Articles | Volume 18, issue 4
https://doi.org/10.5194/acp-18-2601-2018
https://doi.org/10.5194/acp-18-2601-2018
Research article
 | 
22 Feb 2018
Research article |  | 22 Feb 2018

Effects of temperature-dependent NOx emissions on continental ozone production

Paul S. Romer, Kaitlin C. Duffey, Paul J. Wooldridge, Eric Edgerton, Karsten Baumann, Philip A. Feiner, David O. Miller, William H. Brune, Abigail R. Koss, Joost A. de Gouw, Pawel K. Misztal, Allen H. Goldstein, and Ronald C. Cohen

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Cited articles

Atkinson, R., Baulch, D. L., Cox, R. A., Crowley, J. N., Hampson, R. F., Hynes, R. G., Jenkin, M. E., Rossi, M. J., Troe, J., and IUPAC Subcommittee: Evaluated kinetic and photochemical data for atmospheric chemistry: Volume II – gas phase reactions of organic species, Atmos. Chem. Phys., 6, 3625–4055, https://doi.org/10.5194/acp-6-3625-2006, 2006. a
Atkinson, R. W., Yu, D., Armstrong, B. G., Pattenden, S., Wilkinson, P., Doherty, R. M., Heal, M. R., and Anderson, H. R.: Concentration–Response Function for Ozone and Daily Mortality: Results from Five Urban and Five Rural U.K. Populations, Environ. Health Persp., 120, 1411–1417, 2012. a
Ayres, B. R., Allen, H. M., Draper, D. C., Brown, S. S., Wild, R. J., Jimenez, J. L., Day, D. A., Campuzano-Jost, P., Hu, W., de Gouw, J., Koss, A., Cohen, R. C., Duffey, K. C., Romer, P., Baumann, K., Edgerton, E., Takahama, S., Thornton, J. A., Lee, B. H., Lopez-Hilfiker, F. D., Mohr, C., Wennberg, P. O., Nguyen, T. B., Teng, A., Goldstein, A. H., Olson, K., and Fry, J. L.: Organic nitrate aerosol formation via NO3+ biogenic volatile organic compounds in the southeastern United States, Atmos. Chem. Phys., 15, 13377–13392, https://doi.org/10.5194/acp-15-13377-2015, 2015. a
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Baumann, K., Williams, E. J., Angevine, W. M., Roberts, J. M., Norton, R. B., Frost, G. J., Fehsenfeld, F. C., Springston, S. R., Bertman, S. B., and Hartsell, B.: Ozone production and transport near Nashville, Tennessee: Results from the 1994 study at New Hendersonville, J. Geophys. Res., 105, 9137–9153, https://doi.org/10.1029/1999JD901017, 2000. a, b
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Short summary
Observations of increased ozone on hotter days are widely reported, but the mechanisms driving this relationship remain uncertain. We use measurements from the rural southeastern United States to study how temperature affects ozone production. We find that changing NOx emissions, most likely from soil microbes, can be a major driver of increased ozone with temperature in the continental background. These findings suggest that ozone will increase with temperature under a wide range of conditions.
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