Articles | Volume 17, issue 1
https://doi.org/10.5194/acp-17-385-2017
https://doi.org/10.5194/acp-17-385-2017
Research article
 | 
10 Jan 2017
Research article |  | 10 Jan 2017

Direct oceanic emissions unlikely to account for the missing source of atmospheric carbonyl sulfide

Sinikka T. Lennartz, Christa A. Marandino, Marc von Hobe, Pau Cortes, Birgit Quack, Rafel Simo, Dennis Booge, Andrea Pozzer, Tobias Steinhoff, Damian L. Arevalo-Martinez, Corinna Kloss, Astrid Bracher, Rüdiger Röttgers, Elliot Atlas, and Kirstin Krüger

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Cited articles

Andreae, M. O. and Ferek, R.: Photochemical production of carbonyl sulfide in seawater and its emission to the atmosphere, Global Biogeochem. Cy., 6, 175–183, 2002.
Arévalo-Marténez, D. L., Beyer, M., Krumbholz, M., Piller, I., Kock, A., Steinhoff, T., Körtzinger, A., and Bange, H. W.: A new method for continuous measurements of oceanic and atmospheric N2O, CO and CO2: performance of off-axis integrated cavity output spectroscopy (OA-ICOS) coupled to non-dispersive infrared detection (NDIR), Ocean Sci., 9, 1071–1087, https://doi.org/10.5194/os-9-1071-2013, 2013.
Arsene, C., Barnes, I., Becker, K. H., and Mocanu, R.: FT-IR product study on the photo-oxidation of dimethyl sulphide in the presence of NOx – temperature dependence, Atmos. Environ., 35, 3769–3780, 2001.
Asaf, D., Rotenberg, E., Tatarinov, F., Dicken, U., Montzka, S. A., and Yakir, D.: Ecosystem photosynthesis inferred from measurements of carbonyl sulphide flux, Nat. Geosci., 6, 186–190, 2013.
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We present new sea surface and marine boundary layer measurements of carbonyl sulfide, the most abundant sulfur gas in the atmosphere, and calculate an oceanic emission estimate. Our results imply that oceanic emissions are very unlikely to account for the missing source in the atmospheric budget that is currently discussed for OCS.
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