Articles | Volume 18, issue 15
https://doi.org/10.5194/acp-18-11471-2018
https://doi.org/10.5194/acp-18-11471-2018
Research article
 | 
15 Aug 2018
Research article |  | 15 Aug 2018

Characterization of aerosol composition, aerosol acidity, and organic acid partitioning at an agriculturally intensive rural southeastern US site

Theodora Nah, Hongyu Guo, Amy P. Sullivan, Yunle Chen, David J. Tanner, Athanasios Nenes, Armistead Russell, Nga Lee Ng, L. Gregory Huey, and Rodney J. Weber

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Cited articles

Barbier Jr., J. and Duprez, D.: Steam Effects in 3-way catalysis, Appl. Catal. B-Environ., 4, 105–140, https://doi.org/10.1016/0926-3373(94)80046-4, 1994. 
Bertram, A. K., Martin, S. T., Hanna, S. J., Smith, M. L., Bodsworth, A., Chen, Q., Kuwata, M., Liu, A., You, Y., and Zorn, S. R.: Predicting the relative humidities of liquid-liquid phase separation, efflorescence, and deliquescence of mixed particles of ammonium sulfate, organic material, and water using the organic-to-sulfate mass ratio of the particle and the oxygen-to-carbon elemental ratio of the organic component, Atmos. Chem. Phys., 11, 10995–11006, https://doi.org/10.5194/acp-11-10995-2011, 2011. 
Blanchard, C. L., Hidy, G. M., Tanenbaum, S., and Edgerton, E. S.: NMOC, ozone, and organic aerosol in the southeastern United States, 1999–2007: 3. Origins of organic aerosol in Atlanta, Georgia, and surrounding areas, Atmos. Environ., 45, 1291–1302, https://doi.org/10.1016/j.atmosenv.2010.12.004, 2011. 
Blanchard, C. L., Hidy, G. M., Tanenbaum, S., Edgerton, E. S., and Hartsell, B. E.: The Southeastern Aerosol Research and Characterization (SEARCH) study: Spatial variations and chemical climatology, 1999–2010, J. Air Waste Manage., 63, 260–275, https://doi.org/10.1080/10962247.2012.749816, 2013a. 
Blanchard, C. L., Hidy, G. M., Tanenbaum, S., Edgerton, E. S., and Hartsell, B. E.: The Southeastern Aerosol Research and Characterization (SEARCH) study: Temporal trends in gas and PM concentrations and composition, 1999–2010, J. Air Waste Manage., 63, 247–259, https://doi.org/10.1080/10962247.2012.748523, 2013b. 
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We present measurements from a field study conducted in an agriculturally intensive region in the southeastern US during the fall of 2016 to investigate how NH3 affects particle acidity and SOA formation via gas–particle partitioning of semi-volatile organic acids. For this study, higher NH3 concentrations relative to what has been measured in the region in previous studies had minor effects on PM1 organic acids and their influence on the overall organic aerosol and PM1 mass concentrations.
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