Articles | Volume 17, issue 19
https://doi.org/10.5194/acp-17-11971-2017
https://doi.org/10.5194/acp-17-11971-2017
Research article
 | 
10 Oct 2017
Research article |  | 10 Oct 2017

Source attribution of Arctic black carbon constrained by aircraft and surface measurements

Jun-Wei Xu, Randall V. Martin, Andrew Morrow, Sangeeta Sharma, Lin Huang, W. Richard Leaitch, Julia Burkart, Hannes Schulz, Marco Zanatta, Megan D. Willis, Daven K. Henze, Colin J. Lee, Andreas B. Herber, and Jonathan P. D. Abbatt

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Cited articles

AMAP: The Impact of Black Carbon on Arctic Climate, edited by: Quinn, P. K., Stohl, A., Arneth, A., Berntsen, T., Burkhart, J. F., Christensen, J., Flanner, M., Kupiainen, K., Lihavainen, H., Shepherd, M., Shevchenko, V., Skov, H., and Vestreng, V., Arctic Monitoring and Assessment Programme (AMAP), Oslo, 72 pp., 2011.
AMAP: AMAP Assessment 2015: Black Carbon and Ozone as Arctic Climate Forcers, Arctic Monitoring and Assessment Programme (AMAP), Oslo, Norway, 2015.
Barrett, T. E., Robinson, E. M., Usenko, S., and Sheesley, R. J.: Source contributions to wintertime elemental and organic carbon in the Western Arctic based on radiocarbon and tracer apportionment, Environ. Sci. Technol., 49, 11631–11639, https://doi.org/10.1021/acs.est.5b03081, 2015.
Bond, T. C. and Bergstrom, R. W.: Light absorption by carbonaceous particles: an investigative review, Aerosol Sci. Tech., 40, 27–67, https://doi.org/10.1080/02786820500421521, 2006.
Bond, T. C., Anderson, T. L., and Campbell, D.: Calibration and intercomparison of filter-based measurements of visible light absorption by aerosols, Aerosol Sci. Tech., 30, 582–600, https://doi.org/10.1080/027868299304435, 1999.
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We interpret a series of recent airborne and ground-based measurements with the GEOS-Chem model and its adjoint to attribute the sources of Arctic BC. Anthropogenic emissions in eastern and southern Asia make the largest contribution to Arctic BC. Gas flaring emissions from oilfields in western Siberia and from the Tarim oilfield in western China could have striking impacts on Arctic BC loadings.
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