Articles | Volume 16, issue 3
https://doi.org/10.5194/acp-16-1773-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-1773-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
15 Feb 2016
Research article |
| 15 Feb 2016
An exemplary case of a bromine explosion event linked to cyclone development in the Arctic
A.-M. Blechschmidt
CORRESPONDING AUTHOR
Institute of Environmental Physics, University of Bremen, Bremen, Germany
A. Richter
Institute of Environmental Physics, University of Bremen, Bremen, Germany
J. P. Burrows
Institute of Environmental Physics, University of Bremen, Bremen, Germany
L. Kaleschke
Institute of Oceanography, University of Hamburg, Hamburg, Germany
K. Strong
Department of Physics, University of Toronto, Toronto, Ontario, Canada
N. Theys
Belgian Institute for Space Aeronomy (IASB-BIRA), Brussels, Belgium
Institute of Environmental Physics, University of Bremen, Bremen, Germany
Department of Physics, University of Toronto, Toronto, Ontario, Canada
A. Zien
Institute of Environmental Physics, University of Bremen, Bremen, Germany
now at: Energy & Meteo Systems GmbH, Oldenburg, Germany
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FOCAL-CO2M is one of the three operational retrieval algorithms which will be used to derive XCO2 and XCH4 from measurements of the forthcoming European CO2M mission. We present results of applications of FOCAL-CO2M to simulated spectra, from which confidence is gained that the algorithm is able to fulfil the challenging requirements on systematic errors for the CO2M mission (spatio-temporal bias ≤ 0.5 ppm for XCO2 and ≤ 5 ppb for XCH4).
Andrea Orfanoz-Cheuquelaf, Carlo Arosio, Alexei Rozanov, Mark Weber, Annette Ladstätter-Weißenmayer, John P. Burrows, Anne M. Thompson, Ryan M. Stauffer, and Debra E. Kollonige
Atmos. Meas. Tech., 17, 1791–1809, https://doi.org/10.5194/amt-17-1791-2024, https://doi.org/10.5194/amt-17-1791-2024, 2024
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Valuable information on the tropospheric ozone column (TrOC) can be obtained globally by combining space-borne limb and nadir measurements (limb–nadir matching, LNM). This study describes the retrieval of TrOC from the OMPS instrument (since 2012) using the LNM technique. The OMPS-LNM TrOC was compared with ozonesondes and other satellite measurements, showing a good agreement with a negative bias within 1 to 4 DU. This new dataset is suitable for pollution studies.
Kezia Lange, Andreas Richter, Tim Bösch, Bianca Zilker, Miriam Latsch, Lisa K. Behrens, Chisom M. Okafor, Hartmut Bösch, John P. Burrows, Alexis Merlaud, Gaia Pinardi, Caroline Fayt, Martina M. Friedrich, Ermioni Dimitropoulou, Michel Van Roozendael, Steffen Ziegler, Simona Ripperger-Lukosiunaite, Leon Kuhn, Bianca Lauster, Thomas Wagner, Hyunkee Hong, Donghee Kim, Lim-Seok Chang, Kangho Bae, Chang-Keun Song, and Hanlim Lee
EGUsphere, https://doi.org/10.5194/egusphere-2024-617, https://doi.org/10.5194/egusphere-2024-617, 2024
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Instruments for air quality observations on geostationary satellites provide multiple observations per day and allow for the analysis of the diurnal variation of important air pollutants such as nitrogen dioxide (NO2) over large areas. The South Korean instrument GEMS, launched in February 2020, is the first instrument in geostationary orbit and covers a large part of Asia. Our investigations show the observed diurnal evolution of NO2 at different measurement sites.
Viktoria F. Sofieva, Alexei Rozanov, Monika Szelag, John P. Burrows, Christian Retscher, Robert Damadeo, Doug Degenstein, Landon A. Rieger, and Adam Bourassa
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2023-538, https://doi.org/10.5194/essd-2023-538, 2024
Preprint under review for ESSD
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Climate-related studies need information about the distribution of stratospheric aerosols, which influence the energy balance of the Earth’s atmosphere. In this work, we present a merged dataset of vertically resolved stratospheric aerosol extinction coefficients, which is derived from data by six limb and occultation satellite instruments. The created aerosol climate record covers the period from October 1984 until May 2022. It can be used in various climate-related studies.
Luisa von Albedyll, Stefan Hendricks, Nils Hutter, Dmitrii Murashkin, Lars Kaleschke, Sascha Willmes, Linda Thielke, Xiangshan Tian-Kunze, Gunnar Spreen, and Christian Haas
The Cryosphere, 18, 1259–1285, https://doi.org/10.5194/tc-18-1259-2024, https://doi.org/10.5194/tc-18-1259-2024, 2024
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Leads (openings in sea ice cover) are created by sea ice dynamics. Because they are important for many processes in the Arctic winter climate, we aim to detect them with satellites. We present two new techniques to detect lead widths of a few hundred meters at high spatial resolution (700 m) and independent of clouds or sun illumination. We use the MOSAiC drift 2019–2020 in the Arctic for our case study and compare our new products to other existing lead products.
Seunghwan Seo, Si-Wan Kim, Kyoung-Min Kim, Andreas Richter, Kezia Lange, John Philip Burrows, Junsung Park, Hyunkee Hong, Hanlim Lee, Ukkyo Jeong, and Jhoon Kim
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2024-33, https://doi.org/10.5194/amt-2024-33, 2024
Preprint under review for AMT
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Over the Seoul Metropolitan Area, GEMS tropospheric NO2 vertical column densities (NO2 TropVCD) show distinct seasonal characteristics, including the absolute values and diurnal patterns. Also, varying a priori data have the substantial impacts on the GEMS NO2 TropVCD. The a priori data from different CTMs resulted in differences of up to 19.2 %. Notably, diurnal patterns of VCDs are similar for all datasets, although theri a priori data exhibit contrasting diurnal patterns.
Adrien Deroubaix, Marco Vountas, Benjamin Gaubert, Maria Dolores Andrés Hernández, Stephan Borrmann, Guy Brasseur, Bruna Holanda, Yugo Kanaya, Katharina Kaiser, Flora Kluge, Ovid Oktavian Krüger, Inga Labuhn, Michael Lichtenstern, Klaus Pfeilsticker, Mira Pöhlker, Hans Schlager, Johannes Schneider, Guillaume Siour, Basudev Swain, Paolo Tuccella, Kameswara S. Vinjamuri, Mihalis Vrekoussis, Benjamin Weyland, and John P. Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2024-516, https://doi.org/10.5194/egusphere-2024-516, 2024
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This study assesses atmospheric composition using air quality models during aircraft campaigns in Europe and Asia, focusing on carbonaceous aerosols and trace gases. While carbon monoxide is well modeled, other pollutants have moderate to weak agreement with observations. Wind speed modeling is reliable for identifying pollution plumes, where models tend to overestimate concentrations. This highlights challenges in accurately modeling aerosol and trace gas composition, particularly in cities.
Adrien Deroubaix, Marco Vountas, Benjamin Gaubert, Maria Dolores Andrés Hernández, Stephan Borrmann, Guy Brasseur, Bruna Holanda, Yugo Kanaya, Katharina Kaiser, Flora Kluge, Ovid Oktavian Krüger, Inga Labuhn, Michael Lichtenstern, Klaus Pfeilsticker, Mira Pöhlker, Hans Schlager, Johannes Schneider, Guillaume Siour, Basudev Swain, Paolo Tuccella, Kameswara S. Vinjamuri, Mihalis Vrekoussis, Benjamin Weyland, and John P. Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2024-521, https://doi.org/10.5194/egusphere-2024-521, 2024
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This study explores the proportional relationships between carbonaceous aerosols (black and organic carbon) and trace gases using airborne measurements from two campaigns in Europe and East Asia. Differences between regions were found, but air quality models struggled to reproduce them accurately. We show that these proportional relationships can help to constrain models and can be used to infer aerosol concentrations from satellite observations of trace gases, especially in urban areas.
Xiaoyi Zhao, Vitali Fioletov, Debora Griffin, Chris McLinden, Ralf Staebler, Cristian Mihele, Kevin Strawbridge, Jonathan Davies, Ihab Abboud, Sum Chi Lee, Alexander Cede, Martin Tiefengraber, and Robert Swap
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2024-27, https://doi.org/10.5194/amt-2024-27, 2024
Preprint under review for AMT
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This study explores differences between remote sensing and in situ instruments in terms of their vertical, horizontal, and temporal sampling differences. Understanding and resolving these differences are critical for future analyses linking satellite, ground-based remote sensing, and in situ observations in air quality monitoring. It shows the meteorological conditions (wind directions, speed, and boundary layer conditions) will strongly affect the agreement between the two measurements.
Swathi Maratt Satheesan, Kai-Uwe Eichmann, John P. Burrows, Mark Weber, Ryan Stauffer, Anne M. Thompson, and Debra Kollonige
EGUsphere, https://doi.org/10.5194/egusphere-2023-2825, https://doi.org/10.5194/egusphere-2023-2825, 2024
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CHORA, an advanced CCD technique, enhances the accuracy of tropospheric ozone retrievals. Unlike the traditional Pacific cloud reference sector (CPC) scheme, CHORA introduces a local cloud reference sector (CLC ) and an alternative approach (CLCT) for precision. Analysing monthly averaged TROPOMI data from 2018 to 2022 and validating with SHADOZ ozonesonde data, CLCT outperforms other methods, emerging as the preferred choice, especially in future geostationary satellite missions.
Jean-François Müller, Trissevgeni Stavrakou, Glenn-Michael Oomen, Beata Opacka, Isabelle De Smedt, Alex Guenther, Corinne Vigouroux, Bavo Langerock, Carlos Augusto Bauer Aquino, Michel Grutter, James Hannigan, Frank Hase, Rigel Kivi, Erik Lutsch, Emmanuel Mahieu, Maria Makarova, Jean-Marc Metzger, Isamu Morino, Isao Murata, Tomoo Nagahama, Justus Notholt, Ivan Ortega, Mathias Palm, Amelie Röhling, Wolfgang Stremme, Kimberly Strong, Ralf Sussmann, Yao Té, and Alan Fried
Atmos. Chem. Phys., 24, 2207–2237, https://doi.org/10.5194/acp-24-2207-2024, https://doi.org/10.5194/acp-24-2207-2024, 2024
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Formaldehyde observations from satellites can be used to constrain the emissions of volatile organic compounds, but those observations have biases. Using an atmospheric model, aircraft and ground-based remote sensing data, we quantify these biases, propose a correction to the data, and assess the consequence of this correction for the evaluation of emissions.
Blanca Fuentes Andrade, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, Andreas Richter, Hartmut Boesch, and John P. Burrows
Atmos. Meas. Tech., 17, 1145–1173, https://doi.org/10.5194/amt-17-1145-2024, https://doi.org/10.5194/amt-17-1145-2024, 2024
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We developed a method to estimate CO2 emissions from localized sources, such as power plants, using satellite data and applied it to estimate CO2 emissions from the Bełchatów Power Station (Poland). As the detection of CO2 emission plumes from satellite data is difficult, we used observations of co-emitted NO2 to constrain the emission plume region. Our results agree with CO2 emission estimations based on the power-plant-generated power and emission factors.
Steffen Vanselow, Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, Hartmut Boesch, and John P. Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2024-379, https://doi.org/10.5194/egusphere-2024-379, 2024
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We developed an algorithm to automatically detect persistent methane source regions, to quantify their emissions and to determine their source types, by analyzing TROPOMI data from 2018–2021. The over 200 globally detected natural and anthropogenic source regions include small-scale point sources such as individual coal mines and larger-scale source regions such as wetlands and large oil and gas fields.
Alexei Rozanov, Christine Pohl, Carlo Arosio, Adam Bourassa, Klaus Bramstedt, Elizaveta Malinina, Landon Rieger, and John P. Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2024-358, https://doi.org/10.5194/egusphere-2024-358, 2024
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We developed a new algorithm to retrieve vertical distributions of the aerosol extinction coefficient in the stratosphere. The algorithm is applied to measurements of the scattered solar light form the space borne OMPS-LP (Ozone Mapping and Profiler Suite-Limb Profiler) instrument. The retrieval results are compared to the data from other space borne instruments and used to investigate the evolution of the aerosol plume after the eruption of the Hunga Tonga-Hunga Ha'apai volcano in January 2022.
Henk Eskes, Athanasios Tsikerdekis, Melanie Ades, Mihai Alexe, Anna Carlin Benedictow, Yasmine Bennouna, Lewis Blake, Idir Bouarar, Simon Chabrillat, Richard Engelen, Quentin Errera, Johannes Flemming, Sebastien Garrigues, Jan Griesfeller, Vincent Huijnen, Luka Ilic, Antje Inness, John Kapsomenakis, Zak Kipling, Bavo Langerock, Augustin Mortier, Mark Parrington, Isabelle Pison, Mikko Pitkanen, Samuel Remy, Andreas Richter, Anja Schoenhardt, Michael Schulz, Valerie Thouret, Thorsten Warneke, Christos Zerefos, and Vincent-Henri Peuch
EGUsphere, https://doi.org/10.5194/egusphere-2023-3129, https://doi.org/10.5194/egusphere-2023-3129, 2024
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The Copernicus Atmosphere Monitoring Service (CAMS) provides global analyses and forecasts of aerosols and trace gases in the atmosphere. On 27/06/2023 a major upgrade, Cy48R1, became operational. Comparisons with in situ, surface remote sensing, aircraft, balloon and satellite observations, show that the new CAMS system is a significant improvement. The results quantify the skill of CAMS to forecast impactful events, such as wildfires, dust storms and air pollution peaks.
Falco Monsees, Alexei Rozanov, John P. Burrows, Mark Weber, Annette Rinke, Ralf Jaiser, and Peter von der Gathen
EGUsphere, https://doi.org/10.5194/egusphere-2023-3036, https://doi.org/10.5194/egusphere-2023-3036, 2024
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Cyclones strongly influence weather predictability, but still cannot be fully characterized in the Arctic because of the sparse coverage of measurements. A potential approach to compensate this sparse coverage is the use of satellite measurements of ozone, because cyclones impact the tropopause and therefore also ozone. In this study we used this connection to investigate the correlation between ozone and the tropopause in the Arctic and to identify cyclones with satellite ozone observations.
Victoria A. Flood, Kimberly Strong, Cynthia H. Whaley, Kaley A. Walker, Thomas Blumenstock, James W. Hannigan, Johan Mellqvist, Justus Notholt, Mathias Palm, Amelie N. Röhling, Stephen Arnold, Stephen Beagley, Rong-You Chien, Jesper Christensen, Makoto Deushi, Srdjan Dobricic, Xinyi Dong, Joshua S. Fu, Michael Gauss, Wanmin Gong, Joakim Langner, Kathy S. Law, Louis Marelle, Tatsuo Onishi, Naga Oshima, David A. Plummer, Luca Pozzoli, Jean-Christophe Raut, Manu A. Thomas, Svetlana Tsyro, and Steven Turnock
Atmos. Chem. Phys., 24, 1079–1118, https://doi.org/10.5194/acp-24-1079-2024, https://doi.org/10.5194/acp-24-1079-2024, 2024
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It is important to understand the composition of the Arctic atmosphere and how it is changing. Atmospheric models provide simulations that can inform policy. This study examines simulations of CH4, CO, and O3 by 11 models. Model performance is assessed by comparing results matched in space and time to measurements from five high-latitude ground-based infrared spectrometers. This work finds that models generally underpredict the concentrations of these gases in the Arctic troposphere.
Basudev Swain, Marco Vountas, Adrien Deroubaix, Luca Lelli, Yanick Ziegler, Soheila Jafariserajehlou, Sachin S. Gunthe, Andreas Herber, Christoph Ritter, Hartmut Bösch, and John P. Burrows
Atmos. Meas. Tech., 17, 359–375, https://doi.org/10.5194/amt-17-359-2024, https://doi.org/10.5194/amt-17-359-2024, 2024
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Aerosols are suspensions of particles dispersed in the air. In this study, we use a novel retrieval of satellite data to investigate an optical property of aerosols, the aerosol optical depth, in the high Arctic to assess their direct and indirect roles in climate change. This study demonstrates that the presented approach shows good quality and very promising potential.
Jonas Hachmeister, Oliver Schneising, Michael Buchwitz, John P. Burrows, Justus Notholt, and Matthias Buschmann
Atmos. Chem. Phys., 24, 577–595, https://doi.org/10.5194/acp-24-577-2024, https://doi.org/10.5194/acp-24-577-2024, 2024
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We quantified changes in atmospheric methane concentrations using satellite data and a dynamic linear model approach. We calculated global annual methane increases for the years 2019–2022, which are in good agreement with other sources. For zonal methane growth rates, we identified strong inter-hemispheric differences in 2019 and 2022. For 2022, we could attribute decreases in the global growth rate to the Northern Hemisphere, possibly related to a reduction in anthropogenic emissions.
Glenn-Michael Oomen, Jean-François Müller, Trissevgeni Stavrakou, Isabelle De Smedt, Thomas Blumenstock, Rigel Kivi, Maria Makarova, Mathias Palm, Amelie Röhling, Yao Té, Corinne Vigouroux, Martina M. Friedrich, Udo Frieß, François Hendrick, Alexis Merlaud, Ankie Piters, Andreas Richter, Michel Van Roozendael, and Thomas Wagner
Atmos. Chem. Phys., 24, 449–474, https://doi.org/10.5194/acp-24-449-2024, https://doi.org/10.5194/acp-24-449-2024, 2024
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Natural emissions from vegetation have a profound impact on air quality for their role in the formation of harmful tropospheric ozone and organic aerosols, yet these emissions are highly uncertain. In this study, we quantify emissions of organic gases over Europe using high-quality satellite measurements of formaldehyde. These satellite observations suggest that emissions from vegetation are much higher than predicted by models, especially in southern Europe.
Andrea Pazmiño, Florence Goutail, Sophie Godin-Beekmann, Alain Hauchecorne, Jean-Pierre Pommereau, Martyn P. Chipperfield, Wuhu Feng, Franck Lefèvre, Audrey Lecouffe, Michel Van Roozendael, Nis Jepsen, Georg Hansen, Rigel Kivi, Kimberly Strong, and Kaley A. Walker
Atmos. Chem. Phys., 23, 15655–15670, https://doi.org/10.5194/acp-23-15655-2023, https://doi.org/10.5194/acp-23-15655-2023, 2023
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The vortex-averaged ozone loss over the last 3 decades is evaluated for both polar regions using the passive ozone tracer of the chemical transport model TOMCAT/SLIMCAT and total ozone observations from the SAOZ network and MSR2 reanalysis. Three metrics were developed to compute ozone trends since 2000. The study confirms the ozone recovery in the Antarctic and shows a potential sign of quantitative detection of ozone recovery in the Arctic that needs to be robustly confirmed in the future.
Vitali E. Fioletov, Chris A. McLinden, Debora Griffin, Nickolay A. Krotkov, Can Li, Joanna Joiner, Nicolas Theys, and Simon Carn
Atmos. Meas. Tech., 16, 5575–5592, https://doi.org/10.5194/amt-16-5575-2023, https://doi.org/10.5194/amt-16-5575-2023, 2023
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Snow-covered terrain, with its high reflectance in the UV, typically enhances satellite sensitivity to boundary layer pollution. However, a significant fraction of high-quality cloud-free measurements over snow is currently excluded from analyses. In this study, we investigated how satellite SO2 measurements over snow-covered surfaces can be used to improve estimations of annual SO2 emissions.
Michael Kiefer, Dale F. Hurst, Gabriele P. Stiller, Stefan Lossow, Holger Vömel, John Anderson, Faiza Azam, Jean-Loup Bertaux, Laurent Blanot, Klaus Bramstedt, John P. Burrows, Robert Damadeo, Bianca Maria Dinelli, Patrick Eriksson, Maya García-Comas, John C. Gille, Mark Hervig, Yasuko Kasai, Farahnaz Khosrawi, Donal Murtagh, Gerald E. Nedoluha, Stefan Noël, Piera Raspollini, William G. Read, Karen H. Rosenlof, Alexei Rozanov, Christopher E. Sioris, Takafumi Sugita, Thomas von Clarmann, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 16, 4589–4642, https://doi.org/10.5194/amt-16-4589-2023, https://doi.org/10.5194/amt-16-4589-2023, 2023
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We quantify biases and drifts (and their uncertainties) between the stratospheric water vapor measurement records of 15 satellite-based instruments (SATs, with 31 different retrievals) and balloon-borne frost point hygrometers (FPs) launched at 27 globally distributed stations. These comparisons of measurements during the period 2000–2016 are made using robust, consistent statistical methods. With some exceptions, the biases and drifts determined for most SAT–FP pairs are < 10 % and < 1 % yr−1.
Vitali Fioletov, Xiaoyi Zhao, Ihab Abboud, Michael Brohart, Akira Ogyu, Reno Sit, Sum Chi Lee, Irina Petropavlovskikh, Koji Miyagawa, Bryan J. Johnson, Patrick Cullis, John Booth, Glen McConville, and C. Thomas McElroy
Atmos. Chem. Phys., 23, 12731–12751, https://doi.org/10.5194/acp-23-12731-2023, https://doi.org/10.5194/acp-23-12731-2023, 2023
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Stratospheric ozone within the Southern Hemisphere springtime polar vortex has been a subject of intense research since the discovery of the Antarctic ozone hole. The wintertime ozone in the vortex is less studied. We show that the recent wintertime ozone values over the South Pole were about 12 % below the pre-1980s level; i.e., the decline there was nearly twice as large as that over southern midlatitudes. Thus, wintertime ozone there can be used as an indicator of the ozone layer state.
Bianca Zilker, Andreas Richter, Anne-Marlene Blechschmidt, Peter von der Gathen, Ilias Bougoudis, Sora Seo, Tim Bösch, and John Philip Burrows
Atmos. Chem. Phys., 23, 9787–9814, https://doi.org/10.5194/acp-23-9787-2023, https://doi.org/10.5194/acp-23-9787-2023, 2023
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During Arctic spring, near-surface ozone is depleted by bromine released from salty sea ice and/or snow-covered areas under certain meteorological conditions. To study this ozone depletion and the prevailing meteorological conditions, two ozone data sets from Ny-Ålesund, Svalbard, have been evaluated. We found that during ozone depletion events lower pressure over the Barents Sea and higher pressure in the Icelandic Low area led to a transport of cold polar air from the north to Ny-Ålesund.
Shoma Yamanouchi, Stephanie Conway, Kimberly Strong, Orfeo Colebatch, Erik Lutsch, Sébastien Roche, Jeffrey Taylor, Cynthia H. Whaley, and Aldona Wiacek
Earth Syst. Sci. Data, 15, 3387–3418, https://doi.org/10.5194/essd-15-3387-2023, https://doi.org/10.5194/essd-15-3387-2023, 2023
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Nineteen years of atmospheric composition measurements made at the University of Toronto Atmospheric Observatory (TAO; 43.66° N, 79.40° W; 174 m.a.s.l.) are presented. These are retrieved from Fourier transform infrared (FTIR) solar absorption spectra recorded with a spectrometer from May 2002 to December 2020. The retrievals have been optimized for fourteen species: O3, HCl, HF, HNO3, CH4, C2H6, CO, HCN, N2O, C2H2, H2CO, CH3OH, HCOOH, and NH3.
Midhun George, Maria Dolores Andrés Hernández, Vladyslav Nenakhov, Yangzhuoran Liu, John Philip Burrows, Birger Bohn, Eric Förster, Florian Obersteiner, Andreas Zahn, Theresa Harlaß, Helmut Ziereis, Hans Schlager, Benjamin Schreiner, Flora Kluge, Katja Bigge, and Klaus Pfeilsticker
Atmos. Chem. Phys., 23, 7799–7822, https://doi.org/10.5194/acp-23-7799-2023, https://doi.org/10.5194/acp-23-7799-2023, 2023
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The applicability of photostationary steady-state (PSS) assumptions to estimate the amount of the sum of peroxy radicals (RO2*) during the EMeRGe airborne observations from the known radical chemistry and onboard measurements of RO2* precursors, photolysis frequencies, and other trace gases such as NOx and O3 was investigated. The comparison of the calculated RO2* with the actual measurements provides an insight into the main processes controlling their concentration in the air masses measured.
Haokui Xu, Brooke Medley, Leung Tsang, Joel T. Johnson, Kenneth C. Jezek, Macro Brogioni, and Lars Kaleschke
The Cryosphere, 17, 2793–2809, https://doi.org/10.5194/tc-17-2793-2023, https://doi.org/10.5194/tc-17-2793-2023, 2023
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The density profile of polar ice sheets is a major unknown in estimating the mass loss using lidar tomography methods. In this paper, we show that combing the active radar data and passive radiometer data can provide an estimation of density properties using the new model we implemented in this paper. The new model includes the short and long timescale variations in the firn and also the refrozen layers which are not included in the previous modeling work.
Kameswara S. Vinjamuri, Marco Vountas, Luca Lelli, Martin Stengel, Matthew D. Shupe, Kerstin Ebell, and John P. Burrows
Atmos. Meas. Tech., 16, 2903–2918, https://doi.org/10.5194/amt-16-2903-2023, https://doi.org/10.5194/amt-16-2903-2023, 2023
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Clouds play an important role in Arctic amplification. Cloud data from ground-based sites are valuable but cannot represent the whole Arctic. Therefore the use of satellite products is a measure to cover the entire Arctic. However, the quality of such cloud measurements from space is not well known. The paper discusses the differences and commonalities between satellite and ground-based measurements. We conclude that the satellite dataset, with a few exceptions, can be used in the Arctic.
Basudev Swain, Marco Vountas, Adrien Deroubaix, Luca Lelli, Aishwarya Singh, Yanick Ziegler, Sachin S. Gunthe, and John P. Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2023-730, https://doi.org/10.5194/egusphere-2023-730, 2023
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Aerosols are suspensions of particles distributed in the air. Depending on their chemical composition, they scatter and/or absorb sunlight and thus cool or warm the earth's atmosphere and its surface. They also provide as a surface in the atmosphere upon which ice or liquid clouds droplets nucleate and grow. In this study, we use satellite observations and model simulations to investigate the properties of aerosols with the goal of assessing their direct and indirect role in climate change.
Yifan Guan, Gretchen Keppel-Aleks, Scott C. Doney, Christof Petri, Dave Pollard, Debra Wunch, Frank Hase, Hirofumi Ohyama, Isamu Morino, Justus Notholt, Kei Shiomi, Kim Strong, Rigel Kivi, Matthias Buschmann, Nicholas Deutscher, Paul Wennberg, Ralf Sussmann, Voltaire A. Velazco, and Yao Té
Atmos. Chem. Phys., 23, 5355–5372, https://doi.org/10.5194/acp-23-5355-2023, https://doi.org/10.5194/acp-23-5355-2023, 2023
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We characterize spatial–temporal patterns of interannual variability (IAV) in atmospheric CO2 based on NASA’s Orbiting Carbon Observatory-2 (OCO-2). CO2 variation is strongly impacted by climate events, with higher anomalies during El Nino years. We show high correlation in IAV between space-based and ground-based CO2 from long-term sites. Because OCO-2 has near-global coverage, our paper provides a roadmap to study IAV where in situ observation is sparse, such as open oceans and remote lands.
Xiaoyi Zhao, Vitali Fioletov, Alberto Redondas, Julian Gröbner, Luca Egli, Franz Zeilinger, Javier López-Solano, Alberto Berjón Arroyo, James Kerr, Eliane Maillard Barras, Herman Smit, Michael Brohart, Reno Sit, Akira Ogyu, Ihab Abboud, and Sum Chi Lee
Atmos. Meas. Tech., 16, 2273–2295, https://doi.org/10.5194/amt-16-2273-2023, https://doi.org/10.5194/amt-16-2273-2023, 2023
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The Brewer ozone spectrophotometer is one of the World Meteorological Organization (WMO) Global Atmosphere Watch (GAW)'s standard ozone monitoring instruments since the 1980s. This work is aimed at obtaining answers to (1) why Brewer primary calibration work can only be performed at certain sites (e.g., Izaña and MLO) and (2) what is needed to assure the equivalence of calibration quality from different sites.
Ka Lok Chan, Pieter Valks, Klaus-Peter Heue, Ronny Lutz, Pascal Hedelt, Diego Loyola, Gaia Pinardi, Michel Van Roozendael, François Hendrick, Thomas Wagner, Vinod Kumar, Alkis Bais, Ankie Piters, Hitoshi Irie, Hisahiro Takashima, Yugo Kanaya, Yongjoo Choi, Kihong Park, Jihyo Chong, Alexander Cede, Udo Frieß, Andreas Richter, Jianzhong Ma, Nuria Benavent, Robert Holla, Oleg Postylyakov, Claudia Rivera Cárdenas, and Mark Wenig
Earth Syst. Sci. Data, 15, 1831–1870, https://doi.org/10.5194/essd-15-1831-2023, https://doi.org/10.5194/essd-15-1831-2023, 2023
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This paper presents the theoretical basis as well as verification and validation of the Global Ozone Monitoring Experiment-2 (GOME-2) daily and monthly level-3 products.
Viktoria F. Sofieva, Monika Szelag, Johanna Tamminen, Carlo Arosio, Alexei Rozanov, Mark Weber, Doug Degenstein, Adam Bourassa, Daniel Zawada, Michael Kiefer, Alexandra Laeng, Kaley A. Walker, Patrick Sheese, Daan Hubert, Michel van Roozendael, Christian Retscher, Robert Damadeo, and Jerry D. Lumpe
Atmos. Meas. Tech., 16, 1881–1899, https://doi.org/10.5194/amt-16-1881-2023, https://doi.org/10.5194/amt-16-1881-2023, 2023
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The paper presents the updated SAGE-CCI-OMPS+ climate data record of monthly zonal mean ozone profiles. This dataset covers the stratosphere and combines measurements by nine limb and occultation satellite instruments (SAGE II, OSIRIS, MIPAS, SCIAMACHY, GOMOS, ACE-FTS, OMPS-LP, POAM III, and SAGE III/ISS). The update includes new versions of MIPAS, ACE-FTS, and OSIRIS datasets and introduces data from additional sensors (POAM III and SAGE III/ISS) and retrieval processors (OMPS-LP).
Kai Krause, Folkard Wittrock, Andreas Richter, Dieter Busch, Anton Bergen, John P. Burrows, Steffen Freitag, and Olesia Halbherr
Atmos. Meas. Tech., 16, 1767–1787, https://doi.org/10.5194/amt-16-1767-2023, https://doi.org/10.5194/amt-16-1767-2023, 2023
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Inland shipping is an important source of nitrogen oxides (NOx). The amount of emitted NOx depends on the characteristics of the individual vessels and the traffic density. Ship emissions are often characterised by the amount of emitted NOx per unit of burnt fuel, and further knowledge about fuel consumption is needed to quantify the total emissions caused by ship traffic. In this study, a new approach to derive absolute emission rates (in g s−1) from onshore measurements is presented.
Thomas Wagner, Simon Warnach, Steffen Beirle, Nicole Bobrowski, Adrian Jost, Janis Puķīte, and Nicolas Theys
Atmos. Meas. Tech., 16, 1609–1662, https://doi.org/10.5194/amt-16-1609-2023, https://doi.org/10.5194/amt-16-1609-2023, 2023
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We investigate 3D effects of volcanic plumes on the retrieval results of satellite and ground-based UV–Vis observations. With its small ground pixels of 3.5 x 5.5 km², the TROPOMI instrument can detect much smaller volcanic plumes than previous instruments. At the same time, 3D effects become important. The effect of horizontal photon paths especially can lead to a strong underestimation of the derived plume contents of up to > 50 %, which can be further increased for strong absorbers like SO2.
Linlu Mei, Vladimir Rozanov, Alexei Rozanov, and John P. Burrows
Geosci. Model Dev., 16, 1511–1536, https://doi.org/10.5194/gmd-16-1511-2023, https://doi.org/10.5194/gmd-16-1511-2023, 2023
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This paper summarizes recent developments of aerosol, cloud and surface reflectance databases and models in the framework of the software package SCIATRAN. These updates and developments extend the capabilities of the radiative transfer modeling, especially by accounting for different kinds of vertical inhomogeneties. Vertically inhomogeneous clouds and different aerosol types can be easily accounted for within SCIATRAN (V4.6). The widely used surface models and databases are now available.
Kezia Lange, Andreas Richter, Anja Schönhardt, Andreas C. Meier, Tim Bösch, André Seyler, Kai Krause, Lisa K. Behrens, Folkard Wittrock, Alexis Merlaud, Frederik Tack, Caroline Fayt, Martina M. Friedrich, Ermioni Dimitropoulou, Michel Van Roozendael, Vinod Kumar, Sebastian Donner, Steffen Dörner, Bianca Lauster, Maria Razi, Christian Borger, Katharina Uhlmannsiek, Thomas Wagner, Thomas Ruhtz, Henk Eskes, Birger Bohn, Daniel Santana Diaz, Nader Abuhassan, Dirk Schüttemeyer, and John P. Burrows
Atmos. Meas. Tech., 16, 1357–1389, https://doi.org/10.5194/amt-16-1357-2023, https://doi.org/10.5194/amt-16-1357-2023, 2023
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We present airborne imaging DOAS and ground-based stationary and car DOAS measurements conducted during the S5P-VAL-DE-Ruhr campaign in the Rhine-Ruhr region. The measurements are used to validate spaceborne NO2 data products from the Sentinel-5 Precursor TROPOspheric Monitoring Instrument (TROPOMI). Auxiliary data of the TROPOMI NO2 retrieval, such as spatially higher resolved a priori NO2 vertical profiles, surface reflectivity, and cloud treatment are investigated to evaluate their impact.
Nasrin Mostafavi Pak, Jacob K. Hedelius, Sébastien Roche, Liz Cunningham, Bianca Baier, Colm Sweeney, Coleen Roehl, Joshua Laughner, Geoffrey Toon, Paul Wennberg, Harrison Parker, Colin Arrowsmith, Joseph Mendonca, Pierre Fogal, Tyler Wizenberg, Beatriz Herrera, Kimberly Strong, Kaley A. Walker, Felix Vogel, and Debra Wunch
Atmos. Meas. Tech., 16, 1239–1261, https://doi.org/10.5194/amt-16-1239-2023, https://doi.org/10.5194/amt-16-1239-2023, 2023
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Ground-based remote sensing instruments in the Total Carbon Column Observing Network (TCCON) measure greenhouse gases in the atmosphere. Consistency between TCCON measurements is crucial to accurately infer changes in atmospheric composition. We use portable remote sensing instruments (EM27/SUN) to evaluate biases between TCCON stations in North America. We also improve the retrievals of EM27/SUN instruments and evaluate the previous (GGG2014) and newest (GGG2020) retrieval algorithms.
Brendan Byrne, David F. Baker, Sourish Basu, Michael Bertolacci, Kevin W. Bowman, Dustin Carroll, Abhishek Chatterjee, Frédéric Chevallier, Philippe Ciais, Noel Cressie, David Crisp, Sean Crowell, Feng Deng, Zhu Deng, Nicholas M. Deutscher, Manvendra K. Dubey, Sha Feng, Omaira E. García, David W. T. Griffith, Benedikt Herkommer, Lei Hu, Andrew R. Jacobson, Rajesh Janardanan, Sujong Jeong, Matthew S. Johnson, Dylan B. A. Jones, Rigel Kivi, Junjie Liu, Zhiqiang Liu, Shamil Maksyutov, John B. Miller, Scot M. Miller, Isamu Morino, Justus Notholt, Tomohiro Oda, Christopher W. O'Dell, Young-Suk Oh, Hirofumi Ohyama, Prabir K. Patra, Hélène Peiro, Christof Petri, Sajeev Philip, David F. Pollard, Benjamin Poulter, Marine Remaud, Andrew Schuh, Mahesh K. Sha, Kei Shiomi, Kimberly Strong, Colm Sweeney, Yao Té, Hanqin Tian, Voltaire A. Velazco, Mihalis Vrekoussis, Thorsten Warneke, John R. Worden, Debra Wunch, Yuanzhi Yao, Jeongmin Yun, Andrew Zammit-Mangion, and Ning Zeng
Earth Syst. Sci. Data, 15, 963–1004, https://doi.org/10.5194/essd-15-963-2023, https://doi.org/10.5194/essd-15-963-2023, 2023
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Changes in the carbon stocks of terrestrial ecosystems result in emissions and removals of CO2. These can be driven by anthropogenic activities (e.g., deforestation), natural processes (e.g., fires) or in response to rising CO2 (e.g., CO2 fertilization). This paper describes a dataset of CO2 emissions and removals derived from atmospheric CO2 observations. This pilot dataset informs current capabilities and future developments towards top-down monitoring and verification systems.
Chuan-Yao Lin, Wan-Chin Chen, Yi-Yun Chien, Charles C. K. Chou, Chian-Yi Liu, Helmut Ziereis, Hans Schlager, Eric Förster, Florian Obersteiner, Ovid O. Krüger, Bruna A. Holanda, Mira L. Pöhlker, Katharina Kaiser, Johannes Schneider, Birger Bohn, Klaus Pfeilsticker, Benjamin Weyland, Maria Dolores Andrés Hernández, and John P. Burrows
Atmos. Chem. Phys., 23, 2627–2647, https://doi.org/10.5194/acp-23-2627-2023, https://doi.org/10.5194/acp-23-2627-2023, 2023
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During the EMeRGe campaign in Asia, atmospheric pollutants were measured on board the HALO aircraft. The WRF-Chem model was employed to evaluate the biomass burning (BB) plume transported from Indochina and its impact on the downstream areas. The combination of BB aerosol enhancement with cloud water resulted in a reduction in incoming shortwave radiation at the surface in southern China and the East China Sea, which potentially has significant regional climate implications.
Luca Lelli, Marco Vountas, Narges Khosravi, and John Philipp Burrows
Atmos. Chem. Phys., 23, 2579–2611, https://doi.org/10.5194/acp-23-2579-2023, https://doi.org/10.5194/acp-23-2579-2023, 2023
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Arctic amplification describes the recent period in which temperatures have been rising twice as fast as or more than the global average and sea ice and the Greenland ice shelf are approaching a tipping point. Hence, the Arctic ability to reflect solar energy decreases and absorption by the surface increases. Using 2 decades of complementary satellite data, we discover that clouds unexpectedly increase the pan-Arctic reflectance by increasing their liquid water content, thus cooling the Arctic.
Oliver Schneising, Michael Buchwitz, Jonas Hachmeister, Steffen Vanselow, Maximilian Reuter, Matthias Buschmann, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 16, 669–694, https://doi.org/10.5194/amt-16-669-2023, https://doi.org/10.5194/amt-16-669-2023, 2023
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Methane and carbon monoxide are important constituents of the atmosphere in the context of climate change and air pollution. We present the latest advances in the TROPOMI/WFMD algorithm to simultaneously retrieve atmospheric methane and carbon monoxide abundances from space. The changes in the latest product version are described in detail, and the resulting improvements are demonstrated. An overview of the products is provided including a discussion of annual increases and validation results.
John Douros, Henk Eskes, Jos van Geffen, K. Folkert Boersma, Steven Compernolle, Gaia Pinardi, Anne-Marlene Blechschmidt, Vincent-Henri Peuch, Augustin Colette, and Pepijn Veefkind
Geosci. Model Dev., 16, 509–534, https://doi.org/10.5194/gmd-16-509-2023, https://doi.org/10.5194/gmd-16-509-2023, 2023
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We focus on the challenges associated with comparing atmospheric composition models with satellite products such as tropospheric NO2 columns. The aim is to highlight the methodological difficulties and propose sound ways of doing such comparisons. Building on the comparisons, a new satellite product is proposed and made available, which takes advantage of higher-resolution, regional atmospheric modelling to improve estimates of troposheric NO2 columns over Europe.
Marco Brogioni, Mark J. Andrews, Stefano Urbini, Kenneth C. Jezek, Joel T. Johnson, Marion Leduc-Leballeur, Giovanni Macelloni, Stephen F. Ackley, Alexandra Bringer, Ludovic Brucker, Oguz Demir, Giacomo Fontanelli, Caglar Yardim, Lars Kaleschke, Francesco Montomoli, Leung Tsang, Silvia Becagli, and Massimo Frezzotti
The Cryosphere, 17, 255–278, https://doi.org/10.5194/tc-17-255-2023, https://doi.org/10.5194/tc-17-255-2023, 2023
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In 2018 the first Antarctic campaign of UWBRAD was carried out. UWBRAD is a new radiometer able to collect microwave spectral signatures over 0.5–2 GHz, thus outperforming existing similar sensors. It allows us to probe thicker sea ice and ice sheet down to the bedrock. In this work we tried to assess the UWBRAD potentials for sea ice, glaciers, ice shelves and buried lakes. We also highlighted the wider range of information the spectral signature can provide to glaciological studies.
Vitali E. Fioletov, Chris A. McLinden, Debora Griffin, Ihab Abboud, Nickolay Krotkov, Peter J. T. Leonard, Can Li, Joanna Joiner, Nicolas Theys, and Simon Carn
Earth Syst. Sci. Data, 15, 75–93, https://doi.org/10.5194/essd-15-75-2023, https://doi.org/10.5194/essd-15-75-2023, 2023
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Sulfur dioxide (SO2) measurements from three satellite instruments were used to update and extend the previously developed global catalogue of large SO2 emission sources. This version 2 of the global catalogue covers the period of 2005–2021 and includes a total of 759 continuously emitting point sources. The catalogue data show an approximate 50 % decline in global SO2 emissions between 2005 and 2021, although emissions were relatively stable during the last 3 years.
Ali Jalali, Kaley A. Walker, Kimberly Strong, Rebecca R. Buchholz, Merritt N. Deeter, Debra Wunch, Sébastien Roche, Tyler Wizenberg, Erik Lutsch, Erin McGee, Helen M. Worden, Pierre Fogal, and James R. Drummond
Atmos. Meas. Tech., 15, 6837–6863, https://doi.org/10.5194/amt-15-6837-2022, https://doi.org/10.5194/amt-15-6837-2022, 2022
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This study validates MOPITT version 8 carbon monoxide measurements over the Canadian high Arctic for the period 2006 to 2019. The MOPITT products from different detector pixels and channels are compared with ground-based measurements from the Polar Environment Atmospheric Research Laboratory (PEARL) in Eureka, Nunavut, Canada. These results show good consistency between the satellite and ground-based measurements and provide guidance on the usage of these MOPITT data at high latitudes.
Beatriz Herrera, Alejandro Bezanilla, Thomas Blumenstock, Enrico Dammers, Frank Hase, Lieven Clarisse, Adolfo Magaldi, Claudia Rivera, Wolfgang Stremme, Kimberly Strong, Camille Viatte, Martin Van Damme, and Michel Grutter
Atmos. Chem. Phys., 22, 14119–14132, https://doi.org/10.5194/acp-22-14119-2022, https://doi.org/10.5194/acp-22-14119-2022, 2022
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This work investigates atmospheric ammonia (NH3), a key trace gas with consequences for the environment and human health, in Mexico City. The results from the ground-based and satellite instruments show the variability and spatial distribution of NH3 over this region. NH3 in Mexico City has been increasing for the past 10 years and most of its sources are urban. This work contributes to a better understanding of NH3 sources and variability in urban and remote areas.
Miriam Latsch, Andreas Richter, Henk Eskes, Maarten Sneep, Ping Wang, Pepijn Veefkind, Ronny Lutz, Diego Loyola, Athina Argyrouli, Pieter Valks, Thomas Wagner, Holger Sihler, Michel van Roozendael, Nicolas Theys, Huan Yu, Richard Siddans, and John P. Burrows
Atmos. Meas. Tech., 15, 6257–6283, https://doi.org/10.5194/amt-15-6257-2022, https://doi.org/10.5194/amt-15-6257-2022, 2022
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The article investigates different S5P TROPOMI cloud retrieval algorithms for tropospheric trace gas retrievals. The cloud products show differences primarily over snow and ice and for scenes under sun glint. Some issues regarding across-track dependence are found for the cloud fractions as well as for the cloud heights.
Carlo Arosio, Alexei Rozanov, Victor Gorshelev, Alexandra Laeng, and John P. Burrows
Atmos. Meas. Tech., 15, 5949–5967, https://doi.org/10.5194/amt-15-5949-2022, https://doi.org/10.5194/amt-15-5949-2022, 2022
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This paper characterizes the uncertainties affecting the ozone profiles retrieved at the University of Bremen through OMPS limb satellite observations. An accurate knowledge of the uncertainties is relevant for the validation of the product and to correctly interpret the retrieval results. We investigate several sources of uncertainties, estimate a total random and systematic component, and verify the consistency of the combined OMPS-MLS total uncertainty.
Xin Yang, Kimberly Strong, Alison S. Criscitiello, Marta Santos-Garcia, Kristof Bognar, Xiaoyi Zhao, Pierre Fogal, Kaley A. Walker, Sara M. Morris, and Peter Effertz
EGUsphere, https://doi.org/10.5194/egusphere-2022-696, https://doi.org/10.5194/egusphere-2022-696, 2022
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Snow pack in high Arctic plays a key role in polar atmospheric chemistry, especially in spring when photochemistry becomes active. By sampling surface snow from a Canadian high Arctic location at Eureka, Nunavut (80° N, 86° W), we demonstrate that surface snow is a net sink rather than a source of atmospheric reactive bromine and nitrate. This finding is new and opposite to previous conclusions that snowpack is a large and direct source of reactive bromine in polar spring.
Camille Viatte, Rimal Abeed, Shoma Yamanouchi, William C. Porter, Sarah Safieddine, Martin Van Damme, Lieven Clarisse, Beatriz Herrera, Michel Grutter, Pierre-Francois Coheur, Kimberly Strong, and Cathy Clerbaux
Atmos. Chem. Phys., 22, 12907–12922, https://doi.org/10.5194/acp-22-12907-2022, https://doi.org/10.5194/acp-22-12907-2022, 2022
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Large cities can experience high levels of fine particulate matter (PM2.5) pollution linked to ammonia (NH3) mainly emitted from agricultural activities. Using a combination of PM2.5 and NH3 measurements from in situ instruments, satellite infrared spectrometers, and atmospheric model simulations, we have demonstrated the role of NH3 and meteorological conditions on pollution events occurring over Paris, Toronto, and Mexico City.
John T. Sullivan, Arnoud Apituley, Nora Mettig, Karin Kreher, K. Emma Knowland, Marc Allaart, Ankie Piters, Michel Van Roozendael, Pepijn Veefkind, Jerry R. Ziemke, Natalya Kramarova, Mark Weber, Alexei Rozanov, Laurence Twigg, Grant Sumnicht, and Thomas J. McGee
Atmos. Chem. Phys., 22, 11137–11153, https://doi.org/10.5194/acp-22-11137-2022, https://doi.org/10.5194/acp-22-11137-2022, 2022
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A TROPOspheric Monitoring Instrument (TROPOMI) validation campaign (TROLIX-19) was held in the Netherlands in September 2019. The research presented here focuses on using ozone lidars from NASA’s Goddard Space Flight Center to better evaluate the characterization of ozone throughout TROLIX-19 as compared to balloon-borne, space-borne and ground-based passive measurements, as well as a global coupled chemistry meteorology model.
Nicolas Theys, Christophe Lerot, Hugues Brenot, Jeroen van Gent, Isabelle De Smedt, Lieven Clarisse, Mike Burton, Matthew Varnam, Catherine Hayer, Benjamin Esse, and Michel Van Roozendael
Atmos. Meas. Tech., 15, 4801–4817, https://doi.org/10.5194/amt-15-4801-2022, https://doi.org/10.5194/amt-15-4801-2022, 2022
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Sulfur dioxide plume height after a volcanic eruption is an important piece of information for many different scientific studies and applications. Satellite UV retrievals are useful in this respect, but available algorithms have shown so far limited sensitivity to SO2 height. Here we present a new technique to improve the retrieval of SO2 plume height for SO2 columns as low as 5 DU. We demonstrate the algorithm using TROPOMI measurements and compare with other height estimates.
Pieternel F. Levelt, Deborah C. Stein Zweers, Ilse Aben, Maite Bauwens, Tobias Borsdorff, Isabelle De Smedt, Henk J. Eskes, Christophe Lerot, Diego G. Loyola, Fabian Romahn, Trissevgeni Stavrakou, Nicolas Theys, Michel Van Roozendael, J. Pepijn Veefkind, and Tijl Verhoelst
Atmos. Chem. Phys., 22, 10319–10351, https://doi.org/10.5194/acp-22-10319-2022, https://doi.org/10.5194/acp-22-10319-2022, 2022
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Using the COVID-19 lockdown periods as an example, we show how Sentinel-5P/TROPOMI trace gas data (NO2, SO2, CO, HCHO and CHOCHO) can be used to understand impacts on air quality for regions and cities around the globe. We also provide information for both experienced and inexperienced users about how we created the data using state-of-the-art algorithms, where to get the data, methods taking meteorological and seasonal variability into consideration, and insights for future studies.
Matthias Schneider, Benjamin Ertl, Qiansi Tu, Christopher J. Diekmann, Farahnaz Khosrawi, Amelie N. Röhling, Frank Hase, Darko Dubravica, Omaira E. García, Eliezer Sepúlveda, Tobias Borsdorff, Jochen Landgraf, Alba Lorente, André Butz, Huilin Chen, Rigel Kivi, Thomas Laemmel, Michel Ramonet, Cyril Crevoisier, Jérome Pernin, Martin Steinbacher, Frank Meinhardt, Kimberly Strong, Debra Wunch, Thorsten Warneke, Coleen Roehl, Paul O. Wennberg, Isamu Morino, Laura T. Iraci, Kei Shiomi, Nicholas M. Deutscher, David W. T. Griffith, Voltaire A. Velazco, and David F. Pollard
Atmos. Meas. Tech., 15, 4339–4371, https://doi.org/10.5194/amt-15-4339-2022, https://doi.org/10.5194/amt-15-4339-2022, 2022
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We present a computationally very efficient method for the synergetic use of level 2 remote-sensing data products. We apply the method to IASI vertical profile and TROPOMI total column space-borne methane observations and thus gain sensitivity for the tropospheric methane partial columns, which is not achievable by the individual use of TROPOMI and IASI. These synergetic effects are evaluated theoretically and empirically by inter-comparisons to independent references of TCCON, AirCore, and GAW.
Jonas Hachmeister, Oliver Schneising, Michael Buchwitz, Alba Lorente, Tobias Borsdorff, John P. Burrows, Justus Notholt, and Matthias Buschmann
Atmos. Meas. Tech., 15, 4063–4074, https://doi.org/10.5194/amt-15-4063-2022, https://doi.org/10.5194/amt-15-4063-2022, 2022
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Sentinel-5P trace gas retrievals rely on elevation data in their calculations. Outdated or inaccurate data can lead to significant errors in e.g. dry-air mole fractions of methane (XCH4). We show that the use of inadequate elevation data leads to strong XCH4 anomalies in Greenland. Similar problems can be expected for other regions with inaccurate elevation data. However, we expect these to be more localized. We show that updating elevation data used in the retrieval solves this issue.
Ovid O. Krüger, Bruna A. Holanda, Sourangsu Chowdhury, Andrea Pozzer, David Walter, Christopher Pöhlker, Maria Dolores Andrés Hernández, John P. Burrows, Christiane Voigt, Jos Lelieveld, Johannes Quaas, Ulrich Pöschl, and Mira L. Pöhlker
Atmos. Chem. Phys., 22, 8683–8699, https://doi.org/10.5194/acp-22-8683-2022, https://doi.org/10.5194/acp-22-8683-2022, 2022
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The abrupt reduction in human activities during the first COVID-19 lockdown created unprecedented atmospheric conditions. We took the opportunity to quantify changes in black carbon (BC) as a major anthropogenic air pollutant. Therefore, we measured BC on board a research aircraft over Europe during the lockdown and compared the results to measurements from 2017. With model simulations we account for different weather conditions and find a lockdown-related decrease in BC of 41 %.
William G. Read, Gabriele Stiller, Stefan Lossow, Michael Kiefer, Farahnaz Khosrawi, Dale Hurst, Holger Vömel, Karen Rosenlof, Bianca M. Dinelli, Piera Raspollini, Gerald E. Nedoluha, John C. Gille, Yasuko Kasai, Patrick Eriksson, Christopher E. Sioris, Kaley A. Walker, Katja Weigel, John P. Burrows, and Alexei Rozanov
Atmos. Meas. Tech., 15, 3377–3400, https://doi.org/10.5194/amt-15-3377-2022, https://doi.org/10.5194/amt-15-3377-2022, 2022
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This paper attempts to provide an assessment of the accuracy of 21 satellite-based instruments that remotely measure atmospheric humidity in the upper troposphere of the Earth's atmosphere. The instruments made their measurements from 1984 to the present time; however, most of these instruments began operations after 2000, and only a few are still operational. The objective of this study is to quantify the accuracy of each satellite humidity data set.
Gaia Pinardi, Michel Van Roozendael, François Hendrick, Andreas Richter, Pieter Valks, Ramina Alwarda, Kristof Bognar, Udo Frieß, José Granville, Myojeong Gu, Paul Johnston, Cristina Prados-Roman, Richard Querel, Kimberly Strong, Thomas Wagner, Folkard Wittrock, and Margarita Yela Gonzalez
Atmos. Meas. Tech., 15, 3439–3463, https://doi.org/10.5194/amt-15-3439-2022, https://doi.org/10.5194/amt-15-3439-2022, 2022
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We report on the GOME-2A and GOME-2B OClO dataset (2007 to 2016, from the EUMETSAT's AC SAF) validation using data from nine NDACC zenith-scattered-light DOAS (ZSL-DOAS) instruments distributed in both the Arctic and Antarctic. Specific sensitivity tests are performed on the ground-based data to estimate the impact of the different OClO DOAS analysis settings and their typical errors. Good agreement is found for both the inter-annual variability and the overall OClO seasonal behavior.
Stefan Noël, Maximilian Reuter, Michael Buchwitz, Jakob Borchardt, Michael Hilker, Oliver Schneising, Heinrich Bovensmann, John P. Burrows, Antonio Di Noia, Robert J. Parker, Hiroshi Suto, Yukio Yoshida, Matthias Buschmann, Nicholas M. Deutscher, Dietrich G. Feist, David W. T. Griffith, Frank Hase, Rigel Kivi, Cheng Liu, Isamu Morino, Justus Notholt, Young-Suk Oh, Hirofumi Ohyama, Christof Petri, David F. Pollard, Markus Rettinger, Coleen Roehl, Constantina Rousogenous, Mahesh Kumar Sha, Kei Shiomi, Kimberly Strong, Ralf Sussmann, Yao Té, Voltaire A. Velazco, Mihalis Vrekoussis, and Thorsten Warneke
Atmos. Meas. Tech., 15, 3401–3437, https://doi.org/10.5194/amt-15-3401-2022, https://doi.org/10.5194/amt-15-3401-2022, 2022
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We present a new version (v3) of the GOSAT and GOSAT-2 FOCAL products.
In addition to an increased number of XCO2 data, v3 also includes products for XCH4 (full-physics and proxy), XH2O and the relative ratio of HDO to H2O (δD). For GOSAT-2, we also present first XCO and XN2O results. All FOCAL data products show reasonable spatial distribution and temporal variations and agree well with TCCON. Global XN2O maps show a gradient from the tropics to higher latitudes on the order of 15 ppb.
Mark Weber, Carlo Arosio, Melanie Coldewey-Egbers, Vitali E. Fioletov, Stacey M. Frith, Jeannette D. Wild, Kleareti Tourpali, John P. Burrows, and Diego Loyola
Atmos. Chem. Phys., 22, 6843–6859, https://doi.org/10.5194/acp-22-6843-2022, https://doi.org/10.5194/acp-22-6843-2022, 2022
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Long-term trends in column ozone have been determined from five merged total ozone datasets spanning the period 1978–2020. We show that ozone recovery due to the decline in stratospheric halogens after the 1990s (as regulated by the Montreal Protocol) is evident outside the tropical region and amounts to half a percent per decade. The ozone recovery in the Northern Hemisphere is however compensated for by the negative long-term trend contribution from atmospheric dynamics since the year 2000.
Nora Mettig, Mark Weber, Alexei Rozanov, John P. Burrows, Pepijn Veefkind, Anne M. Thompson, Ryan M. Stauffer, Thierry Leblanc, Gerard Ancellet, Michael J. Newchurch, Shi Kuang, Rigel Kivi, Matthew B. Tully, Roeland Van Malderen, Ankie Piters, Bogumil Kois, René Stübi, and Pavla Skrivankova
Atmos. Meas. Tech., 15, 2955–2978, https://doi.org/10.5194/amt-15-2955-2022, https://doi.org/10.5194/amt-15-2955-2022, 2022
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Vertical ozone profiles from combined spectral measurements in the UV and IR spectral ranges were retrieved by using data from TROPOMI/S5P and CrIS/Suomi-NPP. The vertical resolution and accuracy of the ozone profiles are improved by combining both wavelength ranges compared to retrievals limited to UV or IR spectral data only. The advancement of our TOPAS algorithm for combined measurements is required because in the UV-only retrieval the vertical resolution in the troposphere is very limited.
M. Dolores Andrés Hernández, Andreas Hilboll, Helmut Ziereis, Eric Förster, Ovid O. Krüger, Katharina Kaiser, Johannes Schneider, Francesca Barnaba, Mihalis Vrekoussis, Jörg Schmidt, Heidi Huntrieser, Anne-Marlene Blechschmidt, Midhun George, Vladyslav Nenakhov, Theresa Harlass, Bruna A. Holanda, Jennifer Wolf, Lisa Eirenschmalz, Marc Krebsbach, Mira L. Pöhlker, Anna B. Kalisz Hedegaard, Linlu Mei, Klaus Pfeilsticker, Yangzhuoran Liu, Ralf Koppmann, Hans Schlager, Birger Bohn, Ulrich Schumann, Andreas Richter, Benjamin Schreiner, Daniel Sauer, Robert Baumann, Mariano Mertens, Patrick Jöckel, Markus Kilian, Greta Stratmann, Christopher Pöhlker, Monica Campanelli, Marco Pandolfi, Michael Sicard, José L. Gómez-Amo, Manuel Pujadas, Katja Bigge, Flora Kluge, Anja Schwarz, Nikos Daskalakis, David Walter, Andreas Zahn, Ulrich Pöschl, Harald Bönisch, Stephan Borrmann, Ulrich Platt, and John P. Burrows
Atmos. Chem. Phys., 22, 5877–5924, https://doi.org/10.5194/acp-22-5877-2022, https://doi.org/10.5194/acp-22-5877-2022, 2022
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EMeRGe provides a unique set of in situ and remote sensing airborne measurements of trace gases and aerosol particles along selected flight routes in the lower troposphere over Europe. The interpretation uses also complementary collocated ground-based and satellite measurements. The collected data help to improve the current understanding of the complex spatial distribution of trace gases and aerosol particles resulting from mixing, transport, and transformation of pollution plumes over Europe.
Kezia Lange, Andreas Richter, and John P. Burrows
Atmos. Chem. Phys., 22, 2745–2767, https://doi.org/10.5194/acp-22-2745-2022, https://doi.org/10.5194/acp-22-2745-2022, 2022
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In this study, we investigated short time variability of NOx emissions and lifetimes on a global scale. We combined 2 years of satellite Sentinel-5P TROPOMI tropospheric NO2 column data with wind data. Fifty NOx sources distributed around the world are analyzed. The retrieved emissions show a clear seasonal dependence. NOx lifetime shows a latitudinal dependence but only a week seasonal dependence. NOx emissions show a clear weekly pattern which in contrast is not visible for NOx lifetimes.
Thomas E. Taylor, Christopher W. O'Dell, David Crisp, Akhiko Kuze, Hannakaisa Lindqvist, Paul O. Wennberg, Abhishek Chatterjee, Michael Gunson, Annmarie Eldering, Brendan Fisher, Matthäus Kiel, Robert R. Nelson, Aronne Merrelli, Greg Osterman, Frédéric Chevallier, Paul I. Palmer, Liang Feng, Nicholas M. Deutscher, Manvendra K. Dubey, Dietrich G. Feist, Omaira E. García, David W. T. Griffith, Frank Hase, Laura T. Iraci, Rigel Kivi, Cheng Liu, Martine De Mazière, Isamu Morino, Justus Notholt, Young-Suk Oh, Hirofumi Ohyama, David F. Pollard, Markus Rettinger, Matthias Schneider, Coleen M. Roehl, Mahesh Kumar Sha, Kei Shiomi, Kimberly Strong, Ralf Sussmann, Yao Té, Voltaire A. Velazco, Mihalis Vrekoussis, Thorsten Warneke, and Debra Wunch
Earth Syst. Sci. Data, 14, 325–360, https://doi.org/10.5194/essd-14-325-2022, https://doi.org/10.5194/essd-14-325-2022, 2022
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We provide an analysis of an 11-year record of atmospheric carbon dioxide (CO2) concentrations derived using an optimal estimation retrieval algorithm on measurements made by the GOSAT satellite. The new product (version 9) shows improvement over the previous version (v7.3) as evaluated against independent estimates of CO2 from ground-based sensors and atmospheric inversion systems. We also compare the new GOSAT CO2 values to collocated estimates from NASA's Orbiting Carbon Observatory-2.
Tobias Küchler, Stefan Noël, Heinrich Bovensmann, John Philip Burrows, Thomas Wagner, Christian Borger, Tobias Borsdorff, and Andreas Schneider
Atmos. Meas. Tech., 15, 297–320, https://doi.org/10.5194/amt-15-297-2022, https://doi.org/10.5194/amt-15-297-2022, 2022
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We applied the air-mass-corrected differential optical absorption spectroscopy (AMC-DOAS) method to derive total column water vapour (TCWV) from Sentinel-5P measurements and compared it to independent data sets. The correlation coefficients of typically more than 0.9 and the small deviations up to 2.5 kg m−2 reveal good agreement between our data product and other TCWV data sets. In particular for the different Sentinel-5P water vapour products, the deviations are around 1 kg m−2.
Sandip S. Dhomse, Martyn P. Chipperfield, Wuhu Feng, Ryan Hossaini, Graham W. Mann, Michelle L. Santee, and Mark Weber
Atmos. Chem. Phys., 22, 903–916, https://doi.org/10.5194/acp-22-903-2022, https://doi.org/10.5194/acp-22-903-2022, 2022
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Solar flux variations associated with 11-year sunspot cycle is believed to exert important external climate forcing. As largest variations occur at shorter wavelengths such as ultra-violet part of the solar spectrum, associated changes in stratospheric ozone are thought to provide direct evidence for solar climate interaction. Until now, most of the studies reported double-peak structured solar cycle signal (SCS), but relatively new satellite data suggest only single-peak-structured SCS.
Mahtab Majdzadeh, Craig A. Stroud, Christopher Sioris, Paul A. Makar, Ayodeji Akingunola, Chris McLinden, Xiaoyi Zhao, Michael D. Moran, Ihab Abboud, and Jack Chen
Geosci. Model Dev., 15, 219–249, https://doi.org/10.5194/gmd-15-219-2022, https://doi.org/10.5194/gmd-15-219-2022, 2022
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A new lookup table for aerosol optical properties based on a Mie scattering code was calculated and adopted within an improved version of the photolysis module in the GEM-MACH in-line chemical transport model. The modified version of the photolysis module makes use of online interactive aerosol feedback and applies core-shell parameterizations to the black carbon absorption efficiency based on Bond et al. (2006) to the size bins with black carbon mass fraction of less than 40 %.
Christophe Lerot, François Hendrick, Michel Van Roozendael, Leonardo M. A. Alvarado, Andreas Richter, Isabelle De Smedt, Nicolas Theys, Jonas Vlietinck, Huan Yu, Jeroen Van Gent, Trissevgeni Stavrakou, Jean-François Müller, Pieter Valks, Diego Loyola, Hitoshi Irie, Vinod Kumar, Thomas Wagner, Stefan F. Schreier, Vinayak Sinha, Ting Wang, Pucai Wang, and Christian Retscher
Atmos. Meas. Tech., 14, 7775–7807, https://doi.org/10.5194/amt-14-7775-2021, https://doi.org/10.5194/amt-14-7775-2021, 2021
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Global measurements of glyoxal tropospheric columns from the satellite instrument TROPOMI are presented. Such measurements can contribute to the estimation of atmospheric emissions of volatile organic compounds. This new glyoxal product has been fully characterized with a comprehensive error budget, with comparison with other satellite data sets as well as with validation based on independent ground-based remote sensing glyoxal observations.
Sandip S. Dhomse, Carlo Arosio, Wuhu Feng, Alexei Rozanov, Mark Weber, and Martyn P. Chipperfield
Earth Syst. Sci. Data, 13, 5711–5729, https://doi.org/10.5194/essd-13-5711-2021, https://doi.org/10.5194/essd-13-5711-2021, 2021
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High-quality long-term ozone profile data sets are key to estimating short- and long-term ozone variability. Almost all the satellite (and chemical model) data sets show some kind of bias with respect to each other. This is because of differences in measurement methodologies as well as simplified processes in the models. We use satellite data sets and chemical model output to generate 42 years of ozone profile data sets using a random-forest machine-learning algorithm that is named ML-TOMCAT.
Tyler Wizenberg, Kimberly Strong, Kaley Walker, Erik Lutsch, Tobias Borsdorff, and Jochen Landgraf
Atmos. Meas. Tech., 14, 7707–7728, https://doi.org/10.5194/amt-14-7707-2021, https://doi.org/10.5194/amt-14-7707-2021, 2021
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CO is an important atmospheric gas that influences both air quality and the climate. Here, we compare CO measurements from TROPOMI with those from ACE-FTS and an Arctic ground-based FTS at Eureka, Nunavut, to further characterize the accuracy of TROPOMI measurements. CO columns from the instruments agree well but show larger differences at high latitudes. Despite this, the results fall within the TROPOMI accuracy target, indicating good data quality at high latitudes.
Jānis Puķīte, Christian Borger, Steffen Dörner, Myojeong Gu, Udo Frieß, Andreas Carlos Meier, Carl-Fredrik Enell, Uwe Raffalski, Andreas Richter, and Thomas Wagner
Atmos. Meas. Tech., 14, 7595–7625, https://doi.org/10.5194/amt-14-7595-2021, https://doi.org/10.5194/amt-14-7595-2021, 2021
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Chlorine dioxide (OClO) is used as an indicator for chlorine activation. We present a new differential optical absorption spectroscopy retrieval algorithm for OClO from measurements of TROPOMI on the Sentinel-5P satellite. To achieve a substantially improved accuracy for the weak absorber OClO, we consider several additional fit parameters accounting for various higher-order spectral effects. The retrieved OClO slant column densities are compared with ground-based zenith sky measurements.
Joseph Mendonca, Ray Nassar, Christopher W. O'Dell, Rigel Kivi, Isamu Morino, Justus Notholt, Christof Petri, Kimberly Strong, and Debra Wunch
Atmos. Meas. Tech., 14, 7511–7524, https://doi.org/10.5194/amt-14-7511-2021, https://doi.org/10.5194/amt-14-7511-2021, 2021
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Machine learning has become an important tool for pattern recognition in many applications. In this study, we used a neural network to improve the data quality of OCO-2 measurements made at northern high latitudes. The neural network was trained and used as a binary classifier to filter out bad OCO-2 measurements in order to increase the accuracy and precision of OCO-2 XCO2 measurements in the Boreal and Arctic regions.
Sven Krautwurst, Konstantin Gerilowski, Jakob Borchardt, Norman Wildmann, Michał Gałkowski, Justyna Swolkień, Julia Marshall, Alina Fiehn, Anke Roiger, Thomas Ruhtz, Christoph Gerbig, Jaroslaw Necki, John P. Burrows, Andreas Fix, and Heinrich Bovensmann
Atmos. Chem. Phys., 21, 17345–17371, https://doi.org/10.5194/acp-21-17345-2021, https://doi.org/10.5194/acp-21-17345-2021, 2021
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Quantification of anthropogenic CH4 emissions remains challenging, but it is essential for near-term climate mitigation strategies. We use airborne remote sensing observations to assess bottom-up estimates of coal mining emissions from one of Europe's largest CH4 emission hot spots located in Poland. The analysis reveals that emissions from small groups of shafts can be disentangled, but caution is advised when comparing observations to commonly reported annual emissions.
Song Liu, Pieter Valks, Gaia Pinardi, Jian Xu, Ka Lok Chan, Athina Argyrouli, Ronny Lutz, Steffen Beirle, Ehsan Khorsandi, Frank Baier, Vincent Huijnen, Alkiviadis Bais, Sebastian Donner, Steffen Dörner, Myrto Gratsea, François Hendrick, Dimitris Karagkiozidis, Kezia Lange, Ankie J. M. Piters, Julia Remmers, Andreas Richter, Michel Van Roozendael, Thomas Wagner, Mark Wenig, and Diego G. Loyola
Atmos. Meas. Tech., 14, 7297–7327, https://doi.org/10.5194/amt-14-7297-2021, https://doi.org/10.5194/amt-14-7297-2021, 2021
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In this work, an improved tropospheric NO2 retrieval algorithm from TROPOMI measurements over Europe is presented. The stratospheric estimation is implemented with correction for the dependency of the stratospheric NO2 on the viewing geometry. The AMF calculation is implemented using improved surface albedo, a priori NO2 profiles, and cloud correction. The improved tropospheric NO2 data show good correlations with ground-based MAX-DOAS measurements.
Nicolas Theys, Vitali Fioletov, Can Li, Isabelle De Smedt, Christophe Lerot, Chris McLinden, Nickolay Krotkov, Debora Griffin, Lieven Clarisse, Pascal Hedelt, Diego Loyola, Thomas Wagner, Vinod Kumar, Antje Innes, Roberto Ribas, François Hendrick, Jonas Vlietinck, Hugues Brenot, and Michel Van Roozendael
Atmos. Chem. Phys., 21, 16727–16744, https://doi.org/10.5194/acp-21-16727-2021, https://doi.org/10.5194/acp-21-16727-2021, 2021
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We present a new algorithm to retrieve sulfur dioxide from space UV measurements. We apply the technique to high-resolution TROPOMI measurements and demonstrate the high sensitivity of the approach to weak SO2 emissions worldwide with an unprecedented limit of detection of 8 kt yr−1. This result has broad implications for atmospheric science studies dealing with improving emission inventories and identifying and quantifying missing sources, in the context of air quality and climate.
Hugues Brenot, Nicolas Theys, Lieven Clarisse, Jeroen van Gent, Daniel R. Hurtmans, Sophie Vandenbussche, Nikolaos Papagiannopoulos, Lucia Mona, Timo Virtanen, Andreas Uppstu, Mikhail Sofiev, Luca Bugliaro, Margarita Vázquez-Navarro, Pascal Hedelt, Michelle Maree Parks, Sara Barsotti, Mauro Coltelli, William Moreland, Simona Scollo, Giuseppe Salerno, Delia Arnold-Arias, Marcus Hirtl, Tuomas Peltonen, Juhani Lahtinen, Klaus Sievers, Florian Lipok, Rolf Rüfenacht, Alexander Haefele, Maxime Hervo, Saskia Wagenaar, Wim Som de Cerff, Jos de Laat, Arnoud Apituley, Piet Stammes, Quentin Laffineur, Andy Delcloo, Robertson Lennart, Carl-Herbert Rokitansky, Arturo Vargas, Markus Kerschbaum, Christian Resch, Raimund Zopp, Matthieu Plu, Vincent-Henri Peuch, Michel Van Roozendael, and Gerhard Wotawa
Nat. Hazards Earth Syst. Sci., 21, 3367–3405, https://doi.org/10.5194/nhess-21-3367-2021, https://doi.org/10.5194/nhess-21-3367-2021, 2021
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The purpose of the EUNADICS-AV (European Natural Airborne Disaster Information and Coordination System for Aviation) prototype early warning system (EWS) is to develop the combined use of harmonised data products from satellite, ground-based and in situ instruments to produce alerts of airborne hazards (volcanic, dust, smoke and radionuclide clouds), satisfying the requirement of aviation air traffic management (ATM) stakeholders (https://cordis.europa.eu/project/id/723986).
Yu-Wen Chen, Yi-Chun Chen, Charles C.-K. Chou, Hui-Ming Hung, Shih-Yu Chang, Lisa Eirenschmalz, Michael Lichtenstern, Helmut Ziereis, Hans Schlager, Greta Stratmann, Katharina Kaiser, Johannes Schneider, Stephan Borrmann, Florian Obersteiner, Eric Förster, Andreas Zahn, Wei-Nai Chen, Po-Hsiung Lin, Shuenn-Chin Chang, Maria Dolores Andrés Hernández, Pao-Kuan Wang, and John P. Burrows
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-788, https://doi.org/10.5194/acp-2021-788, 2021
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By presenting an approach using EMeRGe-Asia airborne field measurements and surface observations, this study shows that the fraction of OH reactivity due to SO2-OH reaction has a significant correlation with the sulfate concentration. Approximately 30 % of sulfate is produced by SO2-OH reaction. Our results underline the importance of SO2-OH gas-phase oxidation in sulfate formation, and demonstrate that the method can be applied to other regions and under different meteorological conditions.
Elizaveta Malinina, Alexei Rozanov, Ulrike Niemeier, Sandra Wallis, Carlo Arosio, Felix Wrana, Claudia Timmreck, Christian von Savigny, and John P. Burrows
Atmos. Chem. Phys., 21, 14871–14891, https://doi.org/10.5194/acp-21-14871-2021, https://doi.org/10.5194/acp-21-14871-2021, 2021
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In the paper, changes in the stratospheric aerosol loading after the 2018 Ambae eruption were analyzed using OMPS-LP observations. The eruption was also simulated with the MAECHAM5-HAM global climate model. Generally, the model and observations agree very well. We attribute the good consistency of the results to a precisely determined altitude and mass of the volcanic injection, as well as nudging of the meteorological data. The radiative forcing from the eruption was estimated to be −0.13 W m−2.
Marek Muchow, Amelie U. Schmitt, and Lars Kaleschke
The Cryosphere, 15, 4527–4537, https://doi.org/10.5194/tc-15-4527-2021, https://doi.org/10.5194/tc-15-4527-2021, 2021
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Linear-like openings in sea ice, also called leads, occur with widths from meters to kilometers. We use satellite images from Sentinel-2 with a resolution of 10 m to identify leads and measure their widths. With that we investigate the frequency of lead widths using two different statistical methods, since other studies have shown a dependency of heat exchange on the lead width. We are the first to address the sea-ice lead-width distribution in the Weddell Sea, Antarctica.
Mahesh Kumar Sha, Bavo Langerock, Jean-François L. Blavier, Thomas Blumenstock, Tobias Borsdorff, Matthias Buschmann, Angelika Dehn, Martine De Mazière, Nicholas M. Deutscher, Dietrich G. Feist, Omaira E. García, David W. T. Griffith, Michel Grutter, James W. Hannigan, Frank Hase, Pauli Heikkinen, Christian Hermans, Laura T. Iraci, Pascal Jeseck, Nicholas Jones, Rigel Kivi, Nicolas Kumps, Jochen Landgraf, Alba Lorente, Emmanuel Mahieu, Maria V. Makarova, Johan Mellqvist, Jean-Marc Metzger, Isamu Morino, Tomoo Nagahama, Justus Notholt, Hirofumi Ohyama, Ivan Ortega, Mathias Palm, Christof Petri, David F. Pollard, Markus Rettinger, John Robinson, Sébastien Roche, Coleen M. Roehl, Amelie N. Röhling, Constantina Rousogenous, Matthias Schneider, Kei Shiomi, Dan Smale, Wolfgang Stremme, Kimberly Strong, Ralf Sussmann, Yao Té, Osamu Uchino, Voltaire A. Velazco, Corinne Vigouroux, Mihalis Vrekoussis, Pucai Wang, Thorsten Warneke, Tyler Wizenberg, Debra Wunch, Shoma Yamanouchi, Yang Yang, and Minqiang Zhou
Atmos. Meas. Tech., 14, 6249–6304, https://doi.org/10.5194/amt-14-6249-2021, https://doi.org/10.5194/amt-14-6249-2021, 2021
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This paper presents, for the first time, Sentinel-5 Precursor methane and carbon monoxide validation results covering a period from November 2017 to September 2020. For this study, we used global TCCON and NDACC-IRWG network data covering a wide range of atmospheric and surface conditions across different terrains. We also show the influence of a priori alignment, smoothing uncertainties and the sensitivity of the validation results towards the application of advanced co-location criteria.
Nora Mettig, Mark Weber, Alexei Rozanov, Carlo Arosio, John P. Burrows, Pepijn Veefkind, Anne M. Thompson, Richard Querel, Thierry Leblanc, Sophie Godin-Beekmann, Rigel Kivi, and Matthew B. Tully
Atmos. Meas. Tech., 14, 6057–6082, https://doi.org/10.5194/amt-14-6057-2021, https://doi.org/10.5194/amt-14-6057-2021, 2021
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TROPOMI is a nadir-viewing satellite that has observed global atmospheric trace gases at unprecedented spatial resolution since 2017. The retrieval of ozone profiles with high accuracy has been demonstrated using the TOPAS (Tikhonov regularised Ozone Profile retrievAl with SCIATRAN) algorithm and applying appropriate spectral corrections to TROPOMI UV data. Ozone profiles from TROPOMI were compared to ozonesonde and lidar profiles, showing an agreement to within 5 % in the stratosphere.
Kai Krause, Folkard Wittrock, Andreas Richter, Stefan Schmitt, Denis Pöhler, Andreas Weigelt, and John P. Burrows
Atmos. Meas. Tech., 14, 5791–5807, https://doi.org/10.5194/amt-14-5791-2021, https://doi.org/10.5194/amt-14-5791-2021, 2021
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Ships are an important source of key pollutants. Usually, these are measured aboard the ship or on the coast using in situ instruments. This study shows how active optical remote sensing can be used to measure ship emissions and how to determine emission rates of individual ships out of those measurements. These emission rates are valuable input for the assessment of the influence of shipping emissions in regions close to the shipping lanes.
Andrea Orfanoz-Cheuquelaf, Alexei Rozanov, Mark Weber, Carlo Arosio, Annette Ladstätter-Weißenmayer, and John P. Burrows
Atmos. Meas. Tech., 14, 5771–5789, https://doi.org/10.5194/amt-14-5771-2021, https://doi.org/10.5194/amt-14-5771-2021, 2021
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OMPS/NPP (2012–present) allows obtaining the tropospheric ozone column by combining ozone data from limb and nadir observations from the same instrument platform. In a first step, the retrieval of the total ozone column from the OMPS Nadir Mapper using the weighting function fitting approach (WFFA) is described here. The OMPS total ozone was compared with ground-based and other satellite measurements, showing agreement within 2.5 %.
Isabelle De Smedt, Gaia Pinardi, Corinne Vigouroux, Steven Compernolle, Alkis Bais, Nuria Benavent, Folkert Boersma, Ka-Lok Chan, Sebastian Donner, Kai-Uwe Eichmann, Pascal Hedelt, François Hendrick, Hitoshi Irie, Vinod Kumar, Jean-Christopher Lambert, Bavo Langerock, Christophe Lerot, Cheng Liu, Diego Loyola, Ankie Piters, Andreas Richter, Claudia Rivera Cárdenas, Fabian Romahn, Robert George Ryan, Vinayak Sinha, Nicolas Theys, Jonas Vlietinck, Thomas Wagner, Ting Wang, Huan Yu, and Michel Van Roozendael
Atmos. Chem. Phys., 21, 12561–12593, https://doi.org/10.5194/acp-21-12561-2021, https://doi.org/10.5194/acp-21-12561-2021, 2021
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This paper assess the performances of the TROPOMI formaldehyde observations compared to its predecessor OMI at different spatial and temporal scales. We also use a global network of MAX-DOAS instruments to validate both satellite datasets for a large range of HCHO columns. The precision obtained with daily TROPOMI observations is comparable to monthly OMI observations. We present clear detection of weak HCHO column enhancements related to shipping emissions in the Indian Ocean.
Thomas Krumpen, Luisa von Albedyll, Helge F. Goessling, Stefan Hendricks, Bennet Juhls, Gunnar Spreen, Sascha Willmes, H. Jakob Belter, Klaus Dethloff, Christian Haas, Lars Kaleschke, Christian Katlein, Xiangshan Tian-Kunze, Robert Ricker, Philip Rostosky, Janna Rückert, Suman Singha, and Julia Sokolova
The Cryosphere, 15, 3897–3920, https://doi.org/10.5194/tc-15-3897-2021, https://doi.org/10.5194/tc-15-3897-2021, 2021
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We use satellite data records collected along the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) drift to categorize ice conditions that shaped and characterized the floe and surroundings during the expedition. A comparison with previous years is made whenever possible. The aim of this analysis is to provide a basis and reference for subsequent research in the six main research areas of atmosphere, ocean, sea ice, biogeochemistry, remote sensing and ecology.
Stefan F. Schreier, Tim Bösch, Andreas Richter, Kezia Lange, Michael Revesz, Philipp Weihs, Mihalis Vrekoussis, and Christoph Lotteraner
Atmos. Meas. Tech., 14, 5299–5318, https://doi.org/10.5194/amt-14-5299-2021, https://doi.org/10.5194/amt-14-5299-2021, 2021
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This paper reports on the evaluation of aerosol profiling products retrieved from ground-based MAX-DOAS instruments using the BOREAS algorithm. Aerosol extinction profiles, near-surface aerosol extinction, and aerosol optical depth are compared to measurements collected with ceilometer, sun photometer, and in situ instruments. We show that these MAX-DOAS aerosol profiling products provide useful information to study spatial and temporal variations above the urban area of Vienna.
Claire Lamotte, Jonathan Guth, Virginie Marécal, Martin Cussac, Paul David Hamer, Nicolas Theys, and Philipp Schneider
Atmos. Chem. Phys., 21, 11379–11404, https://doi.org/10.5194/acp-21-11379-2021, https://doi.org/10.5194/acp-21-11379-2021, 2021
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Improvements are made in a global chemical transfer model by considering a new volcanic SO2 emissions inventory, with more volcanoes referenced and more information on the altitude of injection. Better constraining volcanic emissions with this inventory improves the global, but mostly local, tropospheric sulfur composition. The tropospheric sulfur budget shows a nonlinearity to the volcanic contribution, especially to the sulfate aerosol burden and sulfur wet deposition.
Johannes de Leeuw, Anja Schmidt, Claire S. Witham, Nicolas Theys, Isabelle A. Taylor, Roy G. Grainger, Richard J. Pope, Jim Haywood, Martin Osborne, and Nina I. Kristiansen
Atmos. Chem. Phys., 21, 10851–10879, https://doi.org/10.5194/acp-21-10851-2021, https://doi.org/10.5194/acp-21-10851-2021, 2021
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Using the NAME dispersion model in combination with high-resolution SO2 satellite data from TROPOMI, we investigate the dispersion of volcanic SO2 from the 2019 Raikoke eruption. NAME accurately simulates the dispersion of SO2 during the first 2–3 weeks after the eruption and illustrates the potential of using high-resolution satellite data to identify potential limitations in dispersion models, which will ultimately help to improve efforts to forecast the dispersion of volcanic clouds.
Lily N. Zhang, Susan Solomon, Kane A. Stone, Jonathan D. Shanklin, Joshua D. Eveson, Steve Colwell, John P. Burrows, Mark Weber, Pieternel F. Levelt, Natalya A. Kramarova, and David P. Haffner
Atmos. Chem. Phys., 21, 9829–9838, https://doi.org/10.5194/acp-21-9829-2021, https://doi.org/10.5194/acp-21-9829-2021, 2021
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In the 1980s, measurements at the British Antarctic Survey station in Halley, Antarctica, led to the discovery of the ozone hole. The Halley total ozone record continues to be uniquely valuable for studies of long-term changes in Antarctic ozone. Environmental conditions in 2017 forced a temporary cessation of operations, leading to a gap in the historic record. We develop and test a method for filling in the Halley record using satellite data and find evidence to further support ozone recovery.
Ilya Stanevich, Dylan B. A. Jones, Kimberly Strong, Martin Keller, Daven K. Henze, Robert J. Parker, Hartmut Boesch, Debra Wunch, Justus Notholt, Christof Petri, Thorsten Warneke, Ralf Sussmann, Matthias Schneider, Frank Hase, Rigel Kivi, Nicholas M. Deutscher, Voltaire A. Velazco, Kaley A. Walker, and Feng Deng
Atmos. Chem. Phys., 21, 9545–9572, https://doi.org/10.5194/acp-21-9545-2021, https://doi.org/10.5194/acp-21-9545-2021, 2021
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We explore the utility of a weak-constraint (WC) four-dimensional variational (4D-Var) data assimilation scheme for mitigating systematic errors in methane simulation in the GEOS-Chem model. We use data from the Greenhouse Gases Observing Satellite (GOSAT) and show that, compared to the traditional 4D-Var approach, the WC scheme improves the agreement between the model and independent observations. We find that the WC corrections to the model provide insight into the source of the errors.
Matthieu Dogniaux, Cyril Crevoisier, Raymond Armante, Virginie Capelle, Thibault Delahaye, Vincent Cassé, Martine De Mazière, Nicholas M. Deutscher, Dietrich G. Feist, Omaira E. Garcia, David W. T. Griffith, Frank Hase, Laura T. Iraci, Rigel Kivi, Isamu Morino, Justus Notholt, David F. Pollard, Coleen M. Roehl, Kei Shiomi, Kimberly Strong, Yao Té, Voltaire A. Velazco, and Thorsten Warneke
Atmos. Meas. Tech., 14, 4689–4706, https://doi.org/10.5194/amt-14-4689-2021, https://doi.org/10.5194/amt-14-4689-2021, 2021
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We present the Adaptable 4A Inversion (5AI), an implementation of the optimal estimation (OE) algorithm, relying on the Automatized Atmospheric Absorption Atlas (4A/OP) radiative transfer model, that enables the retrieval of greenhouse gas atmospheric weighted columns from infrared measurements. It is tested on a sample of Orbiting Carbon Observatory-2 observations, and its results satisfactorily compare to several reference products, thus showing the reliability of 5AI OE implementation.
Linlu Mei, Vladimir Rozanov, Christine Pohl, Marco Vountas, and John P. Burrows
The Cryosphere, 15, 2757–2780, https://doi.org/10.5194/tc-15-2757-2021, https://doi.org/10.5194/tc-15-2757-2021, 2021
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This paper presents a new snow property retrieval algorithm from satellite observations. This is Part 1 of two companion papers and shows the method description and sensitivity study. The paper investigates the major factors, including the assumptions of snow optical properties, snow particle distribution and atmospheric conditions (cloud and aerosol), impacting snow property retrievals from satellite observation.
Linlu Mei, Vladimir Rozanov, Evelyn Jäkel, Xiao Cheng, Marco Vountas, and John P. Burrows
The Cryosphere, 15, 2781–2802, https://doi.org/10.5194/tc-15-2781-2021, https://doi.org/10.5194/tc-15-2781-2021, 2021
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This paper presents a new snow property retrieval algorithm from satellite observations. This is Part 2 of two companion papers and shows the results and validation. The paper performs the new retrieval algorithm on the Sea and Land
Surface Temperature Radiometer (SLSTR) instrument and compares the retrieved snow properties with ground-based measurements, aircraft measurements and other satellite products.
Daniel Zawada, Ghislain Franssens, Robert Loughman, Antti Mikkonen, Alexei Rozanov, Claudia Emde, Adam Bourassa, Seth Dueck, Hannakaisa Lindqvist, Didier Ramon, Vladimir Rozanov, Emmanuel Dekemper, Erkki Kyrölä, John P. Burrows, Didier Fussen, and Doug Degenstein
Atmos. Meas. Tech., 14, 3953–3972, https://doi.org/10.5194/amt-14-3953-2021, https://doi.org/10.5194/amt-14-3953-2021, 2021
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Satellite measurements of atmospheric composition often rely on computer tools known as radiative transfer models to model the propagation of sunlight within the atmosphere. Here we have performed a detailed inter-comparison of seven different radiative transfer models in a variety of conditions. We have found that the models agree remarkably well, at a level better than previously reported. This result provides confidence in our understanding of atmospheric radiative transfer.
Stefan Noël, Maximilian Reuter, Michael Buchwitz, Jakob Borchardt, Michael Hilker, Heinrich Bovensmann, John P. Burrows, Antonio Di Noia, Hiroshi Suto, Yukio Yoshida, Matthias Buschmann, Nicholas M. Deutscher, Dietrich G. Feist, David W. T. Griffith, Frank Hase, Rigel Kivi, Isamu Morino, Justus Notholt, Hirofumi Ohyama, Christof Petri, James R. Podolske, David F. Pollard, Mahesh Kumar Sha, Kei Shiomi, Ralf Sussmann, Yao Té, Voltaire A. Velazco, and Thorsten Warneke
Atmos. Meas. Tech., 14, 3837–3869, https://doi.org/10.5194/amt-14-3837-2021, https://doi.org/10.5194/amt-14-3837-2021, 2021
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We present the first GOSAT and GOSAT-2 XCO2 data derived with the FOCAL retrieval algorithm. Comparisons of the GOSAT-FOCAL product with other data reveal long-term agreement within about 1 ppm over 1 decade, differences in seasonal variations of about 0.5 ppm, and a mean regional bias to ground-based TCCON data of 0.56 ppm with a mean scatter of 1.89 ppm. GOSAT-2-FOCAL data are preliminary only, but first comparisons show that they compare well with the GOSAT-FOCAL results and TCCON.
Viktoria F. Sofieva, Monika Szeląg, Johanna Tamminen, Erkki Kyrölä, Doug Degenstein, Chris Roth, Daniel Zawada, Alexei Rozanov, Carlo Arosio, John P. Burrows, Mark Weber, Alexandra Laeng, Gabriele P. Stiller, Thomas von Clarmann, Lucien Froidevaux, Nathaniel Livesey, Michel van Roozendael, and Christian Retscher
Atmos. Chem. Phys., 21, 6707–6720, https://doi.org/10.5194/acp-21-6707-2021, https://doi.org/10.5194/acp-21-6707-2021, 2021
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The MErged GRIdded Dataset of Ozone Profiles is a long-term (2001–2018) stratospheric ozone profile climate data record with resolved longitudinal structure that combines the data from six limb satellite instruments. The dataset can be used for various analyses, some of which are discussed in the paper. In particular, regionally and vertically resolved ozone trends are evaluated, including trends in the polar regions.
Sébastien Roche, Kimberly Strong, Debra Wunch, Joseph Mendonca, Colm Sweeney, Bianca Baier, Sébastien C. Biraud, Joshua L. Laughner, Geoffrey C. Toon, and Brian J. Connor
Atmos. Meas. Tech., 14, 3087–3118, https://doi.org/10.5194/amt-14-3087-2021, https://doi.org/10.5194/amt-14-3087-2021, 2021
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We evaluate CO2 profile retrievals from ground-based near-infrared solar absorption spectra after implementing several improvements to the GFIT2 retrieval algorithm. Realistic errors in the a priori temperature profile (~ 2 °C in the lower troposphere) are found to be the leading source of differences between the retrieved and true CO2 profiles, differences that are larger than typical CO2 variability. A temperature retrieval or correction is critical to improve CO2 profile retrieval results.
Ioanna Skoulidou, Maria-Elissavet Koukouli, Astrid Manders, Arjo Segers, Dimitris Karagkiozidis, Myrto Gratsea, Dimitris Balis, Alkiviadis Bais, Evangelos Gerasopoulos, Trisevgeni Stavrakou, Jos van Geffen, Henk Eskes, and Andreas Richter
Atmos. Chem. Phys., 21, 5269–5288, https://doi.org/10.5194/acp-21-5269-2021, https://doi.org/10.5194/acp-21-5269-2021, 2021
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The performance of LOTOS-EUROS v2.2.001 regional chemical transport model NO2 simulations is investigated over Greece from June to December 2018. Comparison with in situ NO2 measurements shows a spatial correlation coefficient of 0.86, while the model underestimates the concentrations mostly during daytime (12 to 15:00 local time). Further, the simulated tropospheric NO2 columns are evaluated against ground-based MAX-DOAS NO2 measurements and S5P/TROPOMI observations for July and December 2018.
Xiaoyi Zhao, Vitali Fioletov, Michael Brohart, Volodya Savastiouk, Ihab Abboud, Akira Ogyu, Jonathan Davies, Reno Sit, Sum Chi Lee, Alexander Cede, Martin Tiefengraber, Moritz Müller, Debora Griffin, and Chris McLinden
Atmos. Meas. Tech., 14, 2261–2283, https://doi.org/10.5194/amt-14-2261-2021, https://doi.org/10.5194/amt-14-2261-2021, 2021
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The Brewer spectrophotometer is one of the main instruments for measurements of atmospheric total column ozone. The global Brewer network largely relies on the world reference instruments (the Brewer triad) operated by Environment and Climate Change Canada since the early 1980s. This study provides an updated assessment (1999–2019) of the reference instrument performance, in terms of random uncertainties and long-term stability.
Michael Buchwitz, Maximilian Reuter, Stefan Noël, Klaus Bramstedt, Oliver Schneising, Michael Hilker, Blanca Fuentes Andrade, Heinrich Bovensmann, John P. Burrows, Antonio Di Noia, Hartmut Boesch, Lianghai Wu, Jochen Landgraf, Ilse Aben, Christian Retscher, Christopher W. O'Dell, and David Crisp
Atmos. Meas. Tech., 14, 2141–2166, https://doi.org/10.5194/amt-14-2141-2021, https://doi.org/10.5194/amt-14-2141-2021, 2021
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The COVID-19 pandemic resulted in reduced anthropogenic carbon dioxide (CO2) emissions during 2020 in large parts of the world. We have used a small ensemble of satellite retrievals of column-averaged CO2 (XCO2) to find out if a regional-scale reduction of atmospheric CO2 can be detected from space. We focus on East China and show that it is challenging to reliably detect and to accurately quantify the emission reduction, which only results in regional XCO2 reductions of about 0.1–0.2 ppm.
Jakob Borchardt, Konstantin Gerilowski, Sven Krautwurst, Heinrich Bovensmann, Andrew K. Thorpe, David R. Thompson, Christian Frankenberg, Charles E. Miller, Riley M. Duren, and John Philip Burrows
Atmos. Meas. Tech., 14, 1267–1291, https://doi.org/10.5194/amt-14-1267-2021, https://doi.org/10.5194/amt-14-1267-2021, 2021
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The AVIRIS-NG hyperspectral imager has been used successfully to identify and quantify anthropogenic methane sources utilizing different retrieval and inversion methods. Here, we examine the adaption and application of the WFM-DOAS algorithm to AVIRIS-NG measurements to retrieve local methane column enhancements, compare the results with other retrievals, and quantify the uncertainties resulting from the retrieval method. Additionally, we estimate emissions from five detected methane plumes.
Thomas Blumenstock, Frank Hase, Axel Keens, Denis Czurlok, Orfeo Colebatch, Omaira Garcia, David W. T. Griffith, Michel Grutter, James W. Hannigan, Pauli Heikkinen, Pascal Jeseck, Nicholas Jones, Rigel Kivi, Erik Lutsch, Maria Makarova, Hamud K. Imhasin, Johan Mellqvist, Isamu Morino, Tomoo Nagahama, Justus Notholt, Ivan Ortega, Mathias Palm, Uwe Raffalski, Markus Rettinger, John Robinson, Matthias Schneider, Christian Servais, Dan Smale, Wolfgang Stremme, Kimberly Strong, Ralf Sussmann, Yao Té, and Voltaire A. Velazco
Atmos. Meas. Tech., 14, 1239–1252, https://doi.org/10.5194/amt-14-1239-2021, https://doi.org/10.5194/amt-14-1239-2021, 2021
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This study investigates the level of channeling (optical resonances) of each FTIR spectrometer within the Network for the Detection of Atmospheric Composition Change (NDACC). Since the air gap of the beam splitter is a significant source of channeling, we propose new beam splitters with an increased wedge of the air gap. This study shows the potential for reducing channeling in the FTIR spectrometers operated by the NDACC, thereby increasing the quality of recorded spectra across the network.
Shoma Yamanouchi, Camille Viatte, Kimberly Strong, Erik Lutsch, Dylan B. A. Jones, Cathy Clerbaux, Martin Van Damme, Lieven Clarisse, and Pierre-Francois Coheur
Atmos. Meas. Tech., 14, 905–921, https://doi.org/10.5194/amt-14-905-2021, https://doi.org/10.5194/amt-14-905-2021, 2021
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Ammonia (NH3) is a major source of pollution in the air. As such, there have been increasing efforts to measure the atmospheric abundance of NH3 and its spatial and temporal variability. In this study, long-term measurements of NH3 over Toronto, Canada, derived from multiscale datasets are examined. These NH3 datasets were compared to each other and to a model to better understand NH3 variability and to assess model performance.
Myrto Gratsea, Tim Bösch, Panagiotis Kokkalis, Andreas Richter, Mihalis Vrekoussis, Stelios Kazadzis, Alexandra Tsekeri, Alexandros Papayannis, Maria Mylonaki, Vassilis Amiridis, Nikos Mihalopoulos, and Evangelos Gerasopoulos
Atmos. Meas. Tech., 14, 749–767, https://doi.org/10.5194/amt-14-749-2021, https://doi.org/10.5194/amt-14-749-2021, 2021
Elena Spinei, Martin Tiefengraber, Moritz Müller, Manuel Gebetsberger, Alexander Cede, Luke Valin, James Szykman, Andrew Whitehill, Alexander Kotsakis, Fernando Santos, Nader Abbuhasan, Xiaoyi Zhao, Vitali Fioletov, Sum Chi Lee, and Robert Swap
Atmos. Meas. Tech., 14, 647–663, https://doi.org/10.5194/amt-14-647-2021, https://doi.org/10.5194/amt-14-647-2021, 2021
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Plastics are widely used in everyday life and scientific equipment. This paper presents Delrin plastic off-gassing as a function of temperature on the atmospheric measurements of formaldehyde by Pandora spectroscopic instruments. The sealed telescope assembly containing Delrin components emitted large amounts of formaldehyde at 30–45 °C, interfering with the Pandora measurements. These results have a broader implication since electronic products often experience the same temperature.
Tijl Verhoelst, Steven Compernolle, Gaia Pinardi, Jean-Christopher Lambert, Henk J. Eskes, Kai-Uwe Eichmann, Ann Mari Fjæraa, José Granville, Sander Niemeijer, Alexander Cede, Martin Tiefengraber, François Hendrick, Andrea Pazmiño, Alkiviadis Bais, Ariane Bazureau, K. Folkert Boersma, Kristof Bognar, Angelika Dehn, Sebastian Donner, Aleksandr Elokhov, Manuel Gebetsberger, Florence Goutail, Michel Grutter de la Mora, Aleksandr Gruzdev, Myrto Gratsea, Georg H. Hansen, Hitoshi Irie, Nis Jepsen, Yugo Kanaya, Dimitris Karagkiozidis, Rigel Kivi, Karin Kreher, Pieternel F. Levelt, Cheng Liu, Moritz Müller, Monica Navarro Comas, Ankie J. M. Piters, Jean-Pierre Pommereau, Thierry Portafaix, Cristina Prados-Roman, Olga Puentedura, Richard Querel, Julia Remmers, Andreas Richter, John Rimmer, Claudia Rivera Cárdenas, Lidia Saavedra de Miguel, Valery P. Sinyakov, Wolfgang Stremme, Kimberly Strong, Michel Van Roozendael, J. Pepijn Veefkind, Thomas Wagner, Folkard Wittrock, Margarita Yela González, and Claus Zehner
Atmos. Meas. Tech., 14, 481–510, https://doi.org/10.5194/amt-14-481-2021, https://doi.org/10.5194/amt-14-481-2021, 2021
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This paper reports on the ground-based validation of the NO2 data produced operationally by the TROPOMI instrument on board the Sentinel-5 Precursor satellite. Tropospheric, stratospheric, and total NO2 columns are compared to measurements collected from MAX-DOAS, ZSL-DOAS, and PGN/Pandora instruments respectively. The products are found to satisfy mission requirements in general, though negative mean differences are found at sites with high pollution levels. Potential causes are discussed.
Soheila Jafariserajehlou, Vladimir V. Rozanov, Marco Vountas, Charles K. Gatebe, and John P. Burrows
Atmos. Meas. Tech., 14, 369–389, https://doi.org/10.5194/amt-14-369-2021, https://doi.org/10.5194/amt-14-369-2021, 2021
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In this work, we study retrieval of snow grain morphologies and their impact on the reflectance in a coupled snow–atmosphere system. We present a sensitivity study to highlight the importance of having adequate information about snow and atmosphere. A novel two-stage algorithm for retrieving the size and shape of snow grains is presented. The reflectance simulation results are compared to that of airborne measurements; high correlations of 0.98 at IR and 0.88–0.98 at VIS are achieved.
Maximilian Reuter, Heinrich Bovensmann, Michael Buchwitz, Jakob Borchardt, Sven Krautwurst, Konstantin Gerilowski, Matthias Lindauer, Dagmar Kubistin, and John P. Burrows
Atmos. Meas. Tech., 14, 153–172, https://doi.org/10.5194/amt-14-153-2021, https://doi.org/10.5194/amt-14-153-2021, 2021
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CO2 measurements from a small unmanned aircraft system (sUAS) can provide a cost-effective way to complement and validate satellite-based measurements of anthropogenic CO2 emissions. We introduce an sUAS which is capable of determining atmospheric CO2 mass fluxes from its own sensor data. We show results of validation flights at the ICOS atmospheric station in Steinkimmen and from demonstration flights downwind a CO2-emitting natural gas processing facility.
Jan-Lukas Tirpitz, Udo Frieß, François Hendrick, Carlos Alberti, Marc Allaart, Arnoud Apituley, Alkis Bais, Steffen Beirle, Stijn Berkhout, Kristof Bognar, Tim Bösch, Ilya Bruchkouski, Alexander Cede, Ka Lok Chan, Mirjam den Hoed, Sebastian Donner, Theano Drosoglou, Caroline Fayt, Martina M. Friedrich, Arnoud Frumau, Lou Gast, Clio Gielen, Laura Gomez-Martín, Nan Hao, Arjan Hensen, Bas Henzing, Christian Hermans, Junli Jin, Karin Kreher, Jonas Kuhn, Johannes Lampel, Ang Li, Cheng Liu, Haoran Liu, Jianzhong Ma, Alexis Merlaud, Enno Peters, Gaia Pinardi, Ankie Piters, Ulrich Platt, Olga Puentedura, Andreas Richter, Stefan Schmitt, Elena Spinei, Deborah Stein Zweers, Kimberly Strong, Daan Swart, Frederik Tack, Martin Tiefengraber, René van der Hoff, Michel van Roozendael, Tim Vlemmix, Jan Vonk, Thomas Wagner, Yang Wang, Zhuoru Wang, Mark Wenig, Matthias Wiegner, Folkard Wittrock, Pinhua Xie, Chengzhi Xing, Jin Xu, Margarita Yela, Chengxin Zhang, and Xiaoyi Zhao
Atmos. Meas. Tech., 14, 1–35, https://doi.org/10.5194/amt-14-1-2021, https://doi.org/10.5194/amt-14-1-2021, 2021
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Multi-axis differential optical absorption spectroscopy (MAX-DOAS) is a ground-based remote sensing measurement technique that derives atmospheric aerosol and trace gas vertical profiles from skylight spectra. In this study, consistency and reliability of MAX-DOAS profiles are assessed by applying nine different evaluation algorithms to spectral data recorded during an intercomparison campaign in the Netherlands and by comparing the results to colocated supporting observations.
Xin Yang, Anne-M. Blechschmidt, Kristof Bognar, Audra McClure-Begley, Sara Morris, Irina Petropavlovskikh, Andreas Richter, Henrik Skov, Kimberly Strong, David W. Tarasick, Taneil Uttal, Mika Vestenius, and Xiaoyi Zhao
Atmos. Chem. Phys., 20, 15937–15967, https://doi.org/10.5194/acp-20-15937-2020, https://doi.org/10.5194/acp-20-15937-2020, 2020
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This is a modelling-based study on Arctic surface ozone, with a particular focus on spring ozone depletion events (i.e. with concentrations < 10 ppbv). Model experiments show that model runs with blowing-snow-sourced sea salt aerosols implemented as a source of reactive bromine can reproduce well large-scale ozone depletion events observed in the Arctic. This study supplies modelling evidence of the proposed mechanism of reactive-bromine release from blowing snow on sea ice (Yang et al., 2008).
Robert J. Parker, Alex Webb, Hartmut Boesch, Peter Somkuti, Rocio Barrio Guillo, Antonio Di Noia, Nikoleta Kalaitzi, Jasdeep S. Anand, Peter Bergamaschi, Frederic Chevallier, Paul I. Palmer, Liang Feng, Nicholas M. Deutscher, Dietrich G. Feist, David W. T. Griffith, Frank Hase, Rigel Kivi, Isamu Morino, Justus Notholt, Young-Suk Oh, Hirofumi Ohyama, Christof Petri, David F. Pollard, Coleen Roehl, Mahesh K. Sha, Kei Shiomi, Kimberly Strong, Ralf Sussmann, Yao Té, Voltaire A. Velazco, Thorsten Warneke, Paul O. Wennberg, and Debra Wunch
Earth Syst. Sci. Data, 12, 3383–3412, https://doi.org/10.5194/essd-12-3383-2020, https://doi.org/10.5194/essd-12-3383-2020, 2020
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This work presents the latest release of the University of Leicester GOSAT methane data and acts as the definitive description of this dataset. We detail the processing, validation and evaluation involved in producing these data and highlight its many applications. With now over a decade of global atmospheric methane observations, this dataset has helped, and will continue to help, us better understand the global methane budget and investigate how it may respond to a future changing climate.
Zoé Rehder, Anne Laura Niederdrenk, Lars Kaleschke, and Lars Kutzbach
The Cryosphere, 14, 4201–4215, https://doi.org/10.5194/tc-14-4201-2020, https://doi.org/10.5194/tc-14-4201-2020, 2020
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To better understand the connection between sea ice and permafrost, we investigate how sea ice interacts with the atmosphere over the adjacent landmass in the Laptev Sea region using a climate model. Melt of sea ice in spring is mainly controlled by the atmosphere; in fall, feedback mechanisms are important. Throughout summer, lower-than-usual sea ice leads to more southward transport of heat and moisture, but these links from sea ice to the atmosphere over land are weak.
Gaia Pinardi, Michel Van Roozendael, François Hendrick, Nicolas Theys, Nader Abuhassan, Alkiviadis Bais, Folkert Boersma, Alexander Cede, Jihyo Chong, Sebastian Donner, Theano Drosoglou, Anatoly Dzhola, Henk Eskes, Udo Frieß, José Granville, Jay R. Herman, Robert Holla, Jari Hovila, Hitoshi Irie, Yugo Kanaya, Dimitris Karagkiozidis, Natalia Kouremeti, Jean-Christopher Lambert, Jianzhong Ma, Enno Peters, Ankie Piters, Oleg Postylyakov, Andreas Richter, Julia Remmers, Hisahiro Takashima, Martin Tiefengraber, Pieter Valks, Tim Vlemmix, Thomas Wagner, and Folkard Wittrock
Atmos. Meas. Tech., 13, 6141–6174, https://doi.org/10.5194/amt-13-6141-2020, https://doi.org/10.5194/amt-13-6141-2020, 2020
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We validate several GOME-2 and OMI tropospheric NO2 products with 23 MAX-DOAS and 16 direct sun instruments distributed worldwide, highlighting large horizontal inhomogeneities at several sites affecting the validation results. We propose a method for quantification and correction. We show the application of such correction reduces the satellite underestimation in almost all heterogeneous cases, but a negative bias remains over the MAX-DOAS and direct sun network ensemble for both satellites.
Erik Lutsch, Kimberly Strong, Dylan B. A. Jones, Thomas Blumenstock, Stephanie Conway, Jenny A. Fisher, James W. Hannigan, Frank Hase, Yasuko Kasai, Emmanuel Mahieu, Maria Makarova, Isamu Morino, Tomoo Nagahama, Justus Notholt, Ivan Ortega, Mathias Palm, Anatoly V. Poberovskii, Ralf Sussmann, and Thorsten Warneke
Atmos. Chem. Phys., 20, 12813–12851, https://doi.org/10.5194/acp-20-12813-2020, https://doi.org/10.5194/acp-20-12813-2020, 2020
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This paper describes the use of a network of 10 Arctic and midlatitude ground-based FTIR measurement sites to detect enhancements of the wildfire tracers carbon monoxide, hydrogen cyanide, and ethane from 2003 to 2018. A tagged CO GEOS-Chem simulation is used for source attribution and to evaluate the relative contribution of CO sources to the FTIR measurements. The use of FTIR measurements allowed for the emission ratios of hydrogen cyanide and ethane to be quantified.
Sora Seo, Andreas Richter, Anne-Marlene Blechschmidt, Ilias Bougoudis, and John Philip Burrows
Atmos. Chem. Phys., 20, 12285–12312, https://doi.org/10.5194/acp-20-12285-2020, https://doi.org/10.5194/acp-20-12285-2020, 2020
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In this study, we present spatial distributions of occurrence frequency of enhanced total BrO column and various meteorological parameters affecting it in the Arctic and Antarctic sea ice regions by using 10 years of GOME-2 measurements and meteorological model data. Statistical analysis using the long-term dataset shows clear differences in the meteorological conditions between the mean field and the situation of enhanced total BrO columns in both polar sea ice regions.
Ilias Bougoudis, Anne-Marlene Blechschmidt, Andreas Richter, Sora Seo, John Philip Burrows, Nicolas Theys, and Annette Rinke
Atmos. Chem. Phys., 20, 11869–11892, https://doi.org/10.5194/acp-20-11869-2020, https://doi.org/10.5194/acp-20-11869-2020, 2020
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A 22-year (1996 to 2017) consistent Arctic tropospheric BrO dataset derived from four satellite remote sensing instruments is presented. An increase in tropospheric BrO VCDs over this period, and especially during polar springs, can be seen. Comparisons of tropospheric BrO VCDs with first-year sea ice reveal a moderate spatial and temporal correlation between the two, suggesting that the increase in first-year sea ice in the Arctic has an impact on tropospheric BrO abundancies.
Stefan Noël, Klaus Bramstedt, Alexei Rozanov, Elizaveta Malinina, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 13, 5643–5666, https://doi.org/10.5194/amt-13-5643-2020, https://doi.org/10.5194/amt-13-5643-2020, 2020
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A new approach to derive stratospheric aerosol extinction profiles from SCIAMACHY solar occultation measurements based on an onion-peeling method is presented. The resulting extinctions at 452, 525 and 750 nm compare well with other limb and occultation data from, e.g. SAGE and SCIAMACHY, but show small oscillating features which vanish in monthly anomalies. Major volcanic eruptions, polar stratospheric clouds and influences of the quasi-biennial oscillation can be identified in the time series.
Alexis Merlaud, Livio Belegante, Daniel-Eduard Constantin, Mirjam Den Hoed, Andreas Carlos Meier, Marc Allaart, Magdalena Ardelean, Maxim Arseni, Tim Bösch, Hugues Brenot, Andreea Calcan, Emmanuel Dekemper, Sebastian Donner, Steffen Dörner, Mariana Carmelia Balanica Dragomir, Lucian Georgescu, Anca Nemuc, Doina Nicolae, Gaia Pinardi, Andreas Richter, Adrian Rosu, Thomas Ruhtz, Anja Schönhardt, Dirk Schuettemeyer, Reza Shaiganfar, Kerstin Stebel, Frederik Tack, Sorin Nicolae Vâjâiac, Jeni Vasilescu, Jurgen Vanhamel, Thomas Wagner, and Michel Van Roozendael
Atmos. Meas. Tech., 13, 5513–5535, https://doi.org/10.5194/amt-13-5513-2020, https://doi.org/10.5194/amt-13-5513-2020, 2020
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The AROMAT campaigns took place in Romania in 2014 and 2015. They aimed to test airborne observation systems dedicated to air quality studies and to verify the concept of such campaigns in support of the validation of space-borne atmospheric missions. We show that airborne measurements of NO2 can be valuable for the validation of air quality satellites. For H2CO and SO2, the validation should involve ground-based measurement systems at key locations that the AROMAT measurements help identify.
Hirofumi Ohyama, Isamu Morino, Voltaire A. Velazco, Theresa Klausner, Gerry Bagtasa, Matthäus Kiel, Matthias Frey, Akihiro Hori, Osamu Uchino, Tsuneo Matsunaga, Nicholas M. Deutscher, Joshua P. DiGangi, Yonghoon Choi, Glenn S. Diskin, Sally E. Pusede, Alina Fiehn, Anke Roiger, Michael Lichtenstern, Hans Schlager, Pao K. Wang, Charles C.-K. Chou, Maria Dolores Andrés-Hernández, and John P. Burrows
Atmos. Meas. Tech., 13, 5149–5163, https://doi.org/10.5194/amt-13-5149-2020, https://doi.org/10.5194/amt-13-5149-2020, 2020
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Column-averaged dry-air mole fractions of CO2 and CH4 measured by a solar viewing portable Fourier transform spectrometer (EM27/SUN) were validated with in situ profile data obtained during the transfer flights of two aircraft campaigns. Atmospheric dynamical properties based on ERA5 and WRF-Chem were used as criteria for selecting the best aircraft profiles for the validation. The resulting air-mass-independent correction factors for the EM27/SUN data were 0.9878 for CO2 and 0.9829 for CH4.
Ilya Stanevich, Dylan B. A. Jones, Kimberly Strong, Robert J. Parker, Hartmut Boesch, Debra Wunch, Justus Notholt, Christof Petri, Thorsten Warneke, Ralf Sussmann, Matthias Schneider, Frank Hase, Rigel Kivi, Nicholas M. Deutscher, Voltaire A. Velazco, Kaley A. Walker, and Feng Deng
Geosci. Model Dev., 13, 3839–3862, https://doi.org/10.5194/gmd-13-3839-2020, https://doi.org/10.5194/gmd-13-3839-2020, 2020
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Systematic errors in atmospheric models pose a challenge for inverse modeling studies of methane (CH4) emissions. We evaluated the CH4 simulation in the GEOS-Chem model at the horizontal resolutions of 4° × 5° and 2° × 2.5°. Our analysis identified resolution-dependent biases in the model, which we attributed to discrepancies between the two model resolutions in vertical transport in the troposphere and in stratosphere–troposphere exchange.
Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Steffen Vanselow, Heinrich Bovensmann, and John P. Burrows
Atmos. Chem. Phys., 20, 9169–9182, https://doi.org/10.5194/acp-20-9169-2020, https://doi.org/10.5194/acp-20-9169-2020, 2020
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The switch from the use of coal to natural gas or oil for energy generation potentially reduces the impact on global warming due to lower CO2 emissions with the same energy content. However, this climate benefit is offset by fugitive methane emissions during the production and distribution process. We quantify emission and leakage rates relative to production for several large production regions based on satellite observations to evaluate the climate footprint of the gas and oil industry.
Tina Hilbig, Klaus Bramstedt, Mark Weber, John P. Burrows, and Matthijs Krijger
Atmos. Meas. Tech., 13, 3893–3907, https://doi.org/10.5194/amt-13-3893-2020, https://doi.org/10.5194/amt-13-3893-2020, 2020
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One of the main limitations for long-term space-based measurements is
instrument degradation. We present an optimisation of the
degradation correction approach (Krijger et al. 2014) for SCIAMACHY
on-board Envisat, focusing on the improvement of the solar spectral
irradiance data. The main achievement of this study is the
successful integration of SCIAMACHY’s internal white light source
(WLS) into the existing degradation model and the
characterisation of WLS ageing in space.
Steven Compernolle, Tijl Verhoelst, Gaia Pinardi, José Granville, Daan Hubert, Arno Keppens, Sander Niemeijer, Bruno Rino, Alkis Bais, Steffen Beirle, Folkert Boersma, John P. Burrows, Isabelle De Smedt, Henk Eskes, Florence Goutail, François Hendrick, Alba Lorente, Andrea Pazmino, Ankie Piters, Enno Peters, Jean-Pierre Pommereau, Julia Remmers, Andreas Richter, Jos van Geffen, Michel Van Roozendael, Thomas Wagner, and Jean-Christopher Lambert
Atmos. Chem. Phys., 20, 8017–8045, https://doi.org/10.5194/acp-20-8017-2020, https://doi.org/10.5194/acp-20-8017-2020, 2020
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Tropospheric and stratospheric NO2 columns from the OMI QA4ECV NO2 satellite product are validated by comparison with ground-based measurements at 11 sites. The OMI stratospheric column has a small negative bias, and the OMI tropospheric column has a stronger negative bias relative to the ground-based data. Discrepancies are attributed to comparison errors (e.g. difference in horizontal smoothing) and measurement errors (e.g. clouds, aerosols, vertical smoothing and a priori profile assumptions).
Corinne Vigouroux, Bavo Langerock, Carlos Augusto Bauer Aquino, Thomas Blumenstock, Zhibin Cheng, Martine De Mazière, Isabelle De Smedt, Michel Grutter, James W. Hannigan, Nicholas Jones, Rigel Kivi, Diego Loyola, Erik Lutsch, Emmanuel Mahieu, Maria Makarova, Jean-Marc Metzger, Isamu Morino, Isao Murata, Tomoo Nagahama, Justus Notholt, Ivan Ortega, Mathias Palm, Gaia Pinardi, Amelie Röhling, Dan Smale, Wolfgang Stremme, Kim Strong, Ralf Sussmann, Yao Té, Michel van Roozendael, Pucai Wang, and Holger Winkler
Atmos. Meas. Tech., 13, 3751–3767, https://doi.org/10.5194/amt-13-3751-2020, https://doi.org/10.5194/amt-13-3751-2020, 2020
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We validate the TROPOMI HCHO product with ground-based FTIR (Fourier-transform infrared) measurements from 25 stations. We find that TROPOMI overestimates HCHO under clean conditions, while it underestimates it at high HCHO levels. Both TROPOMI precision and accuracy reach the pre-launch requirements, and its precision can even be 2 times better. The observed TROPOMI seasonal variability is in agreement with the FTIR data. The TROPOMI random uncertainty and data filtering should be refined.
Thomas Krumpen, Florent Birrien, Frank Kauker, Thomas Rackow, Luisa von Albedyll, Michael Angelopoulos, H. Jakob Belter, Vladimir Bessonov, Ellen Damm, Klaus Dethloff, Jari Haapala, Christian Haas, Carolynn Harris, Stefan Hendricks, Jens Hoelemann, Mario Hoppmann, Lars Kaleschke, Michael Karcher, Nikolai Kolabutin, Ruibo Lei, Josefine Lenz, Anne Morgenstern, Marcel Nicolaus, Uwe Nixdorf, Tomash Petrovsky, Benjamin Rabe, Lasse Rabenstein, Markus Rex, Robert Ricker, Jan Rohde, Egor Shimanchuk, Suman Singha, Vasily Smolyanitsky, Vladimir Sokolov, Tim Stanton, Anna Timofeeva, Michel Tsamados, and Daniel Watkins
The Cryosphere, 14, 2173–2187, https://doi.org/10.5194/tc-14-2173-2020, https://doi.org/10.5194/tc-14-2173-2020, 2020
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In October 2019 the research vessel Polarstern was moored to an ice floe in order to travel with it on the 1-year-long MOSAiC journey through the Arctic. Here we provide historical context of the floe's evolution and initial state for upcoming studies. We show that the ice encountered on site was exceptionally thin and was formed on the shallow Siberian shelf. The analyses presented provide the initial state for the analysis and interpretation of upcoming biogeochemical and ecological studies.
Jiayue Huang, Lyatt Jaeglé, Qianjie Chen, Becky Alexander, Tomás Sherwen, Mat J. Evans, Nicolas Theys, and Sungyeon Choi
Atmos. Chem. Phys., 20, 7335–7358, https://doi.org/10.5194/acp-20-7335-2020, https://doi.org/10.5194/acp-20-7335-2020, 2020
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Large-scale enhancements of tropospheric BrO and the depletion of surface ozone are often observed in the springtime Arctic. Here, we use a chemical transport model to examine the role of sea salt aerosol from blowing snow in explaining these phenomena. We find that our simulation can account for the spatiotemporal variability of satellite observations of BrO. However, the model has difficulty in producing the magnitude of observed ozone depletion events.
Marcus Hirtl, Delia Arnold, Rocio Baro, Hugues Brenot, Mauro Coltelli, Kurt Eschbacher, Helmut Hard-Stremayer, Florian Lipok, Christian Maurer, Dieter Meinhard, Lucia Mona, Marie D. Mulder, Nikolaos Papagiannopoulos, Michael Pernsteiner, Matthieu Plu, Lennart Robertson, Carl-Herbert Rokitansky, Barbara Scherllin-Pirscher, Klaus Sievers, Mikhail Sofiev, Wim Som de Cerff, Martin Steinheimer, Martin Stuefer, Nicolas Theys, Andreas Uppstu, Saskia Wagenaar, Roland Winkler, Gerhard Wotawa, Fritz Zobl, and Raimund Zopp
Nat. Hazards Earth Syst. Sci., 20, 1719–1739, https://doi.org/10.5194/nhess-20-1719-2020, https://doi.org/10.5194/nhess-20-1719-2020, 2020
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The paper summarizes the set-up and outcome of a volcanic-hazard demonstration exercise, with the goals of assessing and mitigating the impacts of volcanic ash clouds on civil and military aviation. Experts in the field simulated the sequence of procedures for an artificial eruption of the Etna volcano in Italy. The scope of the exercise ranged from the detection of the assumed event to the issuance of early warnings and optimized rerouting of flights.
Midhun George, Maria Dolores Andrés Hernández, Vladyslav Nenakhov, Yangzhuoran Liu, and John Philip Burrows
Atmos. Meas. Tech., 13, 2577–2600, https://doi.org/10.5194/amt-13-2577-2020, https://doi.org/10.5194/amt-13-2577-2020, 2020
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The accurate measurement of peroxy radicals is essential for understanding the chemistry of air masses probed in the free troposphere. The PeRCEAS instrument has been designed, developed and thoroughly characterised for the measurement of the total sum of peroxy radicals (RO2*) aboard airborne platforms. Parameters expected to affect the precision and accuracy of the measurement have been investigated in detail.
Vitali Fioletov, Chris A. McLinden, Debora Griffin, Nicolas Theys, Diego G. Loyola, Pascal Hedelt, Nickolay A. Krotkov, and Can Li
Atmos. Chem. Phys., 20, 5591–5607, https://doi.org/10.5194/acp-20-5591-2020, https://doi.org/10.5194/acp-20-5591-2020, 2020
Youwen Sun, Cheng Liu, Lin Zhang, Mathias Palm, Justus Notholt, Hao Yin, Corinne Vigouroux, Erik Lutsch, Wei Wang, Changong Shan, Thomas Blumenstock, Tomoo Nagahama, Isamu Morino, Emmanuel Mahieu, Kimberly Strong, Bavo Langerock, Martine De Mazière, Qihou Hu, Huifang Zhang, Christof Petri, and Jianguo Liu
Atmos. Chem. Phys., 20, 5437–5456, https://doi.org/10.5194/acp-20-5437-2020, https://doi.org/10.5194/acp-20-5437-2020, 2020
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We present multiyear time series of ground-based Fourier-transform infrared spectroscopy measurements of HCN in densely populated eastern China. The seasonality and interannual variability of tropospheric HCN columns were investigated. The potential sources that drive the observed HCN seasonality and interannual variability were determined using a GEOS-Chem tagged CO simulation, global fire maps, and potential source contribution function values calculated using HYSPLIT back trajectories.
Karin Kreher, Michel Van Roozendael, Francois Hendrick, Arnoud Apituley, Ermioni Dimitropoulou, Udo Frieß, Andreas Richter, Thomas Wagner, Johannes Lampel, Nader Abuhassan, Li Ang, Monica Anguas, Alkis Bais, Nuria Benavent, Tim Bösch, Kristof Bognar, Alexander Borovski, Ilya Bruchkouski, Alexander Cede, Ka Lok Chan, Sebastian Donner, Theano Drosoglou, Caroline Fayt, Henning Finkenzeller, David Garcia-Nieto, Clio Gielen, Laura Gómez-Martín, Nan Hao, Bas Henzing, Jay R. Herman, Christian Hermans, Syedul Hoque, Hitoshi Irie, Junli Jin, Paul Johnston, Junaid Khayyam Butt, Fahim Khokhar, Theodore K. Koenig, Jonas Kuhn, Vinod Kumar, Cheng Liu, Jianzhong Ma, Alexis Merlaud, Abhishek K. Mishra, Moritz Müller, Monica Navarro-Comas, Mareike Ostendorf, Andrea Pazmino, Enno Peters, Gaia Pinardi, Manuel Pinharanda, Ankie Piters, Ulrich Platt, Oleg Postylyakov, Cristina Prados-Roman, Olga Puentedura, Richard Querel, Alfonso Saiz-Lopez, Anja Schönhardt, Stefan F. Schreier, André Seyler, Vinayak Sinha, Elena Spinei, Kimberly Strong, Frederik Tack, Xin Tian, Martin Tiefengraber, Jan-Lukas Tirpitz, Jeroen van Gent, Rainer Volkamer, Mihalis Vrekoussis, Shanshan Wang, Zhuoru Wang, Mark Wenig, Folkard Wittrock, Pinhua H. Xie, Jin Xu, Margarita Yela, Chengxin Zhang, and Xiaoyi Zhao
Atmos. Meas. Tech., 13, 2169–2208, https://doi.org/10.5194/amt-13-2169-2020, https://doi.org/10.5194/amt-13-2169-2020, 2020
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In September 2016, 36 spectrometers from 24 institutes measured a number of key atmospheric pollutants during an instrument intercomparison campaign (CINDI-2) at Cabauw, the Netherlands. Here we report on the outcome of this intercomparison exercise. The three major goals were to characterise the differences between the participating instruments, to define a robust methodology for performance assessment, and to contribute to the harmonisation of the measurement settings and retrieval methods.
Adrianus de Laat, Margarita Vazquez-Navarro, Nicolas Theys, and Piet Stammes
Nat. Hazards Earth Syst. Sci., 20, 1203–1217, https://doi.org/10.5194/nhess-20-1203-2020, https://doi.org/10.5194/nhess-20-1203-2020, 2020
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TROPOMI satellite measurements can accurately determine the height of thick volcanic ash clouds from a short-lived volcanic eruption of the Sinabung volcano in Indonesia. Standard geostationary satellite detection of volcanic ash was limited due to the presence of water and ice in the upper parts of volcanic ash clouds, a known issue. The TROPOMI satellite measurements do not suffer from this limitation, hence providing information where standard geostationary volcanic ash detection is limited.
Xiaoyi Zhao, Debora Griffin, Vitali Fioletov, Chris McLinden, Alexander Cede, Martin Tiefengraber, Moritz Müller, Kristof Bognar, Kimberly Strong, Folkert Boersma, Henk Eskes, Jonathan Davies, Akira Ogyu, and Sum Chi Lee
Atmos. Meas. Tech., 13, 2131–2159, https://doi.org/10.5194/amt-13-2131-2020, https://doi.org/10.5194/amt-13-2131-2020, 2020
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Pandora NO2 measurements made at three sites located in the Toronto area are used to evaluate the TROPOspheric Monitoring Instrument (TROPOMI) NO2 data products, including standard NO2 and research data developed using a high-resolution regional air quality forecast model. TROPOMI pixels located upwind and downwind from the Pandora sites were analyzed by a new wind-based validation method, which revealed the spatial patterns of local and transported emissions and regional air quality changes.
Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, and John P. Burrows
Atmos. Chem. Phys., 20, 3317–3332, https://doi.org/10.5194/acp-20-3317-2020, https://doi.org/10.5194/acp-20-3317-2020, 2020
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As a consequence of climate change, droughts in California are occurring more often, providing ample fuel for destructive wildfires. The associated smoke is reducing air quality as it contains pollutants considered harmful to public health and the environment such as carbon monoxide (CO). We analyse the statewide distribution of CO during the first days of two specific wildfires using satellite measurements and assess the corresponding air quality burden in major Californian cities.
Anne-Marlene Blechschmidt, Joaquim Arteta, Adriana Coman, Lyana Curier, Henk Eskes, Gilles Foret, Clio Gielen, Francois Hendrick, Virginie Marécal, Frédérik Meleux, Jonathan Parmentier, Enno Peters, Gaia Pinardi, Ankie J. M. Piters, Matthieu Plu, Andreas Richter, Arjo Segers, Mikhail Sofiev, Álvaro M. Valdebenito, Michel Van Roozendael, Julius Vira, Tim Vlemmix, and John P. Burrows
Atmos. Chem. Phys., 20, 2795–2823, https://doi.org/10.5194/acp-20-2795-2020, https://doi.org/10.5194/acp-20-2795-2020, 2020
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MAX-DOAS tropospheric NO2 vertical column retrievals from a set of European measurement stations are compared to regional air quality models which contribute to the operational Copernicus Atmosphere Monitoring Service (CAMS). Correlations are on the order of 35 %–75 %; large differences occur for individual pollution plumes. The results demonstrate that future model development needs to concentrate on improving representation of diurnal cycles and associated temporal scalings.
Leonardo M. A. Alvarado, Andreas Richter, Mihalis Vrekoussis, Andreas Hilboll, Anna B. Kalisz Hedegaard, Oliver Schneising, and John P. Burrows
Atmos. Chem. Phys., 20, 2057–2072, https://doi.org/10.5194/acp-20-2057-2020, https://doi.org/10.5194/acp-20-2057-2020, 2020
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We present CHOCHO and HCHO columns retrieved from measurements by TROPOMI. Elevated amounts of CHOCHO and HCHO are observed during the fire season in BC, Canada, where a large number of fires occurred in 2018. CHOCHO and HCHO plumes from individual fires are observed in air masses travelling over distances of up to 1500 km. Comparison with FLEXPART simulations with different lifetimes shows that effective lifetimes of 20 h and more are needed to explain the observations.
Maximilian Reuter, Michael Buchwitz, Oliver Schneising, Stefan Noël, Heinrich Bovensmann, John P. Burrows, Hartmut Boesch, Antonio Di Noia, Jasdeep Anand, Robert J. Parker, Peter Somkuti, Lianghai Wu, Otto P. Hasekamp, Ilse Aben, Akihiko Kuze, Hiroshi Suto, Kei Shiomi, Yukio Yoshida, Isamu Morino, David Crisp, Christopher W. O'Dell, Justus Notholt, Christof Petri, Thorsten Warneke, Voltaire A. Velazco, Nicholas M. Deutscher, David W. T. Griffith, Rigel Kivi, David F. Pollard, Frank Hase, Ralf Sussmann, Yao V. Té, Kimberly Strong, Sébastien Roche, Mahesh K. Sha, Martine De Mazière, Dietrich G. Feist, Laura T. Iraci, Coleen M. Roehl, Christian Retscher, and Dinand Schepers
Atmos. Meas. Tech., 13, 789–819, https://doi.org/10.5194/amt-13-789-2020, https://doi.org/10.5194/amt-13-789-2020, 2020
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We present new satellite-derived data sets of atmospheric carbon dioxide (CO2) and methane (CH4). The data products are column-averaged dry-air mole fractions of CO2 and CH4, denoted XCO2 and XCH4. The products cover the years 2003–2018 and are merged Level 2 (satellite footprints) and merged Level 3 (gridded at monthly time and 5° x 5° spatial resolution) products obtained from combining several individual sensor products. We present the merging algorithms and product validation results.
Sebastian Donner, Jonas Kuhn, Michel Van Roozendael, Alkiviadis Bais, Steffen Beirle, Tim Bösch, Kristof Bognar, Ilya Bruchkouski, Ka Lok Chan, Steffen Dörner, Theano Drosoglou, Caroline Fayt, Udo Frieß, François Hendrick, Christian Hermans, Junli Jin, Ang Li, Jianzhong Ma, Enno Peters, Gaia Pinardi, Andreas Richter, Stefan F. Schreier, André Seyler, Kimberly Strong, Jan-Lukas Tirpitz, Yang Wang, Pinhua Xie, Jin Xu, Xiaoyi Zhao, and Thomas Wagner
Atmos. Meas. Tech., 13, 685–712, https://doi.org/10.5194/amt-13-685-2020, https://doi.org/10.5194/amt-13-685-2020, 2020
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The calibration of the elevation angles of MAX-DOAS instruments is important for the correct interpretation of such MAX-DOAS measurements. We present and evaluate different methods for the elevation calibration of MAX-DOAS instruments which were applied during the CINDI-2 field campaign.
Maciej Miernecki, Lars Kaleschke, Nina Maaß, Stefan Hendricks, and Sten Schmidl Søbjærg
The Cryosphere, 14, 461–476, https://doi.org/10.5194/tc-14-461-2020, https://doi.org/10.5194/tc-14-461-2020, 2020
Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, John P. Burrows, Tobias Borsdorff, Nicholas M. Deutscher, Dietrich G. Feist, David W. T. Griffith, Frank Hase, Christian Hermans, Laura T. Iraci, Rigel Kivi, Jochen Landgraf, Isamu Morino, Justus Notholt, Christof Petri, David F. Pollard, Sébastien Roche, Kei Shiomi, Kimberly Strong, Ralf Sussmann, Voltaire A. Velazco, Thorsten Warneke, and Debra Wunch
Atmos. Meas. Tech., 12, 6771–6802, https://doi.org/10.5194/amt-12-6771-2019, https://doi.org/10.5194/amt-12-6771-2019, 2019
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We introduce an algorithm that is used to simultaneously derive the abundances of the important atmospheric constituents carbon monoxide and methane from the TROPOMI instrument onboard the Sentinel-5 Precursor satellite, which enables the determination of both gases with an unprecedented level of detail on a global scale. The quality of the resulting data sets is assessed and the first results are presented.
André Seyler, Andreas C. Meier, Folkard Wittrock, Lisa Kattner, Barbara Mathieu-Üffing, Enno Peters, Andreas Richter, Thomas Ruhtz, Anja Schönhardt, Stefan Schmolke, and John P. Burrows
Atmos. Meas. Tech., 12, 5959–5977, https://doi.org/10.5194/amt-12-5959-2019, https://doi.org/10.5194/amt-12-5959-2019, 2019
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This study describes a novel application of an
onion-peelingapproach to MAX-DOAS measurements of shipping emissions to study the inhomogeneous NO2 field above a shipping lane. It is shown how the method can be used to derive the approximate plume positions in the observed area, and, by using a simple Gaussian plume model, to calculate in-plume NO2 volume mixing ratios. For validation, a comparison to airborne imaging DOAS measurements during the NOSE campaign in July 2013 is included.
Susan S. Kulawik, Sean Crowell, David Baker, Junjie Liu, Kathryn McKain, Colm Sweeney, Sebastien C. Biraud, Steve Wofsy, Christopher W. O'Dell, Paul O. Wennberg, Debra Wunch, Coleen M. Roehl, Nicholas M. Deutscher, Matthäus Kiel, David W. T. Griffith, Voltaire A. Velazco, Justus Notholt, Thorsten Warneke, Christof Petri, Martine De Mazière, Mahesh K. Sha, Ralf Sussmann, Markus Rettinger, Dave F. Pollard, Isamu Morino, Osamu Uchino, Frank Hase, Dietrich G. Feist, Sébastien Roche, Kimberly Strong, Rigel Kivi, Laura Iraci, Kei Shiomi, Manvendra K. Dubey, Eliezer Sepulveda, Omaira Elena Garcia Rodriguez, Yao Té, Pascal Jeseck, Pauli Heikkinen, Edward J. Dlugokencky, Michael R. Gunson, Annmarie Eldering, David Crisp, Brendan Fisher, and Gregory B. Osterman
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2019-257, https://doi.org/10.5194/amt-2019-257, 2019
Publication in AMT not foreseen
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This paper provides a benchmark of OCO-2 v8 and ACOS-GOSAT v7.3 XCO2 and lowermost tropospheric (LMT) errors. The paper focuses on the systematic errors and subtracts out validation, co-location, and random errors, looks at the correlation scale-length (spatially and temporally) of systematic errors, finding that the scale lengths are similar to bias correction scale-lengths. The assimilates of the bias correction term is used to place an error on fluxes estimates.
Brendan Byrne, Dylan B. A. Jones, Kimberly Strong, Saroja M. Polavarapu, Anna B. Harper, David F. Baker, and Shamil Maksyutov
Atmos. Chem. Phys., 19, 13017–13035, https://doi.org/10.5194/acp-19-13017-2019, https://doi.org/10.5194/acp-19-13017-2019, 2019
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Interannual variations in net ecosystem exchange (NEE) estimated from the Greenhouse Gases Observing Satellite (GOSAT) XCO2 measurements are shown to be correlated (P < 0.05) with temperature and FLUXCOM NEE anomalies. Furthermore, the GOSAT-informed NEE anomalies are found to be better correlated with temperature and FLUXCOM anomalies than NEE estimates from most terrestrial biosphere models, suggesting that GOSAT CO2 measurements provide a useful constraint on NEE interannual variability.
Jacob K. Hedelius, Tai-Long He, Dylan B. A. Jones, Bianca C. Baier, Rebecca R. Buchholz, Martine De Mazière, Nicholas M. Deutscher, Manvendra K. Dubey, Dietrich G. Feist, David W. T. Griffith, Frank Hase, Laura T. Iraci, Pascal Jeseck, Matthäus Kiel, Rigel Kivi, Cheng Liu, Isamu Morino, Justus Notholt, Young-Suk Oh, Hirofumi Ohyama, David F. Pollard, Markus Rettinger, Sébastien Roche, Coleen M. Roehl, Matthias Schneider, Kei Shiomi, Kimberly Strong, Ralf Sussmann, Colm Sweeney, Yao Té, Osamu Uchino, Voltaire A. Velazco, Wei Wang, Thorsten Warneke, Paul O. Wennberg, Helen M. Worden, and Debra Wunch
Atmos. Meas. Tech., 12, 5547–5572, https://doi.org/10.5194/amt-12-5547-2019, https://doi.org/10.5194/amt-12-5547-2019, 2019
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We seek ways to improve the accuracy of column measurements of carbon monoxide (CO) – an important tracer of pollution – made from the MOPITT satellite instrument. We devise a filtering scheme which reduces the scatter and also eliminates bias among the MOPITT detectors. Compared to ground-based observations, MOPITT measurements are about 6 %–8 % higher. When MOPITT data are implemented in a global assimilation model, they tend to reduce the model mismatch with aircraft measurements.
Xiaoyi Zhao, Debora Griffin, Vitali Fioletov, Chris McLinden, Jonathan Davies, Akira Ogyu, Sum Chi Lee, Alexandru Lupu, Michael D. Moran, Alexander Cede, Martin Tiefengraber, and Moritz Müller
Atmos. Chem. Phys., 19, 10619–10642, https://doi.org/10.5194/acp-19-10619-2019, https://doi.org/10.5194/acp-19-10619-2019, 2019
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New nitrogen dioxide (NO2) retrieval algorithms are developed for Pandora zenith-sky measurements. A column-to-surface conversion look-up table was produced for the Pandora instruments; therefore, quick and practical Pandora-based surface NO2 concentration data can be obtained for air quality monitoring purposes. It is demonstrated that the surface NO2 concentration is controlled not only by the planetary boundary layer height but also by both boundary layer dynamics and photochemistry.
Lisa K. Behrens, Andreas Hilboll, Andreas Richter, Enno Peters, Leonardo M. A. Alvarado, Anna B. Kalisz Hedegaard, Folkard Wittrock, John P. Burrows, and Mihalis Vrekoussis
Atmos. Chem. Phys., 19, 10257–10278, https://doi.org/10.5194/acp-19-10257-2019, https://doi.org/10.5194/acp-19-10257-2019, 2019
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MAX-DOAS measurements were conducted on the research vessel Maria S. Merian during a cruise from the Azores to South Africa in October 2016. The measurements indicate enhanced levels of HCHO and CHOCHO over the remote Atlantic Ocean, which is unexpected due to their short lifetime. Precursors of these gases or gas–aerosol combinations might be transported. Model simulations indicate potential source regions over the African continent, probably related to biomass burning or biogenic emissions.
Enno Peters, Mareike Ostendorf, Tim Bösch, André Seyler, Anja Schönhardt, Stefan F. Schreier, Jeroen Sebastiaan Henzing, Folkard Wittrock, Andreas Richter, Mihalis Vrekoussis, and John P. Burrows
Atmos. Meas. Tech., 12, 4171–4190, https://doi.org/10.5194/amt-12-4171-2019, https://doi.org/10.5194/amt-12-4171-2019, 2019
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A novel imaging-DOAS instrument (IMPACT) is presented for measurements of nitrogen dioxide (NO2) in the atmosphere. The instrument combines full-azimuthal pointing (360°) with a large vertical coverage (40°). Complete panoramic scans and vertical NO2 profiles around the measurement site are acquired at a temporal resolution of 15 min. In addition, information about the aerosol phase function is retrieved from O4 slant columns along multiple almucantar scans measured simultaneously by IMPACT.
Dan Weaver, Kimberly Strong, Kaley A. Walker, Chris Sioris, Matthias Schneider, C. Thomas McElroy, Holger Vömel, Michael Sommer, Katja Weigel, Alexei Rozanov, John P. Burrows, William G. Read, Evan Fishbein, and Gabriele Stiller
Atmos. Meas. Tech., 12, 4039–4063, https://doi.org/10.5194/amt-12-4039-2019, https://doi.org/10.5194/amt-12-4039-2019, 2019
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This work assesses water vapour profiles acquired by Atmospheric Chemistry Experiment (ACE) satellite instruments in the upper troposphere and lower stratosphere (UTLS) using comparisons to radiosondes and ground-based Fourier transform infrared spectrometer measurements acquired at a Canadian high Arctic measurement site in Eureka, Nunavut. Additional comparisons are made between these Eureka measurements and other water vapour satellite datasets for context, including AIRS, MLS, and others.
Maximilian Reuter, Michael Buchwitz, Oliver Schneising, Sven Krautwurst, Christopher W. O'Dell, Andreas Richter, Heinrich Bovensmann, and John P. Burrows
Atmos. Chem. Phys., 19, 9371–9383, https://doi.org/10.5194/acp-19-9371-2019, https://doi.org/10.5194/acp-19-9371-2019, 2019
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The quantification of anthropogenic emissions with current CO2 satellite sensors is difficult, but NO2 is co-emitted, making it a suitable tracer of recently emitted CO2. We analyze enhancements of CO2 and NO2 observed by OCO-2 and S5P and estimate the CO2 plume cross-sectional fluxes that we compare with emission databases. Our results demonstrate the usefulness of simultaneous satellite observations of CO2 and NO2 as envisaged for the European Copernicus anthropogenic CO2 monitoring mission
Hyeong-Ahn Kwon, Rokjin J. Park, Gonzalo González Abad, Kelly Chance, Thomas P. Kurosu, Jhoon Kim, Isabelle De Smedt, Michel Van Roozendael, Enno Peters, and John Burrows
Atmos. Meas. Tech., 12, 3551–3571, https://doi.org/10.5194/amt-12-3551-2019, https://doi.org/10.5194/amt-12-3551-2019, 2019
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The Geostationary Environment Monitoring Spectrometer (GEMS) will be launched by South Korea in 2019, and it will measure radiances ranging from 300 to 500 nm every hour with a fine spatial resolution of 7 km x 8 km over Seoul in South Korea to monitor column concentrations of air pollutants including O3, NO2, SO2, and HCHO, as well as aerosol optical properties. This paper describes a GEMS formaldehyde retrieval algorithm including a number of sensitivity tests for algorithm evaluation.
Elizaveta Malinina, Alexei Rozanov, Landon Rieger, Adam Bourassa, Heinrich Bovensmann, John P. Burrows, and Doug Degenstein
Atmos. Meas. Tech., 12, 3485–3502, https://doi.org/10.5194/amt-12-3485-2019, https://doi.org/10.5194/amt-12-3485-2019, 2019
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This paper covers the problems related to the derivation of aerosol extinction coefficients and Ångström exponents from space-borne instruments working in limb and occultation viewing geometries. Aerosol extinction coefficients and Ångström exponents were calculated from the SCIAMACHY aerosol particle size data set. The results were compared with the data from SAGE II and OSIRIS. The Ångström exponent in the tropical regions and its dependency on particle size parameters are discussed.
Sora Seo, Andreas Richter, Anne-Marlene Blechschmidt, Ilias Bougoudis, and John Philip Burrows
Atmos. Meas. Tech., 12, 2913–2932, https://doi.org/10.5194/amt-12-2913-2019, https://doi.org/10.5194/amt-12-2913-2019, 2019
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TROPOMI on board the Copernicus Sentinel-5 Precursor platform can measure various atmospheric compositions at high spatial resolution and improved spectral resolution compared to its predecessors. Bromine monoxide (BrO) is one of the gases that can be derived from the measured radiances of TROPOMI using the differential optical absorption spectroscopy method. In this paper, we present the first retrieval results of BrO column amounts from TROPOMI observations on global and regional scales.
Thomas Wagner, Steffen Beirle, Nuria Benavent, Tim Bösch, Ka Lok Chan, Sebastian Donner, Steffen Dörner, Caroline Fayt, Udo Frieß, David García-Nieto, Clio Gielen, David González-Bartolome, Laura Gomez, François Hendrick, Bas Henzing, Jun Li Jin, Johannes Lampel, Jianzhong Ma, Kornelia Mies, Mónica Navarro, Enno Peters, Gaia Pinardi, Olga Puentedura, Janis Puķīte, Julia Remmers, Andreas Richter, Alfonso Saiz-Lopez, Reza Shaiganfar, Holger Sihler, Michel Van Roozendael, Yang Wang, and Margarita Yela
Atmos. Meas. Tech., 12, 2745–2817, https://doi.org/10.5194/amt-12-2745-2019, https://doi.org/10.5194/amt-12-2745-2019, 2019
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In this study the consistency between MAX-DOAS measurements and radiative transfer simulations of the atmospheric O4 absorption is investigated. The study is based on measurements (2 selected days during the MADCAT campaign) as well as synthetic spectra. The uncertainties of all relevant aspects (spectral retrieval and radiative transfer simulations) are quantified. For one of the selected days, measurements and simulations do not agree within their uncertainties.
Stefan Lossow, Farahnaz Khosrawi, Michael Kiefer, Kaley A. Walker, Jean-Loup Bertaux, Laurent Blanot, James M. Russell, Ellis E. Remsberg, John C. Gille, Takafumi Sugita, Christopher E. Sioris, Bianca M. Dinelli, Enzo Papandrea, Piera Raspollini, Maya García-Comas, Gabriele P. Stiller, Thomas von Clarmann, Anu Dudhia, William G. Read, Gerald E. Nedoluha, Robert P. Damadeo, Joseph M. Zawodny, Katja Weigel, Alexei Rozanov, Faiza Azam, Klaus Bramstedt, Stefan Noël, John P. Burrows, Hideo Sagawa, Yasuko Kasai, Joachim Urban, Patrick Eriksson, Donal P. Murtagh, Mark E. Hervig, Charlotta Högberg, Dale F. Hurst, and Karen H. Rosenlof
Atmos. Meas. Tech., 12, 2693–2732, https://doi.org/10.5194/amt-12-2693-2019, https://doi.org/10.5194/amt-12-2693-2019, 2019
Stefan F. Schreier, Andreas Richter, and John P. Burrows
Atmos. Chem. Phys., 19, 5853–5879, https://doi.org/10.5194/acp-19-5853-2019, https://doi.org/10.5194/acp-19-5853-2019, 2019
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In this case stuy, we have coupled ground-based remote-sensing measurements with surface in situ measurements to investigate NO2 distributions in the planetary boundary layer in the Viennese metropolitan area. We find that the application of a novel linear regression analysis for the conversion of tropospheric NO2 vertical columns into near-surface NO2 mixing ratios is promising and thus the method needs to be further explored and tested on satellite observations in future studies.
Samantha Tremblay, Jean-Christophe Picard, Jill O. Bachelder, Erik Lutsch, Kimberly Strong, Pierre Fogal, W. Richard Leaitch, Sangeeta Sharma, Felicia Kolonjari, Christopher J. Cox, Rachel Y.-W. Chang, and Patrick L. Hayes
Atmos. Chem. Phys., 19, 5589–5604, https://doi.org/10.5194/acp-19-5589-2019, https://doi.org/10.5194/acp-19-5589-2019, 2019
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Atmospheric aerosols, tiny airborne particles, have an important impact on climate. However, a lack of understanding of the chemistry of aerosols is one of the largest contributors to uncertainty in predictions of climate change. Measurements of aerosols were carried out in the Arctic at Eureka Station, Canada, to better understand what role aerosols play in this fragile environment. It is found that organic aerosols, possibly originating from marine emissions, are ubiquitous during summertime.
Yang Wang, Steffen Dörner, Sebastian Donner, Sebastian Böhnke, Isabelle De Smedt, Russell R. Dickerson, Zipeng Dong, Hao He, Zhanqing Li, Zhengqiang Li, Donghui Li, Dong Liu, Xinrong Ren, Nicolas Theys, Yuying Wang, Yang Wang, Zhenzhu Wang, Hua Xu, Jiwei Xu, and Thomas Wagner
Atmos. Chem. Phys., 19, 5417–5449, https://doi.org/10.5194/acp-19-5417-2019, https://doi.org/10.5194/acp-19-5417-2019, 2019
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A MAX-DOAS instrument was operated to derive tropospheric vertical profiles of NO2, SO2, HONO, HCHO, CHOCHO and aerosols in the central western North China Plain in May and June 2016. The MAX-DOAS results are verified by comparisons with a collocated Raman lidar, overpass aircraft measurements, a sun photometer and in situ measurements. The contributions of regional transports and local emissions to the pollutants are evaluated based on case studies and statistic analysis.
Xiaoyi Zhao, Kristof Bognar, Vitali Fioletov, Andrea Pazmino, Florence Goutail, Luis Millán, Gloria Manney, Cristen Adams, and Kimberly Strong
Atmos. Meas. Tech., 12, 2463–2483, https://doi.org/10.5194/amt-12-2463-2019, https://doi.org/10.5194/amt-12-2463-2019, 2019
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Ozone is one of the most widely monitored trace gases in the atmosphere. It can be measured via its strong absorption bands in the ultraviolet (UV), visible (Vis) and infrared (IR) portions of the spectrum. Using multiple ground-based measurements and modeled data, this work provides a measurement-based evaluation of the impact of clouds on UV-visible total column ozone measurements in the high Arctic.
Carlo Arosio, Alexei Rozanov, Elizaveta Malinina, Mark Weber, and John P. Burrows
Atmos. Meas. Tech., 12, 2423–2444, https://doi.org/10.5194/amt-12-2423-2019, https://doi.org/10.5194/amt-12-2423-2019, 2019
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The aim of this study is the merging of stratospheric ozone profiles from three satellite data sets. The merged time series is used to compute long-term changes as a function of altitude, latitude and longitude to study the evolution of the ozone layer over 1985–2018. During the last 16 years we found positive trends in the upper stratosphere at mid latitudes, a large variability of the ozone changes as a function of longitude and a fluctuation in the tropical middle stratospheric trend.
Elisa Carboni, Tamsin A. Mather, Anja Schmidt, Roy G. Grainger, Melissa A. Pfeffer, Iolanda Ialongo, and Nicolas Theys
Atmos. Chem. Phys., 19, 4851–4862, https://doi.org/10.5194/acp-19-4851-2019, https://doi.org/10.5194/acp-19-4851-2019, 2019
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The 2014–2015 Holuhraun eruption was the largest in Iceland for 200 years, emitting huge quantities of gas into the troposphere, at times overwhelming European anthropogenic emissions. Infrared Atmospheric sounding Interferometer data are used to derive the first time series of daily sulfur dioxide mass and vertical distribution over the eruption period. A scheme is used to estimate sulfur dioxide fluxes, the total erupted mass, and how long the sulfur dioxide remains in the atmosphere.
Udo Frieß, Steffen Beirle, Leonardo Alvarado Bonilla, Tim Bösch, Martina M. Friedrich, François Hendrick, Ankie Piters, Andreas Richter, Michel van Roozendael, Vladimir V. Rozanov, Elena Spinei, Jan-Lukas Tirpitz, Tim Vlemmix, Thomas Wagner, and Yang Wang
Atmos. Meas. Tech., 12, 2155–2181, https://doi.org/10.5194/amt-12-2155-2019, https://doi.org/10.5194/amt-12-2155-2019, 2019
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Multi-axis differential optical absorption spectroscopy (MAX-DOAS) is a widely used measurement technique for the detection of a variety of atmospheric trace gases. It enables the retrieval of aerosol and trace gas vertical profiles in the atmospheric boundary layer using appropriate retrieval algorithms. In this study, the ability of eight profile retrieval algorithms to reconstruct vertical profiles is assessed on the basis of synthetic measurements.
Raid M. Suleiman, Kelly Chance, Xiong Liu, Gonzalo González Abad, Thomas P. Kurosu, Francois Hendrick, and Nicolas Theys
Atmos. Meas. Tech., 12, 2067–2084, https://doi.org/10.5194/amt-12-2067-2019, https://doi.org/10.5194/amt-12-2067-2019, 2019
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This paper presents the retrieval algorithm for the operational OMBRO data product and shows comparisons with correlative measurements and retrieval results. We highlight the physics of the retrieval. We compare the OMBRO products with other satellite and in situ measurements of BrO and illustrate the quality of the product on a global scale. We study OMBRO enhancements in volcanic plumes and over salt lakes. We also discuss the shortcomings and future updates of the OMBRO product.
Antje Inness, Melanie Ades, Anna Agustí-Panareda, Jérôme Barré, Anna Benedictow, Anne-Marlene Blechschmidt, Juan Jose Dominguez, Richard Engelen, Henk Eskes, Johannes Flemming, Vincent Huijnen, Luke Jones, Zak Kipling, Sebastien Massart, Mark Parrington, Vincent-Henri Peuch, Miha Razinger, Samuel Remy, Michael Schulz, and Martin Suttie
Atmos. Chem. Phys., 19, 3515–3556, https://doi.org/10.5194/acp-19-3515-2019, https://doi.org/10.5194/acp-19-3515-2019, 2019
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This paper describes a new global dataset of atmospheric composition data for the years 2003-2016 that has been produced by the Copernicus Atmosphere Monitoring Service (CAMS). It is called the CAMS reanalysis and provides information on aerosols and reactive gases. The CAMS reanalysis shows an improved performance compared to our previous atmospheric composition reanalyses; has smaller biases compared to independent O3, CO, NO2 and aerosol observations; and is more consistent in time.
Soheila Jafariserajehlou, Linlu Mei, Marco Vountas, Vladimir Rozanov, John P. Burrows, and Rainer Hollmann
Atmos. Meas. Tech., 12, 1059–1076, https://doi.org/10.5194/amt-12-1059-2019, https://doi.org/10.5194/amt-12-1059-2019, 2019
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We developed a new algorithm for cloud identification over the Arctic. This algorithm called ASCIA, utilizes time-series measurements of Advanced Along-Track Scanning Radiometer (AATSR) on Envisat and Sea and Land Surface Temperature Radiometer (SLSTR) on Sentinel-3A and -3B.
The data product of ASCIA is compared with three satellite products: ASCIA shows an improved performance compared to them. We validated ASCIA by ground-based measurements and a promising agreement is achieved.
Song Liu, Pieter Valks, Gaia Pinardi, Isabelle De Smedt, Huan Yu, Steffen Beirle, and Andreas Richter
Atmos. Meas. Tech., 12, 1029–1057, https://doi.org/10.5194/amt-12-1029-2019, https://doi.org/10.5194/amt-12-1029-2019, 2019
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Nitrogen dioxide (NO2) plays significant roles in both stratospheric and tropospheric chemistry, and the observations from satellites enable reliable monitoring of NO2 columns on a global scale and on long time scales. This work presents a refined algorithm for the retrieval of NO2 columns from the satellite instrument Global Ozone Monitoring Experiment-2 (GOME-2), which shows a clear improvement comparing to the previous algorithm.
Stefan Bender, Miriam Sinnhuber, Patrick J. Espy, and John P. Burrows
Atmos. Chem. Phys., 19, 2135–2147, https://doi.org/10.5194/acp-19-2135-2019, https://doi.org/10.5194/acp-19-2135-2019, 2019
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We present an empirical model for nitric oxide (NO) in the mesosphere (60–90 km) derived from SCIAMACHY limb scan data. Our model relates the daily (longitudinally) averaged NO number densities from SCIAMACHY as a function of geomagnetic latitude to the solar Lyman-alpha and the geomagnetic AE indices. We use a non-linear regression model, incorporating a finite and seasonally varying lifetime for the geomagnetically induced NO.
Christopher Perro, Thomas J. Duck, Glen Lesins, Kimberly Strong, Penny M. Rowe, James R. Drummond, and Robert J. Sica
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2018-381, https://doi.org/10.5194/amt-2018-381, 2019
Publication in AMT not foreseen
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A satellite retrieval for water vapour column was adapted for use over different surfaces in the wintertime Arctic. The retrieval was validated at multiple locations where there was excellent agreement. Reanalyses were found to be 10–15 % drier compared to our water vapour retrieval. Reanalyses represent the present day understanding of the atmosphere so this discrepancy between reanalyses and our retrieval could have implications for the current understanding of the climate.
Evgenia Galytska, Alexey Rozanov, Martyn P. Chipperfield, Sandip. S. Dhomse, Mark Weber, Carlo Arosio, Wuhu Feng, and John P. Burrows
Atmos. Chem. Phys., 19, 767–783, https://doi.org/10.5194/acp-19-767-2019, https://doi.org/10.5194/acp-19-767-2019, 2019
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In this study we analysed ozone changes in the tropical mid-stratosphere as observed by the SCIAMACHY instrument during 2004–2012. We used simulations from TOMCAT model with different chemical and dynamical forcings to reveal primary causes of ozone changes. We also considered measured NO2 and modelled NOx, NOx, and N2O data. With modelled AoA data we identified seasonal changes in the upwelling speed and explained how those changes affect N2O chemistry which leads to observed ozone changes.
Frederik Tack, Alexis Merlaud, Andreas C. Meier, Tim Vlemmix, Thomas Ruhtz, Marian-Daniel Iordache, Xinrui Ge, Len van der Wal, Dirk Schuettemeyer, Magdalena Ardelean, Andreea Calcan, Daniel Constantin, Anja Schönhardt, Koen Meuleman, Andreas Richter, and Michel Van Roozendael
Atmos. Meas. Tech., 12, 211–236, https://doi.org/10.5194/amt-12-211-2019, https://doi.org/10.5194/amt-12-211-2019, 2019
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We present an intercomparison study of four airborne imaging DOAS instruments, dedicated to the retrieval and high-resolution mapping of tropospheric nitrogen dioxide (NO2) vertical column densities (VCDs). The AROMAPEX campaign took place in Berlin, Germany, in April 2016 with the primary objectives (1) to test and intercompare the performance of experimental airborne imagers and (2) to prepare the validation and calibration campaigns for the Sentinel-5 Precursor/TROPOMI mission.
Joseph Mendonca, Kimberly Strong, Debra Wunch, Geoffrey C. Toon, David A. Long, Joseph T. Hodges, Vincent T. Sironneau, and Jonathan E. Franklin
Atmos. Meas. Tech., 12, 35–50, https://doi.org/10.5194/amt-12-35-2019, https://doi.org/10.5194/amt-12-35-2019, 2019
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In order to study the carbon cycle, accurate remote sensing measurements of XCO2 are required. This means that accurate absorption coefficients of CO2 and O2 in the retrieval algorithm are required. We use high-resolution laboratory spectra of O2 to derive accurate absorption coefficients. By applying the O2 absorption coefficients to the retrieval of XCO2 from ground-based solar absorption spectra we show that the error on retrieved XCO2 is decreased.
Tim Bösch, Vladimir Rozanov, Andreas Richter, Enno Peters, Alexei Rozanov, Folkard Wittrock, Alexis Merlaud, Johannes Lampel, Stefan Schmitt, Marijn de Haij, Stijn Berkhout, Bas Henzing, Arnoud Apituley, Mirjam den Hoed, Jan Vonk, Martin Tiefengraber, Moritz Müller, and John Philip Burrows
Atmos. Meas. Tech., 11, 6833–6859, https://doi.org/10.5194/amt-11-6833-2018, https://doi.org/10.5194/amt-11-6833-2018, 2018
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A new MAX-DOAS profiling algorithm for aerosols and trace
gases was developed.
The performance of this novel algorithm was tested with the help of
synthetic data and measurements from the CINDI-2 campaign in Cabauw, the
Netherlands, in 2016.
Ting Wang, Pucai Wang, Nicolas Theys, Dan Tong, François Hendrick, Qiang Zhang, and Michel Van Roozendael
Atmos. Chem. Phys., 18, 18063–18078, https://doi.org/10.5194/acp-18-18063-2018, https://doi.org/10.5194/acp-18-18063-2018, 2018
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In the last decade, four temporal regimes of SO2 in China have been identified. After an initial rise, SO2 undergoes two sharp drops in 2007–2008 and 2014–2016, during which 5-year rebounding is sustained. Different mechanisms are tied to North and South China. The industrial emission is responsible for SO2 variation in North China, while in South China the meteorological conditions make a large contribution. The result is crucial to the understanding of SO2 changes and future polices.
K. Folkert Boersma, Henk J. Eskes, Andreas Richter, Isabelle De Smedt, Alba Lorente, Steffen Beirle, Jos H. G. M. van Geffen, Marina Zara, Enno Peters, Michel Van Roozendael, Thomas Wagner, Joannes D. Maasakkers, Ronald J. van der A, Joanne Nightingale, Anne De Rudder, Hitoshi Irie, Gaia Pinardi, Jean-Christopher Lambert, and Steven C. Compernolle
Atmos. Meas. Tech., 11, 6651–6678, https://doi.org/10.5194/amt-11-6651-2018, https://doi.org/10.5194/amt-11-6651-2018, 2018
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This paper describes a new, improved data record of 22+ years of coherent nitrogen dioxide (NO2) pollution measurements from different satellite instruments. Our work helps to ensure that climate data are of sufficient quality to draw reliable conclusions and shape decisions. It shows how dedicated intercomparisons of retrieval sub-steps have led to improved NO2 measurements from the GOME, SCIAMACHY, GOME-2(A), and OMI sensors, and how quality assurance of the new data product is achieved.
Christopher W. O'Dell, Annmarie Eldering, Paul O. Wennberg, David Crisp, Michael R. Gunson, Brendan Fisher, Christian Frankenberg, Matthäus Kiel, Hannakaisa Lindqvist, Lukas Mandrake, Aronne Merrelli, Vijay Natraj, Robert R. Nelson, Gregory B. Osterman, Vivienne H. Payne, Thomas E. Taylor, Debra Wunch, Brian J. Drouin, Fabiano Oyafuso, Albert Chang, James McDuffie, Michael Smyth, David F. Baker, Sourish Basu, Frédéric Chevallier, Sean M. R. Crowell, Liang Feng, Paul I. Palmer, Mavendra Dubey, Omaira E. García, David W. T. Griffith, Frank Hase, Laura T. Iraci, Rigel Kivi, Isamu Morino, Justus Notholt, Hirofumi Ohyama, Christof Petri, Coleen M. Roehl, Mahesh K. Sha, Kimberly Strong, Ralf Sussmann, Yao Te, Osamu Uchino, and Voltaire A. Velazco
Atmos. Meas. Tech., 11, 6539–6576, https://doi.org/10.5194/amt-11-6539-2018, https://doi.org/10.5194/amt-11-6539-2018, 2018
Michael Buchwitz, Maximilian Reuter, Oliver Schneising, Stefan Noël, Bettina Gier, Heinrich Bovensmann, John P. Burrows, Hartmut Boesch, Jasdeep Anand, Robert J. Parker, Peter Somkuti, Rob G. Detmers, Otto P. Hasekamp, Ilse Aben, André Butz, Akihiko Kuze, Hiroshi Suto, Yukio Yoshida, David Crisp, and Christopher O'Dell
Atmos. Chem. Phys., 18, 17355–17370, https://doi.org/10.5194/acp-18-17355-2018, https://doi.org/10.5194/acp-18-17355-2018, 2018
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We present a new satellite data set of column-averaged mixing ratios of carbon dioxide (CO2), which covers the time period 2003 to 2016. We used this data set to compute annual mean atmospheric CO2 growth rates. We show that the growth rate is highest during 2015 and 2016 despite nearly constant CO2 emissions from fossil fuel burning in recent years. The high growth rates are attributed to year 2015-2016 El Nino episodes. We present correlations with fossil fuel emissions and ENSO indices.
Corinne Vigouroux, Carlos Augusto Bauer Aquino, Maite Bauwens, Cornelis Becker, Thomas Blumenstock, Martine De Mazière, Omaira García, Michel Grutter, César Guarin, James Hannigan, Frank Hase, Nicholas Jones, Rigel Kivi, Dmitry Koshelev, Bavo Langerock, Erik Lutsch, Maria Makarova, Jean-Marc Metzger, Jean-François Müller, Justus Notholt, Ivan Ortega, Mathias Palm, Clare Paton-Walsh, Anatoly Poberovskii, Markus Rettinger, John Robinson, Dan Smale, Trissevgeni Stavrakou, Wolfgang Stremme, Kim Strong, Ralf Sussmann, Yao Té, and Geoffrey Toon
Atmos. Meas. Tech., 11, 5049–5073, https://doi.org/10.5194/amt-11-5049-2018, https://doi.org/10.5194/amt-11-5049-2018, 2018
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A few ground-based stations have provided time series of HCHO columns until now, which was not optimal for providing good diagnostics for satellite or model validation. In this work, HCHO time series have been determined in a harmonized way at 21 stations ensuring, in addition to a better spatial and level of abundances coverage, that internal biases within the network have been minimized. This data set shows consistent good agreement with model data and is ready for future satellite validation.
Alba Lorente, K. Folkert Boersma, Piet Stammes, L. Gijsbert Tilstra, Andreas Richter, Huan Yu, Said Kharbouche, and Jan-Peter Muller
Atmos. Meas. Tech., 11, 4509–4529, https://doi.org/10.5194/amt-11-4509-2018, https://doi.org/10.5194/amt-11-4509-2018, 2018
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Light reflected by Earth’s surface is different in each direction: it appears brighter or darker in certain viewing directions. Currently this effect is not accounted for in satellite retrievals; thus surface reflectance climatologies and cloud fractions show an east-west bias across orbits (GOME2,OMI). The effect for NO2 measurements in partly cloudy scenes is substantial. We recommend that this effect in UV/Vis sensors coherently accounted for, and will be especially beneficial for TROPOMI.
Farahnaz Khosrawi, Stefan Lossow, Gabriele P. Stiller, Karen H. Rosenlof, Joachim Urban, John P. Burrows, Robert P. Damadeo, Patrick Eriksson, Maya García-Comas, John C. Gille, Yasuko Kasai, Michael Kiefer, Gerald E. Nedoluha, Stefan Noël, Piera Raspollini, William G. Read, Alexei Rozanov, Christopher E. Sioris, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 11, 4435–4463, https://doi.org/10.5194/amt-11-4435-2018, https://doi.org/10.5194/amt-11-4435-2018, 2018
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Time series of stratospheric and lower mesospheric water vapour using 33 data sets from 15 satellite instruments were compared in the framework of the second SPARC water vapour assessment. We find that most data sets can be considered in observational and modelling studies addressing, e.g. stratospheric and lower mesospheric water vapour variability and trends if data-set-specific characteristics (e.g. a drift) and restrictions (e.g. temporal and spatial coverage) are taken into account.
Marina Zara, K. Folkert Boersma, Isabelle De Smedt, Andreas Richter, Enno Peters, Jos H. G. M. van Geffen, Steffen Beirle, Thomas Wagner, Michel Van Roozendael, Sergey Marchenko, Lok N. Lamsal, and Henk J. Eskes
Atmos. Meas. Tech., 11, 4033–4058, https://doi.org/10.5194/amt-11-4033-2018, https://doi.org/10.5194/amt-11-4033-2018, 2018
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Nitrogen dioxide and formaldehyde satellite data are used for air quality and climate studies. We quantify and characterise slant column uncertainties from different research groups. Our evaluation is motivated by recently improved techniques and by a desire to provide fully traceable uncertainty budget for climate records generated within the QA4ECV project. The improved slant columns are in agreement but with substantial differences in the reported uncertainties between groups and instruments.
Landon A. Rieger, Elizaveta P. Malinina, Alexei V. Rozanov, John P. Burrows, Adam E. Bourassa, and Doug A. Degenstein
Atmos. Meas. Tech., 11, 3433–3445, https://doi.org/10.5194/amt-11-3433-2018, https://doi.org/10.5194/amt-11-3433-2018, 2018
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This paper compares aerosol extinction records from two limb scattering instruments, OSIRIS and SCIAMACHY, to that from the occultation instrument SAGE II. Differences are investigated through modelling and retrieval studies and important sources of systematic errors are quantified. It is found that the largest biases come from uncertainties in the aerosol size distribution and the aerosol particle concentration at altitudes above 30 km.
Steffen Tietsche, Magdalena Alonso-Balmaseda, Patricia Rosnay, Hao Zuo, Xiangshan Tian-Kunze, and Lars Kaleschke
The Cryosphere, 12, 2051–2072, https://doi.org/10.5194/tc-12-2051-2018, https://doi.org/10.5194/tc-12-2051-2018, 2018
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We compare Arctic sea-ice thickness from L-band microwave satellite observations and an ocean–sea ice reanalysis. There is good agreement for some regions and times but systematic discrepancy in others. Errors in both the reanalysis and observational products contribute to these discrepancies. Thus, we recommend proceeding with caution when using these observations for model validation or data assimilation. At the same time we emphasise their unique value for improving sea-ice forecast models.
Lisa K. Behrens, Andreas Hilboll, Andreas Richter, Enno Peters, Henk Eskes, and John P. Burrows
Atmos. Meas. Tech., 11, 2769–2795, https://doi.org/10.5194/amt-11-2769-2018, https://doi.org/10.5194/amt-11-2769-2018, 2018
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We developed a novel NO2 DOAS retrieval for the GOME-2A instrument in the UV spectral range, which is compared with a NO2 retrieval in the visible and model values. Regions representative for both anthropogenic and biomass burning NO2 pollution are investigated. Anthropogenic air pollution is mostly located in the boundary layer close to the surface. In contrast, biomass burning NO2 is often uplifted into elevated layers.
Isabelle De Smedt, Nicolas Theys, Huan Yu, Thomas Danckaert, Christophe Lerot, Steven Compernolle, Michel Van Roozendael, Andreas Richter, Andreas Hilboll, Enno Peters, Mattia Pedergnana, Diego Loyola, Steffen Beirle, Thomas Wagner, Henk Eskes, Jos van Geffen, Klaas Folkert Boersma, and Pepijn Veefkind
Atmos. Meas. Tech., 11, 2395–2426, https://doi.org/10.5194/amt-11-2395-2018, https://doi.org/10.5194/amt-11-2395-2018, 2018
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This paper introduces the formaldehyde (HCHO) tropospheric vertical column retrieval algorithm implemented in the TROPOMI/Sentinel-5 Precursor operational processor, and comprehensively describes its various retrieval steps. Furthermore, algorithmic improvements developed in the framework of the EU FP7-project QA4ECV are described for future updates of the processor. Detailed error estimates are discussed in the light of Copernicus user requirements and needs for validation are highlighted.
Carlo Arosio, Alexei Rozanov, Elizaveta Malinina, Kai-Uwe Eichmann, Thomas von Clarmann, and John P. Burrows
Atmos. Meas. Tech., 11, 2135–2149, https://doi.org/10.5194/amt-11-2135-2018, https://doi.org/10.5194/amt-11-2135-2018, 2018
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This paper describes the development of a retrieval algorithm at the University of Bremen which derives stratospheric ozone profiles from limb observations performed by the OMPS satellite instrument. Here we present the implementation of the algorithm and the validation of our results (1 year of data against independent satellite and ground-based measurements). Good agreement is generally found between 20 and 55 km, mostly within 10 % at all latitudes.
Evgenia Galytska, Vassyl Danylevsky, René Hommel, and John P. Burrows
Atmos. Meas. Tech., 11, 2101–2118, https://doi.org/10.5194/amt-11-2101-2018, https://doi.org/10.5194/amt-11-2101-2018, 2018
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This research assesses the influence of biomass burning during forest fires throughout summer 2010 on aerosol load over Ukraine, the European territory of Russia (ETR) and Eastern Europe. We apply and compare ground-based and satellite measurements to determine aerosol content, dynamics, and properties. With the application of modeling techniques (HYSPLIT), we show that the maximum AOD in August 2010 over Ukraine was caused by particle transport from the forest fires in the ETR.
Elizaveta Malinina, Alexei Rozanov, Vladimir Rozanov, Patricia Liebing, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 11, 2085–2100, https://doi.org/10.5194/amt-11-2085-2018, https://doi.org/10.5194/amt-11-2085-2018, 2018
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Stratospheric aerosols play an important role in climate change. This paper presents the retrieval algorithm of two aerosol particle size distribution parameters in the stratosphere from remote sensing instruments. A unique data set was created by implementing this algorithm on SCIAMACHY limb measurements. The general behaviour of the aerosol particle size parameters was revealed. Comparison of the retrieved parameters with another instrument showed good agreement.
Stefan Noël, Katja Weigel, Klaus Bramstedt, Alexei Rozanov, Mark Weber, Heinrich Bovensmann, and John P. Burrows
Atmos. Chem. Phys., 18, 4463–4476, https://doi.org/10.5194/acp-18-4463-2018, https://doi.org/10.5194/acp-18-4463-2018, 2018
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The combined analysis of stratospheric methane and water vapour data derived from SCIAMACHY solar occultation measurements shows the expected anti-correlation and a clear temporal variation related to waves in equatorial zonal winds. Above about 20 km most of the additional water vapour is attributed to the oxidation of methane. The SCIAMACHY data confirm that at lower altitudes water vapour and methane are transported from the tropics to higher latitudes.
Maria Elissavet Koukouli, Nicolas Theys, Jieying Ding, Irene Zyrichidou, Bas Mijling, Dimitrios Balis, and Ronald Johannes van der A
Atmos. Meas. Tech., 11, 1817–1832, https://doi.org/10.5194/amt-11-1817-2018, https://doi.org/10.5194/amt-11-1817-2018, 2018
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Within the framework of the EU FP7 project MarcoPolo (Monitoring and Assessment of Regional air quality in China using space Observations), a new SO2 emission inventory over China was calculated using the CHIMERE CTM simulations, 10 years of OMI/Aura total SO2 columns and the bottom-up Multi-resolution Emission Inventory for China (MEIC v1.2).
Friedrich Richter, Matthias Drusch, Lars Kaleschke, Nina Maaß, Xiangshan Tian-Kunze, and Susanne Mecklenburg
The Cryosphere, 12, 921–933, https://doi.org/10.5194/tc-12-921-2018, https://doi.org/10.5194/tc-12-921-2018, 2018
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L-band (1.4 GHz) brightness temperatures from ESA's Soil Moisture and Ocean Salinity SMOS mission have been used to derive thin sea ice thickness. However, the brightness temperature measurements can potentially be assimilated directly in forecasting systems reducing the data latency and providing a more consistent first guess. We studied the forward (observation) operator that translates geophysical sea ice parameters from the ECMWF Ocean ReAnalysis Pilot 5 (ORAP5) into brightness temperatures.
Linlu Mei, Vladimir Rozanov, Marco Vountas, John P. Burrows, and Andreas Richter
Atmos. Chem. Phys., 18, 2511–2523, https://doi.org/10.5194/acp-18-2511-2018, https://doi.org/10.5194/acp-18-2511-2018, 2018
Mark Weber, Melanie Coldewey-Egbers, Vitali E. Fioletov, Stacey M. Frith, Jeannette D. Wild, John P. Burrows, Craig S. Long, and Diego Loyola
Atmos. Chem. Phys., 18, 2097–2117, https://doi.org/10.5194/acp-18-2097-2018, https://doi.org/10.5194/acp-18-2097-2018, 2018
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This paper commemorates the 30-year anniversary of the initial signing of the Montreal Protocol (MP) on substances that deplete the ozone layer. The MP is so far successful in reducing ozone-depleting substances, and total ozone decline was successfully stopped by the late 1990s. Total ozone levels have been mostly stable since then. In some regions, barely significant upward trends are observed that suggest an emergence into the expected ozone recovery phase.
Thomas Krings, Bruno Neininger, Konstantin Gerilowski, Sven Krautwurst, Michael Buchwitz, John P. Burrows, Carsten Lindemann, Thomas Ruhtz, Dirk Schüttemeyer, and Heinrich Bovensmann
Atmos. Meas. Tech., 11, 721–739, https://doi.org/10.5194/amt-11-721-2018, https://doi.org/10.5194/amt-11-721-2018, 2018
Amirmahdi Zarboo, Stefan Bender, John P. Burrows, Johannes Orphal, and Miriam Sinnhuber
Atmos. Meas. Tech., 11, 473–487, https://doi.org/10.5194/amt-11-473-2018, https://doi.org/10.5194/amt-11-473-2018, 2018
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We present the retrieved volume emission rates (VERs) from the airglow of both the daytime and twilight O2(1Σ) band and O2(1Δ) band emissions in the mesosphere and lower thermosphere (MLT). We have investigated the daily mean latitudinal distributions and the time series of the retrieved VER in the altitude range from 53 to 149 km. These observations provide information about the chemistry and dynamics and can be used to infer ozone, solar heating rates, and temperature in the MLT.
Patricia Liebing, Matthijs Krijger, Ralph Snel, Klaus Bramstedt, Stefan Noël, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 11, 265–289, https://doi.org/10.5194/amt-11-265-2018, https://doi.org/10.5194/amt-11-265-2018, 2018
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This article describes a method to determine the polarization sensitivity of SCIAMACHY, a spectrometer on Envisat, from in-orbit data. Polarization is a preference of a direction in which light oscillates, and many optical instruments suffer from a dependence of their measured signals on this. To measure and correct for this effect, a statistical analysis of in-flight data combined with a model of the atmosphere and the instrument was performed, showing that the instrument changed after launch.
Elizabeth C. Weatherhead, Jerald Harder, Eduardo A. Araujo-Pradere, Greg Bodeker, Jason M. English, Lawrence E. Flynn, Stacey M. Frith, Jeffrey K. Lazo, Peter Pilewskie, Mark Weber, and Thomas N. Woods
Atmos. Chem. Phys., 17, 15069–15093, https://doi.org/10.5194/acp-17-15069-2017, https://doi.org/10.5194/acp-17-15069-2017, 2017
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Satellite overlap is often carried out as a check on the stability of the data collected. We looked at how length of overlap influences how much information can be derived from the overlap period. Several results surprised us: the confidence we could have in the matchup of two records was independent of the offset, and understanding of the relative drift between the two satellite data sets improved significantly with 2–3 years of overlap. Sudden jumps could easily be confused with drift.
Xiaoyi Zhao, Dan Weaver, Kristof Bognar, Gloria Manney, Luis Millán, Xin Yang, Edwin Eloranta, Matthias Schneider, and Kimberly Strong
Atmos. Chem. Phys., 17, 14955–14974, https://doi.org/10.5194/acp-17-14955-2017, https://doi.org/10.5194/acp-17-14955-2017, 2017
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Few scientific questions about surface ozone depletion have been addressed, using a variety of measurements and atmospheric models. The lifetime of reactive bromine is only a few hours in the absence of recycling. Evidence of this recycling over aerosol or blowing-snow/ice particles was found at Eureka. The blowing snow sublimation process is a key step in producing bromine-enriched sea-salt aerosol. Ground-based FTIR isotopologue measurements at Eureka provided evidence of this key step.
Viktoria F. Sofieva, Erkki Kyrölä, Marko Laine, Johanna Tamminen, Doug Degenstein, Adam Bourassa, Chris Roth, Daniel Zawada, Mark Weber, Alexei Rozanov, Nabiz Rahpoe, Gabriele Stiller, Alexandra Laeng, Thomas von Clarmann, Kaley A. Walker, Patrick Sheese, Daan Hubert, Michel van Roozendael, Claus Zehner, Robert Damadeo, Joseph Zawodny, Natalya Kramarova, and Pawan K. Bhartia
Atmos. Chem. Phys., 17, 12533–12552, https://doi.org/10.5194/acp-17-12533-2017, https://doi.org/10.5194/acp-17-12533-2017, 2017
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We present a merged dataset of ozone profiles from several satellite instruments: SAGE II, GOMOS, SCIAMACHY, MIPAS, OSIRIS, ACE-FTS and OMPS. For merging, we used the latest versions of the original ozone datasets.
The merged SAGE–CCI–OMPS dataset is used for evaluating ozone trends in the stratosphere through multiple linear regression. Negative ozone trends in the upper stratosphere are observed before 1997 and positive trends are found after 1997.
Yang Wang, Steffen Beirle, Francois Hendrick, Andreas Hilboll, Junli Jin, Aleksandra A. Kyuberis, Johannes Lampel, Ang Li, Yuhan Luo, Lorenzo Lodi, Jianzhong Ma, Monica Navarro, Ivan Ortega, Enno Peters, Oleg L. Polyansky, Julia Remmers, Andreas Richter, Olga Puentedura, Michel Van Roozendael, André Seyler, Jonathan Tennyson, Rainer Volkamer, Pinhua Xie, Nikolai F. Zobov, and Thomas Wagner
Atmos. Meas. Tech., 10, 3719–3742, https://doi.org/10.5194/amt-10-3719-2017, https://doi.org/10.5194/amt-10-3719-2017, 2017
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Slant column densities of nitrous acid (HONO) derived from different MAX-DOAS instruments and retrieval software are systematically compared for the first time during the Multi Axis DOAS – Comparison campaign for Aerosols and Trace gases (MAD-CAT) campaign held at MPIC in Mainz, Germany, from June to October 2013. Through the inter-comparisons and sensitivity studies we quantified the uncertainties in the DOAS fits of HONO from different sources and concluded a recommended setting.
Kevin S. Olsen, Kimberly Strong, Kaley A. Walker, Chris D. Boone, Piera Raspollini, Johannes Plieninger, Whitney Bader, Stephanie Conway, Michel Grutter, James W. Hannigan, Frank Hase, Nicholas Jones, Martine de Mazière, Justus Notholt, Matthias Schneider, Dan Smale, Ralf Sussmann, and Naoko Saitoh
Atmos. Meas. Tech., 10, 3697–3718, https://doi.org/10.5194/amt-10-3697-2017, https://doi.org/10.5194/amt-10-3697-2017, 2017
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The primary instrument on the Greenhouse gases Observing SATellite (GOSAT) is the Thermal And Near infrared Sensor for carbon Observations (TANSO) Fourier transform spectrometer (FTS). TANSO-FTS has a thermal infrared channel to retrieve vertical profiles of CO2 and CH4 volume mixing ratios in the troposphere. We compare the retrieved vertical profiles of CH4 from TANSO-FTS with those from two other spaceborne FTSs and with ground-based FTS observatories to assess their quality.
Sven Krautwurst, Konstantin Gerilowski, Haflidi H. Jonsson, David R. Thompson, Richard W. Kolyer, Laura T. Iraci, Andrew K. Thorpe, Markus Horstjann, Michael Eastwood, Ira Leifer, Samuel A. Vigil, Thomas Krings, Jakob Borchardt, Michael Buchwitz, Matthew M. Fladeland, John P. Burrows, and Heinrich Bovensmann
Atmos. Meas. Tech., 10, 3429–3452, https://doi.org/10.5194/amt-10-3429-2017, https://doi.org/10.5194/amt-10-3429-2017, 2017
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This study investigates a subset of data collected during the CO2 and Methane EXperiment (COMEX) in 2014. It focuses on airborne measurements to quantify the emissions from landfills in the Los Angeles Basin. Airborne remote sensing data have been used to estimate the emission rate of one particular landfill on four different days. The results have been compared to airborne in situ measurements. Airborne imaging spectroscopy has been used to identify emission hotspots across the landfill.
André Seyler, Folkard Wittrock, Lisa Kattner, Barbara Mathieu-Üffing, Enno Peters, Andreas Richter, Stefan Schmolke, and John P. Burrows
Atmos. Chem. Phys., 17, 10997–11023, https://doi.org/10.5194/acp-17-10997-2017, https://doi.org/10.5194/acp-17-10997-2017, 2017
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Shipping accounts for a significant part of the emissions from the transportation sector. We have analyzed 3 years of MAX-DOAS measurements of NO2 and SO2 from a small island in the German Bight, showing that despite the vicinity to the shipping lane, the contribution of shipping sources to air pollution is only about 40 %. The implementation of stricter fuel sulfur limits led to a significant reduction in SO2-to-NO2 ratios in shipping emissions and ambient SO2 levels at the German coast.
Wolfgang Steinbrecht, Lucien Froidevaux, Ryan Fuller, Ray Wang, John Anderson, Chris Roth, Adam Bourassa, Doug Degenstein, Robert Damadeo, Joe Zawodny, Stacey Frith, Richard McPeters, Pawan Bhartia, Jeannette Wild, Craig Long, Sean Davis, Karen Rosenlof, Viktoria Sofieva, Kaley Walker, Nabiz Rahpoe, Alexei Rozanov, Mark Weber, Alexandra Laeng, Thomas von Clarmann, Gabriele Stiller, Natalya Kramarova, Sophie Godin-Beekmann, Thierry Leblanc, Richard Querel, Daan Swart, Ian Boyd, Klemens Hocke, Niklaus Kämpfer, Eliane Maillard Barras, Lorena Moreira, Gerald Nedoluha, Corinne Vigouroux, Thomas Blumenstock, Matthias Schneider, Omaira García, Nicholas Jones, Emmanuel Mahieu, Dan Smale, Michael Kotkamp, John Robinson, Irina Petropavlovskikh, Neil Harris, Birgit Hassler, Daan Hubert, and Fiona Tummon
Atmos. Chem. Phys., 17, 10675–10690, https://doi.org/10.5194/acp-17-10675-2017, https://doi.org/10.5194/acp-17-10675-2017, 2017
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Thanks to the 1987 Montreal Protocol and its amendments, ozone-depleting chlorine (and bromine) in the stratosphere has declined slowly since the late 1990s. Improved and extended long-term ozone profile observations from satellites and ground-based stations confirm that ozone is responding as expected and has increased by about 2 % per decade since 2000 in the upper stratosphere, around 40 km altitude. At lower altitudes, however, ozone has not changed significantly since 2000.
Debora Griffin, Kaley A. Walker, Stephanie Conway, Felicia Kolonjari, Kimberly Strong, Rebecca Batchelor, Chris D. Boone, Lin Dan, James R. Drummond, Pierre F. Fogal, Dejian Fu, Rodica Lindenmaier, Gloria L. Manney, and Dan Weaver
Atmos. Meas. Tech., 10, 3273–3294, https://doi.org/10.5194/amt-10-3273-2017, https://doi.org/10.5194/amt-10-3273-2017, 2017
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Measurements in the high Arctic from two ground-based and one space-borne infrared Fourier transform spectrometer agree well over an 8-year time period (2006–2013). These comparisons show no notable degradation, indicating the consistency of these data sets and suggesting that the space-borne measurements have been stable. Increasing ozone, as well as increases of some other atmospheric gases, has been found over this same time period.
Martin P. Langowski, Christian von Savigny, John P. Burrows, Didier Fussen, Erin C. M. Dawkins, Wuhu Feng, John M. C. Plane, and Daniel R. Marsh
Atmos. Meas. Tech., 10, 2989–3006, https://doi.org/10.5194/amt-10-2989-2017, https://doi.org/10.5194/amt-10-2989-2017, 2017
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Meteoric metals form metal layers in the upper atmosphere anandplay a role in the formation of middle-atmospheric clouds and aerosols. However, the total metal influx rate is not well known. Global Na datasets from measurements and a model are available, which had not been compared yet on a global scale until this paper. Overall the agreement is good, and many differences between measurements are also found in the model simulations. However, the modeled layer altitude is too low.
Dan Weaver, Kimberly Strong, Matthias Schneider, Penny M. Rowe, Chris Sioris, Kaley A. Walker, Zen Mariani, Taneil Uttal, C. Thomas McElroy, Holger Vömel, Alessio Spassiani, and James R. Drummond
Atmos. Meas. Tech., 10, 2851–2880, https://doi.org/10.5194/amt-10-2851-2017, https://doi.org/10.5194/amt-10-2851-2017, 2017
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We have compared techniques used by several PEARL instruments to measure atmospheric water vapour. No single instrument can comprehensively map the atmosphere. We documented how well these techniques perform and quantified the agreement and biases between them. This work showed that new FTIR datasets at PEARL capture accurate measurements of High Arctic water vapour.
Enrico Dammers, Mark W. Shephard, Mathias Palm, Karen Cady-Pereira, Shannon Capps, Erik Lutsch, Kim Strong, James W. Hannigan, Ivan Ortega, Geoffrey C. Toon, Wolfgang Stremme, Michel Grutter, Nicholas Jones, Dan Smale, Jacob Siemons, Kevin Hrpcek, Denis Tremblay, Martijn Schaap, Justus Notholt, and Jan Willem Erisman
Atmos. Meas. Tech., 10, 2645–2667, https://doi.org/10.5194/amt-10-2645-2017, https://doi.org/10.5194/amt-10-2645-2017, 2017
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Presented here is the validation of the CrIS fast physical retrieval (CFPR) NH3 column and profile measurements using ground-based Fourier transform infrared (FTIR) observations. The overall FTIR and CrIS total columns have a positive correlation of r = 0.77 (N = 218) with very little bias (a slope of 1.02). Furthermore, we find that CrIS and FTIR profile comparison differences are mostly within the range of the estimated retrieval uncertainties, with differences in the range of ~ 20 to 40 %.
Robert Ricker, Stefan Hendricks, Lars Kaleschke, Xiangshan Tian-Kunze, Jennifer King, and Christian Haas
The Cryosphere, 11, 1607–1623, https://doi.org/10.5194/tc-11-1607-2017, https://doi.org/10.5194/tc-11-1607-2017, 2017
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We developed the first merging of CryoSat-2 and SMOS sea-ice thickness retrievals. ESA’s Earth Explorer SMOS satellite can detect thin sea ice, whereas its companion CryoSat-2, designed to observe thicker perennial sea ice, lacks sensitivity. Using these satellite missions together completes the picture of the changing Arctic sea ice and provides a more accurate and comprehensive view on the actual state of Arctic sea-ice thickness.
Klaus Bramstedt, Thomas C. Stone, Manfred Gottwald, Stefan Noël, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 10, 2413–2423, https://doi.org/10.5194/amt-10-2413-2017, https://doi.org/10.5194/amt-10-2413-2017, 2017
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The satellite instrument SCIAMACHY on board the ESA's platform Envisat
(2002–2012) performed observations of the Earth's atmosphere. Using sun and moon observations of the instrument itself, we derived a set of correction
parameters for the determination of the viewing directions of the
instrument. From this work, all vertical profiles of atmospheric parameters
from SCIAMACHY's limb and occultation measurements will be improved by a more
accurate altitude information.
Debra Wunch, Paul O. Wennberg, Gregory Osterman, Brendan Fisher, Bret Naylor, Coleen M. Roehl, Christopher O'Dell, Lukas Mandrake, Camille Viatte, Matthäus Kiel, David W. T. Griffith, Nicholas M. Deutscher, Voltaire A. Velazco, Justus Notholt, Thorsten Warneke, Christof Petri, Martine De Maziere, Mahesh K. Sha, Ralf Sussmann, Markus Rettinger, David Pollard, John Robinson, Isamu Morino, Osamu Uchino, Frank Hase, Thomas Blumenstock, Dietrich G. Feist, Sabrina G. Arnold, Kimberly Strong, Joseph Mendonca, Rigel Kivi, Pauli Heikkinen, Laura Iraci, James Podolske, Patrick W. Hillyard, Shuji Kawakami, Manvendra K. Dubey, Harrison A. Parker, Eliezer Sepulveda, Omaira E. García, Yao Te, Pascal Jeseck, Michael R. Gunson, David Crisp, and Annmarie Eldering
Atmos. Meas. Tech., 10, 2209–2238, https://doi.org/10.5194/amt-10-2209-2017, https://doi.org/10.5194/amt-10-2209-2017, 2017
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This paper describes the comparisons between NASA's Orbiting Carbon Observatory (OCO-2) column-averaged dry-air mole fractions of CO2 with its primary ground-based validation network, the Total Carbon Column Observing Network (TCCON). The paper shows that while the standard bias correction reduces much of the spurious variability in the satellite measurements, residual biases remain.
Rebecca R. Buchholz, Merritt N. Deeter, Helen M. Worden, John Gille, David P. Edwards, James W. Hannigan, Nicholas B. Jones, Clare Paton-Walsh, David W. T. Griffith, Dan Smale, John Robinson, Kimberly Strong, Stephanie Conway, Ralf Sussmann, Frank Hase, Thomas Blumenstock, Emmanuel Mahieu, and Bavo Langerock
Atmos. Meas. Tech., 10, 1927–1956, https://doi.org/10.5194/amt-10-1927-2017, https://doi.org/10.5194/amt-10-1927-2017, 2017
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The study presents the first systematic use of ground-based remote-sensing data from the Network for the Detection of Atmospheric Composition Change (NDACC) to validate satellite-based Measurements of Pollution in the Troposphere (MOPITT) total column carbon monoxide (CO). MOPITT generally shows low bias with respect to the ground-based instruments. The geographic and temporal dependence of validation results are determined. Our findings inform some recommendations for using MOPITT measurements.
Andreas Carlos Meier, Anja Schönhardt, Tim Bösch, Andreas Richter, André Seyler, Thomas Ruhtz, Daniel-Eduard Constantin, Reza Shaiganfar, Thomas Wagner, Alexis Merlaud, Michel Van Roozendael, Livio Belegante, Doina Nicolae, Lucian Georgescu, and John Philip Burrows
Atmos. Meas. Tech., 10, 1831–1857, https://doi.org/10.5194/amt-10-1831-2017, https://doi.org/10.5194/amt-10-1831-2017, 2017
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We present airborne remote sensing measurements of NO2 in the urban area of Bucharest. NO2 is a harmful pollutant, which is emitted in combustion processes. The measurements presented here enable the creation of maps, showing the horizontal NO2 distribution across the whole city within a relatively short time window of 1.5 h. These data provide new insight into urban pollution levels and their spatial distribution.
Michael Buchwitz, Oliver Schneising, Maximilian Reuter, Jens Heymann, Sven Krautwurst, Heinrich Bovensmann, John P. Burrows, Hartmut Boesch, Robert J. Parker, Peter Somkuti, Rob G. Detmers, Otto P. Hasekamp, Ilse Aben, André Butz, Christian Frankenberg, and Alexander J. Turner
Atmos. Chem. Phys., 17, 5751–5774, https://doi.org/10.5194/acp-17-5751-2017, https://doi.org/10.5194/acp-17-5751-2017, 2017
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Methane is an important greenhouse gas and increasing atmospheric concentrations result in global warming. We present a simple method to derive annual methane emission estimates of methane hotspot areas from satellite data. We present results for four source areas. We found that our estimates are in good agreement with other studies/data sets for the Four Corners region in the USA and for Azerbaijan but we also found higher emissions for parts of California and Turkmenistan.
Yang Wang, Steffen Beirle, Johannes Lampel, Mariliza Koukouli, Isabelle De Smedt, Nicolas Theys, Ang Li, Dexia Wu, Pinhua Xie, Cheng Liu, Michel Van Roozendael, Trissevgeni Stavrakou, Jean-François Müller, and Thomas Wagner
Atmos. Chem. Phys., 17, 5007–5033, https://doi.org/10.5194/acp-17-5007-2017, https://doi.org/10.5194/acp-17-5007-2017, 2017
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A long-term MAX-DOAS measurement from 2011 to 2014 was operated in Wuxi, part of the most industrialized area of the Yangtze River delta region of China. The tropospheric VCDs and vertical profiles of NO2, SO2 and HCHO derived from the MAX-DOAS are used to validate the products derived from OMI and GOME-2A/B by different scientific teams (daily- and bimonthly-averaged data). We investigate the effects of clouds, aerosols and a priori profile shapes on satellite retrievals of tropospheric VCDs.
Jia Jia, Annette Ladstätter-Weißenmayer, Xuewei Hou, Alexei Rozanov, and John P. Burrows
Atmos. Chem. Phys., 17, 4915–4930, https://doi.org/10.5194/acp-17-4915-2017, https://doi.org/10.5194/acp-17-4915-2017, 2017
Anja Schönhardt, Andreas Richter, Nicolas Theys, and John P. Burrows
Atmos. Chem. Phys., 17, 4857–4870, https://doi.org/10.5194/acp-17-4857-2017, https://doi.org/10.5194/acp-17-4857-2017, 2017
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Iodine monoxide, IO, is observed in satellite measurements following the eruption of the Kasatochi volcano, Alaska, in August 2008. Large IO columns are detected by SCIAMACHY on ENVISAT and by GOME-2 on MetOp-A for several days. IO amounts are approximately 1 order of magnitude smaller than those of BrO. Details in the spatial distributions differ between IO, BrO and sulfur dioxide, SO2. The total mass of IO in the volcanic plume is determined to be on the order of 10 Mg.
Liang Feng, Paul I. Palmer, Hartmut Bösch, Robert J. Parker, Alex J. Webb, Caio S. C. Correia, Nicholas M. Deutscher, Lucas G. Domingues, Dietrich G. Feist, Luciana V. Gatti, Emanuel Gloor, Frank Hase, Rigel Kivi, Yi Liu, John B. Miller, Isamu Morino, Ralf Sussmann, Kimberly Strong, Osamu Uchino, Jing Wang, and Andreas Zahn
Atmos. Chem. Phys., 17, 4781–4797, https://doi.org/10.5194/acp-17-4781-2017, https://doi.org/10.5194/acp-17-4781-2017, 2017
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We use the GEOS-Chem global 3-D model of atmospheric chemistry and transport and an ensemble Kalman filter to simultaneously infer regional fluxes of methane (CH4) and carbon dioxide (CO2) directly from GOSAT retrievals of XCH4:XCO2, using sparse ground-based CH4 and CO2 mole fraction data to anchor the ratio. Our results show that assimilation of GOSAT data significantly reduced the posterior uncertainty and changed the a priori spatial distribution of CH4 emissions.
Stefan Lossow, Farahnaz Khosrawi, Gerald E. Nedoluha, Faiza Azam, Klaus Bramstedt, John. P. Burrows, Bianca M. Dinelli, Patrick Eriksson, Patrick J. Espy, Maya García-Comas, John C. Gille, Michael Kiefer, Stefan Noël, Piera Raspollini, William G. Read, Karen H. Rosenlof, Alexei Rozanov, Christopher E. Sioris, Gabriele P. Stiller, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 10, 1111–1137, https://doi.org/10.5194/amt-10-1111-2017, https://doi.org/10.5194/amt-10-1111-2017, 2017
Enno Peters, Gaia Pinardi, André Seyler, Andreas Richter, Folkard Wittrock, Tim Bösch, Michel Van Roozendael, François Hendrick, Theano Drosoglou, Alkiviadis F. Bais, Yugo Kanaya, Xiaoyi Zhao, Kimberly Strong, Johannes Lampel, Rainer Volkamer, Theodore Koenig, Ivan Ortega, Olga Puentedura, Mónica Navarro-Comas, Laura Gómez, Margarita Yela González, Ankie Piters, Julia Remmers, Yang Wang, Thomas Wagner, Shanshan Wang, Alfonso Saiz-Lopez, David García-Nieto, Carlos A. Cuevas, Nuria Benavent, Richard Querel, Paul Johnston, Oleg Postylyakov, Alexander Borovski, Alexander Elokhov, Ilya Bruchkouski, Haoran Liu, Cheng Liu, Qianqian Hong, Claudia Rivera, Michel Grutter, Wolfgang Stremme, M. Fahim Khokhar, Junaid Khayyam, and John P. Burrows
Atmos. Meas. Tech., 10, 955–978, https://doi.org/10.5194/amt-10-955-2017, https://doi.org/10.5194/amt-10-955-2017, 2017
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This work is about harmonization of differential optical absorption spectroscopy retrieval codes, which is a remote sensing technique widely used to derive atmospheric trace gas amounts. The study is based on ground-based measurements performed during the Multi-Axis DOAS Comparison campaign for Aerosols and Trace gases (MAD-CAT) in Mainz, Germany, in summer 2013. In total, 17 international groups working in the field of the DOAS technique participated in this study.
Andreas Hilboll, Andreas Richter, and John P. Burrows
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-101, https://doi.org/10.5194/acp-2017-101, 2017
Revised manuscript has not been submitted
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We investigate the temporal evolution of the important tropospheric air pollutant nitrogen dioxide (NO2) since the early 2000s, and correlate NO2 abundances with indicators of economic development. Until 2012, NO2 pollution and economic growth are strongly correlated, with annual increases of up to 4.4 %. Since then, tropospheric NO2 pollution has stabilized or is even declining, probably as a result of a slow-down in Indian economic growth combined with the implementation of cleaner technology.
Alba Lorente, K. Folkert Boersma, Huan Yu, Steffen Dörner, Andreas Hilboll, Andreas Richter, Mengyao Liu, Lok N. Lamsal, Michael Barkley, Isabelle De Smedt, Michel Van Roozendael, Yang Wang, Thomas Wagner, Steffen Beirle, Jin-Tai Lin, Nickolay Krotkov, Piet Stammes, Ping Wang, Henk J. Eskes, and Maarten Krol
Atmos. Meas. Tech., 10, 759–782, https://doi.org/10.5194/amt-10-759-2017, https://doi.org/10.5194/amt-10-759-2017, 2017
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Choices and assumptions made to represent the state of the atmosphere introduce an uncertainty of 42 % in the air mass factor calculation in trace gas satellite retrievals in polluted regions. The AMF strongly depends on the choice of a priori trace gas profile, surface albedo data set and the correction method to account for clouds and aerosols. We call for well-designed validation exercises focusing on situations when AMF structural uncertainty has the highest impact on satellite retrievals.
Ruixiong Zhang, Yuhang Wang, Qiusheng He, Laiguo Chen, Yuzhong Zhang, Hang Qu, Charles Smeltzer, Jianfeng Li, Leonardo M. A. Alvarado, Mihalis Vrekoussis, Andreas Richter, Folkard Wittrock, and John P. Burrows
Atmos. Chem. Phys., 17, 3083–3095, https://doi.org/10.5194/acp-17-3083-2017, https://doi.org/10.5194/acp-17-3083-2017, 2017
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We use short-lived reactive aromatics as proxies to diagnose transport of pollutants to Tibet. In situ observations of short-lived reactive aromatics across the Tibetan Plateau are analyzed using a regional chemistry and transport model. Our results suggest that the cut-off low system is a major pathway for long-range transport of pollutants such as black carbon. The modeling analysis reveals that even the state-of-the-science reanalysis cannot simulate this cut-off system accurately.
Whitney Bader, Benoît Bovy, Stephanie Conway, Kimberly Strong, Dan Smale, Alexander J. Turner, Thomas Blumenstock, Chris Boone, Martine Collaud Coen, Ancelin Coulon, Omaira Garcia, David W. T. Griffith, Frank Hase, Petra Hausmann, Nicholas Jones, Paul Krummel, Isao Murata, Isamu Morino, Hideaki Nakajima, Simon O'Doherty, Clare Paton-Walsh, John Robinson, Rodrigue Sandrin, Matthias Schneider, Christian Servais, Ralf Sussmann, and Emmanuel Mahieu
Atmos. Chem. Phys., 17, 2255–2277, https://doi.org/10.5194/acp-17-2255-2017, https://doi.org/10.5194/acp-17-2255-2017, 2017
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An increase of 0.31 ± 0.03 % year−1 of atmospheric methane is reported using 10 years of solar observations performed at 10 ground-based stations since 2005. These trend agree with a GEOS-Chem-tagged simulation that accounts for the contribution of each emission source and one sink in the total methane. The GEOS-Chem simulation shows that anthropogenic emissions from coal mining and gas and oil transport and exploration have played a major role in the increase methane since 2005.
Ronald J. van der A, Bas Mijling, Jieying Ding, Maria Elissavet Koukouli, Fei Liu, Qing Li, Huiqin Mao, and Nicolas Theys
Atmos. Chem. Phys., 17, 1775–1789, https://doi.org/10.5194/acp-17-1775-2017, https://doi.org/10.5194/acp-17-1775-2017, 2017
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The SO2 concentrations and NOx emissions over China derived from satellite observations are compared with the national fossil fuel consumption and air quality regulations. It is shown that not only NO2 concentrations but also NOx emissions in all Chinese provinces decreased in the last 2 years. We conclude that without the air quality regulations the SO2 concentrations would be about 2.5 times higher and the NO2 concentrations would be at least 25 % higher than they are today in China.
Sabine Barthlott, Matthias Schneider, Frank Hase, Thomas Blumenstock, Matthäus Kiel, Darko Dubravica, Omaira E. García, Eliezer Sepúlveda, Gizaw Mengistu Tsidu, Samuel Takele Kenea, Michel Grutter, Eddy F. Plaza-Medina, Wolfgang Stremme, Kim Strong, Dan Weaver, Mathias Palm, Thorsten Warneke, Justus Notholt, Emmanuel Mahieu, Christian Servais, Nicholas Jones, David W. T. Griffith, Dan Smale, and John Robinson
Earth Syst. Sci. Data, 9, 15–29, https://doi.org/10.5194/essd-9-15-2017, https://doi.org/10.5194/essd-9-15-2017, 2017
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Tropospheric water vapour isotopologue distributions have been consistently generated and quality-filtered for 12 globally distributed ground-based FTIR sites. The products are provided as two data types. The first type is best-suited for tropospheric water vapour distribution studies. The second type is needed for analysing moisture pathways by means of {H2O,δD}-pair distributions. This paper describes the data types and gives recommendations for their correct usage.
Stefan Bender, Miriam Sinnhuber, Martin Langowski, and John P. Burrows
Atmos. Meas. Tech., 10, 209–220, https://doi.org/10.5194/amt-10-209-2017, https://doi.org/10.5194/amt-10-209-2017, 2017
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We present the retrieval of NO number densities from 60 km to 85 km from measurements of SCIAMACHY/Envisat in its nominal limb mode (0–91 km). We derive the densities from the NO gamma bands (230–300 nm). Using prior input reduces the incorrect attribution of NO from the lower thermosphere. The SCIAMACHY nominal limb scans provide almost 10 years of daily NO data in this altitude range, a unique data record to constrain NO in the mesosphere for testing and validating chemistry climate models.
Nicolas Theys, Isabelle De Smedt, Huan Yu, Thomas Danckaert, Jeroen van Gent, Christoph Hörmann, Thomas Wagner, Pascal Hedelt, Heiko Bauer, Fabian Romahn, Mattia Pedergnana, Diego Loyola, and Michel Van Roozendael
Atmos. Meas. Tech., 10, 119–153, https://doi.org/10.5194/amt-10-119-2017, https://doi.org/10.5194/amt-10-119-2017, 2017
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This paper provides a thorough description of the algorithm to retrieve SO2 columns from TROPOMI/Sentinel-5 Precursor measurements. The different algorithmic steps including error analysis are detailed. Scientific verification of the algorithm and validation needs are also discussed.
Dmitry A. Belikov, Shamil Maksyutov, Alexander Ganshin, Ruslan Zhuravlev, Nicholas M. Deutscher, Debra Wunch, Dietrich G. Feist, Isamu Morino, Robert J. Parker, Kimberly Strong, Yukio Yoshida, Andrey Bril, Sergey Oshchepkov, Hartmut Boesch, Manvendra K. Dubey, David Griffith, Will Hewson, Rigel Kivi, Joseph Mendonca, Justus Notholt, Matthias Schneider, Ralf Sussmann, Voltaire A. Velazco, and Shuji Aoki
Atmos. Chem. Phys., 17, 143–157, https://doi.org/10.5194/acp-17-143-2017, https://doi.org/10.5194/acp-17-143-2017, 2017
Patrick E. Sheese, Kaley A. Walker, Chris D. Boone, Chris A. McLinden, Peter F. Bernath, Adam E. Bourassa, John P. Burrows, Doug A. Degenstein, Bernd Funke, Didier Fussen, Gloria L. Manney, C. Thomas McElroy, Donal Murtagh, Cora E. Randall, Piera Raspollini, Alexei Rozanov, James M. Russell III, Makoto Suzuki, Masato Shiotani, Joachim Urban, Thomas von Clarmann, and Joseph M. Zawodny
Atmos. Meas. Tech., 9, 5781–5810, https://doi.org/10.5194/amt-9-5781-2016, https://doi.org/10.5194/amt-9-5781-2016, 2016
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This study validates version 3.5 of the ACE-FTS NOy species data sets by comparing diurnally scaled ACE-FTS data to correlative data from 11 other satellite limb sounders. For all five species examined (NO, NO2, HNO3, N2O5, and ClONO2), there is good agreement between ACE-FTS and the other data sets in various regions of the atmosphere. In these validated regions, these NOy data products can be used for further investigation into the composition, dynamics, and climate of the stratosphere.
Xiaoyi Zhao, Vitali Fioletov, Alexander Cede, Jonathan Davies, and Kimberly Strong
Atmos. Meas. Tech., 9, 5747–5761, https://doi.org/10.5194/amt-9-5747-2016, https://doi.org/10.5194/amt-9-5747-2016, 2016
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This study evaluates the performance of the recently developed Pandora spectrometer by comparing it with the Brewer reference triad. The instrument random uncertainty, total column ozone temperature dependence, and ozone air mass dependence have been determined using two Pandora and six Brewer instruments. In general, Pandora and Brewer instruments both have very low random uncertainty and air mass dependence. However, the Brewer has smaller ozone temperature dependence than Pandora.
Jiping Xie, François Counillon, Laurent Bertino, Xiangshan Tian-Kunze, and Lars Kaleschke
The Cryosphere, 10, 2745–2761, https://doi.org/10.5194/tc-10-2745-2016, https://doi.org/10.5194/tc-10-2745-2016, 2016
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As a potentially operational daily product, the SMOS-Ice can improve the statements of sea ice thickness and concentration. In this study, focusing on the SMOS-Ice data assimilated into the TOPAZ system, the quantitative evaluation for the impacts and the concerned comparison with the present observation system are valuable to understand the further improvement of the accuracy of operational ocean forecasting system.
Saroja M. Polavarapu, Michael Neish, Monique Tanguay, Claude Girard, Jean de Grandpré, Kirill Semeniuk, Sylvie Gravel, Shuzhan Ren, Sébastien Roche, Douglas Chan, and Kimberly Strong
Atmos. Chem. Phys., 16, 12005–12038, https://doi.org/10.5194/acp-16-12005-2016, https://doi.org/10.5194/acp-16-12005-2016, 2016
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CO2 predictions are used to compute model–data mismatches when estimating surfaces fluxes using atmospheric observations together with an atmospheric transport model. By isolating the component of transport error which is due to uncertain meteorological analyses, it is demonstrated that CO2 can only be defined on large spatial scales. Thus, there is a spatial scale below which we cannot infer fluxes simply due to the fact that meteorological analyes are imperfect.
Vitali E. Fioletov, Chris A. McLinden, Nickolay Krotkov, Can Li, Joanna Joiner, Nicolas Theys, Simon Carn, and Mike D. Moran
Atmos. Chem. Phys., 16, 11497–11519, https://doi.org/10.5194/acp-16-11497-2016, https://doi.org/10.5194/acp-16-11497-2016, 2016
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We introduce the first space-based catalogue of SO2 emission sources seen by OMI. The inventory contains about 500 sources. They account for about a half of all SO2 emissions; the remaining half is likely related to sources emitting less than 30 kt yr−1 and not detected by OMI. The sources are grouped by type (volcanoes, power plants, oil- and gas-related sources, and smelters) and country. The catalogue presented herein can be used for verification of available SO2 emission inventories.
Marsailidh M. Twigg, Evgenia Ilyinskaya, Sonya Beccaceci, David C. Green, Matthew R. Jones, Ben Langford, Sarah R. Leeson, Justin J. N. Lingard, Gloria M. Pereira, Heather Carter, Jan Poskitt, Andreas Richter, Stuart Ritchie, Ivan Simmons, Ron I. Smith, Y. Sim Tang, Netty Van Dijk, Keith Vincent, Eiko Nemitz, Massimo Vieno, and Christine F. Braban
Atmos. Chem. Phys., 16, 11415–11431, https://doi.org/10.5194/acp-16-11415-2016, https://doi.org/10.5194/acp-16-11415-2016, 2016
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This study integrates high and low resolution temporal measurements to assess the impact of the Holuhraun effusive eruption in 2014 across the UK. Measurements, modelling and satellite analysis provides details on the transport and chemistry of both gases and particulates during this unique event. The results of the study can be used verify existing atmospheric chemistry models of volcano plumes in order to carry improved risk assessments for future volcanic eruptions.
Mark Weber, Victor Gorshelev, and Anna Serdyuchenko
Atmos. Meas. Tech., 9, 4459–4470, https://doi.org/10.5194/amt-9-4459-2016, https://doi.org/10.5194/amt-9-4459-2016, 2016
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Ozone absorption cross sections measured in the laboratory using spectroscopic means can be a major source of uncertainty in atmospheric ozone retrievals. In this paper we assess the overall uncertainty in three published UV ozone cross-section datasets that are most popular in the remote sensing community. The overall uncertainties were estimated using Monte Carlo simulations. They are important for traceability of atmospheric ozone measuring instruments to common metrological standards.
Vincent Huijnen, Johannes Flemming, Simon Chabrillat, Quentin Errera, Yves Christophe, Anne-Marlene Blechschmidt, Andreas Richter, and Henk Eskes
Geosci. Model Dev., 9, 3071–3091, https://doi.org/10.5194/gmd-9-3071-2016, https://doi.org/10.5194/gmd-9-3071-2016, 2016
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We present a model description and benchmark evaluation of an extension of the tropospheric chemistry module in the ECMWF Integrated Forecasting System (IFS) with stratospheric chemistry. The stratospheric chemistry originates from the one used in the Belgian Assimilation System for Chemical ObsErvations (BASCOE), and is here combined with the modified CB05 chemistry module for the troposphere as currently used operationally in the Copernicus Atmosphere Monitoring Service (CAMS).
Marie Boichu, Isabelle Chiapello, Colette Brogniez, Jean-Christophe Péré, Francois Thieuleux, Benjamin Torres, Luc Blarel, Augustin Mortier, Thierry Podvin, Philippe Goloub, Nathalie Söhne, Lieven Clarisse, Sophie Bauduin, François Hendrick, Nicolas Theys, Michel Van Roozendael, and Didier Tanré
Atmos. Chem. Phys., 16, 10831–10845, https://doi.org/10.5194/acp-16-10831-2016, https://doi.org/10.5194/acp-16-10831-2016, 2016
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Bárðarbunga eruption emitted huge amounts of sulfur into the lower troposphere causing an unprecedented air pollution in the modern era. A wealth of remote sensing and in situ data allows us to jointly analyse the dynamics of volcanic SO2 and sulfate aerosols. Based on this panel of observations, success and challenges in simulating such volcanogenic long-range pollution events are exposed, focusing on the boundary layer dynamics.
Enrico Dammers, Mathias Palm, Martin Van Damme, Corinne Vigouroux, Dan Smale, Stephanie Conway, Geoffrey C. Toon, Nicholas Jones, Eric Nussbaumer, Thorsten Warneke, Christof Petri, Lieven Clarisse, Cathy Clerbaux, Christian Hermans, Erik Lutsch, Kim Strong, James W. Hannigan, Hideaki Nakajima, Isamu Morino, Beatriz Herrera, Wolfgang Stremme, Michel Grutter, Martijn Schaap, Roy J. Wichink Kruit, Justus Notholt, Pierre-F. Coheur, and Jan Willem Erisman
Atmos. Chem. Phys., 16, 10351–10368, https://doi.org/10.5194/acp-16-10351-2016, https://doi.org/10.5194/acp-16-10351-2016, 2016
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Atmospheric ammonia (NH3) measured by the IASI satellite instrument is compared to observations from ground-based FTIR instruments. The seasonal cycles of NH3 in both datasets are consistent for most sites. Correlations are found to be high at sites with considerable NH3 levels, whereas correlations are lower at sites with low NH3 levels close to the detection limit of the IASI instrument. The study's results further indicate that the IASI-NH3 product performs better than earlier estimates.
Birthe Marie Steensen, Michael Schulz, Nicolas Theys, and Hilde Fagerli
Atmos. Chem. Phys., 16, 9745–9760, https://doi.org/10.5194/acp-16-9745-2016, https://doi.org/10.5194/acp-16-9745-2016, 2016
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The Bardarbunga volcanic fissure during the second half of 2014 caused large amounts of SO2 emission. The paper studies the effects of this increase in pollution levels over Europe during the first 3 months of the eruption with a dispersion model. The model results are compared to satellite and surface concentration observations. The biggest differences are found in Iceland and on the coast of northern Norway. For the average pollution levels over Europe, Iceland is located too far away.
Dhanyalekshmi Pillai, Michael Buchwitz, Christoph Gerbig, Thomas Koch, Maximilian Reuter, Heinrich Bovensmann, Julia Marshall, and John P. Burrows
Atmos. Chem. Phys., 16, 9591–9610, https://doi.org/10.5194/acp-16-9591-2016, https://doi.org/10.5194/acp-16-9591-2016, 2016
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Approximately 70 % of total CO2 emissions arise from cities; however, there exist large uncertainties in quantifying urban emissions. The present study investigates the potential of a satellite mission like CarbonSat to retrieve the city emissions via inverse modelling techniques. The study makes a valid conclusion that an instrument like CarbonSat has high potential to provide important information on city emissions when exploiting the observations using a high-resolution modelling system.
Elpida Leventidou, Kai-Uwe Eichmann, Mark Weber, and John P. Burrows
Atmos. Meas. Tech., 9, 3407–3427, https://doi.org/10.5194/amt-9-3407-2016, https://doi.org/10.5194/amt-9-3407-2016, 2016
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Here, we present a 17 years tropical tropospheric ozone columns dataset (1996–2012) using GOME, SCIAMACHY, and GOME-2 data, developed as part of the verification algorithm for TROPOMI on S5p mission.The uncertainty is less than 2 DU. Validation with SHADOZ ozonesonde data showed biases within 5 DU and RMS errors less than 10 DU. Comparisons with tropospheric ozone columns derived from limb–nadir matching showed that the bias and RMS are within the range of the CCD_IUP comparison with the sondes.
Dimitris Balis, Maria-Elissavet Koukouli, Nikolaos Siomos, Spyridon Dimopoulos, Lucia Mona, Gelsomina Pappalardo, Franco Marenco, Lieven Clarisse, Lucy J. Ventress, Elisa Carboni, Roy G. Grainger, Ping Wang, Gijsbert Tilstra, Ronald van der A, Nicolas Theys, and Claus Zehner
Atmos. Chem. Phys., 16, 5705–5720, https://doi.org/10.5194/acp-16-5705-2016, https://doi.org/10.5194/acp-16-5705-2016, 2016
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The ESA-funded SACS-2 and SMASH projects developed and improved dedicated satellite-derived ash plume and sulfur dioxide level assessments. These estimates were validated using ground-based and aircraft lidar measurements. The validation results are promising for most satellite products and are within the estimated uncertainties of each of the comparative data sets. The IASI data show a better consistency concerning the ash optical depth and ash layer height.
Gerrit Holl, Kaley A. Walker, Stephanie Conway, Naoko Saitoh, Chris D. Boone, Kimberly Strong, and James R. Drummond
Atmos. Meas. Tech., 9, 1961–1980, https://doi.org/10.5194/amt-9-1961-2016, https://doi.org/10.5194/amt-9-1961-2016, 2016
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Methane is a powerful greenhouse gas, and we need to measure it globally with satellite instruments. We compare measurements from two satellites with measurements from the ground in Eureka, Nunavut, Canada to assess their different strengths and weaknesses. The differences between measurements are discussed and assessed considering the details of each measurement technique and processing. Recommendations are provided for utilization of these data sets for monitoring methane in the high Arctic.
Stefan Noël, Klaus Bramstedt, Michael Hilker, Patricia Liebing, Johannes Plieninger, Max Reuter, Alexei Rozanov, Christopher E. Sioris, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 9, 1485–1503, https://doi.org/10.5194/amt-9-1485-2016, https://doi.org/10.5194/amt-9-1485-2016, 2016
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Stratospheric methane (CH4) and carbon dioxide (CO2) profiles have been derived from solar occultation measurements of the SCIAMACHY satellite instrument. The accuracy of these profiles is estimated to be about 5–10 % for CH4 and 2–3 % for CO2, mainly limited by unexpected vertical oscillations. Results are available for August 2002 to April 2012 and latitudes between about 50 and 70° N. From these, time series trends have been estimated, which are in reasonable agreement with total column trends.
Kevin S. Olsen, Geoffrey C. Toon, Chris D. Boone, and Kimberly Strong
Atmos. Meas. Tech., 9, 1063–1082, https://doi.org/10.5194/amt-9-1063-2016, https://doi.org/10.5194/amt-9-1063-2016, 2016
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A new version of the Atmospheric Chemistry Experiment Fourier transform spectrometer was intended to be sent to Mars to perform a detailed study of the composition of the Martian atmosphere. Of critical importance for such a mission is a method to accurately determine the temperature and pressure of the atmosphere. This paper presents a new algorithm for measuring temperature and pressure from high-resolution infrared spectra of CO2 absorption and applies it to terrestrial spectra.
Stefan F. Schreier, Andreas Richter, Folkard Wittrock, and John P. Burrows
Atmos. Chem. Phys., 16, 2803–2817, https://doi.org/10.5194/acp-16-2803-2016, https://doi.org/10.5194/acp-16-2803-2016, 2016
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Mixing ratios of NO2 and HCHO in the free troposphere are obtained from MAX-DOAS measurements at two mountain stations at midlatitudes and in the tropics using a modified geometrical approach. The method is applied in the UV wavelength range and, thus, allows the detection of HCHO mixing ratios, in addition to NO2. We find that mixing ratios of both species are increased in the tropical free troposphere due to biomass burning.
Kai-Uwe Eichmann, Luca Lelli, Christian von Savigny, Harjinder Sembhi, and John P. Burrows
Atmos. Meas. Tech., 9, 793–815, https://doi.org/10.5194/amt-9-793-2016, https://doi.org/10.5194/amt-9-793-2016, 2016
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Height-resolved limb radiance spectra of the satellite instrument SCIAMACHY are used to retrieve cloud top heights with a colour index method. Clouds are detectable from the lower to the uppermost troposphere. These cloud heights help to improve the trace gas retrieval for the upper troposphere and lower stratosphere. Comparisons with other data sets have shown good agreement. As clouds and aerosols are not distinguishable, lower stratospheric volcanic aerosol clouds are detected in some years.
Susan Kulawik, Debra Wunch, Christopher O'Dell, Christian Frankenberg, Maximilian Reuter, Tomohiro Oda, Frederic Chevallier, Vanessa Sherlock, Michael Buchwitz, Greg Osterman, Charles E. Miller, Paul O. Wennberg, David Griffith, Isamu Morino, Manvendra K. Dubey, Nicholas M. Deutscher, Justus Notholt, Frank Hase, Thorsten Warneke, Ralf Sussmann, John Robinson, Kimberly Strong, Matthias Schneider, Martine De Mazière, Kei Shiomi, Dietrich G. Feist, Laura T. Iraci, and Joyce Wolf
Atmos. Meas. Tech., 9, 683–709, https://doi.org/10.5194/amt-9-683-2016, https://doi.org/10.5194/amt-9-683-2016, 2016
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To accurately estimate source and sink locations of carbon dioxide, systematic errors in satellite measurements and models must be characterized. This paper examines two satellite data sets (GOSAT, launched 2009, and SCIAMACHY, launched 2002), and two models (CarbonTracker and MACC) vs. the TCCON CO2 validation data set. We assess biases and errors by season and latitude, satellite performance under averaging, and diurnal variability. Our findings are useful for assimilation of satellite data.
Sophie Bauduin, Lieven Clarisse, Juliette Hadji-Lazaro, Nicolas Theys, Cathy Clerbaux, and Pierre-François Coheur
Atmos. Meas. Tech., 9, 721–740, https://doi.org/10.5194/amt-9-721-2016, https://doi.org/10.5194/amt-9-721-2016, 2016
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The paper presents the development of a new retrieval scheme to infer near-surface sulfur dioxide (SO2) concentrations at a global scale from the Infrared Atmospheric Sounding Interferometer (IASI). It demonstrates the capability of such an instrument to globally monitor anthropogenic SO2 pollution in the case of favourable geophysical conditions, especially high thermal contrast and low humidity.
Yuting Wang, Nicholas M. Deutscher, Mathias Palm, Thorsten Warneke, Justus Notholt, Ian Baker, Joe Berry, Parvadha Suntharalingam, Nicholas Jones, Emmanuel Mahieu, Bernard Lejeune, James Hannigan, Stephanie Conway, Joseph Mendonca, Kimberly Strong, J. Elliott Campbell, Adam Wolf, and Stefanie Kremser
Atmos. Chem. Phys., 16, 2123–2138, https://doi.org/10.5194/acp-16-2123-2016, https://doi.org/10.5194/acp-16-2123-2016, 2016
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OCS could provide an additional constraint on the carbon cycle. The FTIR networks have existed for more than 20 years. For the first time, we used FTIR measurements of OCS and CO2 to study their relationship. We put the coupled CO2 and OCS land fluxes from the Simple Biosphere Model (SiB) into a transport model, and compared the simulations to the measurements. Looking at OCS and CO2 together inspires some new thoughts in how the biospheric models reproduce the carbon cycle in the real world.
Sébastien Massart, Anna Agustí-Panareda, Jens Heymann, Michael Buchwitz, Frédéric Chevallier, Maximilian Reuter, Michael Hilker, John P. Burrows, Nicholas M. Deutscher, Dietrich G. Feist, Frank Hase, Ralf Sussmann, Filip Desmet, Manvendra K. Dubey, David W. T. Griffith, Rigel Kivi, Christof Petri, Matthias Schneider, and Voltaire A. Velazco
Atmos. Chem. Phys., 16, 1653–1671, https://doi.org/10.5194/acp-16-1653-2016, https://doi.org/10.5194/acp-16-1653-2016, 2016
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This study presents the European Centre for Medium-Range Weather Forecasts (ECMWF) monitoring of atmospheric CO2 using measurements from the Greenhouse gases Observing Satellite (GOSAT). We show that the modelled CO2 has a better precision than standard CO2 satellite products compared to ground-based measurements. We also present the CO2 forecast based on our best knowledge of the atmospheric CO2 distribution. We show that it has skill to forecast the largest scale CO2 patterns up to day 5.
S. Hassinen, D. Balis, H. Bauer, M. Begoin, A. Delcloo, K. Eleftheratos, S. Gimeno Garcia, J. Granville, M. Grossi, N. Hao, P. Hedelt, F. Hendrick, M. Hess, K.-P. Heue, J. Hovila, H. Jønch-Sørensen, N. Kalakoski, A. Kauppi, S. Kiemle, L. Kins, M. E. Koukouli, J. Kujanpää, J.-C. Lambert, R. Lang, C. Lerot, D. Loyola, M. Pedergnana, G. Pinardi, F. Romahn, M. van Roozendael, R. Lutz, I. De Smedt, P. Stammes, W. Steinbrecht, J. Tamminen, N. Theys, L. G. Tilstra, O. N. E. Tuinder, P. Valks, C. Zerefos, W. Zimmer, and I. Zyrichidou
Atmos. Meas. Tech., 9, 383–407, https://doi.org/10.5194/amt-9-383-2016, https://doi.org/10.5194/amt-9-383-2016, 2016
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The three GOME-2 instruments will provide unique and long data sets for atmospheric research and applications. The complete time period will be 2007–2022, including the period of ozone depletion as well as the beginning of ozone layer recovery. The GOME-2 products (ozone, trace gases, aerosols and UV radiation) are important for ozone chemistry, air quality studies, climate modeling, policy monitoring and hazard warnings. The processing and dissemination is done by EUMETSAT O3M SAF project.
M. P. Langowski, C. von Savigny, J. P. Burrows, V. V. Rozanov, T. Dunker, U.-P. Hoppe, M. Sinnhuber, and A. C. Aikin
Atmos. Meas. Tech., 9, 295–311, https://doi.org/10.5194/amt-9-295-2016, https://doi.org/10.5194/amt-9-295-2016, 2016
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An algorithm has been developed for the retrieval of sodium atom (Na) number density on a latitude and altitude grid from SCIAMACHY limb measurements of the Na resonance fluorescence (multiannual means 2008–2012). The Na layer peaks at 90 to 93 km altitude and has a FWHM of 5 to 15 km. A summer minimum in peak density and width is observed at high latitudes. At low latitudes, a semiannual oscillation is found. The results are compared with other measurements and models and agree well with these.
F. Ebojie, J. P. Burrows, C. Gebhardt, A. Ladstätter-Weißenmayer, C. von Savigny, A. Rozanov, M. Weber, and H. Bovensmann
Atmos. Chem. Phys., 16, 417–436, https://doi.org/10.5194/acp-16-417-2016, https://doi.org/10.5194/acp-16-417-2016, 2016
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The goal of this study is to determine the global and zonal changes in the tropospheric ozone data product derived from SCIAMACHY limb-nadir-matching (LNM) observations during the period 2003–2011.
Tropospheric O3 shows statistically significant increases over some regions of South Asia, the South American continent, Alaska, around Congo in Africa and over some continental outflows. Significant decrease in TOC is observed over some continents and oceans.
K. Weigel, A. Rozanov, F. Azam, K. Bramstedt, R. Damadeo, K.-U. Eichmann, C. Gebhardt, D. Hurst, M. Kraemer, S. Lossow, W. Read, N. Spelten, G. P. Stiller, K. A. Walker, M. Weber, H. Bovensmann, and J. P. Burrows
Atmos. Meas. Tech., 9, 133–158, https://doi.org/10.5194/amt-9-133-2016, https://doi.org/10.5194/amt-9-133-2016, 2016
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The SCanning Imaging Absorption spectroMeter for Atmospheric CHartographY (SCIAMACHY) aboard the Envisat satellite provided measurements between 2002 and 2012 with different viewing geometries. The limb viewing geometry allows the retrieval of water vapour profiles in the UTLS (upper troposphere and lower stratosphere) from the near-infrared spectral range (1353–1410 nm). Here, we present data version 3.01 and compare it to other water vapour data.
F. Khosrawi, J. Urban, S. Lossow, G. Stiller, K. Weigel, P. Braesicke, M. C. Pitts, A. Rozanov, J. P. Burrows, and D. Murtagh
Atmos. Chem. Phys., 16, 101–121, https://doi.org/10.5194/acp-16-101-2016, https://doi.org/10.5194/acp-16-101-2016, 2016
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Our sensitivity studies based on air parcel trajectories confirm that Polar stratospheric cloud (PSC) formation is quite sensitive to water vapour and temperature changes. Considering water vapour time series from satellite measurements we do not find a consistent, significant trend in water vapour in the lower stratosphere during the past 15 years (2000–2014). Thus, the severe dentrification observed in 2010/2011 cannot be directly related to increases in stratospheric water vapour.
A. Wagner, A.-M. Blechschmidt, I. Bouarar, E.-G. Brunke, C. Clerbaux, M. Cupeiro, P. Cristofanelli, H. Eskes, J. Flemming, H. Flentje, M. George, S. Gilge, A. Hilboll, A. Inness, J. Kapsomenakis, A. Richter, L. Ries, W. Spangl, O. Stein, R. Weller, and C. Zerefos
Atmos. Chem. Phys., 15, 14005–14030, https://doi.org/10.5194/acp-15-14005-2015, https://doi.org/10.5194/acp-15-14005-2015, 2015
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The Monitoring Atmospheric Composition and Climate project (MACC) operationally produces global analyses and forecasts of reactive gases and aerosol fields. We have investigated the ability of the model to simulate concentrations of reactive gases (carbon monoxide, nitrogen dioxide and ozone) between 2009 and 2012. The model reproduced reactive gas concentrations with consistent quality, however, with a seasonally dependent bias compared to surface and satellite observations.
C. von Savigny, F. Ernst, A. Rozanov, R. Hommel, K.-U. Eichmann, V. Rozanov, J. P. Burrows, and L. W. Thomason
Atmos. Meas. Tech., 8, 5223–5235, https://doi.org/10.5194/amt-8-5223-2015, https://doi.org/10.5194/amt-8-5223-2015, 2015
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This article presents validation results for stratospheric aerosol extinction profiles retrieved from limb-scatter measurements with the SCIAMACHY instrument on the Envisat satellite. The SCIAMACHY retrievals are compared to co-located measurements with the SAGE II instrument. Very good agreement to within about 15% is found in a global average sense at altitudes above 15 km. The article also presents sample results on the global morphology of the stratospheric aerosol layer from 2003 to 2011.
A. Schönhardt, P. Altube, K. Gerilowski, S. Krautwurst, J. Hartmann, A. C. Meier, A. Richter, and J. P. Burrows
Atmos. Meas. Tech., 8, 5113–5131, https://doi.org/10.5194/amt-8-5113-2015, https://doi.org/10.5194/amt-8-5113-2015, 2015
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The study reports on the application of an aircraft-based instrument (AirMAP) measuring atmospheric nitrogen dioxide. Two-dimensional maps are produced at a spatial resolution of 28m x 30m and with wide spatial coverage. The instrument characteristics are explained and the detailed mapping of a power plant emission plume is demonstrated. Small-scale enhanced amounts of nitrogen dioxide from traffic are observed above a motorway.
I. De Smedt, T. Stavrakou, F. Hendrick, T. Danckaert, T. Vlemmix, G. Pinardi, N. Theys, C. Lerot, C. Gielen, C. Vigouroux, C. Hermans, C. Fayt, P. Veefkind, J.-F. Müller, and M. Van Roozendael
Atmos. Chem. Phys., 15, 12519–12545, https://doi.org/10.5194/acp-15-12519-2015, https://doi.org/10.5194/acp-15-12519-2015, 2015
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We present the new version of the BIRA-IASB algorithm for the retrieval of H2CO columns from OMI and GOME-2A and B measurements. Validation results at seven stations in Europe, China and Africa confirm the capacity of the satellite measurements to resolve diurnal variations in H2CO columns. Furthermore, vertical profiles derived from MAX-DOAS measurements in Beijing and in Bujumbura are used for a more detailed validation exercise. Finally trends are estimated using 10 years of OMI observations.
D. Pendlebury, D. Plummer, J. Scinocca, P. Sheese, K. Strong, K. Walker, and D. Degenstein
Atmos. Chem. Phys., 15, 12465–12485, https://doi.org/10.5194/acp-15-12465-2015, https://doi.org/10.5194/acp-15-12465-2015, 2015
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The CMAM30 data set takes a chemistry-climate model and relaxes the dynamics to reanalysis, which can then provide chemistry fields not available from the reanalysis data set. This paper addresses this gap by comparing temperature, water vapour, ozone and methane to satellite data to determine and document any biases in the model fields. The lack of ozone destruction and dehydration in the SH polar vortex is shown to be due to the treatment of polar stratosphere clouds in the model.
H. Eskes, V. Huijnen, A. Arola, A. Benedictow, A.-M. Blechschmidt, E. Botek, O. Boucher, I. Bouarar, S. Chabrillat, E. Cuevas, R. Engelen, H. Flentje, A. Gaudel, J. Griesfeller, L. Jones, J. Kapsomenakis, E. Katragkou, S. Kinne, B. Langerock, M. Razinger, A. Richter, M. Schultz, M. Schulz, N. Sudarchikova, V. Thouret, M. Vrekoussis, A. Wagner, and C. Zerefos
Geosci. Model Dev., 8, 3523–3543, https://doi.org/10.5194/gmd-8-3523-2015, https://doi.org/10.5194/gmd-8-3523-2015, 2015
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The MACC project is preparing the operational atmosphere service of the European Copernicus Programme, and uses data assimilation to combine atmospheric models with available observations. Our paper provides an overview of the aerosol and trace gas validation activity of MACC. Topics are the validation requirements, the measurement data, the assimilation systems, the upgrade procedure, operational aspects and the scoring methods. A summary is provided of recent results, including special events.
N. Rahpoe, M. Weber, A. V. Rozanov, K. Weigel, H. Bovensmann, J. P. Burrows, A. Laeng, G. Stiller, T. von Clarmann, E. Kyrölä, V. F. Sofieva, J. Tamminen, K. Walker, D. Degenstein, A. E. Bourassa, R. Hargreaves, P. Bernath, J. Urban, and D. P. Murtagh
Atmos. Meas. Tech., 8, 4369–4381, https://doi.org/10.5194/amt-8-4369-2015, https://doi.org/10.5194/amt-8-4369-2015, 2015
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The analyses among six satellite instruments measuring ozone reveals that the relative drift between the sensors is not significant in the stratosphere and we conclude that merging of data from these instruments is possible. The merged ozone profiles can then be ingested in global climate models for long-term forecasts of ozone and climate change in the atmosphere. The added drift uncertainty is estimated at about 3% per decade (1 sigma) and should be applied in the calculation of ozone trends.
A. Wernecke and L. Kaleschke
The Cryosphere, 9, 1955–1968, https://doi.org/10.5194/tc-9-1955-2015, https://doi.org/10.5194/tc-9-1955-2015, 2015
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Leads in Arctic sea ice have a dominant effect on the exchange between the ocean and the atmosphere. Visual MODIS scenes are used to validate and improve the detection of leads from altimeter measurements of the satellite CryoSat-2. The rarely used maximum power of the returning signal shows the best classification properties. Lead area fraction and width distribution estimates based on CryoSat-2 complement other studies and deepen our understanding of lead characteristics.
S. Bender, M. Sinnhuber, T. von Clarmann, G. Stiller, B. Funke, M. López-Puertas, J. Urban, K. Pérot, K. A. Walker, and J. P. Burrows
Atmos. Meas. Tech., 8, 4171–4195, https://doi.org/10.5194/amt-8-4171-2015, https://doi.org/10.5194/amt-8-4171-2015, 2015
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We compare the nitric oxide (NO) daily zonal mean number density data sets in the mesosphere and lower thermosphere (MLT, 60km to 150km) from four instruments: ACE-FTS (2004--2010), MIPAS (2005--2012), SCIAMACHY (2008--2012), and SMR (2003--2012). We find that these data sets from different instruments consistently constrain NO in the MLT. Thus, they offer reliable forcing inputs for climate and chemistry climate models as an initial step to include solar and geomagnetic activity.
L. Kattner, B. Mathieu-Üffing, J. P. Burrows, A. Richter, S. Schmolke, A. Seyler, and F. Wittrock
Atmos. Chem. Phys., 15, 10087–10092, https://doi.org/10.5194/acp-15-10087-2015, https://doi.org/10.5194/acp-15-10087-2015, 2015
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On 1 January 2015, the International Maritime Organisation tightened the regulations for sulfur content of shipping fuels in Sulfur Emission Control Areas. Here we present data from a station near Hamburg harbour in the North Sea SECA, which uses in situ measurements of atmospheric trace gases to deduce the sulphur fuel content of passing ships. We compare data from 2014 before the regulation change and from January 2015 and show how this method can be used for compliance monitoring.
J. Jia, A. Rozanov, A. Ladstätter-Weißenmayer, and J. P. Burrows
Atmos. Meas. Tech., 8, 3369–3383, https://doi.org/10.5194/amt-8-3369-2015, https://doi.org/10.5194/amt-8-3369-2015, 2015
J. Heymann, M. Reuter, M. Hilker, M. Buchwitz, O. Schneising, H. Bovensmann, J. P. Burrows, A. Kuze, H. Suto, N. M. Deutscher, M. K. Dubey, D. W. T. Griffith, F. Hase, S. Kawakami, R. Kivi, I. Morino, C. Petri, C. Roehl, M. Schneider, V. Sherlock, R. Sussmann, V. A. Velazco, T. Warneke, and D. Wunch
Atmos. Meas. Tech., 8, 2961–2980, https://doi.org/10.5194/amt-8-2961-2015, https://doi.org/10.5194/amt-8-2961-2015, 2015
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Long-term data sets of global atmospheric carbon dioxide concentrations based on observations from different satellite instruments may suffer from inconsistencies originating from the use of different retrieval algorithms. This issue has been addressed by applying the Bremen Optimal Estimation DOAS retrieval algorithm to SCIAMACHY and TANSO-FTS observations. Detailed comparisons with TCCON and CarbonTracker show good consistency between the SCIAMACHY and TANSO-FTS data sets.
T. Dinter, V. V. Rozanov, J. P. Burrows, and A. Bracher
Ocean Sci., 11, 373–389, https://doi.org/10.5194/os-11-373-2015, https://doi.org/10.5194/os-11-373-2015, 2015
A. Inness, A.-M. Blechschmidt, I. Bouarar, S. Chabrillat, M. Crepulja, R. J. Engelen, H. Eskes, J. Flemming, A. Gaudel, F. Hendrick, V. Huijnen, L. Jones, J. Kapsomenakis, E. Katragkou, A. Keppens, B. Langerock, M. de Mazière, D. Melas, M. Parrington, V. H. Peuch, M. Razinger, A. Richter, M. G. Schultz, M. Suttie, V. Thouret, M. Vrekoussis, A. Wagner, and C. Zerefos
Atmos. Chem. Phys., 15, 5275–5303, https://doi.org/10.5194/acp-15-5275-2015, https://doi.org/10.5194/acp-15-5275-2015, 2015
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The paper presents results from data assimilation studies with the new Composition-IFS model developed in the MACC project. This system was used in MACC to produce daily analyses and 5-day forecasts of atmospheric composition and is now run daily in the EU’s Copernicus Atmosphere Monitoring Service. The paper looks at the quality of the CO, O3 and NO2 analysis fields obtained with this system, comparing them against observations, a control run and an older version of the model.
J. Flemming, V. Huijnen, J. Arteta, P. Bechtold, A. Beljaars, A.-M. Blechschmidt, M. Diamantakis, R. J. Engelen, A. Gaudel, A. Inness, L. Jones, B. Josse, E. Katragkou, V. Marecal, V.-H. Peuch, A. Richter, M. G. Schultz, O. Stein, and A. Tsikerdekis
Geosci. Model Dev., 8, 975–1003, https://doi.org/10.5194/gmd-8-975-2015, https://doi.org/10.5194/gmd-8-975-2015, 2015
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We describe modules for atmospheric chemistry, wet and dry deposition and lightning NO production, which have been newly introduced in ECMWF's weather forecasting model. With that model, we want to forecast global air pollution as part of the European Copernicus Atmosphere Monitoring Service. We show that the new model results compare as well or better with in situ and satellite observations of ozone, CO, NO2, SO2 and formaldehyde as the previous model.
S. Barthlott, M. Schneider, F. Hase, A. Wiegele, E. Christner, Y. González, T. Blumenstock, S. Dohe, O. E. García, E. Sepúlveda, K. Strong, J. Mendonca, D. Weaver, M. Palm, N. M. Deutscher, T. Warneke, J. Notholt, B. Lejeune, E. Mahieu, N. Jones, D. W. T. Griffith, V. A. Velazco, D. Smale, J. Robinson, R. Kivi, P. Heikkinen, and U. Raffalski
Atmos. Meas. Tech., 8, 1555–1573, https://doi.org/10.5194/amt-8-1555-2015, https://doi.org/10.5194/amt-8-1555-2015, 2015
C. Viatte, K. Strong, J. Hannigan, E. Nussbaumer, L. K. Emmons, S. Conway, C. Paton-Walsh, J. Hartley, J. Benmergui, and J. Lin
Atmos. Chem. Phys., 15, 2227–2246, https://doi.org/10.5194/acp-15-2227-2015, https://doi.org/10.5194/acp-15-2227-2015, 2015
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Seven tropospheric species (CO, HCN, C2H6, C2H2, CH3OH, HCOOH, and H2CO) released by biomass burning events transported to the high Arctic were monitored with two sets of FTIR measurements, located at Eureka (Nunavut, Canada) and Thule (Greenland), from 2008 to 2012. We compared these data sets with the MOZART-4 chemical transport model to help improve its simulations in the Arctic. Emission factors of these biomass burning products were derived and compared to the literature.
M. P. Langowski, C. von Savigny, J. P. Burrows, W. Feng, J. M. C. Plane, D. R. Marsh, D. Janches, M. Sinnhuber, A. C. Aikin, and P. Liebing
Atmos. Chem. Phys., 15, 273–295, https://doi.org/10.5194/acp-15-273-2015, https://doi.org/10.5194/acp-15-273-2015, 2015
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Global concentration fields of Mg and Mg+ in the Earth's upper mesosphere and lower thermosphere (70-150km) are presented. These are retrieved from SCIAMACHY/Envisat satellite grating spectrometer measurements in limb viewing geometry between 2008 and 2012.
These were compared with WACCM-Mg model results and a large fraction of the available measurement results for these species, and an interpretation of the results is done. The variation of these species during NLC presence is discussed.
M. Reuter, M. Buchwitz, M. Hilker, J. Heymann, O. Schneising, D. Pillai, H. Bovensmann, J. P. Burrows, H. Bösch, R. Parker, A. Butz, O. Hasekamp, C. W. O'Dell, Y. Yoshida, C. Gerbig, T. Nehrkorn, N. M. Deutscher, T. Warneke, J. Notholt, F. Hase, R. Kivi, R. Sussmann, T. Machida, H. Matsueda, and Y. Sawa
Atmos. Chem. Phys., 14, 13739–13753, https://doi.org/10.5194/acp-14-13739-2014, https://doi.org/10.5194/acp-14-13739-2014, 2014
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Current knowledge about the European terrestrial biospheric carbon sink relies upon bottom-up and global surface flux inverse model estimates using in situ measurements. Our analysis of five satellite data sets comprises a regional inversion designed to be insensitive to potential retrieval biases and transport errors. We show that the satellite-derived sink is larger (1.0±0.3GtC/a) than previous estimates (0.4±0.4GtC/a).
G. D. Hayman, F. M. O'Connor, M. Dalvi, D. B. Clark, N. Gedney, C. Huntingford, C. Prigent, M. Buchwitz, O. Schneising, J. P. Burrows, C. Wilson, N. Richards, and M. Chipperfield
Atmos. Chem. Phys., 14, 13257–13280, https://doi.org/10.5194/acp-14-13257-2014, https://doi.org/10.5194/acp-14-13257-2014, 2014
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Globally, wetlands are a major source of methane, which is the second most important greenhouse gas. We find the JULES wetland methane scheme to perform well in general, although there is a tendency for it to overpredict emissions in the tropics and underpredict them in northern latitudes. Our study highlights novel uses of satellite data as a major tool to constrain land-atmosphere methane flux models in a warming world.
J. Aschmann, J. P. Burrows, C. Gebhardt, A. Rozanov, R. Hommel, M. Weber, and A. M. Thompson
Atmos. Chem. Phys., 14, 12803–12814, https://doi.org/10.5194/acp-14-12803-2014, https://doi.org/10.5194/acp-14-12803-2014, 2014
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This study compares observations and simulation results of ozone in the lower tropical stratosphere. It shows that ozone in this region decreased from 1985 up to about 2002, which is consistent with an increase in tropical upwelling predicted by climate models. However, the decrease effectively stops after 2002, indicating that significant changes in tropical upwelling have occurred. The most important factor appears to be that the vertical ascent in the tropics is no longer accelerating.
E. Peters, F. Wittrock, A. Richter, L. M. A. Alvarado, V. V. Rozanov, and J. P. Burrows
Atmos. Meas. Tech., 7, 4203–4221, https://doi.org/10.5194/amt-7-4203-2014, https://doi.org/10.5194/amt-7-4203-2014, 2014
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In this study, a correction spectrum accounting for insufficiencies in commonly used liquid water absorption spectra in DOAS applications is retrieved from ship-borne field measurements. The correction spectrum compensates at the same time for broadband parts of vibrational Raman scattering. With this, an entire compensation of liquid water spectral effects in DOAS applications was achieved.
L. M. A. Alvarado, A. Richter, M. Vrekoussis, F. Wittrock, A. Hilboll, S. F. Schreier, and J. P. Burrows
Atmos. Meas. Tech., 7, 4133–4150, https://doi.org/10.5194/amt-7-4133-2014, https://doi.org/10.5194/amt-7-4133-2014, 2014
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An improved glyoxal retrieval for OMI measurements using the DOAS method has been developed. The retrieval is based on sensitivity tests for the selection of most appropriate retrieval parameters. Also, corrections for reduction of interferences with other species have been applied. In addition, the link between pyrogenic emissions and glyoxal over regions with large wildfires have been investigated, and showed that fires are an important source of glyoxal.
A. Laeng, U. Grabowski, T. von Clarmann, G. Stiller, N. Glatthor, M. Höpfner, S. Kellmann, M. Kiefer, A. Linden, S. Lossow, V. Sofieva, I. Petropavlovskikh, D. Hubert, T. Bathgate, P. Bernath, C. D. Boone, C. Clerbaux, P. Coheur, R. Damadeo, D. Degenstein, S. Frith, L. Froidevaux, J. Gille, K. Hoppel, M. McHugh, Y. Kasai, J. Lumpe, N. Rahpoe, G. Toon, T. Sano, M. Suzuki, J. Tamminen, J. Urban, K. Walker, M. Weber, and J. Zawodny
Atmos. Meas. Tech., 7, 3971–3987, https://doi.org/10.5194/amt-7-3971-2014, https://doi.org/10.5194/amt-7-3971-2014, 2014
T. Wang, F. Hendrick, P. Wang, G. Tang, K. Clémer, H. Yu, C. Fayt, C. Hermans, C. Gielen, J.-F. Müller, G. Pinardi, N. Theys, H. Brenot, and M. Van Roozendael
Atmos. Chem. Phys., 14, 11149–11164, https://doi.org/10.5194/acp-14-11149-2014, https://doi.org/10.5194/acp-14-11149-2014, 2014
J. Strandgren, L. Mei, M. Vountas, J. P. Burrows, A. Lyapustin, and Y. Wang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-14-25869-2014, https://doi.org/10.5194/acpd-14-25869-2014, 2014
Revised manuscript not accepted
K. Noguchi, A. Richter, V. Rozanov, A. Rozanov, J. P. Burrows, H. Irie, and K. Kita
Atmos. Meas. Tech., 7, 3497–3508, https://doi.org/10.5194/amt-7-3497-2014, https://doi.org/10.5194/amt-7-3497-2014, 2014
M. Pastel, J.-P. Pommereau, F. Goutail, A. Richter, A. Pazmiño, D. Ionov, and T. Portafaix
Atmos. Meas. Tech., 7, 3337–3354, https://doi.org/10.5194/amt-7-3337-2014, https://doi.org/10.5194/amt-7-3337-2014, 2014
A. Spolaor, P. Vallelonga, J. Gabrieli, T. Martma, M. P. Björkman, E. Isaksson, G. Cozzi, C. Turetta, H. A. Kjær, M. A. J. Curran, A. D. Moy, A. Schönhardt, A.-M. Blechschmidt, J. P. Burrows, J. M. C. Plane, and C. Barbante
Atmos. Chem. Phys., 14, 9613–9622, https://doi.org/10.5194/acp-14-9613-2014, https://doi.org/10.5194/acp-14-9613-2014, 2014
L. L. Mei, Y. Xue, A. A. Kokhanovsky, W. von Hoyningen-Huene, G. de Leeuw, and J. P. Burrows
Atmos. Meas. Tech., 7, 2411–2420, https://doi.org/10.5194/amt-7-2411-2014, https://doi.org/10.5194/amt-7-2411-2014, 2014
E. Sepúlveda, M. Schneider, F. Hase, S. Barthlott, D. Dubravica, O. E. García, A. Gomez-Pelaez, Y. González, J. C. Guerra, M. Gisi, R. Kohlhepp, S. Dohe, T. Blumenstock, K. Strong, D. Weaver, M. Palm, A. Sadeghi, N. M. Deutscher, T. Warneke, J. Notholt, N. Jones, D. W. T. Griffith, D. Smale, G. W. Brailsford, J. Robinson, F. Meinhardt, M. Steinbacher, T. Aalto, and D. Worthy
Atmos. Meas. Tech., 7, 2337–2360, https://doi.org/10.5194/amt-7-2337-2014, https://doi.org/10.5194/amt-7-2337-2014, 2014
A. W. Zien, A. Richter, A. Hilboll, A.-M. Blechschmidt, and J. P. Burrows
Atmos. Chem. Phys., 14, 7367–7396, https://doi.org/10.5194/acp-14-7367-2014, https://doi.org/10.5194/acp-14-7367-2014, 2014
W. Chehade, M. Weber, and J. P. Burrows
Atmos. Chem. Phys., 14, 7059–7074, https://doi.org/10.5194/acp-14-7059-2014, https://doi.org/10.5194/acp-14-7059-2014, 2014
F. Ebojie, C. von Savigny, A. Ladstätter-Weißenmayer, A. Rozanov, M. Weber, K.-U. Eichmann, S. Bötel, N. Rahpoe, H. Bovensmann, and J. P. Burrows
Atmos. Meas. Tech., 7, 2073–2096, https://doi.org/10.5194/amt-7-2073-2014, https://doi.org/10.5194/amt-7-2073-2014, 2014
J. Yoon, J. P. Burrows, M. Vountas, W. von Hoyningen-Huene, D. Y. Chang, A. Richter, and A. Hilboll
Atmos. Chem. Phys., 14, 6881–6902, https://doi.org/10.5194/acp-14-6881-2014, https://doi.org/10.5194/acp-14-6881-2014, 2014
B. Dils, M. Buchwitz, M. Reuter, O. Schneising, H. Boesch, R. Parker, S. Guerlet, I. Aben, T. Blumenstock, J. P. Burrows, A. Butz, N. M. Deutscher, C. Frankenberg, F. Hase, O. P. Hasekamp, J. Heymann, M. De Mazière, J. Notholt, R. Sussmann, T. Warneke, D. Griffith, V. Sherlock, and D. Wunch
Atmos. Meas. Tech., 7, 1723–1744, https://doi.org/10.5194/amt-7-1723-2014, https://doi.org/10.5194/amt-7-1723-2014, 2014
L. Lelli, A. A. Kokhanovsky, V. V. Rozanov, M. Vountas, and J. P. Burrows
Atmos. Chem. Phys., 14, 5679–5692, https://doi.org/10.5194/acp-14-5679-2014, https://doi.org/10.5194/acp-14-5679-2014, 2014
C. Viatte, K. Strong, K. A. Walker, and J. R. Drummond
Atmos. Meas. Tech., 7, 1547–1570, https://doi.org/10.5194/amt-7-1547-2014, https://doi.org/10.5194/amt-7-1547-2014, 2014
X. Tian-Kunze, L. Kaleschke, N. Maaß, M. Mäkynen, N. Serra, M. Drusch, and T. Krumpen
The Cryosphere, 8, 997–1018, https://doi.org/10.5194/tc-8-997-2014, https://doi.org/10.5194/tc-8-997-2014, 2014
B. Hassler, I. Petropavlovskikh, J. Staehelin, T. August, P. K. Bhartia, C. Clerbaux, D. Degenstein, M. De Mazière, B. M. Dinelli, A. Dudhia, G. Dufour, S. M. Frith, L. Froidevaux, S. Godin-Beekmann, J. Granville, N. R. P. Harris, K. Hoppel, D. Hubert, Y. Kasai, M. J. Kurylo, E. Kyrölä, J.-C. Lambert, P. F. Levelt, C. T. McElroy, R. D. McPeters, R. Munro, H. Nakajima, A. Parrish, P. Raspollini, E. E. Remsberg, K. H. Rosenlof, A. Rozanov, T. Sano, Y. Sasano, M. Shiotani, H. G. J. Smit, G. Stiller, J. Tamminen, D. W. Tarasick, J. Urban, R. J. van der A, J. P. Veefkind, C. Vigouroux, T. von Clarmann, C. von Savigny, K. A. Walker, M. Weber, J. Wild, and J. M. Zawodny
Atmos. Meas. Tech., 7, 1395–1427, https://doi.org/10.5194/amt-7-1395-2014, https://doi.org/10.5194/amt-7-1395-2014, 2014
J. W. Halfacre, T. N. Knepp, P. B. Shepson, C. R. Thompson, K. A. Pratt, B. Li, P. K. Peterson, S. J. Walsh, W. R. Simpson, P. A. Matrai, J. W. Bottenheim, S. Netcheva, D. K. Perovich, and A. Richter
Atmos. Chem. Phys., 14, 4875–4894, https://doi.org/10.5194/acp-14-4875-2014, https://doi.org/10.5194/acp-14-4875-2014, 2014
H. Brenot, N. Theys, L. Clarisse, J. van Geffen, J. van Gent, M. Van Roozendael, R. van der A, D. Hurtmans, P.-F. Coheur, C. Clerbaux, P. Valks, P. Hedelt, F. Prata, O. Rasson, K. Sievers, and C. Zehner
Nat. Hazards Earth Syst. Sci., 14, 1099–1123, https://doi.org/10.5194/nhess-14-1099-2014, https://doi.org/10.5194/nhess-14-1099-2014, 2014
M. Horstjann, M. D. Andrés Hernández, V. Nenakhov, A. Chrobry, and J. P. Burrows
Atmos. Meas. Tech., 7, 1245–1257, https://doi.org/10.5194/amt-7-1245-2014, https://doi.org/10.5194/amt-7-1245-2014, 2014
F. Deng, D. B. A. Jones, D. K. Henze, N. Bousserez, K. W. Bowman, J. B. Fisher, R. Nassar, C. O'Dell, D. Wunch, P. O. Wennberg, E. A. Kort, S. C. Wofsy, T. Blumenstock, N. M. Deutscher, D. W. T. Griffith, F. Hase, P. Heikkinen, V. Sherlock, K. Strong, R. Sussmann, and T. Warneke
Atmos. Chem. Phys., 14, 3703–3727, https://doi.org/10.5194/acp-14-3703-2014, https://doi.org/10.5194/acp-14-3703-2014, 2014
R. Hommel, K.-U. Eichmann, J. Aschmann, K. Bramstedt, M. Weber, C. von Savigny, A. Richter, A. Rozanov, F. Wittrock, F. Khosrawi, R. Bauer, and J. P. Burrows
Atmos. Chem. Phys., 14, 3247–3276, https://doi.org/10.5194/acp-14-3247-2014, https://doi.org/10.5194/acp-14-3247-2014, 2014
L. Clarisse, P.-F. Coheur, N. Theys, D. Hurtmans, and C. Clerbaux
Atmos. Chem. Phys., 14, 3095–3111, https://doi.org/10.5194/acp-14-3095-2014, https://doi.org/10.5194/acp-14-3095-2014, 2014
M. Huntemann, G. Heygster, L. Kaleschke, T. Krumpen, M. Mäkynen, and M. Drusch
The Cryosphere, 8, 439–451, https://doi.org/10.5194/tc-8-439-2014, https://doi.org/10.5194/tc-8-439-2014, 2014
S. F. Schreier, A. Richter, J. W. Kaiser, and J. P. Burrows
Atmos. Chem. Phys., 14, 2447–2466, https://doi.org/10.5194/acp-14-2447-2014, https://doi.org/10.5194/acp-14-2447-2014, 2014
V. Gorshelev, A. Serdyuchenko, M. Weber, W. Chehade, and J. P. Burrows
Atmos. Meas. Tech., 7, 609–624, https://doi.org/10.5194/amt-7-609-2014, https://doi.org/10.5194/amt-7-609-2014, 2014
A. Serdyuchenko, V. Gorshelev, M. Weber, W. Chehade, and J. P. Burrows
Atmos. Meas. Tech., 7, 625–636, https://doi.org/10.5194/amt-7-625-2014, https://doi.org/10.5194/amt-7-625-2014, 2014
A. Redondas, R. Evans, R. Stuebi, U. Köhler, and M. Weber
Atmos. Chem. Phys., 14, 1635–1648, https://doi.org/10.5194/acp-14-1635-2014, https://doi.org/10.5194/acp-14-1635-2014, 2014
C. Gebhardt, A. Rozanov, R. Hommel, M. Weber, H. Bovensmann, J. P. Burrows, D. Degenstein, L. Froidevaux, and A. M. Thompson
Atmos. Chem. Phys., 14, 831–846, https://doi.org/10.5194/acp-14-831-2014, https://doi.org/10.5194/acp-14-831-2014, 2014
M. Langowski, M. Sinnhuber, A. C. Aikin, C. von Savigny, and J. P. Burrows
Atmos. Meas. Tech., 7, 29–48, https://doi.org/10.5194/amt-7-29-2014, https://doi.org/10.5194/amt-7-29-2014, 2014
O. Schneising, M. Reuter, M. Buchwitz, J. Heymann, H. Bovensmann, and J. P. Burrows
Atmos. Chem. Phys., 14, 133–141, https://doi.org/10.5194/acp-14-133-2014, https://doi.org/10.5194/acp-14-133-2014, 2014
N. Maaß, L. Kaleschke, X. Tian-Kunze, and M. Drusch
The Cryosphere, 7, 1971–1989, https://doi.org/10.5194/tc-7-1971-2013, https://doi.org/10.5194/tc-7-1971-2013, 2013
M. Buchwitz, M. Reuter, H. Bovensmann, D. Pillai, J. Heymann, O. Schneising, V. Rozanov, T. Krings, J. P. Burrows, H. Boesch, C. Gerbig, Y. Meijer, and A. Löscher
Atmos. Meas. Tech., 6, 3477–3500, https://doi.org/10.5194/amt-6-3477-2013, https://doi.org/10.5194/amt-6-3477-2013, 2013
V. F. Sofieva, N. Rahpoe, J. Tamminen, E. Kyrölä, N. Kalakoski, M. Weber, A. Rozanov, C. von Savigny, A. Laeng, T. von Clarmann, G. Stiller, S. Lossow, D. Degenstein, A. Bourassa, C. Adams, C. Roth, N. Lloyd, P. Bernath, R. J. Hargreaves, J. Urban, D. Murtagh, A. Hauchecorne, F. Dalaudier, M. van Roozendael, N. Kalb, and C. Zehner
Earth Syst. Sci. Data, 5, 349–363, https://doi.org/10.5194/essd-5-349-2013, https://doi.org/10.5194/essd-5-349-2013, 2013
W. Chehade, V. Gorshelev, A. Serdyuchenko, J. P. Burrows, and M. Weber
Atmos. Meas. Tech., 6, 3055–3065, https://doi.org/10.5194/amt-6-3055-2013, https://doi.org/10.5194/amt-6-3055-2013, 2013
N. Rahpoe, C. von Savigny, M. Weber, A.V. Rozanov, H. Bovensmann, and J. P. Burrows
Atmos. Meas. Tech., 6, 2825–2837, https://doi.org/10.5194/amt-6-2825-2013, https://doi.org/10.5194/amt-6-2825-2013, 2013
D. Griffin, K. A. Walker, J. E. Franklin, M. Parrington, C. Whaley, J. Hopper, J. R. Drummond, P. I. Palmer, K. Strong, T. J. Duck, I. Abboud, P. F. Bernath, C. Clerbaux, P.-F. Coheur, K. R. Curry, L. Dan, E. Hyer, J. Kliever, G. Lesins, M. Maurice, A. Saha, K. Tereszchuk, and D. Weaver
Atmos. Chem. Phys., 13, 10227–10241, https://doi.org/10.5194/acp-13-10227-2013, https://doi.org/10.5194/acp-13-10227-2013, 2013
S. Bender, M. Sinnhuber, J. P. Burrows, M. Langowski, B. Funke, and M. López-Puertas
Atmos. Meas. Tech., 6, 2521–2531, https://doi.org/10.5194/amt-6-2521-2013, https://doi.org/10.5194/amt-6-2521-2013, 2013
W. Chehade, B. Gür, P. Spietz, V. Gorshelev, A. Serdyuchenko, J. P. Burrows, and M. Weber
Atmos. Meas. Tech., 6, 1623–1632, https://doi.org/10.5194/amt-6-1623-2013, https://doi.org/10.5194/amt-6-1623-2013, 2013
P. I. Palmer, M. Parrington, J. D. Lee, A. C. Lewis, A. R. Rickard, P. F. Bernath, T. J. Duck, D. L. Waugh, D. W. Tarasick, S. Andrews, E. Aruffo, L. J. Bailey, E. Barrett, S. J.-B. Bauguitte, K. R. Curry, P. Di Carlo, L. Chisholm, L. Dan, G. Forster, J. E. Franklin, M. D. Gibson, D. Griffin, D. Helmig, J. R. Hopkins, J. T. Hopper, M. E. Jenkin, D. Kindred, J. Kliever, M. Le Breton, S. Matthiesen, M. Maurice, S. Moller, D. P. Moore, D. E. Oram, S. J. O'Shea, R. C. Owen, C. M. L. S. Pagniello, S. Pawson, C. J. Percival, J. R. Pierce, S. Punjabi, R. M. Purvis, J. J. Remedios, K. M. Rotermund, K. M. Sakamoto, A. M. da Silva, K. B. Strawbridge, K. Strong, J. Taylor, R. Trigwell, K. A. Tereszchuk, K. A. Walker, D. Weaver, C. Whaley, and J. C. Young
Atmos. Chem. Phys., 13, 6239–6261, https://doi.org/10.5194/acp-13-6239-2013, https://doi.org/10.5194/acp-13-6239-2013, 2013
N. Theys, R. Campion, L. Clarisse, H. Brenot, J. van Gent, B. Dils, S. Corradini, L. Merucci, P.-F. Coheur, M. Van Roozendael, D. Hurtmans, C. Clerbaux, S. Tait, and F. Ferrucci
Atmos. Chem. Phys., 13, 5945–5968, https://doi.org/10.5194/acp-13-5945-2013, https://doi.org/10.5194/acp-13-5945-2013, 2013
M. D. Andrés-Hernández, D. Kartal, J. N. Crowley, V. Sinha, E. Regelin, M. Martínez-Harder, V. Nenakhov, J. Williams, H. Harder, H. Bozem, W. Song, J. Thieser, M. J. Tang, Z. Hosaynali Beigi, and J. P. Burrows
Atmos. Chem. Phys., 13, 5731–5749, https://doi.org/10.5194/acp-13-5731-2013, https://doi.org/10.5194/acp-13-5731-2013, 2013
Z. Mariani, K. Strong, M. Palm, R. Lindenmaier, C. Adams, X. Zhao, V. Savastiouk, C. T. McElroy, F. Goutail, and J. R. Drummond
Atmos. Meas. Tech., 6, 1549–1565, https://doi.org/10.5194/amt-6-1549-2013, https://doi.org/10.5194/amt-6-1549-2013, 2013
G. Wetzel, H. Oelhaf, G. Berthet, A. Bracher, C. Cornacchia, D. G. Feist, H. Fischer, A. Fix, M. Iarlori, A. Kleinert, A. Lengel, M. Milz, L. Mona, S. C. Müller, J. Ovarlez, G. Pappalardo, C. Piccolo, P. Raspollini, J.-B. Renard, V. Rizi, S. Rohs, C. Schiller, G. Stiller, M. Weber, and G. Zhang
Atmos. Chem. Phys., 13, 5791–5811, https://doi.org/10.5194/acp-13-5791-2013, https://doi.org/10.5194/acp-13-5791-2013, 2013
J.-P. Pommereau, F. Goutail, F. Lefèvre, A. Pazmino, C. Adams, V. Dorokhov, P. Eriksen, R. Kivi, K. Stebel, X. Zhao, and M. van Roozendael
Atmos. Chem. Phys., 13, 5299–5308, https://doi.org/10.5194/acp-13-5299-2013, https://doi.org/10.5194/acp-13-5299-2013, 2013
A. Hilboll, A. Richter, and J. P. Burrows
Atmos. Chem. Phys., 13, 4145–4169, https://doi.org/10.5194/acp-13-4145-2013, https://doi.org/10.5194/acp-13-4145-2013, 2013
I. Ermolli, K. Matthes, T. Dudok de Wit, N. A. Krivova, K. Tourpali, M. Weber, Y. C. Unruh, L. Gray, U. Langematz, P. Pilewskie, E. Rozanov, W. Schmutz, A. Shapiro, S. K. Solanki, and T. N. Woods
Atmos. Chem. Phys., 13, 3945–3977, https://doi.org/10.5194/acp-13-3945-2013, https://doi.org/10.5194/acp-13-3945-2013, 2013
O. Schneising, J. Heymann, M. Buchwitz, M. Reuter, H. Bovensmann, and J. P. Burrows
Atmos. Chem. Phys., 13, 2445–2454, https://doi.org/10.5194/acp-13-2445-2013, https://doi.org/10.5194/acp-13-2445-2013, 2013
A. Hilboll, A. Richter, A. Rozanov, Ø. Hodnebrog, A. Heckel, S. Solberg, F. Stordal, and J. P. Burrows
Atmos. Meas. Tech., 6, 565–584, https://doi.org/10.5194/amt-6-565-2013, https://doi.org/10.5194/amt-6-565-2013, 2013
M. Reuter, H. Bösch, H. Bovensmann, A. Bril, M. Buchwitz, A. Butz, J. P. Burrows, C. W. O'Dell, S. Guerlet, O. Hasekamp, J. Heymann, N. Kikuchi, S. Oshchepkov, R. Parker, S. Pfeifer, O. Schneising, T. Yokota, and Y. Yoshida
Atmos. Chem. Phys., 13, 1771–1780, https://doi.org/10.5194/acp-13-1771-2013, https://doi.org/10.5194/acp-13-1771-2013, 2013
A. E. Jones, E. W. Wolff, N. Brough, S. J.-B. Bauguitte, R. Weller, M. Yela, M. Navarro-Comas, H. A. Ochoa, and N. Theys
Atmos. Chem. Phys., 13, 1457–1467, https://doi.org/10.5194/acp-13-1457-2013, https://doi.org/10.5194/acp-13-1457-2013, 2013
G. Pinardi, M. Van Roozendael, N. Abuhassan, C. Adams, A. Cede, K. Clémer, C. Fayt, U. Frieß, M. Gil, J. Herman, C. Hermans, F. Hendrick, H. Irie, A. Merlaud, M. Navarro Comas, E. Peters, A. J. M. Piters, O. Puentedura, A. Richter, A. Schönhardt, R. Shaiganfar, E. Spinei, K. Strong, H. Takashima, M. Vrekoussis, T. Wagner, F. Wittrock, and S. Yilmaz
Atmos. Meas. Tech., 6, 167–185, https://doi.org/10.5194/amt-6-167-2013, https://doi.org/10.5194/amt-6-167-2013, 2013
A. Tetzlaff, L. Kaleschke, C. Lüpkes, F. Ament, and T. Vihma
The Cryosphere, 7, 153–166, https://doi.org/10.5194/tc-7-153-2013, https://doi.org/10.5194/tc-7-153-2013, 2013
T. Krings, K. Gerilowski, M. Buchwitz, J. Hartmann, T. Sachs, J. Erzinger, J. P. Burrows, and H. Bovensmann
Atmos. Meas. Tech., 6, 151–166, https://doi.org/10.5194/amt-6-151-2013, https://doi.org/10.5194/amt-6-151-2013, 2013
C. Adams, K. Strong, X. Zhao, A. E. Bourassa, W. H. Daffer, D. Degenstein, J. R. Drummond, E. E. Farahani, A. Fraser, N. D. Lloyd, G. L. Manney, C. A. McLinden, M. Rex, C. Roth, S. E. Strahan, K. A. Walker, and I. Wohltmann
Atmos. Chem. Phys., 13, 611–624, https://doi.org/10.5194/acp-13-611-2013, https://doi.org/10.5194/acp-13-611-2013, 2013
P. E. Sheese, K. Strong, E. J. Llewellyn, R. L. Gattinger, J. M. Russell III, C. D. Boone, M. E. Hervig, R. J. Sica, and J. Bandoro
Atmos. Meas. Tech., 5, 2993–3006, https://doi.org/10.5194/amt-5-2993-2012, https://doi.org/10.5194/amt-5-2993-2012, 2012
M. Schneider, S. Barthlott, F. Hase, Y. González, K. Yoshimura, O. E. García, E. Sepúlveda, A. Gomez-Pelaez, M. Gisi, R. Kohlhepp, S. Dohe, T. Blumenstock, A. Wiegele, E. Christner, K. Strong, D. Weaver, M. Palm, N. M. Deutscher, T. Warneke, J. Notholt, B. Lejeune, P. Demoulin, N. Jones, D. W. T. Griffith, D. Smale, and J. Robinson
Atmos. Meas. Tech., 5, 3007–3027, https://doi.org/10.5194/amt-5-3007-2012, https://doi.org/10.5194/amt-5-3007-2012, 2012
Related subject area
Subject: Gases | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Ammonia in the upper troposphere–lower stratosphere (UTLS): GLORIA airborne measurements for CAMS model evaluation in the Asian monsoon and in biomass burning plumes above the South Atlantic
A lightweight NO2-to-NOx conversion model for quantifying NOx emissions of point sources from NO2 satellite observations
Towards a sector-specific CO∕CO2 emission ratio: satellite-based observations of CO release from steel production in Germany
Monitoring European anthropogenic NOx emissions from space
Pyrogenic HONO seen from space: insights from global IASI observations
First evaluation of the GEMS formaldehyde product against TROPOMI and ground-based column measurements during the in-orbit test period
High-resolution mapping of nitrogen oxide emissions in large US cities from TROPOMI retrievals of tropospheric nitrogen dioxide columns
Quantifying the tropospheric ozone radiative effect and its temporal evolution in the satellite era
Improving Ground-Level NO2 Estimation in China Using GEMS Measurements and a Nested Machine Learning Model
Quantifying the diurnal variation of atmospheric NO2 from observations of the Geostationary Environment Monitoring Spectrometer (GEMS)
Tropical tropospheric ozone distribution and trends from in situ and satellite data
Investigation of satellite vertical sensitivity on long-term retrieved lower tropospheric ozone trends
A satellite chronology of plumes from the April 2021 eruption of La Soufrière, St Vincent
Investigation of spatial and temporal variability in lower tropospheric ozone from RAL Space UV–Vis satellite products
Two years of satellite-based carbon dioxide emission quantification at the world's largest coal-fired power plants
Tropical tropospheric ozone and carbon monoxide distributions: characteristics, origins, and control factors, as seen by IAGOS and IASI
Investigation of the summer 2018 European ozone air pollution episodes using novel satellite data and modelling
Bridging the spatial gaps of the Ammonia Monitoring Network using satellite ammonia measurements
A roadmap to estimating agricultural ammonia volatilization over Europe using satellite observations and simulation data
Investigation of meteorological conditions and BrO during ozone depletion events in Ny-Ålesund between 2010 and 2021
Quantification of carbon monoxide emissions from African cities using TROPOMI
Nitrogen oxides emissions from selected cities in North America, Europe, and East Asia observed by the TROPOspheric Monitoring Instrument (TROPOMI) before and after the COVID-19 pandemic
Remotely sensed and surface measurement- derived mass-conserving inversion of daily NOx emissions and inferred combustion technologies in energy-rich northern China
Examining TROPOMI formaldehyde to nitrogen dioxide ratios in the Lake Michigan region: implications for ozone exceedances
Impact of different sources of precursors on an ozone pollution outbreak over Europe analysed with IASI+GOME2 multispectral satellite observations and model simulations
Monitoring and quantifying CO2 emissions of isolated power plants from space
Technical note: Constraining the hydroxyl (OH) radical in the tropics with satellite observations of its drivers – first steps toward assessing the feasibility of a global observation strategy
Significant contribution of inland ships to the total NOx emissions along the Yangtze River
Characteristics of interannual variability in space-based XCO2 global observations
Toward a versatile spaceborne architecture for immediate monitoring of the global methane pledge
Methane emissions are predominantly responsible for record-breaking atmospheric methane growth rates in 2020 and 2021
Ground solar absorption observations of total column CO, CO2, CH4, and aerosol optical depth from California's Sequoia Lightning Complex Fire: emission factors and modified combustion efficiency at regional scales
Potential of TROPOMI for understanding spatio-temporal variations in surface NO2 and their dependencies upon land use over the Iberian Peninsula
Mobile MAX-DOAS observations of tropospheric NO2 and HCHO during summer over the Three Rivers' Source region in China
Estimating enhancement ratios of nitrogen dioxide, carbon monoxide and carbon dioxide using satellite observations
Source mechanisms and transport patterns of tropospheric bromine monoxide: findings from long-term multi-axis differential optical absorption spectroscopy measurements at two Antarctic stations
Measurement report: Spatiotemporal variability of peroxy acyl nitrates (PANs) over Mexico City from TES and CrIS satellite measurements
Biomass burning CO, PM and fuel consumption per unit burned area estimates derived across Africa using geostationary SEVIRI fire radiative power and Sentinel-5P CO data
Characterization of errors in satellite-based HCHO ∕ NO2 tropospheric column ratios with respect to chemistry, column-to-PBL translation, spatial representation, and retrieval uncertainties
Evaluation of transport processes over North China Plain and Yangtze River Delta using MAX-DOAS observations
Estimation of biomass burning emission of NO2 and CO from 2019–2020 Australia fires based on satellite observations
Quantifying daily NOx and CO2 emissions from Wuhan using satellite observations from TROPOMI and OCO-2
Estimation of OH in urban plumes using TROPOMI-inferred NO2 ∕ CO
Diagnosing ozone–NOx–VOC sensitivity and revealing causes of ozone increases in China based on 2013–2021 satellite retrievals
Towards sector-based attribution using intra-city variations in satellite-based emission ratios between CO2 and CO
Measurement report: Evolution and distribution of NH3 over Mexico City from ground-based and satellite infrared spectroscopic measurements
Peculiar COVID-19 effects in the Greater Tokyo Area revealed by spatiotemporal variabilities of tropospheric gases and light-absorbing aerosols
Quantifying NOx emissions in Egypt using TROPOMI observations
Satellite quantification of oil and natural gas methane emissions in the US and Canada including contributions from individual basins
Evaluating NOx emissions and their effect on O3 production in Texas using TROPOMI NO2 and HCHO
Sören Johansson, Michael Höpfner, Felix Friedl-Vallon, Norbert Glatthor, Thomas Gulde, Vincent Huijnen, Anne Kleinert, Erik Kretschmer, Guido Maucher, Tom Neubert, Hans Nordmeyer, Christof Piesch, Peter Preusse, Martin Riese, Björn-Martin Sinnhuber, Jörn Ungermann, Gerald Wetzel, and Wolfgang Woiwode
Atmos. Chem. Phys., 24, 8125–8138, https://doi.org/10.5194/acp-24-8125-2024, https://doi.org/10.5194/acp-24-8125-2024, 2024
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We present airborne infrared limb sounding GLORIA measurements of ammonia (NH3) in the upper troposphere of air masses within the Asian monsoon and of those connected with biomass burning. Comparing CAMS (Copernicus Atmosphere Monitoring Service) model data, we find that the model reproduces the measured enhanced NH3 within the Asian monsoon well but not that within biomass burning plumes, where no enhanced NH3 is measured in the upper troposphere but considerable amounts are simulated by CAMS.
Sandro Meier, Erik F. M. Koene, Maarten Krol, Dominik Brunner, Alexander Damm, and Gerrit Kuhlmann
Atmos. Chem. Phys., 24, 7667–7686, https://doi.org/10.5194/acp-24-7667-2024, https://doi.org/10.5194/acp-24-7667-2024, 2024
Short summary
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Nitrogen oxides (NOx = NO + NO2) are important air pollutants. This study addresses the challenge of accurately estimating NOx emissions from NO2 satellite observations. We develop a realistic model to convert NO2 to NOx by using simulated plumes from various power plants. We apply the model to satellite NO2 observations, significantly reducing biases in estimated NOx emissions. The study highlights the potential for a consistent, high-resolution estimation of NOx emissions using satellite data.
Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Michael Weimer, Heinrich Bovensmann, John P. Burrows, and Hartmut Bösch
Atmos. Chem. Phys., 24, 7609–7621, https://doi.org/10.5194/acp-24-7609-2024, https://doi.org/10.5194/acp-24-7609-2024, 2024
Short summary
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Large quantities of CO and CO2 are emitted during conventional steel production. As satellite-based estimates of CO2 emissions at the facility level are challenging, co-emitted CO can indicate the carbon footprint of steel plants. We estimate CO emissions for German steelworks and use CO2 emissions from emissions trading data to derive a sector-specific CO/CO2 emission ratio for the steel industry; it is a prerequisite to use CO as a proxy for CO2 emissions from similar steel production sites.
Ronald J. van der A, Jieying Ding, and Henk Eskes
Atmos. Chem. Phys., 24, 7523–7534, https://doi.org/10.5194/acp-24-7523-2024, https://doi.org/10.5194/acp-24-7523-2024, 2024
Short summary
Short summary
Using observations of the Sentinel-5P satellite and the latest version of the inversion algorithm DECSO, anthropogenic NOx emissions are derived for Europe for the years 2019–2022 with a spatial resolution of 0.2°. The results are compared with European emissions of the Copernicus Atmosphere Monitoring Service.
Bruno Franco, Lieven Clarisse, Nicolas Theys, Juliette Hadji-Lazaro, Cathy Clerbaux, and Pierre Coheur
Atmos. Chem. Phys., 24, 4973–5007, https://doi.org/10.5194/acp-24-4973-2024, https://doi.org/10.5194/acp-24-4973-2024, 2024
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Using IASI global infrared measurements, we retrieve nitrous acid (HONO) in fire plumes from space. We detect large enhancements of pyrogenic HONO worldwide, especially from intense wildfires at Northern Hemisphere mid- and high latitudes. Predominance of IASI nighttime over daytime measurements sheds light on HONO's extended lifetime and secondary formation during long-range transport in smoke plumes. Our findings deepen the understanding of atmospheric HONO, crucial for air quality assessment.
Gitaek T. Lee, Rokjin J. Park, Hyeong-Ahn Kwon, Eunjo S. Ha, Sieun D. Lee, Seunga Shin, Myoung-Hwan Ahn, Mina Kang, Yong-Sang Choi, Gyuyeon Kim, Dong-Won Lee, Deok-Rae Kim, Hyunkee Hong, Bavo Langerock, Corinne Vigouroux, Christophe Lerot, Francois Hendrick, Gaia Pinardi, Isabelle De Smedt, Michel Van Roozendael, Pucai Wang, Heesung Chong, Yeseul Cho, and Jhoon Kim
Atmos. Chem. Phys., 24, 4733–4749, https://doi.org/10.5194/acp-24-4733-2024, https://doi.org/10.5194/acp-24-4733-2024, 2024
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This study evaluates the Geostationary Environment Monitoring Spectrometer (GEMS) HCHO product by comparing its vertical column densities (VCDs) with those of TROPOMI and ground-based observations. Based on some sensitivity tests, obtaining radiance references under clear-sky conditions significantly improves HCHO retrieval quality. GEMS HCHO VCDs captured seasonal and diurnal variations well during the first year of observation, showing consistency with TROPOMI and ground-based observations.
Fei Liu, Steffen Beirle, Joanna Joiner, Sungyeon Choi, Zhining Tao, K. Emma Knowland, Steven J. Smith, Daniel Q. Tong, Siqi Ma, Zachary T. Fasnacht, and Thomas Wagner
Atmos. Chem. Phys., 24, 3717–3728, https://doi.org/10.5194/acp-24-3717-2024, https://doi.org/10.5194/acp-24-3717-2024, 2024
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Using satellite data, we developed a coupled method independent of the chemical transport model to map NOx emissions across US cities. After validating our technique with synthetic data, we charted NOx emissions from 2018–2021 in 39 cities. Our results closely matched EPA estimates but also highlighted some inconsistencies in both magnitude and spatial distribution. This research can help refine strategies for monitoring and managing air quality.
Richard J. Pope, Alexandru Rap, Matilda A. Pimlott, Brice Barret, Eric Le Flochmoen, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Anne Boynard, Christian Retscher, Wuhu Feng, Richard Rigby, Sandip S. Dhomse, Catherine Wespes, and Martyn P. Chipperfield
Atmos. Chem. Phys., 24, 3613–3626, https://doi.org/10.5194/acp-24-3613-2024, https://doi.org/10.5194/acp-24-3613-2024, 2024
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Tropospheric ozone is an important short-lived climate forcer which influences the incoming solar short-wave radiation and the outgoing long-wave radiation in the atmosphere (8–15 km) where the balance between the two yields a net positive (i.e. warming) effect at the surface. Overall, we find that the tropospheric ozone radiative effect ranges between 1.21 and 1.26 W m−2 with a negligible trend (2008–2017), suggesting that tropospheric ozone influences on climate have remained stable with time.
Naveed Ahmad, Changqing Lin, Alexis K. H. Lau, Jhoon Kim, Fangqun Yu, Chengcai Li, Ying Li, Jimmy C. H. Fung, and Xiang Qian Lao
EGUsphere, https://doi.org/10.5194/egusphere-2024-558, https://doi.org/10.5194/egusphere-2024-558, 2024
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This study developed a nested machine learning model to convert the GEMS NO2 column measurements into ground-level concentrations across China. The model directly incorporates the NO2 mixing height (NMH) into the methodological framework. The study underscores the importance of considering NMH when estimating ground-level NO2 from satellite column measurements and highlights the significant advantages of new-generation geostationary satellites in air quality monitoring.
David P. Edwards, Sara Martínez-Alonso, Duseong S. Jo, Ivan Ortega, Louisa K. Emmons, John J. Orlando, Helen M. Worden, Jhoon Kim, Hanlim Lee, Junsung Park, and Hyunkee Hong
EGUsphere, https://doi.org/10.5194/egusphere-2024-570, https://doi.org/10.5194/egusphere-2024-570, 2024
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Until recently, satellite observations of atmospheric pollutants at any location could only be obtained once-a-day at best. New geostationary satellites stare at a region of the Earth to make hourly measurements, and GEMS is the first looking at Asia. We use GEMS data and atmospheric computer simulations to show how the large change seen during the day for one important pollutant that determines air quality depends on a combination of pollution emissions, atmospheric chemistry, and meteorology.
Audrey Gaudel, Ilann Bourgeois, Meng Li, Kai-Lan Chang, Jerald Ziemke, Bastien Sauvage, Ryan M. Stauffer, Anne M. Thompson, Debra E. Kollonige, Nadia Smith, Daan Hubert, Arno Keppens, Juan Cuesta, Klaus-Peter Heue, Pepijn Veefkind, Kenneth Aikin, Jeff Peischl, Chelsea R. Thompson, Thomas B. Ryerson, Gregory J. Frost, Brian C. McDonald, and Owen R. Cooper
EGUsphere, https://doi.org/10.5194/egusphere-2023-3095, https://doi.org/10.5194/egusphere-2023-3095, 2024
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The study examines tropical tropospheric ozone changes. In situ data from 1994−2019 display increased ozone, notably over India, Southeast Asia, and Malaysia/Indonesia. Sparse in situ data limit trend detection for the 15-year period. In situ and satellite data, with limited sampling, struggle to consistently detect trends. Continuous observations are vital over the tropical Pacific Ocean, Indian Ocean, Western Africa, and South Asia for accurate ozone trend estimation in these regions.
Richard J. Pope, Fiona M. O'Connor, Mohit Dalvi, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Brice Barret, Eric Le Flochmoen, Anne Boynard, Martyn P. Chipperfield, Wuhu Feng, Matilda A. Pimlott, Sandip S. Dhomse, Christian Retscher, Catherine Wespes, and Richard Rigby
EGUsphere, https://doi.org/10.5194/egusphere-2023-3109, https://doi.org/10.5194/egusphere-2023-3109, 2024
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Ozone is a potent air pollutant in the lower troposphere with adverse impacts on human health. Satellite records of tropospheric ozone currently show large-scale inconsistencies in their long-term trends. Our detailed study of the potential factors (e.g. satellite errors, where the satellite can observe ozone) potentially driving these inconsistencies found that in North America, Europe and East Asia, the underlying trends are typically small with large uncertainties.
Isabelle A. Taylor, Roy G. Grainger, Andrew T. Prata, Simon R. Proud, Tamsin A. Mather, and David M. Pyle
Atmos. Chem. Phys., 23, 15209–15234, https://doi.org/10.5194/acp-23-15209-2023, https://doi.org/10.5194/acp-23-15209-2023, 2023
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This study looks at sulfur dioxide (SO2) and ash emissions from the April 2021 eruption of La Soufrière on St Vincent. Using satellite data, 35 eruptive events were identified. Satellite data were used to track SO2 as it was transported around the globe. The majority of SO2 was emitted into the upper troposphere and lower stratosphere. Similarities with the 1979 eruption of La Soufrière highlight the value of studying these eruptions to be better prepared for future eruptions.
Richard J. Pope, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Martyn P. Chipperfield, Wuhu Feng, Matilda A. Pimlott, Sandip S. Dhomse, Christian Retscher, and Richard Rigby
Atmos. Chem. Phys., 23, 14933–14947, https://doi.org/10.5194/acp-23-14933-2023, https://doi.org/10.5194/acp-23-14933-2023, 2023
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Ozone is a potent air pollutant, and we present the first study to investigate long-term changes in lower tropospheric column ozone (LTCO3) from space. We have constructed a merged LTCO3 dataset from GOME-1, SCIAMACHY and OMI between 1996 and 2017. Comparing LTCO3 between the 1996–2000 and 2013–2017 5-year averages, we find significant positive increases in the tropics/sub-tropics, while in the northern mid-latitudes, we find small-scale differences.
Daniel H. Cusworth, Andrew K. Thorpe, Charles E. Miller, Alana K. Ayasse, Ralph Jiorle, Riley M. Duren, Ray Nassar, Jon-Paul Mastrogiacomo, and Robert R. Nelson
Atmos. Chem. Phys., 23, 14577–14591, https://doi.org/10.5194/acp-23-14577-2023, https://doi.org/10.5194/acp-23-14577-2023, 2023
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Carbon dioxide (CO2) emissions from combustion sources are uncertain in many places across the globe. Satellites have the ability to detect and quantify emissions from large CO2 point sources, including coal-fired power plants. In this study, we tasked two satellites to routinely observe CO2 emissions at 30 coal-fired power plants between 2021 and 2022. These results present the largest dataset of space-based CO2 emission estimates to date.
Maria Tsivlidou, Bastien Sauvage, Yasmine Bennouna, Romain Blot, Damien Boulanger, Hannah Clark, Eric Le Flochmoën, Philippe Nédélec, Valérie Thouret, Pawel Wolff, and Brice Barret
Atmos. Chem. Phys., 23, 14039–14063, https://doi.org/10.5194/acp-23-14039-2023, https://doi.org/10.5194/acp-23-14039-2023, 2023
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The tropics are a region where the ozone increase has been most apparent since 1980 and where observations are sparse. Using aircraft, satellite, and model data, we document the characteristics of tropospheric ozone and CO over the whole tropics for the last 2 decades. We explore the origin of the observed CO anomalies and investigate transport processes driving the tropical CO and O3 distribution. Our study highlights the importance of anthropogenic emissions, mostly over the northern tropics.
Richard J. Pope, Brian J. Kerridge, Martyn P. Chipperfield, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Matilda A. Pimlott, Wuhu Feng, Edward Comyn-Platt, Garry D. Hayman, Stephen R. Arnold, and Ailish M. Graham
Atmos. Chem. Phys., 23, 13235–13253, https://doi.org/10.5194/acp-23-13235-2023, https://doi.org/10.5194/acp-23-13235-2023, 2023
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In the summer of 2018, Europe experienced several persistent large-scale ozone (O3) pollution episodes. Satellite tropospheric O3 and surface O3 data recorded substantial enhancements in 2018 relative to other years. Targeted model simulations showed that meteorological processes and emissions controlled the elevated surface O3, while mid-tropospheric O3 enhancements were dominated by stratospheric O3 intrusion and advection of North Atlantic O3-rich air masses into Europe.
Rui Wang, Da Pan, Xuehui Guo, Kang Sun, Lieven Clarisse, Martin Van Damme, Pierre-François Coheur, Cathy Clerbaux, Melissa Puchalski, and Mark A. Zondlo
Atmos. Chem. Phys., 23, 13217–13234, https://doi.org/10.5194/acp-23-13217-2023, https://doi.org/10.5194/acp-23-13217-2023, 2023
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Ammonia (NH3) is a key precursor for fine particulate matter (PM2.5) and a primary form of reactive nitrogen, yet it has sparse ground measurements. We perform the first comprehensive comparison between ground observations and satellite retrievals in the US, demonstrating that satellite NH3 data can help fill spatial gaps in the current ground monitoring networks. Trend analyses using both datasets highlight increasing NH3 trends across the US, including the NH3 hotspots and urban areas.
Rimal Abeed, Camille Viatte, William C. Porter, Nikolaos Evangeliou, Cathy Clerbaux, Lieven Clarisse, Martin Van Damme, Pierre-François Coheur, and Sarah Safieddine
Atmos. Chem. Phys., 23, 12505–12523, https://doi.org/10.5194/acp-23-12505-2023, https://doi.org/10.5194/acp-23-12505-2023, 2023
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Ammonia emissions from agricultural activities will inevitably increase with the rise in population. We use a variety of datasets (satellite, reanalysis, and model simulation) to calculate the first regional map of ammonia emission potential during the start of the growing season in Europe. We then apply our developed method using a climate model to show the effect of the temperature increase on future ammonia columns under two possible climate scenarios.
Bianca Zilker, Andreas Richter, Anne-Marlene Blechschmidt, Peter von der Gathen, Ilias Bougoudis, Sora Seo, Tim Bösch, and John Philip Burrows
Atmos. Chem. Phys., 23, 9787–9814, https://doi.org/10.5194/acp-23-9787-2023, https://doi.org/10.5194/acp-23-9787-2023, 2023
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During Arctic spring, near-surface ozone is depleted by bromine released from salty sea ice and/or snow-covered areas under certain meteorological conditions. To study this ozone depletion and the prevailing meteorological conditions, two ozone data sets from Ny-Ålesund, Svalbard, have been evaluated. We found that during ozone depletion events lower pressure over the Barents Sea and higher pressure in the Icelandic Low area led to a transport of cold polar air from the north to Ny-Ålesund.
Gijs Leguijt, Joannes D. Maasakkers, Hugo A. C. Denier van der Gon, Arjo J. Segers, Tobias Borsdorff, and Ilse Aben
Atmos. Chem. Phys., 23, 8899–8919, https://doi.org/10.5194/acp-23-8899-2023, https://doi.org/10.5194/acp-23-8899-2023, 2023
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We present a fast method to evaluate carbon monoxide emissions from cities in Africa. Carbon monoxide is important for climate change in an indirect way, as it is linked to ozone, methane, and carbon dioxide. Our measurements are made with a satellite that sees the entire globe every single day. This means that we can check from space whether the current knowledge of emission rates is up to date. We make the comparison and show that the emission rates in northern Africa are underestimated.
Chantelle R. Lonsdale and Kang Sun
Atmos. Chem. Phys., 23, 8727–8748, https://doi.org/10.5194/acp-23-8727-2023, https://doi.org/10.5194/acp-23-8727-2023, 2023
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The COVID-19 pandemic, which was caused by the SARS-CoV-2 virus, emerged in 2019, and its still evolving variants have resulted in unprecedented shifts in human activities and anthropogenic emissions into the Earth's atmosphere. We present monthly nitrogen oxide emissions over three major continents from May 2018 to January 2023 to capture variations before and after the COVID-19 pandemic. We focus on a diverse collection of 54 cities to quantify the post-COVID-19 perturbations.
Xiaolu Li, Jason Blake Cohen, Kai Qin, Hong Geng, Xiaohui Wu, Liling Wu, Chengli Yang, Rui Zhang, and Liqin Zhang
Atmos. Chem. Phys., 23, 8001–8019, https://doi.org/10.5194/acp-23-8001-2023, https://doi.org/10.5194/acp-23-8001-2023, 2023
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Remotely sensed NO2 and surface NOx are combined with a mathematical method to estimate daily NOx emissions. The results identify new sources and improve existing estimates. The estimation is driven by three flexible factors: thermodynamics of combustion, chemical loss, and atmospheric transport. The thermodynamic term separates power, iron, and cement from coking, boilers, and aluminum. This work finds three causes for the extremes: emissions, UV radiation, and transport.
Juanito Jerrold Mariano Acdan, Robert Bradley Pierce, Angela F. Dickens, Zachariah Adelman, and Tsengel Nergui
Atmos. Chem. Phys., 23, 7867–7885, https://doi.org/10.5194/acp-23-7867-2023, https://doi.org/10.5194/acp-23-7867-2023, 2023
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Ozone is an air pollutant that is harmful to human health. Near the surface of Earth, ozone is created when other pollutants react in the presence of sunlight. This study uses satellite data to investigate how ozone levels can be decreased in the Lake Michigan region of the United States. Our results indicate that ozone levels can be decreased by decreasing volatile organic compound emissions in urban areas and decreasing nitrogen oxide emissions in the region as a whole.
Sachiko Okamoto, Juan Cuesta, Matthias Beekmann, Gaëlle Dufour, Maxim Eremenko, Kazuyuki Miyazaki, Cathy Boonne, Hiroshi Tanimoto, and Hajime Akimoto
Atmos. Chem. Phys., 23, 7399–7423, https://doi.org/10.5194/acp-23-7399-2023, https://doi.org/10.5194/acp-23-7399-2023, 2023
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We present a detailed analysis of the daily evolution of the lowermost tropospheric ozone documented by IASI+GOME2 multispectral satellite observations and that of its precursors from TCR-2 tropospheric chemistry reanalysis. It reveals that the ozone outbreak across Europe in July 2017 was produced during favorable condition for photochemical production of ozone and was associated with multiple sources of ozone precursors: biogenic, anthropogenic, and biomass burning emissions.
Xiaojuan Lin, Ronald van der A, Jos de Laat, Henk Eskes, Frédéric Chevallier, Philippe Ciais, Zhu Deng, Yuanhao Geng, Xuanren Song, Xiliang Ni, Da Huo, Xinyu Dou, and Zhu Liu
Atmos. Chem. Phys., 23, 6599–6611, https://doi.org/10.5194/acp-23-6599-2023, https://doi.org/10.5194/acp-23-6599-2023, 2023
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Satellite observations provide evidence for CO2 emission signals from isolated power plants. We use these satellite observations to quantify emissions. We found that for power plants with multiple observations, the correlation of estimated and reported emissions is significantly improved compared to a single observation case. This demonstrates that accurate estimation of power plant emissions can be achieved by monitoring from future satellite missions with more frequent observations.
Daniel C. Anderson, Bryan N. Duncan, Julie M. Nicely, Junhua Liu, Sarah A. Strode, and Melanie B. Follette-Cook
Atmos. Chem. Phys., 23, 6319–6338, https://doi.org/10.5194/acp-23-6319-2023, https://doi.org/10.5194/acp-23-6319-2023, 2023
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We describe a methodology that combines machine learning, satellite observations, and 3D chemical model output to infer the abundance of the hydroxyl radical (OH), a chemical that removes many trace gases from the atmosphere. The methodology successfully captures the variability of observed OH, although further observations are needed to evaluate absolute accuracy. Current satellite observations are of sufficient quality to infer OH, but retrieval validation in the remote tropics is needed.
Xiumei Zhang, Ronald van der A, Jieying Ding, Xin Zhang, and Yan Yin
Atmos. Chem. Phys., 23, 5587–5604, https://doi.org/10.5194/acp-23-5587-2023, https://doi.org/10.5194/acp-23-5587-2023, 2023
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We compiled a ship emission inventory based on automatic identification system (AIS) signals in the Jiangsu section of the Yangtze River. This ship emission inventory was compared with Chinese bottom-up inventories and the satellite-derived emissions from TROPOMI. The result shows a consistent spatial distribution, with riverine cities having high NOx emissions. Inland ship emissions of NOx are shown to contribute at least 40 % to air pollution along the river.
Yifan Guan, Gretchen Keppel-Aleks, Scott C. Doney, Christof Petri, Dave Pollard, Debra Wunch, Frank Hase, Hirofumi Ohyama, Isamu Morino, Justus Notholt, Kei Shiomi, Kim Strong, Rigel Kivi, Matthias Buschmann, Nicholas Deutscher, Paul Wennberg, Ralf Sussmann, Voltaire A. Velazco, and Yao Té
Atmos. Chem. Phys., 23, 5355–5372, https://doi.org/10.5194/acp-23-5355-2023, https://doi.org/10.5194/acp-23-5355-2023, 2023
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We characterize spatial–temporal patterns of interannual variability (IAV) in atmospheric CO2 based on NASA’s Orbiting Carbon Observatory-2 (OCO-2). CO2 variation is strongly impacted by climate events, with higher anomalies during El Nino years. We show high correlation in IAV between space-based and ground-based CO2 from long-term sites. Because OCO-2 has near-global coverage, our paper provides a roadmap to study IAV where in situ observation is sparse, such as open oceans and remote lands.
Yuchen Wang, Xvli Guo, Yajie Huo, Mengying Li, Yuqing Pan, Shaocai Yu, Alexander Baklanov, Daniel Rosenfeld, John H. Seinfeld, and Pengfei Li
Atmos. Chem. Phys., 23, 5233–5249, https://doi.org/10.5194/acp-23-5233-2023, https://doi.org/10.5194/acp-23-5233-2023, 2023
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Substantial advances have been made in recent years toward detecting and quantifying methane super-emitters from space. However, such advances have rarely been expanded to measure the global methane pledge because large-scale swaths and high-resolution sampling have not been coordinated. Here we present a versatile spaceborne architecture that can juggle planet-scale and plant-level methane retrievals, challenge official emission reports, and remain relevant for stereoscopic measurements.
Liang Feng, Paul I. Palmer, Robert J. Parker, Mark F. Lunt, and Hartmut Bösch
Atmos. Chem. Phys., 23, 4863–4880, https://doi.org/10.5194/acp-23-4863-2023, https://doi.org/10.5194/acp-23-4863-2023, 2023
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Our understanding of recent changes in atmospheric methane has defied explanation. Since 2007, the atmospheric growth of methane has accelerated to record-breaking values in 2020 and 2021. We use satellite observations of methane to show that (1) increasing emissions over the tropics are mostly responsible for these recent atmospheric changes, and (2) changes in the OH sink during the 2020 Covid-19 lockdown can explain up to 34% of changes in atmospheric methane for that year.
Isis Frausto-Vicencio, Sajjan Heerah, Aaron G. Meyer, Harrison A. Parker, Manvendra Dubey, and Francesca M. Hopkins
Atmos. Chem. Phys., 23, 4521–4543, https://doi.org/10.5194/acp-23-4521-2023, https://doi.org/10.5194/acp-23-4521-2023, 2023
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Wildfires are increasing in the western USA, making it critical to understand the impacts of greenhouse gases and air pollutants on the atmosphere. We used a ground-based remote sensing technique to measure the greenhouse gases and aerosol in the atmosphere. We isolate a large smoke plume from a nearby wildfire and calculate variables to understand the fuel properties and combustion phases. We find that a significant amount of methane is emitted from the 2020 California wildfire season.
Hervé Petetin, Marc Guevara, Steven Compernolle, Dene Bowdalo, Pierre-Antoine Bretonnière, Santiago Enciso, Oriol Jorba, Franco Lopez, Albert Soret, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 23, 3905–3935, https://doi.org/10.5194/acp-23-3905-2023, https://doi.org/10.5194/acp-23-3905-2023, 2023
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This study analyses the potential of the TROPOMI space sensor for monitoring the variability of NO2 pollution over the Iberian Peninsula. A reduction of NO2 levels is observed during the weekend and in summer, especially over most urbanized areas, in agreement with surface observations. An enhancement of NO2 is found during summer with TROPOMI over croplands, potentially related to natural soil NO emissions, which illustrates the outstanding value of TROPOMI for complementing surface networks.
Siyang Cheng, Xinghong Cheng, Jianzhong Ma, Xiangde Xu, Wenqian Zhang, Jinguang Lv, Gang Bai, Bing Chen, Siying Ma, Steffen Ziegler, Sebastian Donner, and Thomas Wagner
Atmos. Chem. Phys., 23, 3655–3677, https://doi.org/10.5194/acp-23-3655-2023, https://doi.org/10.5194/acp-23-3655-2023, 2023
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We made mobile MAX-DOAS measurements in the background atmosphere over the Tibetan Plateau in summer 2021. We retrieved the tropospheric NO2 and HCHO vertical column densities (VCDs) along extended driving routes and found a decreasing trend of the VCDs with altitude. Elevated NO2 VCDs along the driving routes could be attributed to enhanced traffic emissions from the towns crossed. The spatio-temporal distribution of the HCHO VCDs correlated strongly with the surface temperature.
Cameron G. MacDonald, Jon-Paul Mastrogiacomo, Joshua L. Laughner, Jacob K. Hedelius, Ray Nassar, and Debra Wunch
Atmos. Chem. Phys., 23, 3493–3516, https://doi.org/10.5194/acp-23-3493-2023, https://doi.org/10.5194/acp-23-3493-2023, 2023
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We use three satellites measuring carbon dioxide (CO2), carbon monoxide (CO) and nitrogen dioxide (NO2) to calculate atmospheric enhancements of these gases from 27 urban areas. We calculate enhancement ratios between the species and compare those to ratios derived from four globally gridded anthropogenic emission inventories. We find that the global inventories generally underestimate CO emissions in many North American and European cities relative to our observed enhancement ratios.
Udo Frieß, Karin Kreher, Richard Querel, Holger Schmithüsen, Dan Smale, Rolf Weller, and Ulrich Platt
Atmos. Chem. Phys., 23, 3207–3232, https://doi.org/10.5194/acp-23-3207-2023, https://doi.org/10.5194/acp-23-3207-2023, 2023
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Reactive bromine compounds, emitted by the sea ice during polar spring, play an important role in the atmospheric chemistry of the coastal regions of Antarctica. We investigate the sources and impacts of reactive bromine in detail using many years of measurements at two Antarctic sites located at opposite sides of the Antarctic continent. Using a multitude of meteorological observations, we were able to identify the main triggers and source regions for reactive bromine in Antarctica.
Madison J. Shogrin, Vivienne H. Payne, Susan S. Kulawik, Kazuyuki Miyazaki, and Emily V. Fischer
Atmos. Chem. Phys., 23, 2667–2682, https://doi.org/10.5194/acp-23-2667-2023, https://doi.org/10.5194/acp-23-2667-2023, 2023
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We evaluate the spatiotemporal variability of peroxy acyl nitrates (PANs), important photochemical pollutants, over Mexico City using satellite observations. PANs exhibit a seasonal cycle that maximizes in spring. Wildfires contribute to observed interannual variability, and the satellite indicates several areas of frequent outflow. Recent changes in NOx emissions are not accompanied by changes in PANs. This work demonstrates analysis approaches that can be applied to other megacities.
Hannah M. Nguyen, Jiangping He, and Martin J. Wooster
Atmos. Chem. Phys., 23, 2089–2118, https://doi.org/10.5194/acp-23-2089-2023, https://doi.org/10.5194/acp-23-2089-2023, 2023
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This work presents novel advances in the estimation of open biomass burning emissions via the first fully "top-down" approach to exploit satellite-derived observations of fire radiative power and carbon monoxide over Africa. We produce a 16-year record of fire-generated CO emissions and dry matter consumed per unit area for Africa and evaluate these emissions estimates through their use in an atmospheric model, whose simulation output is then compared to independent satellite observations of CO.
Amir H. Souri, Matthew S. Johnson, Glenn M. Wolfe, James H. Crawford, Alan Fried, Armin Wisthaler, William H. Brune, Donald R. Blake, Andrew J. Weinheimer, Tijl Verhoelst, Steven Compernolle, Gaia Pinardi, Corinne Vigouroux, Bavo Langerock, Sungyeon Choi, Lok Lamsal, Lei Zhu, Shuai Sun, Ronald C. Cohen, Kyung-Eun Min, Changmin Cho, Sajeev Philip, Xiong Liu, and Kelly Chance
Atmos. Chem. Phys., 23, 1963–1986, https://doi.org/10.5194/acp-23-1963-2023, https://doi.org/10.5194/acp-23-1963-2023, 2023
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We have rigorously characterized different sources of error in satellite-based HCHO / NO2 tropospheric columns, a widely used metric for diagnosing near-surface ozone sensitivity. Specifically, the errors were categorized/quantified into (i) an inherent chemistry error, (ii) the decoupled relationship between columns and the near-surface concentration, (iii) the spatial representativeness error of ground satellite pixels, and (iv) the satellite retrieval errors.
Yuhang Song, Chengzhi Xing, Cheng Liu, Jinan Lin, Hongyu Wu, Ting Liu, Hua Lin, Chengxin Zhang, Wei Tan, Xiangguang Ji, Haoran Liu, and Qihua Li
Atmos. Chem. Phys., 23, 1803–1824, https://doi.org/10.5194/acp-23-1803-2023, https://doi.org/10.5194/acp-23-1803-2023, 2023
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Using the MAX-DOAS network, we successfully analyzed three typical transport types (regional, dust, and transboundary long-range transport), emphasizing the unique advantages provided by the network in monitoring pollutant transport. We think that our findings provide the public with a thorough understanding of pollutant transport phenomena and a reference for designing collaborative air pollution control strategies.
Nenghan Wan, Xiaozhen Xiong, Gerard J. Kluitenberg, J. M. Shawn Hutchinson, Robert Aiken, Haidong Zhao, and Xiaomao Lin
Atmos. Chem. Phys., 23, 711–724, https://doi.org/10.5194/acp-23-711-2023, https://doi.org/10.5194/acp-23-711-2023, 2023
Short summary
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This study used new TROPOMI measurements of NO2 and CO to characterize regional biomass burning characteristics and efficiency. We found that the NO2 / CO emission ratio was consistent with recent studies over temperate forest fires but slightly lower in savanna vegetation fires. Our results can help identify the relative contribution of smoldering and flaming activities as well as their impacts on the regional atmospheric composition and air quality.
Qianqian Zhang, K. Folkert Boersma, Bin Zhao, Henk Eskes, Cuihong Chen, Haotian Zheng, and Xingying Zhang
Atmos. Chem. Phys., 23, 551–563, https://doi.org/10.5194/acp-23-551-2023, https://doi.org/10.5194/acp-23-551-2023, 2023
Short summary
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We developed an improved superposition column model and used the latest released (v2.3.1) TROPOMI satellite NO2 observations to estimate daily city-scale NOx and CO2 emissions. The results are verified against bottom-up emissions and OCO-2 XCO2 observations. We obtained the day-to-day variation of city NOx and CO2 emissions, allowing policymakers to gain real-time information on spatial–temporal emission patterns and the effectiveness of carbon and nitrogen regulation in urban environments.
Srijana Lama, Sander Houweling, K. Folkert Boersma, Ilse Aben, Hugo A. C. Denier van der Gon, and Maarten C. Krol
Atmos. Chem. Phys., 22, 16053–16071, https://doi.org/10.5194/acp-22-16053-2022, https://doi.org/10.5194/acp-22-16053-2022, 2022
Short summary
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Hydroxyl radical (OH) is the important chemical species that determines the lifetime of some greenhouse gases and trace gases. OH plays a vital role in air pollution chemistry. OH has a short lifetime and is extremely difficult to measure directly. OH concentrations derived from the chemistry transport model (CTM) have uncertainties of >50 %. Therefore, in this study, OH is derived indirectly using satellite date in urban plumes.
Jie Ren, Fangfang Guo, and Shaodong Xie
Atmos. Chem. Phys., 22, 15035–15047, https://doi.org/10.5194/acp-22-15035-2022, https://doi.org/10.5194/acp-22-15035-2022, 2022
Short summary
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O3–NOx–VOC sensitivity in China is diagnosed by deriving regional satellite HCHO / NO2 thresholds between O3 production regimes. VOC-limited regimes are found widely over megacity clusters and developed cities. VOCs and NOx emissions are tracked with satellite HCHO and NO2 to evaluate O3 responses to precursors changes. The significant reduction in NOx emissions without effective VOC control since the Clean Air Action Plan in 2013 is responsible for the increase in O3 concentrations in China.
Dien Wu, Junjie Liu, Paul O. Wennberg, Paul I. Palmer, Robert R. Nelson, Matthäus Kiel, and Annmarie Eldering
Atmos. Chem. Phys., 22, 14547–14570, https://doi.org/10.5194/acp-22-14547-2022, https://doi.org/10.5194/acp-22-14547-2022, 2022
Short summary
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Prior studies have derived the combustion efficiency for a region/city using observed CO2 and CO. We further zoomed into the urban domain and accounted for factors affecting the calculation of spatially resolved combustion efficiency from two satellites. The intra-city variability in combustion efficiency was linked to heavy industry within Shanghai and LA without relying on emission inventories. Such an approach can be applied when analyzing data from future geostationary satellites.
Beatriz Herrera, Alejandro Bezanilla, Thomas Blumenstock, Enrico Dammers, Frank Hase, Lieven Clarisse, Adolfo Magaldi, Claudia Rivera, Wolfgang Stremme, Kimberly Strong, Camille Viatte, Martin Van Damme, and Michel Grutter
Atmos. Chem. Phys., 22, 14119–14132, https://doi.org/10.5194/acp-22-14119-2022, https://doi.org/10.5194/acp-22-14119-2022, 2022
Short summary
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This work investigates atmospheric ammonia (NH3), a key trace gas with consequences for the environment and human health, in Mexico City. The results from the ground-based and satellite instruments show the variability and spatial distribution of NH3 over this region. NH3 in Mexico City has been increasing for the past 10 years and most of its sources are urban. This work contributes to a better understanding of NH3 sources and variability in urban and remote areas.
Alessandro Damiani, Hitoshi Irie, Dmitry A. Belikov, Shuei Kaizuka, Hossain Mohammed Syedul Hoque, and Raul R. Cordero
Atmos. Chem. Phys., 22, 12705–12726, https://doi.org/10.5194/acp-22-12705-2022, https://doi.org/10.5194/acp-22-12705-2022, 2022
Short summary
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We analyzed the variabilities in tropospheric gases and aerosols within the Greater Tokyo Area, Japan. Beyond highlighting air quality changes caused by the pandemic during the lockdown, we found that the degree of weekly cycling of most gases and aerosols was enhanced during the whole of 2020. The changes were unprecedented in recent years and potentially related to coincident reduced mobility in Japan, which, in contrast to other countries, was anomalously low on weekends in 2020.
Anthony Rey-Pommier, Frédéric Chevallier, Philippe Ciais, Grégoire Broquet, Theodoros Christoudias, Jonilda Kushta, Didier Hauglustaine, and Jean Sciare
Atmos. Chem. Phys., 22, 11505–11527, https://doi.org/10.5194/acp-22-11505-2022, https://doi.org/10.5194/acp-22-11505-2022, 2022
Short summary
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Emission inventories for air pollutants can be uncertain in developing countries. In order to overcome these uncertainties, we model nitrogen oxide emissions in Egypt using satellite retrievals. We detect a weekly cycle reflecting Egyptian social norms, an annual cycle consistent with electricity consumption and an activity drop due to the COVID-19 pandemic. However, discrepancies with inventories remain high, illustrating the needs for additional data to improve the potential of our method.
Lu Shen, Ritesh Gautam, Mark Omara, Daniel Zavala-Araiza, Joannes D. Maasakkers, Tia R. Scarpelli, Alba Lorente, David Lyon, Jianxiong Sheng, Daniel J. Varon, Hannah Nesser, Zhen Qu, Xiao Lu, Melissa P. Sulprizio, Steven P. Hamburg, and Daniel J. Jacob
Atmos. Chem. Phys., 22, 11203–11215, https://doi.org/10.5194/acp-22-11203-2022, https://doi.org/10.5194/acp-22-11203-2022, 2022
Short summary
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We use 22 months of TROPOMI satellite observations to quantity methane emissions from the oil (O) and natural gas (G) sector in the US and Canada at the scale of both individual basins as well as country-wide aggregates. We find that O/G-related methane emissions are underestimated in these inventories by 80 % for the US and 40 % for Canada, and 70 % of the underestimate in the US is from five O/G basins, including Permian, Haynesville, Anadarko, Eagle Ford, and Barnett.
Daniel L. Goldberg, Monica Harkey, Benjamin de Foy, Laura Judd, Jeremiah Johnson, Greg Yarwood, and Tracey Holloway
Atmos. Chem. Phys., 22, 10875–10900, https://doi.org/10.5194/acp-22-10875-2022, https://doi.org/10.5194/acp-22-10875-2022, 2022
Short summary
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TROPOMI measurements offer a valuable means to validate emissions inventories and ozone formation regimes, with important limitations. Lightning NOx is important to account for in Texas and can contribute up to 24 % of the column NO2 in rural areas and 8 % in urban areas. Modeled NO2 in urban areas agrees with TROPOMI NO2 to within 20 % in most circumstances, with a small underestimate in Dallas (−13 %) and Houston (−20 %). Near Texas power plants, the satellite appears to underrepresent NO2.
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Short summary
A comprehensive case study of a comma-shaped bromine monoxide plume in the Arctic, which was transported by a polar cyclone and was observed by the GOME-2 satellite sensor over several days, is presented. By making combined use of different kinds of satellite data and numerical models, we demonstrate the important role of the frontal weather system in favouring the bromine activation cycle and blowing snow production, which may have acted as a bromine source during the bromine explosion event.
A comprehensive case study of a comma-shaped bromine monoxide plume in the Arctic, which was...
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