrient interaction categories. However, the implications of such categories in terms of nutrient interaction modeling are not clear. We developed a theoretical analysis of nitrogen and phosphorus fertilization experiments, then applied it to current estimates of nutrient limitation in cropland. We found that a true co-limitation could affect up to 42 % of the global maize area when using a given formalism of nutrient interaction.
Simon P. K. Bowring, Ronny Lauerwald, Bertrand Guenet, Dan Zhu, Matthieu Guimberteau, Ardalan Tootchi, Agnès Ducharne, and Philippe Ciais
Geosci. Model Dev., 12, 3503–3521, https://doi.org/10.5194/gmd-12-3503-2019, https://doi.org/10.5194/gmd-12-3503-2019, 2019
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Few Earth system models represent permafrost soil biogeochemistry, contributing to uncertainty in estimating its response and that of the planet to warming. Because the permafrost contains over double the carbon in the present atmosphere, its fate as it is
unlockedby warming is globally significant. One way it can be mobilised is into rivers, the sea, or the atmosphere: a vector previously ignored in climate modelling. We present a model scheme for resolving this vector at a global scale.
Sean Crowell, David Baker, Andrew Schuh, Sourish Basu, Andrew R. Jacobson, Frederic Chevallier, Junjie Liu, Feng Deng, Liang Feng, Kathryn McKain, Abhishek Chatterjee, John B. Miller, Britton B. Stephens, Annmarie Eldering, David Crisp, David Schimel, Ray Nassar, Christopher W. O'Dell, Tomohiro Oda, Colm Sweeney, Paul I. Palmer, and Dylan B. A. Jones
Atmos. Chem. Phys., 19, 9797–9831, https://doi.org/10.5194/acp-19-9797-2019, https://doi.org/10.5194/acp-19-9797-2019, 2019
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Space-based retrievals of carbon dioxide offer the potential to provide dense data in regions that are sparsely observed by the surface network. We find that flux estimates that are informed by the Orbiting Carbon Observatory-2 (OCO-2) show different character from that inferred using surface measurements in tropical land regions, particularly in Africa, with a much larger total emission and larger amplitude seasonal cycle.
Chunjing Qiu, Dan Zhu, Philippe Ciais, Bertrand Guenet, Shushi Peng, Gerhard Krinner, Ardalan Tootchi, Agnès Ducharne, and Adam Hastie
Geosci. Model Dev., 12, 2961–2982, https://doi.org/10.5194/gmd-12-2961-2019, https://doi.org/10.5194/gmd-12-2961-2019, 2019
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We present a model that can simulate the dynamics of peatland area extent and the vertical buildup of peat. The model is validated across a range of northern peatland sites and over the Northern Hemisphere (> 30° N). It is able to reproduce the spatial extent of northern peatlands and peat carbon accumulation over the Holocene.
Anna Agustí-Panareda, Michail Diamantakis, Sébastien Massart, Frédéric Chevallier, Joaquín Muñoz-Sabater, Jérôme Barré, Roger Curcoll, Richard Engelen, Bavo Langerock, Rachel M. Law, Zoë Loh, Josep Anton Morguí, Mark Parrington, Vincent-Henri Peuch, Michel Ramonet, Coleen Roehl, Alex T. Vermeulen, Thorsten Warneke, and Debra Wunch
Atmos. Chem. Phys., 19, 7347–7376, https://doi.org/10.5194/acp-19-7347-2019, https://doi.org/10.5194/acp-19-7347-2019, 2019
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This paper demonstrates the benefits of using global models with high horizontal resolution to represent atmospheric CO2 patterns associated with evolving weather. The modelling of CO2 weather is crucial to interpret the variability from ground-based and satellite CO2 observations, which can then be used to infer CO2 fluxes in atmospheric inversions. The benefits of high resolution come from an improved representation of the topography, winds, tracer transport and CO2 flux distribution.
Yilong Wang, Philippe Ciais, Grégoire Broquet, François-Marie Bréon, Tomohiro Oda, Franck Lespinas, Yasjka Meijer, Armin Loescher, Greet Janssens-Maenhout, Bo Zheng, Haoran Xu, Shu Tao, Kevin R. Gurney, Geoffrey Roest, Diego Santaren, and Yongxian Su
Earth Syst. Sci. Data, 11, 687–703, https://doi.org/10.5194/essd-11-687-2019, https://doi.org/10.5194/essd-11-687-2019, 2019
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We address the question of the global characterization of fossil fuel CO2 emission hotspots that may cause coherent XCO2 plumes in space-borne CO2 images, based on the ODIAC global high-resolution 1 km fossil fuel emission data product. For space imagery with 0.5 ppm precision for a single XCO2 measurement, a total of 11 314 hotspots are identified, covering 72 % of the global emissions. These hotspots define the targets for the purpose of monitoring fossil fuel CO2 emissions from space.
Emmanuel Arzoumanian, Felix R. Vogel, Ana Bastos, Bakhram Gaynullin, Olivier Laurent, Michel Ramonet, and Philippe Ciais
Atmos. Meas. Tech., 12, 2665–2677, https://doi.org/10.5194/amt-12-2665-2019, https://doi.org/10.5194/amt-12-2665-2019, 2019
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We tested commercial lower-cost CO2 sensors in laboratory and field studies to see if they can measure atmospheric CO2 mole fractions with less than 1 ppm bias (with monthly calibration), to allow continuous urban CO2 monitoring.
We find that the sensors' CO2 readings are influenced by temperature, atmospheric pressure and water vapour content, but this can be corrected for by adding sensors (T, p, RH) and carefully calibrating each sensor against a high-precision instrument.
Dominik Brunner, Gerrit Kuhlmann, Julia Marshall, Valentin Clément, Oliver Fuhrer, Grégoire Broquet, Armin Löscher, and Yasjka Meijer
Atmos. Chem. Phys., 19, 4541–4559, https://doi.org/10.5194/acp-19-4541-2019, https://doi.org/10.5194/acp-19-4541-2019, 2019
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Atmospheric transport models are increasingly being used to estimate CO2 emissions from atmospheric CO2 measurements. This study demonstrates the importance of distributing CO2 emissions vertically in the model according to realistic profiles, since a major proportion of CO2 is emitted through tall stacks from power plants and industrial sources. With the traditional approach of emitting all CO2 at the surface, models may significantly overestimate the atmospheric CO2 levels.
Emily D. White, Matthew Rigby, Mark F. Lunt, T. Luke Smallman, Edward Comyn-Platt, Alistair J. Manning, Anita L. Ganesan, Simon O'Doherty, Ann R. Stavert, Kieran Stanley, Mathew Williams, Peter Levy, Michel Ramonet, Grant L. Forster, Andrew C. Manning, and Paul I. Palmer
Atmos. Chem. Phys., 19, 4345–4365, https://doi.org/10.5194/acp-19-4345-2019, https://doi.org/10.5194/acp-19-4345-2019, 2019
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Understanding carbon dioxide (CO2) fluxes from the terrestrial biosphere on a national scale is important for evaluating land use strategies to mitigate climate change. We estimate emissions of CO2 from the UK biosphere using atmospheric data in a top-down approach. Our findings show that bottom-up estimates from models of biospheric fluxes overestimate the amount of CO2 uptake in summer. This suggests these models wrongly estimate or omit key processes, e.g. land disturbance due to harvest.
Felix R. Vogel, Matthias Frey, Johannes Staufer, Frank Hase, Grégoire Broquet, Irène Xueref-Remy, Frédéric Chevallier, Philippe Ciais, Mahesh Kumar Sha, Pascale Chelin, Pascal Jeseck, Christof Janssen, Yao Té, Jochen Groß, Thomas Blumenstock, Qiansi Tu, and Johannes Orphal
Atmos. Chem. Phys., 19, 3271–3285, https://doi.org/10.5194/acp-19-3271-2019, https://doi.org/10.5194/acp-19-3271-2019, 2019
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Providing timely information on greenhouse gas emissions to stakeholders at sub-national scale is an emerging challenge and understanding urban CO2 levels is one key aspect. This study uses atmospheric observations of total column CO2 and compares them to numerical simulations to investigate CO2 levels in the Paris metropolitan area due to natural fluxes and anthropogenic emissions. Our measurements reveal the influence of locally added CO2, which our model is also able to predict.
Matthias Frey, Mahesh K. Sha, Frank Hase, Matthäus Kiel, Thomas Blumenstock, Roland Harig, Gregor Surawicz, Nicholas M. Deutscher, Kei Shiomi, Jonathan E. Franklin, Hartmut Bösch, Jia Chen, Michel Grutter, Hirofumi Ohyama, Youwen Sun, André Butz, Gizaw Mengistu Tsidu, Dragos Ene, Debra Wunch, Zhensong Cao, Omaira Garcia, Michel Ramonet, Felix Vogel, and Johannes Orphal
Atmos. Meas. Tech., 12, 1513–1530, https://doi.org/10.5194/amt-12-1513-2019, https://doi.org/10.5194/amt-12-1513-2019, 2019
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In a 3.5-year long study, the long-term performance of a mobile EM27/SUN spectrometer, used for greenhouse gas observations, is checked with respect to a co-located reference spectrometer. We find that the EM27/SUN is stable on timescales of several years, qualifying it for permanent carbon cycle studies.
The performance of an ensemble of 30 EM27/SUN spectrometers was also tested in the framework of the COllaborative Carbon Column Observing Network (COCCON) and found to be very uniform.
Carole Helfter, Neil Mullinger, Massimo Vieno, Simon O'Doherty, Michel Ramonet, Paul I. Palmer, and Eiko Nemitz
Atmos. Chem. Phys., 19, 3043–3063, https://doi.org/10.5194/acp-19-3043-2019, https://doi.org/10.5194/acp-19-3043-2019, 2019
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We present a novel approach to estimate the annual budgets of carbon dioxide (881.0 ± 128.5 Tg) and methane (2.55 ± 0.48 Tg) of the British Isles from shipborne measurements taken over a 3-year period (2015–2017). This study brings independent verification of the emission budgets estimated using alternative products and investigates the seasonality of these emissions, which is usually not possible.
Pierre Laurent, Florent Mouillot, Maria Vanesa Moreno, Chao Yue, and Philippe Ciais
Biogeosciences, 16, 275–288, https://doi.org/10.5194/bg-16-275-2019, https://doi.org/10.5194/bg-16-275-2019, 2019
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Fire propagation and fire size are usually considered to be proportional to fire intensity. We used a global database of fire patch size and fire radiative power, used as a proxy of fire intensity, to test this relationship at a global scale. We showed that in some regions fire size tends to saturate when a regional fire intensity threshold is reached. We concluded that increasing landscape fragmentation limits fire propagation and this effect should be accounted for in global fire modules.
Benjamin Gaubert, Britton B. Stephens, Sourish Basu, Frédéric Chevallier, Feng Deng, Eric A. Kort, Prabir K. Patra, Wouter Peters, Christian Rödenbeck, Tazu Saeki, David Schimel, Ingrid Van der Laan-Luijkx, Steven Wofsy, and Yi Yin
Biogeosciences, 16, 117–134, https://doi.org/10.5194/bg-16-117-2019, https://doi.org/10.5194/bg-16-117-2019, 2019
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We have compared global carbon budgets calculated from numerical inverse models and CO2 observations, and evaluated how these systems reproduce vertical gradients in atmospheric CO2 from aircraft measurements. We found that available models have converged on near-neutral tropical total fluxes for several decades, implying consistent sinks in intact tropical forests, and that assumed fossil fuel emissions and predicted atmospheric growth rates are now the dominant axes of disagreement.
Anja Rammig, Jens Heinke, Florian Hofhansl, Hans Verbeeck, Timothy R. Baker, Bradley Christoffersen, Philippe Ciais, Hannes De Deurwaerder, Katrin Fleischer, David Galbraith, Matthieu Guimberteau, Andreas Huth, Michelle Johnson, Bart Krujit, Fanny Langerwisch, Patrick Meir, Phillip Papastefanou, Gilvan Sampaio, Kirsten Thonicke, Celso von Randow, Christian Zang, and Edna Rödig
Geosci. Model Dev., 11, 5203–5215, https://doi.org/10.5194/gmd-11-5203-2018, https://doi.org/10.5194/gmd-11-5203-2018, 2018
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We propose a generic approach for a pixel-to-point comparison applicable for evaluation of models and remote-sensing products. We provide statistical measures accounting for the uncertainty in ecosystem variables. We demonstrate our approach by comparing simulated values of aboveground biomass, woody productivity and residence time of woody biomass from four dynamic global vegetation models (DGVMs) with measured inventory data from permanent plots in the Amazon rainforest.
Christopher W. O'Dell, Annmarie Eldering, Paul O. Wennberg, David Crisp, Michael R. Gunson, Brendan Fisher, Christian Frankenberg, Matthäus Kiel, Hannakaisa Lindqvist, Lukas Mandrake, Aronne Merrelli, Vijay Natraj, Robert R. Nelson, Gregory B. Osterman, Vivienne H. Payne, Thomas E. Taylor, Debra Wunch, Brian J. Drouin, Fabiano Oyafuso, Albert Chang, James McDuffie, Michael Smyth, David F. Baker, Sourish Basu, Frédéric Chevallier, Sean M. R. Crowell, Liang Feng, Paul I. Palmer, Mavendra Dubey, Omaira E. García, David W. T. Griffith, Frank Hase, Laura T. Iraci, Rigel Kivi, Isamu Morino, Justus Notholt, Hirofumi Ohyama, Christof Petri, Coleen M. Roehl, Mahesh K. Sha, Kimberly Strong, Ralf Sussmann, Yao Te, Osamu Uchino, and Voltaire A. Velazco
Atmos. Meas. Tech., 11, 6539–6576, https://doi.org/10.5194/amt-11-6539-2018, https://doi.org/10.5194/amt-11-6539-2018, 2018
Corinne Le Quéré, Robbie M. Andrew, Pierre Friedlingstein, Stephen Sitch, Judith Hauck, Julia Pongratz, Penelope A. Pickers, Jan Ivar Korsbakken, Glen P. Peters, Josep G. Canadell, Almut Arneth, Vivek K. Arora, Leticia Barbero, Ana Bastos, Laurent Bopp, Frédéric Chevallier, Louise P. Chini, Philippe Ciais, Scott C. Doney, Thanos Gkritzalis, Daniel S. Goll, Ian Harris, Vanessa Haverd, Forrest M. Hoffman, Mario Hoppema, Richard A. Houghton, George Hurtt, Tatiana Ilyina, Atul K. Jain, Truls Johannessen, Chris D. Jones, Etsushi Kato, Ralph F. Keeling, Kees Klein Goldewijk, Peter Landschützer, Nathalie Lefèvre, Sebastian Lienert, Zhu Liu, Danica Lombardozzi, Nicolas Metzl, David R. Munro, Julia E. M. S. Nabel, Shin-ichiro Nakaoka, Craig Neill, Are Olsen, Tsueno Ono, Prabir Patra, Anna Peregon, Wouter Peters, Philippe Peylin, Benjamin Pfeil, Denis Pierrot, Benjamin Poulter, Gregor Rehder, Laure Resplandy, Eddy Robertson, Matthias Rocher, Christian Rödenbeck, Ute Schuster, Jörg Schwinger, Roland Séférian, Ingunn Skjelvan, Tobias Steinhoff, Adrienne Sutton, Pieter P. Tans, Hanqin Tian, Bronte Tilbrook, Francesco N. Tubiello, Ingrid T. van der Laan-Luijkx, Guido R. van der Werf, Nicolas Viovy, Anthony P. Walker, Andrew J. Wiltshire, Rebecca Wright, Sönke Zaehle, and Bo Zheng
Earth Syst. Sci. Data, 10, 2141–2194, https://doi.org/10.5194/essd-10-2141-2018, https://doi.org/10.5194/essd-10-2141-2018, 2018
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The Global Carbon Budget 2018 describes the data sets and methodology used to quantify the emissions of carbon dioxide and their partitioning among the atmosphere, land, and ocean. These living data are updated every year to provide the highest transparency and traceability in the reporting of CO2, the key driver of climate change.
Haicheng Zhang, Daniel S. Goll, Stefano Manzoni, Philippe Ciais, Bertrand Guenet, and Yuanyuan Huang
Geosci. Model Dev., 11, 4779–4796, https://doi.org/10.5194/gmd-11-4779-2018, https://doi.org/10.5194/gmd-11-4779-2018, 2018
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Carbon use efficiency (CUE) of decomposers depends strongly on the organic matter quality (C : N ratio) and soil nutrient availability rather than a fixed value. A soil biogeochemical model with flexible CUE can better capture the differences in respiration rate of litter with contrasting C : N ratios and under different levels of mineral N availability than the model with fixed CUE, and well represent the effect of varying litter quality (N content) on SOM formation across temporal scales.
Marine Remaud, Frédéric Chevallier, Anne Cozic, Xin Lin, and Philippe Bousquet
Geosci. Model Dev., 11, 4489–4513, https://doi.org/10.5194/gmd-11-4489-2018, https://doi.org/10.5194/gmd-11-4489-2018, 2018
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We compare several versions of a global atmospheric transport model for the simulation of CO2. The representation of subgrid-scale processes modulates the interhemispheric gradient and the amplitude of the seasonal cycle in the Northern Hemisphere. It has the largest impact over Brazil. Refining the horizontal resolution improves the simulation near emission hotspots or along the coastlines. The sensitivities to the land surface model and to the increase in vertical resolution are marginal.
Zun Yin, Catherine Ottlé, Philippe Ciais, Matthieu Guimberteau, Xuhui Wang, Dan Zhu, Fabienne Maignan, Shushi Peng, Shilong Piao, Jan Polcher, Feng Zhou, Hyungjun Kim, and other China-Trend-Stream project members
Hydrol. Earth Syst. Sci., 22, 5463–5484, https://doi.org/10.5194/hess-22-5463-2018, https://doi.org/10.5194/hess-22-5463-2018, 2018
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Simulations in China were performed in ORCHIDEE driven by different forcing datasets: GSWP3, PGF, CRU-NCEP, and WFDEI. Simulated soil moisture was compared to several datasets to evaluate the ability of ORCHIDEE in reproducing soil moisture dynamics. Results showed that ORCHIDEE soil moisture coincided well with other datasets in wet areas and in non-irrigated areas. It suggested that the ORCHIDEE-MICT was suitable for further hydrological studies in China.
Igor B. Konovalov, Daria A. Lvova, Matthias Beekmann, Hiren Jethva, Eugene F. Mikhailov, Jean-Daniel Paris, Boris D. Belan, Valerii S. Kozlov, Philippe Ciais, and Meinrat O. Andreae
Atmos. Chem. Phys., 18, 14889–14924, https://doi.org/10.5194/acp-18-14889-2018, https://doi.org/10.5194/acp-18-14889-2018, 2018
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A good knowledge of black carbon (BC) emissions from open biomass burning (BB) is an important prerequisite for reliable climate predictions, especially in the Arctic. This paper introduces a method to constrain a regional budget of BB BC emissions using satellite measurements of the absorption and extinction optical depths and evaluates its potential application in a large Siberian region.
Minqiang Zhou, Bavo Langerock, Corinne Vigouroux, Mahesh Kumar Sha, Michel Ramonet, Marc Delmotte, Emmanuel Mahieu, Whitney Bader, Christian Hermans, Nicolas Kumps, Jean-Marc Metzger, Valentin Duflot, Zhiting Wang, Mathias Palm, and Martine De Mazière
Atmos. Chem. Phys., 18, 13881–13901, https://doi.org/10.5194/acp-18-13881-2018, https://doi.org/10.5194/acp-18-13881-2018, 2018
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This study focuses on atmospheric CO and CH4 time series and seasonal variations on Reunion Island based on in situ and FTIR measurements from two sites, Saint Denis and Maido. Ground-based in situ and FTIR (NDACC and TCCON) measurements are used to show their complementarity with regards to obtaining the CO and CH4 concentrations at the surface and in the troposphere and stratosphere. FLEXPART and GEOS-Chem models are applied to understand the seasonal variations of CO and CH4 at this site.
Yilong Wang, Philippe Ciais, Daniel Goll, Yuanyuan Huang, Yiqi Luo, Ying-Ping Wang, A. Anthony Bloom, Grégoire Broquet, Jens Hartmann, Shushi Peng, Josep Penuelas, Shilong Piao, Jordi Sardans, Benjamin D. Stocker, Rong Wang, Sönke Zaehle, and Sophie Zechmeister-Boltenstern
Geosci. Model Dev., 11, 3903–3928, https://doi.org/10.5194/gmd-11-3903-2018, https://doi.org/10.5194/gmd-11-3903-2018, 2018
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We present a new modeling framework called Global Observation-based Land-ecosystems Utilization Model of Carbon, Nitrogen and Phosphorus (GOLUM-CNP) that combines a data-constrained C-cycle analysis with data-driven estimates of N and P inputs and losses and with observed stoichiometric ratios. GOLUM-CNP provides a traceable tool, where a consistency between different datasets of global C, N, and P cycles has been achieved.
Cyrille Flamant, Adrien Deroubaix, Patrick Chazette, Joel Brito, Marco Gaetani, Peter Knippertz, Andreas H. Fink, Gaëlle de Coetlogon, Laurent Menut, Aurélie Colomb, Cyrielle Denjean, Rémi Meynadier, Philip Rosenberg, Regis Dupuy, Pamela Dominutti, Jonathan Duplissy, Thierry Bourrianne, Alfons Schwarzenboeck, Michel Ramonet, and Julien Totems
Atmos. Chem. Phys., 18, 12363–12389, https://doi.org/10.5194/acp-18-12363-2018, https://doi.org/10.5194/acp-18-12363-2018, 2018
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This work sheds light on the complex mechanisms by which coastal shallow circulations distribute atmospheric pollutants over the densely populated southern West African region. Pollutants of concern are anthropogenic emissions from coastal cities, as well as biomass burning aerosol and dust associated with long-range transport. The complex vertical distribution of aerosols over coastal southern West Africa is investigated using airborne observations and numerical simulations.
Chloé Largeron, Gerhard Krinner, Philippe Ciais, and Claire Brutel-Vuilmet
Geosci. Model Dev., 11, 3279–3297, https://doi.org/10.5194/gmd-11-3279-2018, https://doi.org/10.5194/gmd-11-3279-2018, 2018
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Peatlands are widely present in boreal regions and contain large carbon stocks due to their hydrologic properties and high water content. We have enhanced the global land surface model ORCHIDEE by introducing boreal peatlands. These are considered as a new type of vegetation in the model, with specific hydrological properties for peat soil. In this paper, we focus on the representation of the hydrology of northern peatlands and on the evaluation of the hydrological impact of this implementation.
Maarten Krol, Marco de Bruine, Lars Killaars, Huug Ouwersloot, Andrea Pozzer, Yi Yin, Frederic Chevallier, Philippe Bousquet, Prabir Patra, Dmitry Belikov, Shamil Maksyutov, Sandip Dhomse, Wuhu Feng, and Martyn P. Chipperfield
Geosci. Model Dev., 11, 3109–3130, https://doi.org/10.5194/gmd-11-3109-2018, https://doi.org/10.5194/gmd-11-3109-2018, 2018
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The TransCom inter-comparison project regularly carries out studies to quantify errors in simulated atmospheric transport. This paper presents the first results of an age of air (AoA) inter-comparison of six global transport models. Following a protocol, six models simulated five tracers from which atmospheric transport times can easily be deduced. Results highlight that inter-model differences associated with atmospheric transport are still large and require further analysis.
Victoria Naipal, Philippe Ciais, Yilong Wang, Ronny Lauerwald, Bertrand Guenet, and Kristof Van Oost
Biogeosciences, 15, 4459–4480, https://doi.org/10.5194/bg-15-4459-2018, https://doi.org/10.5194/bg-15-4459-2018, 2018
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We seek to better understand the links between soil erosion by rainfall and the global carbon (C) cycle by coupling a soil erosion model to the C cycle of a land surface model. With this modeling approach we evaluate the effects of soil removal on soil C stocks in the presence of climate change and land use change. We find that accelerated soil erosion leads to a potential SOC removal flux of 74 ±18 Pg of C globally over the period AD 1850–2005, with significant impacts on the land C balance.
Emilie Joetzjer, Fabienne Maignan, Jérôme Chave, Daniel Goll, Ben Poulter, Jonathan Barichivich, Isabelle Maréchaux, Sebastiaan Luyssaert, Matthieu Guimberteau, Kim Naudts, Damien Bonal, and Philippe Ciais
Biogeosciences Discuss., https://doi.org/10.5194/bg-2018-308, https://doi.org/10.5194/bg-2018-308, 2018
Revised manuscript not accepted
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This study explores the relative contributions of tree demographic, canopy structure and hydraulic processes on the Amazonian carbon and water cycles using large-scale process-based model. Our results imply that explicit coupling of the water and carbon cycles improves the representation of biogeochemical cycles and their spatial variability. Representing the variation in the ecological functioning of Amazonia should be the next step to improve the performance and predictive ability of models.
Xin Lin, Philippe Ciais, Philippe Bousquet, Michel Ramonet, Yi Yin, Yves Balkanski, Anne Cozic, Marc Delmotte, Nikolaos Evangeliou, Nuggehalli K. Indira, Robin Locatelli, Shushi Peng, Shilong Piao, Marielle Saunois, Panangady S. Swathi, Rong Wang, Camille Yver-Kwok, Yogesh K. Tiwari, and Lingxi Zhou
Atmos. Chem. Phys., 18, 9475–9497, https://doi.org/10.5194/acp-18-9475-2018, https://doi.org/10.5194/acp-18-9475-2018, 2018
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We simulate CH4 and CO2 using a zoomed global transport model with a horizontal resolution of ~50 km over South and East Asia, as well as a standard model version for comparison. Model performance is evaluated for both gases and versions at multiple timescales against a new collection of surface stations over this key GHG-emitting region. The evaluation at different timescales and comparisons between gases and model versions have implications for possible model improvements and inversions.
Wei Li, Chao Yue, Philippe Ciais, Jinfeng Chang, Daniel Goll, Dan Zhu, Shushi Peng, and Albert Jornet-Puig
Geosci. Model Dev., 11, 2249–2272, https://doi.org/10.5194/gmd-11-2249-2018, https://doi.org/10.5194/gmd-11-2249-2018, 2018
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We implemented four major lignocellulosic bioenergy crops in ORCHIDEE. We added new PFTs, did new parameterizations of photosynthesis, carbon allocation, and phenology based on a compilation of field measurements, and added a specific harvest module. The resulting ORCHIDEE-MICT-BIOENERGY model is evaluated at 296 locations where field measurements of harvested biomass are available, and the new model can generally reproduce the global bioenergy crop yield observations.
Donghai Wu, Philippe Ciais, Nicolas Viovy, Alan K. Knapp, Kevin Wilcox, Michael Bahn, Melinda D. Smith, Sara Vicca, Simone Fatichi, Jakob Zscheischler, Yue He, Xiangyi Li, Akihiko Ito, Almut Arneth, Anna Harper, Anna Ukkola, Athanasios Paschalis, Benjamin Poulter, Changhui Peng, Daniel Ricciuto, David Reinthaler, Guangsheng Chen, Hanqin Tian, Hélène Genet, Jiafu Mao, Johannes Ingrisch, Julia E. S. M. Nabel, Julia Pongratz, Lena R. Boysen, Markus Kautz, Michael Schmitt, Patrick Meir, Qiuan Zhu, Roland Hasibeder, Sebastian Sippel, Shree R. S. Dangal, Stephen Sitch, Xiaoying Shi, Yingping Wang, Yiqi Luo, Yongwen Liu, and Shilong Piao
Biogeosciences, 15, 3421–3437, https://doi.org/10.5194/bg-15-3421-2018, https://doi.org/10.5194/bg-15-3421-2018, 2018
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Our results indicate that most ecosystem models do not capture the observed asymmetric responses under normal precipitation conditions, suggesting an overestimate of the drought effects and/or underestimate of the watering impacts on primary productivity, which may be the result of inadequate representation of key eco-hydrological processes. Collaboration between modelers and site investigators needs to be strengthened to improve the specific processes in ecosystem models in following studies.
Ye Huang, Bertrand Guenet, Philippe Ciais, Ivan A. Janssens, Jennifer L. Soong, Yilong Wang, Daniel Goll, Evgenia Blagodatskaya, and Yuanyuan Huang
Geosci. Model Dev., 11, 2111–2138, https://doi.org/10.5194/gmd-11-2111-2018, https://doi.org/10.5194/gmd-11-2111-2018, 2018
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ORCHIMIC is a modeling effort trying to improve the representation of SOC dynamics in Earth system models (ESM). It has a structure that can be easily incorporated into CENTURY-based ESMs. In ORCHIMIC, key microbial dynamics (i.e., enzyme production, enzymatic decomposition and microbial dormancy) are included. The ORCHIMIC model can also reproduce the observed temporal dynamics of respiration and priming effects; thus it is an improved tool for climate projections and SOC response predictions.
Sourish Basu, David F. Baker, Frédéric Chevallier, Prabir K. Patra, Junjie Liu, and John B. Miller
Atmos. Chem. Phys., 18, 7189–7215, https://doi.org/10.5194/acp-18-7189-2018, https://doi.org/10.5194/acp-18-7189-2018, 2018
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CO2 measurements from the global surface network and CO2 estimates from satellites such as the Orbiting Carbon Observatory 2 (OCO-2) are currently used to quantify the surface sources and sinks of CO2, using what we know about atmospheric transport of gases. In this work, we quantify the uncertainties in those surface source/sink estimates that stem from errors in our atmospheric transport models, using an observing system simulation experiment (OSSE).
Yilong Wang, Grégoire Broquet, Philippe Ciais, Frédéric Chevallier, Felix Vogel, Lin Wu, Yi Yin, Rong Wang, and Shu Tao
Atmos. Chem. Phys., 18, 4229–4250, https://doi.org/10.5194/acp-18-4229-2018, https://doi.org/10.5194/acp-18-4229-2018, 2018
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This paper assesses the potential of atmospheric 14CO2 observations and a global inversion system to solve for fossil fuel CO2 (FFCO2) emissions in Europe. The estimate of monthly emission budgets is largely improved in high emitting regions. The results are sensitive to the observation network and the prior uncertainty. Using a high-resolution transport model and a systematic evaluation of the uncertainty in current emission inventories should improve the potential to retrieve FFCO2 emissions.
Abdelhadi El Yazidi, Michel Ramonet, Philippe Ciais, Gregoire Broquet, Isabelle Pison, Amara Abbaris, Dominik Brunner, Sebastien Conil, Marc Delmotte, Francois Gheusi, Frederic Guerin, Lynn Hazan, Nesrine Kachroudi, Giorgos Kouvarakis, Nikolaos Mihalopoulos, Leonard Rivier, and Dominique Serça
Atmos. Meas. Tech., 11, 1599–1614, https://doi.org/10.5194/amt-11-1599-2018, https://doi.org/10.5194/amt-11-1599-2018, 2018
Isabelle Pison, Antoine Berchet, Marielle Saunois, Philippe Bousquet, Grégoire Broquet, Sébastien Conil, Marc Delmotte, Anita Ganesan, Olivier Laurent, Damien Martin, Simon O'Doherty, Michel Ramonet, T. Gerard Spain, Alex Vermeulen, and Camille Yver Kwok
Atmos. Chem. Phys., 18, 3779–3798, https://doi.org/10.5194/acp-18-3779-2018, https://doi.org/10.5194/acp-18-3779-2018, 2018
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Methane emissions on the national scale in France in 2012 are inferred by assimilating continuous atmospheric mixing ratio measurements from nine stations of the European network ICOS. Two complementary inversion set-ups are computed and analysed: (i) a regional run correcting for the spatial distribution of fluxes in France and (ii) a sectorial run correcting fluxes for activity sectors on the national scale. The results are compared with existing inventories and other regional inversions.
Marta Camino-Serrano, Bertrand Guenet, Sebastiaan Luyssaert, Philippe Ciais, Vladislav Bastrikov, Bruno De Vos, Bert Gielen, Gerd Gleixner, Albert Jornet-Puig, Klaus Kaiser, Dolly Kothawala, Ronny Lauerwald, Josep Peñuelas, Marion Schrumpf, Sara Vicca, Nicolas Vuichard, David Walmsley, and Ivan A. Janssens
Geosci. Model Dev., 11, 937–957, https://doi.org/10.5194/gmd-11-937-2018, https://doi.org/10.5194/gmd-11-937-2018, 2018
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Global models generally oversimplify the representation of soil organic carbon (SOC), and thus its response to global warming remains uncertain. We present the new soil module ORCHIDEE-SOM, within the global model ORCHIDEE, that refines the representation of SOC dynamics and includes the dissolved organic carbon (DOC) processes. The model is able to reproduce SOC stocks and DOC concentrations in four different ecosystems, opening an opportunity for improved predictions of SOC in global models.
Corinne Le Quéré, Robbie M. Andrew, Pierre Friedlingstein, Stephen Sitch, Julia Pongratz, Andrew C. Manning, Jan Ivar Korsbakken, Glen P. Peters, Josep G. Canadell, Robert B. Jackson, Thomas A. Boden, Pieter P. Tans, Oliver D. Andrews, Vivek K. Arora, Dorothee C. E. Bakker, Leticia Barbero, Meike Becker, Richard A. Betts, Laurent Bopp, Frédéric Chevallier, Louise P. Chini, Philippe Ciais, Catherine E. Cosca, Jessica Cross, Kim Currie, Thomas Gasser, Ian Harris, Judith Hauck, Vanessa Haverd, Richard A. Houghton, Christopher W. Hunt, George Hurtt, Tatiana Ilyina, Atul K. Jain, Etsushi Kato, Markus Kautz, Ralph F. Keeling, Kees Klein Goldewijk, Arne Körtzinger, Peter Landschützer, Nathalie Lefèvre, Andrew Lenton, Sebastian Lienert, Ivan Lima, Danica Lombardozzi, Nicolas Metzl, Frank Millero, Pedro M. S. Monteiro, David R. Munro, Julia E. M. S. Nabel, Shin-ichiro Nakaoka, Yukihiro Nojiri, X. Antonio Padin, Anna Peregon, Benjamin Pfeil, Denis Pierrot, Benjamin Poulter, Gregor Rehder, Janet Reimer, Christian Rödenbeck, Jörg Schwinger, Roland Séférian, Ingunn Skjelvan, Benjamin D. Stocker, Hanqin Tian, Bronte Tilbrook, Francesco N. Tubiello, Ingrid T. van der Laan-Luijkx, Guido R. van der Werf, Steven van Heuven, Nicolas Viovy, Nicolas Vuichard, Anthony P. Walker, Andrew J. Watson, Andrew J. Wiltshire, Sönke Zaehle, and Dan Zhu
Earth Syst. Sci. Data, 10, 405–448, https://doi.org/10.5194/essd-10-405-2018, https://doi.org/10.5194/essd-10-405-2018, 2018
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The Global Carbon Budget 2017 describes data sets and methodology to quantify the five major components of the global carbon budget and their uncertainties. It is the 12th annual update and the 6th published in this journal.
Stephanie C. Pugliese, Jennifer G. Murphy, Felix R. Vogel, Michael D. Moran, Junhua Zhang, Qiong Zheng, Craig A. Stroud, Shuzhan Ren, Douglas Worthy, and Gregoire Broquet
Atmos. Chem. Phys., 18, 3387–3401, https://doi.org/10.5194/acp-18-3387-2018, https://doi.org/10.5194/acp-18-3387-2018, 2018
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We developed the Southern Ontario CO2 Emissions (SOCE) inventory, which identifies the spatial and temporal distribution (2.5 km and hourly, respectively) of CO2 emissions from seven source sectors. When the SOCE inventory was used with a chemistry transport model, we found strong agreement between modelled and measured mixing ratios. We were able to quantify that natural gas combustion contributes > 80 % of CO2 emissions at nighttime while on-road emissions contribute > 70 % during the day.
Irène Xueref-Remy, Elsa Dieudonné, Cyrille Vuillemin, Morgan Lopez, Christine Lac, Martina Schmidt, Marc Delmotte, Frédéric Chevallier, François Ravetta, Olivier Perrussel, Philippe Ciais, François-Marie Bréon, Grégoire Broquet, Michel Ramonet, T. Gerard Spain, and Christophe Ampe
Atmos. Chem. Phys., 18, 3335–3362, https://doi.org/10.5194/acp-18-3335-2018, https://doi.org/10.5194/acp-18-3335-2018, 2018
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Urbanized and industrialized areas are the largest source of fossil CO2. This work analyses the atmospheric CO2 variability observed from the first in situ network deployed in the Paris megacity area. Gradients of several ppm are found between the rural, peri-urban and urban sites at the diurnal to the seasonal scales. Wind direction and speed as well as boundary layer dynamics, correlated to highly variable urban emissions, are shown to be key regulator factors of the observed CO2 records.
Chao Yue, Philippe Ciais, and Wei Li
Biogeosciences, 15, 1185–1201, https://doi.org/10.5194/bg-15-1185-2018, https://doi.org/10.5194/bg-15-1185-2018, 2018
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Gross land use change such as shifting cultivation causes carbon emissions because carbon release in cleared forests is larger than absorption in regrowing ones. However, to appropriately account for this process, vegetation models have to represent sub-grid secondary forest dynamics. We found that gross land use emissions can be overestimated if sub-grid secondary forests are neglected in the model. Conversely, rotation lengths of shifting cultivation have a critical role.
Ben Parkes, Dimitri Defrance, Benjamin Sultan, Philippe Ciais, and Xuhui Wang
Earth Syst. Dynam., 9, 119–134, https://doi.org/10.5194/esd-9-119-2018, https://doi.org/10.5194/esd-9-119-2018, 2018
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We present an analysis of three crops in West Africa and their response to short-term climate change in a world where temperatures are 1.5 °C above the preindustrial levels. We show that the number of crop failures for all crops is due to increase in the future climate. We further show the difference in yield change across several West African countries and show that the yields are not expected to increase fast enough to prevent food shortages.
Grégoire Broquet, François-Marie Bréon, Emmanuel Renault, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, Frédéric Chevallier, Lin Wu, and Philippe Ciais
Atmos. Meas. Tech., 11, 681–708, https://doi.org/10.5194/amt-11-681-2018, https://doi.org/10.5194/amt-11-681-2018, 2018
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This study assesses the potential of space-borne imagery of CO2 atmospheric concentrations for monitoring the emissions from the Paris area. Such imagery could be provided by European and American missions in the next decade. It highlights the difficulty to improve current knowledge on CO2 emissions for urban areas with CO2 observations from satellites, and calls for more technological innovations in the remote sensing of CO2 and in the models that exploit it.
Chunjing Qiu, Dan Zhu, Philippe Ciais, Bertrand Guenet, Gerhard Krinner, Shushi Peng, Mika Aurela, Christian Bernhofer, Christian Brümmer, Syndonia Bret-Harte, Housen Chu, Jiquan Chen, Ankur R. Desai, Jiří Dušek, Eugénie S. Euskirchen, Krzysztof Fortuniak, Lawrence B. Flanagan, Thomas Friborg, Mateusz Grygoruk, Sébastien Gogo, Thomas Grünwald, Birger U. Hansen, David Holl, Elyn Humphreys, Miriam Hurkuck, Gerard Kiely, Janina Klatt, Lars Kutzbach, Chloé Largeron, Fatima Laggoun-Défarge, Magnus Lund, Peter M. Lafleur, Xuefei Li, Ivan Mammarella, Lutz Merbold, Mats B. Nilsson, Janusz Olejnik, Mikaell Ottosson-Löfvenius, Walter Oechel, Frans-Jan W. Parmentier, Matthias Peichl, Norbert Pirk, Olli Peltola, Włodzimierz Pawlak, Daniel Rasse, Janne Rinne, Gaius Shaver, Hans Peter Schmid, Matteo Sottocornola, Rainer Steinbrecher, Torsten Sachs, Marek Urbaniak, Donatella Zona, and Klaudia Ziemblinska
Geosci. Model Dev., 11, 497–519, https://doi.org/10.5194/gmd-11-497-2018, https://doi.org/10.5194/gmd-11-497-2018, 2018
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Northern peatlands store large amount of soil carbon and are vulnerable to climate change. We implemented peatland hydrological and carbon accumulation processes into the ORCHIDEE land surface model. The model was evaluated against EC measurements from 30 northern peatland sites. The model generally well reproduced the spatial gradient and temporal variations in GPP and NEE at these sites. Water table depth was not well predicted but had only small influence on simulated NEE.
Chao Yue, Philippe Ciais, Sebastiaan Luyssaert, Wei Li, Matthew J. McGrath, Jinfeng Chang, and Shushi Peng
Geosci. Model Dev., 11, 409–428, https://doi.org/10.5194/gmd-11-409-2018, https://doi.org/10.5194/gmd-11-409-2018, 2018
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Human alteration of land cover has caused CO2 that is stored in forest biomass and soil to be released into the atmosphere and thus contribute to global warming. Global vegetation models that are used to quantify such carbon emissions from land use change traditionally rarely include shifting cultivation and secondary forest age dynamics. In this study, we expanded one vegetation model to include these features. We found that carbon emissions from land use change are estimated to be smaller.
Wei Li, Natasha MacBean, Philippe Ciais, Pierre Defourny, Céline Lamarche, Sophie Bontemps, Richard A. Houghton, and Shushi Peng
Earth Syst. Sci. Data, 10, 219–234, https://doi.org/10.5194/essd-10-219-2018, https://doi.org/10.5194/essd-10-219-2018, 2018
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We evaluated the land cover changes based on plant functional types (PFTs) derived from the newly released annual ESA land cover maps. We addressed the geographical distributions and temporal trends of the translated PFT maps and compared with other datasets commonly used by the land surface model community. Different choices of these datasets for the applications in land surface models are proposed depending on the research purposes.
Peter Bergamaschi, Ute Karstens, Alistair J. Manning, Marielle Saunois, Aki Tsuruta, Antoine Berchet, Alexander T. Vermeulen, Tim Arnold, Greet Janssens-Maenhout, Samuel Hammer, Ingeborg Levin, Martina Schmidt, Michel Ramonet, Morgan Lopez, Jost Lavric, Tuula Aalto, Huilin Chen, Dietrich G. Feist, Christoph Gerbig, László Haszpra, Ove Hermansen, Giovanni Manca, John Moncrieff, Frank Meinhardt, Jaroslaw Necki, Michal Galkowski, Simon O'Doherty, Nina Paramonova, Hubertus A. Scheeren, Martin Steinbacher, and Ed Dlugokencky
Atmos. Chem. Phys., 18, 901–920, https://doi.org/10.5194/acp-18-901-2018, https://doi.org/10.5194/acp-18-901-2018, 2018
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European methane (CH4) emissions are estimated for 2006–2012 using atmospheric in situ measurements from 18 European monitoring stations and 7 different inverse models. Our analysis highlights the potential significant contribution of natural emissions from wetlands (including peatlands and wet soils) to the total European emissions. The top-down estimates of total EU-28 CH4 emissions are broadly consistent with the sum of reported anthropogenic CH4 emissions and the estimated natural emissions.
Matthieu Guimberteau, Dan Zhu, Fabienne Maignan, Ye Huang, Chao Yue, Sarah Dantec-Nédélec, Catherine Ottlé, Albert Jornet-Puig, Ana Bastos, Pierre Laurent, Daniel Goll, Simon Bowring, Jinfeng Chang, Bertrand Guenet, Marwa Tifafi, Shushi Peng, Gerhard Krinner, Agnès Ducharne, Fuxing Wang, Tao Wang, Xuhui Wang, Yilong Wang, Zun Yin, Ronny Lauerwald, Emilie Joetzjer, Chunjing Qiu, Hyungjun Kim, and Philippe Ciais
Geosci. Model Dev., 11, 121–163, https://doi.org/10.5194/gmd-11-121-2018, https://doi.org/10.5194/gmd-11-121-2018, 2018
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Improved projections of future Arctic and boreal ecosystem transformation require improved land surface models that integrate processes specific to these cold biomes. To this end, this study lays out relevant new parameterizations in the ORCHIDEE-MICT land surface model. These describe the interactions between soil carbon, soil temperature and hydrology, and their resulting feedbacks on water and CO2 fluxes, in addition to a recently developed fire module.
Fei Lun, Junguo Liu, Philippe Ciais, Thomas Nesme, Jinfeng Chang, Rong Wang, Daniel Goll, Jordi Sardans, Josep Peñuelas, and Michael Obersteiner
Earth Syst. Sci. Data, 10, 1–18, https://doi.org/10.5194/essd-10-1-2018, https://doi.org/10.5194/essd-10-1-2018, 2018
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We quantified in detail the P budgets in agricultural systems and PUE on global, regional, and national scales from 2002 to 2010. Globally, half of the total P inputs into agricultural systems accumulated in agricultural soils, with the rest lost to bodies of water. There are great differences in P budgets and PUE in agricultural systems on global, regional, and national scales. International trade played a significant role in P redistribution and P in fertilizer and food among countries.
Wei Li, Philippe Ciais, Chao Yue, Thomas Gasser, Shushi Peng, and Ana Bastos
Biogeosciences, 15, 91–103, https://doi.org/10.5194/bg-15-91-2018, https://doi.org/10.5194/bg-15-91-2018, 2018
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We compared the biomass recovery curves from a recent field-based study with those used in bookkeeping models and demonstrated the importance of considering gross forest changes rather than net forest changes. We also derived a critical gross-to-net forest area change ratio, beyond which the sign of carbon flux will be reversed. This critical ratio was further applied to the high-resolution satellite data in the Amazon to distinguish the sensitive regions.
Arsène Druel, Philippe Peylin, Gerhard Krinner, Philippe Ciais, Nicolas Viovy, Anna Peregon, Vladislav Bastrikov, Natalya Kosykh, and Nina Mironycheva-Tokareva
Geosci. Model Dev., 10, 4693–4722, https://doi.org/10.5194/gmd-10-4693-2017, https://doi.org/10.5194/gmd-10-4693-2017, 2017
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To improve the simulation of vegetation–climate feedbacks at high latitudes, three new circumpolar vegetation types were added in the ORCHIDEE land surface model: bryophytes (mosses) and lichens, Arctic shrubs, and Arctic grasses. This article is an introduction to the modification of vegetation distribution and physical behaviour, implying for example lower productivity, roughness, and higher winter albedo or freshwater discharge in the Arctic Ocean.
Sébastien Ars, Grégoire Broquet, Camille Yver Kwok, Yelva Roustan, Lin Wu, Emmanuel Arzoumanian, and Philippe Bousquet
Atmos. Meas. Tech., 10, 5017–5037, https://doi.org/10.5194/amt-10-5017-2017, https://doi.org/10.5194/amt-10-5017-2017, 2017
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This study presents a new concept for estimating the pollutant emission rates of a site combining the tracer release method, local-scale atmospheric transport modelling and a statistical atmospheric inversion approach. The potential of this new concept is evaluated with a practical implementation based on a series of inversions of controlled methane and tracer point sources in different spatial configurations to assess the efficiency of the method in comparison with the classic tracer method.
Katja Frieler, Stefan Lange, Franziska Piontek, Christopher P. O. Reyer, Jacob Schewe, Lila Warszawski, Fang Zhao, Louise Chini, Sebastien Denvil, Kerry Emanuel, Tobias Geiger, Kate Halladay, George Hurtt, Matthias Mengel, Daisuke Murakami, Sebastian Ostberg, Alexander Popp, Riccardo Riva, Miodrag Stevanovic, Tatsuo Suzuki, Jan Volkholz, Eleanor Burke, Philippe Ciais, Kristie Ebi, Tyler D. Eddy, Joshua Elliott, Eric Galbraith, Simon N. Gosling, Fred Hattermann, Thomas Hickler, Jochen Hinkel, Christian Hof, Veronika Huber, Jonas Jägermeyr, Valentina Krysanova, Rafael Marcé, Hannes Müller Schmied, Ioanna Mouratiadou, Don Pierson, Derek P. Tittensor, Robert Vautard, Michelle van Vliet, Matthias F. Biber, Richard A. Betts, Benjamin Leon Bodirsky, Delphine Deryng, Steve Frolking, Chris D. Jones, Heike K. Lotze, Hermann Lotze-Campen, Ritvik Sahajpal, Kirsten Thonicke, Hanqin Tian, and Yoshiki Yamagata
Geosci. Model Dev., 10, 4321–4345, https://doi.org/10.5194/gmd-10-4321-2017, https://doi.org/10.5194/gmd-10-4321-2017, 2017
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This paper describes the simulation scenario design for the next phase of the Inter-Sectoral Impact Model Intercomparison Project (ISIMIP), which is designed to facilitate a contribution to the scientific basis for the IPCC Special Report on the impacts of 1.5 °C global warming. ISIMIP brings together over 80 climate-impact models, covering impacts on hydrology, biomes, forests, heat-related mortality, permafrost, tropical cyclones, fisheries, agiculture, energy, and coastal infrastructure.
Chao Yue, Philippe Ciais, Ana Bastos, Frederic Chevallier, Yi Yin, Christian Rödenbeck, and Taejin Park
Atmos. Chem. Phys., 17, 13903–13919, https://doi.org/10.5194/acp-17-13903-2017, https://doi.org/10.5194/acp-17-13903-2017, 2017
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The year 2015 appeared as a paradox regarding how global carbon cycle has responded to climate variation: it is the greenest year since 2000 according to satellite observation, but the atmospheric CO2 growth rate is also the highest since 1959. We found that this is due to a only moderate land carbon sink, because high growing-season sink in northern lands has been partly offset by autumn and winter release and the late-year El Niño has led to an abrupt transition to land source in the tropics.
Wei Li, Philippe Ciais, Shushi Peng, Chao Yue, Yilong Wang, Martin Thurner, Sassan S. Saatchi, Almut Arneth, Valerio Avitabile, Nuno Carvalhais, Anna B. Harper, Etsushi Kato, Charles Koven, Yi Y. Liu, Julia E.M.S. Nabel, Yude Pan, Julia Pongratz, Benjamin Poulter, Thomas A. M. Pugh, Maurizio Santoro, Stephen Sitch, Benjamin D. Stocker, Nicolas Viovy, Andy Wiltshire, Rasoul Yousefpour, and Sönke Zaehle
Biogeosciences, 14, 5053–5067, https://doi.org/10.5194/bg-14-5053-2017, https://doi.org/10.5194/bg-14-5053-2017, 2017
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We used several observation-based biomass datasets to constrain the historical land-use change carbon emissions simulated by models. Compared to the range of the original modeled emissions (from 94 to 273 Pg C), the observationally constrained global cumulative emission estimate is 155 ± 50 Pg C (1σ Gaussian error) from 1901 to 2012. Our approach can also be applied to evaluate the LULCC impact of land-based climate mitigation policies.
Zhiting Wang, Thorsten Warneke, Nicholas M. Deutscher, Justus Notholt, Ute Karstens, Marielle Saunois, Matthias Schneider, Ralf Sussmann, Harjinder Sembhi, David W. T. Griffith, Dave F. Pollard, Rigel Kivi, Christof Petri, Voltaire A. Velazco, Michel Ramonet, and Huilin Chen
Atmos. Chem. Phys., 17, 13283–13295, https://doi.org/10.5194/acp-17-13283-2017, https://doi.org/10.5194/acp-17-13283-2017, 2017
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In this paper we separate the biases of atmospheric methane models into stratospheric and tropospheric parts. It is observed in other studies that simulated total columns of atmospheric methane present a latitudinal bias compared to measurements. The latitudinal gradients are considered to be from the stratosphere. However, our results show that the latitudinal biases could come from the troposphere in two of three models evaluated in this study.
Ronny Lauerwald, Pierre Regnier, Marta Camino-Serrano, Bertrand Guenet, Matthieu Guimberteau, Agnès Ducharne, Jan Polcher, and Philippe Ciais
Geosci. Model Dev., 10, 3821–3859, https://doi.org/10.5194/gmd-10-3821-2017, https://doi.org/10.5194/gmd-10-3821-2017, 2017
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ORCHILEAK is a new branch of the terrestrial ecosystem model ORCHIDEE that represents dissolved organic carbon (DOC) production from canopy and soils, DOC and CO2 leaching from soils to streams, DOC decomposition, and CO2 evasion to the atmosphere during its lateral transport in rivers, as well as exchange with the soil carbon and litter stocks on floodplains and in swamps. We parameterized and validated ORCHILEAK for the Amazon basin.
Daniel S. Goll, Nicolas Vuichard, Fabienne Maignan, Albert Jornet-Puig, Jordi Sardans, Aurelie Violette, Shushi Peng, Yan Sun, Marko Kvakic, Matthieu Guimberteau, Bertrand Guenet, Soenke Zaehle, Josep Penuelas, Ivan Janssens, and Philippe Ciais
Geosci. Model Dev., 10, 3745–3770, https://doi.org/10.5194/gmd-10-3745-2017, https://doi.org/10.5194/gmd-10-3745-2017, 2017
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We describe a representation of the terrestrial phosphorus cycle for the ORCHIDEE land surface model. The model is able to reproduce the observed shift from nitrogen to phosphorus limited net primary productivity along a soil formation chronosequence in Hawaii, as well as the contrasting responses of net primary productivity to nutrient addition. However, the simulated nutrient use efficiencies are lower, as observed primarily due to biases in the nutrient content and turnover of woody biomass.
Marielle Saunois, Philippe Bousquet, Ben Poulter, Anna Peregon, Philippe Ciais, Josep G. Canadell, Edward J. Dlugokencky, Giuseppe Etiope, David Bastviken, Sander Houweling, Greet Janssens-Maenhout, Francesco N. Tubiello, Simona Castaldi, Robert B. Jackson, Mihai Alexe, Vivek K. Arora, David J. Beerling, Peter Bergamaschi, Donald R. Blake, Gordon Brailsford, Lori Bruhwiler, Cyril Crevoisier, Patrick Crill, Kristofer Covey, Christian Frankenberg, Nicola Gedney, Lena Höglund-Isaksson, Misa Ishizawa, Akihiko Ito, Fortunat Joos, Heon-Sook Kim, Thomas Kleinen, Paul Krummel, Jean-François Lamarque, Ray Langenfelds, Robin Locatelli, Toshinobu Machida, Shamil Maksyutov, Joe R. Melton, Isamu Morino, Vaishali Naik, Simon O'Doherty, Frans-Jan W. Parmentier, Prabir K. Patra, Changhui Peng, Shushi Peng, Glen P. Peters, Isabelle Pison, Ronald Prinn, Michel Ramonet, William J. Riley, Makoto Saito, Monia Santini, Ronny Schroeder, Isobel J. Simpson, Renato Spahni, Atsushi Takizawa, Brett F. Thornton, Hanqin Tian, Yasunori Tohjima, Nicolas Viovy, Apostolos Voulgarakis, Ray Weiss, David J. Wilton, Andy Wiltshire, Doug Worthy, Debra Wunch, Xiyan Xu, Yukio Yoshida, Bowen Zhang, Zhen Zhang, and Qiuan Zhu
Atmos. Chem. Phys., 17, 11135–11161, https://doi.org/10.5194/acp-17-11135-2017, https://doi.org/10.5194/acp-17-11135-2017, 2017
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Following the Global Methane Budget 2000–2012 published in Saunois et al. (2016), we use the same dataset of bottom-up and top-down approaches to discuss the variations in methane emissions over the period 2000–2012. The changes in emissions are discussed both in terms of trends and quasi-decadal changes. The ensemble gathered here allows us to synthesise the robust changes in terms of regional and sectorial contributions to the increasing methane emissions.
Jakob Zscheischler, Miguel D. Mahecha, Valerio Avitabile, Leonardo Calle, Nuno Carvalhais, Philippe Ciais, Fabian Gans, Nicolas Gruber, Jens Hartmann, Martin Herold, Kazuhito Ichii, Martin Jung, Peter Landschützer, Goulven G. Laruelle, Ronny Lauerwald, Dario Papale, Philippe Peylin, Benjamin Poulter, Deepak Ray, Pierre Regnier, Christian Rödenbeck, Rosa M. Roman-Cuesta, Christopher Schwalm, Gianluca Tramontana, Alexandra Tyukavina, Riccardo Valentini, Guido van der Werf, Tristram O. West, Julie E. Wolf, and Markus Reichstein
Biogeosciences, 14, 3685–3703, https://doi.org/10.5194/bg-14-3685-2017, https://doi.org/10.5194/bg-14-3685-2017, 2017
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Here we synthesize a wide range of global spatiotemporal observational data on carbon exchanges between the Earth surface and the atmosphere. A key challenge was to consistently combining observational products of terrestrial and aquatic surfaces. Our primary goal is to identify today’s key uncertainties and observational shortcomings that would need to be addressed in future measurement campaigns or expansions of in situ observatories.
Thibaud Thonat, Marielle Saunois, Philippe Bousquet, Isabelle Pison, Zeli Tan, Qianlai Zhuang, Patrick M. Crill, Brett F. Thornton, David Bastviken, Ed J. Dlugokencky, Nikita Zimov, Tuomas Laurila, Juha Hatakka, Ove Hermansen, and Doug E. J. Worthy
Atmos. Chem. Phys., 17, 8371–8394, https://doi.org/10.5194/acp-17-8371-2017, https://doi.org/10.5194/acp-17-8371-2017, 2017
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Atmospheric methane simulations in the Arctic have been made for 2012 and compared to continuous observations at six measurement sites. All methane sources significantly affect the measurements at all stations, at least at the synoptic scale, except for biomass burning. An appropriate modelling framework combined with continuous observations of atmospheric methane enables us to gain knowledge on regional methane sources, including those which are usually poorly represented, such as freshwater.
Ana Bastos, Anna Peregon, Érico A. Gani, Sergey Khudyaev, Chao Yue, Wei Li, Célia Gouveia, and Philippe Ciais
Biogeosciences Discuss., https://doi.org/10.5194/bg-2017-267, https://doi.org/10.5194/bg-2017-267, 2017
Revised manuscript not accepted
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The ice-core record indicates a stabilization of atmospheric CO2 in the 1940s, which is not captured by the state-of-the-art reconstructions of CO2 sources and sinks.
The 1940s where marked by major socio-economic disruptions due to war. At the same time, very strong warming was registered in the high-latitudes. Here we evaluate the contributions of these two factors to a possible increase in the terrestrial sink not captured in other datasets, using the Former Soviet Union as a case study.
Eleanor J. Burke, Altug Ekici, Ye Huang, Sarah E. Chadburn, Chris Huntingford, Philippe Ciais, Pierre Friedlingstein, Shushi Peng, and Gerhard Krinner
Biogeosciences, 14, 3051–3066, https://doi.org/10.5194/bg-14-3051-2017, https://doi.org/10.5194/bg-14-3051-2017, 2017
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There are large reserves of carbon within the permafrost which might be released to the atmosphere under global warming. Our models suggest this release may cause an additional global temperature increase of 0.005 to 0.2°C by the year 2100 and 0.01 to 0.34°C by the year 2300. Under climate mitigation scenarios this is between 1.5 and 9 % (by 2100) and between 6 and 16 % (by 2300) of the global mean temperature change. There is a large uncertainty associated with these results.
Anna M. Michalak, Nina A. Randazzo, and Frédéric Chevallier
Atmos. Chem. Phys., 17, 7405–7421, https://doi.org/10.5194/acp-17-7405-2017, https://doi.org/10.5194/acp-17-7405-2017, 2017
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The use of inverse modeling for quantifying emissions of greenhouse gases is increasing. Estimates are very difficult to evaluate objectively, however, due to limited atmospheric observations and the lack of direct emissions measurements at compatible scales. Diagnostic tools have been proposed to partially circumvent these limitations. This paper presents the first systematic review of the scope and applicability of these tools for atmospheric inversions of long-lived greenhouse gases.
Jerónimo Escribano, Olivier Boucher, Frédéric Chevallier, and Nicolás Huneeus
Atmos. Chem. Phys., 17, 7111–7126, https://doi.org/10.5194/acp-17-7111-2017, https://doi.org/10.5194/acp-17-7111-2017, 2017
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Top-down estimates of mineral dust flux usually rely on a single observational dataset whose observational errors propagate onto the emission estimates. Aerosol optical depth from five satellites are assimilated one by one into a source inversion system over northern Africa. We find a relatively large dispersion in flux estimates among the five experiments, which can likely be attributed to differences in the assimilated observational datasets and their associated error statistics.
Sabina Assan, Alexia Baudic, Ali Guemri, Philippe Ciais, Valerie Gros, and Felix R. Vogel
Atmos. Meas. Tech., 10, 2077–2091, https://doi.org/10.5194/amt-10-2077-2017, https://doi.org/10.5194/amt-10-2077-2017, 2017
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This study is dedicated to improving measurement methods when using a Cavity Ring Down Spectroscopy instrument to measure methane at sites with elevated ethane concentrations such as Oil and Gas sites. The research was undertaken after measurements of natural gas samples suggested biased δ13CH4 results. Two instruments were extensively tested to characterize the cross sensitivities to ethane and δ13CH4 and propose corrections. Results indicate that it is imperative to account for the biases.
Daniel S. Goll, Alexander J. Winkler, Thomas Raddatz, Ning Dong, Ian Colin Prentice, Philippe Ciais, and Victor Brovkin
Geosci. Model Dev., 10, 2009–2030, https://doi.org/10.5194/gmd-10-2009-2017, https://doi.org/10.5194/gmd-10-2009-2017, 2017
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The response of soil organic carbon decomposition to warming and the interactions between nitrogen and carbon cycling affect the feedbacks between the land carbon cycle and the climate. In the model JSBACH carbon–nitrogen interactions have only a small effect on the feedbacks, whereas modifications of soil organic carbon decomposition have a large effect. The carbon cycle in the improved model is more resilient to climatic changes than in previous version of the model.
Thomas Gasser, Glen P. Peters, Jan S. Fuglestvedt, William J. Collins, Drew T. Shindell, and Philippe Ciais
Earth Syst. Dynam., 8, 235–253, https://doi.org/10.5194/esd-8-235-2017, https://doi.org/10.5194/esd-8-235-2017, 2017
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Emission metrics such as GWP or GTP are used to put non-CO2 species on a
CO2-equivalentscale. In the fifth IPCC report the metrics are inconsistent, as the climate–carbon feedback is included only for CO2 but not for non-CO2 species. Here, we simulate a new impulse response function for the feedback, and we use it to correct the metrics. For instance, 1 g of CH4 is equivalent to 31 g of CO2 (instead of 28 g) following the corrected GWP100 metric. It is 34 g if other factors are also updated.
Christoph Müller, Joshua Elliott, James Chryssanthacopoulos, Almut Arneth, Juraj Balkovic, Philippe Ciais, Delphine Deryng, Christian Folberth, Michael Glotter, Steven Hoek, Toshichika Iizumi, Roberto C. Izaurralde, Curtis Jones, Nikolay Khabarov, Peter Lawrence, Wenfeng Liu, Stefan Olin, Thomas A. M. Pugh, Deepak K. Ray, Ashwan Reddy, Cynthia Rosenzweig, Alex C. Ruane, Gen Sakurai, Erwin Schmid, Rastislav Skalsky, Carol X. Song, Xuhui Wang, Allard de Wit, and Hong Yang
Geosci. Model Dev., 10, 1403–1422, https://doi.org/10.5194/gmd-10-1403-2017, https://doi.org/10.5194/gmd-10-1403-2017, 2017
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Crop models are increasingly used in climate change impact research and integrated assessments. For the Agricultural Model Intercomparison and Improvement Project (AgMIP), 14 global gridded crop models (GGCMs) have supplied crop yield simulations (1980–2010) for maize, wheat, rice and soybean. We evaluate the performance of these models against observational data at global, national and grid cell level. We propose an open-access benchmark system against which future model versions can be tested.
Dominik Schmithüsen, Scott Chambers, Bernd Fischer, Stefan Gilge, Juha Hatakka, Victor Kazan, Rolf Neubert, Jussi Paatero, Michel Ramonet, Clemens Schlosser, Sabine Schmid, Alex Vermeulen, and Ingeborg Levin
Atmos. Meas. Tech., 10, 1299–1312, https://doi.org/10.5194/amt-10-1299-2017, https://doi.org/10.5194/amt-10-1299-2017, 2017
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A European-wide 222radon/222radon progeny comparison study has been conducted at nine measurement stations in order to determine differences between existing 222radon instrumentation and atmospheric data sets, respectively. Mean differences up to 45 % were found between monitors. These differences need to be taken into account if the data shall serve for quantitative regional atmospheric transport model validation.
Yi Yin, Frederic Chevallier, Philippe Ciais, Gregoire Broquet, Anne Cozic, Sophie Szopa, and Yilong Wang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-166, https://doi.org/10.5194/acp-2017-166, 2017
Revised manuscript not accepted
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CO inverse modelling studies have so far reported significant discrepancies between model concentrations optimised with the Measurement of Pollution in the Troposphere (MOPITT) satellite retrievals and surface in-situ measurements. Here, we assess how well a global CTM fits a large variety of independent CO observations before and after assimilating MOPITTv6 retrievals to optimise CO sources/sink and discuss potential sources of errors and their implications for global CO modelling studies.
Matthieu Guimberteau, Philippe Ciais, Agnès Ducharne, Juan Pablo Boisier, Ana Paula Dutra Aguiar, Hester Biemans, Hannes De Deurwaerder, David Galbraith, Bart Kruijt, Fanny Langerwisch, German Poveda, Anja Rammig, Daniel Andres Rodriguez, Graciela Tejada, Kirsten Thonicke, Celso Von Randow, Rita C. S. Von Randow, Ke Zhang, and Hans Verbeeck
Hydrol. Earth Syst. Sci., 21, 1455–1475, https://doi.org/10.5194/hess-21-1455-2017, https://doi.org/10.5194/hess-21-1455-2017, 2017
Clémence Rose, Karine Sellegri, Isabel Moreno, Fernando Velarde, Michel Ramonet, Kay Weinhold, Radovan Krejci, Marcos Andrade, Alfred Wiedensohler, Patrick Ginot, and Paolo Laj
Atmos. Chem. Phys., 17, 1529–1541, https://doi.org/10.5194/acp-17-1529-2017, https://doi.org/10.5194/acp-17-1529-2017, 2017
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Using an indirect method based on particle size distribution measurements, we show that new particle formation (NPF) is responsible for a large contribution to the cloud condensation nuclei concentration at the highest observatory in the world (Bolivia, 5240 m a.s.l.) as expected from some global model predictions. We also provide unique results related to the influence of the boundary layer on the NPF process, showing direct evidence for the important NPF frequency in the free troposphere.
Thomas Gasser, Philippe Ciais, Olivier Boucher, Yann Quilcaille, Maxime Tortora, Laurent Bopp, and Didier Hauglustaine
Geosci. Model Dev., 10, 271–319, https://doi.org/10.5194/gmd-10-271-2017, https://doi.org/10.5194/gmd-10-271-2017, 2017
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Simple models of the Earth system are useful, especially because of their high computing efficiency. This work describes the OSCAR model: a new simple Earth system model calibrated on state-of-the-art complex models. It will add to the pool of the few simple models currently used by the community, and it will therefore improve the robustness of future studies. Its source code is available upon request.
Sander Houweling, Peter Bergamaschi, Frederic Chevallier, Martin Heimann, Thomas Kaminski, Maarten Krol, Anna M. Michalak, and Prabir Patra
Atmos. Chem. Phys., 17, 235–256, https://doi.org/10.5194/acp-17-235-2017, https://doi.org/10.5194/acp-17-235-2017, 2017
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The aim of this paper is to present an overview of inverse modeling methods, developed over the years, for estimating the global sources and sinks of the greenhouse gas methane from atmospheric measurements. It provides insight into how techniques and estimates have evolved over time, what the remaining shortcomings are, new developments, and promising future directions.
Lamia Ammoura, Irène Xueref-Remy, Felix Vogel, Valérie Gros, Alexia Baudic, Bernard Bonsang, Marc Delmotte, Yao Té, and Frédéric Chevallier
Atmos. Chem. Phys., 16, 15653–15664, https://doi.org/10.5194/acp-16-15653-2016, https://doi.org/10.5194/acp-16-15653-2016, 2016
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We propose a new approach to estimate urban emission ratios that takes advantage of the enhanced local urban signal in the atmosphere at low wind speed. We apply it to estimate monthly ratios between CO2, CO and some VOCs from atmospheric measurement datasets acquired in the centre of Paris between 2010 and 2014. We find that this approach is little sensitive to the regional background level definition. With this new method, we may reveal spatial and seasonal variability in the ratios in Paris.
Christian Folberth, Joshua Elliott, Christoph Müller, Juraj Balkovic, James Chryssanthacopoulos, Roberto C. Izaurralde, Curtis D. Jones, Nikolay Khabarov, Wenfeng Liu, Ashwan Reddy, Erwin Schmid, Rastislav Skalský, Hong Yang, Almut Arneth, Philippe Ciais, Delphine Deryng, Peter J. Lawrence, Stefan Olin, Thomas A. M. Pugh, Alex C. Ruane, and Xuhui Wang
Biogeosciences Discuss., https://doi.org/10.5194/bg-2016-527, https://doi.org/10.5194/bg-2016-527, 2016
Manuscript not accepted for further review
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Global crop models differ in numerous aspects such as algorithms, parameterization, input data, and management assumptions. This study compares five global crop model frameworks, all based on the same field-scale model, to identify differences induced by the latter three. Results indicate that foremost nutrient supply, soil handling, and crop management induce substantial differences in crop yield estimates whereas crop cultivars primarily result in scaling of yield levels.
Marielle Saunois, Philippe Bousquet, Ben Poulter, Anna Peregon, Philippe Ciais, Josep G. Canadell, Edward J. Dlugokencky, Giuseppe Etiope, David Bastviken, Sander Houweling, Greet Janssens-Maenhout, Francesco N. Tubiello, Simona Castaldi, Robert B. Jackson, Mihai Alexe, Vivek K. Arora, David J. Beerling, Peter Bergamaschi, Donald R. Blake, Gordon Brailsford, Victor Brovkin, Lori Bruhwiler, Cyril Crevoisier, Patrick Crill, Kristofer Covey, Charles Curry, Christian Frankenberg, Nicola Gedney, Lena Höglund-Isaksson, Misa Ishizawa, Akihiko Ito, Fortunat Joos, Heon-Sook Kim, Thomas Kleinen, Paul Krummel, Jean-François Lamarque, Ray Langenfelds, Robin Locatelli, Toshinobu Machida, Shamil Maksyutov, Kyle C. McDonald, Julia Marshall, Joe R. Melton, Isamu Morino, Vaishali Naik, Simon O'Doherty, Frans-Jan W. Parmentier, Prabir K. Patra, Changhui Peng, Shushi Peng, Glen P. Peters, Isabelle Pison, Catherine Prigent, Ronald Prinn, Michel Ramonet, William J. Riley, Makoto Saito, Monia Santini, Ronny Schroeder, Isobel J. Simpson, Renato Spahni, Paul Steele, Atsushi Takizawa, Brett F. Thornton, Hanqin Tian, Yasunori Tohjima, Nicolas Viovy, Apostolos Voulgarakis, Michiel van Weele, Guido R. van der Werf, Ray Weiss, Christine Wiedinmyer, David J. Wilton, Andy Wiltshire, Doug Worthy, Debra Wunch, Xiyan Xu, Yukio Yoshida, Bowen Zhang, Zhen Zhang, and Qiuan Zhu
Earth Syst. Sci. Data, 8, 697–751, https://doi.org/10.5194/essd-8-697-2016, https://doi.org/10.5194/essd-8-697-2016, 2016
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An accurate assessment of the methane budget is important to understand the atmospheric methane concentrations and trends and to provide realistic pathways for climate change mitigation. The various and diffuse sources of methane as well and its oxidation by a very short lifetime radical challenge this assessment. We quantify the methane sources and sinks as well as their uncertainties based on both bottom-up and top-down approaches provided by a broad international scientific community.
Sauveur Belviso, Ilja Marco Reiter, Benjamin Loubet, Valérie Gros, Juliette Lathière, David Montagne, Marc Delmotte, Michel Ramonet, Cerise Kalogridis, Benjamin Lebegue, Nicolas Bonnaire, Victor Kazan, Thierry Gauquelin, Catherine Fernandez, and Bernard Genty
Atmos. Chem. Phys., 16, 14909–14923, https://doi.org/10.5194/acp-16-14909-2016, https://doi.org/10.5194/acp-16-14909-2016, 2016
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The role that soil, foliage, and atmospheric dynamics have on surface OCS exchange in a Mediterranean forest ecosystem in southern France (O3HP) was investigated in June of 2012 and 2013 with essentially a top-down approach. Atmospheric data suggest that the site is appropriate for estimating GPP directly from eddy covariance measurements of OCS fluxes, but it is less adequate for scaling NEE to GPP from observations of vertical gradients of OCS relative to CO2 during the daytime.
Johannes Staufer, Grégoire Broquet, François-Marie Bréon, Vincent Puygrenier, Frédéric Chevallier, Irène Xueref-Rémy, Elsa Dieudonné, Morgan Lopez, Martina Schmidt, Michel Ramonet, Olivier Perrussel, Christine Lac, Lin Wu, and Philippe Ciais
Atmos. Chem. Phys., 16, 14703–14726, https://doi.org/10.5194/acp-16-14703-2016, https://doi.org/10.5194/acp-16-14703-2016, 2016
Shushi Peng, Shilong Piao, Philippe Bousquet, Philippe Ciais, Bengang Li, Xin Lin, Shu Tao, Zhiping Wang, Yuan Zhang, and Feng Zhou
Atmos. Chem. Phys., 16, 14545–14562, https://doi.org/10.5194/acp-16-14545-2016, https://doi.org/10.5194/acp-16-14545-2016, 2016
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Methane is an important greenhouse gas, which accounts for about 20 % of the warming induced by long-lived greenhouse gases since 1750. Anthropogenic methane emissions from China may have been growing rapidly in the past decades because of increased coal mining and fast growing livestock. A good long-term methane emissions dataset is still lacking. Here, we produced a detailed bottom-up inventory of anthropogenic methane emissions from the eight major source sectors in China during 1980–2010.
Corinne Le Quéré, Robbie M. Andrew, Josep G. Canadell, Stephen Sitch, Jan Ivar Korsbakken, Glen P. Peters, Andrew C. Manning, Thomas A. Boden, Pieter P. Tans, Richard A. Houghton, Ralph F. Keeling, Simone Alin, Oliver D. Andrews, Peter Anthoni, Leticia Barbero, Laurent Bopp, Frédéric Chevallier, Louise P. Chini, Philippe Ciais, Kim Currie, Christine Delire, Scott C. Doney, Pierre Friedlingstein, Thanos Gkritzalis, Ian Harris, Judith Hauck, Vanessa Haverd, Mario Hoppema, Kees Klein Goldewijk, Atul K. Jain, Etsushi Kato, Arne Körtzinger, Peter Landschützer, Nathalie Lefèvre, Andrew Lenton, Sebastian Lienert, Danica Lombardozzi, Joe R. Melton, Nicolas Metzl, Frank Millero, Pedro M. S. Monteiro, David R. Munro, Julia E. M. S. Nabel, Shin-ichiro Nakaoka, Kevin O'Brien, Are Olsen, Abdirahman M. Omar, Tsuneo Ono, Denis Pierrot, Benjamin Poulter, Christian Rödenbeck, Joe Salisbury, Ute Schuster, Jörg Schwinger, Roland Séférian, Ingunn Skjelvan, Benjamin D. Stocker, Adrienne J. Sutton, Taro Takahashi, Hanqin Tian, Bronte Tilbrook, Ingrid T. van der Laan-Luijkx, Guido R. van der Werf, Nicolas Viovy, Anthony P. Walker, Andrew J. Wiltshire, and Sönke Zaehle
Earth Syst. Sci. Data, 8, 605–649, https://doi.org/10.5194/essd-8-605-2016, https://doi.org/10.5194/essd-8-605-2016, 2016
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The Global Carbon Budget 2016 is the 11th annual update of emissions of carbon dioxide (CO2) and their partitioning among the atmosphere, land, and ocean. This data synthesis brings together measurements, statistical information, and analyses of model results in order to provide an assessment of the global carbon budget and their uncertainties for years 1959 to 2015, with a projection for year 2016.
Igor B. Konovalov, Evgeny V. Berezin, Philippe Ciais, Grégoire Broquet, Ruslan V. Zhuravlev, and Greet Janssens-Maenhout
Atmos. Chem. Phys., 16, 13509–13540, https://doi.org/10.5194/acp-16-13509-2016, https://doi.org/10.5194/acp-16-13509-2016, 2016
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The knowledge of CO2 emissions from fossil-fuel (FF) burning is of paramount importance both for climate prediction and mitigation policy purposes. The paper introduces a method to indirectly constrain a regional budget of FF CO2 emissions by using satellite measurements of "proxy" chemical species and evaluates its potential in application to a western European region.
Marta Camino-Serrano, Elisabeth Graf Pannatier, Sara Vicca, Sebastiaan Luyssaert, Mathieu Jonard, Philippe Ciais, Bertrand Guenet, Bert Gielen, Josep Peñuelas, Jordi Sardans, Peter Waldner, Sophia Etzold, Guia Cecchini, Nicholas Clarke, Zoran Galić, Laure Gandois, Karin Hansen, Jim Johnson, Uwe Klinck, Zora Lachmanová, Antti-Jussi Lindroos, Henning Meesenburg, Tiina M. Nieminen, Tanja G. M. Sanders, Kasia Sawicka, Walter Seidling, Anne Thimonier, Elena Vanguelova, Arne Verstraeten, Lars Vesterdal, and Ivan A. Janssens
Biogeosciences, 13, 5567–5585, https://doi.org/10.5194/bg-13-5567-2016, https://doi.org/10.5194/bg-13-5567-2016, 2016
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We investigated the long-term trends of dissolved organic carbon (DOC) in soil solution and the drivers of changes in over 100 forest monitoring plots across Europe. An overall increasing trend was detected in the organic layers, but no overall trend was found in the mineral horizons. There are strong interactions between controls acting at local and regional scales. Our findings are relevant for researchers focusing on the link between terrestrial and aquatic ecosystems and for C-cycle models.
Natasha MacBean, Philippe Peylin, Frédéric Chevallier, Marko Scholze, and Gregor Schürmann
Geosci. Model Dev., 9, 3569–3588, https://doi.org/10.5194/gmd-9-3569-2016, https://doi.org/10.5194/gmd-9-3569-2016, 2016
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Model projections of the response of the terrestrial biosphere to anthropogenic emissions are uncertain, in part due to unknown fixed parameters in a model. Data assimilation can address this by using observations to optimise these parameter values. Using multiple types of data is beneficial for constraining different model processes, but it can also pose challenges in a DA context. This paper demonstrates and discusses the issues involved using toy models and examples from existing literature.
Lynn Hazan, Jérôme Tarniewicz, Michel Ramonet, Olivier Laurent, and Amara Abbaris
Atmos. Meas. Tech., 9, 4719–4736, https://doi.org/10.5194/amt-9-4719-2016, https://doi.org/10.5194/amt-9-4719-2016, 2016
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The ATC automatically processes atmospheric greenhouse gases mole fractions of data sent daily by the ICOS network, this includes calibration and water vapor corrections. Data are stored in a database which has been developed with an emphasis on traceability. Instrument calibration and manual quality control lead to automatic revaluation of the mole fractions calculated in near-real time. Calibration corrections avoid artificial gradients between sites that could lead to error in flux estimates.
Philippe Peylin, Cédric Bacour, Natasha MacBean, Sébastien Leonard, Peter Rayner, Sylvain Kuppel, Ernest Koffi, Abdou Kane, Fabienne Maignan, Frédéric Chevallier, Philippe Ciais, and Pascal Prunet
Geosci. Model Dev., 9, 3321–3346, https://doi.org/10.5194/gmd-9-3321-2016, https://doi.org/10.5194/gmd-9-3321-2016, 2016
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The study describes a carbon cycle data assimilation system that uses satellite observations of vegetation activity, net ecosystem exchange of carbon and water at many sites and atmospheric CO2 concentrations, in order to optimize the parameters of the ORCHIDEE land surface model. The optimized model is able to fit all three data streams leading to a land carbon uptake similar to independent estimates, which opens new perspectives for better prediction of the land carbon balance.
E. N. Koffi, P. Bergamaschi, U. Karstens, M. Krol, A. Segers, M. Schmidt, I. Levin, A. T. Vermeulen, R. E. Fisher, V. Kazan, H. Klein Baltink, D. Lowry, G. Manca, H. A. J. Meijer, J. Moncrieff, S. Pal, M. Ramonet, H. A. Scheeren, and A. G. Williams
Geosci. Model Dev., 9, 3137–3160, https://doi.org/10.5194/gmd-9-3137-2016, https://doi.org/10.5194/gmd-9-3137-2016, 2016
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We evaluate the capability of the TM5 model to reproduce observations of the boundary layer dynamics and the associated variability of trace gases close to the surface, using 222Rn. Focusing on the European scale, we compare the TM5 boundary layer heights with observations from radiosondes, lidar, and ceilometer. Furthermore, we compare TM5 simulations of 222Rn activity concentrations, using a novel, process-based 222Rn flux map over Europe, with 222Rn harmonized measurements from 10 stations.
Ana Bastos, Philippe Ciais, Jonathan Barichivich, Laurent Bopp, Victor Brovkin, Thomas Gasser, Shushi Peng, Julia Pongratz, Nicolas Viovy, and Cathy M. Trudinger
Biogeosciences, 13, 4877–4897, https://doi.org/10.5194/bg-13-4877-2016, https://doi.org/10.5194/bg-13-4877-2016, 2016
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The ice-core record shows a stabilisation of atmospheric CO2 in the 1940s, despite continued emissions from fossil fuel burning and land-use change (LUC). We use up-to-date reconstructions of the CO2 sources and sinks over the 20th century to evaluate whether these capture the CO2 plateau and to test the previously proposed hypothesis. Both strong terrestrial sink, possibly due to LUC not fully accounted for in the records, and enhanced oceanic uptake are necessary to explain this stall.
Anna Agustí-Panareda, Sébastien Massart, Frédéric Chevallier, Gianpaolo Balsamo, Souhail Boussetta, Emanuel Dutra, and Anton Beljaars
Atmos. Chem. Phys., 16, 10399–10418, https://doi.org/10.5194/acp-16-10399-2016, https://doi.org/10.5194/acp-16-10399-2016, 2016
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This paper presents a method to adjust the sinks and sources of CO2 associated with land ecosystems within a global atmospheric CO2 forecasting system in order to reduce the errors in the forecast. This is done by combining information on (1) retrospective fluxes estimated by a global flux inversion system, (2) land-use information, and (3) simulated fluxes from the model. Because the method is simple and flexible, it can easily run in real time as part of a forecasting system.
Wenli Wang, Annette Rinke, John C. Moore, Duoying Ji, Xuefeng Cui, Shushi Peng, David M. Lawrence, A. David McGuire, Eleanor J. Burke, Xiaodong Chen, Bertrand Decharme, Charles Koven, Andrew MacDougall, Kazuyuki Saito, Wenxin Zhang, Ramdane Alkama, Theodore J. Bohn, Philippe Ciais, Christine Delire, Isabelle Gouttevin, Tomohiro Hajima, Gerhard Krinner, Dennis P. Lettenmaier, Paul A. Miller, Benjamin Smith, Tetsuo Sueyoshi, and Artem B. Sherstiukov
The Cryosphere, 10, 1721–1737, https://doi.org/10.5194/tc-10-1721-2016, https://doi.org/10.5194/tc-10-1721-2016, 2016
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The winter snow insulation is a key process for air–soil temperature coupling and is relevant for permafrost simulations. Differences in simulated air–soil temperature relationships and their modulation by climate conditions are found to be related to the snow model physics. Generally, models with better performance apply multilayer snow schemes.
Cindy Cressot, Isabelle Pison, Peter J. Rayner, Philippe Bousquet, Audrey Fortems-Cheiney, and Frédéric Chevallier
Atmos. Chem. Phys., 16, 9089–9108, https://doi.org/10.5194/acp-16-9089-2016, https://doi.org/10.5194/acp-16-9089-2016, 2016
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Several hypothesis have been made to attribute current trends in atmospheric methane to particular regions. In this context, this work aims at evaluating how well anomalies in methane emissions can be detected at the regional scale with currently available observing systems: two space-borne instruments and a surface network. Our results show that inter-annual analyses of methane emissions inferred by atmospheric inversions should always include an uncertainty assessment.
Peter Rayner, Anna M. Michalak, and Frédéric Chevallier
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2016-148, https://doi.org/10.5194/gmd-2016-148, 2016
Revised manuscript not accepted
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Numerical models are among our most important tools for understanding and prediction. Models include quantities or equations that we cannot verify directly. We learn about these unknowns by comparing model output with observations and using some algorithm to improve the inputs. We show here that the many methods for doing this are special cases of underlying statistics. This provides a unified way of comparing and contrasting such methods.
Jinfeng Chang, Philippe Ciais, Mario Herrero, Petr Havlik, Matteo Campioli, Xianzhou Zhang, Yongfei Bai, Nicolas Viovy, Joanna Joiner, Xuhui Wang, Shushi Peng, Chao Yue, Shilong Piao, Tao Wang, Didier A. Hauglustaine, Jean-Francois Soussana, Anna Peregon, Natalya Kosykh, and Nina Mironycheva-Tokareva
Biogeosciences, 13, 3757–3776, https://doi.org/10.5194/bg-13-3757-2016, https://doi.org/10.5194/bg-13-3757-2016, 2016
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We derived the global maps of grassland management intensity of 1901–2012, including the minimum area of managed grassland with fraction of mown/grazed part. These maps, to our knowledge for the first time, provide global, time-dependent information for drawing up global estimates of management impact on biomass production and yields and for global vegetation models to enable simulations of carbon stocks and GHG budgets beyond simple tuning of grassland productivities to account for management.
Christian Frankenberg, Susan S. Kulawik, Steven C. Wofsy, Frédéric Chevallier, Bruce Daube, Eric A. Kort, Christopher O'Dell, Edward T. Olsen, and Gregory Osterman
Atmos. Chem. Phys., 16, 7867–7878, https://doi.org/10.5194/acp-16-7867-2016, https://doi.org/10.5194/acp-16-7867-2016, 2016
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We use observations from the HIAPER Pole-to-Pole Observations (HIPPO) flights from January 2009 through September 2011 to validate CO2 measurements from satellites (GOSAT, TES, AIRS) and atmospheric inversion models (CarbonTracker CT2013B, MACC v13r1).
Lin Wu, Grégoire Broquet, Philippe Ciais, Valentin Bellassen, Felix Vogel, Frédéric Chevallier, Irène Xueref-Remy, and Yilong Wang
Atmos. Chem. Phys., 16, 7743–7771, https://doi.org/10.5194/acp-16-7743-2016, https://doi.org/10.5194/acp-16-7743-2016, 2016
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This paper advances atmospheric inversion of city CO2 emissions as follows: (1) illustrate how inversion methodology can be tailored to deal with very large urban networks of sensors measuring CO2 concentrations; (2) demonstrate that atmospheric inversion could be a relevant tool of Monitoring, Reporting and Verification (MRV) of city CO2 emissions; (3) clarify the theoretical potential of inversion for reducing uncertainties in the estimates of citywide total and sectoral CO2 emissions.
Khatab Abdalla, Pauline Chivenge, Philippe Ciais, and Vincent Chaplot
Biogeosciences, 13, 3619–3633, https://doi.org/10.5194/bg-13-3619-2016, https://doi.org/10.5194/bg-13-3619-2016, 2016
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Discrepancies exist on the impact of tillage on soil CO2 emissions and on the main soil and environmental controls. Results from a meta-analysis using 174 paired observations comparing CO2 emissions over entire seasons or years from tilled (untilled) soils across different climates, crop types and soil conditions show that on average: (1) tilled soils emit 21 % more CO2 than untilled soils; (2) the difference increase to 29 % in sandy soils from arid climates with low soil organic carbon content.
Stijn Hantson, Almut Arneth, Sandy P. Harrison, Douglas I. Kelley, I. Colin Prentice, Sam S. Rabin, Sally Archibald, Florent Mouillot, Steve R. Arnold, Paulo Artaxo, Dominique Bachelet, Philippe Ciais, Matthew Forrest, Pierre Friedlingstein, Thomas Hickler, Jed O. Kaplan, Silvia Kloster, Wolfgang Knorr, Gitta Lasslop, Fang Li, Stephane Mangeon, Joe R. Melton, Andrea Meyn, Stephen Sitch, Allan Spessa, Guido R. van der Werf, Apostolos Voulgarakis, and Chao Yue
Biogeosciences, 13, 3359–3375, https://doi.org/10.5194/bg-13-3359-2016, https://doi.org/10.5194/bg-13-3359-2016, 2016
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Our ability to predict the magnitude and geographic pattern of past and future fire impacts rests on our ability to model fire regimes. A large variety of models exist, and it is unclear which type of model or degree of complexity is required to model fire adequately at regional to global scales. In this paper we summarize the current state of the art in fire-regime modelling and model evaluation, and outline what lessons may be learned from the Fire Model Intercomparison Project – FireMIP.
Sudhanshu Pandey, Sander Houweling, Maarten Krol, Ilse Aben, Frédéric Chevallier, Edward J. Dlugokencky, Luciana V. Gatti, Emanuel Gloor, John B. Miller, Rob Detmers, Toshinobu Machida, and Thomas Röckmann
Atmos. Chem. Phys., 16, 5043–5062, https://doi.org/10.5194/acp-16-5043-2016, https://doi.org/10.5194/acp-16-5043-2016, 2016
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This study investigates the constraint provided by measurements of Xratio (XCH4/XCO2) from space on surface fluxes of CH4 and CO2. We apply the ratio inversion method described in Pandey et al. (2015) to Xratio retrievals from the GOSAT with the TM5-4DVAR inverse modeling system, to constrain the surface fluxes of CH4 and CO2 for 2009 and 2010. The results are compared to proxy CH4 inversions using model-derived-XCO2 mixing ratios from CarbonTracker and MACC.
Antoine Berchet, Philippe Bousquet, Isabelle Pison, Robin Locatelli, Frédéric Chevallier, Jean-Daniel Paris, Ed J. Dlugokencky, Tuomas Laurila, Juha Hatakka, Yrjo Viisanen, Doug E. J. Worthy, Euan Nisbet, Rebecca Fisher, James France, David Lowry, Viktor Ivakhov, and Ove Hermansen
Atmos. Chem. Phys., 16, 4147–4157, https://doi.org/10.5194/acp-16-4147-2016, https://doi.org/10.5194/acp-16-4147-2016, 2016
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We propose insights based on atmospheric observations around the Arctic circle to evaluate estimates of methane emissions to the atmosphere from the East Siberian Arctic Shelf. Based on a comprehensive statistical analysis of the observations and of high-resolution transport simulations, annual methane emissions from ESAS are estimated to range from 0.0 to 4.5 TgCH4 yr−1, with a maximum in summer and very low emissions in winter.
Benjamin Lebegue, Martina Schmidt, Michel Ramonet, Benoit Wastine, Camille Yver Kwok, Olivier Laurent, Sauveur Belviso, Ali Guemri, Carole Philippon, Jeremiah Smith, and Sebastien Conil
Atmos. Meas. Tech., 9, 1221–1238, https://doi.org/10.5194/amt-9-1221-2016, https://doi.org/10.5194/amt-9-1221-2016, 2016
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In this study, we tested seven N2O analyzers from five different companies and compared the results with established techniques. The test protocols included the characterization of the short-term and long-term repeatability, drift, temperature dependence, linearity and sensitivity to water vapor. All of the analyzers showed a standard deviation better than 0.1 ppb for the 10-min averages. Some analyzers would benefit from improvements in temperature stability and water vapour correction.
X. Wu, N. Vuichard, P. Ciais, N. Viovy, N. de Noblet-Ducoudré, X. Wang, V. Magliulo, M. Wattenbach, L. Vitale, P. Di Tommasi, E. J. Moors, W. Jans, J. Elbers, E. Ceschia, T. Tallec, C. Bernhofer, T. Grünwald, C. Moureaux, T. Manise, A. Ligne, P. Cellier, B. Loubet, E. Larmanou, and D. Ripoche
Geosci. Model Dev., 9, 857–873, https://doi.org/10.5194/gmd-9-857-2016, https://doi.org/10.5194/gmd-9-857-2016, 2016
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The response of crops to changing climate and atmospheric CO2 could have large effects on food production, terrestrial carbon, water, energy fluxes and the climate feedbacks. We developed a new process-oriented terrestrial biogeochemical model named ORCHIDEE-CROP (v0), which integrates a generic crop phenology and harvest module into the land surface model ORCHIDEE. Our model has good ability to capture the spatial gradients of crop phenology, carbon and energy-related variables across Europe.
Bertrand Guenet, Fernando Esteban Moyano, Philippe Peylin, Philippe Ciais, and Ivan A Janssens
Geosci. Model Dev., 9, 841–855, https://doi.org/10.5194/gmd-9-841-2016, https://doi.org/10.5194/gmd-9-841-2016, 2016
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We present a simple conceptual model of soil carbon decomposition (PRIM) able to reproduce priming experiments. Parameters were optimized using a Bayesian framework and evaluated against another set of soil incubation. PRIM better fit data than the original, CENTURY-type soil decomposition model. We then compared both models incorporated into the global land biosphere model ORCHIDEE. Both versions reproduced observed decay litter rates, but only ORCHIDEE-PRIM could simulate the observed priming.
Susan Kulawik, Debra Wunch, Christopher O'Dell, Christian Frankenberg, Maximilian Reuter, Tomohiro Oda, Frederic Chevallier, Vanessa Sherlock, Michael Buchwitz, Greg Osterman, Charles E. Miller, Paul O. Wennberg, David Griffith, Isamu Morino, Manvendra K. Dubey, Nicholas M. Deutscher, Justus Notholt, Frank Hase, Thorsten Warneke, Ralf Sussmann, John Robinson, Kimberly Strong, Matthias Schneider, Martine De Mazière, Kei Shiomi, Dietrich G. Feist, Laura T. Iraci, and Joyce Wolf
Atmos. Meas. Tech., 9, 683–709, https://doi.org/10.5194/amt-9-683-2016, https://doi.org/10.5194/amt-9-683-2016, 2016
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To accurately estimate source and sink locations of carbon dioxide, systematic errors in satellite measurements and models must be characterized. This paper examines two satellite data sets (GOSAT, launched 2009, and SCIAMACHY, launched 2002), and two models (CarbonTracker and MACC) vs. the TCCON CO2 validation data set. We assess biases and errors by season and latitude, satellite performance under averaging, and diurnal variability. Our findings are useful for assimilation of satellite data.
Sébastien Massart, Anna Agustí-Panareda, Jens Heymann, Michael Buchwitz, Frédéric Chevallier, Maximilian Reuter, Michael Hilker, John P. Burrows, Nicholas M. Deutscher, Dietrich G. Feist, Frank Hase, Ralf Sussmann, Filip Desmet, Manvendra K. Dubey, David W. T. Griffith, Rigel Kivi, Christof Petri, Matthias Schneider, and Voltaire A. Velazco
Atmos. Chem. Phys., 16, 1653–1671, https://doi.org/10.5194/acp-16-1653-2016, https://doi.org/10.5194/acp-16-1653-2016, 2016
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This study presents the European Centre for Medium-Range Weather Forecasts (ECMWF) monitoring of atmospheric CO2 using measurements from the Greenhouse gases Observing Satellite (GOSAT). We show that the modelled CO2 has a better precision than standard CO2 satellite products compared to ground-based measurements. We also present the CO2 forecast based on our best knowledge of the atmospheric CO2 distribution. We show that it has skill to forecast the largest scale CO2 patterns up to day 5.
C. Yue, P. Ciais, D. Zhu, T. Wang, S. S. Peng, and S. L. Piao
Biogeosciences, 13, 675–690, https://doi.org/10.5194/bg-13-675-2016, https://doi.org/10.5194/bg-13-675-2016, 2016
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The pan-boreal biome (> N45°) removes CO2 from the atmosphere (i.e., it is a carbon sink). Fires can alter this carbon balance because they release CO2 to the atmosphere but also initiate a long-term carbon sink during post-fire vegetation recovery. We found that historical fires of 1850–2009 have a small net sink contribution (~6 %) to the 2000–2009 regional carbon sink, which is a balance between immediate source effect of fires in 2000–2009 and sink effects of those in 1850–1999.
S. Peng, P. Ciais, G. Krinner, T. Wang, I. Gouttevin, A. D. McGuire, D. Lawrence, E. Burke, X. Chen, B. Decharme, C. Koven, A. MacDougall, A. Rinke, K. Saito, W. Zhang, R. Alkama, T. J. Bohn, C. Delire, T. Hajima, D. Ji, D. P. Lettenmaier, P. A. Miller, J. C. Moore, B. Smith, and T. Sueyoshi
The Cryosphere, 10, 179–192, https://doi.org/10.5194/tc-10-179-2016, https://doi.org/10.5194/tc-10-179-2016, 2016
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Soil temperature change is a key indicator of the dynamics of permafrost. Using nine process-based ecosystem models with permafrost processes, a large spread of soil temperature trends across the models. Air temperature and longwave downward radiation are the main drivers of soil temperature trends. Based on an emerging observation constraint method, the total boreal near-surface permafrost area decrease comprised between 39 ± 14 × 103 and 75 ± 14 × 103 km2 yr−1 from 1960 to 2000.
P. Kountouris, C. Gerbig, K.-U. Totsche, A. J. Dolman, A. G. C. A. Meesters, G. Broquet, F. Maignan, B. Gioli, L. Montagnani, and C. Helfter
Biogeosciences, 12, 7403–7421, https://doi.org/10.5194/bg-12-7403-2015, https://doi.org/10.5194/bg-12-7403-2015, 2015
N. MacBean, F. Maignan, P. Peylin, C. Bacour, F.-M. Bréon, and P. Ciais
Biogeosciences, 12, 7185–7208, https://doi.org/10.5194/bg-12-7185-2015, https://doi.org/10.5194/bg-12-7185-2015, 2015
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Previous model evaluation studies have shown that terrestrial biosphere models (TBMs) need a better representation of the leaf phenology, but the model deficiency could be related to incorrect model parameters or inaccurate model structure. This paper presents a framework for optimising the parameters of phenology models that are commonly used in TBMs. It further demonstrates that the optimisation can result in changes to trends in vegetation productivity and an improvement in gross C fluxes.
Y. Yin, F. Chevallier, P. Ciais, G. Broquet, A. Fortems-Cheiney, I. Pison, and M. Saunois
Atmos. Chem. Phys., 15, 13433–13451, https://doi.org/10.5194/acp-15-13433-2015, https://doi.org/10.5194/acp-15-13433-2015, 2015
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We studied the global CO concentration decline over the recent decade with a sophisticated atmospheric inversion system assimilating MOPITT CO retrievals, surface methane and surface methyl chloroform in situ measurements. The inversion interprets the CO concentration decline as a 23% decrease in the CO emissions from 2002 to 2011, twice the negative trend estimated by emission inventories. In contrast to bottom-up inventories, we find negative trends over China and South-east Asia.
C. Le Quéré, R. Moriarty, R. M. Andrew, J. G. Canadell, S. Sitch, J. I. Korsbakken, P. Friedlingstein, G. P. Peters, R. J. Andres, T. A. Boden, R. A. Houghton, J. I. House, R. F. Keeling, P. Tans, A. Arneth, D. C. E. Bakker, L. Barbero, L. Bopp, J. Chang, F. Chevallier, L. P. Chini, P. Ciais, M. Fader, R. A. Feely, T. Gkritzalis, I. Harris, J. Hauck, T. Ilyina, A. K. Jain, E. Kato, V. Kitidis, K. Klein Goldewijk, C. Koven, P. Landschützer, S. K. Lauvset, N. Lefèvre, A. Lenton, I. D. Lima, N. Metzl, F. Millero, D. R. Munro, A. Murata, J. E. M. S. Nabel, S. Nakaoka, Y. Nojiri, K. O'Brien, A. Olsen, T. Ono, F. F. Pérez, B. Pfeil, D. Pierrot, B. Poulter, G. Rehder, C. Rödenbeck, S. Saito, U. Schuster, J. Schwinger, R. Séférian, T. Steinhoff, B. D. Stocker, A. J. Sutton, T. Takahashi, B. Tilbrook, I. T. van der Laan-Luijkx, G. R. van der Werf, S. van Heuven, D. Vandemark, N. Viovy, A. Wiltshire, S. Zaehle, and N. Zeng
Earth Syst. Sci. Data, 7, 349–396, https://doi.org/10.5194/essd-7-349-2015, https://doi.org/10.5194/essd-7-349-2015, 2015
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Accurate assessment of anthropogenic carbon dioxide emissions and their redistribution among the atmosphere, ocean, and terrestrial biosphere is important to understand the global carbon cycle, support the development of climate policies, and project future climate change. We describe data sets and a methodology to quantify all major components of the global carbon budget, including their uncertainties, based on a range of data and models and their interpretation by a broad scientific community.
H. Lindqvist, C. W. O'Dell, S. Basu, H. Boesch, F. Chevallier, N. Deutscher, L. Feng, B. Fisher, F. Hase, M. Inoue, R. Kivi, I. Morino, P. I. Palmer, R. Parker, M. Schneider, R. Sussmann, and Y. Yoshida
Atmos. Chem. Phys., 15, 13023–13040, https://doi.org/10.5194/acp-15-13023-2015, https://doi.org/10.5194/acp-15-13023-2015, 2015
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Atmospheric carbon dioxide concentration varies seasonally mainly due to plant photosynthesis in the Northern Hemisphere. We found that the satellite GOSAT can capture this variability from space to within 1ppm. We also found that models can differ by more than 1ppm. This implies that the satellite measurements could be useful in evaluating models and their prior estimates of carbon dioxide sources and sinks.
N. Kadygrov, G. Broquet, F. Chevallier, L. Rivier, C. Gerbig, and P. Ciais
Atmos. Chem. Phys., 15, 12765–12787, https://doi.org/10.5194/acp-15-12765-2015, https://doi.org/10.5194/acp-15-12765-2015, 2015
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We study the potential of the European Integrated Carbon Observing System (ICOS) atmospheric network for estimating European CO2 ecosystem fluxes. Regional atmospheric inversions with synthetic data are used to derive it in terms of statistical uncertainty. This potential is high in western Europe and future extensions of the network will increase it in eastern Europe. Future improvements of the models underlying the inversion should also significantly decrease uncertainties at high resolution.
R. J. Parker, H. Boesch, K. Byckling, A. J. Webb, P. I. Palmer, L. Feng, P. Bergamaschi, F. Chevallier, J. Notholt, N. Deutscher, T. Warneke, F. Hase, R. Sussmann, S. Kawakami, R. Kivi, D. W. T. Griffith, and V. Velazco
Atmos. Meas. Tech., 8, 4785–4801, https://doi.org/10.5194/amt-8-4785-2015, https://doi.org/10.5194/amt-8-4785-2015, 2015
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Atmospheric CH4 is an important greenhouse gas. Long-term global observations are necessary to understand its behaviour, with satellite observations playing a key role. The "proxy" retrieval method is one of the most successful but relies on the contribution from atmospheric CO2 models. This work assesses the significance of the uncertainty from the model CO2 within the retrieval and determines that despite this uncertainty the data are still valuable for determining sources and sinks of CH4.
F. Chevallier
Atmos. Chem. Phys., 15, 11133–11145, https://doi.org/10.5194/acp-15-11133-2015, https://doi.org/10.5194/acp-15-11133-2015, 2015
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We demonstrate that the current two-step approach to infer the CO2 surface fluxes from satellite measured radiances, with CO2 retrievals as an intermediate product, is not optimal. This suboptimality corrupts the 4D information flow from the radiance measurements to the surface flux estimates. It is amplified by current retrieval strategies where prior errors are much larger than the performance of prior CO2 simulations used in atmospheric inversions.
M. Lopez, M. Schmidt, M. Ramonet, J.-L. Bonne, A. Colomb, V. Kazan, P. Laj, and J.-M. Pichon
Atmos. Meas. Tech., 8, 3941–3958, https://doi.org/10.5194/amt-8-3941-2015, https://doi.org/10.5194/amt-8-3941-2015, 2015
C. Yver Kwok, O. Laurent, A. Guemri, C. Philippon, B. Wastine, C. W. Rella, C. Vuillemin, F. Truong, M. Delmotte, V. Kazan, M. Darding, B. Lebègue, C. Kaiser, I. Xueref-Rémy, and M. Ramonet
Atmos. Meas. Tech., 8, 3867–3892, https://doi.org/10.5194/amt-8-3867-2015, https://doi.org/10.5194/amt-8-3867-2015, 2015
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We present the results of tests of CRDS instruments in the laboratory (47 instruments) and in the field (15 instruments). We demonstrate that, thanks to rigorous testing, newer models generally perform better than older models, especially in terms of reproducibility between instruments. In the field, we see the importance of individual diagnostics during the installation phase, and we show the value of calibration and target gases that assess the quality of the data.
A. Berchet, I. Pison, F. Chevallier, J.-D. Paris, P. Bousquet, J.-L. Bonne, M. Y. Arshinov, B. D. Belan, C. Cressot, D. K. Davydov, E. J. Dlugokencky, A. V. Fofonov, A. Galanin, J. Lavrič, T. Machida, R. Parker, M. Sasakawa, R. Spahni, B. D. Stocker, and J. Winderlich
Biogeosciences, 12, 5393–5414, https://doi.org/10.5194/bg-12-5393-2015, https://doi.org/10.5194/bg-12-5393-2015, 2015
R. Locatelli, P. Bousquet, M. Saunois, F. Chevallier, and C. Cressot
Atmos. Chem. Phys., 15, 9765–9780, https://doi.org/10.5194/acp-15-9765-2015, https://doi.org/10.5194/acp-15-9765-2015, 2015
X. Lin, N. K. Indira, M. Ramonet, M. Delmotte, P. Ciais, B. C. Bhatt, M. V. Reddy, D. Angchuk, S. Balakrishnan, S. Jorphail, T. Dorjai, T. T. Mahey, S. Patnaik, M. Begum, C. Brenninkmeijer, S. Durairaj, R. Kirubagaran, M. Schmidt, P. S. Swathi, N. V. Vinithkumar, C. Yver Kwok, and V. K. Gaur
Atmos. Chem. Phys., 15, 9819–9849, https://doi.org/10.5194/acp-15-9819-2015, https://doi.org/10.5194/acp-15-9819-2015, 2015
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We present 5-year flask measurements (2007–2011) of greenhouse gases (GHGs) at three atmospheric stations in India. The results suggest significant sources of CO2, CH4, N2O, CO, and H2 over S and NE India, while SF6 sources are weak. The seasonal cycles for each species reflect the seasonality of sources/sinks and influences of the Indian monsoon circulations. The data show potential to infer regional patterns of GHG fluxes and atmospheric transport over this under-documented region.
A. I. Stegehuis, R. Vautard, P. Ciais, A. J. Teuling, D. G. Miralles, and M. Wild
Geosci. Model Dev., 8, 2285–2298, https://doi.org/10.5194/gmd-8-2285-2015, https://doi.org/10.5194/gmd-8-2285-2015, 2015
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Many climate models have difficulties in properly reproducing climate extremes such as heat wave conditions. We use a regional climate model with different atmospheric physics schemes to simulate the heat wave events of 2003 in western Europe and 2010 in Russia. The five best-performing and diverse physics scheme combinations may be used in the future to perform heat wave analysis and to investigate the impact of climate change in summer in Europe.
L. Molina, G. Broquet, P. Imbach, F. Chevallier, B. Poulter, D. Bonal, B. Burban, M. Ramonet, L. V. Gatti, S. C. Wofsy, J. W. Munger, E. Dlugokencky, and P. Ciais
Atmos. Chem. Phys., 15, 8423–8438, https://doi.org/10.5194/acp-15-8423-2015, https://doi.org/10.5194/acp-15-8423-2015, 2015
D. Zhu, S. S. Peng, P. Ciais, N. Viovy, A. Druel, M. Kageyama, G. Krinner, P. Peylin, C. Ottlé, S. L. Piao, B. Poulter, D. Schepaschenko, and A. Shvidenko
Geosci. Model Dev., 8, 2263–2283, https://doi.org/10.5194/gmd-8-2263-2015, https://doi.org/10.5194/gmd-8-2263-2015, 2015
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This study presents a new parameterization of the vegetation dynamics module in the process-based ecosystem model ORCHIDEE for mid- to high-latitude regions, showing significant improvements in the modeled distribution of tree functional types north of 40°N. A new set of metrics is proposed to quantify the performance of ORCHIDEE, which integrates uncertainties in the observational data sets.
C. E. Yver Kwok, D. Müller, C. Caldow, B. Lebègue, J. G. Mønster, C. W. Rella, C. Scheutz, M. Schmidt, M. Ramonet, T. Warneke, G. Broquet, and P. Ciais
Atmos. Meas. Tech., 8, 2853–2867, https://doi.org/10.5194/amt-8-2853-2015, https://doi.org/10.5194/amt-8-2853-2015, 2015
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This study presents two methods for estimating methane emissions from a waste water treatment plant (WWTP) along with results from a measurement campaign at a WWTP in Valence, France. We show that the tracer release method is suitable to quantify facility emissions, while the chamber measurements, provide insights into individual processes. We confirm that the open basins are not a major source of CH4 on the WWTP but that the pretreatment and sludge treatment are the main emitters.
K. Frieler, A. Levermann, J. Elliott, J. Heinke, A. Arneth, M. F. P. Bierkens, P. Ciais, D. B. Clark, D. Deryng, P. Döll, P. Falloon, B. Fekete, C. Folberth, A. D. Friend, C. Gellhorn, S. N. Gosling, I. Haddeland, N. Khabarov, M. Lomas, Y. Masaki, K. Nishina, K. Neumann, T. Oki, R. Pavlick, A. C. Ruane, E. Schmid, C. Schmitz, T. Stacke, E. Stehfest, Q. Tang, D. Wisser, V. Huber, F. Piontek, L. Warszawski, J. Schewe, H. Lotze-Campen, and H. J. Schellnhuber
Earth Syst. Dynam., 6, 447–460, https://doi.org/10.5194/esd-6-447-2015, https://doi.org/10.5194/esd-6-447-2015, 2015
K. Nishina, A. Ito, P. Falloon, A. D. Friend, D. J. Beerling, P. Ciais, D. B. Clark, R. Kahana, E. Kato, W. Lucht, M. Lomas, R. Pavlick, S. Schaphoff, L. Warszawaski, and T. Yokohata
Earth Syst. Dynam., 6, 435–445, https://doi.org/10.5194/esd-6-435-2015, https://doi.org/10.5194/esd-6-435-2015, 2015
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Our study focused on uncertainties in terrestrial C cycling under newly developed scenarios with CMIP5. This study presents first results for examining relative uncertainties of projected terrestrial C cycling in multiple projection components. Only using our new model inter-comparison project data sets enables us to evaluate various uncertainty sources in projection periods. The information on relative uncertainties is useful for climate science and climate change impact evaluation.
E. Joetzjer, C. Delire, H. Douville, P. Ciais, B. Decharme, D. Carrer, H. Verbeeck, M. De Weirdt, and D. Bonal
Geosci. Model Dev., 8, 1709–1727, https://doi.org/10.5194/gmd-8-1709-2015, https://doi.org/10.5194/gmd-8-1709-2015, 2015
R. Wang, Y. Balkanski, O. Boucher, L. Bopp, A. Chappell, P. Ciais, D. Hauglustaine, J. Peñuelas, and S. Tao
Atmos. Chem. Phys., 15, 6247–6270, https://doi.org/10.5194/acp-15-6247-2015, https://doi.org/10.5194/acp-15-6247-2015, 2015
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This study makes a first attempt to estimate the temporal trend of Fe emissions from anthropogenic and natural combustion sources from 1960 to 2007 and the emissions of Fe from mineral dust based on a recent mineralogical database. The new emission inventory is introduced into a global aerosol model. The simulated total Fe and soluble Fe concentrations in surface air as well as the deposition of total Fe are evaluated by observations over major continental and oceanic regions globally.
A. Berchet, I. Pison, F. Chevallier, P. Bousquet, J.-L. Bonne, and J.-D. Paris
Geosci. Model Dev., 8, 1525–1546, https://doi.org/10.5194/gmd-8-1525-2015, https://doi.org/10.5194/gmd-8-1525-2015, 2015
C. Le Quéré, R. Moriarty, R. M. Andrew, G. P. Peters, P. Ciais, P. Friedlingstein, S. D. Jones, S. Sitch, P. Tans, A. Arneth, T. A. Boden, L. Bopp, Y. Bozec, J. G. Canadell, L. P. Chini, F. Chevallier, C. E. Cosca, I. Harris, M. Hoppema, R. A. Houghton, J. I. House, A. K. Jain, T. Johannessen, E. Kato, R. F. Keeling, V. Kitidis, K. Klein Goldewijk, C. Koven, C. S. Landa, P. Landschützer, A. Lenton, I. D. Lima, G. Marland, J. T. Mathis, N. Metzl, Y. Nojiri, A. Olsen, T. Ono, S. Peng, W. Peters, B. Pfeil, B. Poulter, M. R. Raupach, P. Regnier, C. Rödenbeck, S. Saito, J. E. Salisbury, U. Schuster, J. Schwinger, R. Séférian, J. Segschneider, T. Steinhoff, B. D. Stocker, A. J. Sutton, T. Takahashi, B. Tilbrook, G. R. van der Werf, N. Viovy, Y.-P. Wang, R. Wanninkhof, A. Wiltshire, and N. Zeng
Earth Syst. Sci. Data, 7, 47–85, https://doi.org/10.5194/essd-7-47-2015, https://doi.org/10.5194/essd-7-47-2015, 2015
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Carbon dioxide (CO2) emissions from human activities (burning fossil fuels and cement production, deforestation and other land-use change) are set to rise again in 2014.
This study (updated yearly) makes an accurate assessment of anthropogenic CO2 emissions and their redistribution between the atmosphere, ocean, and terrestrial biosphere in order to better understand the global carbon cycle, support the development of climate policies, and project future climate change.
C. Yue, P. Ciais, P. Cadule, K. Thonicke, and T. T. van Leeuwen
Geosci. Model Dev., 8, 1321–1338, https://doi.org/10.5194/gmd-8-1321-2015, https://doi.org/10.5194/gmd-8-1321-2015, 2015
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We conducted parallel simulations using a global land surface model, with and without fires being included, respectively. When the anthropogenic land cover change fire is excluded, we find that natural wildfires have reduced the global land carbon uptake by 0.3Pg C per year over 1901-2012. This is equivalent to 20% of the land carbon uptake in a world without fire. This fire-induced reduction in carbon uptake could be partly explained by climate variability, in particular the ENSO events.
F. M. Bréon, G. Broquet, V. Puygrenier, F. Chevallier, I. Xueref-Remy, M. Ramonet, E. Dieudonné, M. Lopez, M. Schmidt, O. Perrussel, and P. Ciais
Atmos. Chem. Phys., 15, 1707–1724, https://doi.org/10.5194/acp-15-1707-2015, https://doi.org/10.5194/acp-15-1707-2015, 2015
R. Locatelli, P. Bousquet, F. Hourdin, M. Saunois, A. Cozic, F. Couvreux, J.-Y. Grandpeix, M.-P. Lefebvre, C. Rio, P. Bergamaschi, S. D. Chambers, U. Karstens, V. Kazan, S. van der Laan, H. A. J. Meijer, J. Moncrieff, M. Ramonet, H. A. Scheeren, C. Schlosser, M. Schmidt, A. Vermeulen, and A. G. Williams
Geosci. Model Dev., 8, 129–150, https://doi.org/10.5194/gmd-8-129-2015, https://doi.org/10.5194/gmd-8-129-2015, 2015
S. Sitch, P. Friedlingstein, N. Gruber, S. D. Jones, G. Murray-Tortarolo, A. Ahlström, S. C. Doney, H. Graven, C. Heinze, C. Huntingford, S. Levis, P. E. Levy, M. Lomas, B. Poulter, N. Viovy, S. Zaehle, N. Zeng, A. Arneth, G. Bonan, L. Bopp, J. G. Canadell, F. Chevallier, P. Ciais, R. Ellis, M. Gloor, P. Peylin, S. L. Piao, C. Le Quéré, B. Smith, Z. Zhu, and R. Myneni
Biogeosciences, 12, 653–679, https://doi.org/10.5194/bg-12-653-2015, https://doi.org/10.5194/bg-12-653-2015, 2015
D. Butterfield and T. Gardiner
Atmos. Meas. Tech., 8, 463–470, https://doi.org/10.5194/amt-8-463-2015, https://doi.org/10.5194/amt-8-463-2015, 2015
P. Bergamaschi, M. Corazza, U. Karstens, M. Athanassiadou, R. L. Thompson, I. Pison, A. J. Manning, P. Bousquet, A. Segers, A. T. Vermeulen, G. Janssens-Maenhout, M. Schmidt, M. Ramonet, F. Meinhardt, T. Aalto, L. Haszpra, J. Moncrieff, M. E. Popa, D. Lowry, M. Steinbacher, A. Jordan, S. O'Doherty, S. Piacentino, and E. Dlugokencky
Atmos. Chem. Phys., 15, 715–736, https://doi.org/10.5194/acp-15-715-2015, https://doi.org/10.5194/acp-15-715-2015, 2015
E. Joetzjer, C. Delire, H. Douville, P. Ciais, B. Decharme, R. Fisher, B. Christoffersen, J. C. Calvet, A. C. L. da Costa, L. V. Ferreira, and P. Meir
Geosci. Model Dev., 7, 2933–2950, https://doi.org/10.5194/gmd-7-2933-2014, https://doi.org/10.5194/gmd-7-2933-2014, 2014
L. Ammoura, I. Xueref-Remy, V. Gros, A. Baudic, B. Bonsang, J.-E. Petit, O. Perrussel, N. Bonnaire, J. Sciare, and F. Chevallier
Atmos. Chem. Phys., 14, 12871–12882, https://doi.org/10.5194/acp-14-12871-2014, https://doi.org/10.5194/acp-14-12871-2014, 2014
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We present the first study of CO2, VOCs and NOx measured all together in a road tunnel around the Paris megacity with the aim to quantify the ratios of these species co-emitted within traffic emissions. It allows us to independently assess some of the ratios provided in the latest Paris emission inventory. It also reveals a large variability of the ratios to CO2, implying that traffic does not have a unique imprint in the urban plume, but rather leaves various signatures.
M. Van Oijen, J. Balkovi, C. Beer, D. R. Cameron, P. Ciais, W. Cramer, T. Kato, M. Kuhnert, R. Martin, R. Myneni, A. Rammig, S. Rolinski, J.-F. Soussana, K. Thonicke, M. Van der Velde, and L. Xu
Biogeosciences, 11, 6357–6375, https://doi.org/10.5194/bg-11-6357-2014, https://doi.org/10.5194/bg-11-6357-2014, 2014
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We use a new risk analysis method, and six vegetation models, to analyse how climate change may alter drought risks in European ecosystems. The conclusions are (1) drought will pose increasing risks to productivity in the Mediterranean area; (2) this is because severe droughts will become more frequent, not because ecosystems will become more vulnerable; (3) future C sequestration will be at risk because carbon gain in primary productivity will be more affected than carbon loss in respiration.
C. Yue, P. Ciais, P. Cadule, K. Thonicke, S. Archibald, B. Poulter, W. M. Hao, S. Hantson, F. Mouillot, P. Friedlingstein, F. Maignan, and N. Viovy
Geosci. Model Dev., 7, 2747–2767, https://doi.org/10.5194/gmd-7-2747-2014, https://doi.org/10.5194/gmd-7-2747-2014, 2014
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ORCHIDEE-SPITFIRE model could moderately capture the decadal trend and variation of burned area during the 20th century, and the spatial and temporal patterns of contemporary vegetation fires. The model has a better performance in simulating fires for regions dominated by climate-driven fires, such as boreal forests. However, it has limited capability to reproduce the infrequent but important large fires in different ecosystems, where urgent model improvement is needed in the future.
A. Agustí-Panareda, S. Massart, F. Chevallier, S. Boussetta, G. Balsamo, A. Beljaars, P. Ciais, N. M. Deutscher, R. Engelen, L. Jones, R. Kivi, J.-D. Paris, V.-H. Peuch, V. Sherlock, A. T. Vermeulen, P. O. Wennberg, and D. Wunch
Atmos. Chem. Phys., 14, 11959–11983, https://doi.org/10.5194/acp-14-11959-2014, https://doi.org/10.5194/acp-14-11959-2014, 2014
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This paper presents a new operational CO2 forecast product as part of the Copernicus Atmospheric Services suite of atmospheric composition products, using the state-of-the-art numerical weather prediction model from the European Centre of Medium-Range Weather Forecasts.
The evaluation with independent observations shows that the forecast has skill in predicting the synoptic variability of CO2. The online simulation of CO2 fluxes from vegetation contributes to this skill.
S. Kuppel, P. Peylin, F. Maignan, F. Chevallier, G. Kiely, L. Montagnani, and A. Cescatti
Geosci. Model Dev., 7, 2581–2597, https://doi.org/10.5194/gmd-7-2581-2014, https://doi.org/10.5194/gmd-7-2581-2014, 2014
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A consistent calibration of an advanced land surface model was performed by grouping in situ information on land-atmosphere exchanges of carbon and water using broad ecosystem and climate classes. Signatures of improved carbon cycle simulations were found across spatial and temporal scales, along with insights into current model limitations. These results hold promising perspectives within the ongoing efforts towards building robust model-data fusion frameworks for earth system models.
H. Angot, M. Barret, O. Magand, M. Ramonet, and A. Dommergue
Atmos. Chem. Phys., 14, 11461–11473, https://doi.org/10.5194/acp-14-11461-2014, https://doi.org/10.5194/acp-14-11461-2014, 2014
C. Wilson, M. P. Chipperfield, M. Gloor, and F. Chevallier
Geosci. Model Dev., 7, 2485–2500, https://doi.org/10.5194/gmd-7-2485-2014, https://doi.org/10.5194/gmd-7-2485-2014, 2014
I. B. Konovalov, E. V. Berezin, P. Ciais, G. Broquet, M. Beekmann, J. Hadji-Lazaro, C. Clerbaux, M. O. Andreae, J. W. Kaiser, and E.-D. Schulze
Atmos. Chem. Phys., 14, 10383–10410, https://doi.org/10.5194/acp-14-10383-2014, https://doi.org/10.5194/acp-14-10383-2014, 2014
J. P. Boisier, N. de Noblet-Ducoudré, and P. Ciais
Hydrol. Earth Syst. Sci., 18, 3571–3590, https://doi.org/10.5194/hess-18-3571-2014, https://doi.org/10.5194/hess-18-3571-2014, 2014
B. P. Guillod, B. Orlowsky, D. Miralles, A. J. Teuling, P. D. Blanken, N. Buchmann, P. Ciais, M. Ek, K. L. Findell, P. Gentine, B. R. Lintner, R. L. Scott, B. Van den Hurk, and S. I. Seneviratne
Atmos. Chem. Phys., 14, 8343–8367, https://doi.org/10.5194/acp-14-8343-2014, https://doi.org/10.5194/acp-14-8343-2014, 2014
J. B. Fisher, M. Sikka, W. C. Oechel, D. N. Huntzinger, J. R. Melton, C. D. Koven, A. Ahlström, M. A. Arain, I. Baker, J. M. Chen, P. Ciais, C. Davidson, M. Dietze, B. El-Masri, D. Hayes, C. Huntingford, A. K. Jain, P. E. Levy, M. R. Lomas, B. Poulter, D. Price, A. K. Sahoo, K. Schaefer, H. Tian, E. Tomelleri, H. Verbeeck, N. Viovy, R. Wania, N. Zeng, and C. E. Miller
Biogeosciences, 11, 4271–4288, https://doi.org/10.5194/bg-11-4271-2014, https://doi.org/10.5194/bg-11-4271-2014, 2014
M. Schmidt, M. Lopez, C. Yver Kwok, C. Messager, M. Ramonet, B. Wastine, C. Vuillemin, F. Truong, B. Gal, E. Parmentier, O. Cloué, and P. Ciais
Atmos. Meas. Tech., 7, 2283–2296, https://doi.org/10.5194/amt-7-2283-2014, https://doi.org/10.5194/amt-7-2283-2014, 2014
P. Ciais, A. J. Dolman, A. Bombelli, R. Duren, A. Peregon, P. J. Rayner, C. Miller, N. Gobron, G. Kinderman, G. Marland, N. Gruber, F. Chevallier, R. J. Andres, G. Balsamo, L. Bopp, F.-M. Bréon, G. Broquet, R. Dargaville, T. J. Battin, A. Borges, H. Bovensmann, M. Buchwitz, J. Butler, J. G. Canadell, R. B. Cook, R. DeFries, R. Engelen, K. R. Gurney, C. Heinze, M. Heimann, A. Held, M. Henry, B. Law, S. Luyssaert, J. Miller, T. Moriyama, C. Moulin, R. B. Myneni, C. Nussli, M. Obersteiner, D. Ojima, Y. Pan, J.-D. Paris, S. L. Piao, B. Poulter, S. Plummer, S. Quegan, P. Raymond, M. Reichstein, L. Rivier, C. Sabine, D. Schimel, O. Tarasova, R. Valentini, R. Wang, G. van der Werf, D. Wickland, M. Williams, and C. Zehner
Biogeosciences, 11, 3547–3602, https://doi.org/10.5194/bg-11-3547-2014, https://doi.org/10.5194/bg-11-3547-2014, 2014
S. Massart, A. Agusti-Panareda, I. Aben, A. Butz, F. Chevallier, C. Crevoisier, R. Engelen, C. Frankenberg, and O. Hasekamp
Atmos. Chem. Phys., 14, 6139–6158, https://doi.org/10.5194/acp-14-6139-2014, https://doi.org/10.5194/acp-14-6139-2014, 2014
R. L. Thompson, K. Ishijima, E. Saikawa, M. Corazza, U. Karstens, P. K. Patra, P. Bergamaschi, F. Chevallier, E. Dlugokencky, R. G. Prinn, R. F. Weiss, S. O'Doherty, P. J. Fraser, L. P. Steele, P. B. Krummel, A. Vermeulen, Y. Tohjima, A. Jordan, L. Haszpra, M. Steinbacher, S. Van der Laan, T. Aalto, F. Meinhardt, M. E. Popa, J. Moncrieff, and P. Bousquet
Atmos. Chem. Phys., 14, 6177–6194, https://doi.org/10.5194/acp-14-6177-2014, https://doi.org/10.5194/acp-14-6177-2014, 2014
C. Le Quéré, G. P. Peters, R. J. Andres, R. M. Andrew, T. A. Boden, P. Ciais, P. Friedlingstein, R. A. Houghton, G. Marland, R. Moriarty, S. Sitch, P. Tans, A. Arneth, A. Arvanitis, D. C. E. Bakker, L. Bopp, J. G. Canadell, L. P. Chini, S. C. Doney, A. Harper, I. Harris, J. I. House, A. K. Jain, S. D. Jones, E. Kato, R. F. Keeling, K. Klein Goldewijk, A. Körtzinger, C. Koven, N. Lefèvre, F. Maignan, A. Omar, T. Ono, G.-H. Park, B. Pfeil, B. Poulter, M. R. Raupach, P. Regnier, C. Rödenbeck, S. Saito, J. Schwinger, J. Segschneider, B. D. Stocker, T. Takahashi, B. Tilbrook, S. van Heuven, N. Viovy, R. Wanninkhof, A. Wiltshire, and S. Zaehle
Earth Syst. Sci. Data, 6, 235–263, https://doi.org/10.5194/essd-6-235-2014, https://doi.org/10.5194/essd-6-235-2014, 2014
X. Wu, F. Babst, P. Ciais, D. Frank, M. Reichstein, M. Wattenbach, C. Zang, and M. D. Mahecha
Biogeosciences, 11, 3057–3068, https://doi.org/10.5194/bg-11-3057-2014, https://doi.org/10.5194/bg-11-3057-2014, 2014
M. Balzarolo, S. Boussetta, G. Balsamo, A. Beljaars, F. Maignan, J.-C. Calvet, S. Lafont, A. Barbu, B. Poulter, F. Chevallier, C. Szczypta, and D. Papale
Biogeosciences, 11, 2661–2678, https://doi.org/10.5194/bg-11-2661-2014, https://doi.org/10.5194/bg-11-2661-2014, 2014
C. Szczypta, J.-C. Calvet, F. Maignan, W. Dorigo, F. Baret, and P. Ciais
Geosci. Model Dev., 7, 931–946, https://doi.org/10.5194/gmd-7-931-2014, https://doi.org/10.5194/gmd-7-931-2014, 2014
K. Nishina, A. Ito, D. J. Beerling, P. Cadule, P. Ciais, D. B. Clark, P. Falloon, A. D. Friend, R. Kahana, E. Kato, R. Keribin, W. Lucht, M. Lomas, T. T. Rademacher, R. Pavlick, S. Schaphoff, N. Vuichard, L. Warszawaski, and T. Yokohata
Earth Syst. Dynam., 5, 197–209, https://doi.org/10.5194/esd-5-197-2014, https://doi.org/10.5194/esd-5-197-2014, 2014
S. X. Fang, L. X. Zhou, P. P. Tans, P. Ciais, M. Steinbacher, L. Xu, and T. Luan
Atmos. Chem. Phys., 14, 2541–2554, https://doi.org/10.5194/acp-14-2541-2014, https://doi.org/10.5194/acp-14-2541-2014, 2014
R. L. Thompson, F. Chevallier, A. M. Crotwell, G. Dutton, R. L. Langenfelds, R. G. Prinn, R. F. Weiss, Y. Tohjima, T. Nakazawa, P. B. Krummel, L. P. Steele, P. Fraser, S. O'Doherty, K. Ishijima, and S. Aoki
Atmos. Chem. Phys., 14, 1801–1817, https://doi.org/10.5194/acp-14-1801-2014, https://doi.org/10.5194/acp-14-1801-2014, 2014
R. Valentini, A. Arneth, A. Bombelli, S. Castaldi, R. Cazzolla Gatti, F. Chevallier, P. Ciais, E. Grieco, J. Hartmann, M. Henry, R. A. Houghton, M. Jung, W. L. Kutsch, Y. Malhi, E. Mayorga, L. Merbold, G. Murray-Tortarolo, D. Papale, P. Peylin, B. Poulter, P. A. Raymond, M. Santini, S. Sitch, G. Vaglio Laurin, G. R. van der Werf, C. A. Williams, and R. J. Scholes
Biogeosciences, 11, 381–407, https://doi.org/10.5194/bg-11-381-2014, https://doi.org/10.5194/bg-11-381-2014, 2014
C. Cressot, F. Chevallier, P. Bousquet, C. Crevoisier, E. J. Dlugokencky, A. Fortems-Cheiney, C. Frankenberg, R. Parker, I. Pison, R. A. Scheepmaker, S. A. Montzka, P. B. Krummel, L. P. Steele, and R. L. Langenfelds
Atmos. Chem. Phys., 14, 577–592, https://doi.org/10.5194/acp-14-577-2014, https://doi.org/10.5194/acp-14-577-2014, 2014
J. F. Chang, N. Viovy, N. Vuichard, P. Ciais, T. Wang, A. Cozic, R. Lardy, A.-I. Graux, K. Klumpp, R. Martin, and J.-F. Soussana
Geosci. Model Dev., 6, 2165–2181, https://doi.org/10.5194/gmd-6-2165-2013, https://doi.org/10.5194/gmd-6-2165-2013, 2013
B. Guenet, F. E. Moyano, N. Vuichard, G. J. D. Kirk, P. H. Bellamy, S. Zaehle, and P. Ciais
Geosci. Model Dev., 6, 2153–2163, https://doi.org/10.5194/gmd-6-2153-2013, https://doi.org/10.5194/gmd-6-2153-2013, 2013
F. Souty, B. Dorin, T. Brunelle, P. Dumas, and P. Ciais
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmdd-6-6975-2013, https://doi.org/10.5194/gmdd-6-6975-2013, 2013
Revised manuscript has not been submitted
C. Yue, P. Ciais, S. Luyssaert, P. Cadule, J. Harden, J. Randerson, V. Bellassen, T. Wang, S. L. Piao, B. Poulter, and N. Viovy
Biogeosciences, 10, 8233–8252, https://doi.org/10.5194/bg-10-8233-2013, https://doi.org/10.5194/bg-10-8233-2013, 2013
E. Joetzjer, H. Douville, C. Delire, P. Ciais, B. Decharme, and S. Tyteca
Hydrol. Earth Syst. Sci., 17, 4885–4895, https://doi.org/10.5194/hess-17-4885-2013, https://doi.org/10.5194/hess-17-4885-2013, 2013
I. Pison, B. Ringeval, P. Bousquet, C. Prigent, and F. Papa
Atmos. Chem. Phys., 13, 11609–11623, https://doi.org/10.5194/acp-13-11609-2013, https://doi.org/10.5194/acp-13-11609-2013, 2013
C. Rose, J. Boulon, M. Hervo, H. Holmgren, E. Asmi, M. Ramonet, P. Laj, and K. Sellegri
Atmos. Chem. Phys., 13, 11573–11594, https://doi.org/10.5194/acp-13-11573-2013, https://doi.org/10.5194/acp-13-11573-2013, 2013
V. V. S. S. Sarma, A. Lenton, R. M. Law, N. Metzl, P. K. Patra, S. Doney, I. D. Lima, E. Dlugokencky, M. Ramonet, and V. Valsala
Biogeosciences, 10, 7035–7052, https://doi.org/10.5194/bg-10-7035-2013, https://doi.org/10.5194/bg-10-7035-2013, 2013
J.-L. Baray, Y. Courcoux, P. Keckhut, T. Portafaix, P. Tulet, J.-P. Cammas, A. Hauchecorne, S. Godin Beekmann, M. De Mazière, C. Hermans, F. Desmet, K. Sellegri, A. Colomb, M. Ramonet, J. Sciare, C. Vuillemin, C. Hoareau, D. Dionisi, V. Duflot, H. Vérèmes, J. Porteneuve, F. Gabarrot, T. Gaudo, J.-M. Metzger, G. Payen, J. Leclair de Bellevue, C. Barthe, F. Posny, P. Ricaud, A. Abchiche, and R. Delmas
Atmos. Meas. Tech., 6, 2865–2877, https://doi.org/10.5194/amt-6-2865-2013, https://doi.org/10.5194/amt-6-2865-2013, 2013
C. E. Yver-Kwok, D. Müller, C. Caldow, B. Lebegue, J. G. Mønster, C. W. Rella, C. Scheutz, M. Schmidt, M. Ramonet, T. Warneke, G. Broquet, and P. Ciais
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amtd-6-9181-2013, https://doi.org/10.5194/amtd-6-9181-2013, 2013
Revised manuscript not accepted
P. Peylin, R. M. Law, K. R. Gurney, F. Chevallier, A. R. Jacobson, T. Maki, Y. Niwa, P. K. Patra, W. Peters, P. J. Rayner, C. Rödenbeck, I. T. van der Laan-Luijkx, and X. Zhang
Biogeosciences, 10, 6699–6720, https://doi.org/10.5194/bg-10-6699-2013, https://doi.org/10.5194/bg-10-6699-2013, 2013
R. Locatelli, P. Bousquet, F. Chevallier, A. Fortems-Cheney, S. Szopa, M. Saunois, A. Agusti-Panareda, D. Bergmann, H. Bian, P. Cameron-Smith, M. P. Chipperfield, E. Gloor, S. Houweling, S. R. Kawa, M. Krol, P. K. Patra, R. G. Prinn, M. Rigby, R. Saito, and C. Wilson
Atmos. Chem. Phys., 13, 9917–9937, https://doi.org/10.5194/acp-13-9917-2013, https://doi.org/10.5194/acp-13-9917-2013, 2013
B. Mueller, M. Hirschi, C. Jimenez, P. Ciais, P. A. Dirmeyer, A. J. Dolman, J. B. Fisher, M. Jung, F. Ludwig, F. Maignan, D. G. Miralles, M. F. McCabe, M. Reichstein, J. Sheffield, K. Wang, E. F. Wood, Y. Zhang, and S. I. Seneviratne
Hydrol. Earth Syst. Sci., 17, 3707–3720, https://doi.org/10.5194/hess-17-3707-2013, https://doi.org/10.5194/hess-17-3707-2013, 2013
E. V. Berezin, I. B. Konovalov, P. Ciais, A. Richter, S. Tao, G. Janssens-Maenhout, M. Beekmann, and E.-D. Schulze
Atmos. Chem. Phys., 13, 9415–9438, https://doi.org/10.5194/acp-13-9415-2013, https://doi.org/10.5194/acp-13-9415-2013, 2013
G. Broquet, F. Chevallier, F.-M. Bréon, N. Kadygrov, M. Alemanno, F. Apadula, S. Hammer, L. Haszpra, F. Meinhardt, J. A. Morguí, J. Necki, S. Piacentino, M. Ramonet, M. Schmidt, R. L. Thompson, A. T. Vermeulen, C. Yver, and P. Ciais
Atmos. Chem. Phys., 13, 9039–9056, https://doi.org/10.5194/acp-13-9039-2013, https://doi.org/10.5194/acp-13-9039-2013, 2013
M. Lopez, M. Schmidt, M. Delmotte, A. Colomb, V. Gros, C. Janssen, S. J. Lehman, D. Mondelain, O. Perrussel, M. Ramonet, I. Xueref-Remy, and P. Bousquet
Atmos. Chem. Phys., 13, 7343–7358, https://doi.org/10.5194/acp-13-7343-2013, https://doi.org/10.5194/acp-13-7343-2013, 2013
A. Berchet, I. Pison, F. Chevallier, P. Bousquet, S. Conil, M. Geever, T. Laurila, J. Lavrič, M. Lopez, J. Moncrieff, J. Necki, M. Ramonet, M. Schmidt, M. Steinbacher, and J. Tarniewicz
Atmos. Chem. Phys., 13, 7115–7132, https://doi.org/10.5194/acp-13-7115-2013, https://doi.org/10.5194/acp-13-7115-2013, 2013
M. Roland, P. Serrano-Ortiz, A. S. Kowalski, Y. Goddéris, E. P. Sánchez-Cañete, P. Ciais, F. Domingo, S. Cuezva, S. Sanchez-Moral, B. Longdoz, D. Yakir, R. Van Grieken, J. Schott, C. Cardell, and I. A. Janssens
Biogeosciences, 10, 5009–5017, https://doi.org/10.5194/bg-10-5009-2013, https://doi.org/10.5194/bg-10-5009-2013, 2013
L. Menut, B. Bessagnet, D. Khvorostyanov, M. Beekmann, N. Blond, A. Colette, I. Coll, G. Curci, G. Foret, A. Hodzic, S. Mailler, F. Meleux, J.-L. Monge, I. Pison, G. Siour, S. Turquety, M. Valari, R. Vautard, and M. G. Vivanco
Geosci. Model Dev., 6, 981–1028, https://doi.org/10.5194/gmd-6-981-2013, https://doi.org/10.5194/gmd-6-981-2013, 2013
N. Huneeus, O. Boucher, and F. Chevallier
Atmos. Chem. Phys., 13, 6555–6573, https://doi.org/10.5194/acp-13-6555-2013, https://doi.org/10.5194/acp-13-6555-2013, 2013
F. Chevallier
Geosci. Model Dev., 6, 783–790, https://doi.org/10.5194/gmd-6-783-2013, https://doi.org/10.5194/gmd-6-783-2013, 2013
T. Gasser and P. Ciais
Earth Syst. Dynam., 4, 171–186, https://doi.org/10.5194/esd-4-171-2013, https://doi.org/10.5194/esd-4-171-2013, 2013
R. Wang, S. Tao, P. Ciais, H. Z. Shen, Y. Huang, H. Chen, G. F. Shen, B. Wang, W. Li, Y. Y. Zhang, Y. Lu, D. Zhu, Y. C. Chen, X. P. Liu, W. T. Wang, X. L. Wang, W. X. Liu, B. G. Li, and S. L. Piao
Atmos. Chem. Phys., 13, 5189–5203, https://doi.org/10.5194/acp-13-5189-2013, https://doi.org/10.5194/acp-13-5189-2013, 2013
C. Le Quéré, R. J. Andres, T. Boden, T. Conway, R. A. Houghton, J. I. House, G. Marland, G. P. Peters, G. R. van der Werf, A. Ahlström, R. M. Andrew, L. Bopp, J. G. Canadell, P. Ciais, S. C. Doney, C. Enright, P. Friedlingstein, C. Huntingford, A. K. Jain, C. Jourdain, E. Kato, R. F. Keeling, K. Klein Goldewijk, S. Levis, P. Levy, M. Lomas, B. Poulter, M. R. Raupach, J. Schwinger, S. Sitch, B. D. Stocker, N. Viovy, S. Zaehle, and N. Zeng
Earth Syst. Sci. Data, 5, 165–185, https://doi.org/10.5194/essd-5-165-2013, https://doi.org/10.5194/essd-5-165-2013, 2013
M. Ménégoz, G. Krinner, Y. Balkanski, A. Cozic, O. Boucher, and P. Ciais
The Cryosphere, 7, 537–554, https://doi.org/10.5194/tc-7-537-2013, https://doi.org/10.5194/tc-7-537-2013, 2013
J. P. Boisier, N. de Noblet-Ducoudré, and P. Ciais
Biogeosciences, 10, 1501–1516, https://doi.org/10.5194/bg-10-1501-2013, https://doi.org/10.5194/bg-10-1501-2013, 2013
U. Schuster, G. A. McKinley, N. Bates, F. Chevallier, S. C. Doney, A. R. Fay, M. González-Dávila, N. Gruber, S. Jones, J. Krijnen, P. Landschützer, N. Lefèvre, M. Manizza, J. Mathis, N. Metzl, A. Olsen, A. F. Rios, C. Rödenbeck, J. M. Santana-Casiano, T. Takahashi, R. Wanninkhof, and A. J. Watson
Biogeosciences, 10, 607–627, https://doi.org/10.5194/bg-10-607-2013, https://doi.org/10.5194/bg-10-607-2013, 2013
P. K. Patra, J. G. Canadell, R. A. Houghton, S. L. Piao, N.-H. Oh, P. Ciais, K. R. Manjunath, A. Chhabra, T. Wang, T. Bhattacharya, P. Bousquet, J. Hartman, A. Ito, E. Mayorga, Y. Niwa, P. A. Raymond, V. V. S. S. Sarma, and R. Lasco
Biogeosciences, 10, 513–527, https://doi.org/10.5194/bg-10-513-2013, https://doi.org/10.5194/bg-10-513-2013, 2013
B. Ringeval, P. O. Hopcroft, P. J. Valdes, P. Ciais, G. Ramstein, A. J. Dolman, and M. Kageyama
Clim. Past, 9, 149–171, https://doi.org/10.5194/cp-9-149-2013, https://doi.org/10.5194/cp-9-149-2013, 2013
Related subject area
Subject: Gases | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Measurement report: Leaf-scale gas exchange of atmospheric reactive trace species (NO2, NO, O3) at a northern hardwood forest in Michigan
A dedicated flask sampling strategy developed for Integrated Carbon Observation System (ICOS) stations based on CO2 and CO measurements and Stochastic Time-Inverted Lagrangian Transport (STILT) footprint modelling
Ozone affected by a succession of four landfall typhoons in the Yangtze River Delta, China: major processes and health impacts
The increasing atmospheric burden of the greenhouse gas sulfur hexafluoride (SF6)
Understanding nighttime methane signals at the Amazon Tall Tower Observatory (ATTO)
Estimating CH4, CO2, and CO emissions from coal mining and industrial activities in the Upper Silesian Coal Basin using an aircraft-based mass balance approach
Profiling of formaldehyde, glyoxal, methylglyoxal, and CO over the Amazon: Normalised excess mixing ratios and related emission factors in biomass burning plumes
Background heterogeneity and other uncertainties in estimating urban methane flux: results from the Indianapolis Flux Experiment (INFLUX)
Methane emissions from the Munich Oktoberfest
4D dispersion of total gaseous mercury derived from a mining source: identification of criteria to assess risks related with high concentrations of atmospheric mercury
A study of the influence of tropospheric subsidence on spring and summer surface ozone concentrations at the JRC Ispra station in northern Italy
Local and synoptic meteorological influences on daily variability in summertime surface ozone in eastern China
Variability in a four-network composite of atmospheric CO2 differences between three primary baseline sites
Quantifying the impact of synoptic circulation patterns on ozone variability in northern China from April to October 2013–2017
Multivariate statistical air mass classification for the high-alpine observatory at the Zugspitze Mountain, Germany
Evolution of anthropogenic air pollutant emissions in Guangdong Province, China, from 2006 to 2015
Speciated atmospheric mercury and sea–air exchange of gaseous mercury in the South China Sea
Methane emissions from oil and gas platforms in the North Sea
Assessing London CO2, CH4 and CO emissions using aircraft measurements and dispersion modelling
2005–2017 ozone trends and potential benefits of local measures as deduced from air quality measurements in the north of the Barcelona metropolitan area
Country-scale greenhouse gas budgets using shipborne measurements: a case study for the UK and Ireland
Intercomparison of midlatitude tropospheric and lower-stratospheric water vapor measurements and comparison to ECMWF humidity data
Eddy flux measurements of sulfur dioxide deposition to the sea surface
Quantifying uncertainties from mobile-laboratory-derived emissions of well pads using inverse Gaussian methods
Observing local CO2 sources using low-cost, near-surface urban monitors
Spatiotemporal variability of NO2 and PM2.5 over Eastern China: observational and model analyses with a novel statistical method
Spatial–temporal patterns of inorganic nitrogen air concentrations and deposition in eastern China
Phenomenology of summer ozone episodes over the Madrid Metropolitan Area, central Spain
Ship-based MAX-DOAS measurements of tropospheric NO2, SO2, and HCHO distribution along the Yangtze River
Gradient flux measurements of sea–air DMS transfer during the Surface Ocean Aerosol Production (SOAP) experiment
Measurements of atmospheric ethene by solar absorption FTIR spectrometry
Ozone pollution around a coastal region of South China Sea: interaction between marine and continental air
Abundance and sources of atmospheric halocarbons in the Eastern Mediterranean
Diurnal, synoptic and seasonal variability of atmospheric CO2 in the Paris megacity area
Atmospheric carbonyl sulfide (OCS) measured remotely by FTIR solar absorption spectrometry
Temporal variation of VOC fluxes measured with PTR-TOF above a boreal forest
Long-term trends of surface ozone and its influencing factors at the Mt Waliguan GAW station, China – Part 2: The roles of anthropogenic emissions and climate variability
Gaseous elemental mercury (GEM) fluxes over canopy of two typical subtropical forests in south China
Observations of ozone depletion events in a Finnish boreal forest
Mobile measurement of methane emissions from natural gas developments in northeastern British Columbia, Canada
Impacts of large-scale circulation on urban ambient concentrations of gaseous elemental mercury in New York, USA
Wei Wang, Laurens Ganzeveld, Samuel Rossabi, Jacques Hueber, and Detlev Helmig
Atmos. Chem. Phys., 20, 11287–11304, https://doi.org/10.5194/acp-20-11287-2020, https://doi.org/10.5194/acp-20-11287-2020, 2020
Short summary
Short summary
Trees exchange with the atmosphere nitrogen oxides and ozone, affecting the tropospheric composition and consequently air quality and ecosystem health. We examined the leaf-level gas exchanges for four typical tree species (pine, maple, oak, aspen) found in northern Michigan, US. The leaves largely absorb the gases, showing little evidence of emission. We measured the uptake rates that can be used to improve model studies of the source and sink processes controlling these gases in forests.
Ingeborg Levin, Ute Karstens, Markus Eritt, Fabian Maier, Sabrina Arnold, Daniel Rzesanke, Samuel Hammer, Michel Ramonet, Gabriela Vítková, Sebastien Conil, Michal Heliasz, Dagmar Kubistin, and Matthias Lindauer
Atmos. Chem. Phys., 20, 11161–11180, https://doi.org/10.5194/acp-20-11161-2020, https://doi.org/10.5194/acp-20-11161-2020, 2020
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Based on observations and Stochastic Time-Inverted Lagrangian Transport (STILT) footprint modelling, a sampling strategy has been developed for tall tower stations of the Integrated Carbon Observation System (ICOS) research infrastructure atmospheric station network. This strategy allows independent quality control of in situ measurements, provides representative coverage of the influence area of the sites, and is capable of automated targeted sampling of fossil fuel CO2 emission hotspots.
Chenchao Zhan, Min Xie, Chongwu Huang, Tijian Wang, Jane Liu, Meng Xu, Chaoqun Ma, Jianwei Yu, Yumeng Jiao, Mengmeng Li, Shu Li, Bingliang Zhuang, Ming Zhao, and Dongyang Nie
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-554, https://doi.org/10.5194/acp-2020-554, 2020
Revised manuscript accepted for ACP
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The Yangtze River Delta (YRD) region is suffering from severe ozone (O3) pollution in recent years. Synoptic systems, like typhoon, can have significant effect on O3 episode. However, research on landfall typhoon affecting O3 in the YRD is quite limited. This work aims to reveal the main processes of landfall typhoon affecting surface O3, and estimate health impacts of O3 during the study period in the YRD, which can be useful for making reasonable pollution control measures in this area.
Peter G. Simmonds, Matthew Rigby, Alistair J. Manning, Sunyoung Park, Kieran M. Stanley, Archie McCulloch, Stephan Henne, Francesco Graziosi, Michela Maione, Jgor Arduini, Stefan Reimann, Martin K. Vollmer, Jens Mühle, Simon O'Doherty, Dickon Young, Paul B. Krummel, Paul J. Fraser, Ray F. Weiss, Peter K. Salameh, Christina M. Harth, Mi-Kyung Park, Hyeri Park, Tim Arnold, Chris Rennick, L. Paul Steele, Blagoj Mitrevski, Ray H. J. Wang, and Ronald G. Prinn
Atmos. Chem. Phys., 20, 7271–7290, https://doi.org/10.5194/acp-20-7271-2020, https://doi.org/10.5194/acp-20-7271-2020, 2020
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Sulfur hexafluoride (SF6) is a potent greenhouse gas which is regulated under the Kyoto Protocol. From a 40-year record of measurements, collected at five global monitoring sites and archived air samples, we show that its concentration in the atmosphere has steadily increased. Using modelling techniques, we estimate that global emissions have increased by about 24 % over the past decade. We find that this increase is driven by the demand for SF6-insulated switchgear in developing countries.
Santiago Botía, Christoph Gerbig, Julia Marshall, Jost V. Lavric, David Walter, Christopher Pöhlker, Bruna Holanda, Gilberto Fisch, Alessandro Carioca de Araújo, Marta O. Sá, Paulo R. Teixeira, Angélica F. Resende, Cleo Q. Dias-Junior, Hella van Asperen, Pablo S. Oliveira, Michel Stefanello, and Otávio C. Acevedo
Atmos. Chem. Phys., 20, 6583–6606, https://doi.org/10.5194/acp-20-6583-2020, https://doi.org/10.5194/acp-20-6583-2020, 2020
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A long record of atmospheric methane concentrations in central Amazonia was analyzed. We describe events in which concentrations at 79 m are higher than at 4 m. These events are more frequent during the nighttime of dry season, but we found no association with fire signals. Instead, we suggest that a combination of nighttime transport and a nearby source could explain such events. Our research gives insights into how methane is transported in the complex nocturnal atmosphere in Amazonia.
Alina Fiehn, Julian Kostinek, Maximilian Eckl, Theresa Klausner, Michał Gałkowski, Jinxuan Chen, Christoph Gerbig, Thomas Röckmann, Hossein Maazallahi, Martina Schmidt, Piotr Korbeń, Jarosław Nȩcki, Pawel Jagoda, Norman Wildmann, Christian Mallaun, Rostyslav Bun, Anna-Leah Nickl, Patrick Jöckel, Andreas Fix, and Anke Roiger
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-282, https://doi.org/10.5194/acp-2020-282, 2020
Revised manuscript accepted for ACP
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A severe reduction of greenhouse gas emissions is necessary to fulfill the Paris Agreement. We use aircraft- and ground-based in situ observations of trace gases and wind speed from two flights over the Upper Silesian Coal Basin, Poland, for independent emission estimation. The derived methane emission estimates are within the range of emission inventories, carbon dioxide estimates are in the lower range and carbon monoxide emission estimates are slightly higher than emission inventory values.
Flora Kluge, Tilman Hüneke, Matthias Knecht, Michael Lichtenstern, Meike Rotermund, Hans Schlager, Benjamin Schreiner, and Klaus Pfeilsticker
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-129, https://doi.org/10.5194/acp-2020-129, 2020
Revised manuscript accepted for ACP
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The presented study reports on atmospheric measurements of formaldehyde, glyoxal, methylglyoxal and CO over the Amazon basin and lays a special focus on the influence of biomass burning emissions on the atmospheric profiles of these carbonyl compounds within the planetary boundary layer as well as in the free and upper troposphere.
Nikolay V. Balashov, Kenneth J. Davis, Natasha L. Miles, Thomas Lauvaux, Scott J. Richardson, Zachary R. Barkley, and Timothy A. Bonin
Atmos. Chem. Phys., 20, 4545–4559, https://doi.org/10.5194/acp-20-4545-2020, https://doi.org/10.5194/acp-20-4545-2020, 2020
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An accurate independent verification methodology to estimate methane (a powerful greenhouse gas) emissions is essential for the effective implementation of policies that aim to reduce the impacts of climate change. In this paper, four uncertainties that complicate the independent estimation of urban methane emissions are identified: the definition of urban domain, background heterogeneity, emissions temporal variability, and missing sources. Ways to improve emission estimates are suggested.
Jia Chen, Florian Dietrich, Hossein Maazallahi, Andreas Forstmaier, Dominik Winkler, Magdalena E. G. Hofmann, Hugo Denier van der Gon, and Thomas Röckmann
Atmos. Chem. Phys., 20, 3683–3696, https://doi.org/10.5194/acp-20-3683-2020, https://doi.org/10.5194/acp-20-3683-2020, 2020
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We demonstrate for the first time that large festivals can be significant methane sources, though they are not included in emission inventories. We combined in situ measurements with a Gaussian plume model to determine the Oktoberfest emissions and show that they are not due solely to human biogenic emissions, but are instead primarily fossil fuel related. Our study provides the foundation to develop reduction policies for such events and new pathways to mitigate fossil fuel methane emissions.
José M. Esbrí, Pablo L. Higueras, Alba Martínez-Coronado, and Rocío Naharro
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2019-1107, https://doi.org/10.5194/acp-2019-1107, 2020
Revised manuscript accepted for ACP
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The aim of this work was to identify criteria to obtain the minimum amount of data with the maximum meaning and representativeness in order to delimitate risk areas, both in a spatial and temporal respect. We have constructed a model of vertical mercury movements which could be used to predict the location and timing of mercury inhalation risk. Also we have designed a monitoring strategy to identify the relevant criteria and this involved the measurement of gaseous mercury in a vertical section.
Pavlos Kalabokas, Niels Roland Jensen, Mauro Roveri, Jens Hjorth, Maxim Eremenko, Juan Cuesta, Gaëlle Dufour, Gilles Foret, and Matthias Beekmann
Atmos. Chem. Phys., 20, 1861–1885, https://doi.org/10.5194/acp-20-1861-2020, https://doi.org/10.5194/acp-20-1861-2020, 2020
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The influence of tropospheric ozone on the surface measurements at a regional air pollution station in the pre-Alpine area of northern Italy is investigated. During such episodes the local air pollution parameters show generally very low values, while the ozone levels reach high values, occasionally exceeding the ozone air quality standards. Better understanding of ozone variability over the examined region will help in the formulation of more effective policies for the environment and climate.
Han Han, Jane Liu, Lei Shu, Tijian Wang, and Huiling Yuan
Atmos. Chem. Phys., 20, 203–222, https://doi.org/10.5194/acp-20-203-2020, https://doi.org/10.5194/acp-20-203-2020, 2020
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We statistically assessed the impacts of local and synoptic meteorology on daily surface ozone in eastern China in summer during 2013–2018. The results show that the meteorology described by a multiple linear regression model explains 43 % of variations in surface ozone. The most important local meteorological factors vary with location in eastern China. The maximum impact of the predominant synoptic pattern on surface ozone can reach ± 8 µg m-3 or ± 16 % of the daily mean over some regions.
Roger J. Francey, Jorgen S. Frederiksen, L. Paul Steele, and Ray L. Langenfelds
Atmos. Chem. Phys., 19, 14741–14754, https://doi.org/10.5194/acp-19-14741-2019, https://doi.org/10.5194/acp-19-14741-2019, 2019
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25-year composites of interhemispheric baseline CO2 differences demonstrate close agreement between 4 monitoring networks. Variability from monthly to multiyear time frames mostly reflects variability in upper troposphere dynamical indices chosen to represent eddy and mean transport interhemispheric exchange. Monthly interhemispheric atmospheric fluxes are much larger than air–surface terrestrial exchanges. The composite differences offer unusual constraints on transport in global carbon models.
Jingda Liu, Lili Wang, Mingge Li, Zhiheng Liao, Yang Sun, Tao Song, Wenkang Gao, Yonghong Wang, Yan Li, Dongsheng Ji, Bo Hu, Veli-Matti Kerminen, Yuesi Wang, and Markku Kulmala
Atmos. Chem. Phys., 19, 14477–14492, https://doi.org/10.5194/acp-19-14477-2019, https://doi.org/10.5194/acp-19-14477-2019, 2019
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We analyzed the surface ozone variation characteristics and quantified the impact of synoptic and local meteorological factors on northern China during the warm season based on multi-city, in situ ozone and meteorological data, as well as meteorological reanalysis. The results of quantitative exploration on synoptic and local meteorological factors influencing both interannual and day-to-day ozone variations will provide the scientific basis for evaluating emission reduction measures.
Armin Sigmund, Korbinian Freier, Till Rehm, Ludwig Ries, Christian Schunk, Anette Menzel, and Christoph K. Thomas
Atmos. Chem. Phys., 19, 12477–12494, https://doi.org/10.5194/acp-19-12477-2019, https://doi.org/10.5194/acp-19-12477-2019, 2019
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Air masses at the Schneefernerhaus mountain site at Zugspitze Mountain, Germany, were classified with respect to the atmospheric layer from which they originated and their degree of pollution. Measurements of several gases, particulate matter, and standard meteorological quantities indicated that polluted air was lifted to the site in 31 % of cases and clean air descended to the site in approximately 14 % cases while most of the remaining cases were ambiguous.
Yahui Bian, Zhijiong Huang, Jiamin Ou, Zhuangmin Zhong, Yuanqian Xu, Zhiwei Zhang, Xiao Xiao, Xiao Ye, Yuqi Wu, Xiaohong Yin, Cheng Li, Liangfu Chen, Min Shao, and Junyu Zheng
Atmos. Chem. Phys., 19, 11701–11719, https://doi.org/10.5194/acp-19-11701-2019, https://doi.org/10.5194/acp-19-11701-2019, 2019
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During 2006–2015, emissions of SO2, NOx, PM2.5 and PM10 saw an obvious downtrend. However, most emissions still have large reduction potential. On-road mobile sources and solvent use are the two key sources that should receive more effective control measures in GD. Also, controls measures on VOC and NH3 should be weighted since they still increased in 2006–2015. Since most control measures focused on PRD rather than non-PRD in GD, emissions in non-PRD were increasingly important.
Chunjie Wang, Zhangwei Wang, Fan Hui, and Xiaoshan Zhang
Atmos. Chem. Phys., 19, 10111–10127, https://doi.org/10.5194/acp-19-10111-2019, https://doi.org/10.5194/acp-19-10111-2019, 2019
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A low GEM level indicated that the SCS suffered less anthropogenic influence. There was no significant difference in GEM and HgP2.5 values between day and night, but the RGM level was higher in daytime than in nighttime. The size distribution of HgP in PM10 was observed to be bi-modal, but the coarse modal was the dominant size. The annual emission flux of Hg0 from the SCS was estimated to be 159 ton yr-1. The dry deposition was an important pathway for the input of atmospheric Hg to the SCS.
Stuart N. Riddick, Denise L. Mauzerall, Michael Celia, Neil R. P. Harris, Grant Allen, Joseph Pitt, John Staunton-Sykes, Grant L. Forster, Mary Kang, David Lowry, Euan G. Nisbet, and Alistair J. Manning
Atmos. Chem. Phys., 19, 9787–9796, https://doi.org/10.5194/acp-19-9787-2019, https://doi.org/10.5194/acp-19-9787-2019, 2019
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Currently, bottom-up methods estimate that 0.13 % of methane produced by UK North Sea oil and gas installations is lost. Here we measure emissions from eight platforms in the North Sea and, when considered collectively, the methane loss is estimated at 0.19 % of gas production. As this ambient loss is not explicitly accounted for in the bottom-up approach, these measured emissions represent significant additional emissions above previous estimates.
Joseph R. Pitt, Grant Allen, Stéphane J.-B. Bauguitte, Martin W. Gallagher, James D. Lee, Will Drysdale, Beth Nelson, Alistair J. Manning, and Paul I. Palmer
Atmos. Chem. Phys., 19, 8931–8945, https://doi.org/10.5194/acp-19-8931-2019, https://doi.org/10.5194/acp-19-8931-2019, 2019
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This paper presents a new method to assess inventory estimates of greenhouse gas and air pollutant emissions for large cities and their surrounding regions. A case study using data sampled by a research aircraft around London was used to test the method. We found that the UK national inventory agrees with our observations for CO but needed lower emissions for CH4 to agree with the measured data. Repeated studies could help determine how these emissions vary on different timescales.
Jordi Massagué, Cristina Carnerero, Miguel Escudero, José María Baldasano, Andrés Alastuey, and Xavier Querol
Atmos. Chem. Phys., 19, 7445–7465, https://doi.org/10.5194/acp-19-7445-2019, https://doi.org/10.5194/acp-19-7445-2019, 2019
Carole Helfter, Neil Mullinger, Massimo Vieno, Simon O'Doherty, Michel Ramonet, Paul I. Palmer, and Eiko Nemitz
Atmos. Chem. Phys., 19, 3043–3063, https://doi.org/10.5194/acp-19-3043-2019, https://doi.org/10.5194/acp-19-3043-2019, 2019
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We present a novel approach to estimate the annual budgets of carbon dioxide (881.0 ± 128.5 Tg) and methane (2.55 ± 0.48 Tg) of the British Isles from shipborne measurements taken over a 3-year period (2015–2017). This study brings independent verification of the emission budgets estimated using alternative products and investigates the seasonality of these emissions, which is usually not possible.
Stefan Kaufmann, Christiane Voigt, Romy Heller, Tina Jurkat-Witschas, Martina Krämer, Christian Rolf, Martin Zöger, Andreas Giez, Bernhard Buchholz, Volker Ebert, Troy Thornberry, and Ulrich Schumann
Atmos. Chem. Phys., 18, 16729–16745, https://doi.org/10.5194/acp-18-16729-2018, https://doi.org/10.5194/acp-18-16729-2018, 2018
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We present an intercomparison of the airborne water vapor measurements during the ML-CIRRUS mission. Although the agreement of the hygrometers significantly improved compared to studies from recent decades, systematic differences remain under specific meteorological conditions. We compare the measurements to model data, where we observe a model wet bias in the lower stratosphere close to the tropopause, likely caused by a blurred humidity gradient in the model tropopause.
Jack G. Porter, Warren De Bruyn, and Eric S. Saltzman
Atmos. Chem. Phys., 18, 15291–15305, https://doi.org/10.5194/acp-18-15291-2018, https://doi.org/10.5194/acp-18-15291-2018, 2018
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Deposition to the sea surface is a major loss pathway for highly soluble atmospheric trace gases. These fluxes are important to biogeochemical cycles, climate, and air quality. Here we report measurements of air–sea fluxes of sulfur dioxide, sensible heat, and momentum to coastal waters. Transfer velocities derived from the data show a dependence on molecular diffusivity, demonstrating the importance of diffusion in the interfacial layer on the atmospheric side of the air–sea interface.
Dana R. Caulton, Qi Li, Elie Bou-Zeid, Jeffrey P. Fitts, Levi M. Golston, Da Pan, Jessica Lu, Haley M. Lane, Bernhard Buchholz, Xuehui Guo, James McSpiritt, Lars Wendt, and Mark A. Zondlo
Atmos. Chem. Phys., 18, 15145–15168, https://doi.org/10.5194/acp-18-15145-2018, https://doi.org/10.5194/acp-18-15145-2018, 2018
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Mobile laboratory measurements have been widely used to quantify methane emissions from point sources such as oil and gas wells, but the emission uncertainties are poorly constrained. We designed a hierarchical measurement strategy to sample natural gas emissions in the Marcellus Shale play based upon high-resolution modeling of select sites. Our study quantifies the largest sources of error with this approach and provides guidance on how to best implement mobile laboratory sampling protocols.
Alexis A. Shusterman, Jinsol Kim, Kaitlyn J. Lieschke, Catherine Newman, Paul J. Wooldridge, and Ronald C. Cohen
Atmos. Chem. Phys., 18, 13773–13785, https://doi.org/10.5194/acp-18-13773-2018, https://doi.org/10.5194/acp-18-13773-2018, 2018
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We describe the diversity and heterogeneity of urban CO2 levels observed using the BErkeley Atmospheric CO2 Observation Network, a distributed instrument of > 50 CO2 sensors stationed every ~ 2 km across the San Francisco Bay Area. We demonstrate that relatively simple mathematical techniques, applied to these observations, can be used to detect the small changes in highway CO2 emissions expected to result from upcoming fuel economy regulations, affirming the policy relevance of low-cost sensors.
Mengyao Liu, Jintai Lin, Yuchen Wang, Yang Sun, Bo Zheng, Jingyuan Shao, Lulu Chen, Yixuan Zheng, Jinxuan Chen, Tzung-May Fu, Yingying Yan, Qiang Zhang, and Zhaohua Wu
Atmos. Chem. Phys., 18, 12933–12952, https://doi.org/10.5194/acp-18-12933-2018, https://doi.org/10.5194/acp-18-12933-2018, 2018
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Eastern China is heavily polluted by NO2, PM2.5, and other air pollutants. Our study uses EOF–EEMD to analyze the spatiotemporal variability of ground-level NO2, PM2.5, and their associations with meteorological processes. Their regular diurnal cycles are mainly affected by human activities, while irregular day-to-day variations are dominated by weather processes representing synchronous variation or north–south opposing changes over Eastern China.
Wen Xu, Lei Liu, Miaomiao Cheng, Yuanhong Zhao, Lin Zhang, Yuepeng Pan, Xiuming Zhang, Baojing Gu, Yi Li, Xiuying Zhang, Jianlin Shen, Li Lu, Xiaosheng Luo, Yu Zhao, Zhaozhong Feng, Jeffrey L. Collett Jr., Fusuo Zhang, and Xuejun Liu
Atmos. Chem. Phys., 18, 10931–10954, https://doi.org/10.5194/acp-18-10931-2018, https://doi.org/10.5194/acp-18-10931-2018, 2018
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Our main results demonstrate that atmospheric Nr pollution in eastern China is more serious in the northern region than in the southern region. Any effects of current emission controls are not yet apparent in Nr pollution. NH3 emissions from fertilizer use were the largest contributor (36 %) to total inorganic Nr deposition. Our results provide useful information for policy-makers that mitigation of NH3 emissions should be a priority to tackle serious N deposition.
Xavier Querol, Andrés Alastuey, Gotzon Gangoiti, Noemí Perez, Hong K. Lee, Heeram R. Eun, Yonghee Park, Enrique Mantilla, Miguel Escudero, Gloria Titos, Lucio Alonso, Brice Temime-Roussel, Nicolas Marchand, Juan R. Moreta, M. Arantxa Revuelta, Pedro Salvador, Begoña Artíñano, Saúl García dos Santos, Mónica Anguas, Alberto Notario, Alfonso Saiz-Lopez, Roy M. Harrison, Millán Millán, and Kang-Ho Ahn
Atmos. Chem. Phys., 18, 6511–6533, https://doi.org/10.5194/acp-18-6511-2018, https://doi.org/10.5194/acp-18-6511-2018, 2018
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We show the main drivers of high O3 episodes in and around Madrid. High levels of ultrafine particles (UFPs) are evidenced, but we demonstrate that most O3 arises from the fumigation of high atmospheric layers, whereas UFPs are generated inside the PBL. O3 contributions from the fumigation of the vertical recirculation of regional air masses, hemispheric transport, and horizontally from direct urban plume transport are shown. Complexity arises from the need to quantify them to abate surface O3.
Qianqian Hong, Cheng Liu, Ka Lok Chan, Qihou Hu, Zhouqing Xie, Haoran Liu, Fuqi Si, and Jianguo Liu
Atmos. Chem. Phys., 18, 5931–5951, https://doi.org/10.5194/acp-18-5931-2018, https://doi.org/10.5194/acp-18-5931-2018, 2018
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We presented ship-based MAX-DOAS measurements of tropospheric trace gases' distribution along the eastern part of the Yangtze River during winter 2015. Tropospheric VCDs of NO2, SO2, and HCHO were retrieved from MAX-DOAS measurement spectra. Enhanced tropospheric NO2 and SO2 VCDs were detected over downwind areas of industrial zones over the Yangtze River. Our results indicate that different pollution control strategies should be applied in different provinces.
Murray J. Smith, Carolyn F. Walker, Thomas G. Bell, Mike J. Harvey, Eric S. Saltzman, and Cliff S. Law
Atmos. Chem. Phys., 18, 5861–5877, https://doi.org/10.5194/acp-18-5861-2018, https://doi.org/10.5194/acp-18-5861-2018, 2018
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The transfer of gases across the air–sea interface has a significant influence on climate. During a research voyage in the South Pacific we measured the transfer rate of the biogenic gas dimethyl sulfide (DMS) from the ocean using two independent methods. The agreement between the techniques provides confidence in their use in compilations of global gas transfer. We also identified physical conditions under which the observations are not well predicted by a standard gas transfer model.
Geoffrey C. Toon, Jean-Francois L. Blavier, and Keeyoon Sung
Atmos. Chem. Phys., 18, 5075–5088, https://doi.org/10.5194/acp-18-5075-2018, https://doi.org/10.5194/acp-18-5075-2018, 2018
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Remote sensing measurements of ethene have been made from the ground and from balloons. Ethene can be measured at low altitudes in polluted regions, such as the Los Angeles basin. Here ethene amounts have decreased by a factor of 3 over the past 25 years due to increasingly strict emission control regulations (e.g., on vehicle exhaust).
Hao Wang, Xiaopu Lyu, Hai Guo, Yu Wang, Shichun Zou, Zhenhao Ling, Xinming Wang, Fei Jiang, Yangzong Zeren, Wenzhuo Pan, Xiaobo Huang, and Jin Shen
Atmos. Chem. Phys., 18, 4277–4295, https://doi.org/10.5194/acp-18-4277-2018, https://doi.org/10.5194/acp-18-4277-2018, 2018
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While oceanic air is generally thought to be clean, the air pollution over waters in proximity to the coasts is not well recognized. This research indicated that ozone was higher over South China Sea (SCS) than that in the adjacent continental area, while continental anticyclone, tropical cyclone and land breeze favored O3 formation over SCS. In addition, weaker NO titration and stronger atmospheric oxidative capacity led to higher O3 production efficiency over SCS.
Fabian Schoenenberger, Stephan Henne, Matthias Hill, Martin K. Vollmer, Giorgos Kouvarakis, Nikolaos Mihalopoulos, Simon O'Doherty, Michela Maione, Lukas Emmenegger, Thomas Peter, and Stefan Reimann
Atmos. Chem. Phys., 18, 4069–4092, https://doi.org/10.5194/acp-18-4069-2018, https://doi.org/10.5194/acp-18-4069-2018, 2018
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Anthropogenic halocarbon emissions contribute to stratospheric ozone depletion and global warming. We measured atmospheric halocarbons for 6 months on Crete to extend the coverage of the existing observation network to the Eastern Mediterranean. The derived emission estimates showed a contribution of 16.8 % (13.6–23.3 %) and 53.2 % (38.1–84.2 %) of this region to the total HFC and HCFC emissions of the analyzed European domain and a reduction of the underlying uncertainties by 40–80 %.
Irène Xueref-Remy, Elsa Dieudonné, Cyrille Vuillemin, Morgan Lopez, Christine Lac, Martina Schmidt, Marc Delmotte, Frédéric Chevallier, François Ravetta, Olivier Perrussel, Philippe Ciais, François-Marie Bréon, Grégoire Broquet, Michel Ramonet, T. Gerard Spain, and Christophe Ampe
Atmos. Chem. Phys., 18, 3335–3362, https://doi.org/10.5194/acp-18-3335-2018, https://doi.org/10.5194/acp-18-3335-2018, 2018
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Urbanized and industrialized areas are the largest source of fossil CO2. This work analyses the atmospheric CO2 variability observed from the first in situ network deployed in the Paris megacity area. Gradients of several ppm are found between the rural, peri-urban and urban sites at the diurnal to the seasonal scales. Wind direction and speed as well as boundary layer dynamics, correlated to highly variable urban emissions, are shown to be key regulator factors of the observed CO2 records.
Geoffrey C. Toon, Jean-Francois L. Blavier, and Keeyoon Sung
Atmos. Chem. Phys., 18, 1923–1944, https://doi.org/10.5194/acp-18-1923-2018, https://doi.org/10.5194/acp-18-1923-2018, 2018
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OCS is the main form of atmospheric sulfur. It is produced near the earth's surface and destroyed primarily in the stratosphere, where it is converted to stratospheric sulfate aerosol (SSA). SSA plays an important role in atmospheric chemistry and transport and so it is important to better understand the factors that regulate OCS and hence SSA. Ground-based and balloon-borne infrared spectra observed over the past 30 years are analyzed to provide an improved OCS dataset.
Simon Schallhart, Pekka Rantala, Maija K. Kajos, Juho Aalto, Ivan Mammarella, Taina M. Ruuskanen, and Markku Kulmala
Atmos. Chem. Phys., 18, 815–832, https://doi.org/10.5194/acp-18-815-2018, https://doi.org/10.5194/acp-18-815-2018, 2018
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Emissions of volatile organic compounds (VOCs) have impact to air quality, human health and climate. We investigated the development of VOC exchange in a boreal forest between April and June 2013. VOC exchange and diversity increased towards summer, but over 75 % of the biogenic net exchange was driven by methanol, monoterpenes and acetone only. The boreal forest emitted less than 0.2 % carbon in form of VOCs in relation to the carbon uptake.
Wanyun Xu, Xiaobin Xu, Meiyun Lin, Weili Lin, David Tarasick, Jie Tang, Jianzhong Ma, and Xiangdong Zheng
Atmos. Chem. Phys., 18, 773–798, https://doi.org/10.5194/acp-18-773-2018, https://doi.org/10.5194/acp-18-773-2018, 2018
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The impact of anthropogenic emissions and climate variability on the long-term trends and periodicity of surface ozone measured at Mt Waliguan (WLG) for the period of 1994–2013 is studied. STT ozone and rising emissions in eastern China contribute to spring and autumnal increasing trends, respectively. The 2–3-, 3–7-, and 11-year periodicities in the ozone data are linked to the QBO, EASMI, and sunspot cycle, respectively. An empirical model is obtained for normalised monthly ozone at WLG.
Qian Yu, Yao Luo, Shuxiao Wang, Zhiqi Wang, Jiming Hao, and Lei Duan
Atmos. Chem. Phys., 18, 495–509, https://doi.org/10.5194/acp-18-495-2018, https://doi.org/10.5194/acp-18-495-2018, 2018
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This study provides high-quality direct observation data of a clean and a contaminated site in subtropical south China and quantifies the natural forest Hg emission. We find that clean and contaminated forests present a net GEM source with annual average values of 6.67 and 0.30 ng m-2 h-1, respectively; daily variations of GEM fluxes showed a source in the daytime with a peak at 13:00, and as a sink or balance at night; and higher atmospheric GEM concentration restricted the forest GEM emission.
Xuemeng Chen, Lauriane L. J. Quéléver, Pak L. Fung, Jutta Kesti, Matti P. Rissanen, Jaana Bäck, Petri Keronen, Heikki Junninen, Tuukka Petäjä, Veli-Matti Kerminen, and Markku Kulmala
Atmos. Chem. Phys., 18, 49–63, https://doi.org/10.5194/acp-18-49-2018, https://doi.org/10.5194/acp-18-49-2018, 2018
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We analysed a 20-year-long dataset collected in a Finnish boreal forest at SMEAR II station to investigate the frequency and strength of ozone depletion events. We could identify a number of ozone depletion events that lasted for more than 3 h, mainly in the autumn and winter months. Their occurrence was likely related to the formation of a low mixing layer under the conditions of low temperatures, low wind speeds, high relative humidities and limited intensity of solar radiation.
Emmaline Atherton, David Risk, Chelsea Fougère, Martin Lavoie, Alex Marshall, John Werring, James P. Williams, and Christina Minions
Atmos. Chem. Phys., 17, 12405–12420, https://doi.org/10.5194/acp-17-12405-2017, https://doi.org/10.5194/acp-17-12405-2017, 2017
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Methane is a potent greenhouse gas, and leaks from natural gas infrastructure are thought to be a significant emission source. We used a mobile survey method to measure GHGs near Canadian infrastructure. Our results show that ~ 47 % of active wells were emitting. Abandoned and aging wells were also associated with emissions. We estimate methane emissions from this development are just over 111 Mt year−1, which is more than previous government estimates, but less than similar studies in the US.
Huiting Mao, Dolly Hall, Zhuyun Ye, Ying Zhou, Dirk Felton, and Leiming Zhang
Atmos. Chem. Phys., 17, 11655–11671, https://doi.org/10.5194/acp-17-11655-2017, https://doi.org/10.5194/acp-17-11655-2017, 2017
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