Articles | Volume 17, issue 4
https://doi.org/10.5194/acp-17-2525-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-2525-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Technical note
| 
17 Feb 2017
Technical note |
| 17 Feb 2017
Technical note: Simultaneous fully dynamic characterization of multiple input–output relationships in climate models
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, WA, USA
Douglas G. MacMartin
Department of Computing and Mathematical Sciences, California Institute of Technology, Pasadena, CA, USA
Sibley School of Mechanical and Aerospace Engineering, Cornell University, Ithaca, NY, USA
Philip J. Rasch
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, WA, USA
Hailong Wang
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, WA, USA
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Daniele Visioni, Alan Robock, Jim Haywood, Matthew Henry, Simone Tilmes, Douglas G. MacMartin, Ben Kravitz, Sarah J. Doherty, John Moore, Chris Lennard, Shingo Watanabe, Helene Muri, Ulrike Niemeier, Olivier Boucher, Abu Syed, Temitope S. Egbebiyi, Roland Séférian, and Ilaria Quaglia
Geosci. Model Dev., 17, 2583–2596, https://doi.org/10.5194/gmd-17-2583-2024, https://doi.org/10.5194/gmd-17-2583-2024, 2024
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This paper describes a new experimental protocol for the Geoengineering Model Intercomparison Project (GeoMIP). In it, we describe the details of a new simulation of sunlight reflection using the stratospheric aerosols that climate models are supposed to run, and we explain the reasons behind each choice we made when defining the protocol.
Yan Zhang, Douglas G. MacMartin, Daniele Visioni, Ewa M. Bednarz, and Ben Kravitz
Earth Syst. Dynam., 15, 191–213, https://doi.org/10.5194/esd-15-191-2024, https://doi.org/10.5194/esd-15-191-2024, 2024
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Injecting SO2 into the lower stratosphere can temporarily reduce global mean temperature and mitigate some risks associated with climate change, but injecting it at different latitudes and seasons would have different impacts. This study introduces new stratospheric aerosol injection (SAI) strategies and explores the importance of the choice of SAI strategy, demonstrating that it notably affects the distribution of aerosol cloud, injection efficiency, and various surface climate impacts.
Ewa M. Bednarz, Amy H. Butler, Daniele Visioni, Yan Zhang, Ben Kravitz, and Douglas G. MacMartin
Atmos. Chem. Phys., 23, 13665–13684, https://doi.org/10.5194/acp-23-13665-2023, https://doi.org/10.5194/acp-23-13665-2023, 2023
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We use a state-of-the-art Earth system model and a set of stratospheric aerosol injection (SAI) strategies to achieve the same level of global mean surface cooling through different combinations of location and/or timing of the injection. We demonstrate that the choice of SAI strategy can lead to contrasting impacts on stratospheric and tropospheric temperatures, circulation, and chemistry (including stratospheric ozone), thereby leading to different impacts on regional surface climate.
Daniele Visioni, Ben Kravitz, Alan Robock, Simone Tilmes, Jim Haywood, Olivier Boucher, Mark Lawrence, Peter Irvine, Ulrike Niemeier, Lili Xia, Gabriel Chiodo, Chris Lennard, Shingo Watanabe, John C. Moore, and Helene Muri
Atmos. Chem. Phys., 23, 5149–5176, https://doi.org/10.5194/acp-23-5149-2023, https://doi.org/10.5194/acp-23-5149-2023, 2023
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Geoengineering indicates methods aiming to reduce the temperature of the planet by means of reflecting back a part of the incoming radiation before it reaches the surface or allowing more of the planetary radiation to escape into space. It aims to produce modelling experiments that are easy to reproduce and compare with different climate models, in order to understand the potential impacts of these techniques. Here we assess its past successes and failures and talk about its future.
Daniele Visioni, Ewa M. Bednarz, Walker R. Lee, Ben Kravitz, Andy Jones, Jim M. Haywood, and Douglas G. MacMartin
Atmos. Chem. Phys., 23, 663–685, https://doi.org/10.5194/acp-23-663-2023, https://doi.org/10.5194/acp-23-663-2023, 2023
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The paper constitutes Part 1 of a study performing a first systematic inter-model comparison of the atmospheric responses to stratospheric sulfate aerosol injections (SAIs) at various latitudes as simulated by three state-of-the-art Earth system models. We identify similarities and differences in the modeled aerosol burden, investigate the differences in the aerosol approaches between the models, and ultimately show the differences produced in surface climate, temperature and precipitation.
Ewa M. Bednarz, Daniele Visioni, Ben Kravitz, Andy Jones, James M. Haywood, Jadwiga Richter, Douglas G. MacMartin, and Peter Braesicke
Atmos. Chem. Phys., 23, 687–709, https://doi.org/10.5194/acp-23-687-2023, https://doi.org/10.5194/acp-23-687-2023, 2023
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Building on Part 1 of this two-part study, we demonstrate the role of biases in climatological circulation and specific aspects of model microphysics in driving the differences in simulated sulfate distributions amongst three Earth system models. We then characterize the simulated changes in stratospheric and free-tropospheric temperatures, ozone, water vapor, and large-scale circulation, elucidating the role of the above aspects in the surface responses discussed in Part 1.
Mari R. Tye, Katherine Dagon, Maria J. Molina, Jadwiga H. Richter, Daniele Visioni, Ben Kravitz, and Simone Tilmes
Earth Syst. Dynam., 13, 1233–1257, https://doi.org/10.5194/esd-13-1233-2022, https://doi.org/10.5194/esd-13-1233-2022, 2022
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We examined the potential effect of stratospheric aerosol injection (SAI) on extreme temperature and precipitation. SAI may cause daytime temperatures to cool but nighttime to warm. Daytime cooling may occur in all seasons across the globe, with the largest decreases in summer. In contrast, nighttime warming may be greatest at high latitudes in winter. SAI may reduce the frequency and intensity of extreme rainfall. The combined changes may exacerbate drying over parts of the global south.
Ilaria Quaglia, Daniele Visioni, Giovanni Pitari, and Ben Kravitz
Atmos. Chem. Phys., 22, 5757–5773, https://doi.org/10.5194/acp-22-5757-2022, https://doi.org/10.5194/acp-22-5757-2022, 2022
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Carbonyl sulfide is a gas that mixes very well in the atmosphere and can reach the stratosphere, where it reacts with sunlight and produces aerosol. Here we propose that, by increasing surface fluxes by an order of magnitude, the number of stratospheric aerosols produced may be enough to partially offset the warming produced by greenhouse gases. We explore what effect this would have on the atmospheric composition.
Huiying Ren, Erol Cromwell, Ben Kravitz, and Xingyuan Chen
Hydrol. Earth Syst. Sci., 26, 1727–1743, https://doi.org/10.5194/hess-26-1727-2022, https://doi.org/10.5194/hess-26-1727-2022, 2022
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We used a deep learning method called long short-term memory (LSTM) to fill gaps in data collected by hydrologic monitoring networks. LSTM accounted for correlations in space and time and nonlinear trends in data. Compared to a traditional regression-based time-series method, LSTM performed comparably when filling gaps in data with smooth patterns, while it better captured highly dynamic patterns in data. Capturing such dynamics is critical for understanding dynamic complex system behaviors.
Andy Jones, Jim M. Haywood, Adam A. Scaife, Olivier Boucher, Matthew Henry, Ben Kravitz, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Roland Séférian, Simone Tilmes, and Daniele Visioni
Atmos. Chem. Phys., 22, 2999–3016, https://doi.org/10.5194/acp-22-2999-2022, https://doi.org/10.5194/acp-22-2999-2022, 2022
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Simulations by six Earth-system models of geoengineering by introducing sulfuric acid aerosols into the tropical stratosphere are compared. A robust impact on the northern wintertime North Atlantic Oscillation is found, exacerbating precipitation reduction over parts of southern Europe. In contrast, the models show no consistency with regard to impacts on the Quasi-Biennial Oscillation, although results do indicate a risk that the oscillation could become locked into a permanent westerly phase.
Daniele Visioni, Simone Tilmes, Charles Bardeen, Michael Mills, Douglas G. MacMartin, Ben Kravitz, and Jadwiga H. Richter
Atmos. Chem. Phys., 22, 1739–1756, https://doi.org/10.5194/acp-22-1739-2022, https://doi.org/10.5194/acp-22-1739-2022, 2022
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Aerosols are simulated in a simplified way in climate models: in the model analyzed here, they are represented in every grid as described by three simple logarithmic distributions, mixing all different species together. The size can evolve when new particles are formed, particles merge together to create a larger one or particles are deposited to the surface. This approximation normally works fairly well. Here we show however that when large amounts of sulfate are simulated, there are problems.
Yan Zhang, Douglas G. MacMartin, Daniele Visioni, and Ben Kravitz
Earth Syst. Dynam., 13, 201–217, https://doi.org/10.5194/esd-13-201-2022, https://doi.org/10.5194/esd-13-201-2022, 2022
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Adding SO2 to the stratosphere could temporarily cool the planet by reflecting more sunlight back to space. However, adding SO2 at different latitude(s) and season(s) leads to significant differences in regional surface climate. This study shows that, to cool the planet by 1–1.5 °C, there are likely six to eight choices of injection latitude(s) and season(s) that lead to meaningfully different distributions of climate impacts.
Dawn L. Woodard, Alexey N. Shiklomanov, Ben Kravitz, Corinne Hartin, and Ben Bond-Lamberty
Geosci. Model Dev., 14, 4751–4767, https://doi.org/10.5194/gmd-14-4751-2021, https://doi.org/10.5194/gmd-14-4751-2021, 2021
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We have added a representation of the permafrost carbon feedback to the simple, open-source global carbon–climate model Hector and calibrated the results to be consistent with historical data and Earth system model projections. Our results closely match previous work, estimating around 0.2 °C of warming from permafrost this century. This capability will be useful to explore uncertainties in this feedback and for coupling with integrated assessment models for policy and economic analysis.
Daniele Visioni, Douglas G. MacMartin, Ben Kravitz, Olivier Boucher, Andy Jones, Thibaut Lurton, Michou Martine, Michael J. Mills, Pierre Nabat, Ulrike Niemeier, Roland Séférian, and Simone Tilmes
Atmos. Chem. Phys., 21, 10039–10063, https://doi.org/10.5194/acp-21-10039-2021, https://doi.org/10.5194/acp-21-10039-2021, 2021
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A new set of simulations is used to investigate commonalities, differences and sources of uncertainty when simulating the injection of SO2 in the stratosphere in order to mitigate the effects of climate change (solar geoengineering). The models differ in how they simulate the aerosols and how they spread around the stratosphere, resulting in differences in projected regional impacts. Overall, however, the models agree that aerosols have the potential to mitigate the warming produced by GHGs.
Nikolas O. Aksamit, Ben Kravitz, Douglas G. MacMartin, and George Haller
Atmos. Chem. Phys., 21, 8845–8861, https://doi.org/10.5194/acp-21-8845-2021, https://doi.org/10.5194/acp-21-8845-2021, 2021
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There exist robust and influential material features evolving within turbulent fluids that behave as the skeleton for fluid transport pathways. Recent developments in applied mathematics have made the identification of these time-varying structures more rigorous and insightful than ever. Using short-range wind forecasts, we detail how and why these material features can be exploited in an effort to optimize the spread of aerosols in the stratosphere for climate geoengineering.
Ben Kravitz, Douglas G. MacMartin, Daniele Visioni, Olivier Boucher, Jason N. S. Cole, Jim Haywood, Andy Jones, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Alan Robock, Roland Séférian, and Simone Tilmes
Atmos. Chem. Phys., 21, 4231–4247, https://doi.org/10.5194/acp-21-4231-2021, https://doi.org/10.5194/acp-21-4231-2021, 2021
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This study investigates multi-model response to idealized geoengineering (high CO2 with solar reduction) across two different generations of climate models. We find that, with the exception of a few cases, the results are unchanged between the different generations. This gives us confidence that broad conclusions about the response to idealized geoengineering are robust.
Andy Jones, Jim M. Haywood, Anthony C. Jones, Simone Tilmes, Ben Kravitz, and Alan Robock
Atmos. Chem. Phys., 21, 1287–1304, https://doi.org/10.5194/acp-21-1287-2021, https://doi.org/10.5194/acp-21-1287-2021, 2021
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Two different methods of simulating a geoengineering scenario are compared using data from two different Earth system models. One method is very idealised while the other includes details of a plausible mechanism. The results from both models agree that the idealised approach does not capture an impact found when detailed modelling is included, namely that geoengineering induces a positive phase of the North Atlantic Oscillation which leads to warmer, wetter winters in northern Europe.
Walker Lee, Douglas MacMartin, Daniele Visioni, and Ben Kravitz
Earth Syst. Dynam., 11, 1051–1072, https://doi.org/10.5194/esd-11-1051-2020, https://doi.org/10.5194/esd-11-1051-2020, 2020
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The injection of aerosols into the stratosphere to reflect sunlight could reduce global warming, but this type of
geoengineeringwould also impact other variables like precipitation and sea ice. In this study, we model various climate impacts of geoengineering on a 3-D graph to show how trying to meet one climate goal will affect other variables. We also present two computer simulations which validate our model and show that geoengineering could regulate precipitation as well as temperature.
Bethany Sutherland, Ben Kravitz, Philip J. Rasch, and Hailong Wang
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-228, https://doi.org/10.5194/gmd-2020-228, 2020
Preprint withdrawn
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Through a cascade of physical mechanisms, a change in one location can trigger a response in a different location. These responses and the mechanisms that cause them are difficult to detect. Here we propose a method, using global climate models, to detect possible relationships between changes in one region and responses throughout the globe caused by that change. A change in the Pacific ocean is used as a test case to determine the effectiveness of the method.
Simone Tilmes, Douglas G. MacMartin, Jan T. M. Lenaerts, Leo van Kampenhout, Laura Muntjewerf, Lili Xia, Cheryl S. Harrison, Kristen M. Krumhardt, Michael J. Mills, Ben Kravitz, and Alan Robock
Earth Syst. Dynam., 11, 579–601, https://doi.org/10.5194/esd-11-579-2020, https://doi.org/10.5194/esd-11-579-2020, 2020
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This paper introduces new geoengineering model experiments as part of a larger model intercomparison effort, using reflective particles to block some of the incoming solar radiation to reach surface temperature targets. Outcomes of these applications are contrasted based on a high greenhouse gas emission pathway and a pathway with strong mitigation and negative emissions after 2040. We compare quantities that matter for societal and ecosystem impacts between the different scenarios.
Theodore Weber, Austin Corotan, Brian Hutchinson, Ben Kravitz, and Robert Link
Atmos. Chem. Phys., 20, 2303–2317, https://doi.org/10.5194/acp-20-2303-2020, https://doi.org/10.5194/acp-20-2303-2020, 2020
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Climate model emulators can save computer time but are less accurate than full climate models. We use neural networks to build emulators of precipitation, trained on existing climate model runs. By doing so, we can capture nonlinearities and how the past state of a model (to some degree) shapes the future state. Our emulator outperforms a persistence forecast of precipitation.
Robert Link, Abigail Snyder, Cary Lynch, Corinne Hartin, Ben Kravitz, and Ben Bond-Lamberty
Geosci. Model Dev., 12, 1477–1489, https://doi.org/10.5194/gmd-12-1477-2019, https://doi.org/10.5194/gmd-12-1477-2019, 2019
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Earth system models (ESMs) produce the highest-quality future climate data available, but they are costly to run, so only a few runs from each model are publicly available. What is needed are emulators that tell us what would have happened, if we had been able to perform as many ESM runs as we might have liked. Much of the existing work on emulators has focused on deterministic projections of average values. Here we present a way to imbue emulators with the variability seen in ESM runs.
Christopher G. Fletcher, Ben Kravitz, and Bakr Badawy
Atmos. Chem. Phys., 18, 17529–17543, https://doi.org/10.5194/acp-18-17529-2018, https://doi.org/10.5194/acp-18-17529-2018, 2018
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The most important number for future climate projections is Earth's climate sensitivity (CS), or how much warming will result from increased carbon dioxide. We cannot know the true CS, and estimates of CS from climate models have a wide range. This study identifies the major factors that control this range, and we show that the choice of methods used in creating a climate model are three times more important than fine-tuning the details of the model after it is created.
Ben Kravitz, Philip J. Rasch, Hailong Wang, Alan Robock, Corey Gabriel, Olivier Boucher, Jason N. S. Cole, Jim Haywood, Duoying Ji, Andy Jones, Andrew Lenton, John C. Moore, Helene Muri, Ulrike Niemeier, Steven Phipps, Hauke Schmidt, Shingo Watanabe, Shuting Yang, and Jin-Ho Yoon
Atmos. Chem. Phys., 18, 13097–13113, https://doi.org/10.5194/acp-18-13097-2018, https://doi.org/10.5194/acp-18-13097-2018, 2018
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Marine cloud brightening has been proposed as a means of geoengineering/climate intervention, or deliberately altering the climate system to offset anthropogenic climate change. In idealized simulations that highlight contrasts between land and ocean, we find that the globe warms, including the ocean due to transport of heat from land. This study reinforces that no net energy input into the Earth system does not mean that temperature will necessarily remain unchanged.
Duoying Ji, Songsong Fang, Charles L. Curry, Hiroki Kashimura, Shingo Watanabe, Jason N. S. Cole, Andrew Lenton, Helene Muri, Ben Kravitz, and John C. Moore
Atmos. Chem. Phys., 18, 10133–10156, https://doi.org/10.5194/acp-18-10133-2018, https://doi.org/10.5194/acp-18-10133-2018, 2018
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We examine extreme temperature and precipitation under climate-model-simulated solar dimming and stratospheric aerosol injection geoengineering schemes. Both types of geoengineering lead to lower minimum temperatures at higher latitudes and greater cooling of minimum temperatures and maximum temperatures over land compared with oceans. Stratospheric aerosol injection is more effective in reducing tropical extreme precipitation, while solar dimming is more effective over extra-tropical regions.
David P. Keller, Andrew Lenton, Vivian Scott, Naomi E. Vaughan, Nico Bauer, Duoying Ji, Chris D. Jones, Ben Kravitz, Helene Muri, and Kirsten Zickfeld
Geosci. Model Dev., 11, 1133–1160, https://doi.org/10.5194/gmd-11-1133-2018, https://doi.org/10.5194/gmd-11-1133-2018, 2018
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There is little consensus on the impacts and efficacy of proposed carbon dioxide removal (CDR) methods as a potential means of mitigating climate change. To address this need, the Carbon Dioxide Removal Model Intercomparison Project (or CDR-MIP) has been initiated. This project brings together models of the Earth system in a common framework to explore the potential, impacts, and challenges of CDR. Here, we describe the first set of CDR-MIP experiments.
Camilla W. Stjern, Helene Muri, Lars Ahlm, Olivier Boucher, Jason N. S. Cole, Duoying Ji, Andy Jones, Jim Haywood, Ben Kravitz, Andrew Lenton, John C. Moore, Ulrike Niemeier, Steven J. Phipps, Hauke Schmidt, Shingo Watanabe, and Jón Egill Kristjánsson
Atmos. Chem. Phys., 18, 621–634, https://doi.org/10.5194/acp-18-621-2018, https://doi.org/10.5194/acp-18-621-2018, 2018
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Marine cloud brightening (MCB) has been proposed to help limit global warming. We present here the first multi-model assessment of idealized MCB simulations from the Geoengineering Model Intercomparison Project. While all models predict a global cooling as intended, there is considerable spread between the models both in terms of radiative forcing and the climate response, largely linked to the substantial differences in the models' representation of clouds.
Lars Ahlm, Andy Jones, Camilla W. Stjern, Helene Muri, Ben Kravitz, and Jón Egill Kristjánsson
Atmos. Chem. Phys., 17, 13071–13087, https://doi.org/10.5194/acp-17-13071-2017, https://doi.org/10.5194/acp-17-13071-2017, 2017
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We present results from coordinated simulations with three Earth system models focusing on the response of Earth’s radiation balance to the injection of sea salt particles. We find that in most regions the effective radiative forcing by the injected particles is equally large in cloudy and clear-sky conditions, suggesting a more important role of the aerosol direct effect in sea spray climate engineering than previously thought.
Cary Lynch, Corinne Hartin, Ben Bond-Lamberty, and Ben Kravitz
Earth Syst. Sci. Data, 9, 281–292, https://doi.org/10.5194/essd-9-281-2017, https://doi.org/10.5194/essd-9-281-2017, 2017
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Pattern scaling climate model output is a computationally efficient way to produce a large amount of data for purposes of uncertainty quantification. Using a multi-model ensemble we explore pattern scaling methodologies across two future forcing scenarios. We find that the simple least squares approach to pattern scaling produces a close approximation of actual model output, and we use this as a justification for the creation of an open-access pattern library at multiple time increments.
Ben Kravitz, Cary Lynch, Corinne Hartin, and Ben Bond-Lamberty
Geosci. Model Dev., 10, 1889–1902, https://doi.org/10.5194/gmd-10-1889-2017, https://doi.org/10.5194/gmd-10-1889-2017, 2017
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Pattern scaling is a way of approximating regional changes without needing to run a full, complex global climate model. We compare two methods of pattern scaling for precipitation and evaluate which methods is
betterin particular circumstances. We also decompose precipitation into a CO2 portion and a non-CO2 portion. The methodologies discussed in this paper can help provide precipitation fields for other models for a wide variety of scenarios of future climate change.
Hiroki Kashimura, Manabu Abe, Shingo Watanabe, Takashi Sekiya, Duoying Ji, John C. Moore, Jason N. S. Cole, and Ben Kravitz
Atmos. Chem. Phys., 17, 3339–3356, https://doi.org/10.5194/acp-17-3339-2017, https://doi.org/10.5194/acp-17-3339-2017, 2017
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This study analyses shortwave radiation (SW) in the G4 experiment of the Geoengineering Model Intercomparison Project. G4 involves stratospheric injection of 5 Tg yr−1 of SO2 against the RCP4.5 scenario. The global mean forcing of the sulphate geoengineering has an inter-model variablity of −3.6 to −1.6 W m−2, implying a high uncertainty in modelled processes of sulfate aerosols. Changes in water vapour and cloud amounts due to the SO2 injection weaken the forcing at the surface by around 50 %.
Corey J. Gabriel, Alan Robock, Lili Xia, Brian Zambri, and Ben Kravitz
Atmos. Chem. Phys., 17, 595–613, https://doi.org/10.5194/acp-17-595-2017, https://doi.org/10.5194/acp-17-595-2017, 2017
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The National Center for Atmospheric Research CESM-CAM4-CHEM global climate model was modified to simulate a scheme in which the albedo of the ocean surface is raised over the subtropical ocean gyres in the Southern Hemisphere. Global mean surface temperature in G4Foam is 0.6K lower than RCP6.0, with statistically significant cooling relative to RCP6.0 south of 30° N and an increase in rainfall over land, most pronouncedly during the JJA season, relative to both G4SSA and RCP6.0.
Douglas G. MacMartin and Ben Kravitz
Atmos. Chem. Phys., 16, 15789–15799, https://doi.org/10.5194/acp-16-15789-2016, https://doi.org/10.5194/acp-16-15789-2016, 2016
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Solar geoengineering has been proposed as a possible additional approach for managing risks of climate change, by reflecting some sunlight back to space. To project climate effects resulting from future choices regarding both greenhouse gas emissions and solar geoengineering, it is useful to have a computationally efficient "emulator" that approximates the behavior of more complex climate models. We present such an emulator here, and validate the underlying assumption of linearity.
Cary Lynch, Corinne Hartin, Ben Bond-Lamberty, and Ben Kravitz
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2016-170, https://doi.org/10.5194/gmd-2016-170, 2016
Revised manuscript not accepted
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Pattern scaling is used to explore uncertainty in future forcing scenarios and assess local climate sensitivity to global temperature change. This paper examines the two dominant pattern scaling methods using a multi-model ensemble with two future socio-economic storylines. We find that high latitudes show the strongest sensitivity to global temperature change and that the simple least squared regression approach to generation of patterns is a better fit to projected global temperature.
Ben Kravitz, Douglas G. MacMartin, Hailong Wang, and Philip J. Rasch
Earth Syst. Dynam., 7, 469–497, https://doi.org/10.5194/esd-7-469-2016, https://doi.org/10.5194/esd-7-469-2016, 2016
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Most simulations of solar geoengineering prescribe a particular strategy and evaluate its modeled effects. Here we first choose example climate objectives and then design a strategy to meet those objectives in climate models. We show that certain objectives can be met simultaneously even in the presence of uncertainty, and the strategy for meeting those objectives can be ported to other models. This is part of a broader illustration of how uncertainties in solar geoengineering can be managed.
B. Kravitz, A. Robock, S. Tilmes, O. Boucher, J. M. English, P. J. Irvine, A. Jones, M. G. Lawrence, M. MacCracken, H. Muri, J. C. Moore, U. Niemeier, S. J. Phipps, J. Sillmann, T. Storelvmo, H. Wang, and S. Watanabe
Geosci. Model Dev., 8, 3379–3392, https://doi.org/10.5194/gmd-8-3379-2015, https://doi.org/10.5194/gmd-8-3379-2015, 2015
S. Tilmes, M. J. Mills, U. Niemeier, H. Schmidt, A. Robock, B. Kravitz, J.-F. Lamarque, G. Pitari, and J. M. English
Geosci. Model Dev., 8, 43–49, https://doi.org/10.5194/gmd-8-43-2015, https://doi.org/10.5194/gmd-8-43-2015, 2015
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A new Geoengineering Model Intercomparison Project (GeoMIP) experiment “G4 specified stratospheric aerosols” (G4SSA) is proposed to investigate the impact of stratospheric aerosol geoengineering on atmosphere, chemistry, dynamics, climate, and the environment. In contrast to the earlier G4 GeoMIP experiment, which requires an emission of sulfur dioxide (SO2) into the model, a prescribed aerosol forcing file is provided to the community, to be consistently applied to future model experiments.
Weiming Ma, Hailong Wang, Gang Chen, Yun Qian, Ian Baxter, Yiling Huo, and Mark W. Seefeldt
Atmos. Chem. Phys., 24, 4451–4472, https://doi.org/10.5194/acp-24-4451-2024, https://doi.org/10.5194/acp-24-4451-2024, 2024
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Extreme warming events with surface temperature going above 0°C can occur in the high-Arctic winter. Although reanalysis data show that these events were short-lived and occurred rarely during 1980–2021, they have become more frequent, stronger, and longer lasting latterly. A dipole pattern, comprising high- and low-pressure systems, is found to be the key in driving them. These findings have implications for the recent changes in sea ice, hydrological cycle, and ecosystem over the Arctic.
Philip Rasch, Haruki Hirasawa, Mingxuan Wu, Sarah Doherty, Robert Wood, Hailong Wang, Andy Jones, James Haywood, and Hansi Singh
EGUsphere, https://doi.org/10.5194/egusphere-2024-1031, https://doi.org/10.5194/egusphere-2024-1031, 2024
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We introduce a protocol to compare computer climate simulations to better understand a proposed strategy intended to counter warming & climate impacts from greenhouse gas increases. The strategy slightly changes clouds in 6 ocean regions to reflect more sunlight & cool Earth. Example changes in clouds & climate are shown for 3 climate models. Clouds change differently between the models, but precipitation and surface temperature changes are similar when their cooling effects are made similar.
Daniele Visioni, Alan Robock, Jim Haywood, Matthew Henry, Simone Tilmes, Douglas G. MacMartin, Ben Kravitz, Sarah J. Doherty, John Moore, Chris Lennard, Shingo Watanabe, Helene Muri, Ulrike Niemeier, Olivier Boucher, Abu Syed, Temitope S. Egbebiyi, Roland Séférian, and Ilaria Quaglia
Geosci. Model Dev., 17, 2583–2596, https://doi.org/10.5194/gmd-17-2583-2024, https://doi.org/10.5194/gmd-17-2583-2024, 2024
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This paper describes a new experimental protocol for the Geoengineering Model Intercomparison Project (GeoMIP). In it, we describe the details of a new simulation of sunlight reflection using the stratospheric aerosols that climate models are supposed to run, and we explain the reasons behind each choice we made when defining the protocol.
Johannes Mülmenstädt, Andrew S. Ackerman, Ann M. Fridlind, Meng Huang, Po-Lun Ma, Naser Mahfouz, Susanne E. Bauer, Susannah M. Burrows, Matthew W. Christensen, Sudhakar Dipu, Andrew Gettelman, L. Ruby Leung, Florian Tornow, Johannes Quaas, Adam C. Varble, Hailong Wang, Kai Zhang, and Youtong Zheng
EGUsphere, https://doi.org/10.5194/egusphere-2024-778, https://doi.org/10.5194/egusphere-2024-778, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Stratocumulus clouds play a large role in Earth's climate by reflecting incoming solar energy back to space. Turbulence at stratocumulus cloud top mixes in drier, warmer air, which can lead to a reduction in cloud. This process is challenging for coarse-resolution global models to represent. We show that global models nevertheless agree well with our process understanding. Global models also think the process is less important for the climate than other lines of evidence had led us to conclude.
Yan Zhang, Douglas G. MacMartin, Daniele Visioni, Ewa M. Bednarz, and Ben Kravitz
Earth Syst. Dynam., 15, 191–213, https://doi.org/10.5194/esd-15-191-2024, https://doi.org/10.5194/esd-15-191-2024, 2024
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Injecting SO2 into the lower stratosphere can temporarily reduce global mean temperature and mitigate some risks associated with climate change, but injecting it at different latitudes and seasons would have different impacts. This study introduces new stratospheric aerosol injection (SAI) strategies and explores the importance of the choice of SAI strategy, demonstrating that it notably affects the distribution of aerosol cloud, injection efficiency, and various surface climate impacts.
Yawen Liu, Yun Qian, Philip J. Rasch, Kai Zhang, Lai-yung Ruby Leung, Yuhang Wang, Minghuai Wang, Hailong Wang, Xin Huang, and Xiu-Qun Yang
Atmos. Chem. Phys., 24, 3115–3128, https://doi.org/10.5194/acp-24-3115-2024, https://doi.org/10.5194/acp-24-3115-2024, 2024
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Fire management has long been a challenge. Here we report that spring-peak fire activity over southern Mexico and Central America (SMCA) has a distinct quasi-biennial signal by measuring multiple fire metrics. This signal is initially driven by quasi-biennial variability in precipitation and is further amplified by positive feedback of fire–precipitation interaction at short timescales. This work highlights the importance of fire–climate interactions in shaping fires on an interannual scale.
Chen Zhang, John J. Cassano, Mark Seefeldt, Hailong Wang, Weiming Ma, and Wen-wen Tung
EGUsphere, https://doi.org/10.5194/egusphere-2024-320, https://doi.org/10.5194/egusphere-2024-320, 2024
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An atmospheric river (AR) is a long, narrow corridor of moisture transport in the atmosphere. ARs are crucial for moisture and heat transport into the polar regions. Our study examines the role of ARs on the surface energy budget (SEB) in the Arctic. The results reveal distinct seasonality and land-sea-sea ice contrasts due to the impacts of ARs on the SEB. The conclusions provide greater insights into the current and future role of ARs on the Arctic climate system.
Hui Wan, Kai Zhang, Christopher J. Vogl, Carol S. Woodward, Richard C. Easter, Philip J. Rasch, Yan Feng, and Hailong Wang
Geosci. Model Dev., 17, 1387–1407, https://doi.org/10.5194/gmd-17-1387-2024, https://doi.org/10.5194/gmd-17-1387-2024, 2024
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Sophisticated numerical models of the Earth's atmosphere include representations of many physical and chemical processes. In numerical simulations, these processes need to be calculated in a certain sequence. This study reveals the weaknesses of the sequence of calculations used for aerosol processes in a global atmosphere model. A revision of the sequence is proposed and its impacts on the simulated global aerosol climatology are evaluated.
Huisheng Bian, Mian Chin, Peter R. Colarco, Eric C. Apel, Donald R. Blake, Karl Froyd, Rebecca S. Hornbrook, Jose Jimenez, Pedro Campuzano Jost, Michael Lawler, Mingxu Liu, Marianne Tronstad Lund, Hitoshi Matsui, Benjamin A. Nault, Joyce E. Penner, Andrew W. Rollins, Gregory Schill, Ragnhild B. Skeie, Hailong Wang, Lu Xu, Kai Zhang, and Jialei Zhu
Atmos. Chem. Phys., 24, 1717–1741, https://doi.org/10.5194/acp-24-1717-2024, https://doi.org/10.5194/acp-24-1717-2024, 2024
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This work studies sulfur in the remote troposphere at global and seasonal scales using aircraft measurements and multi-model simulations. The goal is to understand the sulfur cycle over remote oceans, spread of model simulations, and observation–model discrepancies. Such an understanding and comparison with real observations are crucial to narrow down the uncertainties in model sulfur simulations and improve understanding of the sulfur cycle in atmospheric air quality, climate, and ecosystems.
Yang Yang, Yang Zhou, Hailong Wang, Mengyun Li, Huimin Li, Pinya Wang, Xu Yue, Ke Li, Jia Zhu, and Hong Liao
Atmos. Chem. Phys., 24, 1177–1191, https://doi.org/10.5194/acp-24-1177-2024, https://doi.org/10.5194/acp-24-1177-2024, 2024
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This study reveals that extreme ozone pollution over the North China Plain and Yangtze River Delta is due to the chemical production related to hot and dry conditions, and the regional transport explains the ozone pollution over the Sichuan Basin and Pearl River Delta. The frequency of meteorological conditions of the extreme ozone pollution increases from the past to the future. The sustainable scenario is the optimal path to retaining clean air in China in the future.
Johannes Mülmenstädt, Edward Gryspeerdt, Sudhakar Dipu, Johannes Quaas, Andrew S. Ackerman, Ann M. Fridlind, Florian Tornow, Susanne E. Bauer, Andrew Gettelman, Yi Ming, Youtong Zheng, Po-Lun Ma, Hailong Wang, Kai Zhang, Matthew W. Christensen, Adam C. Varble, L. Ruby Leung, Xiaohong Liu, David Neubauer, Daniel G. Partridge, Philip Stier, and Toshihiko Takemura
EGUsphere, https://doi.org/10.5194/egusphere-2024-4, https://doi.org/10.5194/egusphere-2024-4, 2024
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Human activities release copious amounts of small particles, called aerosols, into the atmosphere. These particles change how much sunlight clouds reflect to space, an important human perturbation of the climate whose magnitude is highly uncertain. We found that the latest climate models show a negative correlation but a positive causal relationship between aerosols and cloud water. This means we need to be very careful when we interpret observational studies that can only see correlation.
Yang Yang, Shaoxuan Mou, Hailong Wang, Pinya Wang, Baojie Li, and Hong Liao
EGUsphere, https://doi.org/10.5194/egusphere-2023-2552, https://doi.org/10.5194/egusphere-2023-2552, 2024
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We quantify the variations in anthropogenic aerosol concentrations, source contributions, and their subsequent radiative impact in four major emission regions during four historical period. Due to industrial development and the implementation of different economic policies, sources of anthropogenic aerosols show different variations, which has important implications for the pollution prevention/control measures and decision making for global collaboration.
Shuaiqi Tang, Hailong Wang, Xiang-Yu Li, Jingyi Chen, Armin Sorooshian, Xubin Zeng, Ewan Crosbie, Kenneth L. Thornhill, Luke D. Ziemba, and Christiane Voigt
EGUsphere, https://doi.org/10.5194/egusphere-2023-3149, https://doi.org/10.5194/egusphere-2023-3149, 2024
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We examined marine boundary-layer clouds and their interactions with aerosols in the E3SM single-column model (SCM) for a case study. The SCM shows good agreement in simulating the clouds with high-resolution models. It reproduces the relationship between cloud droplet and aerosol particle number concentrations as produced in global models. However, the relationship between cloud liquid water and droplet number concentration are different, which warrants further investigation.
Hamza Ahsan, Hailong Wang, Jingbo Wu, Mingxuan Wu, Steven J. Smith, Susanne Bauer, Harrison Suchyta, Dirk Olivié, Gunnar Myhre, Hitoshi Matsui, Huisheng Bian, Jean-François Lamarque, Ken Carslaw, Larry Horowitz, Leighton Regayre, Mian Chin, Michael Schulz, Ragnhild Bieltvedt Skeie, Toshihiko Takemura, and Vaishali Naik
Atmos. Chem. Phys., 23, 14779–14799, https://doi.org/10.5194/acp-23-14779-2023, https://doi.org/10.5194/acp-23-14779-2023, 2023
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We examine the impact of the assumed effective height of SO2 injection, SO2 and BC emission seasonality, and the assumed fraction of SO2 emissions injected as SO4 on climate and chemistry model results. We find that the SO2 injection height has a large impact on surface SO2 concentrations and, in some models, radiative flux. These assumptions are a
hiddensource of inter-model variability and may be leading to bias in some climate model results.
Ewa M. Bednarz, Amy H. Butler, Daniele Visioni, Yan Zhang, Ben Kravitz, and Douglas G. MacMartin
Atmos. Chem. Phys., 23, 13665–13684, https://doi.org/10.5194/acp-23-13665-2023, https://doi.org/10.5194/acp-23-13665-2023, 2023
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We use a state-of-the-art Earth system model and a set of stratospheric aerosol injection (SAI) strategies to achieve the same level of global mean surface cooling through different combinations of location and/or timing of the injection. We demonstrate that the choice of SAI strategy can lead to contrasting impacts on stratospheric and tropospheric temperatures, circulation, and chemistry (including stratospheric ozone), thereby leading to different impacts on regional surface climate.
Matthew Henry, Jim Haywood, Andy Jones, Mohit Dalvi, Alice Wells, Daniele Visioni, Ewa M. Bednarz, Douglas G. MacMartin, Walker Lee, and Mari R. Tye
Atmos. Chem. Phys., 23, 13369–13385, https://doi.org/10.5194/acp-23-13369-2023, https://doi.org/10.5194/acp-23-13369-2023, 2023
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Solar climate interventions, such as injecting sulfur in the stratosphere, may be used to offset some of the adverse impacts of global warming. We use two independently developed Earth system models to assess the uncertainties around stratospheric sulfur injections. The injection locations and amounts are optimized to maintain the same pattern of surface temperature. While both models show reduced warming, the change in rainfall patterns (even without sulfur injections) is uncertain.
Armin Sorooshian, Mikhail D. Alexandrov, Adam D. Bell, Ryan Bennett, Grace Betito, Sharon P. Burton, Megan E. Buzanowicz, Brian Cairns, Eduard V. Chemyakin, Gao Chen, Yonghoon Choi, Brian L. Collister, Anthony L. Cook, Andrea F. Corral, Ewan C. Crosbie, Bastiaan van Diedenhoven, Joshua P. DiGangi, Glenn S. Diskin, Sanja Dmitrovic, Eva-Lou Edwards, Marta A. Fenn, Richard A. Ferrare, David van Gilst, Johnathan W. Hair, David B. Harper, Miguel Ricardo A. Hilario, Chris A. Hostetler, Nathan Jester, Michael Jones, Simon Kirschler, Mary M. Kleb, John M. Kusterer, Sean Leavor, Joseph W. Lee, Hongyu Liu, Kayla McCauley, Richard H. Moore, Joseph Nied, Anthony Notari, John B. Nowak, David Painemal, Kasey E. Phillips, Claire E. Robinson, Amy Jo Scarino, Joseph S. Schlosser, Shane T. Seaman, Chellappan Seethala, Taylor J. Shingler, Michael A. Shook, Kenneth A. Sinclair, William L. Smith Jr., Douglas A. Spangenberg, Snorre A. Stamnes, Kenneth L. Thornhill, Christiane Voigt, Holger Vömel, Andrzej P. Wasilewski, Hailong Wang, Edward L. Winstead, Kira Zeider, Xubin Zeng, Bo Zhang, Luke D. Ziemba, and Paquita Zuidema
Earth Syst. Sci. Data, 15, 3419–3472, https://doi.org/10.5194/essd-15-3419-2023, https://doi.org/10.5194/essd-15-3419-2023, 2023
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The NASA Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) produced a unique dataset for research into aerosol–cloud–meteorology interactions. HU-25 Falcon and King Air aircraft conducted systematic and spatially coordinated flights over the northwest Atlantic Ocean. This paper describes the ACTIVATE flight strategy, instrument and complementary dataset products, data access and usage details, and data application notes.
Qi Tang, Jean-Christophe Golaz, Luke P. Van Roekel, Mark A. Taylor, Wuyin Lin, Benjamin R. Hillman, Paul A. Ullrich, Andrew M. Bradley, Oksana Guba, Jonathan D. Wolfe, Tian Zhou, Kai Zhang, Xue Zheng, Yunyan Zhang, Meng Zhang, Mingxuan Wu, Hailong Wang, Cheng Tao, Balwinder Singh, Alan M. Rhoades, Yi Qin, Hong-Yi Li, Yan Feng, Yuying Zhang, Chengzhu Zhang, Charles S. Zender, Shaocheng Xie, Erika L. Roesler, Andrew F. Roberts, Azamat Mametjanov, Mathew E. Maltrud, Noel D. Keen, Robert L. Jacob, Christiane Jablonowski, Owen K. Hughes, Ryan M. Forsyth, Alan V. Di Vittorio, Peter M. Caldwell, Gautam Bisht, Renata B. McCoy, L. Ruby Leung, and David C. Bader
Geosci. Model Dev., 16, 3953–3995, https://doi.org/10.5194/gmd-16-3953-2023, https://doi.org/10.5194/gmd-16-3953-2023, 2023
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High-resolution simulations are superior to low-resolution ones in capturing regional climate changes and climate extremes. However, uniformly reducing the grid size of a global Earth system model is too computationally expensive. We provide an overview of the fully coupled regionally refined model (RRM) of E3SMv2 and document a first-of-its-kind set of climate production simulations using RRM at an economic cost. The key to this success is our innovative hybrid time step method.
Taufiq Hassan, Kai Zhang, Jianfeng Li, Balwinder Singh, Shixuan Zhang, Hailong Wang, and Po-Lun Ma
EGUsphere, https://doi.org/10.5194/egusphere-2023-1055, https://doi.org/10.5194/egusphere-2023-1055, 2023
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Anthropogenic aerosol emissions are essential part of the global aerosol models. Significant errors can exist from the loss of emission heterogeneity. We introduced an emission treatment that significantly improved aerosol emission heterogeneity in high-resolution model simulations, with improvements in simulated aerosol surface concentrations. The emission treatment will provide a more accurate representation of aerosol emissions and their effects on climate.
Aishwarya Raman, Thomas Hill, Paul J. DeMott, Balwinder Singh, Kai Zhang, Po-Lun Ma, Mingxuan Wu, Hailong Wang, Simon P. Alexander, and Susannah M. Burrows
Atmos. Chem. Phys., 23, 5735–5762, https://doi.org/10.5194/acp-23-5735-2023, https://doi.org/10.5194/acp-23-5735-2023, 2023
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Ice-nucleating particles (INPs) play an important role in cloud processes and associated precipitation. Yet, INPs are not accurately represented in climate models. This study attempts to uncover these gaps by comparing model-simulated INP concentrations against field campaign measurements in the SO for an entire year, 2017–2018. Differences in INP concentrations and variability between the model and observations have major implications for modeling cloud properties in high latitudes.
Pengwei Li, Yang Yang, Hailong Wang, Su Li, Ke Li, Pinya Wang, Baojie Li, and Hong Liao
Atmos. Chem. Phys., 23, 5403–5417, https://doi.org/10.5194/acp-23-5403-2023, https://doi.org/10.5194/acp-23-5403-2023, 2023
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We use a novel technique that can attribute O3 to precursors to investigate O3 changes in the United States during 1995–2019. We found that the US domestic energy and surface transportation emission reductions are primarily responsible for the O3 decrease in summer. In winter, factors such as nitrogen oxide emission reduction in the context of its inhibition of ozone production, increased aviation and shipping activities, and large-scale circulation changes contribute to the O3 increases.
Daniele Visioni, Ben Kravitz, Alan Robock, Simone Tilmes, Jim Haywood, Olivier Boucher, Mark Lawrence, Peter Irvine, Ulrike Niemeier, Lili Xia, Gabriel Chiodo, Chris Lennard, Shingo Watanabe, John C. Moore, and Helene Muri
Atmos. Chem. Phys., 23, 5149–5176, https://doi.org/10.5194/acp-23-5149-2023, https://doi.org/10.5194/acp-23-5149-2023, 2023
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Geoengineering indicates methods aiming to reduce the temperature of the planet by means of reflecting back a part of the incoming radiation before it reaches the surface or allowing more of the planetary radiation to escape into space. It aims to produce modelling experiments that are easy to reproduce and compare with different climate models, in order to understand the potential impacts of these techniques. Here we assess its past successes and failures and talk about its future.
Mengyun Li, Yang Yang, Hailong Wang, Huimin Li, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 23, 1533–1544, https://doi.org/10.5194/acp-23-1533-2023, https://doi.org/10.5194/acp-23-1533-2023, 2023
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Using the GEOS-Chem model, the impact of the quasi-biennial oscillation (QBO) on summertime tropospheric O3 in China is investigated. In the warm phases of sea surface temperature anomalies over the eastern tropical Pacific, the QBO has a significant positive correlation with near-surface O3 concentrations over central China. The QBO impacts on O3 pollution in China are mainly a result of changing vertical transport of O3.
Huimin Li, Yang Yang, Jianbing Jin, Hailong Wang, Ke Li, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 23, 1131–1145, https://doi.org/10.5194/acp-23-1131-2023, https://doi.org/10.5194/acp-23-1131-2023, 2023
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Future climate change will aggravate ozone pollution in Asia, especially in high-forcing scenarios. Ozone pollution in China will expand from North China to South China and extend into the cold season in a warmer future. The emphasis of this work is to quantify the impacts of future climate change on O3 pollution in Asia, which is of great significance for future O3 pollution mitigation strategies.
Younjoo J. Lee, Wieslaw Maslowski, John J. Cassano, Jaclyn Clement Kinney, Anthony P. Craig, Samy Kamal, Robert Osinski, Mark W. Seefeldt, Julienne Stroeve, and Hailong Wang
The Cryosphere, 17, 233–253, https://doi.org/10.5194/tc-17-233-2023, https://doi.org/10.5194/tc-17-233-2023, 2023
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During 1979–2020, four winter polynyas occurred in December 1986 and February 2011, 2017, and 2018 north of Greenland. Instead of ice melting due to the anomalous warm air intrusion, the extreme wind forcing resulted in greater ice transport offshore. Based on the two ensemble runs, representing a 1980s thicker ice vs. a 2010s thinner ice, a dominant cause of these winter polynyas stems from internal variability of atmospheric forcing rather than from the forced response to a warming climate.
Daniele Visioni, Ewa M. Bednarz, Walker R. Lee, Ben Kravitz, Andy Jones, Jim M. Haywood, and Douglas G. MacMartin
Atmos. Chem. Phys., 23, 663–685, https://doi.org/10.5194/acp-23-663-2023, https://doi.org/10.5194/acp-23-663-2023, 2023
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The paper constitutes Part 1 of a study performing a first systematic inter-model comparison of the atmospheric responses to stratospheric sulfate aerosol injections (SAIs) at various latitudes as simulated by three state-of-the-art Earth system models. We identify similarities and differences in the modeled aerosol burden, investigate the differences in the aerosol approaches between the models, and ultimately show the differences produced in surface climate, temperature and precipitation.
Ewa M. Bednarz, Daniele Visioni, Ben Kravitz, Andy Jones, James M. Haywood, Jadwiga Richter, Douglas G. MacMartin, and Peter Braesicke
Atmos. Chem. Phys., 23, 687–709, https://doi.org/10.5194/acp-23-687-2023, https://doi.org/10.5194/acp-23-687-2023, 2023
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Building on Part 1 of this two-part study, we demonstrate the role of biases in climatological circulation and specific aspects of model microphysics in driving the differences in simulated sulfate distributions amongst three Earth system models. We then characterize the simulated changes in stratospheric and free-tropospheric temperatures, ozone, water vapor, and large-scale circulation, elucidating the role of the above aspects in the surface responses discussed in Part 1.
Dalei Hao, Gautam Bisht, Karl Rittger, Edward Bair, Cenlin He, Huilin Huang, Cheng Dang, Timbo Stillinger, Yu Gu, Hailong Wang, Yun Qian, and L. Ruby Leung
Geosci. Model Dev., 16, 75–94, https://doi.org/10.5194/gmd-16-75-2023, https://doi.org/10.5194/gmd-16-75-2023, 2023
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Snow with the highest albedo of land surface plays a vital role in Earth’s surface energy budget and water cycle. This study accounts for the impacts of snow grain shape and mixing state of light-absorbing particles with snow on snow albedo in the E3SM land model. The findings advance our understanding of the role of snow grain shape and mixing state of LAP–snow in land surface processes and offer guidance for improving snow simulations and radiative forcing estimates in Earth system models.
Jadwiga H. Richter, Daniele Visioni, Douglas G. MacMartin, David A. Bailey, Nan Rosenbloom, Brian Dobbins, Walker R. Lee, Mari Tye, and Jean-Francois Lamarque
Geosci. Model Dev., 15, 8221–8243, https://doi.org/10.5194/gmd-15-8221-2022, https://doi.org/10.5194/gmd-15-8221-2022, 2022
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Solar climate intervention using stratospheric aerosol injection is a proposed method of reducing global mean temperatures to reduce the worst consequences of climate change. We present a new modeling protocol aimed at simulating a plausible deployment of stratospheric aerosol injection and reproducibility of simulations using other Earth system models: Assessing Responses and Impacts of Solar climate intervention on the Earth system with stratospheric aerosol injection (ARISE-SAI).
Yang Yang, Liangying Zeng, Hailong Wang, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 22, 14489–14502, https://doi.org/10.5194/acp-22-14489-2022, https://doi.org/10.5194/acp-22-14489-2022, 2022
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Using an aerosol–climate model, dust pollution in China affected by different spatial and temporal types of El Niño are examined. Both eastern and central Pacific El Niño and short-duration El Niño increase winter dust concentrations over northern China, while long-duration El Niño decreases concentrations. Only long-duration El Niño events can significantly affect dust over China in the following spring. This study has profound implications for air pollution control and dust storm prediction.
Mari R. Tye, Katherine Dagon, Maria J. Molina, Jadwiga H. Richter, Daniele Visioni, Ben Kravitz, and Simone Tilmes
Earth Syst. Dynam., 13, 1233–1257, https://doi.org/10.5194/esd-13-1233-2022, https://doi.org/10.5194/esd-13-1233-2022, 2022
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We examined the potential effect of stratospheric aerosol injection (SAI) on extreme temperature and precipitation. SAI may cause daytime temperatures to cool but nighttime to warm. Daytime cooling may occur in all seasons across the globe, with the largest decreases in summer. In contrast, nighttime warming may be greatest at high latitudes in winter. SAI may reduce the frequency and intensity of extreme rainfall. The combined changes may exacerbate drying over parts of the global south.
Kai Zhang, Wentao Zhang, Hui Wan, Philip J. Rasch, Steven J. Ghan, Richard C. Easter, Xiangjun Shi, Yong Wang, Hailong Wang, Po-Lun Ma, Shixuan Zhang, Jian Sun, Susannah M. Burrows, Manish Shrivastava, Balwinder Singh, Yun Qian, Xiaohong Liu, Jean-Christophe Golaz, Qi Tang, Xue Zheng, Shaocheng Xie, Wuyin Lin, Yan Feng, Minghuai Wang, Jin-Ho Yoon, and L. Ruby Leung
Atmos. Chem. Phys., 22, 9129–9160, https://doi.org/10.5194/acp-22-9129-2022, https://doi.org/10.5194/acp-22-9129-2022, 2022
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Here we analyze the effective aerosol forcing simulated by E3SM version 1 using both century-long free-running and short nudged simulations. The aerosol forcing in E3SMv1 is relatively large compared to other models, mainly due to the large indirect aerosol effect. Aerosol-induced changes in liquid and ice cloud properties in E3SMv1 have a strong correlation. The aerosol forcing estimates in E3SMv1 are sensitive to the parameterization changes in both liquid and ice cloud processes.
Jiyuan Gao, Yang Yang, Hailong Wang, Pinya Wang, Huimin Li, Mengyun Li, Lili Ren, Xu Yue, and Hong Liao
Atmos. Chem. Phys., 22, 7131–7142, https://doi.org/10.5194/acp-22-7131-2022, https://doi.org/10.5194/acp-22-7131-2022, 2022
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China has been implementing a sequence of policies for clean air since the year 2013. The aerosol decline produced a 0.09 ± 0.10°C warming during 2013–2017 estimated in this study, and the increase in ozone in the lower troposphere during this time period accelerated the warming, leading to a total 0.16 ± 0.15°C temperature increase in eastern China. Residential emission reductions led to a cooling effect because of a substantial decrease in light-absorbing aerosols.
Xue Zheng, Qing Li, Tian Zhou, Qi Tang, Luke P. Van Roekel, Jean-Christophe Golaz, Hailong Wang, and Philip Cameron-Smith
Geosci. Model Dev., 15, 3941–3967, https://doi.org/10.5194/gmd-15-3941-2022, https://doi.org/10.5194/gmd-15-3941-2022, 2022
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We document the model experiments for the future climate projection by E3SMv1.0. At the highest future emission scenario, E3SMv1.0 projects a strong surface warming with rapid changes in the atmosphere, ocean, sea ice, and land runoff. Specifically, we detect a significant polar amplification and accelerated warming linked to the unmasking of the aerosol effects. The impact of greenhouse gas forcing is examined in different climate components.
Ilaria Quaglia, Daniele Visioni, Giovanni Pitari, and Ben Kravitz
Atmos. Chem. Phys., 22, 5757–5773, https://doi.org/10.5194/acp-22-5757-2022, https://doi.org/10.5194/acp-22-5757-2022, 2022
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Carbonyl sulfide is a gas that mixes very well in the atmosphere and can reach the stratosphere, where it reacts with sunlight and produces aerosol. Here we propose that, by increasing surface fluxes by an order of magnitude, the number of stratospheric aerosols produced may be enough to partially offset the warming produced by greenhouse gases. We explore what effect this would have on the atmospheric composition.
Susannah M. Burrows, Richard C. Easter, Xiaohong Liu, Po-Lun Ma, Hailong Wang, Scott M. Elliott, Balwinder Singh, Kai Zhang, and Philip J. Rasch
Atmos. Chem. Phys., 22, 5223–5251, https://doi.org/10.5194/acp-22-5223-2022, https://doi.org/10.5194/acp-22-5223-2022, 2022
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Sea spray particles are composed of a mixture of salts and organic substances from oceanic microorganisms. In prior work, our team developed an approach connecting sea spray chemistry to ocean biology, called OCEANFILMS. Here we describe its implementation within an Earth system model, E3SM. We show that simulated sea spray chemistry is consistent with observed seasonal cycles and that sunlight reflected by simulated Southern Ocean clouds increases, consistent with analysis of satellite data.
Po-Lun Ma, Bryce E. Harrop, Vincent E. Larson, Richard B. Neale, Andrew Gettelman, Hugh Morrison, Hailong Wang, Kai Zhang, Stephen A. Klein, Mark D. Zelinka, Yuying Zhang, Yun Qian, Jin-Ho Yoon, Christopher R. Jones, Meng Huang, Sheng-Lun Tai, Balwinder Singh, Peter A. Bogenschutz, Xue Zheng, Wuyin Lin, Johannes Quaas, Hélène Chepfer, Michael A. Brunke, Xubin Zeng, Johannes Mülmenstädt, Samson Hagos, Zhibo Zhang, Hua Song, Xiaohong Liu, Michael S. Pritchard, Hui Wan, Jingyu Wang, Qi Tang, Peter M. Caldwell, Jiwen Fan, Larry K. Berg, Jerome D. Fast, Mark A. Taylor, Jean-Christophe Golaz, Shaocheng Xie, Philip J. Rasch, and L. Ruby Leung
Geosci. Model Dev., 15, 2881–2916, https://doi.org/10.5194/gmd-15-2881-2022, https://doi.org/10.5194/gmd-15-2881-2022, 2022
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An alternative set of parameters for E3SM Atmospheric Model version 1 has been developed based on a tuning strategy that focuses on clouds. When clouds in every regime are improved, other aspects of the model are also improved, even though they are not the direct targets for calibration. The recalibrated model shows a lower sensitivity to anthropogenic aerosols and surface warming, suggesting potential improvements to the simulated climate in the past and future.
Huiying Ren, Erol Cromwell, Ben Kravitz, and Xingyuan Chen
Hydrol. Earth Syst. Sci., 26, 1727–1743, https://doi.org/10.5194/hess-26-1727-2022, https://doi.org/10.5194/hess-26-1727-2022, 2022
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We used a deep learning method called long short-term memory (LSTM) to fill gaps in data collected by hydrologic monitoring networks. LSTM accounted for correlations in space and time and nonlinear trends in data. Compared to a traditional regression-based time-series method, LSTM performed comparably when filling gaps in data with smooth patterns, while it better captured highly dynamic patterns in data. Capturing such dynamics is critical for understanding dynamic complex system behaviors.
Andy Jones, Jim M. Haywood, Adam A. Scaife, Olivier Boucher, Matthew Henry, Ben Kravitz, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Roland Séférian, Simone Tilmes, and Daniele Visioni
Atmos. Chem. Phys., 22, 2999–3016, https://doi.org/10.5194/acp-22-2999-2022, https://doi.org/10.5194/acp-22-2999-2022, 2022
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Simulations by six Earth-system models of geoengineering by introducing sulfuric acid aerosols into the tropical stratosphere are compared. A robust impact on the northern wintertime North Atlantic Oscillation is found, exacerbating precipitation reduction over parts of southern Europe. In contrast, the models show no consistency with regard to impacts on the Quasi-Biennial Oscillation, although results do indicate a risk that the oscillation could become locked into a permanent westerly phase.
Daniele Visioni, Simone Tilmes, Charles Bardeen, Michael Mills, Douglas G. MacMartin, Ben Kravitz, and Jadwiga H. Richter
Atmos. Chem. Phys., 22, 1739–1756, https://doi.org/10.5194/acp-22-1739-2022, https://doi.org/10.5194/acp-22-1739-2022, 2022
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Aerosols are simulated in a simplified way in climate models: in the model analyzed here, they are represented in every grid as described by three simple logarithmic distributions, mixing all different species together. The size can evolve when new particles are formed, particles merge together to create a larger one or particles are deposited to the surface. This approximation normally works fairly well. Here we show however that when large amounts of sulfate are simulated, there are problems.
Yan Zhang, Douglas G. MacMartin, Daniele Visioni, and Ben Kravitz
Earth Syst. Dynam., 13, 201–217, https://doi.org/10.5194/esd-13-201-2022, https://doi.org/10.5194/esd-13-201-2022, 2022
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Adding SO2 to the stratosphere could temporarily cool the planet by reflecting more sunlight back to space. However, adding SO2 at different latitude(s) and season(s) leads to significant differences in regional surface climate. This study shows that, to cool the planet by 1–1.5 °C, there are likely six to eight choices of injection latitude(s) and season(s) that lead to meaningfully different distributions of climate impacts.
Hossein Dadashazar, Majid Alipanah, Miguel Ricardo A. Hilario, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Andrew J. Peters, Amy Jo Scarino, Michael Shook, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Bo Zhang, Luke Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 21, 16121–16141, https://doi.org/10.5194/acp-21-16121-2021, https://doi.org/10.5194/acp-21-16121-2021, 2021
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This study investigates precipitation impacts on long-range transport of North American outflow over the western North Atlantic Ocean (WNAO). Results demonstrate that precipitation scavenging plays a significant role in modifying surface aerosol concentrations over the WNAO, especially in winter and spring due to large-scale scavenging processes. This study highlights how precipitation impacts surface aerosol properties with relevance for other marine regions vulnerable to continental outflow.
Lili Ren, Yang Yang, Hailong Wang, Pinya Wang, Lei Chen, Jia Zhu, and Hong Liao
Atmos. Chem. Phys., 21, 15431–15445, https://doi.org/10.5194/acp-21-15431-2021, https://doi.org/10.5194/acp-21-15431-2021, 2021
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Due to the COVID-19 pandemic, human activities were strictly restricted in China. Even though anthropogenic aerosol emissions largely decreased, haze events still occurred. Our results shows that PM2.5 over the North China Plain is largely contributed by local sources. For other regions in China, PM2.5 is largely contributed from nonlocal sources. As emission reduction is a future goal, aerosol long-range transport and unfavorable meteorology are increasingly important to air quality.
Dawn L. Woodard, Alexey N. Shiklomanov, Ben Kravitz, Corinne Hartin, and Ben Bond-Lamberty
Geosci. Model Dev., 14, 4751–4767, https://doi.org/10.5194/gmd-14-4751-2021, https://doi.org/10.5194/gmd-14-4751-2021, 2021
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We have added a representation of the permafrost carbon feedback to the simple, open-source global carbon–climate model Hector and calibrated the results to be consistent with historical data and Earth system model projections. Our results closely match previous work, estimating around 0.2 °C of warming from permafrost this century. This capability will be useful to explore uncertainties in this feedback and for coupling with integrated assessment models for policy and economic analysis.
Liangying Zeng, Yang Yang, Hailong Wang, Jing Wang, Jing Li, Lili Ren, Huimin Li, Yang Zhou, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 21, 10745–10761, https://doi.org/10.5194/acp-21-10745-2021, https://doi.org/10.5194/acp-21-10745-2021, 2021
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Using an aerosol–climate model, the impacts of El Niño with different durations on aerosols in China are examined. The modulation on aerosol concentrations and haze days by short-duration El Niño events is 2–3 times more than that by long-duration El Niño events in China. The frequency of short-duration El Niño has been increasing significantly in recent decades, suggesting that El Niño events have exerted increasingly intense modulation on aerosol pollution in China over the past few decades.
Hossein Dadashazar, David Painemal, Majid Alipanah, Michael Brunke, Seethala Chellappan, Andrea F. Corral, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Claire Robinson, Amy Jo Scarino, Michael Shook, Kenneth Sinclair, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Xubin Zeng, Luke Ziemba, Paquita Zuidema, and Armin Sorooshian
Atmos. Chem. Phys., 21, 10499–10526, https://doi.org/10.5194/acp-21-10499-2021, https://doi.org/10.5194/acp-21-10499-2021, 2021
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This study investigates the seasonal cycle of cloud drop number concentration (Nd) over the western North Atlantic Ocean (WNAO) using multiple datasets. Reasons for the puzzling discrepancy between the seasonal cycles of Nd and aerosol concentration were identified. Results indicate that Nd is highest in winter (when aerosol proxy values are often lowest) due to conditions both linked to cold-air outbreaks and that promote greater droplet activation.
Daniele Visioni, Douglas G. MacMartin, Ben Kravitz, Olivier Boucher, Andy Jones, Thibaut Lurton, Michou Martine, Michael J. Mills, Pierre Nabat, Ulrike Niemeier, Roland Séférian, and Simone Tilmes
Atmos. Chem. Phys., 21, 10039–10063, https://doi.org/10.5194/acp-21-10039-2021, https://doi.org/10.5194/acp-21-10039-2021, 2021
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A new set of simulations is used to investigate commonalities, differences and sources of uncertainty when simulating the injection of SO2 in the stratosphere in order to mitigate the effects of climate change (solar geoengineering). The models differ in how they simulate the aerosols and how they spread around the stratosphere, resulting in differences in projected regional impacts. Overall, however, the models agree that aerosols have the potential to mitigate the warming produced by GHGs.
Nikolas O. Aksamit, Ben Kravitz, Douglas G. MacMartin, and George Haller
Atmos. Chem. Phys., 21, 8845–8861, https://doi.org/10.5194/acp-21-8845-2021, https://doi.org/10.5194/acp-21-8845-2021, 2021
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There exist robust and influential material features evolving within turbulent fluids that behave as the skeleton for fluid transport pathways. Recent developments in applied mathematics have made the identification of these time-varying structures more rigorous and insightful than ever. Using short-range wind forecasts, we detail how and why these material features can be exploited in an effort to optimize the spread of aerosols in the stratosphere for climate geoengineering.
Ben Kravitz, Douglas G. MacMartin, Daniele Visioni, Olivier Boucher, Jason N. S. Cole, Jim Haywood, Andy Jones, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Alan Robock, Roland Séférian, and Simone Tilmes
Atmos. Chem. Phys., 21, 4231–4247, https://doi.org/10.5194/acp-21-4231-2021, https://doi.org/10.5194/acp-21-4231-2021, 2021
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This study investigates multi-model response to idealized geoengineering (high CO2 with solar reduction) across two different generations of climate models. We find that, with the exception of a few cases, the results are unchanged between the different generations. This gives us confidence that broad conclusions about the response to idealized geoengineering are robust.
Andy Jones, Jim M. Haywood, Anthony C. Jones, Simone Tilmes, Ben Kravitz, and Alan Robock
Atmos. Chem. Phys., 21, 1287–1304, https://doi.org/10.5194/acp-21-1287-2021, https://doi.org/10.5194/acp-21-1287-2021, 2021
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Two different methods of simulating a geoengineering scenario are compared using data from two different Earth system models. One method is very idealised while the other includes details of a plausible mechanism. The results from both models agree that the idealised approach does not capture an impact found when detailed modelling is included, namely that geoengineering induces a positive phase of the North Atlantic Oscillation which leads to warmer, wetter winters in northern Europe.
Walker Lee, Douglas MacMartin, Daniele Visioni, and Ben Kravitz
Earth Syst. Dynam., 11, 1051–1072, https://doi.org/10.5194/esd-11-1051-2020, https://doi.org/10.5194/esd-11-1051-2020, 2020
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The injection of aerosols into the stratosphere to reflect sunlight could reduce global warming, but this type of
geoengineeringwould also impact other variables like precipitation and sea ice. In this study, we model various climate impacts of geoengineering on a 3-D graph to show how trying to meet one climate goal will affect other variables. We also present two computer simulations which validate our model and show that geoengineering could regulate precipitation as well as temperature.
Mingxuan Wu, Xiaohong Liu, Hongbin Yu, Hailong Wang, Yang Shi, Kang Yang, Anton Darmenov, Chenglai Wu, Zhien Wang, Tao Luo, Yan Feng, and Ziming Ke
Atmos. Chem. Phys., 20, 13835–13855, https://doi.org/10.5194/acp-20-13835-2020, https://doi.org/10.5194/acp-20-13835-2020, 2020
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The spatiotemporal distributions of dust aerosol simulated by global climate models (GCMs) are highly uncertain. In this study, we evaluate dust extinction profiles, optical depth, and surface concentrations simulated in three GCMs and one reanalysis against multiple satellite retrievals and surface observations to gain process-level understanding. Our results highlight the importance of correctly representing dust emission, dry/wet deposition, and size distribution in GCMs.
Bethany Sutherland, Ben Kravitz, Philip J. Rasch, and Hailong Wang
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-228, https://doi.org/10.5194/gmd-2020-228, 2020
Preprint withdrawn
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Through a cascade of physical mechanisms, a change in one location can trigger a response in a different location. These responses and the mechanisms that cause them are difficult to detect. Here we propose a method, using global climate models, to detect possible relationships between changes in one region and responses throughout the globe caused by that change. A change in the Pacific ocean is used as a test case to determine the effectiveness of the method.
Yangyang Xu, Lei Lin, Simone Tilmes, Katherine Dagon, Lili Xia, Chenrui Diao, Wei Cheng, Zhili Wang, Isla Simpson, and Lorna Burnell
Earth Syst. Dynam., 11, 673–695, https://doi.org/10.5194/esd-11-673-2020, https://doi.org/10.5194/esd-11-673-2020, 2020
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Two geoengineering schemes to mitigate global warming, (a) capturing atmospheric CO2 and (b) injecting stratospheric sulfur gas, are compared. Based on two sets of large-ensemble model experiments, we show that sulfur injection will effectively mitigate projected terrestrial drying over the Americas, and the mitigation benefit will emerge more quickly than with carbon capture. Innovative means of sulfur injection should continue to be explored as one potential low-cost climate solution.
Lili Ren, Yang Yang, Hailong Wang, Rudong Zhang, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 20, 9067–9085, https://doi.org/10.5194/acp-20-9067-2020, https://doi.org/10.5194/acp-20-9067-2020, 2020
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Observations show that the concentrations of Arctic aerosols have declined since the early 1980s, which potentially contributed to the recent, rapid Arctic warming. We found that changes in sulfate and black carbon aerosols over the midlatitudes of the Northern Hemisphere had a larger impact on Arctic temperature than other regions and that the aerosol-induced temperature change explained approximately 20 % of the observed Arctic warming during 1980–2018.
Simone Tilmes, Douglas G. MacMartin, Jan T. M. Lenaerts, Leo van Kampenhout, Laura Muntjewerf, Lili Xia, Cheryl S. Harrison, Kristen M. Krumhardt, Michael J. Mills, Ben Kravitz, and Alan Robock
Earth Syst. Dynam., 11, 579–601, https://doi.org/10.5194/esd-11-579-2020, https://doi.org/10.5194/esd-11-579-2020, 2020
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This paper introduces new geoengineering model experiments as part of a larger model intercomparison effort, using reflective particles to block some of the incoming solar radiation to reach surface temperature targets. Outcomes of these applications are contrasted based on a high greenhouse gas emission pathway and a pathway with strong mitigation and negative emissions after 2040. We compare quantities that matter for societal and ecosystem impacts between the different scenarios.
Yufei Zou, Yuhang Wang, Zuowei Xie, Hailong Wang, and Philip J. Rasch
Atmos. Chem. Phys., 20, 4999–5017, https://doi.org/10.5194/acp-20-4999-2020, https://doi.org/10.5194/acp-20-4999-2020, 2020
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We analyze the relationship between winter air stagnation and pollution extremes over eastern China and preceding Arctic sea ice loss based on climate modeling and dynamic diagnoses. We find significant increases in both the probability and intensity of air stagnation extremes in the modeling result driven by regional sea ice and sea surface temperature changes over the Pacific sector of the Arctic. We reveal the considerable impact of the Arctic climate change on mid-latitude weather extremes.
Yang Yang, Sijia Lou, Hailong Wang, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 20, 2579–2590, https://doi.org/10.5194/acp-20-2579-2020, https://doi.org/10.5194/acp-20-2579-2020, 2020
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Aerosol concentration decreased in Europe during 1980–2018, of which 7 % was induced by the changes in non-European emissions. Aerosols transported from other source regions are increasingly important to air quality in Europe. Contributions to the sulfate radiative forcing over Europe from both European and non-European emissions should decrease at a comparable rate in the next three decades. Future changes in non-European emissions are important in causing regional climate change in Europe.
Theodore Weber, Austin Corotan, Brian Hutchinson, Ben Kravitz, and Robert Link
Atmos. Chem. Phys., 20, 2303–2317, https://doi.org/10.5194/acp-20-2303-2020, https://doi.org/10.5194/acp-20-2303-2020, 2020
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Climate model emulators can save computer time but are less accurate than full climate models. We use neural networks to build emulators of precipitation, trained on existing climate model runs. By doing so, we can capture nonlinearities and how the past state of a model (to some degree) shapes the future state. Our emulator outperforms a persistence forecast of precipitation.
Hailong Wang, Jeremy G. Fyke, Jan T. M. Lenaerts, Jesse M. Nusbaumer, Hansi Singh, David Noone, Philip J. Rasch, and Rudong Zhang
The Cryosphere, 14, 429–444, https://doi.org/10.5194/tc-14-429-2020, https://doi.org/10.5194/tc-14-429-2020, 2020
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Using a climate model with unique water source tagging, we found that sea-ice anomalies in the Southern Ocean and accompanying SST changes have a significant influence on Antarctic precipitation and its source attribution through their direct impact on moisture sources and indirect impact on moisture transport. This study also highlights the importance of atmospheric dynamics in affecting the thermodynamic impact of sea-ice anomalies on regional Antarctic precipitation.
Edward Gryspeerdt, Johannes Mülmenstädt, Andrew Gettelman, Florent F. Malavelle, Hugh Morrison, David Neubauer, Daniel G. Partridge, Philip Stier, Toshihiko Takemura, Hailong Wang, Minghuai Wang, and Kai Zhang
Atmos. Chem. Phys., 20, 613–623, https://doi.org/10.5194/acp-20-613-2020, https://doi.org/10.5194/acp-20-613-2020, 2020
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Aerosol radiative forcing is a key uncertainty in our understanding of the human forcing of the climate, with much of this uncertainty coming from aerosol impacts on clouds. Observation-based estimates of the radiative forcing are typically smaller than those from global models, but it is not clear if they are more reliable. This work shows how the forcing components in global climate models can be identified, highlighting similarities between the two methods and areas for future investigation.
Hongbin Yu, Yang Yang, Hailong Wang, Qian Tan, Mian Chin, Robert C. Levy, Lorraine A. Remer, Steven J. Smith, Tianle Yuan, and Yingxi Shi
Atmos. Chem. Phys., 20, 139–161, https://doi.org/10.5194/acp-20-139-2020, https://doi.org/10.5194/acp-20-139-2020, 2020
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Emissions and long-range transport of mineral dust and
combustion-related aerosol from burning fossil fuels and biomass vary from year to year, driven by the evolution of the economy and changes in meteorological conditions and environmental regulations. This study offers both satellite and model perspectives on interannual variability and possible trends in combustion aerosol and dust in major continental outflow regions over the past 15 years (2003–2017).
George S. Fanourgakis, Maria Kanakidou, Athanasios Nenes, Susanne E. Bauer, Tommi Bergman, Ken S. Carslaw, Alf Grini, Douglas S. Hamilton, Jill S. Johnson, Vlassis A. Karydis, Alf Kirkevåg, John K. Kodros, Ulrike Lohmann, Gan Luo, Risto Makkonen, Hitoshi Matsui, David Neubauer, Jeffrey R. Pierce, Julia Schmale, Philip Stier, Kostas Tsigaridis, Twan van Noije, Hailong Wang, Duncan Watson-Parris, Daniel M. Westervelt, Yang Yang, Masaru Yoshioka, Nikos Daskalakis, Stefano Decesari, Martin Gysel-Beer, Nikos Kalivitis, Xiaohong Liu, Natalie M. Mahowald, Stelios Myriokefalitakis, Roland Schrödner, Maria Sfakianaki, Alexandra P. Tsimpidi, Mingxuan Wu, and Fangqun Yu
Atmos. Chem. Phys., 19, 8591–8617, https://doi.org/10.5194/acp-19-8591-2019, https://doi.org/10.5194/acp-19-8591-2019, 2019
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Effects of aerosols on clouds are important for climate studies but are among the largest uncertainties in climate projections. This study evaluates the skill of global models to simulate aerosol, cloud condensation nuclei (CCN) and cloud droplet number concentrations (CDNCs). Model results show reduced spread in CDNC compared to CCN due to the negative correlation between the sensitivities of CDNC to aerosol number concentration (air pollution) and updraft velocity (atmospheric dynamics).
Chandan Sarangi, Yun Qian, Karl Rittger, Kathryn J. Bormann, Ying Liu, Hailong Wang, Hui Wan, Guangxing Lin, and Thomas H. Painter
Atmos. Chem. Phys., 19, 7105–7128, https://doi.org/10.5194/acp-19-7105-2019, https://doi.org/10.5194/acp-19-7105-2019, 2019
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Radiative forcing induced by deposition of light-absorbing particles (LAPs) on snow is an important surface forcing. Here, we have used high-resolution WRF-Chem (coupled with online snow–LAP–radiation model) simulations for 2013–2014 to estimate the spatial variation in LAP-induced snow albedo darkening effect in high-mountain Asia. Significant improvement in simulated LAP–snow properties with use of a higher spatial resolution for the same model configuration is illustrated over this region.
Robert Link, Abigail Snyder, Cary Lynch, Corinne Hartin, Ben Kravitz, and Ben Bond-Lamberty
Geosci. Model Dev., 12, 1477–1489, https://doi.org/10.5194/gmd-12-1477-2019, https://doi.org/10.5194/gmd-12-1477-2019, 2019
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Earth system models (ESMs) produce the highest-quality future climate data available, but they are costly to run, so only a few runs from each model are publicly available. What is needed are emulators that tell us what would have happened, if we had been able to perform as many ESM runs as we might have liked. Much of the existing work on emulators has focused on deterministic projections of average values. Here we present a way to imbue emulators with the variability seen in ESM runs.
Yang Yang, Steven J. Smith, Hailong Wang, Catrin M. Mills, and Philip J. Rasch
Atmos. Chem. Phys., 19, 2405–2420, https://doi.org/10.5194/acp-19-2405-2019, https://doi.org/10.5194/acp-19-2405-2019, 2019
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Black carbon (BC) particles exert a potentially large warming influence on the
Earth system. We evaluate regional climate responses, non-linearity, and short-term transient responses to BC emission perturbations. We found that climate responses do not scale linearity with emissions and BC impacts temperature much faster than greenhouse gas forcing. Removing present-day BC emissions results in discernible surface temperature changes for only limited regions of the globe.
Christopher G. Fletcher, Ben Kravitz, and Bakr Badawy
Atmos. Chem. Phys., 18, 17529–17543, https://doi.org/10.5194/acp-18-17529-2018, https://doi.org/10.5194/acp-18-17529-2018, 2018
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The most important number for future climate projections is Earth's climate sensitivity (CS), or how much warming will result from increased carbon dioxide. We cannot know the true CS, and estimates of CS from climate models have a wide range. This study identifies the major factors that control this range, and we show that the choice of methods used in creating a climate model are three times more important than fine-tuning the details of the model after it is created.
Anna Possner, Hailong Wang, Robert Wood, Ken Caldeira, and Thomas P. Ackerman
Atmos. Chem. Phys., 18, 17475–17488, https://doi.org/10.5194/acp-18-17475-2018, https://doi.org/10.5194/acp-18-17475-2018, 2018
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We quantify aerosol–cloud radiative interactions in a regime of deep open-cell stratocumuli (boundary layer depth 1.5 km), a regime which remains largely unexplored within this context and yet is more dominant than cases of shallow stratocumuli previously studied. We simulate substantial increases in albedo in a regime where ship tracks are not found and argue that such changes may escape detection and attribution through remote sensing due to the large natural variability in the system.
Ben Kravitz, Philip J. Rasch, Hailong Wang, Alan Robock, Corey Gabriel, Olivier Boucher, Jason N. S. Cole, Jim Haywood, Duoying Ji, Andy Jones, Andrew Lenton, John C. Moore, Helene Muri, Ulrike Niemeier, Steven Phipps, Hauke Schmidt, Shingo Watanabe, Shuting Yang, and Jin-Ho Yoon
Atmos. Chem. Phys., 18, 13097–13113, https://doi.org/10.5194/acp-18-13097-2018, https://doi.org/10.5194/acp-18-13097-2018, 2018
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Marine cloud brightening has been proposed as a means of geoengineering/climate intervention, or deliberately altering the climate system to offset anthropogenic climate change. In idealized simulations that highlight contrasts between land and ocean, we find that the globe warms, including the ocean due to transport of heat from land. This study reinforces that no net energy input into the Earth system does not mean that temperature will necessarily remain unchanged.
Duoying Ji, Songsong Fang, Charles L. Curry, Hiroki Kashimura, Shingo Watanabe, Jason N. S. Cole, Andrew Lenton, Helene Muri, Ben Kravitz, and John C. Moore
Atmos. Chem. Phys., 18, 10133–10156, https://doi.org/10.5194/acp-18-10133-2018, https://doi.org/10.5194/acp-18-10133-2018, 2018
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We examine extreme temperature and precipitation under climate-model-simulated solar dimming and stratospheric aerosol injection geoengineering schemes. Both types of geoengineering lead to lower minimum temperatures at higher latitudes and greater cooling of minimum temperatures and maximum temperatures over land compared with oceans. Stratospheric aerosol injection is more effective in reducing tropical extreme precipitation, while solar dimming is more effective over extra-tropical regions.
Kai Zhang, Philip J. Rasch, Mark A. Taylor, Hui Wan, Ruby Leung, Po-Lun Ma, Jean-Christophe Golaz, Jon Wolfe, Wuyin Lin, Balwinder Singh, Susannah Burrows, Jin-Ho Yoon, Hailong Wang, Yun Qian, Qi Tang, Peter Caldwell, and Shaocheng Xie
Geosci. Model Dev., 11, 1971–1988, https://doi.org/10.5194/gmd-11-1971-2018, https://doi.org/10.5194/gmd-11-1971-2018, 2018
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The conservation of total water is an important numerical feature for global Earth system models. Even small conservation problems in the water budget can lead to systematic errors in century-long simulations for sea level rise projection. This study quantifies and reduces various sources of water conservation error in the atmosphere component of the Energy Exascale Earth System Model.
Hewen Niu, Shichang Kang, Hailong Wang, Rudong Zhang, Xixi Lu, Yun Qian, Rukumesh Paudyal, Shijin Wang, Xiaofei Shi, and Xingguo Yan
Atmos. Chem. Phys., 18, 6441–6460, https://doi.org/10.5194/acp-18-6441-2018, https://doi.org/10.5194/acp-18-6441-2018, 2018
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Deposition of light-absorbing carbonaceous aerosol on the surface of glaciers can greatly alter the energy fluxes of glaciers. Two years of continuous observations of carbonaceous aerosols in a glacierized region are analyzed. We mainly studied the light absorption properties of carbonaceous aerosol and have employed a global aerosol–climate model to estimate source attributions of atmospheric black carbon.
David P. Keller, Andrew Lenton, Vivian Scott, Naomi E. Vaughan, Nico Bauer, Duoying Ji, Chris D. Jones, Ben Kravitz, Helene Muri, and Kirsten Zickfeld
Geosci. Model Dev., 11, 1133–1160, https://doi.org/10.5194/gmd-11-1133-2018, https://doi.org/10.5194/gmd-11-1133-2018, 2018
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There is little consensus on the impacts and efficacy of proposed carbon dioxide removal (CDR) methods as a potential means of mitigating climate change. To address this need, the Carbon Dioxide Removal Model Intercomparison Project (or CDR-MIP) has been initiated. This project brings together models of the Earth system in a common framework to explore the potential, impacts, and challenges of CDR. Here, we describe the first set of CDR-MIP experiments.
Camilla W. Stjern, Helene Muri, Lars Ahlm, Olivier Boucher, Jason N. S. Cole, Duoying Ji, Andy Jones, Jim Haywood, Ben Kravitz, Andrew Lenton, John C. Moore, Ulrike Niemeier, Steven J. Phipps, Hauke Schmidt, Shingo Watanabe, and Jón Egill Kristjánsson
Atmos. Chem. Phys., 18, 621–634, https://doi.org/10.5194/acp-18-621-2018, https://doi.org/10.5194/acp-18-621-2018, 2018
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Marine cloud brightening (MCB) has been proposed to help limit global warming. We present here the first multi-model assessment of idealized MCB simulations from the Geoengineering Model Intercomparison Project. While all models predict a global cooling as intended, there is considerable spread between the models both in terms of radiative forcing and the climate response, largely linked to the substantial differences in the models' representation of clouds.
Jeremy Fyke, Jan T. M. Lenaerts, and Hailong Wang
The Cryosphere, 11, 2595–2609, https://doi.org/10.5194/tc-11-2595-2017, https://doi.org/10.5194/tc-11-2595-2017, 2017
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In this CESM modeling study, we uncover regional relationships in snowfall across Antarctica that are corroborated by regional modeling and ice core records. These relationships are driven by variability in large-scale atmospheric moisture transport and dampen overall Antarctic snowfall variability, with implications for Antarctic-sourced sea level variability and detection of an emergent anthropogenic signal in Antarctic mass trends.
Lars Ahlm, Andy Jones, Camilla W. Stjern, Helene Muri, Ben Kravitz, and Jón Egill Kristjánsson
Atmos. Chem. Phys., 17, 13071–13087, https://doi.org/10.5194/acp-17-13071-2017, https://doi.org/10.5194/acp-17-13071-2017, 2017
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We present results from coordinated simulations with three Earth system models focusing on the response of Earth’s radiation balance to the injection of sea salt particles. We find that in most regions the effective radiative forcing by the injected particles is equally large in cloudy and clear-sky conditions, suggesting a more important role of the aerosol direct effect in sea spray climate engineering than previously thought.
Yang Yang, Hailong Wang, Steven J. Smith, Richard Easter, Po-Lun Ma, Yun Qian, Hongbin Yu, Can Li, and Philip J. Rasch
Atmos. Chem. Phys., 17, 8903–8922, https://doi.org/10.5194/acp-17-8903-2017, https://doi.org/10.5194/acp-17-8903-2017, 2017
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Sulfate has significant impacts on air quality and climate. Local sulfate pollution could result from remote influences, making domestic mitigation efforts inefficient. Using CESM with a sulfur source-tagging technique, we found that, over regions with relatively low emissions, sulfate concentrations are primarily attributed to non-local sources and sulfate indirect radiative forcing over the Southern Hemisphere is more sensitive to emission perturbation than the polluted Northern Hemisphere.
Cary Lynch, Corinne Hartin, Ben Bond-Lamberty, and Ben Kravitz
Earth Syst. Sci. Data, 9, 281–292, https://doi.org/10.5194/essd-9-281-2017, https://doi.org/10.5194/essd-9-281-2017, 2017
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Pattern scaling climate model output is a computationally efficient way to produce a large amount of data for purposes of uncertainty quantification. Using a multi-model ensemble we explore pattern scaling methodologies across two future forcing scenarios. We find that the simple least squares approach to pattern scaling produces a close approximation of actual model output, and we use this as a justification for the creation of an open-access pattern library at multiple time increments.
Ben Kravitz, Cary Lynch, Corinne Hartin, and Ben Bond-Lamberty
Geosci. Model Dev., 10, 1889–1902, https://doi.org/10.5194/gmd-10-1889-2017, https://doi.org/10.5194/gmd-10-1889-2017, 2017
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Pattern scaling is a way of approximating regional changes without needing to run a full, complex global climate model. We compare two methods of pattern scaling for precipitation and evaluate which methods is
betterin particular circumstances. We also decompose precipitation into a CO2 portion and a non-CO2 portion. The methodologies discussed in this paper can help provide precipitation fields for other models for a wide variety of scenarios of future climate change.
Shi Zhong, Yun Qian, Chun Zhao, Ruby Leung, Hailong Wang, Ben Yang, Jiwen Fan, Huiping Yan, Xiu-Qun Yang, and Dongqing Liu
Atmos. Chem. Phys., 17, 5439–5457, https://doi.org/10.5194/acp-17-5439-2017, https://doi.org/10.5194/acp-17-5439-2017, 2017
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An online climate–chemistry coupled model (WRF-Chem) is integrated for 5 years at cloud-permitting scale to quantify the impacts of urbanization-induced changes in land cover and pollutants emission on regional climate in the Yangtze River Delta region in eastern China. Urbanization over this region increases the frequency of extreme precipitation and heat wave in summer. The results could help China government in making policies in mitigating the environmental impact of urbanization.
Yang Yang, Hailong Wang, Steven J. Smith, Po-Lun Ma, and Philip J. Rasch
Atmos. Chem. Phys., 17, 4319–4336, https://doi.org/10.5194/acp-17-4319-2017, https://doi.org/10.5194/acp-17-4319-2017, 2017
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The source attributions of black carbon (BC) in China are quantified using the Community Earth System Model by source tagging. BC impacts neighboring regions greatly. Transport is important in increasing BC during regional polluted days. Emissions outside China contribute 35 % of BC direct radiative forcing in China. Efficiency analysis shows that reduction in BC emissions over eastern China could have a greater benefit for regional air quality in China, especially in the winter haze season.
Hiroki Kashimura, Manabu Abe, Shingo Watanabe, Takashi Sekiya, Duoying Ji, John C. Moore, Jason N. S. Cole, and Ben Kravitz
Atmos. Chem. Phys., 17, 3339–3356, https://doi.org/10.5194/acp-17-3339-2017, https://doi.org/10.5194/acp-17-3339-2017, 2017
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This study analyses shortwave radiation (SW) in the G4 experiment of the Geoengineering Model Intercomparison Project. G4 involves stratospheric injection of 5 Tg yr−1 of SO2 against the RCP4.5 scenario. The global mean forcing of the sulphate geoengineering has an inter-model variablity of −3.6 to −1.6 W m−2, implying a high uncertainty in modelled processes of sulfate aerosols. Changes in water vapour and cloud amounts due to the SO2 injection weaken the forcing at the surface by around 50 %.
Corey J. Gabriel, Alan Robock, Lili Xia, Brian Zambri, and Ben Kravitz
Atmos. Chem. Phys., 17, 595–613, https://doi.org/10.5194/acp-17-595-2017, https://doi.org/10.5194/acp-17-595-2017, 2017
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The National Center for Atmospheric Research CESM-CAM4-CHEM global climate model was modified to simulate a scheme in which the albedo of the ocean surface is raised over the subtropical ocean gyres in the Southern Hemisphere. Global mean surface temperature in G4Foam is 0.6K lower than RCP6.0, with statistically significant cooling relative to RCP6.0 south of 30° N and an increase in rainfall over land, most pronouncedly during the JJA season, relative to both G4SSA and RCP6.0.
Douglas G. MacMartin and Ben Kravitz
Atmos. Chem. Phys., 16, 15789–15799, https://doi.org/10.5194/acp-16-15789-2016, https://doi.org/10.5194/acp-16-15789-2016, 2016
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Solar geoengineering has been proposed as a possible additional approach for managing risks of climate change, by reflecting some sunlight back to space. To project climate effects resulting from future choices regarding both greenhouse gas emissions and solar geoengineering, it is useful to have a computationally efficient "emulator" that approximates the behavior of more complex climate models. We present such an emulator here, and validate the underlying assumption of linearity.
Cary Lynch, Corinne Hartin, Ben Bond-Lamberty, and Ben Kravitz
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2016-170, https://doi.org/10.5194/gmd-2016-170, 2016
Revised manuscript not accepted
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Pattern scaling is used to explore uncertainty in future forcing scenarios and assess local climate sensitivity to global temperature change. This paper examines the two dominant pattern scaling methods using a multi-model ensemble with two future socio-economic storylines. We find that high latitudes show the strongest sensitivity to global temperature change and that the simple least squared regression approach to generation of patterns is a better fit to projected global temperature.
Ben Kravitz, Douglas G. MacMartin, Hailong Wang, and Philip J. Rasch
Earth Syst. Dynam., 7, 469–497, https://doi.org/10.5194/esd-7-469-2016, https://doi.org/10.5194/esd-7-469-2016, 2016
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Most simulations of solar geoengineering prescribe a particular strategy and evaluate its modeled effects. Here we first choose example climate objectives and then design a strategy to meet those objectives in climate models. We show that certain objectives can be met simultaneously even in the presence of uncertainty, and the strategy for meeting those objectives can be ported to other models. This is part of a broader illustration of how uncertainties in solar geoengineering can be managed.
N. I. Kristiansen, A. Stohl, D. J. L. Olivié, B. Croft, O. A. Søvde, H. Klein, T. Christoudias, D. Kunkel, S. J. Leadbetter, Y. H. Lee, K. Zhang, K. Tsigaridis, T. Bergman, N. Evangeliou, H. Wang, P.-L. Ma, R. C. Easter, P. J. Rasch, X. Liu, G. Pitari, G. Di Genova, S. Y. Zhao, Y. Balkanski, S. E. Bauer, G. S. Faluvegi, H. Kokkola, R. V. Martin, J. R. Pierce, M. Schulz, D. Shindell, H. Tost, and H. Zhang
Atmos. Chem. Phys., 16, 3525–3561, https://doi.org/10.5194/acp-16-3525-2016, https://doi.org/10.5194/acp-16-3525-2016, 2016
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Processes affecting aerosol removal from the atmosphere are not fully understood. In this study we investigate to what extent atmospheric transport models can reproduce observed loss of aerosols. We compare measurements of radioactive isotopes, that attached to ambient sulfate aerosols during the 2011 Fukushima nuclear accident, to 19 models using identical emissions. Results indicate aerosol removal that is too fast in most models, and apply to aerosols that have undergone long-range transport.
Shipeng Zhang, Minghuai Wang, Steven J. Ghan, Aijun Ding, Hailong Wang, Kai Zhang, David Neubauer, Ulrike Lohmann, Sylvaine Ferrachat, Toshihiko Takeamura, Andrew Gettelman, Hugh Morrison, Yunha Lee, Drew T. Shindell, Daniel G. Partridge, Philip Stier, Zak Kipling, and Congbin Fu
Atmos. Chem. Phys., 16, 2765–2783, https://doi.org/10.5194/acp-16-2765-2016, https://doi.org/10.5194/acp-16-2765-2016, 2016
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The variation of aerosol indirect effects (AIE) in several climate models is investigated across different dynamical regimes. Regimes with strong large-scale ascent are shown to be as important as stratocumulus regimes in studying AIE. AIE over regions with high monthly large-scale surface precipitation rate contributes the most to the total aerosol indirect forcing. These results point to the need to reduce the uncertainty in AIE in different dynamical regimes.
X. Liu, P.-L. Ma, H. Wang, S. Tilmes, B. Singh, R. C. Easter, S. J. Ghan, and P. J. Rasch
Geosci. Model Dev., 9, 505–522, https://doi.org/10.5194/gmd-9-505-2016, https://doi.org/10.5194/gmd-9-505-2016, 2016
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In this study, we describe and evaluate a new four-mode version of the Modal Aerosol Module (MAM4) in the Community Atmosphere Model version 5 (CAM5). Compared to the current three-mode version of MAM in CAM5, MAM4 significantly improves the simulation of seasonal variation of BC concentrations in the polar regions, by increasing the BC concentrations in all seasons and particularly in cold seasons.
R. Zhang, H. Wang, D. A. Hegg, Y. Qian, S. J. Doherty, C. Dang, P.-L. Ma, P. J. Rasch, and Q. Fu
Atmos. Chem. Phys., 15, 12805–12822, https://doi.org/10.5194/acp-15-12805-2015, https://doi.org/10.5194/acp-15-12805-2015, 2015
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We use a global climate model with an explicit source tagging technique to quantify contributions of emissions from various geographical regions and sectors to BC in North America. Model results are evaluated against measurements of near-surface and in-snow BC. We found strong spatial variations of BC and its radiative forcing that can be quantitatively attributed to the various source origins, and also identified a significant source of BC in snow that is likely missing in most climate models.
B. Kravitz, A. Robock, S. Tilmes, O. Boucher, J. M. English, P. J. Irvine, A. Jones, M. G. Lawrence, M. MacCracken, H. Muri, J. C. Moore, U. Niemeier, S. J. Phipps, J. Sillmann, T. Storelvmo, H. Wang, and S. Watanabe
Geosci. Model Dev., 8, 3379–3392, https://doi.org/10.5194/gmd-8-3379-2015, https://doi.org/10.5194/gmd-8-3379-2015, 2015
R. Zhang, H. Wang, Y. Qian, P. J. Rasch, R. C. Easter, P.-L. Ma, B. Singh, J. Huang, and Q. Fu
Atmos. Chem. Phys., 15, 6205–6223, https://doi.org/10.5194/acp-15-6205-2015, https://doi.org/10.5194/acp-15-6205-2015, 2015
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We use the CAM5 model with a novel source-tagging technique to characterize the fate of BC particles emitted from various geographical regions and sectors and their transport pathways to the Himalayas and Tibetan Plateau (HTP). We show a comprehensive picture of the seasonal and regional dependence of BC source attributions, and find strong seasonal and spatial variations in BC-in-snow radiative forcing in the HTP that can be quantitatively attributed to the various regional/sectoral sources.
M. Wang, B. Xu, J. Cao, X. Tie, H. Wang, R. Zhang, Y. Qian, P. J. Rasch, S. Zhao, G. Wu, H. Zhao, D. R. Joswiak, J. Li, and Y. Xie
Atmos. Chem. Phys., 15, 1191–1204, https://doi.org/10.5194/acp-15-1191-2015, https://doi.org/10.5194/acp-15-1191-2015, 2015
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Carbonaceous aerosols recorded in a Tibetan glacier present a distinct seasonal dependence and an increasing trend after 1980, which has important implications for the accelerated glacier melting. We use a global aerosol--climate model to quantify the aerosol source--receptor relationships, showing that emissions in South Asia had the largest contribution. The emission inventories and historical fuel consumption in South Asia are consistent with our ice-core analysis and model results.
S. Tilmes, M. J. Mills, U. Niemeier, H. Schmidt, A. Robock, B. Kravitz, J.-F. Lamarque, G. Pitari, and J. M. English
Geosci. Model Dev., 8, 43–49, https://doi.org/10.5194/gmd-8-43-2015, https://doi.org/10.5194/gmd-8-43-2015, 2015
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A new Geoengineering Model Intercomparison Project (GeoMIP) experiment “G4 specified stratospheric aerosols” (G4SSA) is proposed to investigate the impact of stratospheric aerosol geoengineering on atmosphere, chemistry, dynamics, climate, and the environment. In contrast to the earlier G4 GeoMIP experiment, which requires an emission of sulfur dioxide (SO2) into the model, a prescribed aerosol forcing file is provided to the community, to be consistently applied to future model experiments.
C. Zhao, Z. Hu, Y. Qian, L. Ruby Leung, J. Huang, M. Huang, J. Jin, M. G. Flanner, R. Zhang, H. Wang, H. Yan, Z. Lu, and D. G. Streets
Atmos. Chem. Phys., 14, 11475–11491, https://doi.org/10.5194/acp-14-11475-2014, https://doi.org/10.5194/acp-14-11475-2014, 2014
C. Zhao, X. Liu, Y. Qian, J. Yoon, Z. Hou, G. Lin, S. McFarlane, H. Wang, B. Yang, P.-L. Ma, H. Yan, and J. Bao
Atmos. Chem. Phys., 13, 10969–10987, https://doi.org/10.5194/acp-13-10969-2013, https://doi.org/10.5194/acp-13-10969-2013, 2013
H. Wang, R. C. Easter, P. J. Rasch, M. Wang, X. Liu, S. J. Ghan, Y. Qian, J.-H. Yoon, P.-L. Ma, and V. Vinoj
Geosci. Model Dev., 6, 765–782, https://doi.org/10.5194/gmd-6-765-2013, https://doi.org/10.5194/gmd-6-765-2013, 2013
Related subject area
Subject: Dynamics | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Wintertime extreme warming events in the high Arctic: characteristics, drivers, trends, and the role of atmospheric rivers
Influence of lower-tropospheric moisture on local soil moisture–precipitation feedback over the US Southern Great Plains
The Lagrangian Atmospheric Radionuclide Transport Model (ARTM) – sensitivity studies and evaluation using airborne measurements of power plant emissions
Large-eddy-model closure and simulation of turbulent flux patterns over oasis surface
Technical note: Exploring parameter and meteorological uncertainty via emulation in volcanic ash atmospheric dispersion modelling
Impact of the Guinea coast upwelling on atmospheric dynamics, precipitation and pollutant transport over southern West Africa
Investigating multiscale meteorological controls and impact of soil moisture heterogeneity on radiation fog in complex terrain using semi-idealised simulations
Effect of the boundary layer low-level jet on fast fog spatial propagation
Extreme ozone episodes in a major Mediterranean urban area
Mediterranean tropical-like cyclone forecasts and analysis using the ECMWF ensemble forecasting system with physical parameterization perturbations
Using synthetic case studies to explore the spread and calibration of ensemble atmospheric dispersion forecasts
Potential modulation of Indian Ocean basin mode on the interdecadal variations of summer precipitation over the East Asian monsoon boundary zone
Meteorological modeling sensitivity to parameterizations and satellite-derived surface datasets during the 2017 Lake Michigan Ozone Study
Trajectory enhancement of low-earth orbiter thermodynamic retrievals to predict convection: a simulation experiment
Lagrangian transport simulations using the extreme convection parameterization: an assessment for the ECMWF reanalyses
Better-constrained climate sensitivity when accounting for dataset dependency on pattern effect estimates
Determination of the chemical equator from GEOS-Chem model simulation: a focus on the tropical western Pacific region
The influences of El Niño–Southern Oscillation on tropospheric ozone in CMIP6 models
Uncertainty in parameterized convection remains a key obstacle for estimating surface fluxes of carbon dioxide
Antarctic atmospheric Richardson number from radiosonde measurements and AMPS
Divergent convective outflow in large-eddy simulations
Modulation of daily PM2.5 concentrations over China in winter by large-scale circulation and climate change
Modeling of street-scale pollutant dispersion by coupled simulation of chemical reaction, aerosol dynamics, and CFD
Daytime along-valley winds in the Himalayas as simulated by the Weather Research and Forecasting (WRF) model
Evolution of squall line variability and error growth in an ensemble of large eddy simulations
Climatology and variability of air mass transport from the boundary layer to the Asian monsoon anticyclone
Evaluation and bias correction of probabilistic volcanic ash forecasts
The representation of the trade winds in ECMWF forecasts and reanalyses during EUREC4A
Modeling approaches for atmospheric ion–dipole collisions: all-atom trajectory simulations and central field methods
Parameterizing the aerodynamic effect of trees in street canyons for the street network model MUNICH using the CFD model Code_Saturne
Quantifying the impact of meteorological uncertainty on emission estimates and the risk to aviation using source inversion for the Raikoke 2019 eruption
Acceleration of the southern African easterly jet driven by the radiative effect of biomass burning aerosols and its impact on transport during AEROCLO-sA
The Sun's role in decadal climate predictability in the North Atlantic
Future projections of daily haze-conducive and clear weather conditions over the North China Plain using a perturbed parameter ensemble
Refining an ensemble of volcanic ash forecasts using satellite retrievals: Raikoke 2019
Ship-based estimates of momentum transfer coefficient over sea ice and recommendations for its parameterization
Revising the definition of anthropogenic heat flux from buildings: role of human activities and building storage heat flux
An assessment of tropopause characteristics of the ERA5 and ERA-Interim meteorological reanalyses
Distinct evolutions of haze pollution from winter to the following spring over the North China Plain: role of the North Atlantic sea surface temperature anomalies
The foehn effect during easterly flow over Svalbard
Effect of rainfall-induced diabatic heating over southern China on the formation of wintertime haze on the North China Plain
Anthropogenic aerosol effects on tropospheric circulation and sea surface temperature (1980–2020): separating the role of zonally asymmetric forcings
Lightning-ignited wildfires and long continuing current lightning in the Mediterranean Basin: preferential meteorological conditions
Identifying source regions of air masses sampled at the tropical high-altitude site of Chacaltaya using WRF-FLEXPART and cluster analysis
Modelling spatiotemporal variations of the canopy layer urban heat island in Beijing at the neighbourhood scale
Dispersion of particulate matter (PM2.5) from wood combustion for residential heating: optimization of mitigation actions based on large-eddy simulations
Measurement report: Effect of wind shear on PM10 concentration vertical structure in the urban boundary layer in a complex terrain
The effect of forced change and unforced variability in heat waves, temperature extremes, and associated population risk in a CO2-warmed world
Convective self–aggregation in a mean flow
The potential for geostationary remote sensing of NO2 to improve weather prediction
Weiming Ma, Hailong Wang, Gang Chen, Yun Qian, Ian Baxter, Yiling Huo, and Mark W. Seefeldt
Atmos. Chem. Phys., 24, 4451–4472, https://doi.org/10.5194/acp-24-4451-2024, https://doi.org/10.5194/acp-24-4451-2024, 2024
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Extreme warming events with surface temperature going above 0°C can occur in the high-Arctic winter. Although reanalysis data show that these events were short-lived and occurred rarely during 1980–2021, they have become more frequent, stronger, and longer lasting latterly. A dipole pattern, comprising high- and low-pressure systems, is found to be the key in driving them. These findings have implications for the recent changes in sea ice, hydrological cycle, and ecosystem over the Arctic.
Gaoyun Wang, Rong Fu, Yizhou Zhuang, Paul A. Dirmeyer, Joseph A. Santanello, Guiling Wang, Kun Yang, and Kaighin McColl
Atmos. Chem. Phys., 24, 3857–3868, https://doi.org/10.5194/acp-24-3857-2024, https://doi.org/10.5194/acp-24-3857-2024, 2024
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This study investigates the influence of lower-tropospheric humidity on land–atmosphere coupling (LAC) during warm seasons in the US Southern Great Plains. Using radiosonde data and a buoyancy model, we find that elevated LT humidity is crucial for generating afternoon precipitation events under dry soil conditions not accounted for by conventional LAC indices. This underscores the importance of considering LT humidity in understanding LAC over dry soil during droughts in the SGP.
Robert Hanfland, Dominik Brunner, Christiane Voigt, Alina Fiehn, Anke Roiger, and Margit Pattantyús-Ábrahám
Atmos. Chem. Phys., 24, 2511–2534, https://doi.org/10.5194/acp-24-2511-2024, https://doi.org/10.5194/acp-24-2511-2024, 2024
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To show that the three-dimensional dispersion of plumes simulated by the Atmospheric Radionuclide Transport Model within the planetary boundary layer agrees with real plumes, we identify the most important input parameters and analyse the turbulence properties of five different turbulence models in very unstable stratification conditions using their deviation from the well-mixed state. Simulations show that one model agrees slightly better in unstable stratification conditions.
Bangjun Cao, Yaping Shao, Xianyu Yang, Xin Yin, and Shaofeng Liu
Atmos. Chem. Phys., 24, 275–285, https://doi.org/10.5194/acp-24-275-2024, https://doi.org/10.5194/acp-24-275-2024, 2024
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Our novel scheme enhances large-eddy simulations (LESs) for atmosphere–land interactions. It couples LES subgrid closure with Monin–Obukhov similarity theory (MOST), overcoming MOST's limitations. Validated over diverse land surfaces, our approach outperforms existing methods, aligning well with field measurements. Robustness is demonstrated across varying model resolutions. MOST's influence strengthens with decreasing grid spacing, particularly for sensible heat flux.
James M. Salter, Helen N. Webster, and Cameron Saint
EGUsphere, https://doi.org/10.5194/egusphere-2023-2870, https://doi.org/10.5194/egusphere-2023-2870, 2023
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Models are used to make forecasts of volcanic ash dispersion during eruptions. These models have unknown inputs relating to the eruption itself, physical processes, and meteorological conditions. We use statistical models to predict the output of the expensive physical model and show we can account for the effects of the different inputs. We compare the model to real-world observations and show that accounting for all sources of uncertainty may lead to different conclusions about the inputs.
Gaëlle de Coëtlogon, Adrien Deroubaix, Cyrille Flamant, Laurent Menut, and Marco Gaetani
Atmos. Chem. Phys., 23, 15507–15521, https://doi.org/10.5194/acp-23-15507-2023, https://doi.org/10.5194/acp-23-15507-2023, 2023
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Using a numerical atmospheric model, we found that cooling sea surface temperatures along the southern coast of West Africa in July cause the “little dry season”. This effect reduces humidity and pollutant transport inland, potentially enhancing West Africa's synoptic and seasonal forecasting.
Dongqi Lin, Marwan Katurji, Laura E. Revell, Basit Khan, and Andrew Sturman
Atmos. Chem. Phys., 23, 14451–14479, https://doi.org/10.5194/acp-23-14451-2023, https://doi.org/10.5194/acp-23-14451-2023, 2023
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Accurate fog forecasting is difficult in a complex environment. Spatial variations in soil moisture could impact fog. Here, we carried out fog simulations with spatially different soil moisture in complex topography. The soil moisture was calculated using satellite observations. The results show that the spatial variations in soil moisture do not have a significant impact on where fog occurs but do impact how long fog lasts. This finding could improve fog forecasts in the future.
Shuqi Yan, Hongbin Wang, Xiaohui Liu, Fan Zu, and Duanyang Liu
Atmos. Chem. Phys., 23, 13987–14002, https://doi.org/10.5194/acp-23-13987-2023, https://doi.org/10.5194/acp-23-13987-2023, 2023
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In this study, we quantitatively study the effect of the boundary layer low-level jet (BLLJ) on fast fog spatial propagation; i.e., the fog area expands very fast along a certain direction. The wind speed (10 m s−1) and direction (southeast) of the BLLJ core are consistent with fog propagation (9.6 m s−1). The BLLJ-induced temperature and moisture advections are possible reasons for fast fog propagation. The propagation speed would decrease by 6.4 m s−1 if these advections were turned off.
Jordi Massagué, Eduardo Torre-Pascual, Cristina Carnerero, Miguel Escudero, Andrés Alastuey, Marco Pandolfi, Xavier Querol, and Gotzon Gangoiti
EGUsphere, https://doi.org/10.5194/egusphere-2023-2449, https://doi.org/10.5194/egusphere-2023-2449, 2023
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This study analysed extreme ozone episodes in Barcelona, which have occurred only in recent years and are of particular concern due to the city's significant population. The research reveals that these episodes result from a complex interplay of factors, including the effects of pollution transport from regional to local sources and specific weather and emission patterns. These findings advance the understanding of the mechanisms behind these episodes and strengthen predictive capabilities.
Miriam Saraceni, Lorenzo Silvestri, Peter Bechtold, and Paolina Bongioannini Cerlini
Atmos. Chem. Phys., 23, 13883–13909, https://doi.org/10.5194/acp-23-13883-2023, https://doi.org/10.5194/acp-23-13883-2023, 2023
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This study focuses on three medicanes, tropical-like cyclones that form in the Mediterranean Sea, studied by ensemble forecasting. This involved multiple simulations of the same event by varying initial conditions and model physics parameters, especially related to convection, which showed comparable results. It is found that medicane development is influenced by the model's ability to predict precursor events and the interaction between upper and lower atmosphere dynamics and thermodynamics.
Andrew R. Jones, Susan J. Leadbetter, and Matthew C. Hort
Atmos. Chem. Phys., 23, 12477–12503, https://doi.org/10.5194/acp-23-12477-2023, https://doi.org/10.5194/acp-23-12477-2023, 2023
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The paper explores spread and calibration properties of ensemble atmospheric dispersion forecasts for hypothetical release events. Real-time forecasts from an ensemble weather prediction system were used to generate an ensemble of dispersion predictions and assessed against simulations produced using analysis meteorology. Results demonstrate good performance overall but highlight more skilful predictions for material released in the upper air compared with releases near the surface.
Jing Wang, Yanju Liu, Fei Cheng, Chengyu Song, Qiaoping Li, Yihui Ding, and Xiangde Xu
EGUsphere, https://doi.org/10.5194/egusphere-2023-1529, https://doi.org/10.5194/egusphere-2023-1529, 2023
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Based on long-term observational, reanalysis, and numerical model simulation datasets from 1901 through 2014, this study identify that precipitation over the East Asian monsoon boundary zone featured prominent interdecadal changes, with dry summers during the periods preceding 1927, 1968–1982, and 1998–2010, and wet summers during the periods of 1928–1938, 1946–1967, and 2011 onwards. The Indian Ocean basin mode is an important oceanic modulator responsible for its interdecadal variations.
Jason A. Otkin, Lee M. Cronce, Jonathan L. Case, R. Bradley Pierce, Monica Harkey, Allen Lenzen, David S. Henderson, Zac Adelman, Tsengel Nergui, and Christopher R. Hain
Atmos. Chem. Phys., 23, 7935–7954, https://doi.org/10.5194/acp-23-7935-2023, https://doi.org/10.5194/acp-23-7935-2023, 2023
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We performed model simulations to assess the impact of different parameterization schemes, surface initialization datasets, and analysis nudging on lower-tropospheric conditions near Lake Michigan. Simulations were run with high-resolution, real-time datasets depicting lake surface temperatures, green vegetation fraction, and soil moisture. The most accurate results were obtained when using high-resolution sea surface temperature and soil datasets to constrain the model simulations.
Mark T. Richardson, Brian H. Kahn, and Peter Kalmus
Atmos. Chem. Phys., 23, 7699–7717, https://doi.org/10.5194/acp-23-7699-2023, https://doi.org/10.5194/acp-23-7699-2023, 2023
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Convection over land often triggers hours after a satellite last passed overhead and measured the state of the atmosphere, and during those hours the atmosphere can change greatly. Here we show that it is possible to reconstruct most of those changes by using weather forecast winds to predict where warm and moist air parcels will travel. The results can be used to better predict where precipitation is likely to happen in the hours after satellite measurements.
Lars Hoffmann, Paul Konopka, Jan Clemens, and Bärbel Vogel
Atmos. Chem. Phys., 23, 7589–7609, https://doi.org/10.5194/acp-23-7589-2023, https://doi.org/10.5194/acp-23-7589-2023, 2023
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Atmospheric convection plays a key role in tracer transport in the troposphere. Global meteorological forecasts and reanalyses typically have a coarse spatiotemporal resolution that does not adequately resolve the dynamics, transport, and mixing of air associated with storm systems or deep convection. We discuss the application of the extreme convection parameterization in a Lagrangian transport model to improve simulations of tracer transport from the boundary layer into the free troposphere.
Angshuman Modak and Thorsten Mauritsen
Atmos. Chem. Phys., 23, 7535–7549, https://doi.org/10.5194/acp-23-7535-2023, https://doi.org/10.5194/acp-23-7535-2023, 2023
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We provide an improved estimate of equilibrium climate sensitivity (ECS) constrained based on the instrumental temperature record including the corrections for the pattern effect. The improved estimate factors in the uncertainty caused by the underlying sea-surface temperature datasets used in the estimates of pattern effect. This together with the inter-model spread lifts the corresponding IPCC AR6 estimate to 3.2 K [1.8 to 11.0], which is lower and better constrained than in past studies.
Xiaoyu Sun, Mathias Palm, Katrin Müller, Jonas Hachmeister, and Justus Notholt
Atmos. Chem. Phys., 23, 7075–7090, https://doi.org/10.5194/acp-23-7075-2023, https://doi.org/10.5194/acp-23-7075-2023, 2023
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The tropical western Pacific (TWP) is an active interhemispheric transport region contributing significantly to the global climate. A method to determine the chemical equator was developed by model simulations of a virtual passive tracer to analyze transport in the tropics, with a focus on the TWP region. We compare the chemical equator with tropical rain belts and wind fields and obtain a vertical pattern of interhemispheric transport processes which shows tilt structure in certain seasons.
Thanh Le, Seon-Ho Kim, Jae-Yeong Heo, and Deg-Hyo Bae
EGUsphere, https://doi.org/10.5194/egusphere-2023-207, https://doi.org/10.5194/egusphere-2023-207, 2023
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We examined the links between El Niño–Southern Oscillation (ENSO) and tropospheric ozone (O3) using models’ data. Our results show that ENSO impacts on tropospheric O3 are mainly found over oceans, while the signature of ENSO over continents is largely unclear. These impacts in the mid-latitude regions over the southern hemisphere may be more significant than previously known. The responses of O3 to ENSO are weak in the middle troposphere and are stronger in the upper and lower troposphere.
Andrew E. Schuh and Andrew R. Jacobson
Atmos. Chem. Phys., 23, 6285–6297, https://doi.org/10.5194/acp-23-6285-2023, https://doi.org/10.5194/acp-23-6285-2023, 2023
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A comparison of atmospheric carbon dioxide concentrations resulting from two different atmospheric transport models showed large differences in predicted concentrations with significant space–time correlations. The vertical mixing of long-lived trace gases by convection was determined to be the main driver of these differences. The resulting uncertainty was deemed significant to the application of using atmospheric gradients of carbon dioxide to estimate surface fluxes of carbon dioxide.
Qike Yang, Xiaoqing Wu, Xiaodan Hu, Zhiyuan Wang, Chun Qing, Tao Luo, Pengfei Wu, Xianmei Qian, and Yiming Guo
Atmos. Chem. Phys., 23, 6339–6355, https://doi.org/10.5194/acp-23-6339-2023, https://doi.org/10.5194/acp-23-6339-2023, 2023
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The AMPS-forecasted Richardson number was first comprehensively validated over the Antarctic continent. Some potential underlying reasons for the discrepancies between the forecasts and observations were analyzed. The underlying physical processes of triggering atmospheric turbulence in Antarctica were investigated. Our results suggest that the estimated Richardson number by the AMPS is reasonable and the turbulence conditions in Antarctica are well revealed.
Edward Groot and Holger Tost
Atmos. Chem. Phys., 23, 6065–6081, https://doi.org/10.5194/acp-23-6065-2023, https://doi.org/10.5194/acp-23-6065-2023, 2023
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It is shown that the outflow from cumulonimbus clouds or thunderstorms in the upper troposphere and lower stratosphere in idealized high-resolution simulations (LESs) depends linearly on the net amount of latent heat released by the cloud for fixed geometry of the clouds. However, it is shown that, in more realistic situations, convective organization and aggregation (collecting mechanisms of cumulonimbus clouds) affect the amount of outflow non-linearly through non-idealized geometry.
Zixuan Jia, Carlos Ordóñez, Ruth M. Doherty, Oliver Wild, Steven T. Turnock, and Fiona M. O'Connor
Atmos. Chem. Phys., 23, 2829–2842, https://doi.org/10.5194/acp-23-2829-2023, https://doi.org/10.5194/acp-23-2829-2023, 2023
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This study investigates the influence of the winter large-scale circulation on daily concentrations of PM2.5 and their sensitivity to emissions. The new proposed circulation index can effectively distinguish different levels of air pollution and explain changes in PM2.5 sensitivity to emissions from local and surrounding regions. We then project future changes in PM2.5 concentrations using this index and find an increase in PM2.5 concentrations over the region due to climate change.
Chao Lin, Yunyi Wang, Ryozo Ooka, Cédric Flageul, Youngseob Kim, Hideki Kikumoto, Zhizhao Wang, and Karine Sartelet
Atmos. Chem. Phys., 23, 1421–1436, https://doi.org/10.5194/acp-23-1421-2023, https://doi.org/10.5194/acp-23-1421-2023, 2023
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In this study, SSH-aerosol, a modular box model that simulates the evolution of gas, primary, and secondary aerosols, is coupled with the computational fluid dynamics (CFD) software, OpenFOAM and Code_Saturne. The transient dispersion of pollutants emitted from traffic in a street canyon of Greater Paris is simulated. The coupled model achieved better agreement in NO2 and PM10 with measurement data than the conventional CFD simulation which regards pollutants as passive scalars.
Johannes Mikkola, Victoria A. Sinclair, Marja Bister, and Federico Bianchi
Atmos. Chem. Phys., 23, 821–842, https://doi.org/10.5194/acp-23-821-2023, https://doi.org/10.5194/acp-23-821-2023, 2023
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Local winds in four valleys located in the Nepal Himalayas are studied by means of high-resolution meteorological modelling. Well-defined daytime up-valley winds are simulated in all of the valleys with some variation in the flow depth and strength among the valleys and their parts. Parts of the valleys with a steep valley floor inclination (2–5°) are associated with weaker and shallower daytime up-valley winds compared with the parts that have nearly flat valley floors (< 1°).
Edward Groot and Holger Tost
Atmos. Chem. Phys., 23, 565–585, https://doi.org/10.5194/acp-23-565-2023, https://doi.org/10.5194/acp-23-565-2023, 2023
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Thunderstorm systems play an important role in the dynamics of the Earth’s atmosphere, and some of them form a well-organised line: squall lines. Simulations of such squall lines with very small initial perturbations are compared to a reference simulation. The evolution of perturbations and processes amplifying them are analysed. It is shown that the formation of new secondary thunderstorm cells (after the initial primary cells) directly ahead of the line affects the spread strongly.
Matthias Nützel, Sabine Brinkop, Martin Dameris, Hella Garny, Patrick Jöckel, Laura L. Pan, and Mijeong Park
Atmos. Chem. Phys., 22, 15659–15683, https://doi.org/10.5194/acp-22-15659-2022, https://doi.org/10.5194/acp-22-15659-2022, 2022
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During the Asian summer monsoon season, a large high-pressure system is present at levels close to the tropopause above Asia. We analyse how air masses are transported from surface levels to this high-pressure system, which shows distinct features from the surrounding air masses. To this end, we employ multiannual data from two complementary models that allow us to analyse the climatology as well as the interannual and intraseasonal variability of these transport pathways.
Alice Crawford, Tianfeng Chai, Binyu Wang, Allison Ring, Barbara Stunder, Christopher P. Loughner, Michael Pavolonis, and Justin Sieglaff
Atmos. Chem. Phys., 22, 13967–13996, https://doi.org/10.5194/acp-22-13967-2022, https://doi.org/10.5194/acp-22-13967-2022, 2022
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This study describes the development of a workflow which produces probabilistic and quantitative forecasts of volcanic ash in the atmosphere. The workflow includes methods of incorporating satellite observations of the ash cloud into a modeling framework as well as verification statistics that can be used to guide further model development and provide information for risk-based approaches to flight planning.
Alessandro Carlo Maria Savazzi, Louise Nuijens, Irina Sandu, Geet George, and Peter Bechtold
Atmos. Chem. Phys., 22, 13049–13066, https://doi.org/10.5194/acp-22-13049-2022, https://doi.org/10.5194/acp-22-13049-2022, 2022
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Winds are of great importance for the transport of energy and moisture in the atmosphere. In this study we use measurements from the EUREC4A field campaign and several model experiments to understand the wind bias in the forecasts produced by the European Centre for Medium-Range Weather Forecasts. We are able to link the model errors to heights above 2 km and to the representation of the diurnal cycle of winds: the model makes the winds too slow in the morning and too strong in the evening.
Ivo Neefjes, Roope Halonen, Hanna Vehkamäki, and Bernhard Reischl
Atmos. Chem. Phys., 22, 11155–11172, https://doi.org/10.5194/acp-22-11155-2022, https://doi.org/10.5194/acp-22-11155-2022, 2022
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Collisions between ionic and dipolar molecules and clusters facilitate the formation of atmospheric aerosol particles, which affect global climate and air quality. We compared often-used classical approaches for calculating ion–dipole collision rates with robust atomistic computer simulations. While classical approaches work for simple ions and dipoles only, our modeling approach can also efficiently calculate reasonable collision properties for more complex systems.
Alice Maison, Cédric Flageul, Bertrand Carissimo, Yunyi Wang, Andrée Tuzet, and Karine Sartelet
Atmos. Chem. Phys., 22, 9369–9388, https://doi.org/10.5194/acp-22-9369-2022, https://doi.org/10.5194/acp-22-9369-2022, 2022
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This paper presents a parameterization of the tree crown effect on air flow and pollutant dispersion in a street network model used to simulate air quality at the street level. The new parameterization is built using a finer-scale model (computational fluid dynamics). The tree effect increases with the leaf area index and the crown volume fraction of the trees; the street horizontal velocity is reduced by up to 68 % and the vertical transfer into or out of the street by up to 23 %.
Natalie J. Harvey, Helen F. Dacre, Cameron Saint, Andrew T. Prata, Helen N. Webster, and Roy G. Grainger
Atmos. Chem. Phys., 22, 8529–8545, https://doi.org/10.5194/acp-22-8529-2022, https://doi.org/10.5194/acp-22-8529-2022, 2022
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In the event of a volcanic eruption, airlines need to make decisions about which routes are safe to operate and ensure that airborne aircraft land safely. The aim of this paper is to demonstrate the application of a statistical technique that best combines ash information from satellites and a suite of computer forecasts of ash concentration to provide a range of plausible estimates of how much volcanic ash emitted from a volcano is available to undergo long-range transport.
Jean-Pierre Chaboureau, Laurent Labbouz, Cyrille Flamant, and Alma Hodzic
Atmos. Chem. Phys., 22, 8639–8658, https://doi.org/10.5194/acp-22-8639-2022, https://doi.org/10.5194/acp-22-8639-2022, 2022
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Ground-based, spaceborne and rare airborne observations of biomass burning aerosols (BBAs) during the AEROCLO-sA field campaign in 2017 are complemented with convection-permitting simulations with online trajectories. The results show that the radiative effect of the BBA accelerates the southern African easterly jet and generates upward motions that transport the BBAs to higher altitudes and farther southwest.
Annika Drews, Wenjuan Huo, Katja Matthes, Kunihiko Kodera, and Tim Kruschke
Atmos. Chem. Phys., 22, 7893–7904, https://doi.org/10.5194/acp-22-7893-2022, https://doi.org/10.5194/acp-22-7893-2022, 2022
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Solar irradiance varies with a period of approximately 11 years. Using a unique large chemistry–climate model dataset, we investigate the solar surface signal in the North Atlantic and European region and find that it changes over time, depending on the strength of the solar cycle. For the first time, we estimate the potential predictability associated with including realistic solar forcing in a model. These results may improve seasonal to decadal predictions of European climate.
Shipra Jain, Ruth M. Doherty, David Sexton, Steven Turnock, Chaofan Li, Zixuan Jia, Zongbo Shi, and Lin Pei
Atmos. Chem. Phys., 22, 7443–7460, https://doi.org/10.5194/acp-22-7443-2022, https://doi.org/10.5194/acp-22-7443-2022, 2022
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We provide a range of future projections of winter haze and clear conditions over the North China Plain (NCP) using multiple simulations from a climate model for the high-emission scenario (RCP8.5). The frequency of haze conducive weather is likely to increase whereas the frequency of clear weather is likely to decrease in future. The total number of hazy days for a given winter can be as much as ˜3.5 times higher than the number of clear days over the NCP.
Antonio Capponi, Natalie J. Harvey, Helen F. Dacre, Keith Beven, Cameron Saint, Cathie Wells, and Mike R. James
Atmos. Chem. Phys., 22, 6115–6134, https://doi.org/10.5194/acp-22-6115-2022, https://doi.org/10.5194/acp-22-6115-2022, 2022
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Forecasts of the dispersal of volcanic ash in the atmosphere are hampered by uncertainties in parameters describing the characteristics of volcanic plumes. Uncertainty quantification is vital for making robust flight-planning decisions. We present a method using satellite data to refine a series of volcanic ash dispersion forecasts and quantify these uncertainties. We show how we can improve forecast accuracy and potentially reduce the regions of high risk of volcanic ash relevant to aviation.
Piyush Srivastava, Ian M. Brooks, John Prytherch, Dominic J. Salisbury, Andrew D. Elvidge, Ian A. Renfrew, and Margaret J. Yelland
Atmos. Chem. Phys., 22, 4763–4778, https://doi.org/10.5194/acp-22-4763-2022, https://doi.org/10.5194/acp-22-4763-2022, 2022
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The parameterization of surface turbulent fluxes over sea ice remains a weak point in weather forecast and climate models. Recent theoretical developments have introduced more extensive physics but these descriptions are poorly constrained due to a lack of observation data. Here we utilize a large dataset of measurements of turbulent fluxes over sea ice to tune the state-of-the-art parameterization of wind stress, and compare it with a previous scheme.
Yiqing Liu, Zhiwen Luo, and Sue Grimmond
Atmos. Chem. Phys., 22, 4721–4735, https://doi.org/10.5194/acp-22-4721-2022, https://doi.org/10.5194/acp-22-4721-2022, 2022
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Anthropogenic heat emission from buildings is important for atmospheric modelling in cities. The current building anthropogenic heat flux is simplified by building energy consumption. Our research proposes a novel approach to determine ‘real’ building anthropogenic heat emission from the changes in energy balance fluxes between occupied and unoccupied buildings. We hope to provide new insights into future parameterisations of building anthropogenic heat flux in urban climate models.
Lars Hoffmann and Reinhold Spang
Atmos. Chem. Phys., 22, 4019–4046, https://doi.org/10.5194/acp-22-4019-2022, https://doi.org/10.5194/acp-22-4019-2022, 2022
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We present an intercomparison of 2009–2018 lapse rate tropopause characteristics as derived from ECMWF's ERA5 and ERA-Interim reanalyses. Large-scale features are similar, but ERA5 shows notably larger variability, which we mainly attribute to UTLS temperature fluctuations due to gravity waves being better resolved by ECMWF's IFS forecast model. Following evaluation with radiosondes and GPS data, we conclude ERA5 will be a more suitable asset for tropopause-related studies in future work.
Linye Song, Shangfeng Chen, Wen Chen, Jianping Guo, Conglan Cheng, and Yong Wang
Atmos. Chem. Phys., 22, 1669–1688, https://doi.org/10.5194/acp-22-1669-2022, https://doi.org/10.5194/acp-22-1669-2022, 2022
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This study shows that in most years when haze pollution (HP) over the North China Plain (NCP) is more (less) serious in winter, air conditions in the following spring are also worse (better) than normal. Conversely, there are some years when HP in the following spring is opposed to that in winter. It is found that North Atlantic sea surface temperature (SST) anomalies play important roles in HP evolution over the NCP. Thus North Atlantic SST is an important preceding signal for NCP HP evolution.
Anna A. Shestakova, Dmitry G. Chechin, Christof Lüpkes, Jörg Hartmann, and Marion Maturilli
Atmos. Chem. Phys., 22, 1529–1548, https://doi.org/10.5194/acp-22-1529-2022, https://doi.org/10.5194/acp-22-1529-2022, 2022
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This article presents a comprehensive analysis of the easterly orographic wind episode which occurred over Svalbard on 30–31 May 2017. This wind caused a significant temperature rise on the lee side of the mountains and greatly intensified the snowmelt. This episode was investigated on the basis of measurements collected during the ACLOUD/PASCAL field campaigns with the help of numerical modeling.
Xiadong An, Lifang Sheng, Chun Li, Wen Chen, Yulian Tang, and Jingliang Huangfu
Atmos. Chem. Phys., 22, 725–738, https://doi.org/10.5194/acp-22-725-2022, https://doi.org/10.5194/acp-22-725-2022, 2022
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The North China Plain (NCP) suffered many periods of haze in winter during 1985–2015, related to the rainfall-induced diabatic heating over southern China. The haze over the NCP is modulated by an anomalous anticyclone caused by the Rossby wave and a north–south circulation (NSC) induced mainly by diabatic heating. As a Rossby wave source, rainfall-induced diabatic heating supports waves and finally strengthens the anticyclone over the NCP. These changes favor haze over the NCP.
Chenrui Diao, Yangyang Xu, and Shang-Ping Xie
Atmos. Chem. Phys., 21, 18499–18518, https://doi.org/10.5194/acp-21-18499-2021, https://doi.org/10.5194/acp-21-18499-2021, 2021
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Anthropogenic aerosol (AA) emission has shown a zonal redistribution since the 1980s, with a decline in the Western Hemisphere (WH) high latitudes and an increase in the Eastern Hemisphere (EH) low latitudes. This study compares the role of zonally asymmetric forcings affecting the climate. The WH aerosol reduction dominates the poleward shift of the Hadley cell and the North Pacific warming, while the EH AA forcing is largely confined to the emission domain and induces local cooling responses.
Francisco J. Pérez-Invernón, Heidi Huntrieser, Sergio Soler, Francisco J. Gordillo-Vázquez, Nicolau Pineda, Javier Navarro-González, Víctor Reglero, Joan Montanyà, Oscar van der Velde, and Nikos Koutsias
Atmos. Chem. Phys., 21, 17529–17557, https://doi.org/10.5194/acp-21-17529-2021, https://doi.org/10.5194/acp-21-17529-2021, 2021
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Lightning-ignited fires tend to occur in remote areas and can spread significantly before suppression. Long continuing current (LCC) lightning, preferably taking place in dry thunderstorms, is believed to be the main precursor of lightning-ignited fires. We analyze fire databases of lightning-ignited fires in the Mediterranean basin and report the shared meteorological conditions of fire- and LCC-lightning-producing thunderstorms. These results can be useful to improve fire forecasting methods.
Diego Aliaga, Victoria A. Sinclair, Marcos Andrade, Paulo Artaxo, Samara Carbone, Evgeny Kadantsev, Paolo Laj, Alfred Wiedensohler, Radovan Krejci, and Federico Bianchi
Atmos. Chem. Phys., 21, 16453–16477, https://doi.org/10.5194/acp-21-16453-2021, https://doi.org/10.5194/acp-21-16453-2021, 2021
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We investigate the origin of air masses sampled at Mount Chacaltaya, Bolivia. Three-quarters of the measured air has not been influenced by the surface in the previous 4 d. However, it is rare that, at any given time, the sampled air has not been influenced at all by the surface, and often the sampled air has multiple origins. The influence of the surface is more prevalent during day than night. Furthermore, during the 6-month study, one-third of the air masses originated from Amazonia.
Michael Biggart, Jenny Stocker, Ruth M. Doherty, Oliver Wild, David Carruthers, Sue Grimmond, Yiqun Han, Pingqing Fu, and Simone Kotthaus
Atmos. Chem. Phys., 21, 13687–13711, https://doi.org/10.5194/acp-21-13687-2021, https://doi.org/10.5194/acp-21-13687-2021, 2021
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Heat-related illnesses are of increasing concern in China given its rapid urbanisation and our ever-warming climate. We examine the relative impacts that land surface properties and anthropogenic heat have on the urban heat island (UHI) in Beijing using ADMS-Urban. Air temperature measurements and satellite-derived land surface temperatures provide valuable means of evaluating modelled spatiotemporal variations. This work provides critical information for urban planners and UHI mitigation.
Tobias Wolf, Lasse H. Pettersson, and Igor Esau
Atmos. Chem. Phys., 21, 12463–12477, https://doi.org/10.5194/acp-21-12463-2021, https://doi.org/10.5194/acp-21-12463-2021, 2021
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House heating by wood-burning stoves is cozy and needed in boreal cities, e.g., Bergen, Norway. But smoke (aerosols) from stoves may reduce urban air quality. It can be transported over long distance excessively polluting some neighborhoods. Who will suffer the most? Our modelling study looks at urban pollution in unprecedented meter-sized details tracing smoke pathways and turbulent dispersion in a typical city. We prototype effective policy scenarios to mitigate urban air quality problems.
Piotr Sekuła, Anita Bokwa, Jakub Bartyzel, Bogdan Bochenek, Łukasz Chmura, Michał Gałkowski, and Mirosław Zimnoch
Atmos. Chem. Phys., 21, 12113–12139, https://doi.org/10.5194/acp-21-12113-2021, https://doi.org/10.5194/acp-21-12113-2021, 2021
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The wind shear generated on a local scale by the diversified relief’s impact can be a factor which significantly modifies the spatial pattern of PM10 concentration. The vertical profile of PM10 over a city located in a large valley during the events with high surface-level PM10 concentrations may show a sudden decrease with height not only due to the increase in wind speed, but also due to the change in wind direction alone. Vertical aerosanitary urban zones can be distinguished.
Jangho Lee, Jeffrey C. Mast, and Andrew E. Dessler
Atmos. Chem. Phys., 21, 11889–11904, https://doi.org/10.5194/acp-21-11889-2021, https://doi.org/10.5194/acp-21-11889-2021, 2021
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This paper investigates the impact of global warming on heat and humidity extremes. There are three major findings in this study. We quantify how unforced variability in the climate impacts can lead to large variations where heat waves occur, we find that all heat extremes increase as the climate warms, especially between 1.5 and 2.0 °C of the average global warming, and we show that the economic inequity of facing extreme heat will worsen in a warmer world.
Hyunju Jung, Ann Kristin Naumann, and Bjorn Stevens
Atmos. Chem. Phys., 21, 10337–10345, https://doi.org/10.5194/acp-21-10337-2021, https://doi.org/10.5194/acp-21-10337-2021, 2021
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We analyze the behavior of organized convection in a large-scale flow by imposing a mean flow to idealized simulations. In the mean flow, organized convection initially propagates slower than the mean wind speed and becomes stationary. The initial upstream and downstream difference in surface fluxes becomes symmetric as the surface momentum flux acts as a drag, resulting in the stationarity. Meanwhile, the surface enthalpy flux has a minor role in the propagation of the convection.
Xueling Liu, Arthur P. Mizzi, Jeffrey L. Anderson, Inez Fung, and Ronald C. Cohen
Atmos. Chem. Phys., 21, 9573–9583, https://doi.org/10.5194/acp-21-9573-2021, https://doi.org/10.5194/acp-21-9573-2021, 2021
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Observations of winds in the planetary boundary layer remain sparse, making it challenging to simulate and predict the atmospheric conditions that are most important for describing and predicting urban air quality. Here we investigate the application of data assimilation of NO2 columns as will be observed from geostationary orbit to improve predictions and retrospective analysis of wind fields in the boundary layer.
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Short summary
We introduce system identification techniques to climate science wherein multiple dynamic input–output relationships can be simultaneously characterized in a single simulation. This method, involving multiple small perturbations (in space and time) of an input field while monitoring output fields to quantify responses, allows for identification of different timescales of climate response to forcing without substantially pushing the climate far away from a steady state.
We introduce system identification techniques to climate science wherein multiple dynamic...
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