Articles | Volume 20, issue 18
https://doi.org/10.5194/acp-20-10845-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-10845-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
18 Sep 2020
Research article |
| 18 Sep 2020
| 18 Sep 2020
Aerosol solar radiative forcing near the Taklimakan Desert based on radiative transfer and regional meteorological simulations during the Dust Aerosol Observation-Kashi campaign
Li Li
Aerospace Information Research Institute, Chinese Academy of Sciences,
Beijing, China
Zhengqiang Li
CORRESPONDING AUTHOR
Aerospace Information Research Institute, Chinese Academy of Sciences,
Beijing, China
Wenyuan Chang
Institute of Atmospheric Physics, Chinese Academy of Sciences,
Beijing, China
Yang Ou
Aerospace Information Research Institute, Chinese Academy of Sciences,
Beijing, China
Philippe Goloub
Laboratoire d'Optique Atmosphérique, Université de Lille
1/CNRS, Lille, France
Chengzhe Li
Department of Chemical and Biochemical Engineering, University of
Iowa, Iowa City, IA, USA
Kaitao Li
Aerospace Information Research Institute, Chinese Academy of Sciences,
Beijing, China
Qiaoyun Hu
Laboratoire d'Optique Atmosphérique, Université de Lille
1/CNRS, Lille, France
Jianping Wang
Aerospace Information Research Institute, Chinese Academy of Sciences,
Beijing, China
Manfred Wendisch
Leipzig Institute for Meteorology, University of Leipzig, Leipzig, Germany
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Imke Schirmacher, Pavlos Kollias, Katia Lamer, Mario Mech, Lukas Pfitzenmaier, Manfred Wendisch, and Susanne Crewell
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Olivia Linke, Johannes Quaas, Finja Baumer, Sebastian Becker, Jan Chylik, Sandro Dahlke, André Ehrlich, Dörthe Handorf, Christoph Jacobi, Heike Kalesse-Los, Luca Lelli, Sina Mehrdad, Roel A. J. Neggers, Johannes Riebold, Pablo Saavedra Garfias, Niklas Schnierstein, Matthew D. Shupe, Chris Smith, Gunnar Spreen, Baptiste Verneuil, Kameswara S. Vinjamuri, Marco Vountas, and Manfred Wendisch
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Manfred Wendisch, Johannes Stapf, Sebastian Becker, André Ehrlich, Evelyn Jäkel, Marcus Klingebiel, Christof Lüpkes, Michael Schäfer, and Matthew D. Shupe
Atmos. Chem. Phys., 23, 9647–9667, https://doi.org/10.5194/acp-23-9647-2023, https://doi.org/10.5194/acp-23-9647-2023, 2023
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Atmospheric radiation measurements have been conducted during two field campaigns using research aircraft. The data are analyzed to see if the near-surface air in the Arctic is warmed or cooled if warm–humid air masses from the south enter the Arctic or cold–dry air moves from the north from the Arctic to mid-latitude areas. It is important to study these processes and to check if climate models represent them well. Otherwise it is not possible to reliably forecast the future Arctic climate.
Sophie Rosenburg, Charlotte Lange, Evelyn Jäkel, Michael Schäfer, André Ehrlich, and Manfred Wendisch
Atmos. Meas. Tech., 16, 3915–3930, https://doi.org/10.5194/amt-16-3915-2023, https://doi.org/10.5194/amt-16-3915-2023, 2023
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Snow layer melting and melt pond formation on Arctic sea ice are important seasonal processes affecting the surface reflection and energy budget. Sea ice reflectivity was surveyed by airborne imaging spectrometers in May–June 2017. Adapted retrieval approaches were applied to find snow layer liquid water fraction, snow grain effective radius, and melt pond depth. The retrievals show the potential and limitations of spectral airborne imaging to map melting snow layer and melt pond properties.
Manuel Moser, Christiane Voigt, Tina Jurkat-Witschas, Valerian Hahn, Guillaume Mioche, Olivier Jourdan, Régis Dupuy, Christophe Gourbeyre, Alfons Schwarzenboeck, Johannes Lucke, Yvonne Boose, Mario Mech, Stephan Borrmann, André Ehrlich, Andreas Herber, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys., 23, 7257–7280, https://doi.org/10.5194/acp-23-7257-2023, https://doi.org/10.5194/acp-23-7257-2023, 2023
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This study provides a comprehensive microphysical and thermodynamic phase analysis of low-level clouds in the northern Fram Strait, above the sea ice and the open ocean, during spring and summer. Using airborne in situ cloud data, we show that the properties of Arctic low-level clouds vary significantly with seasonal meteorological situations and surface conditions. The observations presented in this study can help one to assess the role of clouds in the Arctic climate system.
Sebastian Becker, André Ehrlich, Michael Schäfer, and Manfred Wendisch
Atmos. Chem. Phys., 23, 7015–7031, https://doi.org/10.5194/acp-23-7015-2023, https://doi.org/10.5194/acp-23-7015-2023, 2023
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Aliki Christodoulou, Iasonas Stavroulas, Mihalis Vrekoussis, Maximillien Desservettaz, Michael Pikridas, Elie Bimenyimana, Jonilda Kushta, Matic Ivančič, Martin Rigler, Philippe Goloub, Konstantina Oikonomou, Roland Sarda-Estève, Chrysanthos Savvides, Charbel Afif, Nikos Mihalopoulos, Stéphane Sauvage, and Jean Sciare
Atmos. Chem. Phys., 23, 6431–6456, https://doi.org/10.5194/acp-23-6431-2023, https://doi.org/10.5194/acp-23-6431-2023, 2023
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Our study presents, for the first time, a detailed source identification of aerosols at an urban background site in Cyprus (eastern Mediterranean), a region strongly impacted by climate change and air pollution. Here, we identify an unexpected high contribution of long-range transported pollution from fossil fuel sources in the Middle East, highlighting an urgent need to further characterize these fast-growing emissions and their impacts on regional atmospheric composition, climate, and health.
Dmitry G. Chechin, Christof Lüpkes, Jörg Hartmann, André Ehrlich, and Manfred Wendisch
Atmos. Chem. Phys., 23, 4685–4707, https://doi.org/10.5194/acp-23-4685-2023, https://doi.org/10.5194/acp-23-4685-2023, 2023
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Clouds represent a very important component of the Arctic climate system, as they strongly reduce the amount of heat lost to space from the sea ice surface. Properties of clouds, as well as their persistence, strongly depend on the complex interaction of such small-scale properties as phase transitions, radiative transfer and turbulence. In this study we use airborne observations to learn more about the effect of clouds and radiative cooling on turbulence in comparison with other factors.
Igor Veselovskii, Nikita Kasianik, Mikhail Korenskii, Qiaoyun Hu, Philippe Goloub, Thierry Podvin, and Dong Liu
Atmos. Meas. Tech., 16, 2055–2065, https://doi.org/10.5194/amt-16-2055-2023, https://doi.org/10.5194/amt-16-2055-2023, 2023
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A five-channel fluorescence lidar was developed for the study of atmospheric aerosol. The fluorescence spectrum induced by 355 nm laser emission is analyzed in five spectral intervals, namely 438 and 29, 472 and 32, 513 and 29, 560 and 40, and 614 and 54 nm. This lidar system was operated during strong forest fires. Our results demonstrate that, for urban aerosol, the maximal fluorescence backscattering is observed at 472 nm, while for smoke, the spectrum is shifted toward longer wavelengths.
Andreas Walbröl, Janosch Michaelis, Sebastian Becker, Henning Dorff, Irina Gorodetskaya, Benjamin Kirbus, Melanie Lauer, Nina Maherndl, Marion Maturilli, Johanna Mayer, Hanno Müller, Roel A. J. Neggers, Fiona M. Paulus, Johannes Röttenbacher, Janna E. Rückert, Imke Schirmacher, Nils Slättberg, André Ehrlich, Manfred Wendisch, and Susanne Crewell
EGUsphere, https://doi.org/10.5194/egusphere-2023-668, https://doi.org/10.5194/egusphere-2023-668, 2023
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We present the weather and sea ice conditions and climatological context of the airborne HALO–(AC)3 campaign, which took place over the North Atlantic sector of the Arctic from 07 March to 12 April 2022. From the ERA5 reanalysis, we identified record breaking warm air intrusions and a large variety of marine cold air outbreaks. Sea ice concentration was mostly within the interquartile range of the climatology. Our study serves as basis for future analyses of the data collected during HALO–(AC)3.
André Ehrlich, Martin Zöger, Andreas Giez, Vladyslav Nenakhov, Christian Mallaun, Rolf Maser, Timo Röschenthaler, Anna E. Luebke, Kevin Wolf, Bjorn Stevens, and Manfred Wendisch
Atmos. Meas. Tech., 16, 1563–1581, https://doi.org/10.5194/amt-16-1563-2023, https://doi.org/10.5194/amt-16-1563-2023, 2023
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Measurements of the broadband radiative energy budget from aircraft are needed to study the effect of clouds, aerosol particles, and surface conditions on the Earth's energy budget. However, the moving aircraft introduces challenges to the instrument performance and post-processing of the data. This study introduces a new radiometer package, outlines a greatly simplifying method to correct thermal offsets, and provides exemplary measurements of solar and thermal–infrared irradiance.
Yunfan Liu, Hang Su, Siwen Wang, Chao Wei, Wei Tao, Mira L. Pöhlker, Christopher Pöhlker, Bruna A. Holanda, Ovid O. Krüger, Thorsten Hoffmann, Manfred Wendisch, Paulo Artaxo, Ulrich Pöschl, Meinrat O. Andreae, and Yafang Cheng
Atmos. Chem. Phys., 23, 251–272, https://doi.org/10.5194/acp-23-251-2023, https://doi.org/10.5194/acp-23-251-2023, 2023
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The origins of the abundant cloud condensation nuclei (CCN) in the upper troposphere (UT) of the Amazon remain unclear. With model developments of new secondary organic aerosol schemes and constrained by observation, we show that strong aerosol nucleation and condensation in the UT is triggered by biogenic organics, and organic condensation is key for UT CCN production. This UT CCN-producing mechanism may prevail over broader vegetation canopies and deserves emphasis in aerosol–climate feedback.
Igor Veselovskii, Qiaoyun Hu, Philippe Goloub, Thierry Podvin, Boris Barchunov, and Mikhail Korenskii
Atmos. Meas. Tech., 15, 4881–4900, https://doi.org/10.5194/amt-15-4881-2022, https://doi.org/10.5194/amt-15-4881-2022, 2022
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An approach to reveal variability in aerosol type at a high spatiotemporal resolution, by combining fluorescence and Mie–Raman lidar data, is presented. We applied this new classification scheme to lidar data obtained by LOA, University of Lille, in 2020–2021. It is demonstrated that the separation of the main particle types, such as smoke, dust, pollen, and urban, can be performed with a height resolution of 60 m and temporal resolution better than 10 min for the current lidar configuration.
Jie Luo, Zhengqiang Li, Chenchong Zhang, Qixing Zhang, Yongming Zhang, Ying Zhang, Gabriele Curci, and Rajan K. Chakrabarty
Atmos. Chem. Phys., 22, 7647–7666, https://doi.org/10.5194/acp-22-7647-2022, https://doi.org/10.5194/acp-22-7647-2022, 2022
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The fractal black carbon was applied to re-evaluate the regional impacts of morphologies on aerosol–radiation interactions (ARIs), and the effects were compared between the US and China. The regional-mean clear-sky ARI is significantly affected by the BC morphology, and relative differences of 17.1 % and 38.7 % between the fractal model with a Df of 1.8 and the spherical model were observed in eastern China and the northwest US, respectively.
Sebastian Becker, André Ehrlich, Evelyn Jäkel, Tim Carlsen, Michael Schäfer, and Manfred Wendisch
Atmos. Meas. Tech., 15, 2939–2953, https://doi.org/10.5194/amt-15-2939-2022, https://doi.org/10.5194/amt-15-2939-2022, 2022
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Airborne radiation measurements are used to characterize the solar directional reflection of a mixture of Arctic sea ice and open-ocean surfaces in the transition zone between both surface types. The mixture reveals reflection properties of both surface types. It is shown that the directional reflection of the mixture can be reconstructed from the directional reflection of the individual surfaces, accounting for the special conditions present in the transition zone.
Jie Luo, Zhengqiang Li, Cheng Fan, Hua Xu, Ying Zhang, Weizhen Hou, Lili Qie, Haoran Gu, Mengyao Zhu, Yinna Li, and Kaitao Li
Atmos. Meas. Tech., 15, 2767–2789, https://doi.org/10.5194/amt-15-2767-2022, https://doi.org/10.5194/amt-15-2767-2022, 2022
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A single model is difficult to represent various shapes of dust. We proposed a tunable model to represent dust with various shapes. Two tunable parameters were used to represent the effects of the erosion degree and binding forces from the mass center. Thus, the model can represent various dust shapes by adjusting the tunable parameters. Besides, the applicability of the spheroid model in calculating the optical properties and polarimetric characteristics is evaluated.
Qiaoyun Hu, Philippe Goloub, Igor Veselovskii, and Thierry Podvin
Atmos. Chem. Phys., 22, 5399–5414, https://doi.org/10.5194/acp-22-5399-2022, https://doi.org/10.5194/acp-22-5399-2022, 2022
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Our lidar observations show that the optical properties of wildfire smoke particles are highly varied after long-range transport. The variabilities are probably relevant to vegetation type, combustion condition and the aging process, which alter the smoke particle properties, as well as their impact on cloud processes and properties. The lidar fluorescence channel provides a good opportunity for smoke characterization and heterogenous ice crystal formation.
Igor Veselovskii, Qiaoyun Hu, Albert Ansmann, Philippe Goloub, Thierry Podvin, and Mikhail Korenskiy
Atmos. Chem. Phys., 22, 5209–5221, https://doi.org/10.5194/acp-22-5209-2022, https://doi.org/10.5194/acp-22-5209-2022, 2022
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A remote sensing method based on fluorescence lidar measurements can detect and quantify the smoke content in the upper troposphere and inside cirrus clouds. Based on two case studies, we demonstrate that the fluorescence lidar technique provides the possibility to estimate the smoke surface area concentration within freshly formed cirrus layers. This value was used in a smoke ice nucleating particle parameterization scheme to predict ice crystal number concentrations in cirrus generation cells.
Michael Schäfer, Kevin Wolf, André Ehrlich, Christoph Hallbauer, Evelyn Jäkel, Friedhelm Jansen, Anna Elizabeth Luebke, Joshua Müller, Jakob Thoböll, Timo Röschenthaler, Bjorn Stevens, and Manfred Wendisch
Atmos. Meas. Tech., 15, 1491–1509, https://doi.org/10.5194/amt-15-1491-2022, https://doi.org/10.5194/amt-15-1491-2022, 2022
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The new airborne thermal infrared imager VELOX is introduced. It measures two-dimensional fields of spectral thermal infrared radiance or brightness temperature within the large atmospheric window. The technical specifications as well as necessary calibration and correction procedures are presented. Example measurements from the first field deployment are analysed with respect to cloud coverage and cloud top altitude.
Anna E. Luebke, André Ehrlich, Michael Schäfer, Kevin Wolf, and Manfred Wendisch
Atmos. Chem. Phys., 22, 2727–2744, https://doi.org/10.5194/acp-22-2727-2022, https://doi.org/10.5194/acp-22-2727-2022, 2022
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A combination of aircraft and satellite observations is used to show how the characteristics of tropical shallow clouds interact with incoming and outgoing energy. A complete depiction of these clouds is challenging to obtain, but such data are useful for understanding how models can correctly represent them. The amount of cloud is found to be the most important factor, while other cloud characteristics become increasingly impactful when more cloud is present.
Kaixu Bai, Ke Li, Mingliang Ma, Kaitao Li, Zhengqiang Li, Jianping Guo, Ni-Bin Chang, Zhuo Tan, and Di Han
Earth Syst. Sci. Data, 14, 907–927, https://doi.org/10.5194/essd-14-907-2022, https://doi.org/10.5194/essd-14-907-2022, 2022
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The Long-term Gap-free High-resolution Air Pollutant concentration dataset, providing gap-free aerosol optical depth (AOD) and PM2.5 and PM10 concentration with a daily 1 km resolution for 2000–2020 in China, is generated and made publicly available. This is the first long-term gap-free high-resolution aerosol dataset in China and has great potential to trigger multidisciplinary applications in Earth observations, climate change, public health, ecosystem assessment, and environment management.
Ramon Campos Braga, Barbara Ervens, Daniel Rosenfeld, Meinrat O. Andreae, Jan-David Förster, Daniel Fütterer, Lianet Hernández Pardo, Bruna A. Holanda, Tina Jurkat-Witschas, Ovid O. Krüger, Oliver Lauer, Luiz A. T. Machado, Christopher Pöhlker, Daniel Sauer, Christiane Voigt, Adrian Walser, Manfred Wendisch, Ulrich Pöschl, and Mira L. Pöhlker
Atmos. Chem. Phys., 21, 17513–17528, https://doi.org/10.5194/acp-21-17513-2021, https://doi.org/10.5194/acp-21-17513-2021, 2021
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Interactions of aerosol particles with clouds represent a large uncertainty in estimates of climate change. Properties of aerosol particles control their ability to act as cloud condensation nuclei. Using aerosol measurements in the Amazon, we performed model studies to compare predicted and measured cloud droplet number concentrations at cloud bases. Our results confirm previous estimates of particle hygroscopicity in this region.
Heike Konow, Florian Ewald, Geet George, Marek Jacob, Marcus Klingebiel, Tobias Kölling, Anna E. Luebke, Theresa Mieslinger, Veronika Pörtge, Jule Radtke, Michael Schäfer, Hauke Schulz, Raphaela Vogel, Martin Wirth, Sandrine Bony, Susanne Crewell, André Ehrlich, Linda Forster, Andreas Giez, Felix Gödde, Silke Groß, Manuel Gutleben, Martin Hagen, Lutz Hirsch, Friedhelm Jansen, Theresa Lang, Bernhard Mayer, Mario Mech, Marc Prange, Sabrina Schnitt, Jessica Vial, Andreas Walbröl, Manfred Wendisch, Kevin Wolf, Tobias Zinner, Martin Zöger, Felix Ament, and Bjorn Stevens
Earth Syst. Sci. Data, 13, 5545–5563, https://doi.org/10.5194/essd-13-5545-2021, https://doi.org/10.5194/essd-13-5545-2021, 2021
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The German research aircraft HALO took part in the research campaign EUREC4A in January and February 2020. The focus area was the tropical Atlantic east of the island of Barbados. We describe the characteristics of the 15 research flights, provide auxiliary information, derive combined cloud mask products from all instruments that observe clouds on board the aircraft, and provide code examples that help new users of the data to get started.
Ramon Campos Braga, Daniel Rosenfeld, Ovid O. Krüger, Barbara Ervens, Bruna A. Holanda, Manfred Wendisch, Trismono Krisna, Ulrich Pöschl, Meinrat O. Andreae, Christiane Voigt, and Mira L. Pöhlker
Atmos. Chem. Phys., 21, 14079–14088, https://doi.org/10.5194/acp-21-14079-2021, https://doi.org/10.5194/acp-21-14079-2021, 2021
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Quantifying the precipitation within clouds is crucial for our understanding of the Earth's hydrological cycle. Using in situ measurements of cloud and rain properties over the Amazon Basin and Atlantic Ocean, we show here a linear relationship between the effective radius (re) and precipitation water content near the tops of convective clouds for different pollution states and temperature levels. Our results emphasize the role of re to determine both initiation and amount of precipitation.
Bjorn Stevens, Sandrine Bony, David Farrell, Felix Ament, Alan Blyth, Christopher Fairall, Johannes Karstensen, Patricia K. Quinn, Sabrina Speich, Claudia Acquistapace, Franziska Aemisegger, Anna Lea Albright, Hugo Bellenger, Eberhard Bodenschatz, Kathy-Ann Caesar, Rebecca Chewitt-Lucas, Gijs de Boer, Julien Delanoë, Leif Denby, Florian Ewald, Benjamin Fildier, Marvin Forde, Geet George, Silke Gross, Martin Hagen, Andrea Hausold, Karen J. Heywood, Lutz Hirsch, Marek Jacob, Friedhelm Jansen, Stefan Kinne, Daniel Klocke, Tobias Kölling, Heike Konow, Marie Lothon, Wiebke Mohr, Ann Kristin Naumann, Louise Nuijens, Léa Olivier, Robert Pincus, Mira Pöhlker, Gilles Reverdin, Gregory Roberts, Sabrina Schnitt, Hauke Schulz, A. Pier Siebesma, Claudia Christine Stephan, Peter Sullivan, Ludovic Touzé-Peiffer, Jessica Vial, Raphaela Vogel, Paquita Zuidema, Nicola Alexander, Lyndon Alves, Sophian Arixi, Hamish Asmath, Gholamhossein Bagheri, Katharina Baier, Adriana Bailey, Dariusz Baranowski, Alexandre Baron, Sébastien Barrau, Paul A. Barrett, Frédéric Batier, Andreas Behrendt, Arne Bendinger, Florent Beucher, Sebastien Bigorre, Edmund Blades, Peter Blossey, Olivier Bock, Steven Böing, Pierre Bosser, Denis Bourras, Pascale Bouruet-Aubertot, Keith Bower, Pierre Branellec, Hubert Branger, Michal Brennek, Alan Brewer, Pierre-Etienne Brilouet, Björn Brügmann, Stefan A. Buehler, Elmo Burke, Ralph Burton, Radiance Calmer, Jean-Christophe Canonici, Xavier Carton, Gregory Cato Jr., Jude Andre Charles, Patrick Chazette, Yanxu Chen, Michal T. Chilinski, Thomas Choularton, Patrick Chuang, Shamal Clarke, Hugh Coe, Céline Cornet, Pierre Coutris, Fleur Couvreux, Susanne Crewell, Timothy Cronin, Zhiqiang Cui, Yannis Cuypers, Alton Daley, Gillian M. Damerell, Thibaut Dauhut, Hartwig Deneke, Jean-Philippe Desbios, Steffen Dörner, Sebastian Donner, Vincent Douet, Kyla Drushka, Marina Dütsch, André Ehrlich, Kerry Emanuel, Alexandros Emmanouilidis, Jean-Claude Etienne, Sheryl Etienne-Leblanc, Ghislain Faure, Graham Feingold, Luca Ferrero, Andreas Fix, Cyrille Flamant, Piotr Jacek Flatau, Gregory R. Foltz, Linda Forster, Iulian Furtuna, Alan Gadian, Joseph Galewsky, Martin Gallagher, Peter Gallimore, Cassandra Gaston, Chelle Gentemann, Nicolas Geyskens, Andreas Giez, John Gollop, Isabelle Gouirand, Christophe Gourbeyre, Dörte de Graaf, Geiske E. de Groot, Robert Grosz, Johannes Güttler, Manuel Gutleben, Kashawn Hall, George Harris, Kevin C. Helfer, Dean Henze, Calvert Herbert, Bruna Holanda, Antonio Ibanez-Landeta, Janet Intrieri, Suneil Iyer, Fabrice Julien, Heike Kalesse, Jan Kazil, Alexander Kellman, Abiel T. Kidane, Ulrike Kirchner, Marcus Klingebiel, Mareike Körner, Leslie Ann Kremper, Jan Kretzschmar, Ovid Krüger, Wojciech Kumala, Armin Kurz, Pierre L'Hégaret, Matthieu Labaste, Tom Lachlan-Cope, Arlene Laing, Peter Landschützer, Theresa Lang, Diego Lange, Ingo Lange, Clément Laplace, Gauke Lavik, Rémi Laxenaire, Caroline Le Bihan, Mason Leandro, Nathalie Lefevre, Marius Lena, Donald Lenschow, Qiang Li, Gary Lloyd, Sebastian Los, Niccolò Losi, Oscar Lovell, Christopher Luneau, Przemyslaw Makuch, Szymon Malinowski, Gaston Manta, Eleni Marinou, Nicholas Marsden, Sebastien Masson, Nicolas Maury, Bernhard Mayer, Margarette Mayers-Als, Christophe Mazel, Wayne McGeary, James C. McWilliams, Mario Mech, Melina Mehlmann, Agostino Niyonkuru Meroni, Theresa Mieslinger, Andreas Minikin, Peter Minnett, Gregor Möller, Yanmichel Morfa Avalos, Caroline Muller, Ionela Musat, Anna Napoli, Almuth Neuberger, Christophe Noisel, David Noone, Freja Nordsiek, Jakub L. Nowak, Lothar Oswald, Douglas J. Parker, Carolyn Peck, Renaud Person, Miriam Philippi, Albert Plueddemann, Christopher Pöhlker, Veronika Pörtge, Ulrich Pöschl, Lawrence Pologne, Michał Posyniak, Marc Prange, Estefanía Quiñones Meléndez, Jule Radtke, Karim Ramage, Jens Reimann, Lionel Renault, Klaus Reus, Ashford Reyes, Joachim Ribbe, Maximilian Ringel, Markus Ritschel, Cesar B. Rocha, Nicolas Rochetin, Johannes Röttenbacher, Callum Rollo, Haley Royer, Pauline Sadoulet, Leo Saffin, Sanola Sandiford, Irina Sandu, Michael Schäfer, Vera Schemann, Imke Schirmacher, Oliver Schlenczek, Jerome Schmidt, Marcel Schröder, Alfons Schwarzenboeck, Andrea Sealy, Christoph J. Senff, Ilya Serikov, Samkeyat Shohan, Elizabeth Siddle, Alexander Smirnov, Florian Späth, Branden Spooner, M. Katharina Stolla, Wojciech Szkółka, Simon P. de Szoeke, Stéphane Tarot, Eleni Tetoni, Elizabeth Thompson, Jim Thomson, Lorenzo Tomassini, Julien Totems, Alma Anna Ubele, Leonie Villiger, Jan von Arx, Thomas Wagner, Andi Walther, Ben Webber, Manfred Wendisch, Shanice Whitehall, Anton Wiltshire, Allison A. Wing, Martin Wirth, Jonathan Wiskandt, Kevin Wolf, Ludwig Worbes, Ethan Wright, Volker Wulfmeyer, Shanea Young, Chidong Zhang, Dongxiao Zhang, Florian Ziemen, Tobias Zinner, and Martin Zöger
Earth Syst. Sci. Data, 13, 4067–4119, https://doi.org/10.5194/essd-13-4067-2021, https://doi.org/10.5194/essd-13-4067-2021, 2021
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The EUREC4A field campaign, designed to test hypothesized mechanisms by which clouds respond to warming and benchmark next-generation Earth-system models, is presented. EUREC4A comprised roughly 5 weeks of measurements in the downstream winter trades of the North Atlantic – eastward and southeastward of Barbados. It was the first campaign that attempted to characterize the full range of processes and scales influencing trade wind clouds.
Igor Veselovskii, Qiaoyun Hu, Philippe Goloub, Thierry Podvin, Marie Choël, Nicolas Visez, and Mikhail Korenskiy
Atmos. Meas. Tech., 14, 4773–4786, https://doi.org/10.5194/amt-14-4773-2021, https://doi.org/10.5194/amt-14-4773-2021, 2021
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The multiwavelength Mie–Raman–fluorescence lidar of the University of Lille was used to characterize aerosols during the pollen season in the north of France for the period March–June 2020. The results of observations demonstrate that the presence of pollen grains in aerosol mixtures leads to an increase in the depolarization ratio and to the enhancement of the fluorescence backscattering.
Cheng Fan, Zhengqiang Li, Ying Li, Jiantao Dong, Ronald van der A, and Gerrit de Leeuw
Atmos. Chem. Phys., 21, 7723–7748, https://doi.org/10.5194/acp-21-7723-2021, https://doi.org/10.5194/acp-21-7723-2021, 2021
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Emission control policy in China has resulted in the decrease of nitrogen dioxide concentrations, which however leveled off and stabilized in recent years, as shown from satellite data. The effects of the further emission reduction during the COVID-19 lockdown in 2020 resulted in an initial improvement of air quality, which, however, was offset by chemical and meteorological effects. The study shows the regional dependence over east China, and results have a wider application than China only.
Ulrike Egerer, André Ehrlich, Matthias Gottschalk, Hannes Griesche, Roel A. J. Neggers, Holger Siebert, and Manfred Wendisch
Atmos. Chem. Phys., 21, 6347–6364, https://doi.org/10.5194/acp-21-6347-2021, https://doi.org/10.5194/acp-21-6347-2021, 2021
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This paper describes a case study of a three-day period with a persistent humidity inversion above a mixed-phase cloud layer in the Arctic. It is based on measurements with a tethered balloon, complemented with results from a dedicated high-resolution large-eddy simulation. Both methods show that the humidity layer acts to provide moisture to the cloud layer through downward turbulent transport. This supply of additional moisture can contribute to the persistence of Arctic clouds.
Johannes Stapf, André Ehrlich, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-279, https://doi.org/10.5194/acp-2021-279, 2021
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Airborne observations of the surface radiative energy budget in the marginal sea ice zone (the region between open ocean and closed sea ice) are presented. Atmospheric thermodynamic profiles and surface properties change on small spatial scales in this area and influence the impact of clouds on the radiative energy budget. The radiation budget over sea ice is compared to available studies in the Arctic and the influence of cold air outbreaks and warm air intrusions is illustrated.
Anton Lopatin, Oleg Dubovik, David Fuertes, Georgiy Stenchikov, Tatyana Lapyonok, Igor Veselovskii, Frank G. Wienhold, Illia Shevchenko, Qiaoyun Hu, and Sagar Parajuli
Atmos. Meas. Tech., 14, 2575–2614, https://doi.org/10.5194/amt-14-2575-2021, https://doi.org/10.5194/amt-14-2575-2021, 2021
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The article presents novelties in characterizing fine particles suspended in the air by means of combining various measurements that observe light propagation in atmosphere. Several non-coincident observations (some of which require sunlight, while others work only at night) could be united under the assumption that aerosol properties do not change drastically at nighttime. It also proposes how to describe particles' composition in a simplified manner that uses new types of observations.
Wenyuan Chang, Ying Zhang, Zhengqiang Li, Jie Chen, and Kaitao Li
Atmos. Chem. Phys., 21, 4403–4430, https://doi.org/10.5194/acp-21-4403-2021, https://doi.org/10.5194/acp-21-4403-2021, 2021
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Aerosol simulation in WRF-Chem often uses the MOSAIC aerosol mechanism. Still, we need variational data assimilation (DA) for the MOSAIC aerosols to blend aerosol optical measurements. This study provides a developed GSI variational DA system, with a tangent linear operator designed for multi-source and multi-wavelength aerosol optical measurements. We successfully applied the DA system in an aerosol field campaign to assimilate aerosol optical data in northwestern China.
Yang Zhang, Zhengqiang Li, Zhihong Liu, Yongqian Wang, Lili Qie, Yisong Xie, Weizhen Hou, and Lu Leng
Atmos. Meas. Tech., 14, 1655–1672, https://doi.org/10.5194/amt-14-1655-2021, https://doi.org/10.5194/amt-14-1655-2021, 2021
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The aerosol fine-mode fraction (FMF) is an important parameter reflecting the content of man-made aerosols. This study carried out the retrieval of FMF in China based on multi-angle polarization data and validated the results. The results of this study can contribute to the FMF retrieval algorithm of multi-angle polarization sensors. At the same time, a high-precision FMF dataset of China was obtained, which can provide basic data for atmospheric environment research.
Evelyn Jäkel, Tim Carlsen, André Ehrlich, Manfred Wendisch, Michael Schäfer, Sophie Rosenburg, Konstantina Nakoudi, Marco Zanatta, Gerit Birnbaum, Veit Helm, Andreas Herber, Larysa Istomina, Linlu Mei, and Anika Rohde
The Cryosphere Discuss., https://doi.org/10.5194/tc-2021-14, https://doi.org/10.5194/tc-2021-14, 2021
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Different approaches to retrieve the optical-equivalent snow grain size using satellite, airborne, and ground-based observations were evaluated and compared to modeled data. The study is focused on low Sun and partly rough surface conditions encountered North of Greenland in March/April 2018. We proposed an adjusted airborne retrieval method to reduce the retrieval uncertainty.
Igor Veselovskii, Qiaoyun Hu, Philippe Goloub, Thierry Podvin, Mikhail Korenskiy, Olivier Pujol, Oleg Dubovik, and Anton Lopatin
Atmos. Meas. Tech., 13, 6691–6701, https://doi.org/10.5194/amt-13-6691-2020, https://doi.org/10.5194/amt-13-6691-2020, 2020
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To study the feasibility of a fluorescence lidar for aerosol characterization, the fluorescence channel is added to the multiwavelength Mie-Raman lidar of Lille University. A part of the fluorescence spectrum is selected by the interference filter of 44 nm bandwidth centered at 466 nm. Such an approach has demonstrated high sensitivity, allowing fluorescence signals from weak aerosol layers to be detected. The technique can also be used for monitoring the aerosol inside the cloud layers.
Johannes Quaas, Antti Arola, Brian Cairns, Matthew Christensen, Hartwig Deneke, Annica M. L. Ekman, Graham Feingold, Ann Fridlind, Edward Gryspeerdt, Otto Hasekamp, Zhanqing Li, Antti Lipponen, Po-Lun Ma, Johannes Mülmenstädt, Athanasios Nenes, Joyce E. Penner, Daniel Rosenfeld, Roland Schrödner, Kenneth Sinclair, Odran Sourdeval, Philip Stier, Matthias Tesche, Bastiaan van Diedenhoven, and Manfred Wendisch
Atmos. Chem. Phys., 20, 15079–15099, https://doi.org/10.5194/acp-20-15079-2020, https://doi.org/10.5194/acp-20-15079-2020, 2020
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Anthropogenic pollution particles – aerosols – serve as cloud condensation nuclei and thus increase cloud droplet concentration and the clouds' reflection of sunlight (a cooling effect on climate). This Twomey effect is poorly constrained by models and requires satellite data for better quantification. The review summarizes the challenges in properly doing so and outlines avenues for progress towards a better use of aerosol retrievals and better retrievals of droplet concentrations.
Qiaoyun Hu, Haofei Wang, Philippe Goloub, Zhengqiang Li, Igor Veselovskii, Thierry Podvin, Kaitao Li, and Mikhail Korenskiy
Atmos. Chem. Phys., 20, 13817–13834, https://doi.org/10.5194/acp-20-13817-2020, https://doi.org/10.5194/acp-20-13817-2020, 2020
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This study presents the characteristics of Taklamakan dust particles derived from lidar measurements collected in the dust aerosol observation field campaign. It provides comprehensive parameters for Taklamakan dust properties and vertical distributions of Taklamakan dust. This paper also points out the importance of polluted dust which was frequently observed in the field campaign. The results contribute to improving knowledge about dust and reducing uncertainties in the climatic model.
Tim Carlsen, Gerit Birnbaum, André Ehrlich, Veit Helm, Evelyn Jäkel, Michael Schäfer, and Manfred Wendisch
The Cryosphere, 14, 3959–3978, https://doi.org/10.5194/tc-14-3959-2020, https://doi.org/10.5194/tc-14-3959-2020, 2020
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The angular reflection of solar radiation by snow surfaces is particularly anisotropic and highly variable. We measured the angular reflection from an aircraft using a digital camera in Antarctica in 2013/14 and studied its variability: the anisotropy increases with a lower Sun but decreases for rougher surfaces and larger snow grains. The applied methodology allows for a direct comparison with satellite observations, which generally underestimated the anisotropy measured within this study.
Jan Kretzschmar, Johannes Stapf, Daniel Klocke, Manfred Wendisch, and Johannes Quaas
Atmos. Chem. Phys., 20, 13145–13165, https://doi.org/10.5194/acp-20-13145-2020, https://doi.org/10.5194/acp-20-13145-2020, 2020
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This study compares simulations with the ICON model at the kilometer scale to airborne radiation and cloud microphysics observations that have been derived during the ACLOUD aircraft campaign around Svalbard, Norway, in May/June 2017. We find an overestimated surface warming effect of clouds compared to the observations in our setup. This bias was reduced by considering subgrid-scale vertical motion in the activation of cloud condensation nuclei in the two-moment microphysical scheme used.
Ying Zhang, Zhengqiang Li, Yu Chen, Gerrit de Leeuw, Chi Zhang, Yisong Xie, and Kaitao Li
Atmos. Chem. Phys., 20, 12795–12811, https://doi.org/10.5194/acp-20-12795-2020, https://doi.org/10.5194/acp-20-12795-2020, 2020
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Observation of atmospheric aerosol components plays an important role in reducing uncertainty in climate assessment. In this study, an improved remote sensing method which can better distinguish scattering components is developed, and the aerosol components in the atmospheric column over China are retrieved based on the Sun–sky radiometer Observation NETwork (SONET). The component distribution shows there could be a sea salt component in northwest China from a paleomarine source in desert land.
Johannes Stapf, André Ehrlich, Evelyn Jäkel, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys., 20, 9895–9914, https://doi.org/10.5194/acp-20-9895-2020, https://doi.org/10.5194/acp-20-9895-2020, 2020
Haofei Wang, Zhengqiang Li, Yang Lv, Ying Zhang, Hua Xu, Jianping Guo, and Philippe Goloub
Atmos. Chem. Phys., 20, 8839–8854, https://doi.org/10.5194/acp-20-8839-2020, https://doi.org/10.5194/acp-20-8839-2020, 2020
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Lidar shows good performance in calculating the convective layer height in the daytime and the residual layer height at night, as well as having the potential to describe the stable layer height at night. The MLH seasonal change in Beijing indicates that it is low in winter and autumn and high in spring and summer. From 2014 to 2018, the magnitude of the diurnal cycle of MLH increased year by year. MLH from lidar shows better accuracy than a radiosonde when calculating surface pollution.
Tobias Donth, Evelyn Jäkel, André Ehrlich, Bernd Heinold, Jacob Schacht, Andreas Herber, Marco Zanatta, and Manfred Wendisch
Atmos. Chem. Phys., 20, 8139–8156, https://doi.org/10.5194/acp-20-8139-2020, https://doi.org/10.5194/acp-20-8139-2020, 2020
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Solar radiative effects of Arctic black carbon (BC) particles (suspended in the atmosphere and in the surface snowpack) were quantified under cloudless and cloudy conditions. An atmospheric and a snow radiative transfer model were coupled to account for radiative interactions between both compartments. It was found that (i) the warming effect of BC in the snowpack overcompensates for the atmospheric BC cooling effect, and (ii) clouds tend to reduce the atmospheric BC cooling and snow BC warming.
Igor Veselovskii, Qiaoyun Hu, Philippe Goloub, Thierry Podvin, Mikhail Korenskiy, Yevgeny Derimian, Michel Legrand, and Patricia Castellanos
Atmos. Chem. Phys., 20, 6563–6581, https://doi.org/10.5194/acp-20-6563-2020, https://doi.org/10.5194/acp-20-6563-2020, 2020
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Atmospheric dust has a significant impact on the Earth's climate system, and this impact remains highly uncertain. The desert dust is always a mixture of various minerals, and the imaginary part of the complex refractive index often exhibits an increase in UV for dust containing iron oxides. Our results demonstrate that multiwavelength Raman lidar measurements allow for the characterization of the spectral dependence of the imaginary part of dust.
Elena Ruiz-Donoso, André Ehrlich, Michael Schäfer, Evelyn Jäkel, Vera Schemann, Susanne Crewell, Mario Mech, Birte Solveig Kulla, Leif-Leonard Kliesch, Roland Neuber, and Manfred Wendisch
Atmos. Chem. Phys., 20, 5487–5511, https://doi.org/10.5194/acp-20-5487-2020, https://doi.org/10.5194/acp-20-5487-2020, 2020
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Mixed-phase clouds, formed of water droplets and ice crystals, appear frequently in Arctic regions. Characterizing the distribution of liquid water and ice inside the cloud appropriately is important because it influences the cloud's impact on the surface temperature. In this study, we combined images of the cloud top with measurements inside the cloud to analyze in detail the 3D spatial distribution of liquid and ice in two mixed-phase clouds occurring under different meteorological scenarios.
Bruna A. Holanda, Mira L. Pöhlker, David Walter, Jorge Saturno, Matthias Sörgel, Jeannine Ditas, Florian Ditas, Christiane Schulz, Marco Aurélio Franco, Qiaoqiao Wang, Tobias Donth, Paulo Artaxo, Henrique M. J. Barbosa, Stephan Borrmann, Ramon Braga, Joel Brito, Yafang Cheng, Maximilian Dollner, Johannes W. Kaiser, Thomas Klimach, Christoph Knote, Ovid O. Krüger, Daniel Fütterer, Jošt V. Lavrič, Nan Ma, Luiz A. T. Machado, Jing Ming, Fernando G. Morais, Hauke Paulsen, Daniel Sauer, Hans Schlager, Johannes Schneider, Hang Su, Bernadett Weinzierl, Adrian Walser, Manfred Wendisch, Helmut Ziereis, Martin Zöger, Ulrich Pöschl, Meinrat O. Andreae, and Christopher Pöhlker
Atmos. Chem. Phys., 20, 4757–4785, https://doi.org/10.5194/acp-20-4757-2020, https://doi.org/10.5194/acp-20-4757-2020, 2020
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Biomass burning smoke from African savanna and grassland is transported across the South Atlantic Ocean in defined layers within the free troposphere. The combination of in situ aircraft and ground-based measurements aided by satellite observations showed that these layers are transported into the Amazon Basin during the early dry season. The influx of aged smoke, enriched in black carbon and cloud condensation nuclei, has important implications for the Amazonian aerosol and cloud cycling.
Fan Mei, Jian Wang, Jennifer M. Comstock, Ralf Weigel, Martina Krämer, Christoph Mahnke, John E. Shilling, Johannes Schneider, Christiane Schulz, Charles N. Long, Manfred Wendisch, Luiz A. T. Machado, Beat Schmid, Trismono Krisna, Mikhail Pekour, John Hubbe, Andreas Giez, Bernadett Weinzierl, Martin Zoeger, Mira L. Pöhlker, Hans Schlager, Micael A. Cecchini, Meinrat O. Andreae, Scot T. Martin, Suzane S. de Sá, Jiwen Fan, Jason Tomlinson, Stephen Springston, Ulrich Pöschl, Paulo Artaxo, Christopher Pöhlker, Thomas Klimach, Andreas Minikin, Armin Afchine, and Stephan Borrmann
Atmos. Meas. Tech., 13, 661–684, https://doi.org/10.5194/amt-13-661-2020, https://doi.org/10.5194/amt-13-661-2020, 2020
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In 2014, the US DOE G1 aircraft and the German HALO aircraft overflew the Amazon basin to study how aerosols influence cloud cycles under a clean condition and around a tropical megacity. This paper describes how to meaningfully compare similar measurements from two research aircraft and identify the potential measurement issue. We also discuss the uncertainty range for each measurement for further usage in model evaluation and satellite data validation.
Pascal Polonik, Christoph Knote, Tobias Zinner, Florian Ewald, Tobias Kölling, Bernhard Mayer, Meinrat O. Andreae, Tina Jurkat-Witschas, Thomas Klimach, Christoph Mahnke, Sergej Molleker, Christopher Pöhlker, Mira L. Pöhlker, Ulrich Pöschl, Daniel Rosenfeld, Christiane Voigt, Ralf Weigel, and Manfred Wendisch
Atmos. Chem. Phys., 20, 1591–1605, https://doi.org/10.5194/acp-20-1591-2020, https://doi.org/10.5194/acp-20-1591-2020, 2020
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A realistic representation of cloud–aerosol interactions is central to accurate climate projections. Here we combine observations collected during the ACRIDICON-CHUVA campaign with chemistry-transport simulations to evaluate the model’s ability to represent the indirect effects of biomass burning aerosol on cloud microphysics. We find an upper limit for the model sensitivity on cloud condensation nuclei concentrations well below the levels reached during the burning season in the Amazon Basin.
Cheng Chen, Oleg Dubovik, Daven K. Henze, Mian Chin, Tatyana Lapyonok, Gregory L. Schuster, Fabrice Ducos, David Fuertes, Pavel Litvinov, Lei Li, Anton Lopatin, Qiaoyun Hu, and Benjamin Torres
Atmos. Chem. Phys., 19, 14585–14606, https://doi.org/10.5194/acp-19-14585-2019, https://doi.org/10.5194/acp-19-14585-2019, 2019
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Global BC, OC and DD aerosol emissions are inverted from POLDER/PARASOL observations for the year 2010 based on the GEOS-Chem inverse modeling framework. The retrieved emissions are 18.4 Tg yr−1 BC, 109.9 Tg yr−1 OC and 731.6 Tg yr−1 DD, which indicate an increase of 166.7 % for BC and 184.0 % for OC, while a decrease of 42.4 % for DD with respect to GEOS-Chem a priori emission inventories is seen. Global annul mean AOD and AAOD resulting from retrieved emissions are 0.119 and 0.0071 at 550 nm.
André Ehrlich, Manfred Wendisch, Christof Lüpkes, Matthias Buschmann, Heiko Bozem, Dmitri Chechin, Hans-Christian Clemen, Régis Dupuy, Olliver Eppers, Jörg Hartmann, Andreas Herber, Evelyn Jäkel, Emma Järvinen, Olivier Jourdan, Udo Kästner, Leif-Leonard Kliesch, Franziska Köllner, Mario Mech, Stephan Mertes, Roland Neuber, Elena Ruiz-Donoso, Martin Schnaiter, Johannes Schneider, Johannes Stapf, and Marco Zanatta
Earth Syst. Sci. Data, 11, 1853–1881, https://doi.org/10.5194/essd-11-1853-2019, https://doi.org/10.5194/essd-11-1853-2019, 2019
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During the Arctic CLoud Observations Using airborne measurements during polar Day (ACLOUD) campaign, two research aircraft (Polar 5 and 6) jointly performed 22 research flights over the transition zone between open ocean and closed sea ice. The data set combines remote sensing and in situ measurement of cloud, aerosol, and trace gas properties, as well as turbulent and radiative fluxes, which will be used to study Arctic boundary layer and mid-level clouds and their role in Arctic amplification.
Lei Li, Oleg Dubovik, Yevgeny Derimian, Gregory L. Schuster, Tatyana Lapyonok, Pavel Litvinov, Fabrice Ducos, David Fuertes, Cheng Chen, Zhengqiang Li, Anton Lopatin, Benjamin Torres, and Huizheng Che
Atmos. Chem. Phys., 19, 13409–13443, https://doi.org/10.5194/acp-19-13409-2019, https://doi.org/10.5194/acp-19-13409-2019, 2019
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A novel methodology to monitor atmospheric aerosol components using remote sensing is presented. The concept is realized within the GRASP (Generalized Retrieval of Aerosol and Surface Properties) project. Application to POLDER/PARASOL and AERONET observations yielded the spatial and temporal variability of absorbing and non-absorbing insoluble and soluble aerosol species in the fine and coarse size fractions. This presents the global-scale aerosol component derived from satellite measurements.
B. Y. Ge, Z. Q. Li, W. Z. Hou, Y. Zhang, and K. T. Li
Int. Arch. Photogramm. Remote Sens. Spatial Inf. Sci., XLII-3-W9, 51–56, https://doi.org/10.5194/isprs-archives-XLII-3-W9-51-2019, https://doi.org/10.5194/isprs-archives-XLII-3-W9-51-2019, 2019
W. Z. Hou, H. F. Wang, Z. Q. Li, L. L. Qie, B. Y. Ge, C. Fan, and S. Li
Int. Arch. Photogramm. Remote Sens. Spatial Inf. Sci., XLII-3-W9, 63–69, https://doi.org/10.5194/isprs-archives-XLII-3-W9-63-2019, https://doi.org/10.5194/isprs-archives-XLII-3-W9-63-2019, 2019
Ulrike Egerer, Matthias Gottschalk, Holger Siebert, André Ehrlich, and Manfred Wendisch
Atmos. Meas. Tech., 12, 4019–4038, https://doi.org/10.5194/amt-12-4019-2019, https://doi.org/10.5194/amt-12-4019-2019, 2019
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In this study, we introduce the new tethered balloon system BELUGA, which includes different modular instrument packages for measuring turbulence and radiation in the atmospheric boundary layer. BELUGA was deployed in an Arctic field campaign in 2017, providing details of boundary layer processes in combination with low-level clouds. Those processes are still not fully understood and in situ measurements in the Arctic improve our understanding of the Arctic response in terms of global warming.
Evelyn Jäkel, Johannes Stapf, Manfred Wendisch, Marcel Nicolaus, Wolfgang Dorn, and Annette Rinke
The Cryosphere, 13, 1695–1708, https://doi.org/10.5194/tc-13-1695-2019, https://doi.org/10.5194/tc-13-1695-2019, 2019
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The sea ice surface albedo parameterization of a coupled regional climate model was validated against aircraft measurements performed in May–June 2017 north of Svalbard. The albedo parameterization was run offline from the model using the measured parameters surface temperature and snow depth to calculate the surface albedo and the individual fractions of the ice surface subtypes. An adjustment of the variables and additionally accounting for cloud cover reduced the root-mean-squared error.
Yang Wang, Steffen Dörner, Sebastian Donner, Sebastian Böhnke, Isabelle De Smedt, Russell R. Dickerson, Zipeng Dong, Hao He, Zhanqing Li, Zhengqiang Li, Donghui Li, Dong Liu, Xinrong Ren, Nicolas Theys, Yuying Wang, Yang Wang, Zhenzhu Wang, Hua Xu, Jiwei Xu, and Thomas Wagner
Atmos. Chem. Phys., 19, 5417–5449, https://doi.org/10.5194/acp-19-5417-2019, https://doi.org/10.5194/acp-19-5417-2019, 2019
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A MAX-DOAS instrument was operated to derive tropospheric vertical profiles of NO2, SO2, HONO, HCHO, CHOCHO and aerosols in the central western North China Plain in May and June 2016. The MAX-DOAS results are verified by comparisons with a collocated Raman lidar, overpass aircraft measurements, a sun photometer and in situ measurements. The contributions of regional transports and local emissions to the pollutants are evaluated based on case studies and statistic analysis.
Kevin Wolf, André Ehrlich, Marek Jacob, Susanne Crewell, Martin Wirth, and Manfred Wendisch
Atmos. Meas. Tech., 12, 1635–1658, https://doi.org/10.5194/amt-12-1635-2019, https://doi.org/10.5194/amt-12-1635-2019, 2019
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Using passive spectral solar radiation and active lidar, radar, and microwave measurements with HALO during NARVAL-II, the cloud droplet number concentration of shallow trade wind cumulus is estimated. With stepwise inclusion of the different instruments into the retrieval, the benefits of the synergetic approach based on artificial measurements and two cloud cases are demonstrated. Significant improvement with the synergetic method compared to the solar-radiation-only method is reported.
Tobias Zinner, Ulrich Schwarz, Tobias Kölling, Florian Ewald, Evelyn Jäkel, Bernhard Mayer, and Manfred Wendisch
Atmos. Meas. Tech., 12, 1167–1181, https://doi.org/10.5194/amt-12-1167-2019, https://doi.org/10.5194/amt-12-1167-2019, 2019
Qiaoyun Hu, Philippe Goloub, Igor Veselovskii, Juan-Antonio Bravo-Aranda, Ioana Elisabeta Popovici, Thierry Podvin, Martial Haeffelin, Anton Lopatin, Oleg Dubovik, Christophe Pietras, Xin Huang, Benjamin Torres, and Cheng Chen
Atmos. Chem. Phys., 19, 1173–1193, https://doi.org/10.5194/acp-19-1173-2019, https://doi.org/10.5194/acp-19-1173-2019, 2019
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Smoke plumes generated in Canadian fire activities were elevated to the lower stratosphere and transported from North America to Europe. The smoke plumes were observed by three lidar systems in northern France. This study provides a comprehensive characterization for aged smoke aerosols at high altitude using lidar observations. It presents that fire activities on the Earth's surface can be an important contributor of stratospheric aerosols and impact the Earth's radiation budget.
Igor Veselovskii, Philippe Goloub, Qiaoyun Hu, Thierry Podvin, David N. Whiteman, Mikhael Korenskiy, and Eduardo Landulfo
Atmos. Meas. Tech., 12, 119–128, https://doi.org/10.5194/amt-12-119-2019, https://doi.org/10.5194/amt-12-119-2019, 2019
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Methane is currently the second most important greenhouse gas of anthropogenic origin (after carbon dioxide) and its concentration can be increased inside the boundary layer. So, the development of instruments for vertical profiling of the methane mixing ratio is an important task. We present the results of methane profiling in the lower troposphere using LILAS Raman lidar from the Lille University observatory platform (France).
Erlend M. Knudsen, Bernd Heinold, Sandro Dahlke, Heiko Bozem, Susanne Crewell, Irina V. Gorodetskaya, Georg Heygster, Daniel Kunkel, Marion Maturilli, Mario Mech, Carolina Viceto, Annette Rinke, Holger Schmithüsen, André Ehrlich, Andreas Macke, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys., 18, 17995–18022, https://doi.org/10.5194/acp-18-17995-2018, https://doi.org/10.5194/acp-18-17995-2018, 2018
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The paper describes the synoptic development during the ACLOUD/PASCAL airborne and ship-based field campaign near Svalbard in spring 2017. This development is presented using near-surface and upperair meteorological observations, satellite, and model data. We first present time series of these data, from which we identify and characterize three key periods. Finally, we put our observations in historical and regional contexts and compare our findings to other Arctic field campaigns.
Emma Järvinen, Olivier Jourdan, David Neubauer, Bin Yao, Chao Liu, Meinrat O. Andreae, Ulrike Lohmann, Manfred Wendisch, Greg M. McFarquhar, Thomas Leisner, and Martin Schnaiter
Atmos. Chem. Phys., 18, 15767–15781, https://doi.org/10.5194/acp-18-15767-2018, https://doi.org/10.5194/acp-18-15767-2018, 2018
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Using light diffraction it is possible to detect microscopic features within ice particles that have not yet been fully characterized. Here, this technique was applied in airborne measurements, where it was found that majority of atmospheric ice particles have features that significantly change the way ice particles interact with solar light. The microscopic features make ice-containing clouds more reflective than previously thought, which could have consequences for predicting our climate.
Christiane Schulz, Johannes Schneider, Bruna Amorim Holanda, Oliver Appel, Anja Costa, Suzane S. de Sá, Volker Dreiling, Daniel Fütterer, Tina Jurkat-Witschas, Thomas Klimach, Christoph Knote, Martina Krämer, Scot T. Martin, Stephan Mertes, Mira L. Pöhlker, Daniel Sauer, Christiane Voigt, Adrian Walser, Bernadett Weinzierl, Helmut Ziereis, Martin Zöger, Meinrat O. Andreae, Paulo Artaxo, Luiz A. T. Machado, Ulrich Pöschl, Manfred Wendisch, and Stephan Borrmann
Atmos. Chem. Phys., 18, 14979–15001, https://doi.org/10.5194/acp-18-14979-2018, https://doi.org/10.5194/acp-18-14979-2018, 2018
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Aerosol chemical composition measurements in the tropical upper troposphere over the Amazon region show that 78 % of the aerosol in the upper troposphere consists of organic matter. Up to 20 % of the organic aerosol can be attributed to isoprene epoxydiol secondary organic aerosol (IEPOX-SOA). Furthermore, organic nitrates were identified, suggesting a connection to the IEPOX-SOA formation.
Michael Schäfer, Katharina Loewe, André Ehrlich, Corinna Hoose, and Manfred Wendisch
Atmos. Chem. Phys., 18, 13115–13133, https://doi.org/10.5194/acp-18-13115-2018, https://doi.org/10.5194/acp-18-13115-2018, 2018
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Airborne observed horizontal fields of cloud optical thickness are compared with semi-idealized large eddy simulations of Arctic stratus. The comparison focuses on horizontal cloud inhomogeneities and directional features of the small-scale cloud structures. Using inhomogeneity parameters and autocorrelation analysis it is investigated, if the observed small-scale cloud inhomogeneities can be represented by the model. Forcings for cloud inhomogeneities are investigated in a sensitivity study.
Jorge Saturno, Florian Ditas, Marloes Penning de Vries, Bruna A. Holanda, Mira L. Pöhlker, Samara Carbone, David Walter, Nicole Bobrowski, Joel Brito, Xuguang Chi, Alexandra Gutmann, Isabella Hrabe de Angelis, Luiz A. T. Machado, Daniel Moran-Zuloaga, Julian Rüdiger, Johannes Schneider, Christiane Schulz, Qiaoqiao Wang, Manfred Wendisch, Paulo Artaxo, Thomas Wagner, Ulrich Pöschl, Meinrat O. Andreae, and Christopher Pöhlker
Atmos. Chem. Phys., 18, 10391–10405, https://doi.org/10.5194/acp-18-10391-2018, https://doi.org/10.5194/acp-18-10391-2018, 2018
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This study uses satellite observations to track volcanic emissions in eastern Congo and their subsequent transport across the Atlantic Ocean into the Amazon Basin. Aircraft and ground-based observations are used to characterize the influence of volcanogenic aerosol on the chemical and microphysical properties of Amazonian aerosols. Further, this work is an illustrative example of the conditions and dynamics driving the transatlantic transport of African emissions to South America.
Luiz A. T. Machado, Alan J. P. Calheiros, Thiago Biscaro, Scott Giangrande, Maria A. F. Silva Dias, Micael A. Cecchini, Rachel Albrecht, Meinrat O. Andreae, Wagner F. Araujo, Paulo Artaxo, Stephan Borrmann, Ramon Braga, Casey Burleyson, Cristiano W. Eichholz, Jiwen Fan, Zhe Feng, Gilberto F. Fisch, Michael P. Jensen, Scot T. Martin, Ulrich Pöschl, Christopher Pöhlker, Mira L. Pöhlker, Jean-François Ribaud, Daniel Rosenfeld, Jaci M. B. Saraiva, Courtney Schumacher, Ryan Thalman, David Walter, and Manfred Wendisch
Atmos. Chem. Phys., 18, 6461–6482, https://doi.org/10.5194/acp-18-6461-2018, https://doi.org/10.5194/acp-18-6461-2018, 2018
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This overview discuss the main precipitation processes and their sensitivities to environmental conditions in the Central Amazon Basin. It presents a review of the knowledge acquired about cloud processes and rainfall formation in Amazonas. In addition, this study provides a characterization of the seasonal variation and rainfall sensitivities to topography, surface cover, and aerosol concentration. Airplane measurements were evaluated to characterize and contrast cloud microphysical properties.
W. Z. Hou, Z. Q. Li, F. X. Zheng, and L. L. Qie
Int. Arch. Photogramm. Remote Sens. Spatial Inf. Sci., XLII-3, 533–537, https://doi.org/10.5194/isprs-archives-XLII-3-533-2018, https://doi.org/10.5194/isprs-archives-XLII-3-533-2018, 2018
K. Li, Z. Li, D. Li, Y. Xie, and H. Xu
Int. Arch. Photogramm. Remote Sens. Spatial Inf. Sci., XLII-3, 849–852, https://doi.org/10.5194/isprs-archives-XLII-3-849-2018, https://doi.org/10.5194/isprs-archives-XLII-3-849-2018, 2018
L. Li, L. L. Qie, H. Xu, and Z. Q. Li
Int. Arch. Photogramm. Remote Sens. Spatial Inf. Sci., XLII-3, 857–863, https://doi.org/10.5194/isprs-archives-XLII-3-857-2018, https://doi.org/10.5194/isprs-archives-XLII-3-857-2018, 2018
Z. Li, Y. Zhang, and J. Hong
Int. Arch. Photogramm. Remote Sens. Spatial Inf. Sci., XLII-3, 981–984, https://doi.org/10.5194/isprs-archives-XLII-3-981-2018, https://doi.org/10.5194/isprs-archives-XLII-3-981-2018, 2018
L. Qie, Z. Li, L. Li, K. Li, D. Li, and H. Xu
Int. Arch. Photogramm. Remote Sens. Spatial Inf. Sci., XLII-3, 1421–1426, https://doi.org/10.5194/isprs-archives-XLII-3-1421-2018, https://doi.org/10.5194/isprs-archives-XLII-3-1421-2018, 2018
Trismono C. Krisna, Manfred Wendisch, André Ehrlich, Evelyn Jäkel, Frank Werner, Ralf Weigel, Stephan Borrmann, Christoph Mahnke, Ulrich Pöschl, Meinrat O. Andreae, Christiane Voigt, and Luiz A. T. Machado
Atmos. Chem. Phys., 18, 4439–4462, https://doi.org/10.5194/acp-18-4439-2018, https://doi.org/10.5194/acp-18-4439-2018, 2018
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The optical thickness and particle effective radius of a cirrus above liquid water clouds and a DCC topped by an anvil cirrus are retrieved based on SMART and MODIS radiance measurements. For the cirrus, retrieved particle effective radius are validated with corresponding in situ data using a vertical weighting method. This approach allows to assess the measurements, retrieval algorithms, and derived cloud products.
Meinrat O. Andreae, Armin Afchine, Rachel Albrecht, Bruna Amorim Holanda, Paulo Artaxo, Henrique M. J. Barbosa, Stephan Borrmann, Micael A. Cecchini, Anja Costa, Maximilian Dollner, Daniel Fütterer, Emma Järvinen, Tina Jurkat, Thomas Klimach, Tobias Konemann, Christoph Knote, Martina Krämer, Trismono Krisna, Luiz A. T. Machado, Stephan Mertes, Andreas Minikin, Christopher Pöhlker, Mira L. Pöhlker, Ulrich Pöschl, Daniel Rosenfeld, Daniel Sauer, Hans Schlager, Martin Schnaiter, Johannes Schneider, Christiane Schulz, Antonio Spanu, Vinicius B. Sperling, Christiane Voigt, Adrian Walser, Jian Wang, Bernadett Weinzierl, Manfred Wendisch, and Helmut Ziereis
Atmos. Chem. Phys., 18, 921–961, https://doi.org/10.5194/acp-18-921-2018, https://doi.org/10.5194/acp-18-921-2018, 2018
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We made airborne measurements of aerosol particle concentrations and properties over the Amazon Basin. We found extremely high concentrations of very small particles in the region between 8 and 14 km altitude all across the basin, which had been recently formed by gas-to-particle conversion at these altitudes. This makes the upper troposphere a very important source region of atmospheric particles with significant implications for the Earth's climate system.
Myungje Choi, Jhoon Kim, Jaehwa Lee, Mijin Kim, Young-Je Park, Brent Holben, Thomas F. Eck, Zhengqiang Li, and Chul H. Song
Atmos. Meas. Tech., 11, 385–408, https://doi.org/10.5194/amt-11-385-2018, https://doi.org/10.5194/amt-11-385-2018, 2018
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This study is a major version upgrade of the aerosol product from GOCI, the first and unique ocean color imager in geostationary earth orbit. It describes the improvement of version 2 of the GOCI Yonsei aerosol retrieval algorithm for near-real-time processing with improved accuracy from the modification of cloud masking, surface reflectance, etc. The product is validated against AERONET/SONET over East Asia with analyses of various errors features, and a pixel-level uncertainty is calculated.
Micael A. Cecchini, Luiz A. T. Machado, Manfred Wendisch, Anja Costa, Martina Krämer, Meinrat O. Andreae, Armin Afchine, Rachel I. Albrecht, Paulo Artaxo, Stephan Borrmann, Daniel Fütterer, Thomas Klimach, Christoph Mahnke, Scot T. Martin, Andreas Minikin, Sergej Molleker, Lianet H. Pardo, Christopher Pöhlker, Mira L. Pöhlker, Ulrich Pöschl, Daniel Rosenfeld, and Bernadett Weinzierl
Atmos. Chem. Phys., 17, 14727–14746, https://doi.org/10.5194/acp-17-14727-2017, https://doi.org/10.5194/acp-17-14727-2017, 2017
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This study introduces and explores the concept of gamma phase space. This space is able to represent all possible variations in the cloud droplet size distributions (DSDs). The methodology was applied to recent in situ aircraft measurements over the Amazon. It is shown that the phase space is able to represent several processes occurring in the clouds in a simple manner. The consequences for cloud studies, modeling, and the representation of the transition from warm to mixed phase are discussed.
Naifang Bei, Jiarui Wu, Miriam Elser, Tian Feng, Junji Cao, Imad El-Haddad, Xia Li, Rujin Huang, Zhengqiang Li, Xin Long, Li Xing, Shuyu Zhao, Xuexi Tie, André S. H. Prévôt, and Guohui Li
Atmos. Chem. Phys., 17, 14579–14591, https://doi.org/10.5194/acp-17-14579-2017, https://doi.org/10.5194/acp-17-14579-2017, 2017
Ramon Campos Braga, Daniel Rosenfeld, Ralf Weigel, Tina Jurkat, Meinrat O. Andreae, Manfred Wendisch, Ulrich Pöschl, Christiane Voigt, Christoph Mahnke, Stephan Borrmann, Rachel I. Albrecht, Sergej Molleker, Daniel A. Vila, Luiz A. T. Machado, and Lucas Grulich
Atmos. Chem. Phys., 17, 14433–14456, https://doi.org/10.5194/acp-17-14433-2017, https://doi.org/10.5194/acp-17-14433-2017, 2017
Tim Carlsen, Gerit Birnbaum, André Ehrlich, Johannes Freitag, Georg Heygster, Larysa Istomina, Sepp Kipfstuhl, Anaïs Orsi, Michael Schäfer, and Manfred Wendisch
The Cryosphere, 11, 2727–2741, https://doi.org/10.5194/tc-11-2727-2017, https://doi.org/10.5194/tc-11-2727-2017, 2017
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The optical size of snow grains (ropt) affects the reflectivity of snow surfaces and thus the local surface energy budget in particular in polar regions. The temporal evolution of ropt retrieved from ground-based, airborne, and spaceborne remote sensing could reproduce optical in situ measurements for a 2-month period in central Antarctica (2013/14). The presented validation study provided a unique testbed for retrievals of ropt under Antarctic conditions where in situ data are scarce.
Anja Costa, Jessica Meyer, Armin Afchine, Anna Luebke, Gebhard Günther, James R. Dorsey, Martin W. Gallagher, Andre Ehrlich, Manfred Wendisch, Darrel Baumgardner, Heike Wex, and Martina Krämer
Atmos. Chem. Phys., 17, 12219–12238, https://doi.org/10.5194/acp-17-12219-2017, https://doi.org/10.5194/acp-17-12219-2017, 2017
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The paper presents 38 h of in situ cloud spectrometer observations of microphysical cloud properties in the Arctic, midlatitudes and tropics. The clouds are classified via particle concentrations, size distributions, and – as a novelty – small particle aspherical fractions. Cloud-type profiles are given for different temperatures and locations. The results confine regions where different cloud transformation processes occurred and emphasise the importance of small particle shape detection.
Marcus Klingebiel, André Ehrlich, Fanny Finger, Timo Röschenthaler, Suad Jakirlić, Matthias Voigt, Stefan Müller, Rolf Maser, Manfred Wendisch, Peter Hoor, Peter Spichtinger, and Stephan Borrmann
Atmos. Meas. Tech., 10, 3485–3498, https://doi.org/10.5194/amt-10-3485-2017, https://doi.org/10.5194/amt-10-3485-2017, 2017
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Microphysical and radiation measurements were collected with the unique AIRcraft TOwed Sensor Shuttle (AIRTOSS) – Learjet tandem platform. It is a combination of a Learjet 35A research aircraft and an instrumented aerodynamic bird, which can be detached from and retracted back to the aircraft during flight.
AIRTOSS and Learjet are equipped with radiative, cloud microphysical, trace gas,
and meteorological instruments to study cirrus clouds.
André Ehrlich, Eike Bierwirth, Larysa Istomina, and Manfred Wendisch
Atmos. Meas. Tech., 10, 3215–3230, https://doi.org/10.5194/amt-10-3215-2017, https://doi.org/10.5194/amt-10-3215-2017, 2017
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In the Arctic, uncertainties in passive solar remote sensing of cloud properties arise from uncertainties in the assumed spectral surface albedo, mainly determined by the generally unknown effective snow grain size. Therefore, a retrieval method is presented that simultaneously derives liquid water cloud and snow surface parameters, including cloud optical thickness, droplet effective radius, and effective snow grain size. Airborne measurements were used to test the retrieval procedure.
Ying Zhang, Zhengqiang Li, Yuhuan Zhang, Donghui Li, Lili Qie, Huizheng Che, and Hua Xu
Atmos. Meas. Tech., 10, 3203–3213, https://doi.org/10.5194/amt-10-3203-2017, https://doi.org/10.5194/amt-10-3203-2017, 2017
Micael A. Cecchini, Luiz A. T. Machado, Meinrat O. Andreae, Scot T. Martin, Rachel I. Albrecht, Paulo Artaxo, Henrique M. J. Barbosa, Stephan Borrmann, Daniel Fütterer, Tina Jurkat, Christoph Mahnke, Andreas Minikin, Sergej Molleker, Mira L. Pöhlker, Ulrich Pöschl, Daniel Rosenfeld, Christiane Voigt, Bernadett Weinzierl, and Manfred Wendisch
Atmos. Chem. Phys., 17, 10037–10050, https://doi.org/10.5194/acp-17-10037-2017, https://doi.org/10.5194/acp-17-10037-2017, 2017
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We study the effects of aerosol particles and updraft speed on the warm phase of Amazonian clouds. We expand the sensitivity analysis usually found in the literature by concomitantly considering cloud evolution and the effects on droplet size distribution (DSD) shape. The quantitative results show that particle concentration is the primary driver for the vertical profiles of effective diameter and droplet concentration in the warm phase of Amazonian convective clouds.
Evelyn Jäkel, Manfred Wendisch, Trismono C. Krisna, Florian Ewald, Tobias Kölling, Tina Jurkat, Christiane Voigt, Micael A. Cecchini, Luiz A. T. Machado, Armin Afchine, Anja Costa, Martina Krämer, Meinrat O. Andreae, Ulrich Pöschl, Daniel Rosenfeld, and Tianle Yuan
Atmos. Chem. Phys., 17, 9049–9066, https://doi.org/10.5194/acp-17-9049-2017, https://doi.org/10.5194/acp-17-9049-2017, 2017
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Vertical profiles of the cloud particle phase state in tropical deep convective clouds (DCCs) were investigated using airborne imaging spectrometer measurements during the ACRIDICON-CHUVA campaign, which was conducted over the Brazilian rainforest in September 2014. A phase discrimination retrieval was applied to observations of clouds formed in different aerosol conditions. The profiles were compared to in situ and satellite measurements.
Ramon Campos Braga, Daniel Rosenfeld, Ralf Weigel, Tina Jurkat, Meinrat O. Andreae, Manfred Wendisch, Mira L. Pöhlker, Thomas Klimach, Ulrich Pöschl, Christopher Pöhlker, Christiane Voigt, Christoph Mahnke, Stephan Borrmann, Rachel I. Albrecht, Sergej Molleker, Daniel A. Vila, Luiz A. T. Machado, and Paulo Artaxo
Atmos. Chem. Phys., 17, 7365–7386, https://doi.org/10.5194/acp-17-7365-2017, https://doi.org/10.5194/acp-17-7365-2017, 2017
Kevin Wolf, André Ehrlich, Tilman Hüneke, Klaus Pfeilsticker, Frank Werner, Martin Wirth, and Manfred Wendisch
Atmos. Chem. Phys., 17, 4283–4303, https://doi.org/10.5194/acp-17-4283-2017, https://doi.org/10.5194/acp-17-4283-2017, 2017
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The potential of airborne radiance measurements in the sideward and nadir directions for cirrus remote sensing is investigated. Therefore radiative transfer simulations were used and the sensitivity of upward radiance with respect to optical thickness, effective radius, surface albedo, wavelength and viewing angle was studied. It was shown that sideward observations lead to more accurate retrieval results. Investigating a case study of ML-CIRRUS, these findings are confirmed.
Michael Schäfer, Eike Bierwirth, André Ehrlich, Evelyn Jäkel, Frank Werner, and Manfred Wendisch
Atmos. Chem. Phys., 17, 2359–2372, https://doi.org/10.5194/acp-17-2359-2017, https://doi.org/10.5194/acp-17-2359-2017, 2017
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Cloud optical thickness fields, retrieved from solar spectral radiance measurements, are used to investigate the directional structure of horizontal cloud inhomogeneities with scalar one-dimensional inhomogeneity parameters, two-dimensional auto-correlation functions, and two-dimensional Fourier analysis. The investigations reveal that it is not sufficient to quantify horizontal cloud inhomogeneities by one-dimensional inhomogeneity parameters; two-dimensional parameters are necessary.
Wanchun Zhang, Jianping Guo, Yucong Miao, Huan Liu, Yong Zhang, Zhengqiang Li, and Panmao Zhai
Atmos. Chem. Phys., 16, 9951–9963, https://doi.org/10.5194/acp-16-9951-2016, https://doi.org/10.5194/acp-16-9951-2016, 2016
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The PBL height retrieval from CALIOP aboard CALIPSO can significantly complement the traditional ground-based methods, which is only for one site. Our study, to our current knowledge, is the first intercomparison study of PBLH on a large scale using long-term radiosonde observations in China. Three matchup schemes were proposed based on the position of radiosondes relative to CALIPSO ground tracks in China. Results indicate that CALIOP is promising for reliable PBLH retrievals.
Fanny Finger, Frank Werner, Marcus Klingebiel, André Ehrlich, Evelyn Jäkel, Matthias Voigt, Stephan Borrmann, Peter Spichtinger, and Manfred Wendisch
Atmos. Chem. Phys., 16, 7681–7693, https://doi.org/10.5194/acp-16-7681-2016, https://doi.org/10.5194/acp-16-7681-2016, 2016
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Solar spectra of optical layer properties of cirrus have been derived from the first truly collocated airborne radiation measurements using an aircraft and a towed sensor platform. The measured layer properties differ slightly due to horizontal cirrus inhomogeneities and the influence of low-level water clouds. Applying a 1-D radiative transfer model sensitivity studies were performed. It was found that if a low-level cloud is not considered, the solar cooling of the cirrus is strongly overestimated.
S. T. Martin, P. Artaxo, L. A. T. Machado, A. O. Manzi, R. A. F. Souza, C. Schumacher, J. Wang, M. O. Andreae, H. M. J. Barbosa, J. Fan, G. Fisch, A. H. Goldstein, A. Guenther, J. L. Jimenez, U. Pöschl, M. A. Silva Dias, J. N. Smith, and M. Wendisch
Atmos. Chem. Phys., 16, 4785–4797, https://doi.org/10.5194/acp-16-4785-2016, https://doi.org/10.5194/acp-16-4785-2016, 2016
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The Observations and Modeling of the Green Ocean Amazon (GoAmazon2014/5) Experiment took place in central Amazonia throughout 2014 and 2015. The experiment focused on the complex links among vegetation, atmospheric chemistry, and aerosol production on the one hand and their connections to aerosols, clouds, and precipitation on the other, especially when altered by urban pollution. This article serves as an introduction to the special issue of publications presenting findings of this experiment.
Miriam Elser, Ru-Jin Huang, Robert Wolf, Jay G. Slowik, Qiyuan Wang, Francesco Canonaco, Guohui Li, Carlo Bozzetti, Kaspar R. Daellenbach, Yu Huang, Renjian Zhang, Zhengqiang Li, Junji Cao, Urs Baltensperger, Imad El-Haddad, and André S. H. Prévôt
Atmos. Chem. Phys., 16, 3207–3225, https://doi.org/10.5194/acp-16-3207-2016, https://doi.org/10.5194/acp-16-3207-2016, 2016
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This work represents the first online chemical characterization of the PM2.5 using a high-resolution time-of flight aerosol mass spectrometer during extreme haze events China. The application of novel source apportionment techniques allowed for an improved identification and quantification of the sources of organic aerosols. The main sources and processes driving the extreme haze events are assessed.
E. Jäkel, B. Mey, R. Levy, X. Gu, T. Yu, Z. Li, D. Althausen, B. Heese, and M. Wendisch
Atmos. Meas. Tech., 8, 5237–5249, https://doi.org/10.5194/amt-8-5237-2015, https://doi.org/10.5194/amt-8-5237-2015, 2015
A. Ehrlich and M. Wendisch
Atmos. Meas. Tech., 8, 3671–3684, https://doi.org/10.5194/amt-8-3671-2015, https://doi.org/10.5194/amt-8-3671-2015, 2015
M. Schäfer, E. Bierwirth, A. Ehrlich, E. Jäkel, and M. Wendisch
Atmos. Chem. Phys., 15, 8147–8163, https://doi.org/10.5194/acp-15-8147-2015, https://doi.org/10.5194/acp-15-8147-2015, 2015
M. Klingebiel, A. de Lozar, S. Molleker, R. Weigel, A. Roth, L. Schmidt, J. Meyer, A. Ehrlich, R. Neuber, M. Wendisch, and S. Borrmann
Atmos. Chem. Phys., 15, 617–631, https://doi.org/10.5194/acp-15-617-2015, https://doi.org/10.5194/acp-15-617-2015, 2015
G. Milinevsky, V. Danylevsky, V. Bovchaliuk, A. Bovchaliuk, Ph. Goloub, O. Dubovik, V. Kabashnikov, A. Chaikovsky, N. Miatselskaya, M. Mishchenko, and M. Sosonkin
Atmos. Meas. Tech., 7, 1459–1474, https://doi.org/10.5194/amt-7-1459-2014, https://doi.org/10.5194/amt-7-1459-2014, 2014
H. Che, X. Xia, J. Zhu, Z. Li, O. Dubovik, B. Holben, P. Goloub, H. Chen, V. Estelles, E. Cuevas-Agulló, L. Blarel, H. Wang, H. Zhao, X. Zhang, Y. Wang, J. Sun, R. Tao, X. Zhang, and G. Shi
Atmos. Chem. Phys., 14, 2125–2138, https://doi.org/10.5194/acp-14-2125-2014, https://doi.org/10.5194/acp-14-2125-2014, 2014
C. Fricke, A. Ehrlich, E. Jäkel, B. Bohn, M. Wirth, and M. Wendisch
Atmos. Chem. Phys., 14, 1943–1958, https://doi.org/10.5194/acp-14-1943-2014, https://doi.org/10.5194/acp-14-1943-2014, 2014
F. Waquet, F. Peers, P. Goloub, F. Ducos, F. Thieuleux, Y. Derimian, J. Riedi, M. Chami, and D. Tanré
Atmos. Chem. Phys., 14, 1755–1768, https://doi.org/10.5194/acp-14-1755-2014, https://doi.org/10.5194/acp-14-1755-2014, 2014
B. Torres, O. Dubovik, C. Toledano, A. Berjon, V. E. Cachorro, T. Lapyonok, P. Litvinov, and P. Goloub
Atmos. Chem. Phys., 14, 847–875, https://doi.org/10.5194/acp-14-847-2014, https://doi.org/10.5194/acp-14-847-2014, 2014
Z. Li, X. Gu, L. Wang, D. Li, Y. Xie, K. Li, O. Dubovik, G. Schuster, P. Goloub, Y. Zhang, L. Li, Y. Ma, and H. Xu
Atmos. Chem. Phys., 13, 10171–10183, https://doi.org/10.5194/acp-13-10171-2013, https://doi.org/10.5194/acp-13-10171-2013, 2013
Y. Karol, D. Tanré, P. Goloub, C. Vervaerde, J. Y. Balois, L. Blarel, T. Podvin, A. Mortier, and A. Chaikovsky
Atmos. Meas. Tech., 6, 2383–2389, https://doi.org/10.5194/amt-6-2383-2013, https://doi.org/10.5194/amt-6-2383-2013, 2013
B. Torres, C. Toledano, A. Berjón, D. Fuertes, V. Molina, R. Gonzalez, M. Canini, V. E. Cachorro, P. Goloub, T. Podvin, L. Blarel, O. Dubovik, Y. Bennouna, and A. M. de Frutos
Atmos. Meas. Tech., 6, 2207–2220, https://doi.org/10.5194/amt-6-2207-2013, https://doi.org/10.5194/amt-6-2207-2013, 2013
A. Lopatin, O. Dubovik, A. Chaikovsky, P. Goloub, T. Lapyonok, D. Tanré, and P. Litvinov
Atmos. Meas. Tech., 6, 2065–2088, https://doi.org/10.5194/amt-6-2065-2013, https://doi.org/10.5194/amt-6-2065-2013, 2013
M. Schäfer, E. Bierwirth, A. Ehrlich, F. Heyner, and M. Wendisch
Atmos. Meas. Tech., 6, 1855–1868, https://doi.org/10.5194/amt-6-1855-2013, https://doi.org/10.5194/amt-6-1855-2013, 2013
A. Bovchaliuk, G. Milinevsky, V. Danylevsky, P. Goloub, O. Dubovik, A. Holdak, F. Ducos, and M. Sosonkin
Atmos. Chem. Phys., 13, 6587–6602, https://doi.org/10.5194/acp-13-6587-2013, https://doi.org/10.5194/acp-13-6587-2013, 2013
E. Bierwirth, A. Ehrlich, M. Wendisch, J.-F. Gayet, C. Gourbeyre, R. Dupuy, A. Herber, R. Neuber, and A. Lampert
Atmos. Meas. Tech., 6, 1189–1200, https://doi.org/10.5194/amt-6-1189-2013, https://doi.org/10.5194/amt-6-1189-2013, 2013
F. Waquet, C. Cornet, J.-L. Deuzé, O. Dubovik, F. Ducos, P. Goloub, M. Herman, T. Lapyonok, L. C. Labonnote, J. Riedi, D. Tanré, F. Thieuleux, and C. Vanbauce
Atmos. Meas. Tech., 6, 991–1016, https://doi.org/10.5194/amt-6-991-2013, https://doi.org/10.5194/amt-6-991-2013, 2013
A. Mortier, P. Goloub, T. Podvin, C. Deroo, A. Chaikovsky, N. Ajtai, L. Blarel, D. Tanre, and Y. Derimian
Atmos. Chem. Phys., 13, 3705–3720, https://doi.org/10.5194/acp-13-3705-2013, https://doi.org/10.5194/acp-13-3705-2013, 2013
E. Jäkel, J. Walter, and M. Wendisch
Atmos. Meas. Tech., 6, 539–547, https://doi.org/10.5194/amt-6-539-2013, https://doi.org/10.5194/amt-6-539-2013, 2013
E. Jäkel, M. Wendisch, and B. Mayer
Atmos. Meas. Tech., 6, 527–537, https://doi.org/10.5194/amt-6-527-2013, https://doi.org/10.5194/amt-6-527-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Effect of wind speed on marine aerosol optical properties over remote oceans with use of spaceborne lidar observations
Assessment of smoke plume height products derived from multisource satellite observations using lidar-derived height metrics for wildfires in the western US
A remote sensing algorithm for vertically resolved cloud condensation nuclei number concentrations from airborne and spaceborne lidar observations
Opinion: Aerosol remote sensing over the next 20 years
Monitoring biomass burning aerosol transport using CALIOP observations and reanalysis models: a Canadian wildfire event in 2019
Thermal infrared observations of a western United States biomass burning aerosol plume
A new look into the impacts of dust radiative effects on the energetics of tropical easterly waves
Wind-driven emissions of coarse-mode particles in an urban environment
Measurement report: Dust and anthropogenic aerosols' vertical distributions over northern China dense aerosols gathered at the top of the mixing layer
Climatological assessment of the vertically resolved optical and microphysical aerosol properties by lidar measurements, sun photometer, and in situ observations over 17 years at Universitat Politècnica de Catalunya (UPC) Barcelona
Aerosol optical depth climatology from the high-resolution MAIAC product over Europe: differences between major European cities and their surrounding environments
Impact of assimilating NOAA VIIRS aerosol optical depth (AOD) observations on global AOD analysis from the Copernicus Atmosphere Monitoring Service (CAMS)
Dust storms from the Taklamakan Desert significantly darken snow surface on surrounding mountains
Spectral dependence of birch and pine pollen optical properties using a synergy of lidar instruments
Opposite effects of aerosols and meteorological parameters on warm clouds in two contrasting regions over eastern China
Validation activities of Aeolus wind products on the southeastern Iberian Peninsula
Thermal infrared dust optical depth and coarse-mode effective diameter over oceans retrieved from collocated MODIS and CALIOP observations
A comprehensive reappraisal of long-term aerosol characteristics, trends, and variability in Asia
Satellite (GOSAT-2 CAI-2) retrieval and surface (ARFINET) observations of aerosol black carbon over India
Spatiotemporal variation characteristics of global fires and their emissions
The (mis)identification of high-latitude dust events using remote sensing methods in the Yukon, Canada: a sub-daily variability analysis
Comparison of dust optical depth from multi-sensor products and MONARCH (Multiscale Online Non-hydrostatic AtmospheRe CHemistry) dust reanalysis over North Africa, the Middle East, and Europe
Understanding day–night differences in dust aerosols over the dust belt of North Africa, the Middle East, and Asia
Satellite observations of smoke–cloud–radiation interactions over the Amazon rainforest
Single-scattering properties of ellipsoidal dust aerosols constrained by measured dust shape distributions
Validation of the TROPOMI/S5P aerosol layer height using EARLINET lidars
Vertical characterization of fine and coarse dust particles during an intense Saharan dust outbreak over the Iberian Peninsula in springtime 2021
Aerosol optical depth regime over megacities of the world
South American 2020 regional smoke plume: intercomparison with previous years, impact on solar radiation, and the role of Pantanal biomass burning season
Circular polarization in atmospheric aerosols
Spatiotemporal continuous estimates of daily 1 km PM2.5 from 2000 to present under the Tracking Air Pollution in China (TAP) framework
Robust evidence for reversal of the trend in aerosol effective climate forcing
Simultaneous retrievals of biomass burning aerosols and trace gases from the ultraviolet to near-infrared over northern Thailand during the 2019 pre-monsoon season
A decadal assessment of the climatology of aerosol and cloud properties over South Africa
Aerosol characterisation in the subtropical eastern North Atlantic region using long-term AERONET measurements
Long-range transport of Asian dust to the Arctic: identification of transport pathways, evolution of aerosol optical properties, and impact assessment on surface albedo changes
Canadian and Alaskan wildfire smoke particle properties, their evolution, and controlling factors, from satellite observations
Evaluation of aerosol optical depths and clear-sky radiative fluxes of the CERES Edition 4.1 SYN1deg data product
Arctic spring and summertime aerosol optical depth baseline from long-term observations and model reanalyses – Part 1: Climatology and trend
Vertical structure of biomass burning aerosol transported over the southeast Atlantic Ocean
Arctic spring and summertime aerosol optical depth baseline from long-term observations and model reanalyses – Part 2: Statistics of extreme AOD events, and implications for the impact of regional biomass burning processes
Aerosol atmospheric rivers: climatology, event characteristics, and detection algorithm sensitivities
Dust transport and advection measurement with spaceborne lidars ALADIN and CALIOP and model reanalysis data
Record-breaking dust loading during two mega dust storm events over northern China in March 2021: aerosol optical and radiative properties and meteorological drivers
Wintertime Saharan dust transport towards the Caribbean: an airborne lidar case study during EUREC4A
Evaluation of aerosol number concentrations from CALIPSO with ATom airborne in situ measurements
Zonal variations in the vertical distribution of atmospheric aerosols over the Indian region and the consequent radiative effects
Global maps of aerosol single scattering albedo using combined CERES-MODIS retrieval
The characterization of long-range transported North American biomass burning plumes: what can a multi-wavelength Mie–Raman-polarization-fluorescence lidar provide?
Fluorescence lidar observations of wildfire smoke inside cirrus: a contribution to smoke–cirrus interaction research
Kangwen Sun, Guangyao Dai, Songhua Wu, Oliver Reitebuch, Holger Baars, Jiqiao Liu, and Suping Zhang
Atmos. Chem. Phys., 24, 4389–4409, https://doi.org/10.5194/acp-24-4389-2024, https://doi.org/10.5194/acp-24-4389-2024, 2024
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This paper investigates the correlation between marine aerosol optical properties and wind speeds over remote oceans using the spaceborne lidars ALADIN and CALIOP. Three remote ocean areas are selected. Pure marine aerosol optical properties at 355 nm are derived from ALADIN. The relationships between marine aerosol optical properties and wind speeds are analyzed within and above the marine atmospheric boundary layer, revealing the effect of wind speed on marine aerosols over remote oceans.
Jingting Huang, S. Marcela Loría-Salazar, Min Deng, Jaehwa Lee, and Heather A. Holmes
Atmos. Chem. Phys., 24, 3673–3698, https://doi.org/10.5194/acp-24-3673-2024, https://doi.org/10.5194/acp-24-3673-2024, 2024
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Increased wildfire intensity has resulted in taller wildfire smoke plumes. We investigate the vertical structure of wildfire smoke plumes using aircraft lidar data and establish two effective smoke plume height metrics. Four novel satellite-based plume height products are evaluated for wildfires in the western US. Our results provide guidance on the strengths and limitations of these satellite products and set the stage for improved plume rise estimates by leveraging satellite products.
Piyushkumar N. Patel, Jonathan H. Jiang, Ritesh Gautam, Harish Gadhavi, Olga Kalashnikova, Michael J. Garay, Lan Gao, Feng Xu, and Ali Omar
Atmos. Chem. Phys., 24, 2861–2883, https://doi.org/10.5194/acp-24-2861-2024, https://doi.org/10.5194/acp-24-2861-2024, 2024
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Global measurements of cloud condensation nuclei (CCN) are essential for understanding aerosol–cloud interactions and predicting climate change. To address this gap, we introduced a remote sensing algorithm that retrieves vertically resolved CCN number concentrations from airborne and spaceborne lidar systems. This innovation offers a global distribution of CCN concentrations from space, facilitating model evaluation and precise quantification of aerosol climate forcing.
Lorraine A. Remer, Robert C. Levy, and J. Vanderlei Martins
Atmos. Chem. Phys., 24, 2113–2127, https://doi.org/10.5194/acp-24-2113-2024, https://doi.org/10.5194/acp-24-2113-2024, 2024
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Aerosols are small liquid or solid particles suspended in the atmosphere, including smoke, particulate pollution, dust, and sea salt. Today, we rely on satellites viewing Earth's atmosphere to learn about these particles. Here, we speculate on the future to imagine how satellite viewing of aerosols will change. We expect more public and private satellites with greater capabilities, better ways to infer information from satellites, and merging of data with models.
Xiaoxia Shang, Antti Lipponen, Maria Filioglou, Anu-Maija Sundström, Mark Parrington, Virginie Buchard, Anton S. Darmenov, Ellsworth J. Welton, Eleni Marinou, Vassilis Amiridis, Michael Sicard, Alejandro Rodríguez-Gómez, Mika Komppula, and Tero Mielonen
Atmos. Chem. Phys., 24, 1329–1344, https://doi.org/10.5194/acp-24-1329-2024, https://doi.org/10.5194/acp-24-1329-2024, 2024
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In June 2019, smoke particles from a Canadian wildfire event were transported to Europe. The long-range-transported smoke plumes were monitored with a spaceborne lidar and reanalysis models. Based on the aerosol mass concentrations estimated from the observations, the reanalysis models had difficulties in reproducing the amount and location of the smoke aerosols during the transport event. Consequently, more spaceborne lidar missions are needed for reliable monitoring of aerosol plumes.
Blake T. Sorenson, Jeffrey S. Reid, Jianglong Zhang, Robert E. Holz, William L. Smith Sr., and Amanda Gumber
Atmos. Chem. Phys., 24, 1231–1248, https://doi.org/10.5194/acp-24-1231-2024, https://doi.org/10.5194/acp-24-1231-2024, 2024
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Smoke particles are typically submicron in size and assumed to have negligible impacts at the thermal infrared spectrum. However, we show that infrared signatures can be observed over dense smoke plumes from satellites. We found that giant particles are unlikely to be the dominant cause. Rather, co-transported water vapor injected to the middle to upper troposphere and surface cooling beneath the plume due to shadowing are significant, with the surface cooling effect being the most dominant.
Farnaz Hosseinpour and Eric M. Wilcox
Atmos. Chem. Phys., 24, 707–724, https://doi.org/10.5194/acp-24-707-2024, https://doi.org/10.5194/acp-24-707-2024, 2024
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This study shows mechanistic relationships between the radiative effect of dust aerosols in the Saharan air layer and the kinetic energy of the African easterly waves across the tropical Atlantic Ocean using 22 years of daily satellite observations and reanalysis data based on satellite assimilation. Our findings suggest that dust aerosols not merely are transported by these waves but also contribute to the growth of waves through the enhancement of diabatic heating induced by dust.
Markus D. Petters, Tyas Pujiastuti, Ajmal Rasheeda Satheesh, Sabin Kasparoglu, Bethany Sutherland, and Nicholas Meskhidze
Atmos. Chem. Phys., 24, 745–762, https://doi.org/10.5194/acp-24-745-2024, https://doi.org/10.5194/acp-24-745-2024, 2024
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This work introduces a new method that uses remote sensing techniques to obtain surface number emissions of particles with a diameter greater than 500 nm. The technique was applied to study particle emissions at an urban site near Houston, TX, USA. The emissions followed a diurnal pattern and peaked near noon local time. The daily averaged emissions correlated with wind speed. The source is likely due to wind-driven erosion of material situated on asphalted and other hard surfaces.
Zhuang Wang, Chune Shi, Hao Zhang, Yujia Chen, Xiyuan Chi, Congzi Xia, Suyao Wang, Yizhi Zhu, Kaidi Zhang, Xintong Chen, Chengzhi Xing, and Cheng Liu
Atmos. Chem. Phys., 23, 14271–14292, https://doi.org/10.5194/acp-23-14271-2023, https://doi.org/10.5194/acp-23-14271-2023, 2023
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The annual cycle of dust and anthropogenic aerosols' vertical distributions was revealed by polarization Raman lidar in Beijing. Anthropogenic aerosols typically accumulate at the top of the mixing layer (ML) due to the hygroscopic growth of atmospheric particles, and this is most significant in summer. There is no significant relationship between bottom dust mass concentration and ML height, while the dust in the upper air tends to be distributed near the mixing layer.
Simone Lolli, Michaël Sicard, Francesco Amato, Adolfo Comeron, Cristina Gíl-Diaz, Tony C. Landi, Constantino Munoz-Porcar, Daniel Oliveira, Federico Dios Otin, Francesc Rocadenbosch, Alejandro Rodriguez-Gomez, Andrés Alastuey, Xavier Querol, and Cristina Reche
Atmos. Chem. Phys., 23, 12887–12906, https://doi.org/10.5194/acp-23-12887-2023, https://doi.org/10.5194/acp-23-12887-2023, 2023
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We evaluated the long-term trends and seasonal variability of the vertically resolved aerosol properties over the past 17 years in Barcelona. Results shows that air quality is improved, with a consistent drop in PM concentrations at the surface, as well as the column aerosol optical depth. The results also show that natural dust outbreaks are more likely in summer, with aerosols reaching an altitude of 5 km, while in winter, aerosols decay as an exponential with a scale height of 600 m.
Ludovico Di Antonio, Claudia Di Biagio, Gilles Foret, Paola Formenti, Guillaume Siour, Jean-François Doussin, and Matthias Beekmann
Atmos. Chem. Phys., 23, 12455–12475, https://doi.org/10.5194/acp-23-12455-2023, https://doi.org/10.5194/acp-23-12455-2023, 2023
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Long-term (2000–2021) 1 km resolution satellite data have been used to investigate the climatological aerosol optical depth (AOD) variability and trends at different scales in Europe. Average enhancements of the local-to-regional AOD ratio at 550 nm of 57 %, 55 %, 39 % and 32 % are found for large metropolitan areas such as Barcelona, Lisbon, Paris and Athens, respectively, suggesting a non-negligible enhancement of the aerosol burden through local emissions.
Sebastien Garrigues, Melanie Ades, Samuel Remy, Johannes Flemming, Zak Kipling, Istvan Laszlo, Mark Parrington, Antje Inness, Roberto Ribas, Luke Jones, Richard Engelen, and Vincent-Henri Peuch
Atmos. Chem. Phys., 23, 10473–10487, https://doi.org/10.5194/acp-23-10473-2023, https://doi.org/10.5194/acp-23-10473-2023, 2023
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The Copernicus Atmosphere Monitoring Service (CAMS) provides global monitoring of aerosols using the ECMWF forecast model constrained by the assimilation of satellite aerosol optical depth (AOD). This work aims at evaluating the assimilation of the NOAA VIIRS AOD product in the ECMWF model. It shows that the introduction of VIIRS in the CAMS data assimilation system enhances the accuracy of the aerosol analysis, particularly over Europe and desert and maritime sites.
Yuxuan Xing, Yang Chen, Shirui Yan, Tenglong Shi, Xiaoyi Cao, Xiaoying Niu, Dongyou Wu, Jiecan Cui, Xin Wang, and Wei Pu
EGUsphere, https://doi.org/10.5194/egusphere-2023-1443, https://doi.org/10.5194/egusphere-2023-1443, 2023
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A study investigated the impact of dust storms from the Taklamakan Desert on surrounding high mountains and regional radiation balance. Using satellite data and simulations, researchers found that dust storms significantly darken the snow surface in the Tien Shan, Kunlun, and Qilian Mountains, reaching mountains up to 1000 km away. This darkening occurs not only in spring but also during summer and autumn, leading to increased absorption of solar radiation.
Maria Filioglou, Ari Leskinen, Ville Vakkari, Ewan O'Connor, Minttu Tuononen, Pekko Tuominen, Samuli Laukkanen, Linnea Toiviainen, Annika Saarto, Xiaoxia Shang, Petri Tiitta, and Mika Komppula
Atmos. Chem. Phys., 23, 9009–9021, https://doi.org/10.5194/acp-23-9009-2023, https://doi.org/10.5194/acp-23-9009-2023, 2023
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Pollen impacts climate and public health, and it can be detected in the atmosphere by lidars which measure the linear particle depolarization ratio (PDR), a shape-relevant optical parameter. As aerosols also cause depolarization, surface aerosol and pollen observations were combined with measurements from ground-based lidars operating at different wavelengths to determine the optical properties of birch and pine pollen and quantify their relative contribution to the PDR.
Yuqin Liu, Tao Lin, Jiahua Zhang, Fu Wang, Yiyi Huang, Xian Wu, Hong Ye, Guoqin Zhang, Xin Cao, and Gerrit de Leeuw
EGUsphere, https://doi.org/10.5194/egusphere-2023-1615, https://doi.org/10.5194/egusphere-2023-1615, 2023
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Aerosols and clouds are very important for their effect on climate. Clouds are formed by condensation of water vapor on aerosol particles. We explore the interactions between aerosols, cloud and meteorological parameters in a highly polluted area over Eastern China and a relatively clean area over the East China Sea, using satellite data and different analysis methods. We describe the opposing effects of aerosol and meteorological parameters on cloud properties in the two areas.
Jesús Abril-Gago, Pablo Ortiz-Amezcua, Diego Bermejo-Pantaleón, Juana Andújar-Maqueda, Juan Antonio Bravo-Aranda, María José Granados-Muñoz, Francisco Navas-Guzmán, Lucas Alados-Arboledas, Inmaculada Foyo-Moreno, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 23, 8453–8471, https://doi.org/10.5194/acp-23-8453-2023, https://doi.org/10.5194/acp-23-8453-2023, 2023
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Validation activities of Aeolus wind products were performed in Granada with different upward-probing instrumentation (Doppler lidar system and radiosondes) and spatiotemporal collocation criteria. Specific advantages and disadvantages of each instrument were identified, and an optimal comparison criterion is proposed. Aeolus was proven to provide reliable wind products, and the upward-probing instruments were proven to be useful for Aeolus wind product validation activities.
Jianyu Zheng, Zhibo Zhang, Hongbin Yu, Anne Garnier, Qianqian Song, Chenxi Wang, Claudia Di Biagio, Jasper F. Kok, Yevgeny Derimian, and Claire Ryder
Atmos. Chem. Phys., 23, 8271–8304, https://doi.org/10.5194/acp-23-8271-2023, https://doi.org/10.5194/acp-23-8271-2023, 2023
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We developed a multi-year satellite-based retrieval of dust optical depth at 10 µm and the coarse-mode dust effective diameter over global oceans. It reveals climatological coarse-mode dust transport patterns and regional differences over the North Atlantic, the Indian Ocean and the North Pacific.
Shikuan Jin, Yingying Ma, Zhongwei Huang, Jianping Huang, Wei Gong, Boming Liu, Weiyan Wang, Ruonan Fan, and Hui Li
Atmos. Chem. Phys., 23, 8187–8210, https://doi.org/10.5194/acp-23-8187-2023, https://doi.org/10.5194/acp-23-8187-2023, 2023
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To better understand the Asian aerosol environment, we studied distributions and trends of aerosol with different sizes and types. Over the past 2 decades, dust, sulfate, and sea salt aerosol decreased by 5.51 %, 3.07 %, and 9.80 %, whereas organic carbon and black carbon aerosol increased by 17.09 % and 6.23 %, respectively. The increase in carbonaceous aerosols was a feature of Asia. An exception is found in East Asia, where the carbonaceous aerosols reduced, owing largely to China's efforts.
Mukunda M. Gogoi, S. Suresh Babu, Ryoichi Imasu, and Makiko Hashimoto
Atmos. Chem. Phys., 23, 8059–8079, https://doi.org/10.5194/acp-23-8059-2023, https://doi.org/10.5194/acp-23-8059-2023, 2023
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Considering the climate warming potential of atmospheric black carbon (BC), satellite-based retrieval is a novel idea. This study highlights the regional distribution of BC based on observations by the Cloud and Aerosol Imager-2 on board the GOSAT-2 satellite and near-surface measurements of BC in ARFINET. The satellite retrieval fairly depicts the regional and seasonal features of BC over the Indian region, which are similar to those recorded by surface observations.
Hao Fan, Xingchuan Yang, Chuanfeng Zhao, Yikun Yang, and Zhenyao Shen
Atmos. Chem. Phys., 23, 7781–7798, https://doi.org/10.5194/acp-23-7781-2023, https://doi.org/10.5194/acp-23-7781-2023, 2023
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Using 20-year multi-source data, this study shows pronounced regional and seasonal variations in fire activities and emissions. Seasonal variability of fires is larger with increasing latitude. The increase in temperature in the Northern Hemisphere's middle- and high-latitude forest regions was primarily responsible for the increase in fires and emissions, while the changes in fire occurrence in tropical regions were more influenced by the decrease in precipitation and relative humidity.
Rosemary Huck, Robert G. Bryant, and James King
Atmos. Chem. Phys., 23, 6299–6318, https://doi.org/10.5194/acp-23-6299-2023, https://doi.org/10.5194/acp-23-6299-2023, 2023
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This study shows that mineral aerosol (dust) emission events in high-latitude areas are under-represented in both ground- and space-based detecting methods. This is done through a suite of ground-based data to prove that dust emissions from the proglacial area, Lhù’ààn Mân, occur almost daily but are not always recorded at different timescales. Dust has multiple effects on atmospheric processes; therefore, accurate quantification is important in the calibration and validation of climate models.
Michail Mytilinaios, Sara Basart, Sergio Ciamprone, Juan Cuesta, Claudio Dema, Enza Di Tomaso, Paola Formenti, Antonis Gkikas, Oriol Jorba, Ralph Kahn, Carlos Pérez García-Pando, Serena Trippetta, and Lucia Mona
Atmos. Chem. Phys., 23, 5487–5516, https://doi.org/10.5194/acp-23-5487-2023, https://doi.org/10.5194/acp-23-5487-2023, 2023
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Multiscale Online Non-hydrostatic AtmospheRe CHemistry model (MONARCH) dust reanalysis provides a high-resolution 3D reconstruction of past dust conditions, allowing better quantification of climate and socioeconomic dust impacts. We assess the performance of the reanalysis needed to reproduce dust optical depth using dust-related products retrieved from satellite and ground-based observations and show that it reproduces the spatial distribution and seasonal variability of atmospheric dust well.
Jacob Z. Tindan, Qinjian Jin, and Bing Pu
Atmos. Chem. Phys., 23, 5435–5466, https://doi.org/10.5194/acp-23-5435-2023, https://doi.org/10.5194/acp-23-5435-2023, 2023
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We use the Infrared Atmospheric Sounder Interferometer (IASI) retrievals of dust variables (dust optical depth and dust layer height) and surface observations to understand the day- and nighttime variations in dust aerosols over the dust belt. Our results show that daytime dust aerosols are significantly different from nighttime, and such day–night variations are influenced by meteorological factors such as wind speed, precipitation, and turbulent motions within the atmospheric boundary layer.
Ross Herbert and Philip Stier
Atmos. Chem. Phys., 23, 4595–4616, https://doi.org/10.5194/acp-23-4595-2023, https://doi.org/10.5194/acp-23-4595-2023, 2023
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We provide robust evidence from multiple sources showing that smoke from fires in the Amazon rainforest significantly modifies the diurnal cycle of convection and cools the climate. Low to moderate amounts of smoke increase deep convective clouds and rain, whilst beyond a threshold amount, the smoke starts to suppress the convection and rain. We are currently at this threshold, suggesting increases in fires from agricultural practices or droughts will reduce cloudiness and rain over the region.
Yue Huang, Jasper F. Kok, Masanori Saito, and Olga Muñoz
Atmos. Chem. Phys., 23, 2557–2577, https://doi.org/10.5194/acp-23-2557-2023, https://doi.org/10.5194/acp-23-2557-2023, 2023
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Global aerosol models and remote sensing retrievals use dust optical models with inconsistent and inaccurate dust shape approximations. Here, we present a new dust optical model constrained by measured dust shape distributions. This new dust optical model is an improvement on the current dust optical models used in models and retrieval algorithms, as quantified by comparisons against laboratory and field observations of dust optics.
Konstantinos Michailidis, Maria-Elissavet Koukouli, Dimitris Balis, J. Pepijn Veefkind, Martin de Graaf, Lucia Mona, Nikolaos Papagianopoulos, Gesolmina Pappalardo, Ioanna Tsikoudi, Vassilis Amiridis, Eleni Marinou, Anna Gialitaki, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Daniele Bortoli, Maria João Costa, Vanda Salgueiro, Alexandros Papayannis, Maria Mylonaki, Lucas Alados-Arboledas, Salvatore Romano, Maria Rita Perrone, and Holger Baars
Atmos. Chem. Phys., 23, 1919–1940, https://doi.org/10.5194/acp-23-1919-2023, https://doi.org/10.5194/acp-23-1919-2023, 2023
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Comparisons with ground-based correlative lidar measurements constitute a key component in the validation of satellite aerosol products. This paper presents the validation of the TROPOMI aerosol layer height (ALH) product, using archived quality assured ground-based data from lidar stations that belong to the EARLINET network. Comparisons between the TROPOMI ALH and co-located EARLINET measurements show good agreement over the ocean.
María Ángeles López-Cayuela, Carmen Córdoba-Jabonero, Diego Bermejo-Pantaleón, Michaël Sicard, Vanda Salgueiro, Francisco Molero, Clara Violeta Carvajal-Pérez, María José Granados-Muñoz, Adolfo Comerón, Flavio T. Couto, Rubén Barragán, María-Paz Zorzano, Juan Antonio Bravo-Aranda, Constantino Muñoz-Porcar, María João Costa, Begoña Artíñano, Alejandro Rodríguez-Gómez, Daniele Bortoli, Manuel Pujadas, Jesús Abril-Gago, Lucas Alados-Arboledas, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 23, 143–161, https://doi.org/10.5194/acp-23-143-2023, https://doi.org/10.5194/acp-23-143-2023, 2023
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An intense Saharan dust outbreak crossing the Iberian Peninsula in springtime was monitored to determinine the specific contribution of fine and coarse dust particles at five lidar stations, strategically covering its SW–central–NE pathway. Expected dust ageing along the transport started unappreciated. A different fine-dust impact on optical (~30 %) and mass (~10 %) properties was found. Use of polarized lidar measurements (mainly in elastic systems) for fine/coarse dust separation is crucial.
Kyriakoula Papachristopoulou, Ioannis-Panagiotis Raptis, Antonis Gkikas, Ilias Fountoulakis, Akriti Masoom, and Stelios Kazadzis
Atmos. Chem. Phys., 22, 15703–15727, https://doi.org/10.5194/acp-22-15703-2022, https://doi.org/10.5194/acp-22-15703-2022, 2022
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Megacities' air quality is determined by atmospheric aerosols. We focus on changes over the last two decades in the 81 largest cities, using satellite data. European and American cities have lower aerosol compared to African and Asian cities. For European, North American and East Asian cities, aerosols are decreasing over time, especially in China and the US. In the remaining cities, aerosol loads are increasing, particularly in India.
Nilton Évora do Rosário, Elisa Thomé Sena, and Marcia Akemi Yamasoe
Atmos. Chem. Phys., 22, 15021–15033, https://doi.org/10.5194/acp-22-15021-2022, https://doi.org/10.5194/acp-22-15021-2022, 2022
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The 2020 burning season in Brazil was marked by an atypically high number of fire spots across Pantanal, leading to high amounts of smoke within the biome. This study shows that smoke over Pantanal, usually a fraction of that over Amazonia, was higher and resulted mainly from fires in conservation and indigenous areas. It also contributes to highlighting Pantanal's 2020 burning season as the worst combination of a climate extreme scenario and inadequately enforced environmental regulations.
Santiago Gassó and Kirk D. Knobelspiesse
Atmos. Chem. Phys., 22, 13581–13605, https://doi.org/10.5194/acp-22-13581-2022, https://doi.org/10.5194/acp-22-13581-2022, 2022
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Atmospheric particles interact with light resulting in observable optical polarization. Thus, we can learn about their composition from space. New satellite sensor technology measures full polarization of reflected sunlight. This paper considers circular polarization, an overlooked category of polarization with distinctive features that could bring new insights. We review existing literature and make novel computations to consider this previously underappreciated category of polarization.
Qingyang Xiao, Guannan Geng, Shigan Liu, Jiajun Liu, Xia Meng, and Qiang Zhang
Atmos. Chem. Phys., 22, 13229–13242, https://doi.org/10.5194/acp-22-13229-2022, https://doi.org/10.5194/acp-22-13229-2022, 2022
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We provided complete coverage PM2.5 concentrations at a 1-km resolution from 2000 to the present, carefully considering the significant changes in land use characteristics in China. This high-resolution PM2.5 data successfully revealed the local-scale PM2.5 variations. We noticed changes in PM2.5 spatial patterns in association with the clean air policies, with the pollution hotspots having transferred from urban centers to rural regions with limited air quality monitoring.
Johannes Quaas, Hailing Jia, Chris Smith, Anna Lea Albright, Wenche Aas, Nicolas Bellouin, Olivier Boucher, Marie Doutriaux-Boucher, Piers M. Forster, Daniel Grosvenor, Stuart Jenkins, Zbigniew Klimont, Norman G. Loeb, Xiaoyan Ma, Vaishali Naik, Fabien Paulot, Philip Stier, Martin Wild, Gunnar Myhre, and Michael Schulz
Atmos. Chem. Phys., 22, 12221–12239, https://doi.org/10.5194/acp-22-12221-2022, https://doi.org/10.5194/acp-22-12221-2022, 2022
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Pollution particles cool climate and offset part of the global warming. However, they are washed out by rain and thus their effect responds quickly to changes in emissions. We show multiple datasets to demonstrate that aerosol emissions and their concentrations declined in many regions influenced by human emissions, as did the effects on clouds. Consequently, the cooling impact on the Earth energy budget became smaller. This change in trend implies a relative warming.
Ukkyo Jeong, Si-Chee Tsay, N. Christina Hsu, David M. Giles, John W. Cooper, Jaehwa Lee, Robert J. Swap, Brent N. Holben, James J. Butler, Sheng-Hsiang Wang, Somporn Chantara, Hyunkee Hong, Donghee Kim, and Jhoon Kim
Atmos. Chem. Phys., 22, 11957–11986, https://doi.org/10.5194/acp-22-11957-2022, https://doi.org/10.5194/acp-22-11957-2022, 2022
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Ultraviolet (UV) measurements from satellite and ground are important for deriving information on several atmospheric trace and aerosol characteristics. Simultaneous retrievals of aerosol and trace gases in this study suggest that water uptake by aerosols is one of the important phenomena affecting aerosol properties over northern Thailand, which is important for regional air quality and climate. Obtained aerosol properties covering the UV are also important for various satellite algorithms.
Abdulaziz Tunde Yakubu and Naven Chetty
Atmos. Chem. Phys., 22, 11065–11087, https://doi.org/10.5194/acp-22-11065-2022, https://doi.org/10.5194/acp-22-11065-2022, 2022
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This study examined the source of atmospheric aerosols and their role in forming clouds and rainfall over South Africa. The research provided answers to the cause of low precipitation, mainly linked to drought and water shortages experienced over the region. Further insight into the cause of occasional flooding that occurs in other parts of the area is provided. Finally, the study described the relationship between aerosol–cloud precipitation based on observation over the region.
África Barreto, Rosa D. García, Carmen Guirado-Fuentes, Emilio Cuevas, A. Fernando Almansa, Celia Milford, Carlos Toledano, Francisco J. Expósito, Juan P. Díaz, and Sergio F. León-Luis
Atmos. Chem. Phys., 22, 11105–11124, https://doi.org/10.5194/acp-22-11105-2022, https://doi.org/10.5194/acp-22-11105-2022, 2022
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A comprehensive characterization of atmospheric aerosols in the subtropical eastern North Atlantic has been carried out in this paper using long-term ground AERONET photometric observations over the period 2005–2020 from a unique network made up of four stations strategically located from sea level to 3555 m height on the island of Tenerife. This is a region that can be considered a key location to study the seasonal dependence of dust transport from the Sahel-Sahara.
Xiaoxi Zhao, Kan Huang, Joshua S. Fu, and Sabur F. Abdullaev
Atmos. Chem. Phys., 22, 10389–10407, https://doi.org/10.5194/acp-22-10389-2022, https://doi.org/10.5194/acp-22-10389-2022, 2022
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Long-range transport of Asian dust to the Arctic was considered an important source of Arctic air pollution. Different transport routes to the Arctic had divergent effects on the evolution of aerosol properties. Depositions of long-range-transported dust particles can reduce the Arctic surface albedo considerably. This study implied that the ubiquitous long-transport dust from China exerted considerable aerosol indirect effects on the Arctic and may have potential biogeochemical significance.
Katherine T. Junghenn Noyes, Ralph A. Kahn, James A. Limbacher, and Zhanqing Li
Atmos. Chem. Phys., 22, 10267–10290, https://doi.org/10.5194/acp-22-10267-2022, https://doi.org/10.5194/acp-22-10267-2022, 2022
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We compare retrievals of wildfire smoke particle size, shape, and light absorption from the MISR satellite instrument to modeling and other satellite data on land cover type, drought conditions, meteorology, and estimates of fire intensity (fire radiative power – FRP). We find statistically significant differences in the particle properties based on burning conditions and land cover type, and we interpret how changes in these properties point to specific aerosol aging mechanisms.
David W. Fillmore, David A. Rutan, Seiji Kato, Fred G. Rose, and Thomas E. Caldwell
Atmos. Chem. Phys., 22, 10115–10137, https://doi.org/10.5194/acp-22-10115-2022, https://doi.org/10.5194/acp-22-10115-2022, 2022
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This paper presents an evaluation of the aerosol analysis incorporated into the Clouds and the Earth's Radiant Energy System (CERES) data products as well as the aerosols' impact on solar radiation reaching the surface. CERES is a NASA Earth observation mission with instruments flying on various polar-orbiting satellites. Its primary objective is the study of the radiative energy balance of the climate system as well as examination of the influence of clouds and aerosols on this balance.
Peng Xian, Jianglong Zhang, Norm T. O'Neill, Travis D. Toth, Blake Sorenson, Peter R. Colarco, Zak Kipling, Edward J. Hyer, James R. Campbell, Jeffrey S. Reid, and Keyvan Ranjbar
Atmos. Chem. Phys., 22, 9915–9947, https://doi.org/10.5194/acp-22-9915-2022, https://doi.org/10.5194/acp-22-9915-2022, 2022
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The study provides baseline Arctic spring and summertime aerosol optical depth climatology, trend, and extreme event statistics from 2003 to 2019 using a combination of aerosol reanalyses, remote sensing, and ground observations. Biomass burning smoke has an overwhelming contribution to black carbon (an efficient climate forcer) compared to anthropogenic sources. Burning's large interannual variability and increasing summer trend have important implications for the Arctic climate.
Harshvardhan Harshvardhan, Richard Ferrare, Sharon Burton, Johnathan Hair, Chris Hostetler, David Harper, Anthony Cook, Marta Fenn, Amy Jo Scarino, Eduard Chemyakin, and Detlef Müller
Atmos. Chem. Phys., 22, 9859–9876, https://doi.org/10.5194/acp-22-9859-2022, https://doi.org/10.5194/acp-22-9859-2022, 2022
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The evolution of aerosol in biomass burning smoke plumes that travel over marine clouds off the Atlantic coast of central Africa was studied using measurements made by a lidar deployed on a high-altitude aircraft. The main finding was that the physical properties of aerosol do not change appreciably once the plume has left land and travels over the ocean over a timescale of 1 to 2 d. Almost all particles in the plume are of radius less than 1 micrometer and spherical in shape.
Peng Xian, Jianglong Zhang, Norm T. O'Neill, Jeffrey S. Reid, Travis D. Toth, Blake Sorenson, Edward J. Hyer, James R. Campbell, and Keyvan Ranjbar
Atmos. Chem. Phys., 22, 9949–9967, https://doi.org/10.5194/acp-22-9949-2022, https://doi.org/10.5194/acp-22-9949-2022, 2022
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The study provides a baseline Arctic spring and summertime aerosol optical depth climatology, trend, and extreme event statistics from 2003 to 2019 using a combination of aerosol reanalyses, remote sensing, and ground observations. Biomass burning smoke has an overwhelming contribution to black carbon (an efficient climate forcer) compared to anthropogenic sources. Burning's large interannual variability and increasing summer trend have important implications for the Arctic climate.
Sudip Chakraborty, Bin Guan, Duane E. Waliser, and Arlindo M. da Silva
Atmos. Chem. Phys., 22, 8175–8195, https://doi.org/10.5194/acp-22-8175-2022, https://doi.org/10.5194/acp-22-8175-2022, 2022
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This study explores extreme aerosol transport events by aerosol atmospheric rivers (AARs) and shows the characteristics of individual AARs such as length, width, length-to-width ratio, transport strength, and dominant transport direction, the seasonal variations, the relationship to the spatial distribution of surface emissions, the vertical profiles of wind, aerosol mixing ratio, and aerosol mass fluxes, and the major planetary-scale aerosol transport pathways.
Guangyao Dai, Kangwen Sun, Xiaoye Wang, Songhua Wu, Xiangying E, Qi Liu, and Bingyi Liu
Atmos. Chem. Phys., 22, 7975–7993, https://doi.org/10.5194/acp-22-7975-2022, https://doi.org/10.5194/acp-22-7975-2022, 2022
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In this paper, a Sahara dust event is tracked with the spaceborne lidars ALADIN and CALIOP and the models ECMWF and HYSPLIT. The performance of ALADIN and CALIOP on tracking the dust event and on the observations of dust optical properties and wind fields during the dust transport is evaluated. The dust mass advection is defined, which is calculated with the combination of data from ALADIN and CALIOP coupled with the products from models to describe the dust transport quantitatively.
Ke Gui, Wenrui Yao, Huizheng Che, Linchang An, Yu Zheng, Lei Li, Hujia Zhao, Lei Zhang, Junting Zhong, Yaqiang Wang, and Xiaoye Zhang
Atmos. Chem. Phys., 22, 7905–7932, https://doi.org/10.5194/acp-22-7905-2022, https://doi.org/10.5194/acp-22-7905-2022, 2022
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This study investigates the aerosol optical and radiative properties and meteorological drivers during two mega SDS events over Northern China in March 2021. The MODIS-retrieved DOD data registered these two events as the most intense episode in the same period in history over the past 20 years. These two extreme SDS events were associated with both atmospheric circulation extremes and local meteorological anomalies that favor enhanced dust emissions in the Gobi Desert.
Manuel Gutleben, Silke Groß, Christian Heske, and Martin Wirth
Atmos. Chem. Phys., 22, 7319–7330, https://doi.org/10.5194/acp-22-7319-2022, https://doi.org/10.5194/acp-22-7319-2022, 2022
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The main transportation route of Saharan mineral dust particles leads over the subtropical Atlantic Ocean and is subject to a seasonal variation. This study investigates the characteristics of wintertime transatlantic dust transport towards the Caribbean by means of airborne lidar measurements. It is found that dust particles are transported at low atmospheric altitudes (<3.5 km) embedded in a relatively moist mixture with two other particle types, namely marine and biomass-burning particles.
Goutam Choudhury, Albert Ansmann, and Matthias Tesche
Atmos. Chem. Phys., 22, 7143–7161, https://doi.org/10.5194/acp-22-7143-2022, https://doi.org/10.5194/acp-22-7143-2022, 2022
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Lidars provide height-resolved type-specific aerosol properties and are key in studying vertically collocated aerosols and clouds. In this study, we compare the aerosol number concentrations derived from spaceborne lidar with the in situ flight measurements. Our results show a reasonable agreement between both datasets. Such an agreement has not been achieved yet. It shows the potential of spaceborne lidar in studying aerosol–cloud interactions, which is needed to improve our climate forecasts.
Nair K. Kala, Narayana Sarma Anand, Mohanan R. Manoj, Harshavardhana S. Pathak, Krishnaswamy K. Moorthy, and Sreedharan K. Satheesh
Atmos. Chem. Phys., 22, 6067–6085, https://doi.org/10.5194/acp-22-6067-2022, https://doi.org/10.5194/acp-22-6067-2022, 2022
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We present the 3-D distribution of atmospheric aerosols and highlight its variation with respect to longitudes over the Indian mainland and the surrounding oceans using long-term satellite observations and realistic synthesised data. The atmospheric heating due to the 3-D distribution of aerosols is estimated using radiative transfer calculations. We believe that our findings will have strong implications for aerosol–radiation interactions in regional climate simulations.
Archana Devi and Sreedharan K. Satheesh
Atmos. Chem. Phys., 22, 5365–5376, https://doi.org/10.5194/acp-22-5365-2022, https://doi.org/10.5194/acp-22-5365-2022, 2022
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Global maps of aerosol absorption were generated using a multi-satellite retrieval algorithm. The retrieved values were validated with available aircraft-based measurements and compared with other global datasets. Seasonal and spatial distributions of aerosol absorption over various regions are also presented. The global maps of single scattering albedo with improved accuracy provide important input to climate models for assessing the climatic impact of aerosols on regional and global scales.
Qiaoyun Hu, Philippe Goloub, Igor Veselovskii, and Thierry Podvin
Atmos. Chem. Phys., 22, 5399–5414, https://doi.org/10.5194/acp-22-5399-2022, https://doi.org/10.5194/acp-22-5399-2022, 2022
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Our lidar observations show that the optical properties of wildfire smoke particles are highly varied after long-range transport. The variabilities are probably relevant to vegetation type, combustion condition and the aging process, which alter the smoke particle properties, as well as their impact on cloud processes and properties. The lidar fluorescence channel provides a good opportunity for smoke characterization and heterogenous ice crystal formation.
Igor Veselovskii, Qiaoyun Hu, Albert Ansmann, Philippe Goloub, Thierry Podvin, and Mikhail Korenskiy
Atmos. Chem. Phys., 22, 5209–5221, https://doi.org/10.5194/acp-22-5209-2022, https://doi.org/10.5194/acp-22-5209-2022, 2022
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A remote sensing method based on fluorescence lidar measurements can detect and quantify the smoke content in the upper troposphere and inside cirrus clouds. Based on two case studies, we demonstrate that the fluorescence lidar technique provides the possibility to estimate the smoke surface area concentration within freshly formed cirrus layers. This value was used in a smoke ice nucleating particle parameterization scheme to predict ice crystal number concentrations in cirrus generation cells.
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Short summary
Dust Aerosol Observation-Kashi (DAO-K) campaign was conducted near the Taklimakan Desert in April 2019 to obtain comprehensive aerosol, atmosphere, and surface parameters. Estimations of aerosol solar radiative forcing by a radiative transfer (RT) model were improved based on the measured aerosol parameters, additionally considering atmospheric profiles and diurnal variations of surface albedo. RT simulations agree well with simultaneous irradiance observations, even in dust-polluted conditions.
Dust Aerosol Observation-Kashi (DAO-K) campaign was conducted near the Taklimakan Desert in...
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