Articles | Volume 22, issue 22
https://doi.org/10.5194/acp-22-15135-2022
https://doi.org/10.5194/acp-22-15135-2022
Research article
 | 
28 Nov 2022
Research article |  | 28 Nov 2022

Enhanced sulfur in the upper troposphere and lower stratosphere in spring 2020

Laura Tomsche, Andreas Marsing, Tina Jurkat-Witschas, Johannes Lucke, Stefan Kaufmann, Katharina Kaiser, Johannes Schneider, Monika Scheibe, Hans Schlager, Lenard Röder, Horst Fischer, Florian Obersteiner, Andreas Zahn, Martin Zöger, Jos Lelieveld, and Christiane Voigt

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Cited articles

Arnold, F., Schneider, J., Gollinger, K., Schlager, H., Schulte, P., Hagen, D. E., Whitefield, P. D., and van Velthoven, P.: Observation of upper tropospheric sulfur dioxide- and acetone-pollution: Potential implications for hydroxyl radicaland aerosol formation, Geophys. Res. Lett., 24, 57–60, https://doi.org/10.1029/96gl03693, 1997. 
Brock, C., Hamill, P., Wilson, J., Jonsson, H., and Chan, K.: Particle formation in the upper tropical troposphere: A source of nuclei for the stratospheric aerosol, Science, 270, 1650–1653, 1995. 
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Short summary
The detection of sulfur compounds in the upper troposphere (UT) and lower stratosphere (LS) is a challenge. In-flight measurements of SO2 and sulfate aerosol were performed during the BLUESKY mission in spring 2020 under exceptional atmospheric conditions. Reduced sinks in the dry UTLS and lower but still significant air traffic influenced the enhanced SO2 in the UT, and aged volcanic plumes enhanced the LS sulfate aerosol impacting the atmospheric radiation budget and global climate.
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