Articles | Volume 23, issue 3
https://doi.org/10.5194/acp-23-1941-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-1941-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
06 Feb 2023
Research article |
| 06 Feb 2023
| 06 Feb 2023
Observations of microphysical properties and radiative effects of a contrail cirrus outbreak over the North Atlantic
Institute of Atmospheric Physics, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 82234 Oberpfaffenhofen, Germany
Meteorological Institute, Ludwig Maximilian University of Munich, 80333 Munich, Germany
Institute of Atmospheric Physics, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 82234 Oberpfaffenhofen, Germany
Tina Jurkat-Witschas
Institute of Atmospheric Physics, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 82234 Oberpfaffenhofen, Germany
Romy Heller
Institute of Atmospheric Physics, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 82234 Oberpfaffenhofen, Germany
Ulrike Burkhardt
Institute of Atmospheric Physics, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 82234 Oberpfaffenhofen, Germany
Helmut Ziereis
Institute of Atmospheric Physics, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 82234 Oberpfaffenhofen, Germany
Georgios Dekoutsidis
Institute of Atmospheric Physics, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 82234 Oberpfaffenhofen, Germany
Martin Wirth
Institute of Atmospheric Physics, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 82234 Oberpfaffenhofen, Germany
Silke Groß
Institute of Atmospheric Physics, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 82234 Oberpfaffenhofen, Germany
Simon Kirschler
Institute of Atmospheric Physics, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 82234 Oberpfaffenhofen, Germany
Institute of Atmospheric Physics, Johannes Gutenberg University Mainz, 55128 Mainz, Germany
Stefan Kaufmann
Institute of Atmospheric Physics, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 82234 Oberpfaffenhofen, Germany
Christiane Voigt
Institute of Atmospheric Physics, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 82234 Oberpfaffenhofen, Germany
Institute of Atmospheric Physics, Johannes Gutenberg University Mainz, 55128 Mainz, Germany
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Ziming Wang, Luca Bugliaro, Klaus Gierens, Michaela I. Hegglin, Susanne Rohs, Andreas Petzold, Stefan Kaufmann, and Christiane Voigt
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Ziming Wang, Husi Letu, Huazhe Shang, and Luca Bugliaro
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Philipp Joppe, Johannes Schneider, Katharina Kaiser, Horst Fischer, Peter Hoor, Daniel Kunkel, Hans-Christoph Lachnitt, Andreas Marsing, Lenard Röder, Hans Schlager, Laura Tomsche, Christiane Voigt, Andreas Zahn, and Stephan Borrmann
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Clémantyne Aubry, Julien Delanoë, Silke Groß, Florian Ewald, Frédéric Tridon, Olivier Jourdan, and Guillaume Mioche
Atmos. Meas. Tech., 17, 3863–3881, https://doi.org/10.5194/amt-17-3863-2024, https://doi.org/10.5194/amt-17-3863-2024, 2024
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Roger Teoh, Zebediah Engberg, Ulrich Schumann, Christiane Voigt, Marc Shapiro, Susanne Rohs, and Marc E. J. Stettler
Atmos. Chem. Phys., 24, 6071–6093, https://doi.org/10.5194/acp-24-6071-2024, https://doi.org/10.5194/acp-24-6071-2024, 2024
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The radiative forcing (RF) due to aviation contrails is comparable to that caused by CO2. We estimate that global contrail net RF in 2019 was 62.1 mW m−2. This is ~1/2 the previous best estimate for 2018. Contrail RF varies regionally due to differences in conditions required for persistent contrails. COVID-19 reduced contrail RF by 54% in 2020 relative to 2019. Globally, 2 % of all flights account for 80 % of the annual contrail energy forcing, suggesting a opportunity to mitigate contrail RF.
Georgios Dekoutsidis, Martin Wirth, and Silke Groß
Atmos. Chem. Phys., 24, 5971–5987, https://doi.org/10.5194/acp-24-5971-2024, https://doi.org/10.5194/acp-24-5971-2024, 2024
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For decades the earth's temperature has been rising. The Arctic regions are warming faster. Cirrus clouds can contribute to this phenomenon. During warm-air intrusions, air masses are transported into the Arctic from the mid-latitudes. The HALO-(AC)3 campaign took place to measure cirrus during intrusion events and under normal conditions. We study the two cloud types based on these measurements and find differences in their geometry, relative humidity distribution and vertical structure.
Nina Maherndl, Manuel Moser, Imke Schirmacher, Aaron Bansemer, Johannes Lucke, Christiane Voigt, and Maximilian Maahn
EGUsphere, https://doi.org/10.5194/egusphere-2024-1214, https://doi.org/10.5194/egusphere-2024-1214, 2024
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Raphael Satoru Märkl, Christiane Voigt, Daniel Sauer, Rebecca Katharina Dischl, Stefan Kaufmann, Theresa Harlaß, Valerian Hahn, Anke Roiger, Cornelius Weiß-Rehm, Ulrike Burkhardt, Ulrich Schumann, Andreas Marsing, Monika Scheibe, Andreas Dörnbrack, Charles Renard, Maxime Gauthier, Peter Swann, Paul Madden, Darren Luff, Reetu Sallinen, Tobias Schripp, and Patrick Le Clercq
Atmos. Chem. Phys., 24, 3813–3837, https://doi.org/10.5194/acp-24-3813-2024, https://doi.org/10.5194/acp-24-3813-2024, 2024
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In situ measurements of contrails from a large passenger aircraft burning 100 % sustainable aviation fuel (SAF) show a 56 % reduction in contrail ice crystal numbers compared to conventional Jet A-1. Results from a climate model initialized with the observations suggest a significant decrease in radiative forcing from contrails. Our study confirms that future increased use of low aromatic SAF can reduce the climate impact from aviation.
Robert Hanfland, Dominik Brunner, Christiane Voigt, Alina Fiehn, Anke Roiger, and Margit Pattantyús-Ábrahám
Atmos. Chem. Phys., 24, 2511–2534, https://doi.org/10.5194/acp-24-2511-2024, https://doi.org/10.5194/acp-24-2511-2024, 2024
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To show that the three-dimensional dispersion of plumes simulated by the Atmospheric Radionuclide Transport Model within the planetary boundary layer agrees with real plumes, we identify the most important input parameters and analyse the turbulence properties of five different turbulence models in very unstable stratification conditions using their deviation from the well-mixed state. Simulations show that one model agrees slightly better in unstable stratification conditions.
Andreas Bier, Simon Unterstrasser, Josef Zink, Dennis Hillenbrand, Tina Jurkat-Witschas, and Annemarie Lottermoser
Atmos. Chem. Phys., 24, 2319–2344, https://doi.org/10.5194/acp-24-2319-2024, https://doi.org/10.5194/acp-24-2319-2024, 2024
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Using hydrogen as aviation fuel affects contrails' climate impact. We study contrail formation behind aircraft with H2 combustion. Due to the absence of soot emissions, contrail ice crystals are assumed to form only on ambient particles mixed into the plume. The ice crystal number, which strongly varies with temperature and aerosol number density, is decreased by more than 80 %–90 % compared to kerosene contrails. However H2 contrails can form at lower altitudes due to higher H2O emissions.
Silke Groß, Volker Freudenthaler, Moritz Haarig, Albert Ansmann, Carlos Toledano, David Mateos, Petra Seibert, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Josef Gasteiger, Maximilian Dollner, Anne Tipka, Manuel Schöberl, Marilena Teri, and Bernadett Weinzierl
EGUsphere, https://doi.org/10.5194/egusphere-2024-140, https://doi.org/10.5194/egusphere-2024-140, 2024
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Aerosols contribute to the largest uncertainties in climate change predictions. Especially absorbing aerosols propose difficulties in our understanding. The eastern Mediterranean is a hot spot for aerosols with natural and anthropogenic contributions. We present lidar measurements performed during the A-LIFE field experiment to characterize aerosols and aerosol mixtures. We extend current classification and separation schemes and compare different classification schemes.
Marcus Klingebiel, André Ehrlich, Elena Ruiz-Donoso, Nils Risse, Imke Schirmacher, Evelyn Jäkel, Michael Schäfer, Kevin Wolf, Mario Mech, Manuel Moser, Christiane Voigt, and Manfred Wendisch
Atmos. Chem. Phys., 23, 15289–15304, https://doi.org/10.5194/acp-23-15289-2023, https://doi.org/10.5194/acp-23-15289-2023, 2023
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In this study we explain how we use aircraft measurements from two Arctic research campaigns to identify cloud properties (like droplet size) over sea-ice and ice-free ocean. To make sure that our measurements make sense, we compare them with other observations. Our results show, e.g., larger cloud droplets in early summer than in spring. Moreover, the cloud droplets are also larger over ice-free ocean than compared to sea ice. In the future, our data can be used to improve climate models.
Yann Cohen, Didier Hauglustaine, Bastien Sauvage, Susanne Rohs, Patrick Konjari, Ulrich Bundke, Andreas Petzold, Valérie Thouret, Andreas Zahn, and Helmut Ziereis
Atmos. Chem. Phys., 23, 14973–15009, https://doi.org/10.5194/acp-23-14973-2023, https://doi.org/10.5194/acp-23-14973-2023, 2023
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The upper troposphere–lower stratosphere (UTLS) is a key region regarding the lower atmospheric composition. This study consists of a comprehensive evaluation of an up-to-date chemistry–climate model in this layer, using regular in situ measurements based on passenger aircraft. For this purpose, a specific software (Interpol-IAGOS) has been updated and made publicly available. The model reproduces the carbon monoxide peaks due to biomass burning over the continental tropics particularly well.
Elena De La Torre Castro, Tina Jurkat-Witschas, Armin Afchine, Volker Grewe, Valerian Hahn, Simon Kirschler, Martina Krämer, Johannes Lucke, Nicole Spelten, Heini Wernli, Martin Zöger, and Christiane Voigt
Atmos. Chem. Phys., 23, 13167–13189, https://doi.org/10.5194/acp-23-13167-2023, https://doi.org/10.5194/acp-23-13167-2023, 2023
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In this study, we show the differences in the microphysical properties between high-latitude (HL) cirrus and mid-latitude (ML) cirrus over the Arctic, North Atlantic, and central Europe during summer. The in situ measurements are combined with backward trajectories to investigate the influence of the region on cloud formation. We show that HL cirrus are characterized by a lower concentration of larger ice crystals when compared to ML cirrus.
Simon Kirschler, Christiane Voigt, Bruce E. Anderson, Gao Chen, Ewan C. Crosbie, Richard A. Ferrare, Valerian Hahn, Johnathan W. Hair, Stefan Kaufmann, Richard H. Moore, David Painemal, Claire E. Robinson, Kevin J. Sanchez, Amy J. Scarino, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Edward L. Winstead, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 23, 10731–10750, https://doi.org/10.5194/acp-23-10731-2023, https://doi.org/10.5194/acp-23-10731-2023, 2023
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In this study we present an overview of liquid and mixed-phase clouds and precipitation in the marine boundary layer over the western North Atlantic Ocean. We compare microphysical properties of pure liquid clouds to mixed-phase clouds and show that the initiation of the ice phase in mixed-phase clouds promotes precipitation. The observational data presented in this study are well suited for investigating the processes that give rise to liquid and mixed-phase clouds, ice, and precipitation.
Armin Sorooshian, Mikhail D. Alexandrov, Adam D. Bell, Ryan Bennett, Grace Betito, Sharon P. Burton, Megan E. Buzanowicz, Brian Cairns, Eduard V. Chemyakin, Gao Chen, Yonghoon Choi, Brian L. Collister, Anthony L. Cook, Andrea F. Corral, Ewan C. Crosbie, Bastiaan van Diedenhoven, Joshua P. DiGangi, Glenn S. Diskin, Sanja Dmitrovic, Eva-Lou Edwards, Marta A. Fenn, Richard A. Ferrare, David van Gilst, Johnathan W. Hair, David B. Harper, Miguel Ricardo A. Hilario, Chris A. Hostetler, Nathan Jester, Michael Jones, Simon Kirschler, Mary M. Kleb, John M. Kusterer, Sean Leavor, Joseph W. Lee, Hongyu Liu, Kayla McCauley, Richard H. Moore, Joseph Nied, Anthony Notari, John B. Nowak, David Painemal, Kasey E. Phillips, Claire E. Robinson, Amy Jo Scarino, Joseph S. Schlosser, Shane T. Seaman, Chellappan Seethala, Taylor J. Shingler, Michael A. Shook, Kenneth A. Sinclair, William L. Smith Jr., Douglas A. Spangenberg, Snorre A. Stamnes, Kenneth L. Thornhill, Christiane Voigt, Holger Vömel, Andrzej P. Wasilewski, Hailong Wang, Edward L. Winstead, Kira Zeider, Xubin Zeng, Bo Zhang, Luke D. Ziemba, and Paquita Zuidema
Earth Syst. Sci. Data, 15, 3419–3472, https://doi.org/10.5194/essd-15-3419-2023, https://doi.org/10.5194/essd-15-3419-2023, 2023
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The NASA Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) produced a unique dataset for research into aerosol–cloud–meteorology interactions. HU-25 Falcon and King Air aircraft conducted systematic and spatially coordinated flights over the northwest Atlantic Ocean. This paper describes the ACTIVATE flight strategy, instrument and complementary dataset products, data access and usage details, and data application notes.
Valerian Hahn, Ralf Meerkötter, Christiane Voigt, Sonja Gisinger, Daniel Sauer, Valéry Catoire, Volker Dreiling, Hugh Coe, Cyrille Flamant, Stefan Kaufmann, Jonas Kleine, Peter Knippertz, Manuel Moser, Philip Rosenberg, Hans Schlager, Alfons Schwarzenboeck, and Jonathan Taylor
Atmos. Chem. Phys., 23, 8515–8530, https://doi.org/10.5194/acp-23-8515-2023, https://doi.org/10.5194/acp-23-8515-2023, 2023
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During the DACCIWA campaign in West Africa, we found a 35 % increase in the cloud droplet concentration that formed in a polluted compared with a less polluted environment and a decrease of 17 % in effective droplet diameter. Radiative transfer simulations, based on the measured cloud properties, reveal that these low-level polluted clouds radiate only 2.6 % more energy back to space, compared with a less polluted cloud. The corresponding additional decrease in temperature is rather small.
Silke Groß, Tina Jurkat-Witschas, Qiang Li, Martin Wirth, Benedikt Urbanek, Martina Krämer, Ralf Weigel, and Christiane Voigt
Atmos. Chem. Phys., 23, 8369–8381, https://doi.org/10.5194/acp-23-8369-2023, https://doi.org/10.5194/acp-23-8369-2023, 2023
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Aviation-emitted aerosol can have an impact on cirrus clouds. We present optical and microphysical properties of mid-latitude cirrus clouds which were formed under the influence of aviation-emitted aerosol or which were formed under rather pristine conditions. We find that cirrus clouds affected by aviation-emitted aerosol show larger values of the particle linear depolarization ratio, larger mean effective ice particle diameters and decreased ice particle number concentrations.
Midhun George, Maria Dolores Andrés Hernández, Vladyslav Nenakhov, Yangzhuoran Liu, John Philip Burrows, Birger Bohn, Eric Förster, Florian Obersteiner, Andreas Zahn, Theresa Harlaß, Helmut Ziereis, Hans Schlager, Benjamin Schreiner, Flora Kluge, Katja Bigge, and Klaus Pfeilsticker
Atmos. Chem. Phys., 23, 7799–7822, https://doi.org/10.5194/acp-23-7799-2023, https://doi.org/10.5194/acp-23-7799-2023, 2023
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The applicability of photostationary steady-state (PSS) assumptions to estimate the amount of the sum of peroxy radicals (RO2*) during the EMeRGe airborne observations from the known radical chemistry and onboard measurements of RO2* precursors, photolysis frequencies, and other trace gases such as NOx and O3 was investigated. The comparison of the calculated RO2* with the actual measurements provides an insight into the main processes controlling their concentration in the air masses measured.
Markus Kilian, Volker Grewe, Patrick Jöckel, Astrid Kerkweg, Mariano Mertens, Andreas Zahn, and Helmut Ziereis
EGUsphere, https://doi.org/10.5194/egusphere-2023-528, https://doi.org/10.5194/egusphere-2023-528, 2023
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Anthropogenic emissions are a major source of precursors for tropospheric ozone formation. As ozone formation is highly non-linear, we apply a global-regional chemistry-climate model with a source attribution method (tagging) to quantify the contribution of anthropogenic emissions to ozone. We focus on two major polluted areas in Europe, the Po Valley and the Benelux region. Our analysis shows that in particular anthropogenic emissions from Europe contribute largely to ground-level ozone.
Manuel Moser, Christiane Voigt, Tina Jurkat-Witschas, Valerian Hahn, Guillaume Mioche, Olivier Jourdan, Régis Dupuy, Christophe Gourbeyre, Alfons Schwarzenboeck, Johannes Lucke, Yvonne Boose, Mario Mech, Stephan Borrmann, André Ehrlich, Andreas Herber, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys., 23, 7257–7280, https://doi.org/10.5194/acp-23-7257-2023, https://doi.org/10.5194/acp-23-7257-2023, 2023
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This study provides a comprehensive microphysical and thermodynamic phase analysis of low-level clouds in the northern Fram Strait, above the sea ice and the open ocean, during spring and summer. Using airborne in situ cloud data, we show that the properties of Arctic low-level clouds vary significantly with seasonal meteorological situations and surface conditions. The observations presented in this study can help one to assess the role of clouds in the Arctic climate system.
Georgios Dekoutsidis, Silke Groß, Martin Wirth, Martina Krämer, and Christian Rolf
Atmos. Chem. Phys., 23, 3103–3117, https://doi.org/10.5194/acp-23-3103-2023, https://doi.org/10.5194/acp-23-3103-2023, 2023
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Cirrus clouds affect Earth's atmosphere, deeming our study important. Here we use water vapor measurements by lidar and study the relative humidity (RHi) within and around midlatitude cirrus clouds. We find high supersaturations in the cloud-free air and within the clouds, especially near the cloud top. We study two cloud types with different formation processes. Finally, we conclude that the shape of the distribution of RHi can be used as an indicator of different cloud evolutionary stages.
Dominik Brunner, Gerrit Kuhlmann, Stephan Henne, Erik Koene, Bastian Kern, Sebastian Wolff, Christiane Voigt, Patrick Jöckel, Christoph Kiemle, Anke Roiger, Alina Fiehn, Sven Krautwurst, Konstantin Gerilowski, Heinrich Bovensmann, Jakob Borchardt, Michal Galkowski, Christoph Gerbig, Julia Marshall, Andrzej Klonecki, Pascal Prunet, Robert Hanfland, Margit Pattantyús-Ábrahám, Andrzej Wyszogrodzki, and Andreas Fix
Atmos. Chem. Phys., 23, 2699–2728, https://doi.org/10.5194/acp-23-2699-2023, https://doi.org/10.5194/acp-23-2699-2023, 2023
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We evaluated six atmospheric transport models for their capability to simulate the CO2 plumes from two of the largest power plants in Europe by comparing the models against aircraft observations collected during the CoMet (Carbon Dioxide and Methane Mission) campaign in 2018. The study analyzed how realistically such plumes can be simulated at different model resolutions and how well the planned European satellite mission CO2M will be able to quantify emissions from power plants.
Chuan-Yao Lin, Wan-Chin Chen, Yi-Yun Chien, Charles C. K. Chou, Chian-Yi Liu, Helmut Ziereis, Hans Schlager, Eric Förster, Florian Obersteiner, Ovid O. Krüger, Bruna A. Holanda, Mira L. Pöhlker, Katharina Kaiser, Johannes Schneider, Birger Bohn, Klaus Pfeilsticker, Benjamin Weyland, Maria Dolores Andrés Hernández, and John P. Burrows
Atmos. Chem. Phys., 23, 2627–2647, https://doi.org/10.5194/acp-23-2627-2023, https://doi.org/10.5194/acp-23-2627-2023, 2023
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During the EMeRGe campaign in Asia, atmospheric pollutants were measured on board the HALO aircraft. The WRF-Chem model was employed to evaluate the biomass burning (BB) plume transported from Indochina and its impact on the downstream areas. The combination of BB aerosol enhancement with cloud water resulted in a reduction in incoming shortwave radiation at the surface in southern China and the East China Sea, which potentially has significant regional climate implications.
Yun Li, Christoph Mahnke, Susanne Rohs, Ulrich Bundke, Nicole Spelten, Georgios Dekoutsidis, Silke Groß, Christiane Voigt, Ulrich Schumann, Andreas Petzold, and Martina Krämer
Atmos. Chem. Phys., 23, 2251–2271, https://doi.org/10.5194/acp-23-2251-2023, https://doi.org/10.5194/acp-23-2251-2023, 2023
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The radiative effect of aviation-induced cirrus is closely related to ambient conditions and its microphysical properties. Our study investigated the occurrence of contrail and natural cirrus measured above central Europe in spring 2014. It finds that contrail cirrus appears frequently in the pressure range 200 to 245 hPa and occurs more often in slightly ice-subsaturated environments than expected. Avoiding slightly ice-subsaturated regions by aviation might help mitigate contrail cirrus.
Andreas Schäfler, Michael Sprenger, Heini Wernli, Andreas Fix, and Martin Wirth
Atmos. Chem. Phys., 23, 999–1018, https://doi.org/10.5194/acp-23-999-2023, https://doi.org/10.5194/acp-23-999-2023, 2023
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In this study, airborne lidar profile measurements of H2O and O3 across a midlatitude jet stream are combined with analyses in tracer–trace space and backward trajectories. We highlight that transport and mixing processes in the history of the observed air masses are governed by interacting tropospheric weather systems on synoptic timescales. We show that these weather systems play a key role in the high variability of the paired H2O and O3 distributions near the tropopause.
Andreas Marsing, Ralf Meerkötter, Romy Heller, Stefan Kaufmann, Tina Jurkat-Witschas, Martina Krämer, Christian Rolf, and Christiane Voigt
Atmos. Chem. Phys., 23, 587–609, https://doi.org/10.5194/acp-23-587-2023, https://doi.org/10.5194/acp-23-587-2023, 2023
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We employ highly resolved aircraft measurements of profiles of the ice water content (IWC) in Arctic cirrus clouds in winter and spring, when solar irradiation is low. Using radiation transfer calculations, we assess the cloud radiative effect over different surfaces like snow or ocean. The variability in the IWC of the clouds affects their overall radiative effect and drives internal processes. This helps understand the role of cirrus in a rapidly changing Arctic environment.
Johannes Lucke, Tina Jurkat-Witschas, Romy Heller, Valerian Hahn, Matthew Hamman, Wolfgang Breitfuss, Venkateshwar Reddy Bora, Manuel Moser, and Christiane Voigt
Atmos. Meas. Tech., 15, 7375–7394, https://doi.org/10.5194/amt-15-7375-2022, https://doi.org/10.5194/amt-15-7375-2022, 2022
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Flight testing in icing conditions requires instruments that are able to accurately measure the liquid water content of supercooled large droplets (SLDs). This work finds that the 12 mm cone of the Nevzorov hot-wire probe has excellent collection properties for SLDs. We also derive a correction to compensate for the low collision efficiency of small droplets with the cone. The results provide a procedure to evaluate LWC measurements of the 12 mm cone during wind tunnel and airborne experiments.
Qiang Li and Silke Groß
Atmos. Chem. Phys., 22, 15963–15980, https://doi.org/10.5194/acp-22-15963-2022, https://doi.org/10.5194/acp-22-15963-2022, 2022
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The IPCC report identified that cirrus clouds have a significant impact on the radiation balance comparable to the CO2 effects, which, however, is still hard to parameterize. The current study investigates the possible impact of aviation on cirrus properties based on the analysis of 10-year lidar measurements of CALIPSO. The results reveal that there is a significant positive trend in cirrus depolarization ratio in the last 10 years before COVID-19, which is strongly correlated with aviation.
Konstantin Krüger, Andreas Schäfler, Martin Wirth, Martin Weissmann, and George C. Craig
Atmos. Chem. Phys., 22, 15559–15577, https://doi.org/10.5194/acp-22-15559-2022, https://doi.org/10.5194/acp-22-15559-2022, 2022
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A comprehensive data set of airborne lidar water vapour profiles is compared with ERA5 reanalyses for a robust characterization of the vertical structure of the mid-latitude lower-stratospheric moist bias. We confirm a moist bias of up to 55 % at 1.3 km altitude above the tropopause and uncover a decreasing bias beyond. Collocated O3 and H2O observations reveal a particularly strong bias in the mixing layer, indicating insufficiently modelled transport processes fostering the bias.
Laura Tomsche, Andreas Marsing, Tina Jurkat-Witschas, Johannes Lucke, Stefan Kaufmann, Katharina Kaiser, Johannes Schneider, Monika Scheibe, Hans Schlager, Lenard Röder, Horst Fischer, Florian Obersteiner, Andreas Zahn, Martin Zöger, Jos Lelieveld, and Christiane Voigt
Atmos. Chem. Phys., 22, 15135–15151, https://doi.org/10.5194/acp-22-15135-2022, https://doi.org/10.5194/acp-22-15135-2022, 2022
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The detection of sulfur compounds in the upper troposphere (UT) and lower stratosphere (LS) is a challenge. In-flight measurements of SO2 and sulfate aerosol were performed during the BLUESKY mission in spring 2020 under exceptional atmospheric conditions. Reduced sinks in the dry UTLS and lower but still significant air traffic influenced the enhanced SO2 in the UT, and aged volcanic plumes enhanced the LS sulfate aerosol impacting the atmospheric radiation budget and global climate.
Hossein Dadashazar, Andrea F. Corral, Ewan Crosbie, Sanja Dmitrovic, Simon Kirschler, Kayla McCauley, Richard Moore, Claire Robinson, Joseph S. Schlosser, Michael Shook, K. Lee Thornhill, Christiane Voigt, Edward Winstead, Luke Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 22, 13897–13913, https://doi.org/10.5194/acp-22-13897-2022, https://doi.org/10.5194/acp-22-13897-2022, 2022
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Multi-season airborne data over the northwestern Atlantic show that organic mass fraction and the relative amount of oxygenated organics within that fraction are enhanced in droplet residual particles as compared to particles below and above cloud. In-cloud aqueous processing is shown to be a potential driver of this compositional shift in cloud. This implies that aerosol–cloud interactions in the region reduce aerosol hygroscopicity due to the jump in the organic : sulfate ratio in cloud.
Roger Teoh, Ulrich Schumann, Edward Gryspeerdt, Marc Shapiro, Jarlath Molloy, George Koudis, Christiane Voigt, and Marc E. J. Stettler
Atmos. Chem. Phys., 22, 10919–10935, https://doi.org/10.5194/acp-22-10919-2022, https://doi.org/10.5194/acp-22-10919-2022, 2022
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Aircraft condensation trails (contrails) contribute to over half of the climate forcing attributable to aviation. This study uses historical air traffic and weather data to simulate contrails in the North Atlantic over 5 years, from 2016 to 2021. We found large intra- and inter-year variability in contrail radiative forcing and observed a 66 % reduction due to COVID-19. Most warming contrails predominantly result from night-time flights in winter.
Simon F. Reifenberg, Anna Martin, Matthias Kohl, Sara Bacer, Zaneta Hamryszczak, Ivan Tadic, Lenard Röder, Daniel J. Crowley, Horst Fischer, Katharina Kaiser, Johannes Schneider, Raphael Dörich, John N. Crowley, Laura Tomsche, Andreas Marsing, Christiane Voigt, Andreas Zahn, Christopher Pöhlker, Bruna A. Holanda, Ovid Krüger, Ulrich Pöschl, Mira Pöhlker, Patrick Jöckel, Marcel Dorf, Ulrich Schumann, Jonathan Williams, Birger Bohn, Joachim Curtius, Hardwig Harder, Hans Schlager, Jos Lelieveld, and Andrea Pozzer
Atmos. Chem. Phys., 22, 10901–10917, https://doi.org/10.5194/acp-22-10901-2022, https://doi.org/10.5194/acp-22-10901-2022, 2022
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In this work we use a combination of observational data from an aircraft campaign and model results to investigate the effect of the European lockdown due to COVID-19 in spring 2020. Using model results, we show that the largest relative changes to the atmospheric composition caused by the reduced emissions are located in the upper troposphere around aircraft cruise altitude, while the largest absolute changes are present at the surface.
Pooja Verma and Ulrike Burkhardt
Atmos. Chem. Phys., 22, 8819–8842, https://doi.org/10.5194/acp-22-8819-2022, https://doi.org/10.5194/acp-22-8819-2022, 2022
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This paper investigates contrail ice formation within cirrus and the impact of natural cirrus on the contrail ice formation in the high-resolution ICON-LEM simulations over Germany. Contrail formation often leads to increases in cirrus ice crystal number concentration by a few orders of magnitude. Contrail formation is affected by pre-existing cirrus, leading to changes in contrail formation conditions and ice nucleation rates that can be significant in optically thick cirrus.
Ovid O. Krüger, Bruna A. Holanda, Sourangsu Chowdhury, Andrea Pozzer, David Walter, Christopher Pöhlker, Maria Dolores Andrés Hernández, John P. Burrows, Christiane Voigt, Jos Lelieveld, Johannes Quaas, Ulrich Pöschl, and Mira L. Pöhlker
Atmos. Chem. Phys., 22, 8683–8699, https://doi.org/10.5194/acp-22-8683-2022, https://doi.org/10.5194/acp-22-8683-2022, 2022
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The abrupt reduction in human activities during the first COVID-19 lockdown created unprecedented atmospheric conditions. We took the opportunity to quantify changes in black carbon (BC) as a major anthropogenic air pollutant. Therefore, we measured BC on board a research aircraft over Europe during the lockdown and compared the results to measurements from 2017. With model simulations we account for different weather conditions and find a lockdown-related decrease in BC of 41 %.
Eleni Tetoni, Florian Ewald, Martin Hagen, Gregor Köcher, Tobias Zinner, and Silke Groß
Atmos. Meas. Tech., 15, 3969–3999, https://doi.org/10.5194/amt-15-3969-2022, https://doi.org/10.5194/amt-15-3969-2022, 2022
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We use the C-band POLDIRAD and the Ka-band MIRA-35 to perform snowfall dual-wavelength polarimetric radar measurements. We develop an ice microphysics retrieval for mass, apparent shape, and median size of the particle size distribution by comparing observations to T-matrix ice spheroid simulations while varying the mass–size relationship. We furthermore show how the polarimetric measurements from POLDIRAD help to narrow down ambiguities between ice particle shape and size.
Simon Kirschler, Christiane Voigt, Bruce Anderson, Ramon Campos Braga, Gao Chen, Andrea F. Corral, Ewan Crosbie, Hossein Dadashazar, Richard A. Ferrare, Valerian Hahn, Johannes Hendricks, Stefan Kaufmann, Richard Moore, Mira L. Pöhlker, Claire Robinson, Amy J. Scarino, Dominik Schollmayer, Michael A. Shook, K. Lee Thornhill, Edward Winstead, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 22, 8299–8319, https://doi.org/10.5194/acp-22-8299-2022, https://doi.org/10.5194/acp-22-8299-2022, 2022
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In this study we show that the vertical velocity dominantly impacts the cloud droplet number concentration (NC) of low-level clouds over the western North Atlantic in the winter and summer season, while the cloud condensation nuclei concentration, aerosol size distribution and chemical composition impact NC within a season. The observational data presented in this study can evaluate and improve the representation of aerosol–cloud interactions for a wide range of conditions.
Manuel Gutleben, Silke Groß, Christian Heske, and Martin Wirth
Atmos. Chem. Phys., 22, 7319–7330, https://doi.org/10.5194/acp-22-7319-2022, https://doi.org/10.5194/acp-22-7319-2022, 2022
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The main transportation route of Saharan mineral dust particles leads over the subtropical Atlantic Ocean and is subject to a seasonal variation. This study investigates the characteristics of wintertime transatlantic dust transport towards the Caribbean by means of airborne lidar measurements. It is found that dust particles are transported at low atmospheric altitudes (<3.5 km) embedded in a relatively moist mixture with two other particle types, namely marine and biomass-burning particles.
Theresa Mieslinger, Bjorn Stevens, Tobias Kölling, Manfred Brath, Martin Wirth, and Stefan A. Buehler
Atmos. Chem. Phys., 22, 6879–6898, https://doi.org/10.5194/acp-22-6879-2022, https://doi.org/10.5194/acp-22-6879-2022, 2022
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The trades are home to a plethora of small cumulus clouds that are often barely visible to the human eye and difficult to detect with active and passive remote sensing methods. With the help of a new method and by means of high-resolution data we can detect small and particularly thin clouds. We find that optically thin clouds are a common phenomenon in the trades, covering a large area and influencing the radiative effect of clouds if they are undetected and contaminate the cloud-free signal.
M. Dolores Andrés Hernández, Andreas Hilboll, Helmut Ziereis, Eric Förster, Ovid O. Krüger, Katharina Kaiser, Johannes Schneider, Francesca Barnaba, Mihalis Vrekoussis, Jörg Schmidt, Heidi Huntrieser, Anne-Marlene Blechschmidt, Midhun George, Vladyslav Nenakhov, Theresa Harlass, Bruna A. Holanda, Jennifer Wolf, Lisa Eirenschmalz, Marc Krebsbach, Mira L. Pöhlker, Anna B. Kalisz Hedegaard, Linlu Mei, Klaus Pfeilsticker, Yangzhuoran Liu, Ralf Koppmann, Hans Schlager, Birger Bohn, Ulrich Schumann, Andreas Richter, Benjamin Schreiner, Daniel Sauer, Robert Baumann, Mariano Mertens, Patrick Jöckel, Markus Kilian, Greta Stratmann, Christopher Pöhlker, Monica Campanelli, Marco Pandolfi, Michael Sicard, José L. Gómez-Amo, Manuel Pujadas, Katja Bigge, Flora Kluge, Anja Schwarz, Nikos Daskalakis, David Walter, Andreas Zahn, Ulrich Pöschl, Harald Bönisch, Stephan Borrmann, Ulrich Platt, and John P. Burrows
Atmos. Chem. Phys., 22, 5877–5924, https://doi.org/10.5194/acp-22-5877-2022, https://doi.org/10.5194/acp-22-5877-2022, 2022
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EMeRGe provides a unique set of in situ and remote sensing airborne measurements of trace gases and aerosol particles along selected flight routes in the lower troposphere over Europe. The interpretation uses also complementary collocated ground-based and satellite measurements. The collected data help to improve the current understanding of the complex spatial distribution of trace gases and aerosol particles resulting from mixing, transport, and transformation of pollution plumes over Europe.
Mireia Papke Chica, Valerian Hahn, Tiziana Braeuer, Elena de la Torre Castro, Florian Ewald, Mathias Gergely, Simon Kirschler, Luca Bugliaro Goggia, Stefanie Knobloch, Martina Kraemer, Johannes Lucke, Johanna Mayer, Raphael Maerkl, Manuel Moser, Laura Tomsche, Tina Jurkat-Witschas, Martin Zoeger, Christian von Savigny, and Christiane Voigt
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-255, https://doi.org/10.5194/acp-2022-255, 2022
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The mixed-phase temperature regime in convective clouds challenges our understanding of microphysical and radiative cloud properties. We provide a rare and unique dataset of aircraft in situ measurements in a strong mid-latitude convective system. We find that mechanisms initiating ice nucleation and growth strongly depend on temperature, relative humidity, and vertical velocity and variate within the measured system, resulting in altitude dependent changes of the cloud liquid and ice fraction.
Luca Bugliaro, Dennis Piontek, Stephan Kox, Marius Schmidl, Bernhard Mayer, Richard Müller, Margarita Vázquez-Navarro, Daniel M. Peters, Roy G. Grainger, Josef Gasteiger, and Jayanta Kar
Nat. Hazards Earth Syst. Sci., 22, 1029–1054, https://doi.org/10.5194/nhess-22-1029-2022, https://doi.org/10.5194/nhess-22-1029-2022, 2022
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The monitoring of ash dispersion in the atmosphere is an important task for satellite remote sensing since ash represents a threat to air traffic. We present an AI-based method that retrieves the spatial extension and properties of volcanic ash clouds with high temporal resolution during day and night by means of geostationary satellite measurements. This algorithm, trained on realistic observations simulated with a radiative transfer model, runs operationally at the German Weather Service.
Helmut Ziereis, Peter Hoor, Jens-Uwe Grooß, Andreas Zahn, Greta Stratmann, Paul Stock, Michael Lichtenstern, Jens Krause, Vera Bense, Armin Afchine, Christian Rolf, Wolfgang Woiwode, Marleen Braun, Jörn Ungermann, Andreas Marsing, Christiane Voigt, Andreas Engel, Björn-Martin Sinnhuber, and Hermann Oelhaf
Atmos. Chem. Phys., 22, 3631–3654, https://doi.org/10.5194/acp-22-3631-2022, https://doi.org/10.5194/acp-22-3631-2022, 2022
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Airborne observations were conducted in the lowermost Arctic stratosphere during the winter of 2015/2016. The observed distribution of reactive nitrogen shows clear indications of nitrification in mid-winter and denitrification in late winter. This was caused by the formation of polar stratospheric cloud particles, which were observed during several flights. The sedimentation and evaporation of these particles and the descent of air masses cause a redistribution of reactive nitrogen.
Adrien Deroubaix, Laurent Menut, Cyrille Flamant, Peter Knippertz, Andreas H. Fink, Anneke Batenburg, Joel Brito, Cyrielle Denjean, Cheikh Dione, Régis Dupuy, Valerian Hahn, Norbert Kalthoff, Fabienne Lohou, Alfons Schwarzenboeck, Guillaume Siour, Paolo Tuccella, and Christiane Voigt
Atmos. Chem. Phys., 22, 3251–3273, https://doi.org/10.5194/acp-22-3251-2022, https://doi.org/10.5194/acp-22-3251-2022, 2022
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During the summer monsoon in West Africa, pollutants emitted in urbanized areas modify cloud cover and precipitation patterns. We analyze these patterns with the WRF-CHIMERE model, integrating the effects of aerosols on meteorology, based on the numerous observations provided by the Dynamics-Aerosol-Climate-Interactions campaign. This study adds evidence to recent findings that increased pollution levels in West Africa delay the breakup time of low-level clouds and reduce precipitation.
Martin Hagen, Florian Ewald, Silke Groß, Lothar Oswald, David A. Farrell, Marvin Forde, Manuel Gutleben, Johann Heumos, Jens Reimann, Eleni Tetoni, Gregor Köcher, Eleni Marinou, Christoph Kiemle, Qiang Li, Rebecca Chewitt-Lucas, Alton Daley, Delando Grant, and Kashawn Hall
Earth Syst. Sci. Data, 13, 5899–5914, https://doi.org/10.5194/essd-13-5899-2021, https://doi.org/10.5194/essd-13-5899-2021, 2021
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The German polarimetric weather radar Poldirad was deployed for the international campaign EUREC4A on Barbados. The focus was monitoring clouds and precipitation in the trade wind region east of Barbados. Observations were with a temporal sequence of 5 min and a maximum range of 375 km. Examples of mesoscale precipitation patterns, rain rate accumulation, diurnal cycle, and vertical distribution show the potential for further studies on the life cycle of precipitating shallow cumulus clouds.
Matthieu Plu, Guillaume Bigeard, Bojan Sič, Emanuele Emili, Luca Bugliaro, Laaziz El Amraoui, Jonathan Guth, Beatrice Josse, Lucia Mona, and Dennis Piontek
Nat. Hazards Earth Syst. Sci., 21, 3731–3747, https://doi.org/10.5194/nhess-21-3731-2021, https://doi.org/10.5194/nhess-21-3731-2021, 2021
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Volcanic eruptions that spread out ash over large areas, like Eyjafjallajökull in 2010, may have huge economic consequences due to flight cancellations. In this article, we demonstrate the benefits of source term improvement and of data assimilation for quantifying volcanic ash concentrations. The work, which was supported by the EUNADICS-AV project, is the first one, to our knowledge, that demonstrates the benefit of the assimilation of ground-based lidar data over Europe during an eruption.
Ramon Campos Braga, Barbara Ervens, Daniel Rosenfeld, Meinrat O. Andreae, Jan-David Förster, Daniel Fütterer, Lianet Hernández Pardo, Bruna A. Holanda, Tina Jurkat-Witschas, Ovid O. Krüger, Oliver Lauer, Luiz A. T. Machado, Christopher Pöhlker, Daniel Sauer, Christiane Voigt, Adrian Walser, Manfred Wendisch, Ulrich Pöschl, and Mira L. Pöhlker
Atmos. Chem. Phys., 21, 17513–17528, https://doi.org/10.5194/acp-21-17513-2021, https://doi.org/10.5194/acp-21-17513-2021, 2021
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Interactions of aerosol particles with clouds represent a large uncertainty in estimates of climate change. Properties of aerosol particles control their ability to act as cloud condensation nuclei. Using aerosol measurements in the Amazon, we performed model studies to compare predicted and measured cloud droplet number concentrations at cloud bases. Our results confirm previous estimates of particle hygroscopicity in this region.
Silke Trömel, Clemens Simmer, Ulrich Blahak, Armin Blanke, Sabine Doktorowski, Florian Ewald, Michael Frech, Mathias Gergely, Martin Hagen, Tijana Janjic, Heike Kalesse-Los, Stefan Kneifel, Christoph Knote, Jana Mendrok, Manuel Moser, Gregor Köcher, Kai Mühlbauer, Alexander Myagkov, Velibor Pejcic, Patric Seifert, Prabhakar Shrestha, Audrey Teisseire, Leonie von Terzi, Eleni Tetoni, Teresa Vogl, Christiane Voigt, Yuefei Zeng, Tobias Zinner, and Johannes Quaas
Atmos. Chem. Phys., 21, 17291–17314, https://doi.org/10.5194/acp-21-17291-2021, https://doi.org/10.5194/acp-21-17291-2021, 2021
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The article introduces the ACP readership to ongoing research in Germany on cloud- and precipitation-related process information inherent in polarimetric radar measurements, outlines pathways to inform atmospheric models with radar-based information, and points to remaining challenges towards an improved fusion of radar polarimetry and atmospheric modelling.
Heike Konow, Florian Ewald, Geet George, Marek Jacob, Marcus Klingebiel, Tobias Kölling, Anna E. Luebke, Theresa Mieslinger, Veronika Pörtge, Jule Radtke, Michael Schäfer, Hauke Schulz, Raphaela Vogel, Martin Wirth, Sandrine Bony, Susanne Crewell, André Ehrlich, Linda Forster, Andreas Giez, Felix Gödde, Silke Groß, Manuel Gutleben, Martin Hagen, Lutz Hirsch, Friedhelm Jansen, Theresa Lang, Bernhard Mayer, Mario Mech, Marc Prange, Sabrina Schnitt, Jessica Vial, Andreas Walbröl, Manfred Wendisch, Kevin Wolf, Tobias Zinner, Martin Zöger, Felix Ament, and Bjorn Stevens
Earth Syst. Sci. Data, 13, 5545–5563, https://doi.org/10.5194/essd-13-5545-2021, https://doi.org/10.5194/essd-13-5545-2021, 2021
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The German research aircraft HALO took part in the research campaign EUREC4A in January and February 2020. The focus area was the tropical Atlantic east of the island of Barbados. We describe the characteristics of the 15 research flights, provide auxiliary information, derive combined cloud mask products from all instruments that observe clouds on board the aircraft, and provide code examples that help new users of the data to get started.
Tiziana Bräuer, Christiane Voigt, Daniel Sauer, Stefan Kaufmann, Valerian Hahn, Monika Scheibe, Hans Schlager, Felix Huber, Patrick Le Clercq, Richard H. Moore, and Bruce E. Anderson
Atmos. Chem. Phys., 21, 16817–16826, https://doi.org/10.5194/acp-21-16817-2021, https://doi.org/10.5194/acp-21-16817-2021, 2021
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Over half of aviation climate impact is caused by contrails. Biofuels can reduce the ice crystal numbers in contrails and mitigate the climate impact. The experiment ECLIF II/NDMAX in 2018 assessed the effects of biofuels on contrails and aviation emissions. The NASA DC-8 aircraft performed measurements inside the contrail of the DLR A320. One reference fuel and two blends of the biofuel HEFA and kerosene are analysed. We find a max reduction of contrail ice numbers through biofuel use of 40 %.
Hugues Brenot, Nicolas Theys, Lieven Clarisse, Jeroen van Gent, Daniel R. Hurtmans, Sophie Vandenbussche, Nikolaos Papagiannopoulos, Lucia Mona, Timo Virtanen, Andreas Uppstu, Mikhail Sofiev, Luca Bugliaro, Margarita Vázquez-Navarro, Pascal Hedelt, Michelle Maree Parks, Sara Barsotti, Mauro Coltelli, William Moreland, Simona Scollo, Giuseppe Salerno, Delia Arnold-Arias, Marcus Hirtl, Tuomas Peltonen, Juhani Lahtinen, Klaus Sievers, Florian Lipok, Rolf Rüfenacht, Alexander Haefele, Maxime Hervo, Saskia Wagenaar, Wim Som de Cerff, Jos de Laat, Arnoud Apituley, Piet Stammes, Quentin Laffineur, Andy Delcloo, Robertson Lennart, Carl-Herbert Rokitansky, Arturo Vargas, Markus Kerschbaum, Christian Resch, Raimund Zopp, Matthieu Plu, Vincent-Henri Peuch, Michel Van Roozendael, and Gerhard Wotawa
Nat. Hazards Earth Syst. Sci., 21, 3367–3405, https://doi.org/10.5194/nhess-21-3367-2021, https://doi.org/10.5194/nhess-21-3367-2021, 2021
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The purpose of the EUNADICS-AV (European Natural Airborne Disaster Information and Coordination System for Aviation) prototype early warning system (EWS) is to develop the combined use of harmonised data products from satellite, ground-based and in situ instruments to produce alerts of airborne hazards (volcanic, dust, smoke and radionuclide clouds), satisfying the requirement of aviation air traffic management (ATM) stakeholders (https://cordis.europa.eu/project/id/723986).
Hossein Dadashazar, Majid Alipanah, Miguel Ricardo A. Hilario, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Andrew J. Peters, Amy Jo Scarino, Michael Shook, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Bo Zhang, Luke Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 21, 16121–16141, https://doi.org/10.5194/acp-21-16121-2021, https://doi.org/10.5194/acp-21-16121-2021, 2021
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This study investigates precipitation impacts on long-range transport of North American outflow over the western North Atlantic Ocean (WNAO). Results demonstrate that precipitation scavenging plays a significant role in modifying surface aerosol concentrations over the WNAO, especially in winter and spring due to large-scale scavenging processes. This study highlights how precipitation impacts surface aerosol properties with relevance for other marine regions vulnerable to continental outflow.
Yu-Wen Chen, Yi-Chun Chen, Charles C.-K. Chou, Hui-Ming Hung, Shih-Yu Chang, Lisa Eirenschmalz, Michael Lichtenstern, Helmut Ziereis, Hans Schlager, Greta Stratmann, Katharina Kaiser, Johannes Schneider, Stephan Borrmann, Florian Obersteiner, Eric Förster, Andreas Zahn, Wei-Nai Chen, Po-Hsiung Lin, Shuenn-Chin Chang, Maria Dolores Andrés Hernández, Pao-Kuan Wang, and John P. Burrows
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-788, https://doi.org/10.5194/acp-2021-788, 2021
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By presenting an approach using EMeRGe-Asia airborne field measurements and surface observations, this study shows that the fraction of OH reactivity due to SO2-OH reaction has a significant correlation with the sulfate concentration. Approximately 30 % of sulfate is produced by SO2-OH reaction. Our results underline the importance of SO2-OH gas-phase oxidation in sulfate formation, and demonstrate that the method can be applied to other regions and under different meteorological conditions.
Matthieu Plu, Barbara Scherllin-Pirscher, Delia Arnold Arias, Rocio Baro, Guillaume Bigeard, Luca Bugliaro, Ana Carvalho, Laaziz El Amraoui, Kurt Eschbacher, Marcus Hirtl, Christian Maurer, Marie D. Mulder, Dennis Piontek, Lennart Robertson, Carl-Herbert Rokitansky, Fritz Zobl, and Raimund Zopp
Nat. Hazards Earth Syst. Sci., 21, 2973–2992, https://doi.org/10.5194/nhess-21-2973-2021, https://doi.org/10.5194/nhess-21-2973-2021, 2021
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Past volcanic eruptions that spread out ash over large areas, like Eyjafjallajökull in 2010, forced the cancellation of thousands of flights and had huge economic consequences.
In this article, an international team in the H2020 EU-funded EUNADICS-AV project has designed a probabilistic model approach to quantify ash concentrations. This approach is evaluated against measurements, and its potential use to mitigate the impact of future large-scale eruptions is discussed.
Qiang Li and Silke Groß
Atmos. Chem. Phys., 21, 14573–14590, https://doi.org/10.5194/acp-21-14573-2021, https://doi.org/10.5194/acp-21-14573-2021, 2021
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Aircraft emit exhaust gases and particles directly into the atmosphere, which may contribute to climate change. We present a significant reduction in the occurrence rate and particle linear depolarization ratio of cirrus clouds based on the analysis of measurements with the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) satellite during COVID-19 when air traffic was significantly reduced. The findings imply that these clouds formed with less influence from aviation.
Ramon Campos Braga, Daniel Rosenfeld, Ovid O. Krüger, Barbara Ervens, Bruna A. Holanda, Manfred Wendisch, Trismono Krisna, Ulrich Pöschl, Meinrat O. Andreae, Christiane Voigt, and Mira L. Pöhlker
Atmos. Chem. Phys., 21, 14079–14088, https://doi.org/10.5194/acp-21-14079-2021, https://doi.org/10.5194/acp-21-14079-2021, 2021
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Quantifying the precipitation within clouds is crucial for our understanding of the Earth's hydrological cycle. Using in situ measurements of cloud and rain properties over the Amazon Basin and Atlantic Ocean, we show here a linear relationship between the effective radius (re) and precipitation water content near the tops of convective clouds for different pollution states and temperature levels. Our results emphasize the role of re to determine both initiation and amount of precipitation.
Bjorn Stevens, Sandrine Bony, David Farrell, Felix Ament, Alan Blyth, Christopher Fairall, Johannes Karstensen, Patricia K. Quinn, Sabrina Speich, Claudia Acquistapace, Franziska Aemisegger, Anna Lea Albright, Hugo Bellenger, Eberhard Bodenschatz, Kathy-Ann Caesar, Rebecca Chewitt-Lucas, Gijs de Boer, Julien Delanoë, Leif Denby, Florian Ewald, Benjamin Fildier, Marvin Forde, Geet George, Silke Gross, Martin Hagen, Andrea Hausold, Karen J. Heywood, Lutz Hirsch, Marek Jacob, Friedhelm Jansen, Stefan Kinne, Daniel Klocke, Tobias Kölling, Heike Konow, Marie Lothon, Wiebke Mohr, Ann Kristin Naumann, Louise Nuijens, Léa Olivier, Robert Pincus, Mira Pöhlker, Gilles Reverdin, Gregory Roberts, Sabrina Schnitt, Hauke Schulz, A. Pier Siebesma, Claudia Christine Stephan, Peter Sullivan, Ludovic Touzé-Peiffer, Jessica Vial, Raphaela Vogel, Paquita Zuidema, Nicola Alexander, Lyndon Alves, Sophian Arixi, Hamish Asmath, Gholamhossein Bagheri, Katharina Baier, Adriana Bailey, Dariusz Baranowski, Alexandre Baron, Sébastien Barrau, Paul A. Barrett, Frédéric Batier, Andreas Behrendt, Arne Bendinger, Florent Beucher, Sebastien Bigorre, Edmund Blades, Peter Blossey, Olivier Bock, Steven Böing, Pierre Bosser, Denis Bourras, Pascale Bouruet-Aubertot, Keith Bower, Pierre Branellec, Hubert Branger, Michal Brennek, Alan Brewer, Pierre-Etienne Brilouet, Björn Brügmann, Stefan A. Buehler, Elmo Burke, Ralph Burton, Radiance Calmer, Jean-Christophe Canonici, Xavier Carton, Gregory Cato Jr., Jude Andre Charles, Patrick Chazette, Yanxu Chen, Michal T. Chilinski, Thomas Choularton, Patrick Chuang, Shamal Clarke, Hugh Coe, Céline Cornet, Pierre Coutris, Fleur Couvreux, Susanne Crewell, Timothy Cronin, Zhiqiang Cui, Yannis Cuypers, Alton Daley, Gillian M. Damerell, Thibaut Dauhut, Hartwig Deneke, Jean-Philippe Desbios, Steffen Dörner, Sebastian Donner, Vincent Douet, Kyla Drushka, Marina Dütsch, André Ehrlich, Kerry Emanuel, Alexandros Emmanouilidis, Jean-Claude Etienne, Sheryl Etienne-Leblanc, Ghislain Faure, Graham Feingold, Luca Ferrero, Andreas Fix, Cyrille Flamant, Piotr Jacek Flatau, Gregory R. Foltz, Linda Forster, Iulian Furtuna, Alan Gadian, Joseph Galewsky, Martin Gallagher, Peter Gallimore, Cassandra Gaston, Chelle Gentemann, Nicolas Geyskens, Andreas Giez, John Gollop, Isabelle Gouirand, Christophe Gourbeyre, Dörte de Graaf, Geiske E. de Groot, Robert Grosz, Johannes Güttler, Manuel Gutleben, Kashawn Hall, George Harris, Kevin C. Helfer, Dean Henze, Calvert Herbert, Bruna Holanda, Antonio Ibanez-Landeta, Janet Intrieri, Suneil Iyer, Fabrice Julien, Heike Kalesse, Jan Kazil, Alexander Kellman, Abiel T. Kidane, Ulrike Kirchner, Marcus Klingebiel, Mareike Körner, Leslie Ann Kremper, Jan Kretzschmar, Ovid Krüger, Wojciech Kumala, Armin Kurz, Pierre L'Hégaret, Matthieu Labaste, Tom Lachlan-Cope, Arlene Laing, Peter Landschützer, Theresa Lang, Diego Lange, Ingo Lange, Clément Laplace, Gauke Lavik, Rémi Laxenaire, Caroline Le Bihan, Mason Leandro, Nathalie Lefevre, Marius Lena, Donald Lenschow, Qiang Li, Gary Lloyd, Sebastian Los, Niccolò Losi, Oscar Lovell, Christopher Luneau, Przemyslaw Makuch, Szymon Malinowski, Gaston Manta, Eleni Marinou, Nicholas Marsden, Sebastien Masson, Nicolas Maury, Bernhard Mayer, Margarette Mayers-Als, Christophe Mazel, Wayne McGeary, James C. McWilliams, Mario Mech, Melina Mehlmann, Agostino Niyonkuru Meroni, Theresa Mieslinger, Andreas Minikin, Peter Minnett, Gregor Möller, Yanmichel Morfa Avalos, Caroline Muller, Ionela Musat, Anna Napoli, Almuth Neuberger, Christophe Noisel, David Noone, Freja Nordsiek, Jakub L. Nowak, Lothar Oswald, Douglas J. Parker, Carolyn Peck, Renaud Person, Miriam Philippi, Albert Plueddemann, Christopher Pöhlker, Veronika Pörtge, Ulrich Pöschl, Lawrence Pologne, Michał Posyniak, Marc Prange, Estefanía Quiñones Meléndez, Jule Radtke, Karim Ramage, Jens Reimann, Lionel Renault, Klaus Reus, Ashford Reyes, Joachim Ribbe, Maximilian Ringel, Markus Ritschel, Cesar B. Rocha, Nicolas Rochetin, Johannes Röttenbacher, Callum Rollo, Haley Royer, Pauline Sadoulet, Leo Saffin, Sanola Sandiford, Irina Sandu, Michael Schäfer, Vera Schemann, Imke Schirmacher, Oliver Schlenczek, Jerome Schmidt, Marcel Schröder, Alfons Schwarzenboeck, Andrea Sealy, Christoph J. Senff, Ilya Serikov, Samkeyat Shohan, Elizabeth Siddle, Alexander Smirnov, Florian Späth, Branden Spooner, M. Katharina Stolla, Wojciech Szkółka, Simon P. de Szoeke, Stéphane Tarot, Eleni Tetoni, Elizabeth Thompson, Jim Thomson, Lorenzo Tomassini, Julien Totems, Alma Anna Ubele, Leonie Villiger, Jan von Arx, Thomas Wagner, Andi Walther, Ben Webber, Manfred Wendisch, Shanice Whitehall, Anton Wiltshire, Allison A. Wing, Martin Wirth, Jonathan Wiskandt, Kevin Wolf, Ludwig Worbes, Ethan Wright, Volker Wulfmeyer, Shanea Young, Chidong Zhang, Dongxiao Zhang, Florian Ziemen, Tobias Zinner, and Martin Zöger
Earth Syst. Sci. Data, 13, 4067–4119, https://doi.org/10.5194/essd-13-4067-2021, https://doi.org/10.5194/essd-13-4067-2021, 2021
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The EUREC4A field campaign, designed to test hypothesized mechanisms by which clouds respond to warming and benchmark next-generation Earth-system models, is presented. EUREC4A comprised roughly 5 weeks of measurements in the downstream winter trades of the North Atlantic – eastward and southeastward of Barbados. It was the first campaign that attempted to characterize the full range of processes and scales influencing trade wind clouds.
Florian Ewald, Silke Groß, Martin Wirth, Julien Delanoë, Stuart Fox, and Bernhard Mayer
Atmos. Meas. Tech., 14, 5029–5047, https://doi.org/10.5194/amt-14-5029-2021, https://doi.org/10.5194/amt-14-5029-2021, 2021
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In this study, we show how solar radiance observations can be used to validate and further constrain ice cloud microphysics retrieved from the synergy of radar–lidar measurements. Since most radar–lidar retrievals rely on a global assumption about the ice particle shape, ice water content and particle size biases are to be expected in individual cloud regimes. In this work, we identify and correct these biases by reconciling simulated and measured solar radiation reflected from these clouds.
Hossein Dadashazar, David Painemal, Majid Alipanah, Michael Brunke, Seethala Chellappan, Andrea F. Corral, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Claire Robinson, Amy Jo Scarino, Michael Shook, Kenneth Sinclair, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Xubin Zeng, Luke Ziemba, Paquita Zuidema, and Armin Sorooshian
Atmos. Chem. Phys., 21, 10499–10526, https://doi.org/10.5194/acp-21-10499-2021, https://doi.org/10.5194/acp-21-10499-2021, 2021
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This study investigates the seasonal cycle of cloud drop number concentration (Nd) over the western North Atlantic Ocean (WNAO) using multiple datasets. Reasons for the puzzling discrepancy between the seasonal cycles of Nd and aerosol concentration were identified. Results indicate that Nd is highest in winter (when aerosol proxy values are often lowest) due to conditions both linked to cold-air outbreaks and that promote greater droplet activation.
Lukas Krasauskas, Jörn Ungermann, Peter Preusse, Felix Friedl-Vallon, Andreas Zahn, Helmut Ziereis, Christian Rolf, Felix Plöger, Paul Konopka, Bärbel Vogel, and Martin Riese
Atmos. Chem. Phys., 21, 10249–10272, https://doi.org/10.5194/acp-21-10249-2021, https://doi.org/10.5194/acp-21-10249-2021, 2021
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A Rossby wave (RW) breaking event was observed over the North Atlantic during the WISE measurement campaign in October 2017. Infrared limb sounding measurements of trace gases in the lower stratosphere, including high-resolution 3-D tomographic reconstruction, revealed complex spatial structures in stratospheric tracers near the polar jet related to previous RW breaking events. Backward-trajectory analysis and tracer correlations were used to study mixing and stratosphere–troposphere exchange.
Ulrich Schumann, Ian Poll, Roger Teoh, Rainer Koelle, Enrico Spinielli, Jarlath Molloy, George S. Koudis, Robert Baumann, Luca Bugliaro, Marc Stettler, and Christiane Voigt
Atmos. Chem. Phys., 21, 7429–7450, https://doi.org/10.5194/acp-21-7429-2021, https://doi.org/10.5194/acp-21-7429-2021, 2021
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The roughly 70 % reduction of air traffic during the COVID-19 pandemic from March–August 2020 compared to 2019 provides a test case for the relationship between air traffic density, contrails, and their radiative forcing of climate change. This paper investigates the induced traffic and contrail changes in a model study. Besides strong weather changes, the model results indicate aviation-induced cirrus and top-of-the-atmosphere irradiance changes, which can be tested with observations.
Sebastian Wolff, Gerhard Ehret, Christoph Kiemle, Axel Amediek, Mathieu Quatrevalet, Martin Wirth, and Andreas Fix
Atmos. Meas. Tech., 14, 2717–2736, https://doi.org/10.5194/amt-14-2717-2021, https://doi.org/10.5194/amt-14-2717-2021, 2021
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We report on CO2 emissions of a coal-fired power plant derived from flight measurements performed with the IPDA lidar CHARM-F during the CoMet campaign in spring 2018. Despite the results being in broad agreement with reported emissions, we observe strong variations between successive flyovers. Using a high-resolution large eddy simulation, we identify strong atmospheric turbulence as the cause for the variations and recommend more favorable measurement conditions for future campaign planning.
Maxi Boettcher, Andreas Schäfler, Michael Sprenger, Harald Sodemann, Stefan Kaufmann, Christiane Voigt, Hans Schlager, Donato Summa, Paolo Di Girolamo, Daniele Nerini, Urs Germann, and Heini Wernli
Atmos. Chem. Phys., 21, 5477–5498, https://doi.org/10.5194/acp-21-5477-2021, https://doi.org/10.5194/acp-21-5477-2021, 2021
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Warm conveyor belts (WCBs) are important airstreams in extratropical cyclones, often leading to the formation of intense precipitation. We present a case study that involves aircraft, lidar and radar observations of water and clouds in a WCB ascending from western Europe across the Alps towards the Baltic Sea during the field campaigns HyMeX and T-NAWDEX-Falcon in October 2012. A probabilistic trajectory measure and an airborne tracer experiment were used to confirm the long pathway of the WCB.
Andreas Schäfler, Andreas Fix, and Martin Wirth
Atmos. Chem. Phys., 21, 5217–5234, https://doi.org/10.5194/acp-21-5217-2021, https://doi.org/10.5194/acp-21-5217-2021, 2021
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First-ever, collocated ozone and water vapor lidar observations across the tropopause are applied to investigate the extratropical transition layer (ExTL). The combined view of a quasi-instantaneous cross section and its tracer–tracer depiction allows us to analyze the ExTL shape and composition and the formation of mixing lines in relation to the dynamic situation. Such lidar data are relevant for future upper-tropospheric and lower-stratospheric investigations and model validations.
Harald Rybka, Ulrike Burkhardt, Martin Köhler, Ioanna Arka, Luca Bugliaro, Ulrich Görsdorf, Ákos Horváth, Catrin I. Meyer, Jens Reichardt, Axel Seifert, and Johan Strandgren
Atmos. Chem. Phys., 21, 4285–4318, https://doi.org/10.5194/acp-21-4285-2021, https://doi.org/10.5194/acp-21-4285-2021, 2021
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Estimating the impact of convection on the upper-tropospheric water budget remains a problem for models employing resolutions of several kilometers or more. A sub-kilometer high-resolution model is used to study summertime convection. The results suggest mostly close agreement with ground- and satellite-based observational data while slightly overestimating total frozen water path and anvil lifetime. The simulations are well suited to supplying information for parameterization development.
Inken Knop, Stephan E. Bansmer, Valerian Hahn, and Christiane Voigt
Atmos. Meas. Tech., 14, 1761–1781, https://doi.org/10.5194/amt-14-1761-2021, https://doi.org/10.5194/amt-14-1761-2021, 2021
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Knowledge on droplet size and concentration is essential for several applications of atomizers. After having developed a new spray system for our icing wind tunnel, we did intercomparison tests of different droplet measurement techniques including two commercial probes. The probes proved the good repeatability of the spray conditions and showed good overall agreement in measuring size and concentration. Furthermore, we could identify limitations and error sources of the measuring techniques.
Ourania Soupiona, Alexandros Papayannis, Panagiotis Kokkalis, Romanos Foskinis, Guadalupe Sánchez Hernández, Pablo Ortiz-Amezcua, Maria Mylonaki, Christina-Anna Papanikolaou, Nikolaos Papagiannopoulos, Stefanos Samaras, Silke Groß, Rodanthi-Elisavet Mamouri, Lucas Alados-Arboledas, Aldo Amodeo, and Basil Psiloglou
Atmos. Chem. Phys., 20, 15147–15166, https://doi.org/10.5194/acp-20-15147-2020, https://doi.org/10.5194/acp-20-15147-2020, 2020
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51 dust events over the Mediterranean from EARLINET were studied regarding the aerosol geometrical, optical and microphysical properties and radiative forcing. We found δp532 values of 0.24–0.28, LR532 values of 49–52 sr and AOT532 of 0.11–0.40. The aerosol mixing state was also examined. Depending on the dust properties, intensity and solar zenith angle, the estimated solar radiative forcing ranged from −59 to −22 W m−2 at the surface and from −24 to −1 W m−2 at the TOA (cooling effect).
Anna Gialitaki, Alexandra Tsekeri, Vassilis Amiridis, Romain Ceolato, Lucas Paulien, Anna Kampouri, Antonis Gkikas, Stavros Solomos, Eleni Marinou, Moritz Haarig, Holger Baars, Albert Ansmann, Tatyana Lapyonok, Anton Lopatin, Oleg Dubovik, Silke Groß, Martin Wirth, Maria Tsichla, Ioanna Tsikoudi, and Dimitris Balis
Atmos. Chem. Phys., 20, 14005–14021, https://doi.org/10.5194/acp-20-14005-2020, https://doi.org/10.5194/acp-20-14005-2020, 2020
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Stratospheric smoke particles are found to significantly depolarize incident light, while this effect is also accompanied by a strong spectral dependence. We utilize scattering simulations to show that this behaviour can be attributed to the near-spherical shape of the particles. We also examine whether an extension of the current AERONET scattering model to include the near-spherical shapes could be of benefit to the AERONET retrieval for stratospheric smoke associated with enhanced PLDR.
Bettina Hottmann, Sascha Hafermann, Laura Tomsche, Daniel Marno, Monica Martinez, Hartwig Harder, Andrea Pozzer, Marco Neumaier, Andreas Zahn, Birger Bohn, Greta Stratmann, Helmut Ziereis, Jos Lelieveld, and Horst Fischer
Atmos. Chem. Phys., 20, 12655–12673, https://doi.org/10.5194/acp-20-12655-2020, https://doi.org/10.5194/acp-20-12655-2020, 2020
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During OMO we observed enhanced mixing ratios of hydroperoxides (ROOH) in the Asian monsoon anticyclone (AMA) relative to the background. The observed mixing ratios are higher than steady-state calculations and EMAC simulations, especially in the AMA, indicating atmospheric transport of ROOH. Uncertainties in the scavenging efficiencies likely cause deviations from EMAC. Longitudinal gradients indicate a pool of ROOH towards the center of the AMA associated with upwind convection over India.
Manuel Gutleben, Silke Groß, Martin Wirth, and Bernhard Mayer
Atmos. Chem. Phys., 20, 12313–12327, https://doi.org/10.5194/acp-20-12313-2020, https://doi.org/10.5194/acp-20-12313-2020, 2020
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Airborne lidar measurements in the vicinity of Barbados are used to investigate radiative effects of long-range-transported Saharan air layers. Derived atmospheric heating rates indicate that observed enhanced water vapor concentrations inside these layers are the main drivers for dust vertical mixing inside the layers. Additionally, they may play a major role for the suppression of subjacent convective cloud development.
Christof G. Beer, Johannes Hendricks, Mattia Righi, Bernd Heinold, Ina Tegen, Silke Groß, Daniel Sauer, Adrian Walser, and Bernadett Weinzierl
Geosci. Model Dev., 13, 4287–4303, https://doi.org/10.5194/gmd-13-4287-2020, https://doi.org/10.5194/gmd-13-4287-2020, 2020
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Mineral dust aerosol plays an important role in the climate system. Previously, dust emissions have often been represented in global models by prescribed monthly-mean emission fields representative of a specific year. We now apply an online calculation of wind-driven dust emissions. This results in an improved agreement with observations, due to a better representation of the highly variable dust emissions. Increasing the model resolution led to an additional performance gain.
Montserrat Costa-Surós, Odran Sourdeval, Claudia Acquistapace, Holger Baars, Cintia Carbajal Henken, Christa Genz, Jonas Hesemann, Cristofer Jimenez, Marcel König, Jan Kretzschmar, Nils Madenach, Catrin I. Meyer, Roland Schrödner, Patric Seifert, Fabian Senf, Matthias Brueck, Guido Cioni, Jan Frederik Engels, Kerstin Fieg, Ksenia Gorges, Rieke Heinze, Pavan Kumar Siligam, Ulrike Burkhardt, Susanne Crewell, Corinna Hoose, Axel Seifert, Ina Tegen, and Johannes Quaas
Atmos. Chem. Phys., 20, 5657–5678, https://doi.org/10.5194/acp-20-5657-2020, https://doi.org/10.5194/acp-20-5657-2020, 2020
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The impact of anthropogenic aerosols on clouds is a key uncertainty in climate change. This study analyses large-domain simulations with a new high-resolution model to investigate the differences in clouds between 1985 and 2013 comparing multiple observational datasets. The differences in aerosol and in cloud droplet concentrations are clearly detectable. For other quantities, the detection and attribution proved difficult, despite a substantial impact on the Earth's energy budget.
Bruna A. Holanda, Mira L. Pöhlker, David Walter, Jorge Saturno, Matthias Sörgel, Jeannine Ditas, Florian Ditas, Christiane Schulz, Marco Aurélio Franco, Qiaoqiao Wang, Tobias Donth, Paulo Artaxo, Henrique M. J. Barbosa, Stephan Borrmann, Ramon Braga, Joel Brito, Yafang Cheng, Maximilian Dollner, Johannes W. Kaiser, Thomas Klimach, Christoph Knote, Ovid O. Krüger, Daniel Fütterer, Jošt V. Lavrič, Nan Ma, Luiz A. T. Machado, Jing Ming, Fernando G. Morais, Hauke Paulsen, Daniel Sauer, Hans Schlager, Johannes Schneider, Hang Su, Bernadett Weinzierl, Adrian Walser, Manfred Wendisch, Helmut Ziereis, Martin Zöger, Ulrich Pöschl, Meinrat O. Andreae, and Christopher Pöhlker
Atmos. Chem. Phys., 20, 4757–4785, https://doi.org/10.5194/acp-20-4757-2020, https://doi.org/10.5194/acp-20-4757-2020, 2020
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Biomass burning smoke from African savanna and grassland is transported across the South Atlantic Ocean in defined layers within the free troposphere. The combination of in situ aircraft and ground-based measurements aided by satellite observations showed that these layers are transported into the Amazon Basin during the early dry season. The influx of aged smoke, enriched in black carbon and cloud condensation nuclei, has important implications for the Amazonian aerosol and cloud cycling.
Mattia Righi, Johannes Hendricks, Ulrike Lohmann, Christof Gerhard Beer, Valerian Hahn, Bernd Heinold, Romy Heller, Martina Krämer, Michael Ponater, Christian Rolf, Ina Tegen, and Christiane Voigt
Geosci. Model Dev., 13, 1635–1661, https://doi.org/10.5194/gmd-13-1635-2020, https://doi.org/10.5194/gmd-13-1635-2020, 2020
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A new cloud microphysical scheme is implemented in the global EMAC-MADE3 aerosol model and evaluated. The new scheme features a detailed parameterization for aerosol-driven ice formation in cirrus clouds, accounting for the competition between homogeneous and heterogeneous ice formation processes. The comparison against satellite data and in situ measurements shows that the model performance is in line with similar global coupled models featuring ice cloud parameterizations.
Pascal Polonik, Christoph Knote, Tobias Zinner, Florian Ewald, Tobias Kölling, Bernhard Mayer, Meinrat O. Andreae, Tina Jurkat-Witschas, Thomas Klimach, Christoph Mahnke, Sergej Molleker, Christopher Pöhlker, Mira L. Pöhlker, Ulrich Pöschl, Daniel Rosenfeld, Christiane Voigt, Ralf Weigel, and Manfred Wendisch
Atmos. Chem. Phys., 20, 1591–1605, https://doi.org/10.5194/acp-20-1591-2020, https://doi.org/10.5194/acp-20-1591-2020, 2020
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A realistic representation of cloud–aerosol interactions is central to accurate climate projections. Here we combine observations collected during the ACRIDICON-CHUVA campaign with chemistry-transport simulations to evaluate the model’s ability to represent the indirect effects of biomass burning aerosol on cloud microphysics. We find an upper limit for the model sensitivity on cloud condensation nuclei concentrations well below the levels reached during the burning season in the Amazon Basin.
Carlos Toledano, Benjamín Torres, Cristian Velasco-Merino, Dietrich Althausen, Silke Groß, Matthias Wiegner, Bernadett Weinzierl, Josef Gasteiger, Albert Ansmann, Ramiro González, David Mateos, David Farrel, Thomas Müller, Moritz Haarig, and Victoria E. Cachorro
Atmos. Chem. Phys., 19, 14571–14583, https://doi.org/10.5194/acp-19-14571-2019, https://doi.org/10.5194/acp-19-14571-2019, 2019
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Ground-based sun photometers have been used to analyze the properties of long-range transported Saharan dust over Barbados. The measurements were carried out as part of the Saharan Aerosol Long-Range Transport and Aerosol–Cloud-Interaction Experiment (SALTRACE), carried out in the Caribbean in 2013. A variety of instruments, ground-based and airborne, were used in this research. In this paper, the sun photometer data are presented and related to data collected from other co-located instruments.
Marleen Braun, Jens-Uwe Grooß, Wolfgang Woiwode, Sören Johansson, Michael Höpfner, Felix Friedl-Vallon, Hermann Oelhaf, Peter Preusse, Jörn Ungermann, Björn-Martin Sinnhuber, Helmut Ziereis, and Peter Braesicke
Atmos. Chem. Phys., 19, 13681–13699, https://doi.org/10.5194/acp-19-13681-2019, https://doi.org/10.5194/acp-19-13681-2019, 2019
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We analyse nitrification of the LMS in the Arctic winter 2015–2016 based on GLORIA measurements. Vertical cross sections of HNO3 for several flights show complex fine–scale structures and enhanced values down to 9 km. The extent of overall nitrification is quantified based on HNO3–O3 correlations and reaches between 5 ppbv and 7 ppbv at potential temperature levels between 350 and 380 K. Further, we compare our result with the atmospheric model CLaMS.
Eleni Marinou, Matthias Tesche, Athanasios Nenes, Albert Ansmann, Jann Schrod, Dimitra Mamali, Alexandra Tsekeri, Michael Pikridas, Holger Baars, Ronny Engelmann, Kalliopi-Artemis Voudouri, Stavros Solomos, Jean Sciare, Silke Groß, Florian Ewald, and Vassilis Amiridis
Atmos. Chem. Phys., 19, 11315–11342, https://doi.org/10.5194/acp-19-11315-2019, https://doi.org/10.5194/acp-19-11315-2019, 2019
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We assess the feasibility of ground-based and spaceborne lidars to retrieve profiles of cloud-relevant aerosol concentrations and ice-nucleating particles. The retrieved profiles are in good agreement with airborne in situ measurements. Our methodology will be applied to satellite observations in the future so as to provide a global 3D product of cloud-relevant properties.
Andreas Marsing, Tina Jurkat-Witschas, Jens-Uwe Grooß, Stefan Kaufmann, Romy Heller, Andreas Engel, Peter Hoor, Jens Krause, and Christiane Voigt
Atmos. Chem. Phys., 19, 10757–10772, https://doi.org/10.5194/acp-19-10757-2019, https://doi.org/10.5194/acp-19-10757-2019, 2019
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We study the partitioning of inorganic chlorine into active (ozone-depleting) and reservoir species in the lowermost stratosphere of the Arctic polar vortex, using novel in situ aircraft measurements in winter 2015/2016. We observe a change in recovery pathways of the reservoirs HCl and ClONO2 with increasing potential temperature. A comparison with the CLaMS model relates the observations to the vortex-wide evolution and confirms unresolved discrepancies in the mid-winter HCl distribution.
Manuel Gutleben, Silke Groß, and Martin Wirth
Atmos. Chem. Phys., 19, 10659–10673, https://doi.org/10.5194/acp-19-10659-2019, https://doi.org/10.5194/acp-19-10659-2019, 2019
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This study concentrates on airborne lidar measurements conducted during the NARVAL field experiments over the western subtropical North Atlantic Ocean to study differences between shallow marine cloud macro-physical properties (i.e. cloud fraction, cloud top height, cloud length, cloud gap length) in Saharan-dust-laden and dust-free trade wind regions. Cloud top heights, cloud fractions and cloud lengths are found to be lower and smaller in Saharan-dust-laden compared to dust-free regions.
Jonathan W. Taylor, Sophie L. Haslett, Keith Bower, Michael Flynn, Ian Crawford, James Dorsey, Tom Choularton, Paul J. Connolly, Valerian Hahn, Christiane Voigt, Daniel Sauer, Régis Dupuy, Joel Brito, Alfons Schwarzenboeck, Thierry Bourriane, Cyrielle Denjean, Phil Rosenberg, Cyrille Flamant, James D. Lee, Adam R. Vaughan, Peter G. Hill, Barbara Brooks, Valéry Catoire, Peter Knippertz, and Hugh Coe
Atmos. Chem. Phys., 19, 8503–8522, https://doi.org/10.5194/acp-19-8503-2019, https://doi.org/10.5194/acp-19-8503-2019, 2019
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Low-level clouds cover a wide area of southern West Africa (SWA) and play an important role in the region's climate, reflecting sunlight away from the surface. We performed aircraft measurements of aerosols and clouds over SWA during the 2016 summer monsoon and found pollution, and polluted clouds, across the whole region. Smoke from biomass burning in Central Africa is transported to West Africa, causing a polluted background which limits the effect of local pollution on cloud properties.
Lisa Bock and Ulrike Burkhardt
Atmos. Chem. Phys., 19, 8163–8174, https://doi.org/10.5194/acp-19-8163-2019, https://doi.org/10.5194/acp-19-8163-2019, 2019
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The climate impact of air traffic is to a large degree caused by changes in cirrus cloudiness resulting from the formation of contrails. We use an atmospheric climate model with a contrail cirrus parameterization to investigate the climate impact of contrail cirrus for the year 2050. The strong increase in contrail cirrus radiative forcing due to the projected increase in air traffic volume cannot be compensated for by the reduction of soot emissions and by improvements in propulsion efficiency.
Marek Jacob, Felix Ament, Manuel Gutleben, Heike Konow, Mario Mech, Martin Wirth, and Susanne Crewell
Atmos. Meas. Tech., 12, 3237–3254, https://doi.org/10.5194/amt-12-3237-2019, https://doi.org/10.5194/amt-12-3237-2019, 2019
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Tropical clouds are a key climate component but are still not fully understood. Therefore, we analyze airborne remote sensing measurements that were taken in the dry and wet seasons over the Atlantic east of Barbados. From these we derive sub-kilometer resolution data of vertically integrated atmospheric water vapor and liquid water. Results show that although the humidity is lower in the dry season, clouds are more frequent, contain more water, and produce more rain than in the wet season.
Quitterie Cazenave, Marie Ceccaldi, Julien Delanoë, Jacques Pelon, Silke Groß, and Andrew Heymsfield
Atmos. Meas. Tech., 12, 2819–2835, https://doi.org/10.5194/amt-12-2819-2019, https://doi.org/10.5194/amt-12-2819-2019, 2019
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The impact of ice clouds on the water cycle and radiative budget is still uncertain due to the complexity of cloud processes that makes it difficult to acquire adequate observations of ice cloud properties and parameterize them into climate and weather prediction models. In this paper we present the latest refinements brought to the DARDAR-CLOUD product, which contains ice cloud microphysical properties retrieved from the cloud radar and lidar measurements from the A-Train space mission.
Florian Ewald, Silke Groß, Martin Hagen, Lutz Hirsch, Julien Delanoë, and Matthias Bauer-Pfundstein
Atmos. Meas. Tech., 12, 1815–1839, https://doi.org/10.5194/amt-12-1815-2019, https://doi.org/10.5194/amt-12-1815-2019, 2019
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This study gives a summary of lessons learned during the absolute calibration of the airborne, high-power Ka-band cloud radar HAMP MIRA on board the German research aircraft HALO. The first part covers the internal calibration of the instrument where individual instrument components are characterized in the laboratory. In the second part, the internal calibration is validated with external reference sources like the ocean surface backscatter and different air- and spaceborne cloud radars.
Kevin Wolf, André Ehrlich, Marek Jacob, Susanne Crewell, Martin Wirth, and Manfred Wendisch
Atmos. Meas. Tech., 12, 1635–1658, https://doi.org/10.5194/amt-12-1635-2019, https://doi.org/10.5194/amt-12-1635-2019, 2019
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Using passive spectral solar radiation and active lidar, radar, and microwave measurements with HALO during NARVAL-II, the cloud droplet number concentration of shallow trade wind cumulus is estimated. With stepwise inclusion of the different instruments into the retrieval, the benefits of the synergetic approach based on artificial measurements and two cloud cases are demonstrated. Significant improvement with the synergetic method compared to the solar-radiation-only method is reported.
Michael Weger, Bernd Heinold, Christa Engler, Ulrich Schumann, Axel Seifert, Romy Fößig, Christiane Voigt, Holger Baars, Ulrich Blahak, Stephan Borrmann, Corinna Hoose, Stefan Kaufmann, Martina Krämer, Patric Seifert, Fabian Senf, Johannes Schneider, and Ina Tegen
Atmos. Chem. Phys., 18, 17545–17572, https://doi.org/10.5194/acp-18-17545-2018, https://doi.org/10.5194/acp-18-17545-2018, 2018
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The impact of desert dust on cloud formation is investigated for a major Saharan dust event over Europe by interactive regional dust modeling. Dust particles are very efficient ice-nucleating particles promoting the formation of ice crystals in clouds. The simulations show that the observed extensive cirrus development was likely related to the above-average dust load. The interactive dust–cloud feedback in the model significantly improves the agreement with aircraft and satellite observations.
Stefan Kaufmann, Christiane Voigt, Romy Heller, Tina Jurkat-Witschas, Martina Krämer, Christian Rolf, Martin Zöger, Andreas Giez, Bernhard Buchholz, Volker Ebert, Troy Thornberry, and Ulrich Schumann
Atmos. Chem. Phys., 18, 16729–16745, https://doi.org/10.5194/acp-18-16729-2018, https://doi.org/10.5194/acp-18-16729-2018, 2018
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We present an intercomparison of the airborne water vapor measurements during the ML-CIRRUS mission. Although the agreement of the hygrometers significantly improved compared to studies from recent decades, systematic differences remain under specific meteorological conditions. We compare the measurements to model data, where we observe a model wet bias in the lower stratosphere close to the tropopause, likely caused by a blurred humidity gradient in the model tropopause.
Christiane Voigt, Andreas Dörnbrack, Martin Wirth, Silke M. Groß, Michael C. Pitts, Lamont R. Poole, Robert Baumann, Benedikt Ehard, Björn-Martin Sinnhuber, Wolfgang Woiwode, and Hermann Oelhaf
Atmos. Chem. Phys., 18, 15623–15641, https://doi.org/10.5194/acp-18-15623-2018, https://doi.org/10.5194/acp-18-15623-2018, 2018
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The 2015–2016 stratospheric winter was the coldest in the 36-year climatological data record. The extreme conditions promoted the formation of persistent Arctic polar stratospheric ice clouds. An extended ice PSC detected by airborne lidar in January 2016 shows a second mode with higher particle depolarization ratios. Back-trajectories from the high-depol ice matched to CALIOP PSC curtains provide evidence for ice nucleation on NAT. The novel data consolidate our understanding of PSC formation.
Yoann Tellier, Clémence Pierangelo, Martin Wirth, Fabien Gibert, and Fabien Marnas
Atmos. Meas. Tech., 11, 5865–5884, https://doi.org/10.5194/amt-11-5865-2018, https://doi.org/10.5194/amt-11-5865-2018, 2018
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The French and German space agencies (CNES, DLR) are currently developing MERLIN, a satellite that will measure atmospheric concentration of methane, a powerful greenhouse gas. To reach the desired precision, horizontally averaging the measurements along the satellite track is performed but leads to a processing bias due to non-linear equations. This article studies the processing biases for several averaging schemes and bias correction algorithms and recommends a best approach to limit biases.
Christiane Schulz, Johannes Schneider, Bruna Amorim Holanda, Oliver Appel, Anja Costa, Suzane S. de Sá, Volker Dreiling, Daniel Fütterer, Tina Jurkat-Witschas, Thomas Klimach, Christoph Knote, Martina Krämer, Scot T. Martin, Stephan Mertes, Mira L. Pöhlker, Daniel Sauer, Christiane Voigt, Adrian Walser, Bernadett Weinzierl, Helmut Ziereis, Martin Zöger, Meinrat O. Andreae, Paulo Artaxo, Luiz A. T. Machado, Ulrich Pöschl, Manfred Wendisch, and Stephan Borrmann
Atmos. Chem. Phys., 18, 14979–15001, https://doi.org/10.5194/acp-18-14979-2018, https://doi.org/10.5194/acp-18-14979-2018, 2018
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Aerosol chemical composition measurements in the tropical upper troposphere over the Amazon region show that 78 % of the aerosol in the upper troposphere consists of organic matter. Up to 20 % of the organic aerosol can be attributed to isoprene epoxydiol secondary organic aerosol (IEPOX-SOA). Furthermore, organic nitrates were identified, suggesting a connection to the IEPOX-SOA formation.
Franz Slemr, Andreas Weigelt, Ralf Ebinghaus, Johannes Bieser, Carl A. M. Brenninkmeijer, Armin Rauthe-Schöch, Markus Hermann, Bengt G. Martinsson, Peter van Velthoven, Harald Bönisch, Marco Neumaier, Andreas Zahn, and Helmut Ziereis
Atmos. Chem. Phys., 18, 12329–12343, https://doi.org/10.5194/acp-18-12329-2018, https://doi.org/10.5194/acp-18-12329-2018, 2018
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Total and elemental mercury were measured in the upper troposphere and lower stratosphere onboard a passenger aircraft. Their concentrations in the upper troposphere were comparable implying low concentrations of oxidized mercury in this region. Large scale seasonally dependent influence of emissions from biomass burning was also observed. Their distributions in the lower stratosphere implies a long stratospheric lifetime, which precludes significant mercury oxidation by ozone.
Sören Johansson, Wolfgang Woiwode, Michael Höpfner, Felix Friedl-Vallon, Anne Kleinert, Erik Kretschmer, Thomas Latzko, Johannes Orphal, Peter Preusse, Jörn Ungermann, Michelle L. Santee, Tina Jurkat-Witschas, Andreas Marsing, Christiane Voigt, Andreas Giez, Martina Krämer, Christian Rolf, Andreas Zahn, Andreas Engel, Björn-Martin Sinnhuber, and Hermann Oelhaf
Atmos. Meas. Tech., 11, 4737–4756, https://doi.org/10.5194/amt-11-4737-2018, https://doi.org/10.5194/amt-11-4737-2018, 2018
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We present two-dimensional cross sections of temperature, HNO3, O3, ClONO2, H2O and CFC-12 from measurements of the GLORIA infrared limb imager during the POLSTRACC/GW-LCYCLE/SALSA aircraft campaigns in the Arctic winter 2015/2016. GLORIA sounded the atmosphere between 5 and 14 km with vertical resolutions of 0.4–1 km. Estimated errors are in the range of 1–2 K (temperature) and 10 %–20 % (trace gases). Comparisons to in situ instruments onboard the aircraft and to Aura/MLS are shown.
Aurélien Chauvigné, Olivier Jourdan, Alfons Schwarzenboeck, Christophe Gourbeyre, Jean François Gayet, Christiane Voigt, Hans Schlager, Stefan Kaufmann, Stephan Borrmann, Sergej Molleker, Andreas Minikin, Tina Jurkat, and Ulrich Schumann
Atmos. Chem. Phys., 18, 9803–9822, https://doi.org/10.5194/acp-18-9803-2018, https://doi.org/10.5194/acp-18-9803-2018, 2018
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This paper demonstrates a new form of statistical analysis of contrail to cirrus evolution. The authors show well-separated analyses of the different stages of the contrail's evolution, which allows us to study their optical, microphysical, and chemical properties. These results could be used to develop representative parameterizations of the scattering and geometrical properties of the ice crystals’ shapes and sizes, observed in the visible wavelength range.
Armin Afchine, Christian Rolf, Anja Costa, Nicole Spelten, Martin Riese, Bernhard Buchholz, Volker Ebert, Romy Heller, Stefan Kaufmann, Andreas Minikin, Christiane Voigt, Martin Zöger, Jessica Smith, Paul Lawson, Alexey Lykov, Sergey Khaykin, and Martina Krämer
Atmos. Meas. Tech., 11, 4015–4031, https://doi.org/10.5194/amt-11-4015-2018, https://doi.org/10.5194/amt-11-4015-2018, 2018
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The ice water content (IWC) of cirrus clouds is an essential parameter that determines their radiative properties and is thus important for climate simulations. Experimental investigations of IWCs measured on board research aircraft reveal that their accuracy is influenced by the sampling position. IWCs detected at the aircraft roof deviate significantly from wing, side or bottom IWCs. The reasons are deflections of the gas streamlines and ice particle trajectories behind the aircraft cockpit.
Stephan E. Bansmer, Arne Baumert, Stephan Sattler, Inken Knop, Delphine Leroy, Alfons Schwarzenboeck, Tina Jurkat-Witschas, Christiane Voigt, Hugo Pervier, and Biagio Esposito
Atmos. Meas. Tech., 11, 3221–3249, https://doi.org/10.5194/amt-11-3221-2018, https://doi.org/10.5194/amt-11-3221-2018, 2018
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Snow, frost formation and ice cubes in our drinks are part of our daily life. But what about our technical innovations like aviation, electrical power transmission and wind-energy production, can they cope with icing? Icing Wind Tunnels are an ideal laboratory environment to answer that question. In this paper, we show how the icing wind tunnel in Braunschweig (Germany) was built and how we can use it for engineering and climate research.
Klaus-Dirk Gottschaldt, Hans Schlager, Robert Baumann, Duy Sinh Cai, Veronika Eyring, Phoebe Graf, Volker Grewe, Patrick Jöckel, Tina Jurkat-Witschas, Christiane Voigt, Andreas Zahn, and Helmut Ziereis
Atmos. Chem. Phys., 18, 5655–5675, https://doi.org/10.5194/acp-18-5655-2018, https://doi.org/10.5194/acp-18-5655-2018, 2018
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This study places aircraft trace gas measurements from within the Asian summer monsoon anticyclone into the context of regional, intra- and interannual variability. We find that the processes reflected in the measurements are present throughout multiple simulated monsoon seasons. Dynamical instabilities, photochemical ozone production, lightning and entrainments from the lower troposphere and from the tropopause region determine the distinct composition of the anticyclone and its outflow.
Trismono C. Krisna, Manfred Wendisch, André Ehrlich, Evelyn Jäkel, Frank Werner, Ralf Weigel, Stephan Borrmann, Christoph Mahnke, Ulrich Pöschl, Meinrat O. Andreae, Christiane Voigt, and Luiz A. T. Machado
Atmos. Chem. Phys., 18, 4439–4462, https://doi.org/10.5194/acp-18-4439-2018, https://doi.org/10.5194/acp-18-4439-2018, 2018
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The optical thickness and particle effective radius of a cirrus above liquid water clouds and a DCC topped by an anvil cirrus are retrieved based on SMART and MODIS radiance measurements. For the cirrus, retrieved particle effective radius are validated with corresponding in situ data using a vertical weighting method. This approach allows to assess the measurements, retrieval algorithms, and derived cloud products.
Meinrat O. Andreae, Armin Afchine, Rachel Albrecht, Bruna Amorim Holanda, Paulo Artaxo, Henrique M. J. Barbosa, Stephan Borrmann, Micael A. Cecchini, Anja Costa, Maximilian Dollner, Daniel Fütterer, Emma Järvinen, Tina Jurkat, Thomas Klimach, Tobias Konemann, Christoph Knote, Martina Krämer, Trismono Krisna, Luiz A. T. Machado, Stephan Mertes, Andreas Minikin, Christopher Pöhlker, Mira L. Pöhlker, Ulrich Pöschl, Daniel Rosenfeld, Daniel Sauer, Hans Schlager, Martin Schnaiter, Johannes Schneider, Christiane Schulz, Antonio Spanu, Vinicius B. Sperling, Christiane Voigt, Adrian Walser, Jian Wang, Bernadett Weinzierl, Manfred Wendisch, and Helmut Ziereis
Atmos. Chem. Phys., 18, 921–961, https://doi.org/10.5194/acp-18-921-2018, https://doi.org/10.5194/acp-18-921-2018, 2018
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We made airborne measurements of aerosol particle concentrations and properties over the Amazon Basin. We found extremely high concentrations of very small particles in the region between 8 and 14 km altitude all across the basin, which had been recently formed by gas-to-particle conversion at these altitudes. This makes the upper troposphere a very important source region of atmospheric particles with significant implications for the Earth's climate system.
Volker Freudenthaler, Holger Linné, Anatoli Chaikovski, Dieter Rabus, and Silke Groß
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2017-395, https://doi.org/10.5194/amt-2017-395, 2018
Revised manuscript has not been submitted
Romy Heller, Christiane Voigt, Stuart Beaton, Andreas Dörnbrack, Andreas Giez, Stefan Kaufmann, Christian Mallaun, Hans Schlager, Johannes Wagner, Kate Young, and Markus Rapp
Atmos. Chem. Phys., 17, 14853–14869, https://doi.org/10.5194/acp-17-14853-2017, https://doi.org/10.5194/acp-17-14853-2017, 2017
Ramon Campos Braga, Daniel Rosenfeld, Ralf Weigel, Tina Jurkat, Meinrat O. Andreae, Manfred Wendisch, Ulrich Pöschl, Christiane Voigt, Christoph Mahnke, Stephan Borrmann, Rachel I. Albrecht, Sergej Molleker, Daniel A. Vila, Luiz A. T. Machado, and Lucas Grulich
Atmos. Chem. Phys., 17, 14433–14456, https://doi.org/10.5194/acp-17-14433-2017, https://doi.org/10.5194/acp-17-14433-2017, 2017
Johan Strandgren, Jennifer Fricker, and Luca Bugliaro
Atmos. Meas. Tech., 10, 4317–4339, https://doi.org/10.5194/amt-10-4317-2017, https://doi.org/10.5194/amt-10-4317-2017, 2017
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We characterise the the performance of a set of artificial neural networks used for the remote sensing of cirrus clouds from the geostationary Meteosat Second Generation satellites. The retrievals show little interference with the underlying land surface type as well as with possible liquid water clouds or aerosol layers below the cirrus cloud. We also characterise the retrievals as a funtion of optical thickness and top height and gain better understanding of the retrival uncertainties of CiPS
Tilman Hüneke, Oliver-Alex Aderhold, Jannik Bounin, Marcel Dorf, Eric Gentry, Katja Grossmann, Jens-Uwe Grooß, Peter Hoor, Patrick Jöckel, Mareike Kenntner, Marvin Knapp, Matthias Knecht, Dominique Lörks, Sabrina Ludmann, Sigrun Matthes, Rasmus Raecke, Marcel Reichert, Jannis Weimar, Bodo Werner, Andreas Zahn, Helmut Ziereis, and Klaus Pfeilsticker
Atmos. Meas. Tech., 10, 4209–4234, https://doi.org/10.5194/amt-10-4209-2017, https://doi.org/10.5194/amt-10-4209-2017, 2017
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This paper describes a novel instrument for the aircraft-borne remote sensing of trace gases and liquid and solid water. Until recently, such measurements could only be evaluated under clear-sky conditions. We present a characterization and error assessment of the novel "scaling method", which allows for the retrieval of absolute trace gas concentrations under all sky conditions, significantly expanding the applicability of such measurements to study atmospheric photochemistry.
Johan Strandgren, Luca Bugliaro, Frank Sehnke, and Leon Schröder
Atmos. Meas. Tech., 10, 3547–3573, https://doi.org/10.5194/amt-10-3547-2017, https://doi.org/10.5194/amt-10-3547-2017, 2017
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The new algorithm CiPS is presented and validated. CiPS detects cirrus clouds, identifies opaque pixels and retrieves the corresponding optical thickness, cloud top height and ice water path from the geostationary imager MSG/SEVIRI. CiPS utilises a set of four artificial neural networks trained with space-borne lidar data, thermal MSG/SEVIRI observations, model data and auxiliary data.
To demonstrate the capabilities of CiPS, the life cycle of a thin cirrus cloud is analysed.
Moritz Haarig, Albert Ansmann, Dietrich Althausen, André Klepel, Silke Groß, Volker Freudenthaler, Carlos Toledano, Rodanthi-Elisavet Mamouri, David A. Farrell, Damien A. Prescod, Eleni Marinou, Sharon P. Burton, Josef Gasteiger, Ronny Engelmann, and Holger Baars
Atmos. Chem. Phys., 17, 10767–10794, https://doi.org/10.5194/acp-17-10767-2017, https://doi.org/10.5194/acp-17-10767-2017, 2017
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Our measurements performed with a lidar on Barbados give a vertical profile of Saharan dust, which was transported over 5000 km across the Atlantic. The new triple-wavelength depolarization technique reveals more information about the shape and size of dust, which will improve our understanding of the aging process of dust in the atmosphere and its representation in dust models. Changing properties of dust particles influence the solar radiation and the cloud properties and thus our climate.
Micael A. Cecchini, Luiz A. T. Machado, Meinrat O. Andreae, Scot T. Martin, Rachel I. Albrecht, Paulo Artaxo, Henrique M. J. Barbosa, Stephan Borrmann, Daniel Fütterer, Tina Jurkat, Christoph Mahnke, Andreas Minikin, Sergej Molleker, Mira L. Pöhlker, Ulrich Pöschl, Daniel Rosenfeld, Christiane Voigt, Bernadett Weinzierl, and Manfred Wendisch
Atmos. Chem. Phys., 17, 10037–10050, https://doi.org/10.5194/acp-17-10037-2017, https://doi.org/10.5194/acp-17-10037-2017, 2017
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We study the effects of aerosol particles and updraft speed on the warm phase of Amazonian clouds. We expand the sensitivity analysis usually found in the literature by concomitantly considering cloud evolution and the effects on droplet size distribution (DSD) shape. The quantitative results show that particle concentration is the primary driver for the vertical profiles of effective diameter and droplet concentration in the warm phase of Amazonian convective clouds.
Evelyn Jäkel, Manfred Wendisch, Trismono C. Krisna, Florian Ewald, Tobias Kölling, Tina Jurkat, Christiane Voigt, Micael A. Cecchini, Luiz A. T. Machado, Armin Afchine, Anja Costa, Martina Krämer, Meinrat O. Andreae, Ulrich Pöschl, Daniel Rosenfeld, and Tianle Yuan
Atmos. Chem. Phys., 17, 9049–9066, https://doi.org/10.5194/acp-17-9049-2017, https://doi.org/10.5194/acp-17-9049-2017, 2017
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Vertical profiles of the cloud particle phase state in tropical deep convective clouds (DCCs) were investigated using airborne imaging spectrometer measurements during the ACRIDICON-CHUVA campaign, which was conducted over the Brazilian rainforest in September 2014. A phase discrimination retrieval was applied to observations of clouds formed in different aerosol conditions. The profiles were compared to in situ and satellite measurements.
Marianne T. Lund, Borgar Aamaas, Terje Berntsen, Lisa Bock, Ulrike Burkhardt, Jan S. Fuglestvedt, and Keith P. Shine
Earth Syst. Dynam., 8, 547–563, https://doi.org/10.5194/esd-8-547-2017, https://doi.org/10.5194/esd-8-547-2017, 2017
Ramon Campos Braga, Daniel Rosenfeld, Ralf Weigel, Tina Jurkat, Meinrat O. Andreae, Manfred Wendisch, Mira L. Pöhlker, Thomas Klimach, Ulrich Pöschl, Christopher Pöhlker, Christiane Voigt, Christoph Mahnke, Stephan Borrmann, Rachel I. Albrecht, Sergej Molleker, Daniel A. Vila, Luiz A. T. Machado, and Paulo Artaxo
Atmos. Chem. Phys., 17, 7365–7386, https://doi.org/10.5194/acp-17-7365-2017, https://doi.org/10.5194/acp-17-7365-2017, 2017
Klaus-D. Gottschaldt, Hans Schlager, Robert Baumann, Heiko Bozem, Veronika Eyring, Peter Hoor, Patrick Jöckel, Tina Jurkat, Christiane Voigt, Andreas Zahn, and Helmut Ziereis
Atmos. Chem. Phys., 17, 6091–6111, https://doi.org/10.5194/acp-17-6091-2017, https://doi.org/10.5194/acp-17-6091-2017, 2017
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We present upper-tropospheric trace gas measurements in the Asian summer monsoon anticyclone, obtained with the HALO research aircraft in September 2012. The anticyclone is one of the largest atmospheric features on Earth, but many aspects of it are not well understood. With the help of model simulations we find that entrainments from the tropopause region and the lower troposphere, combined with photochemistry and dynamical instabilities, can explain the observations.
Benedikt Urbanek, Silke Groß, Andreas Schäfler, and Martin Wirth
Atmos. Meas. Tech., 10, 1653–1664, https://doi.org/10.5194/amt-10-1653-2017, https://doi.org/10.5194/amt-10-1653-2017, 2017
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Cirrus evolution from nucleation to cloud breakup can be investigated with a novel classification scheme based on airborne lidar data. Applying it to a case study from the ML-CIRRUS campaign, we investigate the impact of large-scale dynamics and small-scale gravity lee waves on the detailed spatial distribution of evolution stages in individual clouds. Our scheme may help to gain more insights in optical and radiative properties of cirrus under various formation and life cycle conditions.
Kevin Wolf, André Ehrlich, Tilman Hüneke, Klaus Pfeilsticker, Frank Werner, Martin Wirth, and Manfred Wendisch
Atmos. Chem. Phys., 17, 4283–4303, https://doi.org/10.5194/acp-17-4283-2017, https://doi.org/10.5194/acp-17-4283-2017, 2017
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The potential of airborne radiance measurements in the sideward and nadir directions for cirrus remote sensing is investigated. Therefore radiative transfer simulations were used and the sensitivity of upward radiance with respect to optical thickness, effective radius, surface albedo, wavelength and viewing angle was studied. It was shown that sideward observations lead to more accurate retrieval results. Investigating a case study of ML-CIRRUS, these findings are confirmed.
Ulrich Schumann, Christoph Kiemle, Hans Schlager, Ralf Weigel, Stephan Borrmann, Francesco D'Amato, Martina Krämer, Renaud Matthey, Alain Protat, Christiane Voigt, and C. Michael Volk
Atmos. Chem. Phys., 17, 2311–2346, https://doi.org/10.5194/acp-17-2311-2017, https://doi.org/10.5194/acp-17-2311-2017, 2017
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A long-lived (1 h) contrail and overshooting convection were observed in the tropics, near Darwin, Australia. The data are used to study the contrail life cycle at low temperatures and cirrus from deep overturning convection in the lower tropical stratosphere. Airborne in situ, lidar, profiler, radar, and satellite data, as well as a photo, are used to distinguish contrail cirrus from convective cirrus and to study the origin of the observed ice and aerosol, up to 2.3 km above the tropopause.
Tobias Sirch, Luca Bugliaro, Tobias Zinner, Matthias Möhrlein, and Margarita Vazquez-Navarro
Atmos. Meas. Tech., 10, 409–429, https://doi.org/10.5194/amt-10-409-2017, https://doi.org/10.5194/amt-10-409-2017, 2017
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A novel approach for the nowcasting of clouds and direct normal irradiance (DNI) based on the geostationary satellite MSG is presented. The basis of the algorithm is an optical flow method to derive cloud motion vectors for low and high level clouds separately. DNI is calculated from the forecasted optical thickness of the clouds. Validation against MSG observations shows good performance: compared to persistence an improvement of forecast horizon by a factor of 2 is reached for 2 h forecasts.
Ulrich Schumann, Robert Baumann, Darrel Baumgardner, Sarah T. Bedka, David P. Duda, Volker Freudenthaler, Jean-Francois Gayet, Andrew J. Heymsfield, Patrick Minnis, Markus Quante, Ehrhard Raschke, Hans Schlager, Margarita Vázquez-Navarro, Christiane Voigt, and Zhien Wang
Atmos. Chem. Phys., 17, 403–438, https://doi.org/10.5194/acp-17-403-2017, https://doi.org/10.5194/acp-17-403-2017, 2017
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The initially linear clouds often seen behind aircraft are known as contrails. Contrails are prototype cirrus clouds forming under well-known conditions, but with less certain life cycle and climate effects. This paper collects contrail data from a large set of measurements and compares them among each other and with models. The observations show consistent contrail properties over a wide range of aircraft and atmosphere conditions. The dataset is available for further research.
Josef Gasteiger, Silke Groß, Daniel Sauer, Moritz Haarig, Albert Ansmann, and Bernadett Weinzierl
Atmos. Chem. Phys., 17, 297–311, https://doi.org/10.5194/acp-17-297-2017, https://doi.org/10.5194/acp-17-297-2017, 2017
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To study aerosol transport in the Saharan Air Layer (SAL) from Africa to the Caribbean, we combine advanced optical models of Saharan aerosols with Stokes settling and two hypotheses about the occurrence of vertical mixing. By testing our hypotheses with lidar and in situ profiles measured near the top of the transported SAL, we find strong evidence that vertical mixing occurs in the SAL over the Atlantic with significant consequences for size distribution of the transported Saharan aerosols.
Christiane Voigt, Andreas Dörnbrack, Martin Wirth, Silke M. Groß, Robert Baumann, Benedikt Ehard, Michael C. Pitts, Lamont R. Poole, Björn-Martin Sinnhuber, and Hermann Oelhaf
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-1082, https://doi.org/10.5194/acp-2016-1082, 2016
Revised manuscript not accepted
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The letter describes unprecedented observations of widespread and persistent polar stratospheric ice clouds (ice PSCs) in the exceptionally cold Arctic stratospheric winter 2015/16. The unique observations are of global relevance because trends in Arctic ozone loss and in polar temperatures are highly uncertain. The new observations at cold conditions serve to enhance our knowledge on ice PSC formation, Arctic ozone loss and polar stratrospheric temperatures in a changing climate.
Manuel Gutleben, Silke Gross, Martin Wirth, and Andreas Schäfler
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2016-333, https://doi.org/10.5194/amt-2016-333, 2016
Revised manuscript not accepted
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Shallow marine cumulus convection over the Atlantic ocean is studied with observations by airborne and spaceborne lidar instruments. Cloud top height as well as cloud length and cloud gap length distributions are calculated by use of a newly developed algorithm. The distribution of cloud top heights during wintertime measurements shows a two-layer structure. However, significant differences in cloud top height distributions compared to summertime measurements are found.
Ralf Weigel, Peter Spichtinger, Christoph Mahnke, Marcus Klingebiel, Armin Afchine, Andreas Petzold, Martina Krämer, Anja Costa, Sergej Molleker, Philipp Reutter, Miklós Szakáll, Max Port, Lucas Grulich, Tina Jurkat, Andreas Minikin, and Stephan Borrmann
Atmos. Meas. Tech., 9, 5135–5162, https://doi.org/10.5194/amt-9-5135-2016, https://doi.org/10.5194/amt-9-5135-2016, 2016
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The subject of our study concerns measurements with optical array probes (OAPs) on fast-flying aircraft such as the G550 (HALO or HIAPER). At up to Mach 0.7 the effect of air compression upstream of underwing-mounted instruments and particles' inertia need consideration for determining ambient particle concentrations. Compared to conventional practices the introduced correction procedure eliminates ambiguities and exhibits consistency over flight speeds between 50 and 250 m s−.
Valery Shcherbakov, Olivier Jourdan, Christiane Voigt, Jean-Francois Gayet, Aurélien Chauvigne, Alfons Schwarzenboeck, Andreas Minikin, Marcus Klingebiel, Ralf Weigel, Stephan Borrmann, Tina Jurkat, Stefan Kaufmann, Romy Schlage, Christophe Gourbeyre, Guy Febvre, Tatyana Lapyonok, Wiebke Frey, Sergej Molleker, and Bernadett Weinzierl
Atmos. Chem. Phys., 16, 11883–11897, https://doi.org/10.5194/acp-16-11883-2016, https://doi.org/10.5194/acp-16-11883-2016, 2016
Tobias Zinner, Petra Hausmann, Florian Ewald, Luca Bugliaro, Claudia Emde, and Bernhard Mayer
Atmos. Meas. Tech., 9, 4615–4632, https://doi.org/10.5194/amt-9-4615-2016, https://doi.org/10.5194/amt-9-4615-2016, 2016
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A new retrieval of optical thickness and effective particle size of ice clouds over a wide range of optical thickness from transmittance measurements is presented. A visible range spectral slope is used to resolve the transmittance optical thickness ambiguity. Retrieval sensitivity to ice crystal habit, aerosol, albedo, sensor accuracy and lookup table interpolation is presented as well as an application of the method and comparison to satellite products for 2 days.
Silke Groß, Josef Gasteiger, Volker Freudenthaler, Thomas Müller, Daniel Sauer, Carlos Toledano, and Albert Ansmann
Atmos. Chem. Phys., 16, 11535–11546, https://doi.org/10.5194/acp-16-11535-2016, https://doi.org/10.5194/acp-16-11535-2016, 2016
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Dual-wavelength depolarization sensitive Raman lidar measurements were used to characterize the optical properties of the dust loaded convective boundary layer over the Caribbean. Furthermore we derived the dust volume fraction and dust mass concentration within the convective boundary layer.
Claudia Emde, Robert Buras-Schnell, Arve Kylling, Bernhard Mayer, Josef Gasteiger, Ulrich Hamann, Jonas Kylling, Bettina Richter, Christian Pause, Timothy Dowling, and Luca Bugliaro
Geosci. Model Dev., 9, 1647–1672, https://doi.org/10.5194/gmd-9-1647-2016, https://doi.org/10.5194/gmd-9-1647-2016, 2016
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libradtran is a widely used software package for radiative transfer calculations. It allows one to compute (polarized) radiances, irradiance, and actinic fluxes in the solar and thermal spectral regions. This paper gives an overview of libradtran version 2.0 with focus on new features (e.g. polarization, Raman scattering, absorption parameterization, cloud and aerosol optical properties). libRadtran is freely available at http://www.libradtran.org.
Tina Jurkat, Stefan Kaufmann, Christiane Voigt, Dominik Schäuble, Philipp Jeßberger, and Helmut Ziereis
Atmos. Meas. Tech., 9, 1907–1923, https://doi.org/10.5194/amt-9-1907-2016, https://doi.org/10.5194/amt-9-1907-2016, 2016
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The paper details novel mass spectrometric measurements with AIMS-TG aboard the new German research aircraft HALO. The measurements comprise a wide range of tracers with characteristic source regions. Using these tracers, stratospheric and tropospheric air in the UTLS is tagged. The instrument is equipped with a new discharge ionization source, an in-flight calibration and improved transmission of adhesive gases like HNO3 and HCl. AIMS was built to characterize transport and mixing in the UTLS.
Andreas Weigelt, Ralf Ebinghaus, Nicola Pirrone, Johannes Bieser, Jan Bödewadt, Giulio Esposito, Franz Slemr, Peter F. J. van Velthoven, Andreas Zahn, and Helmut Ziereis
Atmos. Chem. Phys., 16, 4135–4146, https://doi.org/10.5194/acp-16-4135-2016, https://doi.org/10.5194/acp-16-4135-2016, 2016
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We show the first mercury profile measurements over Europe since 1996. Besides gaseous elemental mercury (GEM) and total gaseous mercury (TGM), the gases CO, SO2, NOx, and O3 were measured from aboard a research aircraft over four European locations. Compared to the boundary layer, the concentration of GEM and TGM in the free troposphere was 10–30% lower. Inside the individual layers no vertical gradient was apparent. Combined with CARIBIC data, a unique profile from 0.4 to 10.5 km is provided.
Armin Rauthe-Schöch, Angela K. Baker, Tanja J. Schuck, Carl A. M. Brenninkmeijer, Andreas Zahn, Markus Hermann, Greta Stratmann, Helmut Ziereis, Peter F. J. van Velthoven, and Jos Lelieveld
Atmos. Chem. Phys., 16, 3609–3629, https://doi.org/10.5194/acp-16-3609-2016, https://doi.org/10.5194/acp-16-3609-2016, 2016
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The flying laboratory CARIBIC onboard a passenger aircraft measured trace gases and aerosol particles in the upper tropospheric Indian summer monsoon anticyclone in summer 2008. We used the measurements together with meteorological analyses to investigate the chemical signature of the northern and southern part of the monsoon, the source regions from where the air was entrained into the monsoon and which parts of the world received polluted air that had been chemically processed in the monsoon.
Ulla Wandinger, Volker Freudenthaler, Holger Baars, Aldo Amodeo, Ronny Engelmann, Ina Mattis, Silke Groß, Gelsomina Pappalardo, Aldo Giunta, Giuseppe D'Amico, Anatoli Chaikovsky, Fiodor Osipenko, Alexander Slesar, Doina Nicolae, Livio Belegante, Camelia Talianu, Ilya Serikov, Holger Linné, Friedhelm Jansen, Arnoud Apituley, Keith M. Wilson, Martin de Graaf, Thomas Trickl, Helmut Giehl, Mariana Adam, Adolfo Comerón, Constantino Muñoz-Porcar, Francesc Rocadenbosch, Michaël Sicard, Sergio Tomás, Diego Lange, Dhiraj Kumar, Manuel Pujadas, Francisco Molero, Alfonso J. Fernández, Lucas Alados-Arboledas, Juan Antonio Bravo-Aranda, Francisco Navas-Guzmán, Juan Luis Guerrero-Rascado, María José Granados-Muñoz, Jana Preißler, Frank Wagner, Michael Gausa, Ivan Grigorov, Dimitar Stoyanov, Marco Iarlori, Vincenco Rizi, Nicola Spinelli, Antonella Boselli, Xuan Wang, Teresa Lo Feudo, Maria Rita Perrone, Ferdinando De Tomasi, and Pasquale Burlizzi
Atmos. Meas. Tech., 9, 1001–1023, https://doi.org/10.5194/amt-9-1001-2016, https://doi.org/10.5194/amt-9-1001-2016, 2016
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We introduce the quality-assurance efforts of the European Aerosol Research Lidar Network (EARLINET) at instrument level. Within several campaigns, 21 EARLINET systems from 18 EARLINET stations were intercompared. A comprehensive strategy for campaign setup and data evaluation was established. The intercomparisons have reinforced our confidence in the EARLINET data quality and allowed us to draw conclusions on necessary system improvements and to identify major challenges for our future work.
Stefan Kaufmann, Christiane Voigt, Tina Jurkat, Troy Thornberry, David W. Fahey, Ru-Shan Gao, Romy Schlage, Dominik Schäuble, and Martin Zöger
Atmos. Meas. Tech., 9, 939–953, https://doi.org/10.5194/amt-9-939-2016, https://doi.org/10.5194/amt-9-939-2016, 2016
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We present the development of a new airborne mass spectrometer AIMS-H2O for the fast and accurate measurement of water vapor in the upper troposphere and lower stratosphere. The high accuracy needed for e.g. quantification of atmospheric water vapor transport processes or cloud formation is achieved by an in-flight calibration of the instrument. AIMS-H2O is deployed on the DLR research aircraft HALO and Falcon where it covers a range of water vapor mixing ratios from 1 to 500 ppmv.
S. Groß, V. Freudenthaler, K. Schepanski, C. Toledano, A. Schäfler, A. Ansmann, and B. Weinzierl
Atmos. Chem. Phys., 15, 11067–11080, https://doi.org/10.5194/acp-15-11067-2015, https://doi.org/10.5194/acp-15-11067-2015, 2015
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In June and July 2013 dual-wavelength lidar measurements were performed in Barbados to study long-range transported Saharan dust across the Atlantic Ocean and investigate transport-induced changes. The focus of our measurements is the intensive optical properties, the lidar ratio and the particle linear depolarization ratio. While the lidar ratio shows no differences compared to the values of fresh Saharan dust, the particle linear depolarization ratio shows slight differences.
F. Chouza, O. Reitebuch, S. Groß, S. Rahm, V. Freudenthaler, C. Toledano, and B. Weinzierl
Atmos. Meas. Tech., 8, 2909–2926, https://doi.org/10.5194/amt-8-2909-2015, https://doi.org/10.5194/amt-8-2909-2015, 2015
J. Ungermann, J. Blank, M. Dick, A. Ebersoldt, F. Friedl-Vallon, A. Giez, T. Guggenmoser, M. Höpfner, T. Jurkat, M. Kaufmann, S. Kaufmann, A. Kleinert, M. Krämer, T. Latzko, H. Oelhaf, F. Olchewski, P. Preusse, C. Rolf, J. Schillings, O. Suminska-Ebersoldt, V. Tan, N. Thomas, C. Voigt, A. Zahn, M. Zöger, and M. Riese
Atmos. Meas. Tech., 8, 2473–2489, https://doi.org/10.5194/amt-8-2473-2015, https://doi.org/10.5194/amt-8-2473-2015, 2015
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The GLORIA sounder is an airborne infrared limb-imager combining a two-dimensional infrared detector with a Fourier transform spectrometer. It was operated aboard the new German Gulfstream G550 research aircraft HALO during the TACTS and ESMVAL campaigns in summer 2012. This paper describes the retrieval of temperature, as well as H2O, HNO3, and O3 cross sections from GLORIA dynamics mode spectra. A high correlation is achieved between the remote sensing and the in situ trace gas measurements.
S. Kox, L. Bugliaro, and A. Ostler
Atmos. Meas. Tech., 7, 3233–3246, https://doi.org/10.5194/amt-7-3233-2014, https://doi.org/10.5194/amt-7-3233-2014, 2014
U. Hamann, A. Walther, B. Baum, R. Bennartz, L. Bugliaro, M. Derrien, P. N. Francis, A. Heidinger, S. Joro, A. Kniffka, H. Le Gléau, M. Lockhoff, H.-J. Lutz, J. F. Meirink, P. Minnis, R. Palikonda, R. Roebeling, A. Thoss, S. Platnick, P. Watts, and G. Wind
Atmos. Meas. Tech., 7, 2839–2867, https://doi.org/10.5194/amt-7-2839-2014, https://doi.org/10.5194/amt-7-2839-2014, 2014
S. Groß, M. Wirth, A. Schäfler, A. Fix, S. Kaufmann, and C. Voigt
Atmos. Meas. Tech., 7, 2745–2755, https://doi.org/10.5194/amt-7-2745-2014, https://doi.org/10.5194/amt-7-2745-2014, 2014
K.-P. Heue, H. Riede, D. Walter, C. A. M. Brenninkmeijer, T. Wagner, U. Frieß, U. Platt, A. Zahn, G. Stratmann, and H. Ziereis
Atmos. Chem. Phys., 14, 6621–6642, https://doi.org/10.5194/acp-14-6621-2014, https://doi.org/10.5194/acp-14-6621-2014, 2014
F. Dahlkötter, M. Gysel, D. Sauer, A. Minikin, R. Baumann, P. Seifert, A. Ansmann, M. Fromm, C. Voigt, and B. Weinzierl
Atmos. Chem. Phys., 14, 6111–6137, https://doi.org/10.5194/acp-14-6111-2014, https://doi.org/10.5194/acp-14-6111-2014, 2014
B. Reinhardt, R. Buras, L. Bugliaro, S. Wilbert, and B. Mayer
Atmos. Meas. Tech., 7, 823–838, https://doi.org/10.5194/amt-7-823-2014, https://doi.org/10.5194/amt-7-823-2014, 2014
J. E. Williams, G. Le Bras, A. Kukui, H. Ziereis, and C. A. M. Brenninkmeijer
Atmos. Chem. Phys., 14, 2363–2382, https://doi.org/10.5194/acp-14-2363-2014, https://doi.org/10.5194/acp-14-2363-2014, 2014
J.-F. Gayet, V. Shcherbakov, L. Bugliaro, A. Protat, J. Delanoë, J. Pelon, and A. Garnier
Atmos. Chem. Phys., 14, 899–912, https://doi.org/10.5194/acp-14-899-2014, https://doi.org/10.5194/acp-14-899-2014, 2014
P. Jeßberger, C. Voigt, U. Schumann, I. Sölch, H. Schlager, S. Kaufmann, A. Petzold, D. Schäuble, and J.-F. Gayet
Atmos. Chem. Phys., 13, 11965–11984, https://doi.org/10.5194/acp-13-11965-2013, https://doi.org/10.5194/acp-13-11965-2013, 2013
T. D. Thornberry, A. W. Rollins, R. S. Gao, L. A. Watts, S. J. Ciciora, R. J. McLaughlin, C. Voigt, B. Hall, and D. W. Fahey
Atmos. Meas. Tech., 6, 1461–1475, https://doi.org/10.5194/amt-6-1461-2013, https://doi.org/10.5194/amt-6-1461-2013, 2013
G. Pappalardo, L. Mona, G. D'Amico, U. Wandinger, M. Adam, A. Amodeo, A. Ansmann, A. Apituley, L. Alados Arboledas, D. Balis, A. Boselli, J. A. Bravo-Aranda, A. Chaikovsky, A. Comeron, J. Cuesta, F. De Tomasi, V. Freudenthaler, M. Gausa, E. Giannakaki, H. Giehl, A. Giunta, I. Grigorov, S. Groß, M. Haeffelin, A. Hiebsch, M. Iarlori, D. Lange, H. Linné, F. Madonna, I. Mattis, R.-E. Mamouri, M. A. P. McAuliffe, V. Mitev, F. Molero, F. Navas-Guzman, D. Nicolae, A. Papayannis, M. R. Perrone, C. Pietras, A. Pietruczuk, G. Pisani, J. Preißler, M. Pujadas, V. Rizi, A. A. Ruth, J. Schmidt, F. Schnell, P. Seifert, I. Serikov, M. Sicard, V. Simeonov, N. Spinelli, K. Stebel, M. Tesche, T. Trickl, X. Wang, F. Wagner, M. Wiegner, and K. M. Wilson
Atmos. Chem. Phys., 13, 4429–4450, https://doi.org/10.5194/acp-13-4429-2013, https://doi.org/10.5194/acp-13-4429-2013, 2013
K. Gottschaldt, C. Voigt, P. Jöckel, M. Righi, R. Deckert, and S. Dietmüller
Atmos. Chem. Phys., 13, 3003–3025, https://doi.org/10.5194/acp-13-3003-2013, https://doi.org/10.5194/acp-13-3003-2013, 2013
S. Groß, M. Esselborn, B. Weinzierl, M. Wirth, A. Fix, and A. Petzold
Atmos. Chem. Phys., 13, 2487–2505, https://doi.org/10.5194/acp-13-2487-2013, https://doi.org/10.5194/acp-13-2487-2013, 2013
S. Groß, M. Esselborn, F. Abicht, M. Wirth, A. Fix, and A. Minikin
Atmos. Chem. Phys., 13, 2435–2444, https://doi.org/10.5194/acp-13-2435-2013, https://doi.org/10.5194/acp-13-2435-2013, 2013
F. Ewald, L. Bugliaro, H. Mannstein, and B. Mayer
Atmos. Meas. Tech., 6, 309–322, https://doi.org/10.5194/amt-6-309-2013, https://doi.org/10.5194/amt-6-309-2013, 2013
Related subject area
Subject: Clouds and Precipitation | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Air mass history linked to the development of Arctic mixed-phase clouds
Distinct structure, radiative effects, and precipitation characteristics of deep convection systems in the Tibetan Plateau compared to the tropical Indian Ocean
The correlation between Arctic sea ice, cloud phase and radiation using A-Train satellites
Technical note: Retrieval of the supercooled liquid fraction in mixed-phase clouds from Himawari-8 observations
Characterisation of low-base and mid-base clouds and their thermodynamic phase over the Southern Ocean and Arctic marine regions
Technical note: Applicability of physics-based and machine-learning-based algorithms of geostationary satellite in retrieving the diurnal cycle of cloud base height
A survey of radiative and physical properties of North Atlantic mesoscale cloud morphologies from multiple identification methodologies
Extensive coverage of ultrathin tropical tropopause layer cirrus clouds revealed by balloon-borne lidar observations
The effects of warm-air intrusions in the high Arctic on cirrus clouds
Observing convective activities in the complex organizations and their contributions to the precipitation and anvil amount
The characteristics of cloud macro-parameters caused by the seeder–feeder process inside clouds measured by millimeter-wave cloud radar in Xi'an, China
Weak liquid water path response in ship tracks
Shallow- and deep-convection characteristics in the greater Houston, Texas, area using cell tracking methodology
Observations of the macrophysical properties of cumulus cloud fields over the tropical western Pacific and their connection to meteorological variables
A Lagrangian perspective on the lifecycle and cloud radiative effect of deep convective clouds over Africa
How does the lifetime of detrained cirrus impact the high cloud radiative effect in the tropics?
Daytime variation in the aerosol indirect effect for warm marine boundary layer clouds in the eastern North Atlantic
Technical note: Bimodal parameterizations of in situ ice cloud particle size distributions
Inter-relations of precipitation, aerosols, and clouds over Andalusia, southern Spain, revealed by the Andalusian Global ObseRvatory of the Atmosphere (AGORA)
On the relationship between mesoscale cellular convection and meteorological forcing: comparing the Southern Ocean against the North Pacific
Aerosol-related effects on the occurrence of heterogeneous ice formation over Lauder, New Zealand ∕ Aotearoa
Low-level Arctic clouds: a blind zone in our knowledge of the radiation budget
Climatologically invariant scale invariance seen in distributions of cloud horizontal sizes
Variability and properties of liquid-dominated clouds over the ice-free and sea-ice-covered Arctic Ocean
Asymmetries in cloud microphysical properties ascribed to sea ice leads via water vapour transport in the central Arctic
Quantifying the dependence of drop spectrum width on cloud drop number concentration for cloud remote sensing
The evolution of deep convective systems and their associated cirrus outflows
Wildfire smoke triggers cirrus formation: lidar observations over the eastern Mediterranean
Rapid saturation of cloud water adjustments to shipping emissions
Sensitivities of cloud radiative effects to large-scale meteorology and aerosols from global observations
Distinct secondary ice production processes observed in radar Doppler spectra: insights from a case study
Investigating the development of clouds within marine cold-air outbreaks
Detection of large-scale cloud microphysical changes within a major shipping corridor after implementation of the International Maritime Organization 2020 fuel sulfur regulations
Examining cloud vertical structure and radiative effects from satellite retrievals and evaluation of CMIP6 scenarios
Influence of cloud microphysics schemes on weather model predictions of heavy precipitation
Convective organization and 3D structure of tropical cloud systems deduced from synergistic A-Train observations and machine learning
Seasonal controls on isolated convective storm drafts, precipitation intensity, and life cycle as observed during GoAmazon2014/5
Uncertainty in aerosol–cloud radiative forcing is driven by clean conditions
Surface-based observations of cold-air outbreak clouds during the COMBLE field campaign
Boundary layer moisture variability at the Atmospheric Radiation Measurement (ARM) Eastern North Atlantic observatory during marine conditions
Profile-based estimated inversion strength
Characteristics of supersaturation in midlatitude cirrus clouds and their adjacent cloud-free air
Establishment of an analytical model for remote sensing of typical stratocumulus cloud profiles under various precipitation and entrainment conditions
Satellite remote sensing of regional and seasonal Arctic cooling showing a multi-decadal trend towards brighter and more liquid clouds
Microphysical processes of super typhoon Lekima (2019) and their impacts on polarimetric radar remote sensing of precipitation
The impacts of dust aerosol and convective available potential energy on precipitation vertical structure in southeastern China as seen from multisource observations
Heavy snowfall event over the Swiss Alps: did wind shear impact secondary ice production?
On the global relationship between polarimetric radio occultation differential phase shift and ice water content
Natural marine cloud brightening in the Southern Ocean
Distinct regional meteorological influences on low-cloud albedo susceptibility over global marine stratocumulus regions
Rebecca J. Murray-Watson and Edward Gryspeerdt
Atmos. Chem. Phys., 24, 11115–11132, https://doi.org/10.5194/acp-24-11115-2024, https://doi.org/10.5194/acp-24-11115-2024, 2024
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The formation of mixed-phase clouds during marine cold-air outbreaks is not well understood. Our study, using satellite data and Lagrangian trajectories, reveals that the occurrence of these clouds depends on both time and temperature, influenced partly by the presence of biological ice-nucleating particles. This highlights the importance of comprehending local aerosol dynamics for precise modelling of cloud-phase transitions in the Arctic.
Yuxin Zhao, Jiming Li, Deyu Wen, Yarong Li, Yuan Wang, and Jianping Huang
Atmos. Chem. Phys., 24, 9435–9457, https://doi.org/10.5194/acp-24-9435-2024, https://doi.org/10.5194/acp-24-9435-2024, 2024
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This study identifies deep convection systems (DCSs), including deep convection cores and anvils, over the Tibetan Plateau (TP) and tropical Indian Ocean (TO). The DCSs over the TP are less frequent, showing narrower and thinner cores and anvils compared to those over the TO. TP DCSs show a stronger longwave cloud radiative effect at the surface and in the low-level atmosphere. Distinct aerosol–cloud–precipitation interaction is found in TP DCSs, probably due to the cold cloud bases.
Grégory V. Cesana, Olivia Pierpaoli, Matteo Ottaviani, Linh Vu, Zhonghai Jin, and Israel Silber
Atmos. Chem. Phys., 24, 7899–7909, https://doi.org/10.5194/acp-24-7899-2024, https://doi.org/10.5194/acp-24-7899-2024, 2024
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Better characterizing the relationship between sea ice and clouds is key to understanding Arctic climate because clouds and sea ice affect surface radiation and modulate Arctic surface warming. Our results indicate that Arctic liquid clouds robustly increase in response to sea ice decrease. This increase has a cooling effect on the surface because more solar radiation is reflected back to space, and it should contribute to dampening future Arctic surface warming.
Ziming Wang, Husi Letu, Huazhe Shang, and Luca Bugliaro
Atmos. Chem. Phys., 24, 7559–7574, https://doi.org/10.5194/acp-24-7559-2024, https://doi.org/10.5194/acp-24-7559-2024, 2024
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The supercooled liquid fraction (SLF) in mixed-phase clouds is retrieved for the first time using passive geostationary satellite observations based on differences in liquid droplet and ice particle radiative properties. The retrieved results are comparable to global distributions observed by active instruments, and the feasibility of the retrieval method to analyze the observed trends of the SLF has been validated.
Barbara Dietel, Odran Sourdeval, and Corinna Hoose
Atmos. Chem. Phys., 24, 7359–7383, https://doi.org/10.5194/acp-24-7359-2024, https://doi.org/10.5194/acp-24-7359-2024, 2024
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Uncertainty with respect to cloud phases over the Southern Ocean and Arctic marine regions leads to large uncertainties in the radiation budget of weather and climate models. This study investigates the phases of low-base and mid-base clouds using satellite-based remote sensing data. A comprehensive analysis of the correlation of cloud phase with various parameters, such as temperature, aerosols, sea ice, vertical and horizontal cloud extent, and cloud radiative effect, is presented.
Mengyuan Wang, Min Min, Jun Li, Han Lin, Yongen Liang, Binlong Chen, Zhigang Yao, Na Xu, and Miao Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2024-1516, https://doi.org/10.5194/egusphere-2024-1516, 2024
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Although machine learning technology is advanced in the field of satellite remote sensing, the physical inversion algorithm based on cloud base height can better capture the daily variation characteristics of cloud base.
Ryan Eastman, Isabel L. McCoy, Hauke Schulz, and Robert Wood
Atmos. Chem. Phys., 24, 6613–6634, https://doi.org/10.5194/acp-24-6613-2024, https://doi.org/10.5194/acp-24-6613-2024, 2024
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Cloud types are determined using machine learning image classifiers applied to satellite imagery for 1 year in the North Atlantic. This survey of these cloud types shows that the climate impact of a cloud scene is, in part, a function of cloud type. Each type displays a different mix of thick and thin cloud cover, with the fraction of thin cloud cover having the strongest impact on the clouds' radiative effect. Future studies must account for differing properties and processes among cloud types.
Thomas Lesigne, François Ravetta, Aurélien Podglajen, Vincent Mariage, and Jacques Pelon
Atmos. Chem. Phys., 24, 5935–5952, https://doi.org/10.5194/acp-24-5935-2024, https://doi.org/10.5194/acp-24-5935-2024, 2024
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Upper tropical clouds have a strong impact on Earth's climate but are challenging to observe. We report the first long-duration observations of tropical clouds from lidars flying on board stratospheric balloons. Comparisons with spaceborne observations reveal the enhanced sensitivity of balloon-borne lidar to optically thin cirrus. These clouds, which have a significant coverage and lie in the uppermost troposphere, are linked with the dehydration of air masses on their way to the stratosphere.
Georgios Dekoutsidis, Martin Wirth, and Silke Groß
Atmos. Chem. Phys., 24, 5971–5987, https://doi.org/10.5194/acp-24-5971-2024, https://doi.org/10.5194/acp-24-5971-2024, 2024
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For decades the earth's temperature has been rising. The Arctic regions are warming faster. Cirrus clouds can contribute to this phenomenon. During warm-air intrusions, air masses are transported into the Arctic from the mid-latitudes. The HALO-(AC)3 campaign took place to measure cirrus during intrusion events and under normal conditions. We study the two cloud types based on these measurements and find differences in their geometry, relative humidity distribution and vertical structure.
Zhenquan Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-1318, https://doi.org/10.5194/egusphere-2024-1318, 2024
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The connected but independent convective systems are divided from the complicated organizations and tracked. The duration, precipitation and anvil amount of the tracked organization segments have a strong log-linear relationship with its brightness temperature structures. Most precipitation are contributed by the cold long-lived but less frequent convective structures, while anvils are produced by both the cold long-lived and the warm short-lived but frequent convective structures.
Huige Di and Yun Yuan
Atmos. Chem. Phys., 24, 5783–5801, https://doi.org/10.5194/acp-24-5783-2024, https://doi.org/10.5194/acp-24-5783-2024, 2024
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We observed the seeder–feeder process among double-layer clouds using a cloud radar and microwave radiometer. By defining the parameters of the seeding depth and seeding time of the upper cloud affecting the lower cloud, we find that the cloud particle terminal velocity is significantly enhanced during the seeder–feeder period, and the lower the height and thinner the thickness of the height difference between double-layer clouds, the lower the height and thicker the thickness of seeding depth.
Anna Tippett, Edward Gryspeerdt, Peter Manshausen, Philip Stier, and Tristan W. P. Smith
EGUsphere, https://doi.org/10.5194/egusphere-2024-1479, https://doi.org/10.5194/egusphere-2024-1479, 2024
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Ship emissions can form artificially brightened clouds, known as ship tracks, and provide us with an opportunity to investigate how aerosols interact with clouds. Previous studies that used ship tracks suggest that clouds can experience large increases in the amount of water (LWP) from aerosols. Here, we show that there is a bias in previous research, and that when we account for this bias, the LWP response to aerosols is much weaker than previously reported.
Kristofer S. Tuftedal, Bernat Puigdomènech Treserras, Mariko Oue, and Pavlos Kollias
Atmos. Chem. Phys., 24, 5637–5657, https://doi.org/10.5194/acp-24-5637-2024, https://doi.org/10.5194/acp-24-5637-2024, 2024
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This study analyzed coastal convective cells from June through September 2018–2021. The cells were classified and their lifecycles were analyzed to better understand their characteristics. Features such as convective-core growth, for example, are shown. The study found differences in the initiation location of shallow convection and in the aerosol loading in deep convective environments. This work provides a foundation for future analyses of convection or other tracked events elsewhere.
Michie Vianca De Vera, Larry Di Girolamo, Guangyu Zhao, Robert M. Rauber, Stephen W. Nesbitt, and Greg M. McFarquhar
Atmos. Chem. Phys., 24, 5603–5623, https://doi.org/10.5194/acp-24-5603-2024, https://doi.org/10.5194/acp-24-5603-2024, 2024
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Tropical oceanic low clouds remain a dominant source of uncertainty in cloud feedback in climate models due to their macrophysical properties (fraction, size, height, shape, distribution) being misrepresented. High-resolution satellite imagery over the Philippine oceans is used here to characterize cumulus macrophysical properties and their relationship to meteorological variables. Such information can act as a benchmark for cloud models and can improve low-cloud generation in climate models.
William K. Jones, Martin Stengel, and Philip Stier
Atmos. Chem. Phys., 24, 5165–5180, https://doi.org/10.5194/acp-24-5165-2024, https://doi.org/10.5194/acp-24-5165-2024, 2024
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Storm clouds cover large areas of the tropics. These clouds both reflect incoming sunlight and trap heat from the atmosphere below, regulating the temperature of the tropics. Over land, storm clouds occur in the late afternoon and evening and so exist both during the daytime and at night. Changes in this timing could upset the balance of the respective cooling and heating effects of these clouds. We find that isolated storms have a larger effect on this balance than their small size suggests.
George Horner and Edward Gryspeerdt
EGUsphere, https://doi.org/10.5194/egusphere-2024-1090, https://doi.org/10.5194/egusphere-2024-1090, 2024
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This work tracks the lifecycle of thin cirrus clouds that flow out of tropical convective storms. These cirrus clouds are found to have a warming effect on the atmosphere over their whole lifetime. Thin cirrus that originate from land origin convection warm more than those of ocean origin. Moreover, if the lifetime of these cirrus clouds increase, the warming they exert over their whole lifetime also increases. These results help us understand how these clouds might change in a future climate.
Shaoyue Qiu, Xue Zheng, David Painemal, Christopher R. Terai, and Xiaoli Zhou
Atmos. Chem. Phys., 24, 2913–2935, https://doi.org/10.5194/acp-24-2913-2024, https://doi.org/10.5194/acp-24-2913-2024, 2024
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The aerosol indirect effect (AIE) depends on cloud states, which exhibit significant diurnal variations in the northeastern Atlantic. Yet the AIE diurnal cycle remains poorly understood. Using satellite retrievals, we find a pronounced “U-shaped” diurnal variation in the AIE, which is contributed to by the transition of cloud states combined with the lagged cloud responses. This suggests that polar-orbiting satellites with overpass times at noon underestimate daytime mean values of the AIE.
Irene Bartolomé García, Odran Sourdeval, Reinhold Spang, and Martina Krämer
Atmos. Chem. Phys., 24, 1699–1716, https://doi.org/10.5194/acp-24-1699-2024, https://doi.org/10.5194/acp-24-1699-2024, 2024
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How many ice crystals of each size are in a cloud is a key parameter for the retrieval of cloud properties. The distribution of ice crystals is obtained from in situ measurements and used to create parameterizations that can be used when analyzing the remote-sensing data. Current parameterizations are based on data sets that do not include reliable measurements of small crystals, but in our study we use a data set that includes very small ice crystals to improve these parameterizations.
Wenyue Wang, Klemens Hocke, Leonardo Nania, Alberto Cazorla, Gloria Titos, Renaud Matthey, Lucas Alados-Arboledas, Agustín Millares, and Francisco Navas-Guzmán
Atmos. Chem. Phys., 24, 1571–1585, https://doi.org/10.5194/acp-24-1571-2024, https://doi.org/10.5194/acp-24-1571-2024, 2024
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The south-central interior of Andalusia experiences complex precipitation patterns as a result of the semi-arid Mediterranean climate and the influence of Saharan dust. This study monitored the inter-relations between aerosols, clouds, meteorological variables, and precipitation systems using ground-based remote sensing and in situ instruments.
Francisco Lang, Steven T. Siems, Yi Huang, Tahereh Alinejadtabrizi, and Luis Ackermann
Atmos. Chem. Phys., 24, 1451–1466, https://doi.org/10.5194/acp-24-1451-2024, https://doi.org/10.5194/acp-24-1451-2024, 2024
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Marine low-level clouds play a crucial role in the Earth's energy balance, trapping heat from the surface and reflecting sunlight back into space. These clouds are distinguishable by their large-scale spatial structures, primarily characterized as hexagonal patterns with either filled (closed) or empty (open) cells. Utilizing satellite observations, these two cloud type patterns have been categorized over the Southern Ocean and North Pacific Ocean through a pattern recognition program.
Julian Hofer, Patric Seifert, J. Ben Liley, Martin Radenz, Osamu Uchino, Isamu Morino, Tetsu Sakai, Tomohiro Nagai, and Albert Ansmann
Atmos. Chem. Phys., 24, 1265–1280, https://doi.org/10.5194/acp-24-1265-2024, https://doi.org/10.5194/acp-24-1265-2024, 2024
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An 11-year dataset of polarization lidar observations from Lauder, New Zealand / Aotearoa, was used to distinguish the thermodynamic phase of natural clouds. The cloud dataset was separated to assess the impact of air mass origin on the frequency of heterogeneous ice formation. Ice formation efficiency in clouds above Lauder was found to be lower than in the polluted Northern Hemisphere midlatitudes but higher than in very clean and pristine environments, such as Punta Arenas in southern Chile.
Hannes Jascha Griesche, Carola Barrientos-Velasco, Hartwig Deneke, Anja Hünerbein, Patric Seifert, and Andreas Macke
Atmos. Chem. Phys., 24, 597–612, https://doi.org/10.5194/acp-24-597-2024, https://doi.org/10.5194/acp-24-597-2024, 2024
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The Arctic is strongly affected by climate change and the role of clouds therein is not yet completely understood. Measurements from the Arctic expedition PS106 were used to simulate radiative fluxes with and without clouds at very low altitudes (below 165 m), and their radiative effect was calculated to be 54 Wm-2. The low heights of these clouds make them hard to observe. This study shows the importance of accurate measurements and simulations of clouds and gives suggestions for improvements.
Thomas D. DeWitt, Timothy J. Garrett, Karlie N. Rees, Corey Bois, Steven K. Krueger, and Nicolas Ferlay
Atmos. Chem. Phys., 24, 109–122, https://doi.org/10.5194/acp-24-109-2024, https://doi.org/10.5194/acp-24-109-2024, 2024
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Viewed from space, a defining feature of Earth's atmosphere is the wide spectrum of cloud sizes. A recent study predicted the distribution of cloud sizes, and this paper compares the prediction to observations. Although there is nuance in viewing perspective, we find robust agreement with theory across different climatological conditions, including land–ocean contrasts, time of year, or latitude, suggesting a minor role for Coriolis forces, aerosol loading, or surface temperature.
Marcus Klingebiel, André Ehrlich, Elena Ruiz-Donoso, Nils Risse, Imke Schirmacher, Evelyn Jäkel, Michael Schäfer, Kevin Wolf, Mario Mech, Manuel Moser, Christiane Voigt, and Manfred Wendisch
Atmos. Chem. Phys., 23, 15289–15304, https://doi.org/10.5194/acp-23-15289-2023, https://doi.org/10.5194/acp-23-15289-2023, 2023
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In this study we explain how we use aircraft measurements from two Arctic research campaigns to identify cloud properties (like droplet size) over sea-ice and ice-free ocean. To make sure that our measurements make sense, we compare them with other observations. Our results show, e.g., larger cloud droplets in early summer than in spring. Moreover, the cloud droplets are also larger over ice-free ocean than compared to sea ice. In the future, our data can be used to improve climate models.
Pablo Saavedra Garfias, Heike Kalesse-Los, Luisa von Albedyll, Hannes Griesche, and Gunnar Spreen
Atmos. Chem. Phys., 23, 14521–14546, https://doi.org/10.5194/acp-23-14521-2023, https://doi.org/10.5194/acp-23-14521-2023, 2023
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An important Arctic climate process is the release of heat fluxes from sea ice openings to the atmosphere that influence the clouds. The characterization of this process is the objective of this study. Using synergistic observations from the MOSAiC expedition, we found that single-layer cloud properties show significant differences when clouds are coupled or decoupled to the water vapour transport which is used as physical link between the upwind sea ice openings and the cloud under observation.
Matthew D. Lebsock and Mikael Witte
Atmos. Chem. Phys., 23, 14293–14305, https://doi.org/10.5194/acp-23-14293-2023, https://doi.org/10.5194/acp-23-14293-2023, 2023
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This paper evaluates measurements of cloud drop size distributions made from airplanes. We find that as the number of cloud drops increases the distribution of the cloud drop sizes narrows. The data are used to develop a simple equation that relates the drop number to the width of the drop sizes. We then use this equation to demonstrate that existing approaches to observe the drop number from satellites contain errors that can be corrected by including the new relationship.
George Horner and Edward Gryspeerdt
Atmos. Chem. Phys., 23, 14239–14253, https://doi.org/10.5194/acp-23-14239-2023, https://doi.org/10.5194/acp-23-14239-2023, 2023
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Tropical deep convective clouds, and the thin cirrus (ice) clouds that flow out from them, are important for modulating the energy budget of the tropical atmosphere. This work uses a new method to track the evolution of the properties of these clouds across their entire lifetimes. We find these clouds cool the atmosphere in the first 6 h before switching to a warming regime after the deep convective core has dissipated, which is sustained beyond 120 h from the initial convective event.
Rodanthi-Elisavet Mamouri, Albert Ansmann, Kevin Ohneiser, Daniel A. Knopf, Argyro Nisantzi, Johannes Bühl, Ronny Engelmann, Annett Skupin, Patric Seifert, Holger Baars, Dragos Ene, Ulla Wandinger, and Diofantos Hadjimitsis
Atmos. Chem. Phys., 23, 14097–14114, https://doi.org/10.5194/acp-23-14097-2023, https://doi.org/10.5194/acp-23-14097-2023, 2023
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For the first time, rather clear evidence is found that wildfire smoke particles can trigger strong cirrus formation. This finding is of importance because intensive and large wildfires may occur increasingly often in the future as climate change proceeds. Based on lidar observations in Cyprus in autumn 2020, we provide detailed insight into the cirrus formation at the tropopause in the presence of aged wildfire smoke (here, 8–9 day old Californian wildfire smoke).
Peter Manshausen, Duncan Watson-Parris, Matthew W. Christensen, Jukka-Pekka Jalkanen, and Philip Stier
Atmos. Chem. Phys., 23, 12545–12555, https://doi.org/10.5194/acp-23-12545-2023, https://doi.org/10.5194/acp-23-12545-2023, 2023
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Aerosol from burning fuel changes cloud properties, e.g., the number of droplets and the content of water. Here, we study how clouds respond to different amounts of shipping aerosol. Droplet numbers increase linearly with increasing aerosol over a broad range until they stop increasing, while the amount of liquid water always increases, independently of emission amount. These changes in cloud properties can make them reflect more or less sunlight, which is important for the earth's climate.
Hendrik Andersen, Jan Cermak, Alyson Douglas, Timothy A. Myers, Peer Nowack, Philip Stier, Casey J. Wall, and Sarah Wilson Kemsley
Atmos. Chem. Phys., 23, 10775–10794, https://doi.org/10.5194/acp-23-10775-2023, https://doi.org/10.5194/acp-23-10775-2023, 2023
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This study uses an observation-based cloud-controlling factor framework to study near-global sensitivities of cloud radiative effects to a large number of meteorological and aerosol controls. We present near-global sensitivity patterns to selected thermodynamic, dynamic, and aerosol factors and discuss the physical mechanisms underlying the derived sensitivities. Our study hopes to guide future analyses aimed at constraining cloud feedbacks and aerosol–cloud interactions.
Anne-Claire Billault-Roux, Paraskevi Georgakaki, Josué Gehring, Louis Jaffeux, Alfons Schwarzenboeck, Pierre Coutris, Athanasios Nenes, and Alexis Berne
Atmos. Chem. Phys., 23, 10207–10234, https://doi.org/10.5194/acp-23-10207-2023, https://doi.org/10.5194/acp-23-10207-2023, 2023
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Secondary ice production plays a key role in clouds and precipitation. In this study, we analyze radar measurements from a snowfall event in the Jura Mountains. Complex signatures are observed, which reveal that ice crystals were formed through various processes. An analysis of multi-sensor data suggests that distinct ice multiplication processes were taking place. Both the methods used and the insights gained through this case study contribute to a better understanding of snowfall microphysics.
Rebecca J. Murray-Watson, Edward Gryspeerdt, and Tom Goren
Atmos. Chem. Phys., 23, 9365–9383, https://doi.org/10.5194/acp-23-9365-2023, https://doi.org/10.5194/acp-23-9365-2023, 2023
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Clouds formed in Arctic marine cold air outbreaks undergo a distinct evolution, but the factors controlling their transition from high-coverage to broken cloud fields are poorly understood. We use satellite and reanalysis data to study how these clouds develop in time and the different influences on their evolution. The aerosol concentration is correlated with cloud break-up; more aerosol is linked to prolonged coverage and a stronger cooling effect, with implications for a more polluted Arctic.
Michael S. Diamond
Atmos. Chem. Phys., 23, 8259–8269, https://doi.org/10.5194/acp-23-8259-2023, https://doi.org/10.5194/acp-23-8259-2023, 2023
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Fuel sulfur regulations were implemented for ships in 2020 to improve air quality but may also accelerate global warming. We use spatial statistics and satellite retrievals to detect changes in the size of cloud droplets and find evidence for a resulting decrease in cloud brightness within a major shipping corridor after the sulfur limits went into effect. Our results confirm both that the regulations are being followed and that they are having a warming influence via their effect on clouds.
Hao Luo, Johannes Quaas, and Yong Han
Atmos. Chem. Phys., 23, 8169–8186, https://doi.org/10.5194/acp-23-8169-2023, https://doi.org/10.5194/acp-23-8169-2023, 2023
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Clouds exhibit a wide range of vertical structures with varying microphysical and radiative properties. We show a global survey of spatial distribution, vertical extent and radiative effect of various classified cloud vertical structures using joint satellite observations from the new CCCM datasets during 2007–2010. Moreover, the long-term trends in CVSs are investigated based on different CMIP6 future scenarios to capture the cloud variations with different, increasing anthropogenic forcings.
Gregor Köcher, Tobias Zinner, and Christoph Knote
Atmos. Chem. Phys., 23, 6255–6269, https://doi.org/10.5194/acp-23-6255-2023, https://doi.org/10.5194/acp-23-6255-2023, 2023
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Polarimetric radar observations of 30 d of convective precipitation events are used to statistically analyze 5 state-of-the-art microphysics schemes of varying complexity. The frequency and area of simulated heavy-precipitation events are in some cases significantly different from those observed, depending on the microphysics scheme. Analysis of simulated particle size distributions and reflectivities shows that some schemes have problems reproducing the correct particle size distributions.
Claudia J. Stubenrauch, Giulio Mandorli, and Elisabeth Lemaitre
Atmos. Chem. Phys., 23, 5867–5884, https://doi.org/10.5194/acp-23-5867-2023, https://doi.org/10.5194/acp-23-5867-2023, 2023
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Organized convection leads to large convective cloud systems and intense rain and may change with a warming climate. Their complete 3D description, attained by machine learning techniques in combination with various satellite observations, together with a cloud system concept, link convection to anvil properties, while convective organization can be identified by the horizontal structure of intense rain.
Scott E. Giangrande, Thiago S. Biscaro, and John M. Peters
Atmos. Chem. Phys., 23, 5297–5316, https://doi.org/10.5194/acp-23-5297-2023, https://doi.org/10.5194/acp-23-5297-2023, 2023
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Our study tracks thunderstorms observed during the wet and dry seasons of the Amazon Basin using weather radar. We couple this precipitation tracking with opportunistic overpasses of a wind profiler and other ground observations to add unique insights into the upwards and downwards air motions within these clouds at various stages in the storm life cycle. The results of a simple updraft model are provided to give physical explanations for observed seasonal differences.
Edward Gryspeerdt, Adam C. Povey, Roy G. Grainger, Otto Hasekamp, N. Christina Hsu, Jane P. Mulcahy, Andrew M. Sayer, and Armin Sorooshian
Atmos. Chem. Phys., 23, 4115–4122, https://doi.org/10.5194/acp-23-4115-2023, https://doi.org/10.5194/acp-23-4115-2023, 2023
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The impact of aerosols on clouds is one of the largest uncertainties in the human forcing of the climate. Aerosol can increase the concentrations of droplets in clouds, but observational and model studies produce widely varying estimates of this effect. We show that these estimates can be reconciled if only polluted clouds are studied, but this is insufficient to constrain the climate impact of aerosol. The uncertainty in aerosol impact on clouds is currently driven by cases with little aerosol.
Zackary Mages, Pavlos Kollias, Zeen Zhu, and Edward P. Luke
Atmos. Chem. Phys., 23, 3561–3574, https://doi.org/10.5194/acp-23-3561-2023, https://doi.org/10.5194/acp-23-3561-2023, 2023
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Cold-air outbreaks (when cold air is advected over warm water and creates low-level convection) are a dominant cloud regime in the Arctic, and we capitalized on ground-based observations, which did not previously exist, from the COMBLE field campaign to study them. We characterized the extent and strength of the convection and turbulence and found evidence of secondary ice production. This information is useful for model intercomparison studies that will represent cold-air outbreak processes.
Maria P. Cadeddu, Virendra P. Ghate, David D. Turner, and Thomas E. Surleta
Atmos. Chem. Phys., 23, 3453–3470, https://doi.org/10.5194/acp-23-3453-2023, https://doi.org/10.5194/acp-23-3453-2023, 2023
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We analyze the variability in marine boundary layer moisture at the Eastern North Atlantic site on a monthly and daily temporal scale and examine its fundamental role in the control of boundary layer cloudiness and precipitation. The study also highlights the complex interaction between large-scale and local processes controlling the boundary layer moisture and the importance of the mesoscale spatial distribution of vapor to support convection and precipitation.
Zhenquan Wang, Jian Yuan, Robert Wood, Yifan Chen, and Tiancheng Tong
Atmos. Chem. Phys., 23, 3247–3266, https://doi.org/10.5194/acp-23-3247-2023, https://doi.org/10.5194/acp-23-3247-2023, 2023
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This study develops a novel profile-based algorithm based on the ERA5 to estimate the inversion strength in the planetary boundary layer better than the previous inversion index, which is a key low-cloud-controlling factor. This improved measure is more effective at representing the meteorological influence on low-cloud variations. It can better constrain the meteorological influence on low clouds to better isolate cloud responses to aerosols or to estimate low cloud feedbacks in climate models.
Georgios Dekoutsidis, Silke Groß, Martin Wirth, Martina Krämer, and Christian Rolf
Atmos. Chem. Phys., 23, 3103–3117, https://doi.org/10.5194/acp-23-3103-2023, https://doi.org/10.5194/acp-23-3103-2023, 2023
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Cirrus clouds affect Earth's atmosphere, deeming our study important. Here we use water vapor measurements by lidar and study the relative humidity (RHi) within and around midlatitude cirrus clouds. We find high supersaturations in the cloud-free air and within the clouds, especially near the cloud top. We study two cloud types with different formation processes. Finally, we conclude that the shape of the distribution of RHi can be used as an indicator of different cloud evolutionary stages.
Huazhe Shang, Souichiro Hioki, Guillaume Penide, Céline Cornet, Husi Letu, and Jérôme Riedi
Atmos. Chem. Phys., 23, 2729–2746, https://doi.org/10.5194/acp-23-2729-2023, https://doi.org/10.5194/acp-23-2729-2023, 2023
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We find that cloud profiles can be divided into four prominent patterns, and the frequency of these four patterns is related to intensities of cloud-top entrainment and precipitation. Based on these analyses, we further propose a cloud profile parameterization scheme allowing us to represent these patterns. Our results shed light on how to facilitate the representation of cloud profiles and how to link them to cloud entrainment or precipitating status in future remote-sensing applications.
Luca Lelli, Marco Vountas, Narges Khosravi, and John Philipp Burrows
Atmos. Chem. Phys., 23, 2579–2611, https://doi.org/10.5194/acp-23-2579-2023, https://doi.org/10.5194/acp-23-2579-2023, 2023
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Arctic amplification describes the recent period in which temperatures have been rising twice as fast as or more than the global average and sea ice and the Greenland ice shelf are approaching a tipping point. Hence, the Arctic ability to reflect solar energy decreases and absorption by the surface increases. Using 2 decades of complementary satellite data, we discover that clouds unexpectedly increase the pan-Arctic reflectance by increasing their liquid water content, thus cooling the Arctic.
Yabin Gou, Haonan Chen, Hong Zhu, and Lulin Xue
Atmos. Chem. Phys., 23, 2439–2463, https://doi.org/10.5194/acp-23-2439-2023, https://doi.org/10.5194/acp-23-2439-2023, 2023
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This article investigates the complex precipitation microphysics associated with super typhoon Lekima using a host of in situ and remote sensing observations, including rain gauge and disdrometer data, as well as polarimetric radar observations. The impacts of precipitation microphysics on multi-source data consistency and radar precipitation estimation are quantified. It is concluded that the dynamical precipitation microphysical processes must be considered in radar precipitation estimation.
Hongxia Zhu, Rui Li, Shuping Yang, Chun Zhao, Zhe Jiang, and Chen Huang
Atmos. Chem. Phys., 23, 2421–2437, https://doi.org/10.5194/acp-23-2421-2023, https://doi.org/10.5194/acp-23-2421-2023, 2023
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The impacts of atmospheric dust aerosols and cloud dynamic conditions on precipitation vertical development in southeastern China were studied using multiple satellite observations. It was found that the precipitating drops under dusty conditions grow faster in the middle layer but slower in the upper and lower layers compared with their pristine counterparts. Quantitative estimation of the sensitivity of the precipitation top temperature to the dust aerosol optical depth is also provided.
Zane Dedekind, Jacopo Grazioli, Philip H. Austin, and Ulrike Lohmann
Atmos. Chem. Phys., 23, 2345–2364, https://doi.org/10.5194/acp-23-2345-2023, https://doi.org/10.5194/acp-23-2345-2023, 2023
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Simulations allowing ice particles to collide with one another producing more ice particles represented surface observations of ice particles accurately. An increase in ice particles formed through collisions was related to sharp changes in the wind direction and speed with height. Changes in wind speed and direction can therefore cause more enhanced collisions between ice particles and alter how fast and how much precipitation forms. Simulations were conducted with the atmospheric model COSMO.
Ramon Padullés, Estel Cardellach, and F. Joseph Turk
Atmos. Chem. Phys., 23, 2199–2214, https://doi.org/10.5194/acp-23-2199-2023, https://doi.org/10.5194/acp-23-2199-2023, 2023
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The results of comparing the polarimetric radio occultation observables and the ice water content retrieved from the CloudSat radar in a global and statistical way show a strong correlation between the geographical patterns of both quantities for a wide range of heights. This implies that horizontally oriented hydrometeors are systematically present through the whole globe and through all vertical levels, which could provide insights on the physical processes leading to precipitation.
Gerald G. Mace, Sally Benson, Ruhi Humphries, Peter M. Gombert, and Elizabeth Sterner
Atmos. Chem. Phys., 23, 1677–1685, https://doi.org/10.5194/acp-23-1677-2023, https://doi.org/10.5194/acp-23-1677-2023, 2023
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The number of cloud droplets per unit volume is a significantly important property of clouds that controls their reflective properties. Computer models of the Earth's atmosphere and climate have low skill at predicting the reflective properties of Southern Ocean clouds. Here we investigate the properties of those clouds using satellite data and find that the cloud droplet number and cloud albedo in the Southern Ocean are related to the oceanic phytoplankton abundance near Antarctica.
Jianhao Zhang and Graham Feingold
Atmos. Chem. Phys., 23, 1073–1090, https://doi.org/10.5194/acp-23-1073-2023, https://doi.org/10.5194/acp-23-1073-2023, 2023
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Using observations from space, we show maps of potential brightness changes in marine warm clouds in response to increases in cloud droplet concentrations. The environmental and aerosol conditions in which these clouds reside covary differently in each ocean basin, leading to distinct evolutions of cloud brightness changes. This work stresses the central importance of the covariability between meteorology and aerosol for scaling up the radiative response of cloud brightness changes.
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Short summary
Differences in the microphysical properties of contrail cirrus and natural cirrus in a contrail outbreak situation during the ML-CIRRUS campaign over the North Atlantic flight corridor can be observed from in situ measurements. The cirrus radiative effect in the area of the outbreak, derived from satellite observation-based radiative transfer modeling, is warming in the early morning and cooling during the day.
Differences in the microphysical properties of contrail cirrus and natural cirrus in a contrail...
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