Articles | Volume 24, issue 1
https://doi.org/10.5194/acp-24-689-2024
https://doi.org/10.5194/acp-24-689-2024
Research article
 | 
17 Jan 2024
Research article |  | 17 Jan 2024

The interhemispheric gradient of SF6 in the upper troposphere

Tanja J. Schuck, Johannes Degen, Eric Hintsa, Peter Hoor, Markus Jesswein, Timo Keber, Daniel Kunkel, Fred Moore, Florian Obersteiner, Matt Rigby, Thomas Wagenhäuser, Luke M. Western, Andreas Zahn, and Andreas Engel

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Cited articles

Belikov, D. A., Saitoh, N., and Patra, P. K.: An Analysis of Interhemispheric Transport Pathways Based on Three-Dimensional Methane Data by GOSAT Observations and Model Simulations, J. Geophys. Res.-Atmos., 127, e2021JD035688, https://doi.org/10.1029/2021JD035688, 2022. a, b
Bischof, W., Borchers, R., Fabian, P., and Krüger, B.: Increased concentration and vertical distribution of carbon dioxide in the stratosphere, Nature, 316, 708–710, https://doi.org/10.1038/316708a0, 1985. a
Bönisch, H., Engel, A., Birner, Th., Hoor, P., Tarasick, D. W., and Ray, E. A.: On the structural changes in the Brewer-Dobson circulation after 2000, Atmos. Chem. Phys., 11, 3937–3948, https://doi.org/10.5194/acp-11-3937-2011, 2011. a
Brenninkmeijer, C. A. M., Crutzen, P., Boumard, F., Dauer, T., Dix, B., Ebinghaus, R., Filippi, D., Fischer, H., Franke, H., Frieβ, U., Heintzenberg, J., Helleis, F., Hermann, M., Kock, H. H., Koeppel, C., Lelieveld, J., Leuenberger, M., Martinsson, B. G., Miemczyk, S., Moret, H. P., Nguyen, H. N., Nyfeler, P., Oram, D., O'Sullivan, D., Penkett, S., Platt, U., Pupek, M., Ramonet, M., Randa, B., Reichelt, M., Rhee, T. S., Rohwer, J., Rosenfeld, K., Scharffe, D., Schlager, H., Schumann, U., Slemr, F., Sprung, D., Stock, P., Thaler, R., Valentino, F., van Velthoven, P., Waibel, A., Wandel, A., Waschitschek, K., Wiedensohler, A., Xueref-Remy, I., Zahn, A., Zech, U., and Ziereis, H.: Civil Aircraft for the regular investigation of the atmosphere based on an instrumented container: The new CARIBIC system, Atmos. Chem. Phys., 7, 4953–4976, https://doi.org/10.5194/acp-7-4953-2007, 2007. a
Chen, G., Orbe, C., and Waugh, D.: The role of monsoon-like zonally asymmetric heating in interhemispheric transport, J. Geophys. Res.-Atmos., 122, 3282–3298, https://doi.org/10.1002/2016JD026427, 2017. a
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We study the interhemispheric gradient of sulfur hexafluoride (SF6), a strong long-lived greenhouse gas. Its emissions are stronger in the Northern Hemisphere; therefore, mixing ratios in the Southern Hemisphere lag behind. Comparing the observations to a box model, the model predicts air in the Southern Hemisphere to be older. For a better agreement, the emissions used as model input need to be increased (and their spatial pattern changed), and we need to modify north–south transport.
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