Articles | Volume 22, issue 7
https://doi.org/10.5194/acp-22-4277-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-4277-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| Highlight paper
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04 Apr 2022
Research article | Highlight paper |
| 04 Apr 2022
| 04 Apr 2022
A stratospheric prognostic ozone for seamless Earth system models: performance, impacts and future
Beatriz M. Monge-Sanz
CORRESPONDING AUTHOR
Department of Physics, University of Oxford, Oxford, United Kingdom
National Centre for Atmospheric Science, University of Oxford, Oxford, United Kingdom
Alessio Bozzo
European Organisation for the Exploitation of Meteorological Satellites, Darmstadt, Germany
formerly at: European Centre for Medium-Range Weather Forecasts, Reading, United Kingdom
Nicholas Byrne
Department of Meteorology, University of Reading, Reading, United Kingdom
Martyn P. Chipperfield
School of Earth and Environment, University of Leeds, Leeds, United Kingdom
National Centre for Earth Observation, University of Leeds, Leeds, United Kingdom
Michail Diamantakis
European Centre for Medium-Range Weather Forecasts, Reading, United Kingdom
Johannes Flemming
European Centre for Medium-Range Weather Forecasts, Reading, United Kingdom
Lesley J. Gray
Department of Physics, University of Oxford, Oxford, United Kingdom
National Centre for Atmospheric Science, University of Oxford, Oxford, United Kingdom
Robin J. Hogan
European Centre for Medium-Range Weather Forecasts, Reading, United Kingdom
Department of Meteorology, University of Reading, Reading, United Kingdom
Luke Jones
European Centre for Medium-Range Weather Forecasts, Reading, United Kingdom
Linus Magnusson
European Centre for Medium-Range Weather Forecasts, Reading, United Kingdom
Inna Polichtchouk
European Centre for Medium-Range Weather Forecasts, Reading, United Kingdom
Theodore G. Shepherd
Department of Meteorology, University of Reading, Reading, United Kingdom
Nils Wedi
European Centre for Medium-Range Weather Forecasts, Reading, United Kingdom
Antje Weisheimer
Department of Physics, University of Oxford, Oxford, United Kingdom
National Centre for Atmospheric Science, University of Oxford, Oxford, United Kingdom
European Centre for Medium-Range Weather Forecasts, Reading, United Kingdom
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Robert Schoetter, Robin James Hogan, Cyril Caliot, and Valéry Masson
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Matilda A. Pimlott, Richard J. Pope, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Wuhu Feng, and Martyn P. Chipperfield
EGUsphere, https://doi.org/10.5194/egusphere-2024-3717, https://doi.org/10.5194/egusphere-2024-3717, 2024
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Tropospheric ozone (O3) is a harmful secondary atmospheric pollutant and an important greenhouse gas. Here, we present an in-depth analysis of lower-tropospheric sub-column O3 (LTCO3, surface – 6 km) records from three satellite products produced by the Rutherford Appleton Laboratory (RAL) over Europe between 1996 and 2017. Overall, we detect moderate negative trends in the satellite records, but corresponding model simulations and ozonesonde measurements show negligible trends.
Augustin Colette, Gaëlle Collin, François Besson, Etienne Blot, Vincent Guidard, Frederik Meleux, Adrien Royer, Valentin Petiot, Claire Miller, Oihana Fermond, Alizé Jeant, Mario Adani, Joaquim Arteta, Anna Benedictow, Robert Bergström, Dene Bowdalo, Jorgen Brandt, Gino Briganti, Ana C. Carvalho, Jesper Heile Christensen, Florian Couvidat, Ilia D’Elia, Massimo D’Isidoro, Hugo Denier van der Gon, Gaël Descombes, Enza Di Tomaso, John Douros, Jeronimo Escribano, Henk Eskes, Hilde Fagerli, Yalda Fatahi, Johannes Flemming, Elmar Friese, Lise Frohn, Michael Gauss, Camilla Geels, Guido Guarnieri, Marc Guevara, Antoine Guion, Jonathan Guth, Risto Hänninen, Kaj Hansen, Ulas Im, Ruud Janssen, Marine Jeoffrion, Mathieu Joly, Luke Jones, Oriol Jorba, Evgeni Kadantsev, Michael Kahnert, Jacek W. Kaminski, Rostislav Kouznetsov, Richard Kranenburg, Jeroen Kuenen, Anne Caroline Lange, Joachim Langner, Victor Lannuque, Francesca Macchia, Astrid Manders, Mihaela Mircea, Agnes Nyiri, Miriam Olid, Carlos Pérez García-Pando, Yuliia Palamarchuk, Antonio Piersanti, Blandine Raux, Miha Razinger, Lennard Robertson, Arjo Segers, Martijn Schaap, Pilvi Siljamo, David Simpson, Mikhail Sofiev, Anders Stangel, Joanna Struzewska, Carles Tena, Renske Timmermans, Thanos Tsikerdekis, Svetlana Tsyro, Svyatoslav Tyuryakov, Anthony Ung, Andreas Uppstu, Alvaro Valdebenito, Peter van Velthoven, Lina Vitali, Zhuyun Ye, Vincent-Henri Peuch, and Laurence Rouïl
EGUsphere, https://doi.org/10.5194/egusphere-2024-3744, https://doi.org/10.5194/egusphere-2024-3744, 2024
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DCE (1,2-dichloroethane) is an industrial chemical used to produce PVC (polyvinyl chloride). We analysed DCE production data to estimate global DCE emissions (2002–2020). The emissions were included in an atmospheric model and evaluated by comparing simulated DCE to DCE measurements in the troposphere. We show that DCE contributes ozone-depleting Cl to the stratosphere and that this has increased with increasing DCE emissions. DCE’s impact on stratospheric O3 is currently small but non-zero.
Aleena M. Jaison, Lesley J. Gray, Scott M. Osprey, Jeff R. Knight, and Martin B. Andrews
Weather Clim. Dynam., 5, 1489–1504, https://doi.org/10.5194/wcd-5-1489-2024, https://doi.org/10.5194/wcd-5-1489-2024, 2024
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Models have biases in semi-annual oscillation (SAO) representation, mainly due to insufficient eastward wave forcing. We examined if the bias is from increased wave absorption due to circulation biases in the low–middle stratosphere. Alleviating biases at lower altitudes improves the SAO, but substantial bias remains. Alternative methods like gravity wave parameterization changes should be explored to enhance the modelled SAO, potentially improving sudden stratospheric warming predictability.
Jason Williams, Swen Metzer, Samuel Remy, Vincent Huijnen, and Johannes Flemming
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-188, https://doi.org/10.5194/gmd-2024-188, 2024
Revised manuscript under review for GMD
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One of the main constituents of Particulate Matter at the surface are Secondary Inorganic Aerosols (SIA) which are influenced by both anthropogenic emissions and the acidity of clouds and aerosols. This study shows improvements in introduced into the IFS-COMPO simulating the surface concentrations of SIA and the resulting changes in the total wet deposition for Europe, the US and South-East Asia.
Kaah P. Menang, Stefan A. Buehler, Lukas Kluft, Robin J. Hogan, and Florian E. Roemer
EGUsphere, https://doi.org/10.5194/egusphere-2024-3051, https://doi.org/10.5194/egusphere-2024-3051, 2024
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We investigated how the uncertainty in representing water vapour continuum absorption in the shortwave affects clear-sky shortwave radiative feedback. For current surface temperature, the impact is modest (<2 %). In a warmer world, continuum induced error in estimated shortwave feedback is up to ~5 %. Using the MT_CKD model in radiative transfer calculations may lead to an underestimation of the shortwave feedback. Constraining shortwave continuum will contribute to reducing these discrepancies.
Rachel W.-Y. Wu, Gabriel Chiodo, Inna Polichtchouk, and Daniela I. V. Domeisen
Atmos. Chem. Phys., 24, 12259–12275, https://doi.org/10.5194/acp-24-12259-2024, https://doi.org/10.5194/acp-24-12259-2024, 2024
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Strong variations in the strength of the stratospheric polar vortex can profoundly affect surface weather extremes; therefore, accurately predicting the stratosphere can improve surface weather forecasts. The research reveals how uncertainty in the stratosphere is linked to the troposphere. The findings suggest that refining models to better represent the identified sources and impact regions in the troposphere is likely to improve the prediction of the stratosphere and its surface impacts.
Samuel Rémy, Swen Metzger, Vincent Huijnen, Jason E. Williams, and Johannes Flemming
Geosci. Model Dev., 17, 7539–7567, https://doi.org/10.5194/gmd-17-7539-2024, https://doi.org/10.5194/gmd-17-7539-2024, 2024
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In this paper we describe the development of the future operational cycle 49R1 of the IFS-COMPO system, used for operational forecasts of atmospheric composition in the CAMS project, and focus on the implementation of the thermodynamical model EQSAM4Clim version 12. The implementation of EQSAM4Clim significantly improves the simulated secondary inorganic aerosol surface concentration. The new aerosol and precipitation acidity diagnostics showed good agreement against observational datasets.
Jorge E. Pachón, Mariel A. Opazo, Pablo Lichtig, Nicolas Huneeus, Idir Bouarar, Guy Brasseur, Cathy W. Y. Li, Johannes Flemming, Laurent Menut, Camilo Menares, Laura Gallardo, Michael Gauss, Mikhail Sofiev, Rostislav Kouznetsov, Julia Palamarchuk, Andreas Uppstu, Laura Dawidowski, Nestor Y. Rojas, María de Fátima Andrade, Mario E. Gavidia-Calderón, Alejandro H. Delgado Peralta, and Daniel Schuch
Geosci. Model Dev., 17, 7467–7512, https://doi.org/10.5194/gmd-17-7467-2024, https://doi.org/10.5194/gmd-17-7467-2024, 2024
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Latin America (LAC) has some of the most populated urban areas in the world, with high levels of air pollution. Air quality management in LAC has been traditionally focused on surveillance and building emission inventories. This study performed the first intercomparison and model evaluation in LAC, with interesting and insightful findings for the region. A multiscale modeling ensemble chain was assembled as a first step towards an air quality forecasting system.
Sebastian Rhode, Peter Preusse, Jörn Ungermann, Inna Polichtchouk, Kaoru Sato, Shingo Watanabe, Manfred Ern, Karlheinz Nogai, Björn-Martin Sinnhuber, and Martin Riese
Atmos. Meas. Tech., 17, 5785–5819, https://doi.org/10.5194/amt-17-5785-2024, https://doi.org/10.5194/amt-17-5785-2024, 2024
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We investigate the capabilities of a proposed satellite mission, CAIRT, for observing gravity waves throughout the middle atmosphere and present the necessary methodology for in-depth wave analysis. Our findings suggest that such a satellite mission is highly capable of resolving individual wave parameters and could give new insights into the role of gravity waves in general atmospheric circulation and atmospheric processes.
Chris Wilson, Brian J. Kerridge, Richard Siddans, David P. Moore, Lucy J. Ventress, Emily Dowd, Wuhu Feng, Martyn P. Chipperfield, and John J. Remedios
Atmos. Chem. Phys., 24, 10639–10653, https://doi.org/10.5194/acp-24-10639-2024, https://doi.org/10.5194/acp-24-10639-2024, 2024
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The leaks from the Nord Stream gas pipelines in September 2022 released a large amount of methane (CH4) into the atmosphere. We provide observational data from a satellite instrument that shows a large CH4 plume over the North Sea off the coast of Scandinavia. We use this together with atmospheric models to quantify the CH4 leaked into the atmosphere from the pipelines. We find that 219–427 Gg CH4 was emitted, making this the largest individual fossil-fuel-related CH4 leak on record.
Joshua Dorrington, Marta Wenta, Federico Grazzini, Linus Magnusson, Frederic Vitart, and Christian M. Grams
Nat. Hazards Earth Syst. Sci., 24, 2995–3012, https://doi.org/10.5194/nhess-24-2995-2024, https://doi.org/10.5194/nhess-24-2995-2024, 2024
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Extreme rainfall is the leading weather-related source of damages in Europe, but it is still difficult to predict on long timescales. A recent example of this was the devastating floods in the Italian region of Emiglia Romagna in May 2023. We present perspectives based on large-scale dynamical information that allows us to better understand and predict such events.
Henk Eskes, Athanasios Tsikerdekis, Melanie Ades, Mihai Alexe, Anna Carlin Benedictow, Yasmine Bennouna, Lewis Blake, Idir Bouarar, Simon Chabrillat, Richard Engelen, Quentin Errera, Johannes Flemming, Sebastien Garrigues, Jan Griesfeller, Vincent Huijnen, Luka Ilić, Antje Inness, John Kapsomenakis, Zak Kipling, Bavo Langerock, Augustin Mortier, Mark Parrington, Isabelle Pison, Mikko Pitkänen, Samuel Remy, Andreas Richter, Anja Schoenhardt, Michael Schulz, Valerie Thouret, Thorsten Warneke, Christos Zerefos, and Vincent-Henri Peuch
Atmos. Chem. Phys., 24, 9475–9514, https://doi.org/10.5194/acp-24-9475-2024, https://doi.org/10.5194/acp-24-9475-2024, 2024
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The Copernicus Atmosphere Monitoring Service (CAMS) provides global analyses and forecasts of aerosols and trace gases in the atmosphere. On 27 June 2023 a major upgrade, Cy48R1, became operational. Comparisons with in situ, surface remote sensing, aircraft, and balloon and satellite observations show that the new CAMS system is a significant improvement. The results quantify the skill of CAMS to forecast impactful events, such as wildfires, dust storms and air pollution peaks.
Paula L. M. Gonzalez, Lesley J. Gray, Stergios Misios, Scott Osprey, and Hedi Ma
EGUsphere, https://doi.org/10.5194/egusphere-2024-2487, https://doi.org/10.5194/egusphere-2024-2487, 2024
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This study has examined a set of reanalyses, both modern and 20th Century, to evaluate the robustness of the signatures of the 11-yr solar cycle in the North Atlantic climate. We find a robust response to the 11-yr solar cycle over the North Atlantic sector with a positive SLP anomaly north of the Azores region at lags of +2–3 years following solar maximum. An ocean reanalysis dataset shows that thermal inertia of the ocean could explain the lag in the SC response.
Richard J. Pope, Fiona M. O'Connor, Mohit Dalvi, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Brice Barret, Eric Le Flochmoen, Anne Boynard, Martyn P. Chipperfield, Wuhu Feng, Matilda A. Pimlott, Sandip S. Dhomse, Christian Retscher, Catherine Wespes, and Richard Rigby
Atmos. Chem. Phys., 24, 9177–9195, https://doi.org/10.5194/acp-24-9177-2024, https://doi.org/10.5194/acp-24-9177-2024, 2024
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Ozone is a potent air pollutant in the lower troposphere, with adverse impacts on human health. Satellite records of tropospheric ozone currently show large-scale inconsistencies in long-term trends. Our detailed study of the potential factors (e.g. satellite errors, where the satellite can observe ozone) potentially driving these inconsistencies found that, in North America, Europe, and East Asia, the underlying trends are typically small with large uncertainties.
Sebastian Sippel, Clair Barnes, Camille Cadiou, Erich Fischer, Sarah Kew, Marlene Kretschmer, Sjoukje Philip, Theodore G. Shepherd, Jitendra Singh, Robert Vautard, and Pascal Yiou
Weather Clim. Dynam., 5, 943–957, https://doi.org/10.5194/wcd-5-943-2024, https://doi.org/10.5194/wcd-5-943-2024, 2024
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Winter temperatures in central Europe have increased. But cold winters can still cause problems for energy systems, infrastructure, or human health. Here we tested whether a record-cold winter, such as the one observed in 1963 over central Europe, could still occur despite climate change. The answer is yes: it is possible, but it is very unlikely. Our results rely on climate model simulations and statistical rare event analysis. In conclusion, society must be prepared for such cold winters.
Yang Li, Wuhu Feng, Xin Zhou, Yajuan Li, and Martyn P. Chipperfield
Atmos. Chem. Phys., 24, 8277–8293, https://doi.org/10.5194/acp-24-8277-2024, https://doi.org/10.5194/acp-24-8277-2024, 2024
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The Tibetan Plateau (TP), the highest and largest plateau, experiences strong surface solar UV radiation, whose excess can cause harmful influences on local biota. Hence, it is critical to study TP ozone. We find ENSO, the strongest interannual phenomenon, tends to induce tropospheric temperature change and thus modulate tropopause variability, which in turn favours ozone change over the TP. Our results have implications for a better understanding of the interannual variability of TP ozone.
Johannes Röttenbacher, André Ehrlich, Hanno Müller, Florian Ewald, Anna E. Luebke, Benjamin Kirbus, Robin J. Hogan, and Manfred Wendisch
Atmos. Chem. Phys., 24, 8085–8104, https://doi.org/10.5194/acp-24-8085-2024, https://doi.org/10.5194/acp-24-8085-2024, 2024
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Weather prediction models simplify the physical processes related to light scattering by clouds consisting of complex ice crystals. Whether these simplifications are the cause for uncertainties in their prediction can be evaluated by comparing them with measurement data. Here we do this for Arctic ice clouds over sea ice using airborne measurements from two case studies. The model performs well for thick ice clouds but not so well for thin ones. This work can be used to improve the model.
Masatomo Fujiwara, Patrick Martineau, Jonathon S. Wright, Marta Abalos, Petr Šácha, Yoshio Kawatani, Sean M. Davis, Thomas Birner, and Beatriz M. Monge-Sanz
Atmos. Chem. Phys., 24, 7873–7898, https://doi.org/10.5194/acp-24-7873-2024, https://doi.org/10.5194/acp-24-7873-2024, 2024
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A climatology of the major variables and terms of the transformed Eulerian-mean (TEM) momentum and thermodynamic equations from four global atmospheric reanalyses is evaluated. The spread among reanalysis TEM momentum balance terms is around 10 % in Northern Hemisphere winter and up to 50 % in Southern Hemisphere winter. The largest uncertainties in the thermodynamic equation (about 50 %) are in the vertical advection, which does not show a structure consistent with the differences in heating.
Swen Metzger, Samuel Rémy, Jason E. Williams, Vincent Huijnen, and Johannes Flemming
Geosci. Model Dev., 17, 5009–5021, https://doi.org/10.5194/gmd-17-5009-2024, https://doi.org/10.5194/gmd-17-5009-2024, 2024
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EQSAM4Clim has recently been revised to provide an accurate and efficient method for calculating the acidity of atmospheric particles. It is based on an analytical concept that is sufficiently fast and free of numerical noise, which makes it attractive for air quality forecasting. Version 12 allows the calculation of aerosol composition based on the gas–liquid–solid and the reduced gas–liquid partitioning with the associated water uptake for both cases, including the acidity of the aerosols.
Peng Xian, Jeffrey S. Reid, Melanie Ades, Angela Benedetti, Peter R. Colarco, Arlindo da Silva, Tom F. Eck, Johannes Flemming, Edward J. Hyer, Zak Kipling, Samuel Rémy, Tsuyoshi Thomas Sekiyama, Taichu Tanaka, Keiya Yumimoto, and Jianglong Zhang
Atmos. Chem. Phys., 24, 6385–6411, https://doi.org/10.5194/acp-24-6385-2024, https://doi.org/10.5194/acp-24-6385-2024, 2024
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The study compares and evaluates monthly AOD of four reanalyses (RA) and their consensus (i.e., ensemble mean). The basic verification characteristics of these RA versus both AERONET and MODIS retrievals are presented. The study discusses the strength of each RA and identifies regions where divergence and challenges are prominent. The RA consensus usually performs very well on a global scale in terms of how well it matches the observational data, making it a good choice for various applications.
Robin J. Hogan, Anthony J. Illingworth, Pavlos Kollias, Hajime Okamoto, and Ulla Wandinger
Atmos. Meas. Tech., 17, 3081–3083, https://doi.org/10.5194/amt-17-3081-2024, https://doi.org/10.5194/amt-17-3081-2024, 2024
Hanno Müller, André Ehrlich, Evelyn Jäkel, Johannes Röttenbacher, Benjamin Kirbus, Michael Schäfer, Robin J. Hogan, and Manfred Wendisch
Atmos. Chem. Phys., 24, 4157–4175, https://doi.org/10.5194/acp-24-4157-2024, https://doi.org/10.5194/acp-24-4157-2024, 2024
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A weather model is used to compare solar radiation with measurements from an aircraft campaign in the Arctic. Model and observations agree on the downward radiation but show differences in the radiation reflected by the surface and the clouds, which in the model is too low above sea ice and too high above open ocean. The model–observation bias is reduced above open ocean by a realistic fraction of clouds and less cloud liquid water and above sea ice by less dark sea ice and more cloud droplets.
Wilson C. H. Chan, Nigel W. Arnell, Geoff Darch, Katie Facer-Childs, Theodore G. Shepherd, and Maliko Tanguy
Nat. Hazards Earth Syst. Sci., 24, 1065–1078, https://doi.org/10.5194/nhess-24-1065-2024, https://doi.org/10.5194/nhess-24-1065-2024, 2024
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The most recent drought in the UK was declared in summer 2022. We pooled a large sample of plausible winters from seasonal hindcasts and grouped them into four clusters based on their atmospheric circulation configurations. Drought storylines representative of what the drought could have looked like if winter 2022/23 resembled each winter circulation storyline were created to explore counterfactuals of how bad the 2022 drought could have been over winter 2022/23 and beyond.
Richard J. Pope, Alexandru Rap, Matilda A. Pimlott, Brice Barret, Eric Le Flochmoen, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Anne Boynard, Christian Retscher, Wuhu Feng, Richard Rigby, Sandip S. Dhomse, Catherine Wespes, and Martyn P. Chipperfield
Atmos. Chem. Phys., 24, 3613–3626, https://doi.org/10.5194/acp-24-3613-2024, https://doi.org/10.5194/acp-24-3613-2024, 2024
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Tropospheric ozone is an important short-lived climate forcer which influences the incoming solar short-wave radiation and the outgoing long-wave radiation in the atmosphere (8–15 km) where the balance between the two yields a net positive (i.e. warming) effect at the surface. Overall, we find that the tropospheric ozone radiative effect ranges between 1.21 and 1.26 W m−2 with a negligible trend (2008–2017), suggesting that tropospheric ozone influences on climate have remained stable with time.
Emily Dowd, Alistair J. Manning, Bryn Orth-Lashley, Marianne Girard, James France, Rebecca E. Fisher, Dave Lowry, Mathias Lanoisellé, Joseph R. Pitt, Kieran M. Stanley, Simon O'Doherty, Dickon Young, Glen Thistlethwaite, Martyn P. Chipperfield, Emanuel Gloor, and Chris Wilson
Atmos. Meas. Tech., 17, 1599–1615, https://doi.org/10.5194/amt-17-1599-2024, https://doi.org/10.5194/amt-17-1599-2024, 2024
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We provide the first validation of the satellite-derived emission estimates using surface-based mobile greenhouse gas surveys of an active gas leak detected near Cheltenham, UK. GHGSat’s emission estimates broadly agree with the surface-based mobile survey and steps were taken to fix the leak, highlighting the importance of satellite data in identifying emissions and helping to reduce our human impact on climate change.
Martyn P. Chipperfield and Slimane Bekki
Atmos. Chem. Phys., 24, 2783–2802, https://doi.org/10.5194/acp-24-2783-2024, https://doi.org/10.5194/acp-24-2783-2024, 2024
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We give a personal perspective on recent issues related to the depletion of stratospheric ozone and some newly emerging challenges. We first provide a brief review of historic work on understanding the ozone layer and review ozone recovery from the effects of halogenated source gases and the Montreal Protocol. We then discuss the recent observations of ozone depletion from Australian fires in early 2020 and the Hunga Tonga–Hunga Ha'apai volcano in January 2022.
Shannon L. Mason, Howard W. Barker, Jason N. S. Cole, Nicole Docter, David P. Donovan, Robin J. Hogan, Anja Hünerbein, Pavlos Kollias, Bernat Puigdomènech Treserras, Zhipeng Qu, Ulla Wandinger, and Gerd-Jan van Zadelhoff
Atmos. Meas. Tech., 17, 875–898, https://doi.org/10.5194/amt-17-875-2024, https://doi.org/10.5194/amt-17-875-2024, 2024
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When the EarthCARE mission enters its operational phase, many retrieval data products will be available, which will overlap both in terms of the measurements they use and the geophysical quantities they report. In this pre-launch study, we use simulated EarthCARE scenes to compare the coverage and performance of many data products from the European Space Agency production model, with the intention of better understanding the relation between products and providing a compact guide to users.
Ailish M. Graham, Richard J. Pope, Martyn P. Chipperfield, Sandip S. Dhomse, Matilda Pimlott, Wuhu Feng, Vikas Singh, Ying Chen, Oliver Wild, Ranjeet Sokhi, and Gufran Beig
Atmos. Chem. Phys., 24, 789–806, https://doi.org/10.5194/acp-24-789-2024, https://doi.org/10.5194/acp-24-789-2024, 2024
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Our paper uses novel satellite datasets and high-resolution emissions datasets alongside a back-trajectory model to investigate the balance of local and external sources influencing NOx air pollution changes in Delhi. We find in the post-monsoon season that NOx from local and non-local transport emissions contributes most to poor air quality in Delhi. Therefore, air quality mitigation strategies in Delhi and surrounding regions are used to control this issue.
Andrea Pazmiño, Florence Goutail, Sophie Godin-Beekmann, Alain Hauchecorne, Jean-Pierre Pommereau, Martyn P. Chipperfield, Wuhu Feng, Franck Lefèvre, Audrey Lecouffe, Michel Van Roozendael, Nis Jepsen, Georg Hansen, Rigel Kivi, Kimberly Strong, and Kaley A. Walker
Atmos. Chem. Phys., 23, 15655–15670, https://doi.org/10.5194/acp-23-15655-2023, https://doi.org/10.5194/acp-23-15655-2023, 2023
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The vortex-averaged ozone loss over the last 3 decades is evaluated for both polar regions using the passive ozone tracer of the chemical transport model TOMCAT/SLIMCAT and total ozone observations from the SAOZ network and MSR2 reanalysis. Three metrics were developed to compute ozone trends since 2000. The study confirms the ozone recovery in the Antarctic and shows a potential sign of quantitative detection of ozone recovery in the Arctic that needs to be robustly confirmed in the future.
Richard J. Pope, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Martyn P. Chipperfield, Wuhu Feng, Matilda A. Pimlott, Sandip S. Dhomse, Christian Retscher, and Richard Rigby
Atmos. Chem. Phys., 23, 14933–14947, https://doi.org/10.5194/acp-23-14933-2023, https://doi.org/10.5194/acp-23-14933-2023, 2023
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Ozone is a potent air pollutant, and we present the first study to investigate long-term changes in lower tropospheric column ozone (LTCO3) from space. We have constructed a merged LTCO3 dataset from GOME-1, SCIAMACHY and OMI between 1996 and 2017. Comparing LTCO3 between the 1996–2000 and 2013–2017 5-year averages, we find significant positive increases in the tropics/sub-tropics, while in the northern mid-latitudes, we find small-scale differences.
Sandip S. Dhomse and Martyn P. Chipperfield
Earth Syst. Sci. Data, 15, 5105–5120, https://doi.org/10.5194/essd-15-5105-2023, https://doi.org/10.5194/essd-15-5105-2023, 2023
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There are no long-term stratospheric profile data sets for two very important greenhouse gases: methane (CH4) and nitrous oxide (N2O). Along with radiative feedback, these species play an important role in controlling ozone loss in the stratosphere. Here, we use machine learning to fuse satellite measurements with a chemical model to construct long-term gap-free profile data sets for CH4 and N2O. We aim to construct similar data sets for other important trace gases (e.g. O3, Cly, NOy species).
Ewa M. Bednarz, Ryan Hossaini, and Martyn P. Chipperfield
Atmos. Chem. Phys., 23, 13701–13711, https://doi.org/10.5194/acp-23-13701-2023, https://doi.org/10.5194/acp-23-13701-2023, 2023
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We quantify, for the first time, the time-varying impact of uncontrolled emissions of chlorinated very short-lived substances (Cl-VSLSs) on stratospheric ozone using a state-of-the-art chemistry-climate model. We demonstrate that Cl-VSLSs already have a non-negligible impact on stratospheric ozone, including a local reduction of up to ~7 DU in Arctic ozone in the cold winter of 2019/20, and any so future growth in emissions will continue to offset some of the benefits of the Montreal Protocol.
Ewa M. Bednarz, Ryan Hossaini, N. Luke Abraham, and Martyn P. Chipperfield
Geosci. Model Dev., 16, 6187–6209, https://doi.org/10.5194/gmd-16-6187-2023, https://doi.org/10.5194/gmd-16-6187-2023, 2023
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Development and performance of the new DEST chemistry scheme of UM–UKCA is described. The scheme extends the standard StratTrop scheme by including important updates to the halogen chemistry, thus allowing process-oriented studies of stratospheric ozone depletion and recovery, including impacts from both controlled long-lived ozone-depleting substances and emerging issues around uncontrolled, very short-lived substances. It will thus aid studies in support of future ozone assessment reports.
Megan A. Stretton, William Morrison, Robin J. Hogan, and Sue Grimmond
Geosci. Model Dev., 16, 5931–5947, https://doi.org/10.5194/gmd-16-5931-2023, https://doi.org/10.5194/gmd-16-5931-2023, 2023
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Cities' materials and forms impact radiative fluxes. We evaluate the SPARTACUS-Urban multi-layer approach to modelling longwave radiation, describing realistic 3D geometry statistically using the explicit DART (Discrete Anisotropic Radiative Transfer) model. The temperature configurations used are derived from thermal camera observations. SPARTACUS-Urban accurately predicts longwave fluxes, with a low computational time (cf. DART), but has larger errors with sunlit/shaded surface temperatures.
Richard J. Pope, Brian J. Kerridge, Martyn P. Chipperfield, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Matilda A. Pimlott, Wuhu Feng, Edward Comyn-Platt, Garry D. Hayman, Stephen R. Arnold, and Ailish M. Graham
Atmos. Chem. Phys., 23, 13235–13253, https://doi.org/10.5194/acp-23-13235-2023, https://doi.org/10.5194/acp-23-13235-2023, 2023
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In the summer of 2018, Europe experienced several persistent large-scale ozone (O3) pollution episodes. Satellite tropospheric O3 and surface O3 data recorded substantial enhancements in 2018 relative to other years. Targeted model simulations showed that meteorological processes and emissions controlled the elevated surface O3, while mid-tropospheric O3 enhancements were dominated by stratospheric O3 intrusion and advection of North Atlantic O3-rich air masses into Europe.
Yajuan Li, Sandip S. Dhomse, Martyn P. Chipperfield, Wuhu Feng, Jianchun Bian, Yuan Xia, and Dong Guo
Atmos. Chem. Phys., 23, 13029–13047, https://doi.org/10.5194/acp-23-13029-2023, https://doi.org/10.5194/acp-23-13029-2023, 2023
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For the first time a regularized multivariate regression model is used to estimate stratospheric ozone trends. Regularized regression avoids the over-fitting issue due to correlation among explanatory variables. We demonstrate that there are considerable differences in satellite-based and chemical-model-based ozone trends, highlighting large uncertainties in our understanding about ozone variability. We argue that caution is needed when interpreting results with different methods and datasets.
Sebastien Garrigues, Melanie Ades, Samuel Remy, Johannes Flemming, Zak Kipling, Istvan Laszlo, Mark Parrington, Antje Inness, Roberto Ribas, Luke Jones, Richard Engelen, and Vincent-Henri Peuch
Atmos. Chem. Phys., 23, 10473–10487, https://doi.org/10.5194/acp-23-10473-2023, https://doi.org/10.5194/acp-23-10473-2023, 2023
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The Copernicus Atmosphere Monitoring Service (CAMS) provides global monitoring of aerosols using the ECMWF forecast model constrained by the assimilation of satellite aerosol optical depth (AOD). This work aims at evaluating the assimilation of the NOAA VIIRS AOD product in the ECMWF model. It shows that the introduction of VIIRS in the CAMS data assimilation system enhances the accuracy of the aerosol analysis, particularly over Europe and desert and maritime sites.
Michael P. Cartwright, Richard J. Pope, Jeremy J. Harrison, Martyn P. Chipperfield, Chris Wilson, Wuhu Feng, David P. Moore, and Parvadha Suntharalingam
Atmos. Chem. Phys., 23, 10035–10056, https://doi.org/10.5194/acp-23-10035-2023, https://doi.org/10.5194/acp-23-10035-2023, 2023
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A 3-D chemical transport model, TOMCAT, is used to simulate global atmospheric carbonyl sulfide (OCS) distribution. Modelled OCS compares well with satellite observations of OCS from limb-sounding satellite observations. Model simulations also compare adequately with surface and atmospheric observations and suitably capture the seasonality of OCS and background concentrations.
Olivia E. Clifton, Donna Schwede, Christian Hogrefe, Jesse O. Bash, Sam Bland, Philip Cheung, Mhairi Coyle, Lisa Emberson, Johannes Flemming, Erick Fredj, Stefano Galmarini, Laurens Ganzeveld, Orestis Gazetas, Ignacio Goded, Christopher D. Holmes, László Horváth, Vincent Huijnen, Qian Li, Paul A. Makar, Ivan Mammarella, Giovanni Manca, J. William Munger, Juan L. Pérez-Camanyo, Jonathan Pleim, Limei Ran, Roberto San Jose, Sam J. Silva, Ralf Staebler, Shihan Sun, Amos P. K. Tai, Eran Tas, Timo Vesala, Tamás Weidinger, Zhiyong Wu, and Leiming Zhang
Atmos. Chem. Phys., 23, 9911–9961, https://doi.org/10.5194/acp-23-9911-2023, https://doi.org/10.5194/acp-23-9911-2023, 2023
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A primary sink of air pollutants is dry deposition. Dry deposition estimates differ across the models used to simulate atmospheric chemistry. Here, we introduce an effort to examine dry deposition schemes from atmospheric chemistry models. We provide our approach’s rationale, document the schemes, and describe datasets used to drive and evaluate the schemes. We also launch the analysis of results by evaluating against observations and identifying the processes leading to model–model differences.
Luana S. Basso, Chris Wilson, Martyn P. Chipperfield, Graciela Tejada, Henrique L. G. Cassol, Egídio Arai, Mathew Williams, T. Luke Smallman, Wouter Peters, Stijn Naus, John B. Miller, and Manuel Gloor
Atmos. Chem. Phys., 23, 9685–9723, https://doi.org/10.5194/acp-23-9685-2023, https://doi.org/10.5194/acp-23-9685-2023, 2023
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The Amazon’s carbon balance may have changed due to forest degradation, deforestation and warmer climate. We used an atmospheric model and atmospheric CO2 observations to quantify Amazonian carbon emissions (2010–2018). The region was a small carbon source to the atmosphere, mostly due to fire emissions. Forest uptake compensated for ~ 50 % of the fire emissions, meaning that the remaining forest is still a small carbon sink. We found no clear evidence of weakening carbon uptake over the period.
Giorgia Di Capua, Dim Coumou, Bart van den Hurk, Antje Weisheimer, Andrew G. Turner, and Reik V. Donner
Weather Clim. Dynam., 4, 701–723, https://doi.org/10.5194/wcd-4-701-2023, https://doi.org/10.5194/wcd-4-701-2023, 2023
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Heavy rainfall in tropical regions interacts with mid-latitude circulation patterns, and this interaction can explain weather patterns in the Northern Hemisphere during summer. In this analysis we detect these tropical–extratropical interaction pattern both in observational datasets and data obtained by atmospheric models and assess how well atmospheric models can reproduce the observed patterns. We find a good agreement although these relationships are weaker in model data.
Shannon L. Mason, Robin J. Hogan, Alessio Bozzo, and Nicola L. Pounder
Atmos. Meas. Tech., 16, 3459–3486, https://doi.org/10.5194/amt-16-3459-2023, https://doi.org/10.5194/amt-16-3459-2023, 2023
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We present a method for accurately estimating the contents and properties of clouds, snow, rain, and aerosols through the atmosphere, using the combined measurements of the radar, lidar, and radiometer instruments aboard the upcoming EarthCARE satellite, and evaluate the performance of the retrieval, using test scenes simulated from a numerical forecast model. When EarthCARE is in operation, these quantities and their estimated uncertainties will be distributed in a data product called ACM-CAP.
Emily Dowd, Chris Wilson, Martyn P. Chipperfield, Emanuel Gloor, Alistair Manning, and Ruth Doherty
Atmos. Chem. Phys., 23, 7363–7382, https://doi.org/10.5194/acp-23-7363-2023, https://doi.org/10.5194/acp-23-7363-2023, 2023
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Surface observations of methane show that the seasonal cycle amplitude (SCA) of methane is decreasing in the northern high latitudes (NHLs) but increased globally (1995–2020). The NHL decrease is counterintuitive, as we expect the SCA to increase with increasing concentrations. We use a chemical transport model to investigate changes in SCA in the NHLs. We find well-mixed methane and changes in emissions from Canada, the Middle East, and Europe are the largest contributors to the SCA in NHLs.
Nicholas Williams, Nicholas Byrne, Daniel Feltham, Peter Jan Van Leeuwen, Ross Bannister, David Schroeder, Andrew Ridout, and Lars Nerger
The Cryosphere, 17, 2509–2532, https://doi.org/10.5194/tc-17-2509-2023, https://doi.org/10.5194/tc-17-2509-2023, 2023
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Observations show that the Arctic sea ice cover has reduced over the last 40 years. This study uses ensemble-based data assimilation in a stand-alone sea ice model to investigate the impacts of assimilating three different kinds of sea ice observation, including the novel assimilation of sea ice thickness distribution. We show that assimilating ice thickness distribution has a positive impact on thickness and volume estimates within the ice pack, especially for very thick ice.
Peter Ukkonen and Robin J. Hogan
Geosci. Model Dev., 16, 3241–3261, https://doi.org/10.5194/gmd-16-3241-2023, https://doi.org/10.5194/gmd-16-3241-2023, 2023
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Climate and weather models suffer from uncertainties resulting from approximated processes. Solar and thermal radiation is one example, as it is computationally too costly to simulate precisely. This has led to attempts to replace radiation codes based on physical equations with neural networks (NNs) that are faster but uncertain. In this paper we use global weather simulations to demonstrate that a middle-ground approach of using NNs only to predict optical properties is accurate and reliable.
Abdanour Irbah, Julien Delanoë, Gerd-Jan van Zadelhoff, David P. Donovan, Pavlos Kollias, Bernat Puigdomènech Treserras, Shannon Mason, Robin J. Hogan, and Aleksandra Tatarevic
Atmos. Meas. Tech., 16, 2795–2820, https://doi.org/10.5194/amt-16-2795-2023, https://doi.org/10.5194/amt-16-2795-2023, 2023
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The Cloud Profiling Radar (CPR) and ATmospheric LIDar (ATLID) aboard the EarthCARE satellite are used to probe the Earth's atmosphere by measuring cloud and aerosol profiles. ATLID is sensitive to aerosols and small cloud particles and CPR to large ice particles, snowflakes and raindrops. It is the synergy of the measurements of these two instruments that allows a better classification of the atmospheric targets and the description of the associated products, which are the subject of this paper.
Peter Joyce, Cristina Ruiz Villena, Yahui Huang, Alex Webb, Manuel Gloor, Fabien H. Wagner, Martyn P. Chipperfield, Rocío Barrio Guilló, Chris Wilson, and Hartmut Boesch
Atmos. Meas. Tech., 16, 2627–2640, https://doi.org/10.5194/amt-16-2627-2023, https://doi.org/10.5194/amt-16-2627-2023, 2023
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Methane emissions are responsible for a lot of the warming caused by the greenhouse effect, much of which comes from a small number of point sources. We can identify methane point sources by analysing satellite data, but it requires a lot of time invested by experts and is prone to very high errors. Here, we produce a neural network that can automatically identify methane point sources and estimate the mass of methane that is being released per hour and are able to do so with far smaller errors.
Antonio G. Bruno, Jeremy J. Harrison, Martyn P. Chipperfield, David P. Moore, Richard J. Pope, Christopher Wilson, Emmanuel Mahieu, and Justus Notholt
Atmos. Chem. Phys., 23, 4849–4861, https://doi.org/10.5194/acp-23-4849-2023, https://doi.org/10.5194/acp-23-4849-2023, 2023
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A 3-D chemical transport model, TOMCAT; satellite data; and ground-based observations have been used to investigate hydrogen cyanide (HCN) variability. We found that the oxidation by O(1D) drives the HCN loss in the middle stratosphere and the currently JPL-recommended OH reaction rate overestimates HCN atmospheric loss. We also evaluated two different ocean uptake schemes. We found them to be unrealistic, and we need to scale these schemes to obtain good agreement with HCN observations.
Anna Agustí-Panareda, Jérôme Barré, Sébastien Massart, Antje Inness, Ilse Aben, Melanie Ades, Bianca C. Baier, Gianpaolo Balsamo, Tobias Borsdorff, Nicolas Bousserez, Souhail Boussetta, Michael Buchwitz, Luca Cantarello, Cyril Crevoisier, Richard Engelen, Henk Eskes, Johannes Flemming, Sébastien Garrigues, Otto Hasekamp, Vincent Huijnen, Luke Jones, Zak Kipling, Bavo Langerock, Joe McNorton, Nicolas Meilhac, Stefan Noël, Mark Parrington, Vincent-Henri Peuch, Michel Ramonet, Miha Razinger, Maximilian Reuter, Roberto Ribas, Martin Suttie, Colm Sweeney, Jérôme Tarniewicz, and Lianghai Wu
Atmos. Chem. Phys., 23, 3829–3859, https://doi.org/10.5194/acp-23-3829-2023, https://doi.org/10.5194/acp-23-3829-2023, 2023
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We present a global dataset of atmospheric CO2 and CH4, the two most important human-made greenhouse gases, which covers almost 2 decades (2003–2020). It is produced by combining satellite data of CO2 and CH4 with a weather and air composition prediction model, and it has been carefully evaluated against independent observations to ensure validity and point out deficiencies to the user. This dataset can be used for scientific studies in the field of climate change and the global carbon cycle.
Wolfgang Wicker, Inna Polichtchouk, and Daniela I. V. Domeisen
Weather Clim. Dynam., 4, 81–93, https://doi.org/10.5194/wcd-4-81-2023, https://doi.org/10.5194/wcd-4-81-2023, 2023
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Sudden stratospheric warmings are extreme weather events where the winter polar stratosphere warms by about 25 K. An improved representation of small-scale gravity waves in sub-seasonal prediction models can reduce forecast errors since their impact on the large-scale circulation is predictable multiple weeks ahead. After a sudden stratospheric warming, vertically propagating gravity waves break at a lower altitude than usual, which strengthens the long-lasting positive temperature anomalies.
Philipp Breul, Paulo Ceppi, and Theodore G. Shepherd
Weather Clim. Dynam., 4, 39–47, https://doi.org/10.5194/wcd-4-39-2023, https://doi.org/10.5194/wcd-4-39-2023, 2023
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Accurately predicting the response of the midlatitude jet stream to climate change is very important, but models show a variety of possible scenarios. Previous work identified a relationship between climatological jet latitude and future jet shift in the southern hemispheric winter. We show that the relationship does not hold in separate sectors and propose that zonal asymmetries are the ultimate cause in the zonal mean. This questions the usefulness of the relationship.
Robert J. Parker, Chris Wilson, Edward Comyn-Platt, Garry Hayman, Toby R. Marthews, A. Anthony Bloom, Mark F. Lunt, Nicola Gedney, Simon J. Dadson, Joe McNorton, Neil Humpage, Hartmut Boesch, Martyn P. Chipperfield, Paul I. Palmer, and Dai Yamazaki
Biogeosciences, 19, 5779–5805, https://doi.org/10.5194/bg-19-5779-2022, https://doi.org/10.5194/bg-19-5779-2022, 2022
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Wetlands are the largest natural source of methane, one of the most important climate gases. The JULES land surface model simulates these emissions. We use satellite data to evaluate how well JULES reproduces the methane seasonal cycle over different tropical wetlands. It performs well for most regions; however, it struggles for some African wetlands influenced heavily by river flooding. We explain the reasons for these deficiencies and highlight how future development will improve these areas.
Stijn Naus, Lucas G. Domingues, Maarten Krol, Ingrid T. Luijkx, Luciana V. Gatti, John B. Miller, Emanuel Gloor, Sourish Basu, Caio Correia, Gerbrand Koren, Helen M. Worden, Johannes Flemming, Gabrielle Pétron, and Wouter Peters
Atmos. Chem. Phys., 22, 14735–14750, https://doi.org/10.5194/acp-22-14735-2022, https://doi.org/10.5194/acp-22-14735-2022, 2022
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We assimilate MOPITT CO satellite data in the TM5-4D-Var inverse modelling framework to estimate Amazon fire CO emissions for 2003–2018. We show that fire emissions have decreased over the analysis period, coincident with a decrease in deforestation rates. However, interannual variations in fire emissions are large, and they correlate strongly with soil moisture. Our results reveal an important role for robust, top-down fire CO emissions in quantifying and attributing Amazon fire intensity.
Sebastien Garrigues, Samuel Remy, Julien Chimot, Melanie Ades, Antje Inness, Johannes Flemming, Zak Kipling, Istvan Laszlo, Angela Benedetti, Roberto Ribas, Soheila Jafariserajehlou, Bertrand Fougnie, Shobha Kondragunta, Richard Engelen, Vincent-Henri Peuch, Mark Parrington, Nicolas Bousserez, Margarita Vazquez Navarro, and Anna Agusti-Panareda
Atmos. Chem. Phys., 22, 14657–14692, https://doi.org/10.5194/acp-22-14657-2022, https://doi.org/10.5194/acp-22-14657-2022, 2022
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The Copernicus Atmosphere Monitoring Service (CAMS) provides global monitoring of aerosols using the ECMWF forecast model constrained by the assimilation of satellite aerosol optical depth (AOD). This work aims at evaluating two new satellite AODs to enhance the CAMS aerosol global forecast. It highlights the spatial and temporal differences between the satellite AOD products at the model spatial resolution, which is essential information to design multi-satellite AOD data assimilation schemes.
Antje Inness, Ilse Aben, Melanie Ades, Tobias Borsdorff, Johannes Flemming, Luke Jones, Jochen Landgraf, Bavo Langerock, Philippe Nedelec, Mark Parrington, and Roberto Ribas
Atmos. Chem. Phys., 22, 14355–14376, https://doi.org/10.5194/acp-22-14355-2022, https://doi.org/10.5194/acp-22-14355-2022, 2022
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The Copernicus Atmosphere Monitoring Service (CAMS) provides daily global air quality forecasts to users worldwide. One of the species of interest is carbon monoxide (CO), an important trace gas in the atmosphere with anthropogenic and natural sources, produced by incomplete combustion, for example, by wildfires. This paper looks at how well CAMS can model CO in the atmosphere and shows that the fields can be improved when blending CO data from the TROPOMI instrument with the CAMS model.
Ewa M. Bednarz, Ryan Hossaini, Martyn P. Chipperfield, N. Luke Abraham, and Peter Braesicke
Atmos. Chem. Phys., 22, 10657–10676, https://doi.org/10.5194/acp-22-10657-2022, https://doi.org/10.5194/acp-22-10657-2022, 2022
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Atmospheric impacts of chlorinated very short-lived substances (Cl-VSLS) over the first two decades of the 21st century are assessed using the UM-UKCA chemistry–climate model. Stratospheric input of Cl from Cl-VSLS is estimated at ~130 ppt in 2019. The use of model set-up with constrained meteorology significantly increases the abundance of Cl-VSLS in the lower stratosphere relative to the free-running set-up. The growth in Cl-VSLS emissions significantly impacted recent HCl and COCl2 trends.
Yajuan Li, Sandip S. Dhomse, Martyn P. Chipperfield, Wuhu Feng, Andreas Chrysanthou, Yuan Xia, and Dong Guo
Atmos. Chem. Phys., 22, 10635–10656, https://doi.org/10.5194/acp-22-10635-2022, https://doi.org/10.5194/acp-22-10635-2022, 2022
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Chemical transport models forced with (re)analysis meteorological fields are ideally suited for interpreting the influence of important physical processes on the ozone variability. We use TOMCAT forced by ECMWF ERA-Interim and ERA5 reanalysis data sets to investigate the effects of reanalysis forcing fields on ozone changes. Our results show that models forced by ERA5 reanalyses may not yet be capable of reproducing observed changes in stratospheric ozone, particularly in the lower stratosphere.
Zachary D. Lawrence, Marta Abalos, Blanca Ayarzagüena, David Barriopedro, Amy H. Butler, Natalia Calvo, Alvaro de la Cámara, Andrew Charlton-Perez, Daniela I. V. Domeisen, Etienne Dunn-Sigouin, Javier García-Serrano, Chaim I. Garfinkel, Neil P. Hindley, Liwei Jia, Martin Jucker, Alexey Y. Karpechko, Hera Kim, Andrea L. Lang, Simon H. Lee, Pu Lin, Marisol Osman, Froila M. Palmeiro, Judith Perlwitz, Inna Polichtchouk, Jadwiga H. Richter, Chen Schwartz, Seok-Woo Son, Irene Erner, Masakazu Taguchi, Nicholas L. Tyrrell, Corwin J. Wright, and Rachel W.-Y. Wu
Weather Clim. Dynam., 3, 977–1001, https://doi.org/10.5194/wcd-3-977-2022, https://doi.org/10.5194/wcd-3-977-2022, 2022
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Forecast models that are used to predict weather often struggle to represent the Earth’s stratosphere. This may impact their ability to predict surface weather weeks in advance, on subseasonal-to-seasonal (S2S) timescales. We use data from many S2S forecast systems to characterize and compare the stratospheric biases present in such forecast models. These models have many similar stratospheric biases, but they tend to be worse in systems with low model tops located within the stratosphere.
Matilda A. Pimlott, Richard J. Pope, Brian J. Kerridge, Barry G. Latter, Diane S. Knappett, Dwayne E. Heard, Lucy J. Ventress, Richard Siddans, Wuhu Feng, and Martyn P. Chipperfield
Atmos. Chem. Phys., 22, 10467–10488, https://doi.org/10.5194/acp-22-10467-2022, https://doi.org/10.5194/acp-22-10467-2022, 2022
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We present a new method to derive global information of the hydroxyl radical (OH), an important atmospheric oxidant. OH controls the lifetime of trace gases important to air quality and climate. We use satellite observations of ozone, carbon monoxide, methane and water vapour in a simple expression to derive OH around 3–4 km altitude. The derived OH compares well to model and aircraft OH data. We then apply the method to 10 years of satellite data to study the inter-annual variability of OH.
Vincent Huijnen, Philippe Le Sager, Marcus O. Köhler, Glenn Carver, Samuel Rémy, Johannes Flemming, Simon Chabrillat, Quentin Errera, and Twan van Noije
Geosci. Model Dev., 15, 6221–6241, https://doi.org/10.5194/gmd-15-6221-2022, https://doi.org/10.5194/gmd-15-6221-2022, 2022
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We report on the first implementation of atmospheric chemistry and aerosol as part of the OpenIFS model, based on the CAMS global model. We give an overview of the model and evaluate two reference model configurations, with and without the stratospheric chemistry extension, against a variety of observational datasets. This OpenIFS version with atmospheric composition components is open to the scientific user community under a standard OpenIFS license.
Jorge L. García-Franco, Lesley J. Gray, Scott Osprey, Robin Chadwick, and Zane Martin
Weather Clim. Dynam., 3, 825–844, https://doi.org/10.5194/wcd-3-825-2022, https://doi.org/10.5194/wcd-3-825-2022, 2022
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This paper establishes robust links between the stratospheric quasi-biennial oscillation (QBO) and several features of tropical climate. Robust precipitation responses, as well as changes to the Walker circulation, were found to be robustly linked to the variability in the lower stratosphere associated with the QBO using a 500-year simulation of a state-of-the-art climate model.
Jonathan J. Day, Sarah Keeley, Gabriele Arduini, Linus Magnusson, Kristian Mogensen, Mark Rodwell, Irina Sandu, and Steffen Tietsche
Weather Clim. Dynam., 3, 713–731, https://doi.org/10.5194/wcd-3-713-2022, https://doi.org/10.5194/wcd-3-713-2022, 2022
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A recent drive to develop seamless forecasting systems has culminated in the development of weather forecasting systems that include a coupled representation of the atmosphere, ocean and sea ice. Before this, sea ice and sea surface temperature anomalies were typically fixed throughout a given forecast. We show that the dynamic coupling is most beneficial during periods of rapid ice advance, where persistence is a poor forecast of the sea ice and leads to large errors in the uncoupled system.
Samuel Rémy, Zak Kipling, Vincent Huijnen, Johannes Flemming, Pierre Nabat, Martine Michou, Melanie Ades, Richard Engelen, and Vincent-Henri Peuch
Geosci. Model Dev., 15, 4881–4912, https://doi.org/10.5194/gmd-15-4881-2022, https://doi.org/10.5194/gmd-15-4881-2022, 2022
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This article describes a new version of IFS-AER, the tropospheric aerosol scheme used to provide global aerosol products within the Copernicus Atmosphere Monitoring Service (CAMS) cycle. Several components of the model have been updated, such as the dynamical dust and sea salt aerosol emission schemes. New deposition schemes have also been incorporated but are not yet used operationally. This new version of IFS-AER has been evaluated and shown to have a greater skill than previous versions.
Jason E. Williams, Vincent Huijnen, Idir Bouarar, Mehdi Meziane, Timo Schreurs, Sophie Pelletier, Virginie Marécal, Beatrice Josse, and Johannes Flemming
Geosci. Model Dev., 15, 4657–4687, https://doi.org/10.5194/gmd-15-4657-2022, https://doi.org/10.5194/gmd-15-4657-2022, 2022
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The global CAMS air quality model is used for providing tropospheric ozone information to end users. This paper updates the chemical mechanism employed (CBA) and compares it against two other mechanisms (MOCAGE, MOZART) and a multi-decadal dataset based on a previous version of CBA. We perform extensive validation for the US using multiple surface and aircraft datasets, providing an assessment of biases and the extent of correlation across different seasons during 2014.
Philipp Breul, Paulo Ceppi, and Theodore G. Shepherd
Weather Clim. Dynam., 3, 645–658, https://doi.org/10.5194/wcd-3-645-2022, https://doi.org/10.5194/wcd-3-645-2022, 2022
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Understanding how the mid-latitude jet stream will respond to a changing climate is highly important. Unfortunately, climate models predict a wide variety of possible responses. Theoretical frameworks can link an internal jet variability timescale to its response. However, we show that stratospheric influence approximately doubles the internal timescale, inflating predicted responses. We demonstrate an approach to account for the stratospheric influence and recover correct response predictions.
Dimitris Akritidis, Andrea Pozzer, Johannes Flemming, Antje Inness, Philippe Nédélec, and Prodromos Zanis
Atmos. Chem. Phys., 22, 6275–6289, https://doi.org/10.5194/acp-22-6275-2022, https://doi.org/10.5194/acp-22-6275-2022, 2022
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We perform a process-oriented evaluation of Copernicus Atmosphere Monitoring Service (CAMS) reanalysis (CAMSRA) O3 over Europe using WOUDC (World Ozone and Ultraviolet Radiation Data Centre) ozonesondes and IAGOS (In-service Aircraft for a Global Observing System) aircraft measurements. Chemical data assimilation assists CAMSRA to reproduce the observed O3 increases in the troposphere during the examined folding events, but it mostly results in O3 overestimation in the upper troposphere.
Oscar Dimdore-Miles, Lesley Gray, Scott Osprey, Jon Robson, Rowan Sutton, and Bablu Sinha
Atmos. Chem. Phys., 22, 4867–4893, https://doi.org/10.5194/acp-22-4867-2022, https://doi.org/10.5194/acp-22-4867-2022, 2022
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This study examines interactions between variations in the strength of polar stratospheric winds and circulation in the North Atlantic in a climate model simulation. It finds that the Atlantic Meridional Overturning Circulation (AMOC) responds with oscillations to sets of consecutive Northern Hemisphere winters, which show all strong or all weak polar vortex conditions. The study also shows that a set of strong vortex winters in the 1990s contributed to the recent slowdown in the observed AMOC.
Wilson C. H. Chan, Theodore G. Shepherd, Katie Facer-Childs, Geoff Darch, and Nigel W. Arnell
Hydrol. Earth Syst. Sci., 26, 1755–1777, https://doi.org/10.5194/hess-26-1755-2022, https://doi.org/10.5194/hess-26-1755-2022, 2022
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We select the 2010–2012 UK drought and investigate an alternative unfolding of the drought from changes to its attributes. We created storylines of drier preconditions, alternative seasonal contributions, a third dry winter, and climate change. Storylines of the 2010–2012 drought show alternative situations that could have resulted in worse conditions than observed. Event-based storylines exploring plausible situations are used that may lead to high impacts and help stress test existing systems.
Richard J. Pope, Rebecca Kelly, Eloise A. Marais, Ailish M. Graham, Chris Wilson, Jeremy J. Harrison, Savio J. A. Moniz, Mohamed Ghalaieny, Steve R. Arnold, and Martyn P. Chipperfield
Atmos. Chem. Phys., 22, 4323–4338, https://doi.org/10.5194/acp-22-4323-2022, https://doi.org/10.5194/acp-22-4323-2022, 2022
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Nitrogen oxides (NOx) are potent air pollutants which directly impact on human health. In this study, we use satellite nitrogen dioxide (NO2) data to evaluate the spatial distribution and temporal evolution of the UK official NOx emissions inventory, with reasonable agreement. We also derived satellite-based NOx emissions for several UK cities. In the case of London and Birmingham, the NAEI NOx emissions are potentially too low by >50%.
Piera Raspollini, Enrico Arnone, Flavio Barbara, Massimo Bianchini, Bruno Carli, Simone Ceccherini, Martyn P. Chipperfield, Angelika Dehn, Stefano Della Fera, Bianca Maria Dinelli, Anu Dudhia, Jean-Marie Flaud, Marco Gai, Michael Kiefer, Manuel López-Puertas, David P. Moore, Alessandro Piro, John J. Remedios, Marco Ridolfi, Harjinder Sembhi, Luca Sgheri, and Nicola Zoppetti
Atmos. Meas. Tech., 15, 1871–1901, https://doi.org/10.5194/amt-15-1871-2022, https://doi.org/10.5194/amt-15-1871-2022, 2022
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The MIPAS instrument onboard the ENVISAT satellite provided 10 years of measurements of the atmospheric emission al limb that allow for the retrieval of latitude- and altitude-resolved atmospheric composition. We describe the improvements implemented in the retrieval algorithm used for the full mission reanalysis, which allows for the generation of the global distributions of 21 atmospheric constituents plus temperature with increased accuracy with respect to previously generated data.
Adam A. Scaife, Mark P. Baldwin, Amy H. Butler, Andrew J. Charlton-Perez, Daniela I. V. Domeisen, Chaim I. Garfinkel, Steven C. Hardiman, Peter Haynes, Alexey Yu Karpechko, Eun-Pa Lim, Shunsuke Noguchi, Judith Perlwitz, Lorenzo Polvani, Jadwiga H. Richter, John Scinocca, Michael Sigmond, Theodore G. Shepherd, Seok-Woo Son, and David W. J. Thompson
Atmos. Chem. Phys., 22, 2601–2623, https://doi.org/10.5194/acp-22-2601-2022, https://doi.org/10.5194/acp-22-2601-2022, 2022
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Great progress has been made in computer modelling and simulation of the whole climate system, including the stratosphere. Since the late 20th century we also gained a much clearer understanding of how the stratosphere interacts with the lower atmosphere. The latest generation of numerical prediction systems now explicitly represents the stratosphere and its interaction with surface climate, and here we review its role in long-range predictions and projections from weeks to decades ahead.
Antje Inness, Melanie Ades, Dimitris Balis, Dmitry Efremenko, Johannes Flemming, Pascal Hedelt, Maria-Elissavet Koukouli, Diego Loyola, and Roberto Ribas
Geosci. Model Dev., 15, 971–994, https://doi.org/10.5194/gmd-15-971-2022, https://doi.org/10.5194/gmd-15-971-2022, 2022
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This paper describes the way that the Copernicus Atmosphere Monitoring Service (CAMS) produces forecasts of volcanic SO2. These forecasts are provided routinely every day. They are created by blending SO2 data from satellite instruments (TROPOMI and GOME-2) with the CAMS model. We show that the quality of the CAMS SO2 forecasts can be improved if additional information about the height of volcanic plumes is provided in the satellite data.
Sandip S. Dhomse, Martyn P. Chipperfield, Wuhu Feng, Ryan Hossaini, Graham W. Mann, Michelle L. Santee, and Mark Weber
Atmos. Chem. Phys., 22, 903–916, https://doi.org/10.5194/acp-22-903-2022, https://doi.org/10.5194/acp-22-903-2022, 2022
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Solar flux variations associated with 11-year sunspot cycle is believed to exert important external climate forcing. As largest variations occur at shorter wavelengths such as ultra-violet part of the solar spectrum, associated changes in stratospheric ozone are thought to provide direct evidence for solar climate interaction. Until now, most of the studies reported double-peak structured solar cycle signal (SCS), but relatively new satellite data suggest only single-peak-structured SCS.
Martin Wegmann, Yvan Orsolini, Antje Weisheimer, Bart van den Hurk, and Gerrit Lohmann
Weather Clim. Dynam., 2, 1245–1261, https://doi.org/10.5194/wcd-2-1245-2021, https://doi.org/10.5194/wcd-2-1245-2021, 2021
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Northern Hemisphere winter weather is influenced by the strength of westerly winds 30 km above the surface, the so-called polar vortex. Eurasian autumn snow cover is thought to modulate the polar vortex. So far, however, the modeled influence of snow on the polar vortex did not fit the observed influence. By analyzing a model experiment for the time span of 110 years, we could show that the causality of this impact is indeed sound and snow cover can weaken the polar vortex.
Sandip S. Dhomse, Carlo Arosio, Wuhu Feng, Alexei Rozanov, Mark Weber, and Martyn P. Chipperfield
Earth Syst. Sci. Data, 13, 5711–5729, https://doi.org/10.5194/essd-13-5711-2021, https://doi.org/10.5194/essd-13-5711-2021, 2021
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High-quality long-term ozone profile data sets are key to estimating short- and long-term ozone variability. Almost all the satellite (and chemical model) data sets show some kind of bias with respect to each other. This is because of differences in measurement methodologies as well as simplified processes in the models. We use satellite data sets and chemical model output to generate 42 years of ozone profile data sets using a random-forest machine-learning algorithm that is named ML-TOMCAT.
Paul D. Hamer, Virginie Marécal, Ryan Hossaini, Michel Pirre, Gisèle Krysztofiak, Franziska Ziska, Andreas Engel, Stephan Sala, Timo Keber, Harald Bönisch, Elliot Atlas, Kirstin Krüger, Martyn Chipperfield, Valery Catoire, Azizan A. Samah, Marcel Dorf, Phang Siew Moi, Hans Schlager, and Klaus Pfeilsticker
Atmos. Chem. Phys., 21, 16955–16984, https://doi.org/10.5194/acp-21-16955-2021, https://doi.org/10.5194/acp-21-16955-2021, 2021
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Bromoform is a stratospheric ozone-depleting gas released by seaweed and plankton transported to the stratosphere via convection in the tropics. We study the chemical interactions of bromoform and its derivatives within convective clouds using a cloud-scale model and observations. Our findings are that soluble bromine gases are efficiently washed out and removed within the convective clouds and that most bromine is transported vertically to the upper troposphere in the form of bromoform.
Meike K. Rotermund, Vera Bense, Martyn P. Chipperfield, Andreas Engel, Jens-Uwe Grooß, Peter Hoor, Tilman Hüneke, Timo Keber, Flora Kluge, Benjamin Schreiner, Tanja Schuck, Bärbel Vogel, Andreas Zahn, and Klaus Pfeilsticker
Atmos. Chem. Phys., 21, 15375–15407, https://doi.org/10.5194/acp-21-15375-2021, https://doi.org/10.5194/acp-21-15375-2021, 2021
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Airborne total bromine (Brtot) and tracer measurements suggest Brtot-rich air masses persistently protruded into the lower stratosphere (LS), creating a high Brtot region over the North Atlantic in fall 2017. The main source is via isentropic transport by the Asian monsoon and to a lesser extent transport across the extratropical tropopause as quantified by a Lagrange model. The transport of Brtot via Central American hurricanes is also observed. Lastly, the impact of Brtot on LS O3 is assessed.
David Meyer, Thomas Nagler, and Robin J. Hogan
Geosci. Model Dev., 14, 5205–5215, https://doi.org/10.5194/gmd-14-5205-2021, https://doi.org/10.5194/gmd-14-5205-2021, 2021
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A major limitation in training machine-learning emulators is often caused by the lack of data. This paper presents a cheap way to increase the size of training datasets using statistical techniques and thereby improve the performance of machine-learning emulators.
Christian Zeman, Nils P. Wedi, Peter D. Dueben, Nikolina Ban, and Christoph Schär
Geosci. Model Dev., 14, 4617–4639, https://doi.org/10.5194/gmd-14-4617-2021, https://doi.org/10.5194/gmd-14-4617-2021, 2021
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Kilometer-scale atmospheric models allow us to partially resolve thunderstorms and thus improve their representation. We present an intercomparison between two distinct atmospheric models for 2 summer days with heavy thunderstorms over Europe. We show the dependence of precipitation and vertical wind speed on spatial and temporal resolution and also discuss the possible influence of the system of equations, numerical methods, and diffusion in the models.
Chris Wilson, Martyn P. Chipperfield, Manuel Gloor, Robert J. Parker, Hartmut Boesch, Joey McNorton, Luciana V. Gatti, John B. Miller, Luana S. Basso, and Sarah A. Monks
Atmos. Chem. Phys., 21, 10643–10669, https://doi.org/10.5194/acp-21-10643-2021, https://doi.org/10.5194/acp-21-10643-2021, 2021
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Methane (CH4) is an important greenhouse gas emitted from wetlands like those found in the basin of the Amazon River. Using an atmospheric model and observations from GOSAT, we quantified CH4 emissions from Amazonia during the previous decade. We found that the largest emissions came from a region in the eastern basin and that emissions there were rising faster than in other areas of South America. This finding was supported by CH4 observations made on aircraft within the basin.
Thomas von Clarmann, Udo Grabowski, Gabriele P. Stiller, Beatriz M. Monge-Sanz, Norbert Glatthor, and Sylvia Kellmann
Atmos. Chem. Phys., 21, 8823–8843, https://doi.org/10.5194/acp-21-8823-2021, https://doi.org/10.5194/acp-21-8823-2021, 2021
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Measurements of long-lived trace gases (SF6, CFC-11, CFC-12, HCFC-12, CCl4, N2O, CH4, H2O, and CO) performed with the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) have been used to infer the stratospheric and mesospheric meridional circulation. The MIPAS data set covers the time period from July 2002 to April 2012. The method used for this purpose was the direct inversion of the two-dimensional continuity equation. Multiannual monthly mean circulation fields are presented.
Sarah Sparrow, Andrew Bowery, Glenn D. Carver, Marcus O. Köhler, Pirkka Ollinaho, Florian Pappenberger, David Wallom, and Antje Weisheimer
Geosci. Model Dev., 14, 3473–3486, https://doi.org/10.5194/gmd-14-3473-2021, https://doi.org/10.5194/gmd-14-3473-2021, 2021
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This paper describes how the research version of the European Centre for Medium-Range Weather Forecasts’ Integrated Forecast System is combined with climateprediction.net’s public volunteer computing resource to develop OpenIFS@home. Thousands of volunteer personal computers simulated slightly different realizations of Tropical Cyclone Karl to demonstrate the performance of the large-ensemble forecast. OpenIFS@Home offers researchers a new tool to study weather forecasts and related questions.
Jérôme Barré, Hervé Petetin, Augustin Colette, Marc Guevara, Vincent-Henri Peuch, Laurence Rouil, Richard Engelen, Antje Inness, Johannes Flemming, Carlos Pérez García-Pando, Dene Bowdalo, Frederik Meleux, Camilla Geels, Jesper H. Christensen, Michael Gauss, Anna Benedictow, Svetlana Tsyro, Elmar Friese, Joanna Struzewska, Jacek W. Kaminski, John Douros, Renske Timmermans, Lennart Robertson, Mario Adani, Oriol Jorba, Mathieu Joly, and Rostislav Kouznetsov
Atmos. Chem. Phys., 21, 7373–7394, https://doi.org/10.5194/acp-21-7373-2021, https://doi.org/10.5194/acp-21-7373-2021, 2021
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This study provides a comprehensive assessment of air quality changes across the main European urban areas induced by the COVID-19 lockdown using satellite observations, surface site measurements, and the forecasting system from the Copernicus Atmospheric Monitoring Service (CAMS). We demonstrate the importance of accounting for weather and seasonal variability when calculating such estimates.
Graeme Marlton, Andrew Charlton-Perez, Giles Harrison, Inna Polichtchouk, Alain Hauchecorne, Philippe Keckhut, Robin Wing, Thierry Leblanc, and Wolfgang Steinbrecht
Atmos. Chem. Phys., 21, 6079–6092, https://doi.org/10.5194/acp-21-6079-2021, https://doi.org/10.5194/acp-21-6079-2021, 2021
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A network of Rayleigh lidars have been used to infer the upper-stratosphere temperature bias in ECMWF ERA-5 and ERA-Interim reanalyses during 1990–2017. Results show that ERA-Interim exhibits a cold bias of −3 to −4 K between 10 and 1 hPa. Comparisons with ERA-5 found a smaller bias of 1 K which varies between cold and warm between 10 and 3 hPa, indicating a good thermal representation of the atmosphere to 3 hPa. These biases must be accounted for in stratospheric studies using these reanalyses.
Akash Biswal, Vikas Singh, Shweta Singh, Amit P. Kesarkar, Khaiwal Ravindra, Ranjeet S. Sokhi, Martyn P. Chipperfield, Sandip S. Dhomse, Richard J. Pope, Tanbir Singh, and Suman Mor
Atmos. Chem. Phys., 21, 5235–5251, https://doi.org/10.5194/acp-21-5235-2021, https://doi.org/10.5194/acp-21-5235-2021, 2021
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Satellite and surface observations show a reduction in NO2 levels over India during the lockdown compared to business-as-usual years. A substantial reduction, proportional to the population, was observed over the urban areas. The changes in NO2 levels at the surface during the lockdown appear to be present in the satellite observations. However, TROPOMI showed a better correlation with surface NO2 and was more sensitive to the changes than OMI because of the finer resolution.
Jun-Ichi Yano and Nils P. Wedi
Atmos. Chem. Phys., 21, 4759–4778, https://doi.org/10.5194/acp-21-4759-2021, https://doi.org/10.5194/acp-21-4759-2021, 2021
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Sensitivities of forecasts of the Madden–Julian oscillation (MJO) to various different configurations of the physics are examined with the global model of ECMWF's Integrated Forecasting System (IFS). The motivation for the study was to simulate the MJO as a nonlinear free wave. To emulate free dynamics in the IFS,
various momentum dissipation terms (
friction) as well as diabatic heating were selectively turned off over the tropics for the range of the latitudes from 20° S to 20° N.
Oscar Dimdore-Miles, Lesley Gray, and Scott Osprey
Weather Clim. Dynam., 2, 205–231, https://doi.org/10.5194/wcd-2-205-2021, https://doi.org/10.5194/wcd-2-205-2021, 2021
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Observations of the stratosphere span roughly half a century, preventing analysis of multi-decadal variability in circulation using these data. Instead, we rely on long simulations of climate models. Here, we use a model to examine variations in northern polar stratospheric winds and find they vary with a period of around 90 years. We show that this is possibly due to variations in the size of winds over the Equator. This result may improve understanding of Equator–polar stratospheric coupling.
Linda van Garderen, Frauke Feser, and Theodore G. Shepherd
Nat. Hazards Earth Syst. Sci., 21, 171–186, https://doi.org/10.5194/nhess-21-171-2021, https://doi.org/10.5194/nhess-21-171-2021, 2021
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The storyline method is used to quantify the effect of climate change on a particular extreme weather event using a global atmospheric model by simulating the event with and without climate change. We present the method and its successful application for the climate change signals of the European 2003 and the Russian 2010 heatwaves.
Robin J. Hogan and Marco Matricardi
Geosci. Model Dev., 13, 6501–6521, https://doi.org/10.5194/gmd-13-6501-2020, https://doi.org/10.5194/gmd-13-6501-2020, 2020
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A key component of computer models used to predict weather and climate is the radiation scheme, which calculates how solar and infrared radiation heats and cools the atmosphere and surface, including the important role of greenhouse gases. This paper describes the experimental protocol and large datasets for a new project, CKDMIP, to evaluate and improve the accuracy of the treatment of atmospheric gases in the radiation schemes used worldwide, as well as their computational speed.
Wolfgang Woiwode, Andreas Dörnbrack, Inna Polichtchouk, Sören Johansson, Ben Harvey, Michael Höpfner, Jörn Ungermann, and Felix Friedl-Vallon
Atmos. Chem. Phys., 20, 15379–15387, https://doi.org/10.5194/acp-20-15379-2020, https://doi.org/10.5194/acp-20-15379-2020, 2020
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The lowermost-stratosphere moist bias in ECMWF analyses and 12 h forecasts is diagnosed for the Arctic winter-spring 2016 period by using two-dimensional GLORIA water vapor observations. The bias is already present in the initial conditions (i.e., the analyses), and sensitivity forecasts on time scales of < 12 h show hardly any sensitivity to modified spatial resolution and output frequency.
Robert J. Parker, Chris Wilson, A. Anthony Bloom, Edward Comyn-Platt, Garry Hayman, Joe McNorton, Hartmut Boesch, and Martyn P. Chipperfield
Biogeosciences, 17, 5669–5691, https://doi.org/10.5194/bg-17-5669-2020, https://doi.org/10.5194/bg-17-5669-2020, 2020
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Wetlands contribute the largest uncertainty to the atmospheric methane budget. WetCHARTs is a simple, data-driven model that estimates wetland emissions using observations of precipitation and temperature. We perform the first detailed evaluation of WetCHARTs against satellite data and find it performs well in reproducing the observed wetland methane seasonal cycle for the majority of wetland regions. In regions where it performs poorly, we highlight incorrect wetland extent as a key reason.
Marlene Kretschmer, Giuseppe Zappa, and Theodore G. Shepherd
Weather Clim. Dynam., 1, 715–730, https://doi.org/10.5194/wcd-1-715-2020, https://doi.org/10.5194/wcd-1-715-2020, 2020
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The winds in the polar stratosphere affect the weather in the mid-latitudes, making it important to understand potential changes in response to global warming. However, climate model projections disagree on how this so-called polar vortex will change in the future. Here we show that sea ice loss in the Barents and Kara (BK) seas plays a central role in this. The time when the BK seas become ice-free differs between models, which explains some of the disagreement regarding vortex projections.
Christopher H. O'Reilly, Daniel J. Befort, and Antje Weisheimer
Earth Syst. Dynam., 11, 1033–1049, https://doi.org/10.5194/esd-11-1033-2020, https://doi.org/10.5194/esd-11-1033-2020, 2020
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This study examines how the output of large single-model ensembles can be calibrated using observational data to provide improved future projections over Europe. Using an out-of-sample
imperfect modeltest, in which calibration techniques are applied to individual climate model realisations, these techniques are shown to generally improve the reliability of European climate projections for the next 40 years, particularly for regional surface temperature.
Sandip S. Dhomse, Graham W. Mann, Juan Carlos Antuña Marrero, Sarah E. Shallcross, Martyn P. Chipperfield, Kenneth S. Carslaw, Lauren Marshall, N. Luke Abraham, and Colin E. Johnson
Atmos. Chem. Phys., 20, 13627–13654, https://doi.org/10.5194/acp-20-13627-2020, https://doi.org/10.5194/acp-20-13627-2020, 2020
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We confirm downward adjustment of SO2 emission to simulate the Pinatubo aerosol cloud with aerosol microphysics models. Similar adjustment is also needed to simulate the El Chichón and Agung volcanic cloud, indicating potential missing removal or vertical redistribution process in models. Important inhomogeneities in the CMIP6 forcing datasets after Agung and El Chichón eruptions are difficult to reconcile. Quasi-biennial oscillation plays an important role in modifying stratospheric warming.
Dimitris Akritidis, Eleni Katragkou, Aristeidis K. Georgoulias, Prodromos Zanis, Stergios Kartsios, Johannes Flemming, Antje Inness, John Douros, and Henk Eskes
Atmos. Chem. Phys., 20, 13557–13578, https://doi.org/10.5194/acp-20-13557-2020, https://doi.org/10.5194/acp-20-13557-2020, 2020
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We assess the Copernicus Atmosphere Monitoring Service (CAMS) global and regional forecasts performance during a complex aerosol transport event over Europe induced by the passage of Storm Ophelia in mid-October 2017. Comparison with satellite observations reveals a satisfactory performance of CAMS global forecast assisted by data assimilation, while comparison with ground-based measurements indicates that the CAMS regional system over-performs compared to the global one in terms of air quality.
Benjamin Birner, Martyn P. Chipperfield, Eric J. Morgan, Britton B. Stephens, Marianna Linz, Wuhu Feng, Chris Wilson, Jonathan D. Bent, Steven C. Wofsy, Jeffrey Severinghaus, and Ralph F. Keeling
Atmos. Chem. Phys., 20, 12391–12408, https://doi.org/10.5194/acp-20-12391-2020, https://doi.org/10.5194/acp-20-12391-2020, 2020
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With new high-precision observations from nine aircraft campaigns and 3-D chemical transport modeling, we show that the argon-to-nitrogen ratio (Ar / N2) in the lowermost stratosphere provides a useful constraint on the “age of air” (the time elapsed since entry of an air parcel into the stratosphere). Therefore, Ar / N2 in combination with traditional age-of-air indicators, such as CO2 and N2O, could provide new insights into atmospheric mixing and transport.
Matthew J. Rowlinson, Alexandru Rap, Douglas S. Hamilton, Richard J. Pope, Stijn Hantson, Steve R. Arnold, Jed O. Kaplan, Almut Arneth, Martyn P. Chipperfield, Piers M. Forster, and Lars Nieradzik
Atmos. Chem. Phys., 20, 10937–10951, https://doi.org/10.5194/acp-20-10937-2020, https://doi.org/10.5194/acp-20-10937-2020, 2020
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Tropospheric ozone is an important greenhouse gas which contributes to anthropogenic climate change; however, the effect of human emissions is uncertain because pre-industrial ozone concentrations are not well understood. We use revised inventories of pre-industrial natural emissions to estimate the human contribution to changes in tropospheric ozone. We find that tropospheric ozone radiative forcing is up to 34 % lower when using improved pre-industrial biomass burning and vegetation emissions.
Cited articles
Badia, A., Jorba, O., Voulgarakis, A., Dabdub, D., Pérez García-Pando, C., Hilboll, A., Gonçalves, M., and Janjic, Z.: Description and evaluation of the Multiscale Online Nonhydrostatic AtmospheRe CHemistry model (NMMB-MONARCH) version 1.0: gas-phase chemistry at global scale, Geosci. Model Dev., 10, 609–638, https://doi.org/10.5194/gmd-10-609-2017, 2017. a, b
Baldwin, M. P. and Dunkerton, T. J.: Stratospheric Harbingers of Anomalous
Weather Regimes, Science, 294, 581–584, https://doi.org/10.1126/science.1063315, 2001. a
Buehler, T., Raible, C. C., and Stocker, T. F.: The relationship of winter
season North Atlantic blocking frequencies to extreme cold or dry spells in
the ERA-40, Tellus A, 63, 174–187, https://doi.org/10.1111/j.1600-0870.2010.00492.x, 2011. a
Butler, A. H., Sjoberg, J. P., Seidel, D. J., and Rosenlof, K. H.: A sudden stratospheric warming compendium, Earth Syst. Sci. Data, 9, 63–76, https://doi.org/10.5194/essd-9-63-2017, 2017. a
Byrne, N. J. and Shepherd, T. G.: Seasonal Persistence of Circulation Anomalies
in the Southern Hemisphere Stratosphere and Its Implications for the
Troposphere, J. Climate, 31, 3467–3483,
https://doi.org/10.1175/JCLI-D-17-0557.1, 2018. a
Cariolle, D. and Déqué, M.: Southern Hemisphere Medium-Scale Waves and
Total Ozone Disturbances in a Spectral General Circulation Model, J. Geophys. Res., 91, 10825–10846, 1986. a
Cariolle, D. and Teyssèdre, H.: A revised linear ozone photochemistry parameterization for use in transport and general circulation models: multi-annual simulations, Atmos. Chem. Phys., 7, 2183–2196, https://doi.org/10.5194/acp-7-2183-2007, 2007. a, b, c
Cattiaux, J., Vautard, R., Cassou, C., Yiou, P., Masson-Delmotte, V., and
Codron, F.: Winter 2010 in Europe: A cold extreme in a warming climate,
Geophys. Res. Lett., 37, L20704, https://doi.org/10.1029/2010GL044613, 2010. a
Dee, D. P., Uppala, S. M., Simmons, A. J., Berrisford, P., Poli, P., Kobayashi,
S., Andrae, U., Balmaseda, M. A., Balsamo, G., Bauer, P., Bechtold, P.,
Beljaars, A. C. M., van de Berg, L., Bidlot, J., Bormann, N., Delsol, C.,
Dragani, R., Fuentes, M., Geer, A. J., Haimberger, L., Healy, S., Hersbach,
H., Hólm, E. V., Isaksen, L., Kållberg, P., Köhler, M.,
Matricardi, M., McNally, A. P., Monge-Sanz, B. M., Morcrette, J.-J., Peubey,
C., de Rosnay, P., Tavolato, C., Thépaut, J.-N., and Vitart, F.: The
ERA-Interim reanalysis: Configuration and performance of the data
assimilation system, Q. J. Roy. Meteor. Soc., 137, 553–597,
https://doi.org/10.1002/qj.828, 2011. a, b
Diamantakis, M.: Improving ECMWF forecasts of sudden stratospheric warmings,
ECMWF Newsletter, 141, 30–36, https://doi.org/10.21957/pq2zizgf, 2014. a, b
ECMWF: Archive Catalogue, ECMWF Reanalysis data, ECMWF [data set], https://apps.ecmwf.int/archive-catalogue/ (last access: 12 January 2021), 2022.
Eyring, V., Waugh, D. W., Bodeker, G. E., Cordero, E., Akiyoshi, H., Austin,
J., Beagley, S. R., Boville, B. A., Braesicke, P., Brühl, C., Butchart,
N., Chipperfield, M. P., Dameris, M., Deckert, R., Deushi, M., Frith, S. M.,
Garcia, R. R., Gettelman, A., Giorgetta, M. A., Kinnison, D. E., Mancini, E.,
Manzini, E., Marsh, D. R., Matthes, S., Nagashima, T., Newman, P. A.,
Nielsen, J. E., Pawson, S., Pitari, G., Plummer, D. A., Rozanov, E.,
Schraner, M., Scinocca, J. F., Semeniuk, K., Shepherd, T. G., Shibata, K.,
Steil, B., Stolarski, R. S., Tian, W., and Yoshiki, M.: Multimodel
projections of stratospheric ozone in the 21st century, J. Geophys. Res.,
112, D16303, https://doi.org/10.1029/2006JD008332, 2007. a
Flemming, J., Benedetti, A., Inness, A., Engelen, R. J., Jones, L., Huijnen, V., Remy, S., Parrington, M., Suttie, M., Bozzo, A., Peuch, V.-H., Akritidis, D., and Katragkou, E.: The CAMS interim Reanalysis of Carbon Monoxide, Ozone and Aerosol for 2003–2015, Atmos. Chem. Phys., 17, 1945–1983, https://doi.org/10.5194/acp-17-1945-2017, 2017. a, b, c
Fujiwara, M., Wright, J. S., Manney, G. L., Gray, L. J., Anstey, J., Birner, T., Davis, S., Gerber, E. P., Harvey, V. L., Hegglin, M. I., Homeyer, C. R., Knox, J. A., Krüger, K., Lambert, A., Long, C. S., Martineau, P., Molod, A., Monge-Sanz, B. M., Santee, M. L., Tegtmeier, S., Chabrillat, S., Tan, D. G. H., Jackson, D. R., Polavarapu, S., Compo, G. P., Dragani, R., Ebisuzaki, W., Harada, Y., Kobayashi, C., McCarty, W., Onogi, K., Pawson, S., Simmons, A., Wargan, K., Whitaker, J. S., and Zou, C.-Z.: Introduction to the SPARC Reanalysis Intercomparison Project (S-RIP) and overview of the reanalysis systems, Atmos. Chem. Phys., 17, 1417–1452, https://doi.org/10.5194/acp-17-1417-2017, 2017. a
Haase, S., Fricke, J., Kruschke, T., Wahl, S., and Matthes, K.: Sensitivity of the Southern Hemisphere circumpolar jet response to Antarctic ozone depletion: prescribed versus interactive chemistry, Atmos. Chem. Phys., 20, 14043–14061, https://doi.org/10.5194/acp-20-14043-2020, 2020. a
Hanson, D. and Mauersberger, K.: Laboratory studies of the nitric acid
trihydrate: Implications for the South Polar stratosphere, Geophys. Res.
Lett., 15, 855–858, 1988. a
Harris, N. R. P., Carpenter, L. J., Lee, J. D., Vaughan, G., Filus, M. T.,
Jones, R. L., OuYang, B., Pyle, J. A., Robinson, A. D., Andrews, S. J.,
Lewis, A. C., Minaeian, J., Vaughan, A., Dorsey, J. R., Gallagher, M. W.,
Breton, M. L., Newton, R., Percival, C. J., Ricketts, H. M. A., Bauguitte, S. J. B., Nott, G. J., Wellpott, A., Ashfold, M. J., Flemming, J., Butler, R.,
Palmer, P. I., Kaye, P. H., Stopford, C., Chemel, C., Boesch, H., Humpage,
N., Vick, A., MacKenzie, A. R., Hyde, R., Angelov, P., Meneguz, E., and
Manning, A. J.: Coordinated Airborne Studies in the Tropics (CAST),
B. Am. Meteorol. Soc., 98, 145–162,
https://doi.org/10.1175/BAMS-D-14-00290.1, 2017. a
Hogan, R., Ahlgrimm, M., Balsamo, G., Beljaars, A., Berrisford, P., Bozzo, A.,
Giuseppe, F. D., Forbes, R. M., Haiden, T., Lang, S., Mayer, M.,
Polichtchouk, I., Sandu, I., Vitart, F., and Wedi, N.: Radiation in Numerical
Weather Prediction, European Centre for Medium-Range Weather Forecasts (ECMWF), Reading, U.K., Tech. Mem. No. 816, https://doi.org/10.21957/2bd5dkj8x, 2017. a
Inness, A., Baier, F., Benedetti, A., Bouarar, I., Chabrillat, S., Clark, H., Clerbaux, C., Coheur, P., Engelen, R. J., Errera, Q., Flemming, J., George, M., Granier, C., Hadji-Lazaro, J., Huijnen, V., Hurtmans, D., Jones, L., Kaiser, J. W., Kapsomenakis, J., Lefever, K., Leitão, J., Razinger, M., Richter, A., Schultz, M. G., Simmons, A. J., Suttie, M., Stein, O., Thépaut, J.-N., Thouret, V., Vrekoussis, M., Zerefos, C., and the MACC team: The MACC reanalysis: an 8 yr data set of atmospheric composition, Atmos. Chem. Phys., 13, 4073–4109, https://doi.org/10.5194/acp-13-4073-2013, 2013. a
Jeong, G.-R., Monge-Sanz, B. M., Lee, E.-H., and Ziemke, J. R.: Simulation of
stratospheric ozone in global forecast model using linear photochemistry
parameterization, Asia-Pac. J. Atmos. Sci., 52,
479–494, https://doi.org/10.1007/s13143-016-0032-x, 2016. a, b
Johnson, S. J., Stockdale, T. N., Ferranti, L., Balmaseda, M. A., Molteni, F., Magnusson, L., Tietsche, S., Decremer, D., Weisheimer, A., Balsamo, G., Keeley, S. P. E., Mogensen, K., Zuo, H., and Monge-Sanz, B. M.: SEAS5: the new ECMWF seasonal forecast system, Geosci. Model Dev., 12, 1087–1117, https://doi.org/10.5194/gmd-12-1087-2019, 2019. a, b
Kang, S. M., Polvani, L. M., Fyfe, J. C., and Sigmond, M.: Impact of polar
ozone depletion on subtropical precipitation, Science, 332, 951–954, 2011. a
Knight, J., Andrews, M., Stockdale, T., Monge-Sanz, B., Déqué, M.,
Guérémy, J.-F., Saint-Martin, D., Caian, M., and Orsolini, Y.:
Sensitivity to improvements in stratospheric processes and variations in
solar forcings, SPECS Report Deliverable D43.1, https://www.specs-fp7.eu/sites/default/files/u1/SPECS_D43.1.pdf (last access: 21 February 2022), 2016. a, b
Kolstad, E. W., Breiteig, T., and Scaife, A. A.: The association between
stratospheric weak polar vortex events and cold air outbreaks in the Northern
Hemisphere, Q. J. Roy. Meteor. Soc., 136,
886–893, https://doi.org/10.1002/qj.620, 2010. a, b
Kretschmer, M., Coumou, D., Agel, L., Barlow, M., Tziperman, E., and Cohen, J.:
More-Persistent Weak Stratospheric Polar Vortex States Linked to Cold
Extremes, B. Am. Meteorol. Soc., 99, 49–60,
https://doi.org/10.1175/BAMS-D-16-0259.1, 2018. a
Krüger, K., Naujokat, B., and Labitzke, K.: The Unusual Midwinter Warming in
the Southern Hemisphere Stratosphere 2002: A Comparison to Northern
Hemisphere Phenomena, J. Atmos. Sci., 62, 603–613,
https://doi.org/10.1175/JAS-3316.1, 2005. a
Lehtonen, I. and Karpechko, A. Y.: Observed and modeled tropospheric cold
anomalies associated with sudden stratospheric warmings, J.
Geophys. Res.-Atmos., 121, 1591–1610,
https://doi.org/10.1002/2015JD023860, 2016. a
Manney, G. L. and Lawrence, Z. D.: The major stratospheric final warming in 2016: dispersal of vortex air and termination of Arctic chemical ozone loss, Atmos. Chem. Phys., 16, 15371–15396, https://doi.org/10.5194/acp-16-15371-2016, 2016. a, b
Manney, G. L., Daffer, W. H., Strawbridge, K. B., Walker, K. A., Boone, C. D., Bernath, P. F., Kerzenmacher, T., Schwartz, M. J., Strong, K., Sica, R. J., Krüger, K., Pumphrey, H. C., Lambert, A., Santee, M. L., Livesey, N. J., Remsberg, E. E., Mlynczak, M. G., and Russell III, J. R.: The high Arctic in extreme winters: vortex, temperature, and MLS and ACE-FTS trace gas evolution, Atmos. Chem. Phys., 8, 505–522, https://doi.org/10.5194/acp-8-505-2008, 2008. a
McCormack, J. P., Eckermann, S. D., Siskind, D. E., and McGee, T. J.: CHEM2D-OPP: A new linearized gas-phase ozone photochemistry parameterization for high-altitude NWP and climate models, Atmos. Chem. Phys., 6, 4943–4972, https://doi.org/10.5194/acp-6-4943-2006, 2006. a
McLinden, C. A., Olsen, S. C., Hannegan, B., Wild, O., and Prather, M. J.:
Stratospheric Ozone in 3-D Models: A simple chemistry and the
cross-tropopause flux, J. Geophys. Res., 105, 14635–14665, 2000. a
Monge-Sanz, B. M., Chipperfield, M. P., Cariolle, D., and Feng, W.: Results from a new linear O3 scheme with embedded heterogeneous chemistry compared with the parent full-chemistry 3-D CTM, Atmos. Chem. Phys., 11, 1227–1242, https://doi.org/10.5194/acp-11-1227-2011, 2011. a, b, c, d, e, f, g, h, i, j, k, l, m, n, o, p, q, r
Monge-Sanz, B. M., Chipperfield, M. P., Untch, A., Morcrette, J.-J., Rap, A., and Simmons, A. J.: On the uses of a new linear scheme for stratospheric methane in global models: water source, transport tracer and radiative forcing, Atmos. Chem. Phys., 13, 9641–9660, https://doi.org/10.5194/acp-13-9641-2013, 2013. a, b
Monge-Sanz, B. M., Birner, T., Chabrillat, S., Diallo, M., Haenel, F., Konopka, P., Legras, B., Ploeger, F., Reddmann, T., Stiller, G., Wright, J. S., Abalos, M., Boenisch, H. Davis, S., Garny, H., Hitchcock, P., Miyazaki, K., Roscoe., H., Sato, K., Tao, M. C., and Waugh, D.: Brewer-Dobson Circulation in the
SPARC Reanalyses Intercomparison Project (SRIP), SPARC
Reanalyses Intercomparison Project Report No. 10, chap. 5, https://www.sparc-climate.org/wp-content/uploads/sites/5/2022/01/05_S-RIP_Report_Ch05.pdf (last access: 12 March 2022), 2021. a
Morgenstern, O., Hegglin, M. I., Rozanov, E., O'Connor, F. M., Abraham, N. L., Akiyoshi, H., Archibald, A. T., Bekki, S., Butchart, N., Chipperfield, M. P., Deushi, M., Dhomse, S. S., Garcia, R. R., Hardiman, S. C., Horowitz, L. W., Jöckel, P., Josse, B., Kinnison, D., Lin, M., Mancini, E., Manyin, M. E., Marchand, M., Marécal, V., Michou, M., Oman, L. D., Pitari, G., Plummer, D. A., Revell, L. E., Saint-Martin, D., Schofield, R., Stenke, A., Stone, K., Sudo, K., Tanaka, T. Y., Tilmes, S., Yamashita, Y., Yoshida, K., and Zeng, G.: Review of the global models used within phase 1 of the Chemistry–Climate Model Initiative (CCMI), Geosci. Model Dev., 10, 639–671, https://doi.org/10.5194/gmd-10-639-2017, 2017. a
Nakajima, H., Wohltmann, I., Wegner, T., Takeda, M., Pitts, M. C., Poole, L. R., Lehmann, R., Santee, M. L., and Rex, M.: Polar stratospheric cloud evolution and chlorine activation measured by CALIPSO and MLS, and modeled by ATLAS, Atmos. Chem. Phys., 16, 3311–3325, https://doi.org/10.5194/acp-16-3311-2016, 2016. a
Orr, A., Bracegirdle, T. J., Hosking, J. S., Jung, T., Haigh, J. D., Phillips,
T., and Feng, W.: Possible Dynamical Mechanisms for Southern Hemisphere
Climate Change due to the Ozone Hole, J. Atmos. Sci.,
69, 2917–2932, https://doi.org/10.1175/JAS-D-11-0210.1, 2012. a
Polvani, L. M., Waugh, D. W., Correa, G. J. P., and Son, S.-W.: Stratospheric
Ozone Depletion: The Main Driver of Twentieth-Century Atmospheric Circulation
Changes in the Southern Hemisphere, J. Climate, 24, 795–812,
https://doi.org/10.1175/2010JCLI3772.1, 2011. a
Roscoe, H. K., Shanklin, J. D., and Colwell, S. R.: Has the Antarctic Vortex
Split before 2002?, J. Atmos. Sci., 62, 581–588,
https://doi.org/10.1175/JAS-3331.1,
2005. a
Scaife, A. A., Arribas, A., Blockley, E., Brookshaw, A., Clark, R. T.,
Dunstone, N., Eade, R., Fereday, D., Folland, C. K., Gordon, M., Hermanson,
L., Knight, J. R., Lea, D. J., MacLachlan, C., Maidens, A., Martin, M.,
Peterson, A. K., Smith, D., Vellinga, M., Wallace, E., Waters, J., and
Williams, A.: Skillful long-range prediction of European and North American
winters, Geophys. Res. Lett., 41, 2514–2519,
https://doi.org/10.1002/2014GL059637, 2014. a
Scaife, A. A., Karpechko, A. Y., Baldwin, M. P., Brookshaw, A., Butler, A. H.,
Eade, R., Gordon, M., MacLachlan, C., Martin, N., Dunstone, N., and Smith,
D.: Seasonal winter forecasts and the stratosphere, Atmos. Sci. Lett., 17, 51–56, https://doi.org/10.1002/asl.598, 2016. a
Schulz, A., Rex, M., Harris, N. R. P., Braathen, G. O., Reimer, E., Alfier, R.,
Kilbane-Dawe, I., Eckermann, S., Allaart, M., Alpers, M., Bojkov, B.,
Cisneros, J., Claude, H., Cuevas, E., Davies, J., De Backer, H., Dier, H.,
Dorokhov, V., Fast, H., Godin, S., Johnson, B., Kois, B., Kondo, Y.,
Kosmidis, E., Kyrö, E., Litynska, Z., Mikkelsen, I. S., Molyneux, M. J.,
Murphy, G., Nagai, T., Nakane, H., O'Connor, F., Parrondo, C., Schmidlin,
F. J., Skrivankova, P., Varotsos, C., Vialle, C., Viatte, P., Yushkov, V.,
Zerefos, C., and von der Gathen, P.: Arctic ozone loss in threshold
conditions: Match observations in 1997/1998 and 1998/1999, J. Geophys. Res.-Atmos., 106, 7495–7503, https://doi.org/10.1029/2000JD900653, 2001. a
Searle, K. R., Chipperfield, M. P., Bekki, S., and Pyle, J. A.: The impact of
spatial averaging on calculated polar ozone loss 2. Theoretical analysis,
J. Geophys. Res., 103, 25409–25416, 1998. a
Solomon, S., Haskins, J., Ivy, D. J., and Min, F.: Fundamental differences
between Arctic and Antarctic ozone depletion, P. Natl. Acad. Sci. USA,
111, 6220–6225, https://doi.org/10.1073/pnas.1319307111, 2014. a
Son, S.-W., Polvani, L., Waugh, D., Akiyoshi, H., Garcia, R., Kinnison, D.,
Pawson, S., Rozanov, E., Shepherd, T., and Shibata, K.: The impact of
stratospheric ozone recovery in the Southern Hemisphere westerly jet,
Science, 320, 1486–1489, 2008. a
Strahan, S. E., Douglass, A. R., and Steenrod, S. D.: Chemical and dynamical
impacts of stratospheric sudden warmings on Arctic ozone variability, J. Geophys. Res.-Atmos., 121, 11836–11851,
https://doi.org/10.1002/2016JD025128, 2016. a, b
Thompson, A. M., Witte, J. C., Sterling, C., Jordan, A., Johnson, B. J.,
Oltmans, S. J., Fujiwara, M., Vömel, H., Allaart, M., Piters, A., Coetzee,
G. J. R., Posny, F., Corrales, E., Diaz, J. A., Félix, C., Komala, N., Lai,
N., Ahn Nguyen, H. T., Maata, M., Mani, F., Zainal, Z., Ogino, S.-Y.,
Paredes, F., Penha, T. L. B., da Silva, F. R., Sallons-Mitro, S., Selkirk,
H. B., Schmidlin, F. J., Stübi, R., and Thiongo, K.: First Reprocessing of
Southern Hemisphere Additional Ozonesondes (SHADOZ) Ozone Profiles
(1998–2016): 2. Comparisons With Satellites and Ground-Based Instruments,
J. Geophys. Res.-Atmos., 122, 13000–13025, https://doi.org/10.1002/2017JD027406,
2017. a
Tritscher, I., Pitts, M. C., Poole, L. R., Alexander, S. P., Cairo, F.,
Chipperfield, M. P., Grooß, J.-U., Höpfner, M., Lambert, A., Luo, B.,
Molleker, S., Orr, A., Salawitch, R., Snels, M., Spang, R., Woiwode, W., and
Peter, T.: Polar Stratospheric Clouds: Satellite Observations, Processes, and
Role in Ozone Depletion, Rev. Geophys., 59, e2020RG000702,
https://doi.org/10.1029/2020RG000702, 2021. a, b
Waugh, D. W., Sobel, A. H., and Polvani, L. M.: What Is the Polar Vortex and
How Does It Influence Weather?, B. Am. Meteorol.
Soc., 98, 37–44, https://doi.org/10.1175/BAMS-D-15-00212.1, 2017. a
Short summary
The stratosphere is emerging as one of the keys to improve tropospheric weather and climate predictions. This study provides evidence of the role the stratospheric ozone layer plays in improving weather predictions at different timescales. Using a new ozone modelling approach suitable for high-resolution global models that provide operational forecasts from days to seasons, we find significant improvements in stratospheric meteorological fields and stratosphere–troposphere coupling.
The stratosphere is emerging as one of the keys to improve tropospheric weather and climate...
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