Articles | Volume 21, issue 7
https://doi.org/10.5194/acp-21-5499-2021
https://doi.org/10.5194/acp-21-5499-2021
Research article
 | 
08 Apr 2021
Research article |  | 08 Apr 2021

Formation of nighttime sulfuric acid from the ozonolysis of alkenes in Beijing

Yishuo Guo, Chao Yan, Chang Li, Wei Ma, Zemin Feng, Ying Zhou, Zhuohui Lin, Lubna Dada, Dominik Stolzenburg, Rujing Yin, Jenni Kontkanen, Kaspar R. Daellenbach, Juha Kangasluoma, Lei Yao, Biwu Chu, Yonghong Wang, Runlong Cai, Federico Bianchi, Yongchun Liu, and Markku Kulmala

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Cited articles

Aalto, P., Hämeri, K., Becker, E., Weber, R., Salm, J., Mäkelä, J. M., Hoell, C., O'dowd, C. D., Hansson, H.-C., Väkevä, M., Koponen, I. K., Buzorius, G., and Kulmala, M.: Physical characterization of aerosol particles during nucleation events, Tellus B, 53, 344–358, https://doi.org/10.3402/tellusb.v53i4.17127, 2001. 
Ahn, J. Y., Okerlund, R., Fry, A., and Eddings, E. G.: Sulfur trioxide formation during oxy-coal combustion, Int. J. Greenh. Gas Con., 5, 127–135, https://doi.org/10.1016/j.ijggc.2011.05.009, 2011. 
Armendariz, A. J. and Leith, D.: Concentration measurement and counting efficiency for the aerodynamic particle sizer 3320, J. Aerosol Sci., 33, 133–148, https://doi.org/10.1016/S0021-8502(01)00152-5, 2002. 
Arnold, F., Pirjola, L., Aufmhoff, H., Schuck, T., Lahde, T., and Hameri, K.: First gaseous sulfuric acid measurements in automobile exhaust: Implications for volatile nanoparticle formation, Atmos. Environ., 40, 7097–7105, https://doi.org/10.1016/j.atmosenv.2006.06.038, 2006. 
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Short summary
Fog, cloud and haze are very common natural phenomena. Sulfuric acid (SA) is one of the key compounds forming those suspended particles, technically called aerosols, through gas-to-particle conversion. Therefore, the concentration level, source and sink of SA is very important. Our results show that ozonolysis of alkenes plays a major role in nighttime SA formation under unpolluted conditions in urban Beijing, and nighttime cluster mode particles are probably driven by SA in urban environments.
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