Articles | Volume 17, issue 5
https://doi.org/10.5194/acp-17-3233-2017
https://doi.org/10.5194/acp-17-3233-2017
Research article
 | 
06 Mar 2017
Research article |  | 06 Mar 2017

Sources and formation mechanisms of carbonaceous aerosol at a regional background site in the Netherlands: insights from a year-long radiocarbon study

Ulrike Dusek, Regina Hitzenberger, Anne Kasper-Giebl, Magdalena Kistler, Harro A. J. Meijer, Sönke Szidat, Lukas Wacker, Rupert Holzinger, and Thomas Röckmann

Related authors

Aerosol optical properties within the atmospheric boundary layer predicted from ground-based observations compared to Raman lidar retrievals during RITA-2021
Xinya Liu, Diego Alves Gouveia, Bas Henzing, Arnoud Apituley, Arjan Hensen, Danielle van Dinther, Rujin Huang, and Ulrike Dusek
Atmos. Chem. Phys., 24, 9597–9614, https://doi.org/10.5194/acp-24-9597-2024,https://doi.org/10.5194/acp-24-9597-2024, 2024
Short summary
Measurement report: Evaluation of the TOF-ACSM-CV for PM1.0 and PM2.5 measurements during the RITA-2021 field campaign
Xinya Liu, Bas Henzing, Arjan Hensen, Jan Mulder, Peng Yao, Danielle van Dinther, Jerry van Bronckhorst, Rujin Huang, and Ulrike Dusek
Atmos. Chem. Phys., 24, 3405–3420, https://doi.org/10.5194/acp-24-3405-2024,https://doi.org/10.5194/acp-24-3405-2024, 2024
Short summary
What chemical species are responsible for new particle formation and growth in the Netherlands? A hybrid positive matrix factorization (PMF) analysis using aerosol composition (ACSM) and size (SMPS)
Farhan R. Nursanto, Roy Meinen, Rupert Holzinger, Maarten C. Krol, Xinya Liu, Ulrike Dusek, Bas Henzing, and Juliane L. Fry
Atmos. Chem. Phys., 23, 10015–10034, https://doi.org/10.5194/acp-23-10015-2023,https://doi.org/10.5194/acp-23-10015-2023, 2023
Short summary
A quadcopter unmanned aerial system (UAS)-based methodology for measuring biomass burning emission factors
Roland Vernooij, Patrik Winiger, Martin Wooster, Tercia Strydom, Laurent Poulain, Ulrike Dusek, Mark Grosvenor, Gareth J. Roberts, Nick Schutgens, and Guido R. van der Werf
Atmos. Meas. Tech., 15, 4271–4294, https://doi.org/10.5194/amt-15-4271-2022,https://doi.org/10.5194/amt-15-4271-2022, 2022
Short summary
Stable carbon isotopic composition of biomass burning emissions – implications for estimating the contribution of C3 and C4 plants
Roland Vernooij, Ulrike Dusek, Maria Elena Popa, Peng Yao, Anupam Shaikat, Chenxi Qiu, Patrik Winiger, Carina van der Veen, Thomas Callum Eames, Natasha Ribeiro, and Guido R. van der Werf
Atmos. Chem. Phys., 22, 2871–2890, https://doi.org/10.5194/acp-22-2871-2022,https://doi.org/10.5194/acp-22-2871-2022, 2022
Short summary

Related subject area

Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Measurement report: In situ vertical profiles of below-cloud aerosol over the central Greenland Ice Sheet
Heather Guy, Andrew S. Martin, Erik Olson, Ian M. Brooks, and Ryan R. Neely III
Atmos. Chem. Phys., 24, 11103–11114, https://doi.org/10.5194/acp-24-11103-2024,https://doi.org/10.5194/acp-24-11103-2024, 2024
Short summary
Occurrence, abundance, and formation of atmospheric tarballs from a wide range of wildfires in the western US
Kouji Adachi, Jack E. Dibb, Joseph M. Katich, Joshua P. Schwarz, Hongyu Guo, Pedro Campuzano-Jost, Jose L. Jimenez, Jeff Peischl, Christopher D. Holmes, and James Crawford
Atmos. Chem. Phys., 24, 10985–11004, https://doi.org/10.5194/acp-24-10985-2024,https://doi.org/10.5194/acp-24-10985-2024, 2024
Short summary
Measurement report: Contribution of atmospheric new particle formation to ultrafine particle concentration, cloud condensation nuclei, and radiative forcing – results from 5-year observations in central Europe
Jia Sun, Markus Hermann, Kay Weinhold, Maik Merkel, Wolfram Birmili, Yifan Yang, Thomas Tuch, Harald Flentje, Björn Briel, Ludwig Ries, Cedric Couret, Michael Elsasser, Ralf Sohmer, Klaus Wirtz, Frank Meinhardt, Maik Schütze, Olaf Bath, Bryan Hellack, Veli-Matti Kerminen, Markku Kulmala, Nan Ma, and Alfred Wiedensohler
Atmos. Chem. Phys., 24, 10667–10687, https://doi.org/10.5194/acp-24-10667-2024,https://doi.org/10.5194/acp-24-10667-2024, 2024
Short summary
Simulated contrail-processed aviation soot aerosols are poor ice-nucleating particles at cirrus temperatures
Baptiste Testa, Lukas Durdina, Jacinta Edebeli, Curdin Spirig, and Zamin A. Kanji
Atmos. Chem. Phys., 24, 10409–10424, https://doi.org/10.5194/acp-24-10409-2024,https://doi.org/10.5194/acp-24-10409-2024, 2024
Short summary
Biological and dust aerosols as sources of ice-nucleating particles in the eastern Mediterranean: source apportionment, atmospheric processing and parameterization
Kunfeng Gao, Franziska Vogel, Romanos Foskinis, Stergios Vratolis, Maria I. Gini, Konstantinos Granakis, Anne-Claire Billault-Roux, Paraskevi Georgakaki, Olga Zografou, Prodromos Fetfatzis, Alexis Berne, Alexandros Papayannis, Konstantinos Eleftheridadis, Ottmar Möhler, and Athanasios Nenes
Atmos. Chem. Phys., 24, 9939–9974, https://doi.org/10.5194/acp-24-9939-2024,https://doi.org/10.5194/acp-24-9939-2024, 2024
Short summary

Cited articles

Aiken, A. C., de Foy, B., Wiedinmyer, C., DeCarlo, P. F., Ulbrich, I. M., Wehrli, M. N., Szidat, S., Prévôt, A. S. H., Noda, J., Wacker, L., Volkamer, R., Fortner, E., Wang, J., Laskin, A., Shutthanandan, V., Zheng, J., Zhang, R., Paredes-Miranda, G., Arnott, W. P., Molina, L. T., Sosa, G., Querol, X., and Jimenez, J. L.: Mexico city aerosol analysis during MILAGRO using high resolution aerosol mass spectrometry at the urban supersite (T0) – Part 2: Analysis of the biomass burning contribution and the non-fossil carbon fraction, Atmos. Chem. Phys., 10, 5315–5341, https://doi.org/10.5194/acp-10-5315-2010, 2010.
Allan, J. D., Williams, P. I., Morgan, W. T., Martin, C. L., Flynn, M. J., Lee, J., Nemitz, E., Phillips, G. J., Gallagher, M. W., and Coe, H.: Contributions from transport, solid fuel burning and cooking to primary organic aerosols in two UK cities, Atmos. Chem. Phys., 10, 647–668, https://doi.org/10.5194/acp-10-647-2010, 2010.
Bench, G.: Measurement of Contemporary and Fossil Carbon Contents of PM Aerosols?: Results from Turtleback Dome, Yosemite National Park, Enviorn. Sci. Technol., 38, 2424–2427, 2004.
Bennett, M., Volckens, J., Stanglmaier, R., McNichol, A. P., Ellenson, W. D., and Lewis, C. W.: Biodiesel effects on particulate radiocarbon (14C) emissions from a diesel engine, J. Aerosol Sci., 39, 667–678, 2008.
Bernardoni, V., Calzolai, G., Chiari, M., Fedi, M., Lucarelli, F., Nava, S., Piazzalunga, A., Riccobono, F., Taccetti, F., Valli, G., and Vecchi, R.: Radiocarbon analysis on organic and elemental carbon in aerosol samples and source apportionment at an urban site in Northern Italy, J. Aerosol Sci., 56, 88–99, 2013.
Download
Short summary
Measurements of the radioactive carbon isotope 14C allow to identify the sources of aerosol carbon. We report an extensive 14C source apportionment record in the Netherlands with samples covering a whole year. We discovered that long-range transport has a large influence on aerosol carbon levels. Fossil fuel carbon is least influenced by long-range transport and more regional in origin. Biomass burning seems to be a minor source of aerosol carbon in the Netherlands.
Altmetrics
Final-revised paper
Preprint