Articles | Volume 21, issue 8
https://doi.org/10.5194/acp-21-6509-2021
https://doi.org/10.5194/acp-21-6509-2021
Research article
 | 
30 Apr 2021
Research article |  | 30 Apr 2021

Chemical composition and source attribution of sub-micrometre aerosol particles in the summertime Arctic lower troposphere

Franziska Köllner, Johannes Schneider, Megan D. Willis, Hannes Schulz, Daniel Kunkel, Heiko Bozem, Peter Hoor, Thomas Klimach, Frank Helleis, Julia Burkart, W. Richard Leaitch, Amir A. Aliabadi, Jonathan P. D. Abbatt, Andreas B. Herber, and Stephan Borrmann

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Cited articles

Abbatt, J., Broekhuizen, K., and Pradeep Kumar, P.: Cloud condensation nucleus activity of internally mixed ammonium sulfate/organic acid aerosol particles, Atmos. Environ., 39, 4767–4778, https://doi.org/10.1016/j.atmosenv.2005.04.029, 2005. a
Abbatt, J. P. D., Leaitch, W. R., Aliabadi, A. A., Bertram, A. K., Blanchet, J.-P., Boivin-Rioux, A., Bozem, H., Burkart, J., Chang, R. Y. W., Charette, J., Chaubey, J. P., Christensen, R. J., Cirisan, A., Collins, D. B., Croft, B., Dionne, J., Evans, G. J., Fletcher, C. G., Galí, M., Ghahremaninezhad, R., Girard, E., Gong, W., Gosselin, M., Gourdal, M., Hanna, S. J., Hayashida, H., Herber, A. B., Hesaraki, S., Hoor, P., Huang, L., Hussherr, R., Irish, V. E., Keita, S. A., Kodros, J. K., Köllner, F., Kolonjari, F., Kunkel, D., Ladino, L. A., Law, K., Levasseur, M., Libois, Q., Liggio, J., Lizotte, M., Macdonald, K. M., Mahmood, R., Martin, R. V., Mason, R. H., Miller, L. A., Moravek, A., Mortenson, E., Mungall, E. L., Murphy, J. G., Namazi, M., Norman, A.-L., O'Neill, N. T., Pierce, J. R., Russell, L. M., Schneider, J., Schulz, H., Sharma, S., Si, M., Staebler, R. M., Steiner, N. S., Thomas, J. L., von Salzen, K., Wentzell, J. J. B., Willis, M. D., Wentworth, G. R., Xu, J.-W., and Yakobi-Hancock, J. D.: Overview paper: New insights into aerosol and climate in the Arctic, Atmos. Chem. Phys., 19, 2527–2560, https://doi.org/10.5194/acp-19-2527-2019, 2019. a, b
Abbatt, J. P. D., Liu, M., Aliabadi, A. A., Herber, A. B., Schulz, H., Willis, M. D., Leaitch, W. R., Schneider, J., Köllner, F., Bozem, H., Hoor, P., Staebler, R., and Norman, A.-L.: Data from the NETCARE POLAR6 2014 campaign, Environment and Climate Change Canada, available at: https://crd-data-donnees-rdc.ec.gc.ca/CCCMA/products/NETCARE/NETCARE%202014%20POLAR6%20aircraft%20campaign-%20Campagne%20a%c3%a9rienne%20POLAR6%20de%202014%20/, last access: 30 April 2021. a
Acosta Navarro, J. C., Varma, V., Riipinen, I., Seland, Ø., Kirkevåg, A., Struthers, H., Iversen, T., Hansson, H.-C., and Ekman, A. M. L.: Amplification of Arctic warming by past air pollution reductions in Europe, Nat. Geosci., 9, 277–281, https://doi.org/10.1038/ngeo2673, 2016. a
Aliabadi, A. A., Staebler, R. M., and Sharma, S.: Air quality monitoring in communities of the Canadian Arctic during the high shipping season with a focus on local and marine pollution, Atmos. Chem. Phys., 15, 2651–2673, https://doi.org/10.5194/acp-15-2651-2015, 2015. a
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We present in situ observations of vertically resolved particle chemical composition in the summertime Arctic lower troposphere. Our analysis demonstrates the strong vertical contrast between particle properties within the boundary layer and aloft. Emissions from vegetation fires and anthropogenic sources in northern Canada, Europe, and East Asia influenced particle composition in the free troposphere. Organics detected in Arctic aerosol particles can partly be identified as dicarboxylic acids.
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