Articles | Volume 15, issue 20
https://doi.org/10.5194/acp-15-11753-2015
https://doi.org/10.5194/acp-15-11753-2015
Research article
 | 
22 Oct 2015
Research article |  | 22 Oct 2015

Modelling marine emissions and atmospheric distributions of halocarbons and dimethyl sulfide: the influence of prescribed water concentration vs. prescribed emissions

S. T. Lennartz, G. Krysztofiak, C. A. Marandino, B.-M. Sinnhuber, S. Tegtmeier, F. Ziska, R. Hossaini, K. Krüger, S. A. Montzka, E. Atlas, D. E. Oram, T. Keber, H. Bönisch, and B. Quack

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Cited articles

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Asher, W. E. and Wanninkhof, R.: The effect of bubble-mediated gas transfer on purposeful dual-gaseous tracer experiments, J. Geophys. Res.-Oceans, 103, 10555–10560, https://doi.org/10.1029/98jc00245, 1998.
Ayers, G. P., Bentley, S. T., Ivey, J. P., and Forgan, B. W.: Dimethylsulfide in marine air at cape grim, 41° s, J. Geophysical Res.-Atmos., 100, 21013–21021, https://doi.org/10.1029/95jd02144, 1995.
Barnes, I., Hjorth, J., and Mihalopoulos, N.: Dimethyl sulfide and dimethyl sulfoxide and their oxidation in the atmosphere, Chemical Rev., 106, 940–975, https://doi.org/10.1021/cr020529+, 2006.
Bates, T. S., Lamb, B. K., Guenther, A., Dignon, J., and Stoiber, R. E.: Sulfur emissions to the atmosphere from natural sources, J. Atmos. Chem., 14, 315–337, https://doi.org/10.1007/bf00115242, 1992.
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Short summary
Marine-produced short-lived trace gases such as halocarbons and DMS significantly impact atmospheric chemistry. To assess this impact on ozone depletion and the radiative budget, it is critical that their marine emissions in atmospheric chemistry models are quantified as accurately as possible. We show that calculating emissions online with an interactive atmosphere improves the agreement with current observations and should be employed regularly in models where marine sources are important.
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