Articles | Volume 21, issue 3
https://doi.org/10.5194/acp-21-2067-2021
https://doi.org/10.5194/acp-21-2067-2021
Research article
 | 
11 Feb 2021
Research article |  | 11 Feb 2021

High-resolution hybrid inversion of IASI ammonia columns to constrain US ammonia emissions using the CMAQ adjoint model

Yilin Chen, Huizhong Shen, Jennifer Kaiser, Yongtao Hu, Shannon L. Capps, Shunliu Zhao, Amir Hakami, Jhih-Shyang Shih, Gertrude K. Pavur, Matthew D. Turner, Daven K. Henze, Jaroslav Resler, Athanasios Nenes, Sergey L. Napelenok, Jesse O. Bash, Kathleen M. Fahey, Gregory R. Carmichael, Tianfeng Chai, Lieven Clarisse, Pierre-François Coheur, Martin Van Damme, and Armistead G. Russell

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Cited articles

Appel, K. W., Foley, K. M., Bash, J. O., Pinder, R. W., Dennis, R. L., Allen, D. J., and Pickering, K.: A multi-resolution assessment of the Community Multiscale Air Quality (CMAQ) model v4.7 wet deposition estimates for 2002–2006, Geosci. Model Dev., 4, 357–371, https://doi.org/10.5194/gmd-4-357-2011, 2011. 
Bash, J. O., Cooter, E. J., Dennis, R. L., Walker, J. T., and Pleim, J. E.: Evaluation of a regional air-quality model with bidirectional NH3 exchange coupled to an agroecosystem model, Biogeosciences, 10, 1635–1645, https://doi.org/10.5194/bg-10-1635-2013, 2013. 
Bobbink, R. and Hicks, W. K.: Factors affecting nitrogen deposition impacts on biodiversity: an overview, in: Nitrogen deposition, critical loads and biodiversity, edited by: Sutton, M. A., Mason, K. E., Sheppard, L. J., Sverdrup, H., Haeuber, R., and Hicks, W. K., Springer Netherlands, Dordrecht, 127–138, 2014. 
Brasseur, G. P. and Jacob, D. J.: Modeling of atmospheric chemistry, Cambridge University Press, Cambridge, UK, 520–525, 2017. 
Byrd, R. H., Lu, P., Nocedal, J., and Zhu, C.: A limited memory algorithm for bound constrained optimization, SIAM J. Sci. Comput., 16, 1190–1208, https://doi.org/10.1137/0916069, 1995. 
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Ammonia (NH3) emissions can exert adverse impacts on air quality and ecosystem well-being. NH3 emission inventories are viewed as highly uncertain. Here we optimize the NH3 emission estimates in the US using an air quality model and NH3 measurements from the IASI satellite instruments. The optimized NH3 emissions are much higher than the National Emissions Inventory estimates in April. The optimized NH3 emissions improved model performance when evaluated against independent observation.
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