Articles | Volume 23, issue 12
https://doi.org/10.5194/acp-23-6963-2023
https://doi.org/10.5194/acp-23-6963-2023
Research article
 | 
23 Jun 2023
Research article |  | 23 Jun 2023

A 1-year aerosol chemical speciation monitor (ACSM) source analysis of organic aerosol particle contributions from anthropogenic sources after long-range transport at the TROPOS research station Melpitz

Samira Atabakhsh, Laurent Poulain, Gang Chen, Francesco Canonaco, André S. H. Prévôt, Mira Pöhlker, Alfred Wiedensohler, and Hartmut Herrmann

Related authors

Microphysical properties of refractory black carbon aerosols for different air masses at a central European background site
Yifan Yang, Thomas Müller, Laurent Poulain, Samira Atabakhsh, Bruna A. Holanda, Jens Voigtländer, Shubhi Arora, and Mira L. Pöhlker
EGUsphere, https://doi.org/10.5194/egusphere-2024-3539,https://doi.org/10.5194/egusphere-2024-3539, 2024
Short summary

Related subject area

Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Multiple eco-regions contribute to the seasonal cycle of Antarctic aerosol size distributions
James Brean, David C. S. Beddows, Eija Asmi, Aki Virkkula, Lauriane L. J. Quéléver, Mikko Sipilä, Floortje Van Den Heuvel, Thomas Lachlan-Cope, Anna Jones, Markus Frey, Angelo Lupi, Jiyeon Park, Young Jun Yoon, Rolf Weller, Giselle L. Marincovich, Gabriela C. Mulena, Roy M. Harrison, and Manuel Dall'Osto
Atmos. Chem. Phys., 25, 1145–1162, https://doi.org/10.5194/acp-25-1145-2025,https://doi.org/10.5194/acp-25-1145-2025, 2025
Short summary
Seasonal investigation of ultrafine-particle organic composition in an eastern Amazonian rainforest
Adam E. Thomas, Hayley S. Glicker, Alex B. Guenther, Roger Seco, Oscar Vega Bustillos, Julio Tota, Rodrigo A. F. Souza, and James N. Smith
Atmos. Chem. Phys., 25, 959–977, https://doi.org/10.5194/acp-25-959-2025,https://doi.org/10.5194/acp-25-959-2025, 2025
Short summary
High-resolution analyses of concentrations and sizes of refractory black carbon particles deposited in northwestern Greenland over the past 350 years – Part 2: Seasonal and temporal trends in refractory black carbon originated from fossil fuel combustion and biomass burning
Kumiko Goto-Azuma, Yoshimi Ogawa-Tsukagawa, Kaori Fukuda, Koji Fujita, Motohiro Hirabayashi, Remi Dallmayr, Jun Ogata, Nobuhiro Moteki, Tatsuhiro Mori, Sho Ohata, Yutaka Kondo, Makoto Koike, Sumito Matoba, Moe Kadota, Akane Tsushima, Naoko Nagatsuka, and Teruo Aoki
Atmos. Chem. Phys., 25, 657–683, https://doi.org/10.5194/acp-25-657-2025,https://doi.org/10.5194/acp-25-657-2025, 2025
Short summary
Significant role of biomass burning in heavy haze formation in Nanjing, a megacity in China: molecular-level insights from intensive PM2.5 sampling on winter hazy days
Mingjie Kang, Mengying Bao, Wenhuai Song, Aduburexiati Abulimiti, Changliu Wu, Fang Cao, Sönke Szidat, and Yanlin Zhang
Atmos. Chem. Phys., 25, 73–91, https://doi.org/10.5194/acp-25-73-2025,https://doi.org/10.5194/acp-25-73-2025, 2025
Short summary
Widespread trace bromine and iodine in remote tropospheric non-sea-salt aerosols
Gregory P. Schill, Karl D. Froyd, Daniel M. Murphy, Christina J. Williamson, Charles A. Brock, Tomás Sherwen, Mat J. Evans, Eric A. Ray, Eric C. Apel, Rebecca S. Hornbrook, Alan J. Hills, Jeff Peischl, Thomas B. Ryerson, Chelsea R. Thompson, Ilann Bourgeois, Donald R. Blake, Joshua P. DiGangi, and Glenn S. Diskin
Atmos. Chem. Phys., 25, 45–71, https://doi.org/10.5194/acp-25-45-2025,https://doi.org/10.5194/acp-25-45-2025, 2025
Short summary

Cited articles

Alfarra, M. R., Prevot, A. S. H., Szidat, S., Sandradewi, J., Weimer, S., Lanz, V. A., Schreiber, D., Mohr, M., and Baltensperger, U.: Identification of the mass spectral signature of organic aerosols from wood burning emissions, Environ. Sci. Technol., 41, 5770–5777, https://doi.org/10.1021/es062289b, 2007. 
Allan, J. D., Delia, A. E., Coe, H., Bower, K. N., Alfarra, M. R., Jimenez, J. L., Middlebrook, A. M., Drewnick, F., Onasch, T. B., Canagaratna, M. R., Jayne, J. T., and Worsnop, D. R.: A generalised method for the extraction of chemically resolved mass spectra from Aerodyne aerosol mass spectrometer data, J. Aerosol Sci., 35, 909–922, https://doi.org/10.1016/j.jaerosci.2004.02.007, 2004. 
Birmili, W., Stratmann, F., and Wiedensohler, A.: Technical note design of a DMA-based size spectrometer for a large particle size range and stable operation, J. Aerosol Sci., 30, 549–553, https://doi.org/10.1016/S0021-8502(98)00047-0, 1999. 
Birmili, W., Wiedensohler, A., Mueller, K., Birmili, W., Weinhold, K., Nordmann, S., Wiedensohler, A., Spindler, G., Müller, K., Herrmann, H., Gnauk, T., Pitz, M., Cyrys, J., Flentje, H., Nickel, C., J Kuhlbusch, T. A., Löschau, G., Haase, D., Meinhardt, F., F., Schwerin, A., Ries, L., and Wirtz, K.: Atmospheric aerosol measurements in the German Ultrafine Aerosol Network (GUAN) Korngrößendifferenzierte Feinstaubbelastung in Straßennähe in Ballungsgebieten Sachsens (2003–2005) View project Chemistry, Air Quality and Climate View project Atmospheric aerosol measurements in the German Ultrafine Aerosol Network (GUAN) Part 1: Soot and particle number size distributions, https://www.researchgate.net/publication/232089057 (last access: 21 March 2023), 2009. 
Download
Short summary
The study focuses on the aerosol chemical variations found in the rural-background station of Melpitz based on ACSM and MAAP measurements. Source apportionment on both organic aerosol (OA) and black carbon (eBC) was performed, and source seasonality was also linked to air mass trajectories. Overall, three anthropogenic sources were identified in OA and eBC plus two additional aged OA. Our results demonstrate the influence of transported coal-combustion-related OA even during summer time.
Share
Altmetrics
Final-revised paper
Preprint