Articles | Volume 17, issue 12
https://doi.org/10.5194/acp-17-7853-2017
https://doi.org/10.5194/acp-17-7853-2017
Research article
 | 
29 Jun 2017
Research article |  | 29 Jun 2017

Estimation of the Paris NOx emissions from mobile MAX-DOAS observations and CHIMERE model simulations during the MEGAPOLI campaign using the closed integral method

Reza Shaiganfar, Steffen Beirle, Hugo Denier van der Gon, Sander Jonkers, Jeroen Kuenen, Herve Petetin, Qijie Zhang, Matthias Beekmann, and Thomas Wagner

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Cited articles

Airparif: Ile-de-France gridded emission inventory 2005 (version2008), http://www.airparif.asso.fr/ (last access: 19 June 2017), 2010.
Beirle, S., Boersma, F., Platt, U., Lawrence, M. G., and Wagner, T.: Megacity emissions and lifetimes of nitrogen oxides probes from space, Science, 333, 1737–1739, https://doi.org/10.1126/science.1207824, 2011.
Denier van der Gon, H. A. C., Beevers, S., D'Allura, A., Finardi, S., Honoré, C., Kuenen, J., Perrussel, O., Radice, P., Theloke, J., Uzbasich, M., and Visschedijk, A.: Discrepancies Between Top-Down and Bottom-Up Emission Inventories of Megacities: The Causes and Relevance for Modeling Concentrations and Exposure, in: Air Pollution Modeling and its Application XXI, NATO Science for Peace and Security Series C: Environmental Security, edited by: Steyn D. and Trini Castelli, S., Springer, Dordrecht, 2011.
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We determine NOx emissions for Paris in summer 2009 and winter 2009/2010 by combining car MAX-DOAS measurements of NO2 with wind fields. We compare the results with simulations from the CHIMERE model. We derive daily average NOx emissions for Paris of 4.0 × 1025 molecules s−1 for summer and of 6.9 × 1025 molecules s−1 in winter. These values are a factor of about 1.4 and 2.0 larger than the corresponding emissions in the MACC-III emission inventory.
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