Articles | Volume 14, issue 15
https://doi.org/10.5194/acp-14-7909-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-14-7909-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
11 Aug 2014
Research article |
| 11 Aug 2014
Long-term MAX-DOAS network observations of NO2 in Russia and Asia (MADRAS) during the period 2007–2012: instrumentation, elucidation of climatology, and comparisons with OMI satellite observations and global model simulations
Y. Kanaya
Department of Environmental Geochemical Cycle Research, Japan Agency for Marine-Earth Science and Technology, Yokohama 2360001, Japan
H. Irie
Department of Environmental Geochemical Cycle Research, Japan Agency for Marine-Earth Science and Technology, Yokohama 2360001, Japan
now at: Chiba University, Chiba 2638522, Japan
H. Takashima
Department of Environmental Geochemical Cycle Research, Japan Agency for Marine-Earth Science and Technology, Yokohama 2360001, Japan
now at: Fukuoka University, Fukuoka 8140180, Japan
H. Iwabuchi
Department of Environmental Geochemical Cycle Research, Japan Agency for Marine-Earth Science and Technology, Yokohama 2360001, Japan
now at: Tohoku University, Sendai 9808578, Japan
H. Akimoto
Department of Environmental Geochemical Cycle Research, Japan Agency for Marine-Earth Science and Technology, Yokohama 2360001, Japan
now at: Asia Center for Air Pollution Research, Niigata 9502144, Japan
Nagoya University, Nagoya 4648601, Japan
M. Gu
Gwangju Institute of Science and Technology (GIST), Gwangju 500712, Korea
J. Chong
Gwangju Institute of Science and Technology (GIST), Gwangju 500712, Korea
Y. J. Kim
Gwangju Institute of Science and Technology (GIST), Gwangju 500712, Korea
H. Lee
Gwangju Institute of Science and Technology (GIST), Gwangju 500712, Korea
now at: Pukyong National University, Pusan 608737, Korea
A. Li
Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei 230031, China
F. Si
Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei 230031, China
J. Xu
Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei 230031, China
P.-H. Xie
Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei 230031, China
W.-Q. Liu
Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei 230031, China
A. Dzhola
A. M. Obukhov Institute of Atmospheric Physics, Russian Academy of Sciences, Moscow 119017, Russia
O. Postylyakov
A. M. Obukhov Institute of Atmospheric Physics, Russian Academy of Sciences, Moscow 119017, Russia
V. Ivanov
A. M. Obukhov Institute of Atmospheric Physics, Russian Academy of Sciences, Moscow 119017, Russia
now at: National Ozone Monitoring Research and Educational Center of Belarusian State University (NOMREC BSU), Minsk 220064, Belarus
E. Grechko
A. M. Obukhov Institute of Atmospheric Physics, Russian Academy of Sciences, Moscow 119017, Russia
S. Terpugova
V. E. Zuev Institute of Atmospheric Optics, Siberian Branch of the Russian Academy of Sciences, Tomsk 634021, Russia
M. Panchenko
V. E. Zuev Institute of Atmospheric Optics, Siberian Branch of the Russian Academy of Sciences, Tomsk 634021, Russia
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Sho Ohata, Tatsuhiro Mori, Yutaka Kondo, Sangeeta Sharma, Antti Hyvärinen, Elisabeth Andrews, Peter Tunved, Eija Asmi, John Backman, Henri Servomaa, Daniel Veber, Makoto Koike, Yugo Kanaya, Atsushi Yoshida, Nobuhiro Moteki, Yongjing Zhao, Junji Matsushita, and Naga Oshima
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-1190, https://doi.org/10.5194/acp-2020-1190, 2020
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Yongjoo Choi, Yugo Kanaya, Masayuki Takigawa, Chunmao Zhu, Seung-Myung Park, Atsushi Matsuki, Yasuhiro Sadanaga, Sang-Woo Kim, Xiaole Pan, and Ignacio Pisso
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Kazuyuki Miyazaki, Kevin Bowman, Takashi Sekiya, Henk Eskes, Folkert Boersma, Helen Worden, Nathaniel Livesey, Vivienne H. Payne, Kengo Sudo, Yugo Kanaya, Masayuki Takigawa, and Koji Ogochi
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Mengyao Liu, Jintai Lin, Hao Kong, K. Folkert Boersma, Henk Eskes, Yugo Kanaya, Qin He, Xin Tian, Kai Qin, Pinhua Xie, Robert Spurr, Ruijing Ni, Yingying Yan, Hongjian Weng, and Jingxu Wang
Atmos. Meas. Tech., 13, 4247–4259, https://doi.org/10.5194/amt-13-4247-2020, https://doi.org/10.5194/amt-13-4247-2020, 2020
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Nitrogen oxides (NOx = NO + NO2) are important air pollutants in the troposphere and play crucial roles in the formation of ozone and particulate matter. The recently launched TROPOspheric Monitoring Instrument (TROPOMI) provides an opportunity to retrieve tropospheric concentrations of nitrogen dioxide (NO2) at an unprecedented high horizontal resolution. This work presents a new NO2 retrieval product over East Asia and further quantifies key factors affecting the retrieval, including aerosol.
Yugo Kanaya, Kazuyo Yamaji, Takuma Miyakawa, Fumikazu Taketani, Chunmao Zhu, Yongjoo Choi, Yuichi Komazaki, Kohei Ikeda, Yutaka Kondo, and Zbigniew Klimont
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Chunmao Zhu, Yugo Kanaya, Masayuki Takigawa, Kohei Ikeda, Hiroshi Tanimoto, Fumikazu Taketani, Takuma Miyakawa, Hideki Kobayashi, and Ignacio Pisso
Atmos. Chem. Phys., 20, 1641–1656, https://doi.org/10.5194/acp-20-1641-2020, https://doi.org/10.5194/acp-20-1641-2020, 2020
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Black carbon is believed to be one of the causes of the rapid warming and glacier melting in the Arctic. The results of our study show that processes associated with the petroleum industry, such as gas flaring in Russia, are the main BC source at the Arctic surface. Emissions in East Asia are the main BC sources at high altitudes in the Arctic. Wildfires in Siberia, Alaska, and Canada are another important Arctic BC source in summer.
Yongjoo Choi, Yugo Kanaya, Seung-Myung Park, Atsushi Matsuki, Yasuhiro Sadanaga, Sang-Woo Kim, Itsushi Uno, Xiaole Pan, Meehye Lee, Hyunjae Kim, and Dong Hee Jung
Atmos. Chem. Phys., 20, 83–98, https://doi.org/10.5194/acp-20-83-2020, https://doi.org/10.5194/acp-20-83-2020, 2020
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The relationship between black carbon (BC) and carbon monoxide (CO) can differ by the different structure of fuel consumption. By investigating the representativeness of the BC and CO emission inventory for real-world comparison with reliable observations, this study suggested that accurate CO emissions should be preferentially investigated to enhance the accuracy of the BC emission rate over East Asia.
Yugo Kanaya, Kazuyuki Miyazaki, Fumikazu Taketani, Takuma Miyakawa, Hisahiro Takashima, Yuichi Komazaki, Xiaole Pan, Saki Kato, Kengo Sudo, Takashi Sekiya, Jun Inoue, Kazutoshi Sato, and Kazuhiro Oshima
Atmos. Chem. Phys., 19, 7233–7254, https://doi.org/10.5194/acp-19-7233-2019, https://doi.org/10.5194/acp-19-7233-2019, 2019
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Ozone and carbon monoxide levels were uniquely observed (for > 10 000 h) over oceans from 67° S to 75° N. Tropospheric chemistry reanalysis v2 reproduced the observed evolution of pollution plumes from continents but underpredicted and overpredicted ozone levels in the Arctic and in the western Pacific equatorial region, respectively. Processes to explain the gaps are proposed, including halogen-mediated destruction in the low latitudes. Our open data set will complement the TOAR data collection.
Wenfu Tang, Avelino F. Arellano, Joshua P. DiGangi, Yonghoon Choi, Glenn S. Diskin, Anna Agustí-Panareda, Mark Parrington, Sebastien Massart, Benjamin Gaubert, Youngjae Lee, Danbi Kim, Jinsang Jung, Jinkyu Hong, Je-Woo Hong, Yugo Kanaya, Mindo Lee, Ryan M. Stauffer, Anne M. Thompson, James H. Flynn, and Jung-Hun Woo
Atmos. Chem. Phys., 18, 11007–11030, https://doi.org/10.5194/acp-18-11007-2018, https://doi.org/10.5194/acp-18-11007-2018, 2018
Juan Cuesta, Yugo Kanaya, Masayuki Takigawa, Gaëlle Dufour, Maxim Eremenko, Gilles Foret, Kazuyuki Miyazaki, and Matthias Beekmann
Atmos. Chem. Phys., 18, 9499–9525, https://doi.org/10.5194/acp-18-9499-2018, https://doi.org/10.5194/acp-18-9499-2018, 2018
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This paper tackles a major issue for air quality over East Asia: ozone pollution produced over a major source, like the North China Plain, and the contribution of ozone produced while being transported across the continent and the surrounding seas. The main originality of the paper lays in the fact that this photochemical production of ozone is observationally quantified with new multispectral satellite observations offering unique skills to observe the ozone pollution plumes near the surface.
Itsushi Uno, Kazuo Osada, Keiya Yumimoto, Zhe Wang, Syuichi Itahashi, Xiaole Pan, Yukari Hara, Yugo Kanaya, Shigekazu Yamamoto, and Thomas Duncan Fairlie
Atmos. Chem. Phys., 17, 14181–14197, https://doi.org/10.5194/acp-17-14181-2017, https://doi.org/10.5194/acp-17-14181-2017, 2017
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We analyzed long-term fine- and coarse-mode nitrate and related aerosols synergetic observations at Fukuoka, Japan. GEOS Chem model including dust and sea-salt acid uptake processes was used to assess the observed seasonal variation, and the impact of long-range transport from the Asian continent. A numerical model reproduced the seasonal variations of fine aerosols. For coarse nitrate, large-scale dust-nitrate outflow from China was confirmed during all dust events between January and June.
Xiaole Pan, Yugo Kanaya, Fumikazu Taketani, Takuma Miyakawa, Satoshi Inomata, Yuichi Komazaki, Hiroshi Tanimoto, Zhe Wang, Itsushi Uno, and Zifa Wang
Atmos. Chem. Phys., 17, 13001–13016, https://doi.org/10.5194/acp-17-13001-2017, https://doi.org/10.5194/acp-17-13001-2017, 2017
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Characteristics of refractory black carbon (rBC) from open biomass burning (OBB) have a great impact on regional pollution and climate, in particular in East Asia. However, experimental study on characteristics of rBC from agricultural residue burning in East China was limited. This study performed laboratory experiments: we found that emission of rBC is highly related to flaming burning, and non-rBC to smoldering burning. Rapid condensation of semi-volatile organics resulted in coated rBC.
Kohei Ikeda, Hiroshi Tanimoto, Takafumi Sugita, Hideharu Akiyoshi, Yugo Kanaya, Chunmao Zhu, and Fumikazu Taketani
Atmos. Chem. Phys., 17, 10515–10533, https://doi.org/10.5194/acp-17-10515-2017, https://doi.org/10.5194/acp-17-10515-2017, 2017
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Black carbon (BC), also known as soot particles, plays a key role in Arctic warming; hence, an understanding of the major source regions and types is important for its mitigation. We found that Russia was the dominant contributor to Arctic BC at the surface level, while the East Asian contribution was the largest in the middle troposphere and the burden over the Arctic, suggesting that BC emission reduction from Russia and East Asia can help mitigate warming in the Arctic.
Takuma Miyakawa, Naga Oshima, Fumikazu Taketani, Yuichi Komazaki, Ayako Yoshino, Akinori Takami, Yutaka Kondo, and Yugo Kanaya
Atmos. Chem. Phys., 17, 5851–5864, https://doi.org/10.5194/acp-17-5851-2017, https://doi.org/10.5194/acp-17-5851-2017, 2017
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We have deployed a single particle soot photometer (SP2) to characterize black carbon (BC) aerosols near industrial sources in Japan in the early summer of 2014 and at a remote island in the spring of 2015. The observed changes in the SP2-derived size distributions and mixing state of BC-containing particles with air mass transport are connected to meteorological variability (transport pathways and air mass histories) in spring in east Asia.
Syuichi Itahashi, Itsushi Uno, Kazuo Osada, Yusuke Kamiguchi, Shigekazu Yamamoto, Kei Tamura, Zhe Wang, Yasunori Kurosaki, and Yugo Kanaya
Atmos. Chem. Phys., 17, 3823–3843, https://doi.org/10.5194/acp-17-3823-2017, https://doi.org/10.5194/acp-17-3823-2017, 2017
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Over East Asia, the transboundary air pollution of SO42− has been recognized. The importance of the transboundary air pollution of NO3− in winter was demonstrated in this study through synergetic ground-based observations with state-of-the-art measurements of secondary inorganic aerosols (SO42−, NO3−, and NH4+) and a regional chemical transport model analysis. This study will help to refine the understanding of transboundary heavy PM2.5 pollution in winter.
Enno Peters, Gaia Pinardi, André Seyler, Andreas Richter, Folkard Wittrock, Tim Bösch, Michel Van Roozendael, François Hendrick, Theano Drosoglou, Alkiviadis F. Bais, Yugo Kanaya, Xiaoyi Zhao, Kimberly Strong, Johannes Lampel, Rainer Volkamer, Theodore Koenig, Ivan Ortega, Olga Puentedura, Mónica Navarro-Comas, Laura Gómez, Margarita Yela González, Ankie Piters, Julia Remmers, Yang Wang, Thomas Wagner, Shanshan Wang, Alfonso Saiz-Lopez, David García-Nieto, Carlos A. Cuevas, Nuria Benavent, Richard Querel, Paul Johnston, Oleg Postylyakov, Alexander Borovski, Alexander Elokhov, Ilya Bruchkouski, Haoran Liu, Cheng Liu, Qianqian Hong, Claudia Rivera, Michel Grutter, Wolfgang Stremme, M. Fahim Khokhar, Junaid Khayyam, and John P. Burrows
Atmos. Meas. Tech., 10, 955–978, https://doi.org/10.5194/amt-10-955-2017, https://doi.org/10.5194/amt-10-955-2017, 2017
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This work is about harmonization of differential optical absorption spectroscopy retrieval codes, which is a remote sensing technique widely used to derive atmospheric trace gas amounts. The study is based on ground-based measurements performed during the Multi-Axis DOAS Comparison campaign for Aerosols and Trace gases (MAD-CAT) in Mainz, Germany, in summer 2013. In total, 17 international groups working in the field of the DOAS technique participated in this study.
Kazuyuki Miyazaki, Henk Eskes, Kengo Sudo, K. Folkert Boersma, Kevin Bowman, and Yugo Kanaya
Atmos. Chem. Phys., 17, 807–837, https://doi.org/10.5194/acp-17-807-2017, https://doi.org/10.5194/acp-17-807-2017, 2017
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Global surface emissions of nitrogen oxides (NOx) over a 10-year period (2005–2014) are estimated from assimilation of multiple satellite datasets. We present detailed distributions of the estimated NOx emission distributions for all major regions, the diurnal, seasonal, and decadal variability. The estimated emissions show a positive trend over India, China, and the Middle East, and a negative trend over the United States, southern Africa, and western Europe.
Yugo Kanaya, Xiaole Pan, Takuma Miyakawa, Yuichi Komazaki, Fumikazu Taketani, Itsushi Uno, and Yutaka Kondo
Atmos. Chem. Phys., 16, 10689–10705, https://doi.org/10.5194/acp-16-10689-2016, https://doi.org/10.5194/acp-16-10689-2016, 2016
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Wet removal of atmospheric black carbon particles was quantitatively characterized in terms of accumulated precipitation along a backward trajectory (APT) using long-term observations at Fukue Island, western Japan, receiving Asian continental outflow with variable degrees of influence from precipitation. The emission inventory of BC over East Asia was assessed in terms of the observed BC/CO ratios. Model simulations should be diagnosed with these improved knowledge on the emission and removal.
G. Dufour, M. Eremenko, J. Cuesta, C. Doche, G. Foret, M. Beekmann, A. Cheiney, Y. Wang, Z. Cai, Y. Liu, M. Takigawa, Y. Kanaya, and J.-M. Flaud
Atmos. Chem. Phys., 15, 10839–10856, https://doi.org/10.5194/acp-15-10839-2015, https://doi.org/10.5194/acp-15-10839-2015, 2015
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We identify the stratospheric and the photochemical sources contributing to the late-spring O3 distribution over East Asia using IASI O3 and CO observations. Reversible subsiding O3 transfers in the UTLS associated with low-pressure systems impact lower-tropospheric O3 north of 40°N. By contrast, photochemical production from primary pollutants significantly contributes to the enhanced lower-tropospheric O3 over the NCP and photochemical processing occurs within the plume exported from the NCP.
X. Pan, Y. Kanaya, H. Tanimoto, S. Inomata, Z. Wang, S. Kudo, and I. Uno
Atmos. Chem. Phys., 15, 6101–6111, https://doi.org/10.5194/acp-15-6101-2015, https://doi.org/10.5194/acp-15-6101-2015, 2015
H. Matsui, M. Koike, Y. Kondo, A. Takami, J. D. Fast, Y. Kanaya, and M. Takigawa
Atmos. Chem. Phys., 14, 9513–9535, https://doi.org/10.5194/acp-14-9513-2014, https://doi.org/10.5194/acp-14-9513-2014, 2014
Y. Kanaya, H. Akimoto, Z.-F. Wang, P. Pochanart, K. Kawamura, Y. Liu, J. Li, Y. Komazaki, H. Irie, X.-L. Pan, F. Taketani, K. Yamaji, H. Tanimoto, S. Inomata, S. Kato, J. Suthawaree, K. Okuzawa, G. Wang, S. G. Aggarwal, P. Q. Fu, T. Wang, J. Gao, Y. Wang, and G. Zhuang
Atmos. Chem. Phys., 13, 8265–8283, https://doi.org/10.5194/acp-13-8265-2013, https://doi.org/10.5194/acp-13-8265-2013, 2013
K. Kawamura, E. Tachibana, K. Okuzawa, S. G. Aggarwal, Y. Kanaya, and Z. F. Wang
Atmos. Chem. Phys., 13, 8285–8302, https://doi.org/10.5194/acp-13-8285-2013, https://doi.org/10.5194/acp-13-8285-2013, 2013
N. He, K. Kawamura, K. Okuzawa, Y. Kanaya, and Z. F. Wang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-13-16699-2013, https://doi.org/10.5194/acpd-13-16699-2013, 2013
Revised manuscript not accepted
K. Kawamura, K. Okuzawa, S. G. Aggarwal, H. Irie, Y. Kanaya, and Z. Wang
Atmos. Chem. Phys., 13, 5369–5380, https://doi.org/10.5194/acp-13-5369-2013, https://doi.org/10.5194/acp-13-5369-2013, 2013
Fanhao Meng, Baobin Han, Min Qin, Wu Fang, Ke Tang, Dou Shao, Zhitang Liao, Jun Duan, Yan Feng, Yong Huang, Ting Ni, and Pinhua Xie
Atmos. Chem. Phys., 24, 14191–14208, https://doi.org/10.5194/acp-24-14191-2024, https://doi.org/10.5194/acp-24-14191-2024, 2024
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Comprehensive observations of HONO and NOx fluxes were conducted over paddy fields in the Huaihe River Basin. Consecutive peaks in HONO and NO fluxes suggest a potentially enhanced release of HONO and NO due to soil tillage, whereas waterlogged soil may inhibit microbial nitrification processes following irrigation. Notably, biological processes and light-driven NO2 reactions at the surface may serve as sources of HONO and influence the local HONO budget during rotary tillage.
Xiao Lu, Yiming Liu, Jiayin Su, Xiang Weng, Tabish Ansari, Yuqiang Zhang, Guowen He, Yuqi Zhu, Haolin Wang, Ganquan Zeng, Jingyu Li, Cheng He, Shuai Li, Teerachai Amnuaylojaroen, Tim Butler, Qi Fan, Shaojia Fan, Grant L. Forster, Meng Gao, Jianlin Hu, Yugo Kanaya, Mohd Talib Latif, Keding Lu, Philippe Nédélec, Peer Nowack, Bastien Sauvage, Xiaobin Xu, Lin Zhang, Ke Li, Ja-Ho Koo, and Tatsuya Nagashima
EGUsphere, https://doi.org/10.5194/egusphere-2024-3702, https://doi.org/10.5194/egusphere-2024-3702, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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This study analyzes summertime ozone trends in East and Southeast Asia derived from a comprehensive observational database spanning from 1995 to 2019, incorporating aircraft observations, ozonesonde data, and measurements from 2500 surface sites. Multiple models are applied to attribute to changes in anthropogenic emissions and climate. The results highlight increases in anthropogenic emission are the primary driver of ozone increases both in the free troposphere and at the surface.
Phuc Thi Minh Ha, Yugo Kanaya, Kazuyo Yamaji, Syuichi Itahashi, Satoru Chatani, Takashi Sekiya, Maria Dolores Andrés Hernández, John Philip Burrows, Hans Schlager, Michael Lichtenstern, Mira Poehlker, and Bruna Holanda
EGUsphere, https://doi.org/10.5194/egusphere-2024-2064, https://doi.org/10.5194/egusphere-2024-2064, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Black carbon and CO are important to climate change. EMeRGe airborne observation can identify the suitability of emission inventories used in CMAQv5.0.2 model for Asian polluted regions. GFEDv4.1s is suitable for fire emissions. Anthropogenic BC and CO emissions from Philippines (REASv2.1) are insufficient. The estimated Chinese emissions in 2018 are 0.65±0.25 TgBC, 166±65 TgCO and 12.4±4.8 PgCO2, suggesting a reduction and increment for China's BC and CO emissions in the HTAPv2.2z inventory.
Yuhang Zhang, Huan Yu, Isabelle De Smedt, Jintai Lin, Nicolas Theys, Michel Van Roozendael, Gaia Pinardi, Steven Compernolle, Ruijing Ni, Fangxuan Ren, Sijie Wang, Lulu Chen, Jos Van Geffen, Mengyao Liu, Alexander Cede, Alexis Merlaud, Martina Friedrich, Andreas Richter, Ankie Piters, Vinod Kumar, Vinayak Sinha, Thomas Wagner, Yongjoo Choi, Hisahiro Takashima, Yugo Kanaya, Hitoshi Irie, Robert Spurr, Wenfu Sun, and Lorenzo Fabris
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2024-182, https://doi.org/10.5194/amt-2024-182, 2024
Preprint under review for AMT
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We developed an advanced POMINO algorithm for global retrieval of TROPOMI HCHO and NO2 VCDs with much improved consistency. Sensitivity tests demonstrate the complexity and non-linear interactions of auxiliary parameters in the AMF calculation. An improved agreement is found with measurements from a global ground-based instrument network. The POMINO retrieval provides a useful source of information for studies combining HCHO and NO2.
Eunjo S. Ha, Rokjin J. Park, Hyeong-Ahn Kwon, Gitaek T. Lee, Sieun D. Lee, Seunga Shin, Dong-Won Lee, Hyunkee Hong, Christophe Lerot, Isabelle De Smedt, Thomas Danckaert, Francois Hendrick, and Hitoshi Irie
Atmos. Meas. Tech., 17, 6369–6384, https://doi.org/10.5194/amt-17-6369-2024, https://doi.org/10.5194/amt-17-6369-2024, 2024
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In this study, we evaluated the GEMS glyoxal products by comparing them with TROPOMI and MAX-DOAS measurements. GEMS and TROPOMI VCDs present similar spatial distributions. Monthly variations in GEMS VCDs and TROPOMI and MAX-DOAS VCDs differ in northeastern Asia, which we attributed to a polluted reference spectrum and high NO2 concentrations. GEMS glyoxal products with unparalleled temporal resolution would enrich our understanding of VOC emissions and diurnal variation.
Kezia Lange, Andreas Richter, Tim Bösch, Bianca Zilker, Miriam Latsch, Lisa K. Behrens, Chisom M. Okafor, Hartmut Bösch, John P. Burrows, Alexis Merlaud, Gaia Pinardi, Caroline Fayt, Martina M. Friedrich, Ermioni Dimitropoulou, Michel Van Roozendael, Steffen Ziegler, Simona Ripperger-Lukosiunaite, Leon Kuhn, Bianca Lauster, Thomas Wagner, Hyunkee Hong, Donghee Kim, Lim-Seok Chang, Kangho Bae, Chang-Keun Song, Jong-Uk Park, and Hanlim Lee
Atmos. Meas. Tech., 17, 6315–6344, https://doi.org/10.5194/amt-17-6315-2024, https://doi.org/10.5194/amt-17-6315-2024, 2024
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Instruments for air quality observations on geostationary satellites provide multiple observations per day and allow for the analysis of the diurnal variation of important air pollutants such as nitrogen dioxide (NO2) over large areas. The South Korean instrument GEMS, launched in February 2020, is the first instrument in geostationary orbit and covers a large part of Asia. Our investigations show the observed diurnal evolution of NO2 at different measurement sites.
Thi Nhu Ngoc Do, Kengo Sudo, Akihiko Ito, Louisa Emmons, Vaishali Naik, Kostas Tsigaridis, Øyvind Seland, Gerd A. Folberth, and Douglas I. Kelley
EGUsphere, https://doi.org/10.5194/egusphere-2024-2313, https://doi.org/10.5194/egusphere-2024-2313, 2024
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Understanding historical isoprene emission changes is important for predicting future climate, but trends and their controlling factors remain uncertain. This study shows that long-term isoprene trends vary among Earth System Models mainly due to partially incorporating CO2 effects and land cover changes rather than climate. Future models that refine these factors’ effects on isoprene emissions, along with long-term observations, are essential for better understanding plant-climate interactions.
Yujin J. Oak, Daniel J. Jacob, Nicholas Balasus, Laura H. Yang, Heesung Chong, Junsung Park, Hanlim Lee, Gitaek T. Lee, Eunjo S. Ha, Rokjin J. Park, Hyeong-Ahn Kwon, and Jhoon Kim
Atmos. Meas. Tech., 17, 5147–5159, https://doi.org/10.5194/amt-17-5147-2024, https://doi.org/10.5194/amt-17-5147-2024, 2024
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We present an improved NO2 product from GEMS by calibrating it to TROPOMI using machine learning and by reprocessing both satellite products to adopt common NO2 profiles. Our corrected GEMS product combines the high data density of GEMS with the accuracy of TROPOMI, supporting the combined use for analyses of East Asia air quality including emissions and chemistry. This method can be extended to other species and geostationary satellites including TEMPO and Sentinel-4.
Jiangman Xu, Ang Li, Zhaokun Hu, Hairong Zhang, and Min Qin
EGUsphere, https://doi.org/10.5194/egusphere-2024-1695, https://doi.org/10.5194/egusphere-2024-1695, 2024
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This article introduces an experimental system for rapidly acquiring trace gas profiles using multi-channel spectroscopy, significantly enhancing the time resolution of spectral collection. Owing to the improved temporal resolution, the gas profile obtained by the FS MAX-DOAS can show more details than MAX-DOAS. This work can also be integrated with mobile platforms for navigational observation research, which is crucial for achieving mobile MAX-DOAS profile measurements.
Renzhi Hu, Guoxian Zhang, Haotian Cai, Jingyi Guo, Keding Lu, Xin Li, Shengrong Lou, Zhaofeng Tan, Changjin Hu, Pinhua Xie, and Wenqing Liu
EGUsphere, https://doi.org/10.5194/egusphere-2024-2494, https://doi.org/10.5194/egusphere-2024-2494, 2024
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A full suite of radical measurements (OH, HO2, RO2, and kOH) was established to accurately elucidate the limitations of oxidation in chemical-complex atmosphere. Sensitivity tests revealed that the incorporation of complex processes enabled a balance in both radical concentrations and coordinate ratios, and effectively addressing the deficiency in the ozone generation mechanism. The full-chain radical detection untangled a gap-bridge between the photochemistry and the intensive oxidation level.
Hossain Mohammed Syedul Hoque, Kengo Sudo, Hitoshi Irie, Yanfeng He, and Md Firoz Khan
Geosci. Model Dev., 17, 5545–5571, https://doi.org/10.5194/gmd-17-5545-2024, https://doi.org/10.5194/gmd-17-5545-2024, 2024
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Using multi-platform observations, we validated global formaldehyde (HCHO) simulations from a chemistry transport model. HCHO is a crucial intermediate in the chemical catalytic cycle that governs the ozone formation in the troposphere. The model was capable of replicating the observed spatiotemporal variability in HCHO. In a few cases, the model's capability was limited. This is attributed to the uncertainties in the observations and the model parameters.
Yu-Wen Chen, K. Sebastian Schmidt, Hong Chen, Steven T. Massie, Susan S. Kulawik, and Hironobu Iwabuchi
EGUsphere, https://doi.org/10.5194/egusphere-2024-1936, https://doi.org/10.5194/egusphere-2024-1936, 2024
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Retrievals of CO2 column-averaged dry air mole fractions from space can be done with spaceborne spectrometers such as OCO-2. Clouds in the vicinity of a footprint lead to spectral perturbations that bias those retrievals well beyond the required accuracy for global assessments of CO2 sources and sinks. This paper presents two physics-based mitigation techniques for these biases based on accompanying imagery, which can be used operationally.
Laura Hyesung Yang, Daniel J. Jacob, Ruijun Dang, Yujin J. Oak, Haipeng Lin, Jhoon Kim, Shixian Zhai, Nadia K. Colombi, Drew C. Pendergrass, Ellie Beaudry, Viral Shah, Xu Feng, Robert M. Yantosca, Heesung Chong, Junsung Park, Hanlim Lee, Won-Jin Lee, Soontae Kim, Eunhye Kim, Katherine R. Travis, James H. Crawford, and Hong Liao
Atmos. Chem. Phys., 24, 7027–7039, https://doi.org/10.5194/acp-24-7027-2024, https://doi.org/10.5194/acp-24-7027-2024, 2024
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The Geostationary Environment Monitoring Spectrometer (GEMS) provides hourly measurements of NO2. We use the chemical transport model to find how emissions, chemistry, and transport drive the changes in NO2 observed by GEMS at different times of the day. In winter, the chemistry plays a minor role, and high daytime emissions dominate the diurnal variation in NO2, balanced by transport. In summer, emissions, chemistry, and transport play an important role in shaping the diurnal variation in NO2.
Drew C. Pendergrass, Daniel J. Jacob, Yujin J. Oak, Jeewoo Lee, Minseok Kim, Jhoon Kim, Seoyoung Lee, Shixian Zhai, Hitoshi Irie, and Hong Liao
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-172, https://doi.org/10.5194/essd-2024-172, 2024
Preprint withdrawn
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Fine particles suspended in the atmosphere are a major form of air pollution and an important public health burden. However, measurements of particulate matter are sparse in space and in places like East Asia monitors are established after regulatory policies to improve pollution have changed. In this paper, we use machine learning to fill in the gaps. We train an algorithm to predict pollution at the surface from the atmosphere’s opacity, then produce high resolution maps of data without gaps.
Adrien Deroubaix, Marco Vountas, Benjamin Gaubert, Maria Dolores Andrés Hernández, Stephan Borrmann, Guy Brasseur, Bruna Holanda, Yugo Kanaya, Katharina Kaiser, Flora Kluge, Ovid Oktavian Krüger, Inga Labuhn, Michael Lichtenstern, Klaus Pfeilsticker, Mira Pöhlker, Hans Schlager, Johannes Schneider, Guillaume Siour, Basudev Swain, Paolo Tuccella, Kameswara S. Vinjamuri, Mihalis Vrekoussis, Benjamin Weyland, and John P. Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2024-516, https://doi.org/10.5194/egusphere-2024-516, 2024
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This study assesses atmospheric composition using air quality models during aircraft campaigns in Europe and Asia, focusing on carbonaceous aerosols and trace gases. While carbon monoxide is well modeled, other pollutants have moderate to weak agreement with observations. Wind speed modeling is reliable for identifying pollution plumes, where models tend to overestimate concentrations. This highlights challenges in accurately modeling aerosol and trace gas composition, particularly in cities.
Adrien Deroubaix, Marco Vountas, Benjamin Gaubert, Maria Dolores Andrés Hernández, Stephan Borrmann, Guy Brasseur, Bruna Holanda, Yugo Kanaya, Katharina Kaiser, Flora Kluge, Ovid Oktavian Krüger, Inga Labuhn, Michael Lichtenstern, Klaus Pfeilsticker, Mira Pöhlker, Hans Schlager, Johannes Schneider, Guillaume Siour, Basudev Swain, Paolo Tuccella, Kameswara S. Vinjamuri, Mihalis Vrekoussis, Benjamin Weyland, and John P. Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2024-521, https://doi.org/10.5194/egusphere-2024-521, 2024
Preprint archived
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This study explores the proportional relationships between carbonaceous aerosols (black and organic carbon) and trace gases using airborne measurements from two campaigns in Europe and East Asia. Differences between regions were found, but air quality models struggled to reproduce them accurately. We show that these proportional relationships can help to constrain models and can be used to infer aerosol concentrations from satellite observations of trace gases, especially in urban areas.
Kaori Kawana, Fumikazu Taketani, Kazuhiko Matsumoto, Yutaka Tobo, Yoko Iwamoto, Takuma Miyakawa, Akinori Ito, and Yugo Kanaya
Atmos. Chem. Phys., 24, 1777–1799, https://doi.org/10.5194/acp-24-1777-2024, https://doi.org/10.5194/acp-24-1777-2024, 2024
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Based on comprehensive shipborne observations, we found strong links between sea-surface biological materials and the formation of atmospheric fluorescent bioaerosols, cloud condensation nuclei, and ice-nucleating particles over the Arctic Ocean and Bering Sea during autumn 2019. Taking the wind-speed effect into account, we propose equations to approximate the links for this cruise, which can be used as a guide for modeling as well as for systematic comparisons with other observations.
Guoxian Zhang, Renzhi Hu, Pinhua Xie, Changjin Hu, Xiaoyan Liu, Liujun Zhong, Haotian Cai, Bo Zhu, Shiyong Xia, Xiaofeng Huang, Xin Li, and Wenqing Liu
Atmos. Chem. Phys., 24, 1825–1839, https://doi.org/10.5194/acp-24-1825-2024, https://doi.org/10.5194/acp-24-1825-2024, 2024
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Comprehensive observation of HOx radicals was conducted at a coastal site in the Pearl River Delta. Radical chemistry was influenced by different air masses in a time-dependent way. Land mass promotes a more active photochemical process, with daily averages of 7.1 × 106 and 5.2 × 108 cm−3 for OH and HO2 respectively. The rapid oxidation process was accompanied by a higher diurnal HONO concentration, which influences the ozone-sensitive system and eventually magnifies the background ozone.
Takeshi Kinase, Fumikazu Taketani, Masayuki Takigawa, Chunmao Zhu, Yongwon Kim, Petr Mordovskoi, and Yugo Kanaya
EGUsphere, https://doi.org/10.5194/egusphere-2023-2764, https://doi.org/10.5194/egusphere-2023-2764, 2023
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Boreal forest wildfires in interior Alaska represent an important black carbon (BC) source for the Arctic and surrounding regions. We observed BC and carbon monoxide (CO) concentration in the Poker Flat Research Range since 2016 and found a positive correlation between the observed BC/∆CO ratio and fire radiative power (FRP) observed in Alaska and Canada. Our finding suggests the BC emission factor or/and inventory could be potentially improved by using FRP.
Nofel Lagrosas, Kosuke Okubo, Hitoshi Irie, Yutaka Matsumi, Tomoki Nakayama, Yutaka Sugita, Takashi Okada, and Tatsuo Shiina
Atmos. Meas. Tech., 16, 5937–5951, https://doi.org/10.5194/amt-16-5937-2023, https://doi.org/10.5194/amt-16-5937-2023, 2023
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This work examines the near-ground aerosol–weather relationship from 7-month continuous lidar and weather observations in Chiba, Japan. Optical parameters from lidar data are compared with weather parameters to understand and quantify the aerosol–weather relationship and how these optical parameters are affected by the weather and season. The results provide insights into analyzing optical properties of radioactive aerosols when the lidar system is continuously operated in a radioactive area.
Takuma Miyakawa, Akinori Ito, Chunmao Zhu, Atsushi Shimizu, Erika Matsumoto, Yusuke Mizuno, and Yugo Kanaya
Atmos. Chem. Phys., 23, 14609–14626, https://doi.org/10.5194/acp-23-14609-2023, https://doi.org/10.5194/acp-23-14609-2023, 2023
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This study conducted semi-continuous measurements of PM2.5 aerosols and their elemental composition in western Japan, during spring 2018. It analyzed the emissions, transport, and wet removal of elements such as Pb, Cu, Fe, and Mn. It also assessed the accuracy of modeled concentrations and found overestimations of BC and underestimations of Cu and anthropogenic Fe in East Asia. Insights into emissions, removals, and source apportionment of trace metals in the East Asian outflow were provided.
Yanfeng He and Kengo Sudo
Atmos. Chem. Phys., 23, 13061–13085, https://doi.org/10.5194/acp-23-13061-2023, https://doi.org/10.5194/acp-23-13061-2023, 2023
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Lightning has big social impacts. Lightning-produced NOx (LNOx) plays a vital role in atmospheric chemistry and climate. Investigating past lightning and LNOx trends can provide essential indicators of all lightning-related phenomena. Simulations show almost flat global lightning and LNOx trends during 1960–2014. Past global warming enhances the trends positively, but increases in aerosol have the opposite effect. Moreover, global lightning decreased markedly after the Pinatubo eruption.
Yuhang Zhang, Jintai Lin, Jhoon Kim, Hanlim Lee, Junsung Park, Hyunkee Hong, Michel Van Roozendael, Francois Hendrick, Ting Wang, Pucai Wang, Qin He, Kai Qin, Yongjoo Choi, Yugo Kanaya, Jin Xu, Pinhua Xie, Xin Tian, Sanbao Zhang, Shanshan Wang, Siyang Cheng, Xinghong Cheng, Jianzhong Ma, Thomas Wagner, Robert Spurr, Lulu Chen, Hao Kong, and Mengyao Liu
Atmos. Meas. Tech., 16, 4643–4665, https://doi.org/10.5194/amt-16-4643-2023, https://doi.org/10.5194/amt-16-4643-2023, 2023
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Our tropospheric NO2 vertical column density product with high spatiotemporal resolution is based on the Geostationary Environment Monitoring Spectrometer (GEMS) and named POMINO–GEMS. Strong hotspot signals and NO2 diurnal variations are clearly seen. Validations with multiple satellite products and ground-based, mobile car and surface measurements exhibit the overall great performance of the POMINO–GEMS product, indicating its capability for application in environmental studies.
Serin Kim, Daewon Kim, Hyunkee Hong, Lim-Seok Chang, Hanlim Lee, Deok-Rae Kim, Donghee Kim, Jeong-Ah Yu, Dongwon Lee, Ukkyo Jeong, Chang-Kuen Song, Sang-Woo Kim, Sang Seo Park, Jhoon Kim, Thomas F. Hanisco, Junsung Park, Wonei Choi, and Kwangyul Lee
Atmos. Meas. Tech., 16, 3959–3972, https://doi.org/10.5194/amt-16-3959-2023, https://doi.org/10.5194/amt-16-3959-2023, 2023
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A first evaluation of the Geostationary Environmental Monitoring Spectrometer (GEMS) NO2 was carried out via comparison with the NO2 data obtained from the ground-based Pandora direct-sun measurements at four sites in Seosan, Republic of Korea. Comparisons between GEMS NO2 and Pandora NO2 were performed according to GEMS cloud fraction. GEMS NO2 showed good agreement with that of Pandora NO2 under less cloudy conditions.
Ka Lok Chan, Pieter Valks, Klaus-Peter Heue, Ronny Lutz, Pascal Hedelt, Diego Loyola, Gaia Pinardi, Michel Van Roozendael, François Hendrick, Thomas Wagner, Vinod Kumar, Alkis Bais, Ankie Piters, Hitoshi Irie, Hisahiro Takashima, Yugo Kanaya, Yongjoo Choi, Kihong Park, Jihyo Chong, Alexander Cede, Udo Frieß, Andreas Richter, Jianzhong Ma, Nuria Benavent, Robert Holla, Oleg Postylyakov, Claudia Rivera Cárdenas, and Mark Wenig
Earth Syst. Sci. Data, 15, 1831–1870, https://doi.org/10.5194/essd-15-1831-2023, https://doi.org/10.5194/essd-15-1831-2023, 2023
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This paper presents the theoretical basis as well as verification and validation of the Global Ozone Monitoring Experiment-2 (GOME-2) daily and monthly level-3 products.
Hong Chen, K. Sebastian Schmidt, Steven T. Massie, Vikas Nataraja, Matthew S. Norgren, Jake J. Gristey, Graham Feingold, Robert E. Holz, and Hironobu Iwabuchi
Atmos. Meas. Tech., 16, 1971–2000, https://doi.org/10.5194/amt-16-1971-2023, https://doi.org/10.5194/amt-16-1971-2023, 2023
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We introduce the Education and Research 3D Radiative Transfer Toolbox (EaR3T) and propose a radiance self-consistency approach for quantifying and mitigating 3D bias in legacy airborne and spaceborne imagery retrievals due to spatially inhomogeneous clouds and surfaces.
Jagat S. H. Bisht, Prabir K. Patra, Masayuki Takigawa, Takashi Sekiya, Yugo Kanaya, Naoko Saitoh, and Kazuyuki Miyazaki
Geosci. Model Dev., 16, 1823–1838, https://doi.org/10.5194/gmd-16-1823-2023, https://doi.org/10.5194/gmd-16-1823-2023, 2023
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In this study, we estimated CH4 fluxes using an advanced 4D-LETKF method. The system was tested and optimized using observation system simulation experiments (OSSEs), where a known surface emission distribution is retrieved from synthetic observations. The availability of satellite measurements has increased, and there are still many missions focused on greenhouse gas observations that have not yet launched. The technique being referred to has the potential to improve estimates of CH4 fluxes.
Phuc Thi Minh Ha, Yugo Kanaya, Fumikazu Taketani, Maria Dolores Andrés Hernández, Benjamin Schreiner, Klaus Pfeilsticker, and Kengo Sudo
Geosci. Model Dev., 16, 927–960, https://doi.org/10.5194/gmd-16-927-2023, https://doi.org/10.5194/gmd-16-927-2023, 2023
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HONO affects tropospheric oxidizing capacity; thus, it is implemented into the chemistry–climate model CHASER. The model substantially underpredicts daytime HONO, while nitrate photolysis on surfaces can supplement the daytime HONO budget. Current HONO chemistry predicts reductions of 20.4 % for global tropospheric NOx, 40–67 % for OH, and 30–45 % for O3 in the summer North Pacific. In contrast, OH and O3 winter levels in China are greatly enhanced.
Alessandro Damiani, Hitoshi Irie, Dmitry A. Belikov, Shuei Kaizuka, Hossain Mohammed Syedul Hoque, and Raul R. Cordero
Atmos. Chem. Phys., 22, 12705–12726, https://doi.org/10.5194/acp-22-12705-2022, https://doi.org/10.5194/acp-22-12705-2022, 2022
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We analyzed the variabilities in tropospheric gases and aerosols within the Greater Tokyo Area, Japan. Beyond highlighting air quality changes caused by the pandemic during the lockdown, we found that the degree of weekly cycling of most gases and aerosols was enhanced during the whole of 2020. The changes were unprecedented in recent years and potentially related to coincident reduced mobility in Japan, which, in contrast to other countries, was anomalously low on weekends in 2020.
Hossain Mohammed Syedul Hoque, Kengo Sudo, Hitoshi Irie, Alessandro Damiani, Manish Naja, and Al Mashroor Fatmi
Atmos. Chem. Phys., 22, 12559–12589, https://doi.org/10.5194/acp-22-12559-2022, https://doi.org/10.5194/acp-22-12559-2022, 2022
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Nitrogen dioxide (NO2) and formaldehyde (HCHO) are essential trace graces regulating tropospheric ozone chemistry. These trace constituents are measured using an optical passive remote sensing technique. In addition, NO2 and HCHO are simulated with a computer model and evaluated against the observations. Such evaluations are essential to assess model uncertainties and improve their predictability. The results yielded good agreement between the two datasets with some discrepancies.
Vikas Nataraja, Sebastian Schmidt, Hong Chen, Takanobu Yamaguchi, Jan Kazil, Graham Feingold, Kevin Wolf, and Hironobu Iwabuchi
Atmos. Meas. Tech., 15, 5181–5205, https://doi.org/10.5194/amt-15-5181-2022, https://doi.org/10.5194/amt-15-5181-2022, 2022
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A convolutional neural network (CNN) is introduced to retrieve cloud optical thickness (COT) from passive cloud imagery. The CNN, trained on large eddy simulations from the Sulu Sea, learns from spatial information at multiple scales to reduce cloud inhomogeneity effects. By considering the spatial context of a pixel, the CNN outperforms the traditional independent pixel approximation (IPA) across several cloud morphology metrics.
Yanfeng He, Hossain Mohammed Syedul Hoque, and Kengo Sudo
Geosci. Model Dev., 15, 5627–5650, https://doi.org/10.5194/gmd-15-5627-2022, https://doi.org/10.5194/gmd-15-5627-2022, 2022
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Lightning-produced NOx (LNOx) is a major source of NOx. Hence, it is crucial to improve the prediction accuracy of lightning and LNOx in chemical climate models. By modifying existing lightning schemes and testing them in the chemical climate model CHASER, we improved the prediction accuracy of lightning in CHASER. Different lightning schemes respond very differently under global warming, which indicates further research is needed considering the reproducibility of long-term trends of lightning.
Boris D. Belan, Gerard Ancellet, Irina S. Andreeva, Pavel N. Antokhin, Viktoria G. Arshinova, Mikhail Y. Arshinov, Yurii S. Balin, Vladimir E. Barsuk, Sergei B. Belan, Dmitry G. Chernov, Denis K. Davydov, Alexander V. Fofonov, Georgii A. Ivlev, Sergei N. Kotel'nikov, Alexander S. Kozlov, Artem V. Kozlov, Katharine Law, Andrey V. Mikhal'chishin, Igor A. Moseikin, Sergei V. Nasonov, Philippe Nédélec, Olesya V. Okhlopkova, Sergei E. Ol'kin, Mikhail V. Panchenko, Jean-Daniel Paris, Iogannes E. Penner, Igor V. Ptashnik, Tatyana M. Rasskazchikova, Irina K. Reznikova, Oleg A. Romanovskii, Alexander S. Safatov, Denis E. Savkin, Denis V. Simonenkov, Tatyana K. Sklyadneva, Gennadii N. Tolmachev, Semyon V. Yakovlev, and Polina N. Zenkova
Atmos. Meas. Tech., 15, 3941–3967, https://doi.org/10.5194/amt-15-3941-2022, https://doi.org/10.5194/amt-15-3941-2022, 2022
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The change of the global climate is most pronounced in the Arctic, where the air temperature increases faster than the global average. This is associated with an increase in the concentration of greenhouse gases in the atmosphere. It is important to study how the air composition in the Arctic changes in the changing climate. Thus this integrated experiment was carried out to measure the composition of the troposphere in the Russian sector of the Arctic from on board the aircraft laboratory.
Cynthia H. Whaley, Rashed Mahmood, Knut von Salzen, Barbara Winter, Sabine Eckhardt, Stephen Arnold, Stephen Beagley, Silvia Becagli, Rong-You Chien, Jesper Christensen, Sujay Manish Damani, Xinyi Dong, Konstantinos Eleftheriadis, Nikolaos Evangeliou, Gregory Faluvegi, Mark Flanner, Joshua S. Fu, Michael Gauss, Fabio Giardi, Wanmin Gong, Jens Liengaard Hjorth, Lin Huang, Ulas Im, Yugo Kanaya, Srinath Krishnan, Zbigniew Klimont, Thomas Kühn, Joakim Langner, Kathy S. Law, Louis Marelle, Andreas Massling, Dirk Olivié, Tatsuo Onishi, Naga Oshima, Yiran Peng, David A. Plummer, Olga Popovicheva, Luca Pozzoli, Jean-Christophe Raut, Maria Sand, Laura N. Saunders, Julia Schmale, Sangeeta Sharma, Ragnhild Bieltvedt Skeie, Henrik Skov, Fumikazu Taketani, Manu A. Thomas, Rita Traversi, Kostas Tsigaridis, Svetlana Tsyro, Steven Turnock, Vito Vitale, Kaley A. Walker, Minqi Wang, Duncan Watson-Parris, and Tahya Weiss-Gibbons
Atmos. Chem. Phys., 22, 5775–5828, https://doi.org/10.5194/acp-22-5775-2022, https://doi.org/10.5194/acp-22-5775-2022, 2022
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Air pollutants, like ozone and soot, play a role in both global warming and air quality. Atmospheric models are often used to provide information to policy makers about current and future conditions under different emissions scenarios. In order to have confidence in those simulations, in this study we compare simulated air pollution from 18 state-of-the-art atmospheric models to measured air pollution in order to assess how well the models perform.
Hisahiro Takashima, Yugo Kanaya, Saki Kato, Martina M. Friedrich, Michel Van Roozendael, Fumikazu Taketani, Takuma Miyakawa, Yuichi Komazaki, Carlos A. Cuevas, Alfonso Saiz-Lopez, and Takashi Sekiya
Atmos. Chem. Phys., 22, 4005–4018, https://doi.org/10.5194/acp-22-4005-2022, https://doi.org/10.5194/acp-22-4005-2022, 2022
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We have undertaken atmospheric iodine monoxide (IO) observations in the global marine boundary layer with a wide latitudinal coverage and sea surface temperature (SST) range. We conclude that atmospheric iodine is abundant over the Western Pacific warm pool, appearing as an iodine fountain, where ozone (O3) minima occur. Our study also found negative correlations between IO and O3 concentrations over IO maxima, which requires reconsideration of the initiation process of halogen activation.
Pradeep Khatri, Tadahiro Hayasaka, Hitoshi Irie, Husi Letu, Takashi Y. Nakajima, Hiroshi Ishimoto, and Tamio Takamura
Atmos. Meas. Tech., 15, 1967–1982, https://doi.org/10.5194/amt-15-1967-2022, https://doi.org/10.5194/amt-15-1967-2022, 2022
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Cloud properties observed by the Second-generation Global Imager (SGLI) onboard the Global Change Observation Mission – Climate (GCOM-C) satellite are evaluated using surface observation data. The study finds that SGLI-observed cloud properties are qualitative enough, although water cloud properties are suggested to be more qualitative, and both water and ice cloud properties can reproduce surface irradiance quite satisfactorily. Thus, SGLI cloud products are very useful for different studies.
Takashi Sekiya, Kazuyuki Miyazaki, Henk Eskes, Kengo Sudo, Masayuki Takigawa, and Yugo Kanaya
Atmos. Meas. Tech., 15, 1703–1728, https://doi.org/10.5194/amt-15-1703-2022, https://doi.org/10.5194/amt-15-1703-2022, 2022
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This study gives a systematic comparison of TROPOMI version 1.2 and OMI QA4ECV tropospheric NO2 column through global chemical data assimilation (DA) integration for April–May 2018. DA performance is controlled by measurement sensitivities, retrieval errors, and coverage. Due to reduced errors in TROPOMI, agreements against assimilated and independent observations were improved by TROPOMI DA compared to OMI DA. These results demonstrate that TROPOMI DA improves global analyses of NO2 and ozone.
Baoye Hu, Jun Duan, Youwei Hong, Lingling Xu, Mengren Li, Yahui Bian, Min Qin, Wu Fang, Pinhua Xie, and Jinsheng Chen
Atmos. Chem. Phys., 22, 371–393, https://doi.org/10.5194/acp-22-371-2022, https://doi.org/10.5194/acp-22-371-2022, 2022
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There has been a lack of research into HONO in coastal cities with low concentrations of PM2.5, but strong sunlight and high humidity. Insufficient research on coastal cities with good air quality has resulted in certain obstacles to assessing the photochemical processes in these areas. Furthermore, HONO contributes to the atmospheric photochemistry depending on the season. Therefore, observations of HONO across four seasons in the southeastern coastal area of China are urgently needed.
Christophe Lerot, François Hendrick, Michel Van Roozendael, Leonardo M. A. Alvarado, Andreas Richter, Isabelle De Smedt, Nicolas Theys, Jonas Vlietinck, Huan Yu, Jeroen Van Gent, Trissevgeni Stavrakou, Jean-François Müller, Pieter Valks, Diego Loyola, Hitoshi Irie, Vinod Kumar, Thomas Wagner, Stefan F. Schreier, Vinayak Sinha, Ting Wang, Pucai Wang, and Christian Retscher
Atmos. Meas. Tech., 14, 7775–7807, https://doi.org/10.5194/amt-14-7775-2021, https://doi.org/10.5194/amt-14-7775-2021, 2021
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Global measurements of glyoxal tropospheric columns from the satellite instrument TROPOMI are presented. Such measurements can contribute to the estimation of atmospheric emissions of volatile organic compounds. This new glyoxal product has been fully characterized with a comprehensive error budget, with comparison with other satellite data sets as well as with validation based on independent ground-based remote sensing glyoxal observations.
Kaori Kawana, Kazuhiko Matsumoto, Fumikazu Taketani, Takuma Miyakawa, and Yugo Kanaya
Atmos. Chem. Phys., 21, 15969–15983, https://doi.org/10.5194/acp-21-15969-2021, https://doi.org/10.5194/acp-21-15969-2021, 2021
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Atmospheric autofluorescent particles observed over the central Pacific Ocean were identified as bioaerosols from comparisons to a DNA-nuclear-staining method. Their number concentrations in the pristine marine air masses showed high correlations with concentrations of bacteria and transparent exopolymer particles in the surface seawater, providing strong evidence of their marine origins. We propose equations to derive the atmospheric bioaerosol number concentrations from oceanic parameters.
Hossain M. S. Hoque, Kengo Sudo, Hitoshi Irie, Alessandro Damiani, and Al Mashroor Fatmi
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-815, https://doi.org/10.5194/acp-2021-815, 2021
Revised manuscript not accepted
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Nitrogen dioxide (NO2) and formaldehyde (HCHO) profiles, retrieved from remote sensing observations, are used to evaluate the global chemistry transport model CHASER. Overall, CHASER has demonstrated good skills in reproducing the seasonal climatology of NO2 and HCHO on a local scale at sites in South and East Asia. Around mountainous terrains, the model performs better on a regional scale. The improved spatial resolution of CHASER can likely reduce the observed discrepancies in the datasets.
Sho Ohata, Tatsuhiro Mori, Yutaka Kondo, Sangeeta Sharma, Antti Hyvärinen, Elisabeth Andrews, Peter Tunved, Eija Asmi, John Backman, Henri Servomaa, Daniel Veber, Konstantinos Eleftheriadis, Stergios Vratolis, Radovan Krejci, Paul Zieger, Makoto Koike, Yugo Kanaya, Atsushi Yoshida, Nobuhiro Moteki, Yongjing Zhao, Yutaka Tobo, Junji Matsushita, and Naga Oshima
Atmos. Meas. Tech., 14, 6723–6748, https://doi.org/10.5194/amt-14-6723-2021, https://doi.org/10.5194/amt-14-6723-2021, 2021
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Reliable values of mass absorption cross sections (MACs) of black carbon (BC) are required to determine mass concentrations of BC at Arctic sites using different types of filter-based absorption photometers. We successfully estimated MAC values for these instruments through comparison with independent measurements of BC by a continuous soot monitoring system called COSMOS. These MAC values are consistent with each other and applicable to study spatial and temporal variation in BC in the Arctic.
Igor B. Konovalov, Nikolai A. Golovushkin, Matthias Beekmann, Mikhail V. Panchenko, and Meinrat O. Andreae
Atmos. Meas. Tech., 14, 6647–6673, https://doi.org/10.5194/amt-14-6647-2021, https://doi.org/10.5194/amt-14-6647-2021, 2021
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The absorption of solar light by organic matter, known as brown carbon (BrC), contributes significantly to the radiative budget of the Earth’s atmosphere, but its representation in atmospheric models is uncertain. This paper advances a methodology to constrain model parameters characterizing BrC absorption of atmospheric aerosol originating from biomass burning with the available remote ground-based observations of atmospheric aerosol.
Xin Tian, Yang Wang, Steffen Beirle, Pinhua Xie, Thomas Wagner, Jin Xu, Ang Li, Steffen Dörner, Bo Ren, and Xiaomei Li
Atmos. Chem. Phys., 21, 12867–12894, https://doi.org/10.5194/acp-21-12867-2021, https://doi.org/10.5194/acp-21-12867-2021, 2021
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The performances of two MAX-DOAS inversion algorithms were evaluated for various aerosol pollution scenarios. One inversion algorithm is based on optimal estimation; the other uses a parameterized approach. In this analysis, three types of profile shapes for aerosols and NO2 were considered: exponential, Boltzmann, and Gaussian. The evaluation results can effectively guide the application of the two inversion algorithms in the actual atmosphere and improve the accuracy of the actual inversion.
Isabelle De Smedt, Gaia Pinardi, Corinne Vigouroux, Steven Compernolle, Alkis Bais, Nuria Benavent, Folkert Boersma, Ka-Lok Chan, Sebastian Donner, Kai-Uwe Eichmann, Pascal Hedelt, François Hendrick, Hitoshi Irie, Vinod Kumar, Jean-Christopher Lambert, Bavo Langerock, Christophe Lerot, Cheng Liu, Diego Loyola, Ankie Piters, Andreas Richter, Claudia Rivera Cárdenas, Fabian Romahn, Robert George Ryan, Vinayak Sinha, Nicolas Theys, Jonas Vlietinck, Thomas Wagner, Ting Wang, Huan Yu, and Michel Van Roozendael
Atmos. Chem. Phys., 21, 12561–12593, https://doi.org/10.5194/acp-21-12561-2021, https://doi.org/10.5194/acp-21-12561-2021, 2021
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This paper assess the performances of the TROPOMI formaldehyde observations compared to its predecessor OMI at different spatial and temporal scales. We also use a global network of MAX-DOAS instruments to validate both satellite datasets for a large range of HCHO columns. The precision obtained with daily TROPOMI observations is comparable to monthly OMI observations. We present clear detection of weak HCHO column enhancements related to shipping emissions in the Indian Ocean.
Phuc T. M. Ha, Ryoki Matsuda, Yugo Kanaya, Fumikazu Taketani, and Kengo Sudo
Geosci. Model Dev., 14, 3813–3841, https://doi.org/10.5194/gmd-14-3813-2021, https://doi.org/10.5194/gmd-14-3813-2021, 2021
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Policies to mitigate air pollution require an understanding of tropospheric oxidizing capacity, which is controlled by mechanisms including heterogeneous processes on aerosols and clouds. This study uses a chemistry–climate model CHASER (MIROC) to explore the heterogeneous effects in the troposphere for -2.96 % O3, -2.19 % NOx, +3.28 % CO, and +5.91 % CH4 lifetime. Besides, these processes affect polluted areas and remote areas and can bring challenges to pollution reduction efforts.
Na Zhao, Xinyi Dong, Kan Huang, Joshua S. Fu, Marianne Tronstad Lund, Kengo Sudo, Daven Henze, Tom Kucsera, Yun Fat Lam, Mian Chin, and Simone Tilmes
Atmos. Chem. Phys., 21, 8637–8654, https://doi.org/10.5194/acp-21-8637-2021, https://doi.org/10.5194/acp-21-8637-2021, 2021
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Black carbon acts as a strong climate forcer, especially in vulnerable pristine regions such as the Arctic. This work utilizes ensemble modeling results from the task force Hemispheric Transport of Air Pollution Phase 2 to investigate the responses of Arctic black carbon and surface temperature to various source emission reductions. East Asia contributed the most to Arctic black carbon. The response of Arctic temperature to black carbon was substantially more sensitive than the global average.
Mizuo Kajino, Makoto Deushi, Tsuyoshi Thomas Sekiyama, Naga Oshima, Keiya Yumimoto, Taichu Yasumichi Tanaka, Joseph Ching, Akihiro Hashimoto, Tetsuya Yamamoto, Masaaki Ikegami, Akane Kamada, Makoto Miyashita, Yayoi Inomata, Shin-ichiro Shima, Pradeep Khatri, Atsushi Shimizu, Hitoshi Irie, Kouji Adachi, Yuji Zaizen, Yasuhito Igarashi, Hiromasa Ueda, Takashi Maki, and Masao Mikami
Geosci. Model Dev., 14, 2235–2264, https://doi.org/10.5194/gmd-14-2235-2021, https://doi.org/10.5194/gmd-14-2235-2021, 2021
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This study compares performance of aerosol representation methods of the Japan Meteorological Agency's regional-scale nonhydrostatic meteorology–chemistry model (NHM-Chem). It indicates separate treatment of sea salt and dust in coarse mode and that of light-absorptive and non-absorptive particles in fine mode could provide accurate assessments on aerosol feedback processes.
Santosh Kumar Verma, Kimitaka Kawamura, Fei Yang, Pingqing Fu, Yugo Kanaya, and Zifa Wang
Atmos. Chem. Phys., 21, 4959–4978, https://doi.org/10.5194/acp-21-4959-2021, https://doi.org/10.5194/acp-21-4959-2021, 2021
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We studied aerosol samples collected in autumn 2007 with day and night intervals in a rural site of Mangshan, north of Beijing, for sugar compounds (SCs) that are abundant organic aerosol components and can influence the air quality and climate. We found higher concentrations of biomass burning (BB) products at nighttime than daytime, whereas pollen tracers and other SCs showed an opposite diurnal trend, because this site is meteorologically characterized by a mountain/valley breeze.
Tijl Verhoelst, Steven Compernolle, Gaia Pinardi, Jean-Christopher Lambert, Henk J. Eskes, Kai-Uwe Eichmann, Ann Mari Fjæraa, José Granville, Sander Niemeijer, Alexander Cede, Martin Tiefengraber, François Hendrick, Andrea Pazmiño, Alkiviadis Bais, Ariane Bazureau, K. Folkert Boersma, Kristof Bognar, Angelika Dehn, Sebastian Donner, Aleksandr Elokhov, Manuel Gebetsberger, Florence Goutail, Michel Grutter de la Mora, Aleksandr Gruzdev, Myrto Gratsea, Georg H. Hansen, Hitoshi Irie, Nis Jepsen, Yugo Kanaya, Dimitris Karagkiozidis, Rigel Kivi, Karin Kreher, Pieternel F. Levelt, Cheng Liu, Moritz Müller, Monica Navarro Comas, Ankie J. M. Piters, Jean-Pierre Pommereau, Thierry Portafaix, Cristina Prados-Roman, Olga Puentedura, Richard Querel, Julia Remmers, Andreas Richter, John Rimmer, Claudia Rivera Cárdenas, Lidia Saavedra de Miguel, Valery P. Sinyakov, Wolfgang Stremme, Kimberly Strong, Michel Van Roozendael, J. Pepijn Veefkind, Thomas Wagner, Folkard Wittrock, Margarita Yela González, and Claus Zehner
Atmos. Meas. Tech., 14, 481–510, https://doi.org/10.5194/amt-14-481-2021, https://doi.org/10.5194/amt-14-481-2021, 2021
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This paper reports on the ground-based validation of the NO2 data produced operationally by the TROPOMI instrument on board the Sentinel-5 Precursor satellite. Tropospheric, stratospheric, and total NO2 columns are compared to measurements collected from MAX-DOAS, ZSL-DOAS, and PGN/Pandora instruments respectively. The products are found to satisfy mission requirements in general, though negative mean differences are found at sites with high pollution levels. Potential causes are discussed.
Jan-Lukas Tirpitz, Udo Frieß, François Hendrick, Carlos Alberti, Marc Allaart, Arnoud Apituley, Alkis Bais, Steffen Beirle, Stijn Berkhout, Kristof Bognar, Tim Bösch, Ilya Bruchkouski, Alexander Cede, Ka Lok Chan, Mirjam den Hoed, Sebastian Donner, Theano Drosoglou, Caroline Fayt, Martina M. Friedrich, Arnoud Frumau, Lou Gast, Clio Gielen, Laura Gomez-Martín, Nan Hao, Arjan Hensen, Bas Henzing, Christian Hermans, Junli Jin, Karin Kreher, Jonas Kuhn, Johannes Lampel, Ang Li, Cheng Liu, Haoran Liu, Jianzhong Ma, Alexis Merlaud, Enno Peters, Gaia Pinardi, Ankie Piters, Ulrich Platt, Olga Puentedura, Andreas Richter, Stefan Schmitt, Elena Spinei, Deborah Stein Zweers, Kimberly Strong, Daan Swart, Frederik Tack, Martin Tiefengraber, René van der Hoff, Michel van Roozendael, Tim Vlemmix, Jan Vonk, Thomas Wagner, Yang Wang, Zhuoru Wang, Mark Wenig, Matthias Wiegner, Folkard Wittrock, Pinhua Xie, Chengzhi Xing, Jin Xu, Margarita Yela, Chengxin Zhang, and Xiaoyi Zhao
Atmos. Meas. Tech., 14, 1–35, https://doi.org/10.5194/amt-14-1-2021, https://doi.org/10.5194/amt-14-1-2021, 2021
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Multi-axis differential optical absorption spectroscopy (MAX-DOAS) is a ground-based remote sensing measurement technique that derives atmospheric aerosol and trace gas vertical profiles from skylight spectra. In this study, consistency and reliability of MAX-DOAS profiles are assessed by applying nine different evaluation algorithms to spectral data recorded during an intercomparison campaign in the Netherlands and by comparing the results to colocated supporting observations.
Sho Ohata, Tatsuhiro Mori, Yutaka Kondo, Sangeeta Sharma, Antti Hyvärinen, Elisabeth Andrews, Peter Tunved, Eija Asmi, John Backman, Henri Servomaa, Daniel Veber, Makoto Koike, Yugo Kanaya, Atsushi Yoshida, Nobuhiro Moteki, Yongjing Zhao, Junji Matsushita, and Naga Oshima
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-1190, https://doi.org/10.5194/acp-2020-1190, 2020
Preprint withdrawn
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Reliable values of mass absorption cross sections (MAC) of black carbon (BC) are required to determine mass concentrations of BC at Arctic sites using different types of filter-based absorption photometers. We successfully estimated MAC values for these instruments through comparison with independent measurements of BC by continuous soot monitoring system called COSMOS. These MAC values are consistent with each other and applicable to study spatial and temporal variation of BC in the Arctic.
Ke Tang, Min Qin, Wu Fang, Jun Duan, Fanhao Meng, Kaidi Ye, Helu Zhang, Pinhua Xie, Yabai He, Wenbin Xu, Jianguo Liu, and Wenqing Liu
Atmos. Meas. Tech., 13, 6487–6499, https://doi.org/10.5194/amt-13-6487-2020, https://doi.org/10.5194/amt-13-6487-2020, 2020
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We present an improved instrument for the simultaneous detection of atmospheric nitrous acid (HONO) and nitrogen dioxide (NO2). The robustness of the system is verified by simulating the influence of the relative change in light intensity on the measurement results. The instrument's capability to make fast high-sensitivity measurements of HONO and NO2 is of great significance for understanding the source of HONO and studying its role in atmospheric chemistry.
Gaia Pinardi, Michel Van Roozendael, François Hendrick, Nicolas Theys, Nader Abuhassan, Alkiviadis Bais, Folkert Boersma, Alexander Cede, Jihyo Chong, Sebastian Donner, Theano Drosoglou, Anatoly Dzhola, Henk Eskes, Udo Frieß, José Granville, Jay R. Herman, Robert Holla, Jari Hovila, Hitoshi Irie, Yugo Kanaya, Dimitris Karagkiozidis, Natalia Kouremeti, Jean-Christopher Lambert, Jianzhong Ma, Enno Peters, Ankie Piters, Oleg Postylyakov, Andreas Richter, Julia Remmers, Hisahiro Takashima, Martin Tiefengraber, Pieter Valks, Tim Vlemmix, Thomas Wagner, and Folkard Wittrock
Atmos. Meas. Tech., 13, 6141–6174, https://doi.org/10.5194/amt-13-6141-2020, https://doi.org/10.5194/amt-13-6141-2020, 2020
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We validate several GOME-2 and OMI tropospheric NO2 products with 23 MAX-DOAS and 16 direct sun instruments distributed worldwide, highlighting large horizontal inhomogeneities at several sites affecting the validation results. We propose a method for quantification and correction. We show the application of such correction reduces the satellite underestimation in almost all heterogeneous cases, but a negative bias remains over the MAX-DOAS and direct sun network ensemble for both satellites.
Yongjoo Choi, Yugo Kanaya, Masayuki Takigawa, Chunmao Zhu, Seung-Myung Park, Atsushi Matsuki, Yasuhiro Sadanaga, Sang-Woo Kim, Xiaole Pan, and Ignacio Pisso
Atmos. Chem. Phys., 20, 13655–13670, https://doi.org/10.5194/acp-20-13655-2020, https://doi.org/10.5194/acp-20-13655-2020, 2020
Yeyuan Huang, Ang Li, Thomas Wagner, Yang Wang, Zhaokun Hu, Pinhua Xie, Jin Xu, Hongmei Ren, Julia Remmers, Xiaoyi Fang, and Bing Dang
Atmos. Meas. Tech., 13, 6025–6051, https://doi.org/10.5194/amt-13-6025-2020, https://doi.org/10.5194/amt-13-6025-2020, 2020
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Mobile DOAS has become an important tool for the quantification of emission sources. In this study, we focused on the error budget of mobile DOAS measurements from NOx and SO2 point sources based on the model simulations, and we also offered recommendations for the optimum settings of such measurements.
Yang Wang, Arnoud Apituley, Alkiviadis Bais, Steffen Beirle, Nuria Benavent, Alexander Borovski, Ilya Bruchkouski, Ka Lok Chan, Sebastian Donner, Theano Drosoglou, Henning Finkenzeller, Martina M. Friedrich, Udo Frieß, David Garcia-Nieto, Laura Gómez-Martín, François Hendrick, Andreas Hilboll, Junli Jin, Paul Johnston, Theodore K. Koenig, Karin Kreher, Vinod Kumar, Aleksandra Kyuberis, Johannes Lampel, Cheng Liu, Haoran Liu, Jianzhong Ma, Oleg L. Polyansky, Oleg Postylyakov, Richard Querel, Alfonso Saiz-Lopez, Stefan Schmitt, Xin Tian, Jan-Lukas Tirpitz, Michel Van Roozendael, Rainer Volkamer, Zhuoru Wang, Pinhua Xie, Chengzhi Xing, Jin Xu, Margarita Yela, Chengxin Zhang, and Thomas Wagner
Atmos. Meas. Tech., 13, 5087–5116, https://doi.org/10.5194/amt-13-5087-2020, https://doi.org/10.5194/amt-13-5087-2020, 2020
Kazuyuki Miyazaki, Kevin Bowman, Takashi Sekiya, Henk Eskes, Folkert Boersma, Helen Worden, Nathaniel Livesey, Vivienne H. Payne, Kengo Sudo, Yugo Kanaya, Masayuki Takigawa, and Koji Ogochi
Earth Syst. Sci. Data, 12, 2223–2259, https://doi.org/10.5194/essd-12-2223-2020, https://doi.org/10.5194/essd-12-2223-2020, 2020
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This study presents the results from the Tropospheric Chemistry Reanalysis version 2 (TCR-2) for 2005–2018 obtained from the assimilation of multiple satellite measurements of ozone, CO, NO2, HNO3, and SO2 from the OMI, SCIAMACHY, GOME-2, TES, MLS, and MOPITT instruments. The evaluation results demonstrate the capability of the reanalysis products to improve understanding of the processes controlling variations in atmospheric composition, including long-term changes in air quality and emissions.
Baoye Hu, Jun Duan, Youwei Hong, Lingling Xu, Mengren Li, Yahui Bian, Min Qin, Wu Fang, Pinhua Xie, and Jinsheng Chen
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-880, https://doi.org/10.5194/acp-2020-880, 2020
Revised manuscript not accepted
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There has been a lack of research into HONO in coastal cities with low concentrations of NOx and PM2.5, but strong sunlight and high humidity. Insufficient research on coastal cities with good air quality has resulted in certain obstacles to assessing the photochemical processes in these areas. Furthermore, HONO contributes to the atmospheric photochemistry depending on the season. Therefore, observations of HONO across four seasons in the southeastern coastal area of China are urgently needed.
Matt Amos, Paul J. Young, J. Scott Hosking, Jean-François Lamarque, N. Luke Abraham, Hideharu Akiyoshi, Alexander T. Archibald, Slimane Bekki, Makoto Deushi, Patrick Jöckel, Douglas Kinnison, Ole Kirner, Markus Kunze, Marion Marchand, David A. Plummer, David Saint-Martin, Kengo Sudo, Simone Tilmes, and Yousuke Yamashita
Atmos. Chem. Phys., 20, 9961–9977, https://doi.org/10.5194/acp-20-9961-2020, https://doi.org/10.5194/acp-20-9961-2020, 2020
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We present an updated projection of Antarctic ozone hole recovery using an ensemble of chemistry–climate models. To do so, we employ a method, more advanced and skilful than the current multi-model mean standard, which is applicable to other ensemble analyses. It calculates the performance and similarity of the models, which we then use to weight the model. Calculating model similarity allows us to account for models which are constructed from similar components.
Mengyao Liu, Jintai Lin, Hao Kong, K. Folkert Boersma, Henk Eskes, Yugo Kanaya, Qin He, Xin Tian, Kai Qin, Pinhua Xie, Robert Spurr, Ruijing Ni, Yingying Yan, Hongjian Weng, and Jingxu Wang
Atmos. Meas. Tech., 13, 4247–4259, https://doi.org/10.5194/amt-13-4247-2020, https://doi.org/10.5194/amt-13-4247-2020, 2020
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Nitrogen oxides (NOx = NO + NO2) are important air pollutants in the troposphere and play crucial roles in the formation of ozone and particulate matter. The recently launched TROPOspheric Monitoring Instrument (TROPOMI) provides an opportunity to retrieve tropospheric concentrations of nitrogen dioxide (NO2) at an unprecedented high horizontal resolution. This work presents a new NO2 retrieval product over East Asia and further quantifies key factors affecting the retrieval, including aerosol.
Teruyuki Nakajima, Monica Campanelli, Huizheng Che, Victor Estellés, Hitoshi Irie, Sang-Woo Kim, Jhoon Kim, Dong Liu, Tomoaki Nishizawa, Govindan Pandithurai, Vijay Kumar Soni, Boossarasiri Thana, Nas-Urt Tugjsurn, Kazuma Aoki, Sujung Go, Makiko Hashimoto, Akiko Higurashi, Stelios Kazadzis, Pradeep Khatri, Natalia Kouremeti, Rei Kudo, Franco Marenco, Masahiro Momoi, Shantikumar S. Ningombam, Claire L. Ryder, Akihiro Uchiyama, and Akihiro Yamazaki
Atmos. Meas. Tech., 13, 4195–4218, https://doi.org/10.5194/amt-13-4195-2020, https://doi.org/10.5194/amt-13-4195-2020, 2020
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This paper overviews the progress in sky radiometer technology and the development of the network called SKYNET. It is found that the technology has produced useful on-site calibration methods, retrieval algorithms, and data analyses from sky radiometer observations of aerosol, cloud, water vapor, and ozone. The paper also discusses current issues of SKYNET to provide better information for the community.
Tuukka Petäjä, Ella-Maria Duplissy, Ksenia Tabakova, Julia Schmale, Barbara Altstädter, Gerard Ancellet, Mikhail Arshinov, Yurii Balin, Urs Baltensperger, Jens Bange, Alison Beamish, Boris Belan, Antoine Berchet, Rossana Bossi, Warren R. L. Cairns, Ralf Ebinghaus, Imad El Haddad, Beatriz Ferreira-Araujo, Anna Franck, Lin Huang, Antti Hyvärinen, Angelika Humbert, Athina-Cerise Kalogridis, Pavel Konstantinov, Astrid Lampert, Matthew MacLeod, Olivier Magand, Alexander Mahura, Louis Marelle, Vladimir Masloboev, Dmitri Moisseev, Vaios Moschos, Niklas Neckel, Tatsuo Onishi, Stefan Osterwalder, Aino Ovaska, Pauli Paasonen, Mikhail Panchenko, Fidel Pankratov, Jakob B. Pernov, Andreas Platis, Olga Popovicheva, Jean-Christophe Raut, Aurélie Riandet, Torsten Sachs, Rosamaria Salvatori, Roberto Salzano, Ludwig Schröder, Martin Schön, Vladimir Shevchenko, Henrik Skov, Jeroen E. Sonke, Andrea Spolaor, Vasileios K. Stathopoulos, Mikko Strahlendorff, Jennie L. Thomas, Vito Vitale, Sterios Vratolis, Carlo Barbante, Sabine Chabrillat, Aurélien Dommergue, Konstantinos Eleftheriadis, Jyri Heilimo, Kathy S. Law, Andreas Massling, Steffen M. Noe, Jean-Daniel Paris, André S. H. Prévôt, Ilona Riipinen, Birgit Wehner, Zhiyong Xie, and Hanna K. Lappalainen
Atmos. Chem. Phys., 20, 8551–8592, https://doi.org/10.5194/acp-20-8551-2020, https://doi.org/10.5194/acp-20-8551-2020, 2020
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The role of polar regions is increasing in terms of megatrends such as globalization, new transport routes, demography, and the use of natural resources with consequent effects on regional and transported pollutant concentrations. Here we summarize initial results from our integrative project exploring the Arctic environment and pollution to deliver data products, metrics, and indicators for stakeholders.
Yugo Kanaya, Kazuyo Yamaji, Takuma Miyakawa, Fumikazu Taketani, Chunmao Zhu, Yongjoo Choi, Yuichi Komazaki, Kohei Ikeda, Yutaka Kondo, and Zbigniew Klimont
Atmos. Chem. Phys., 20, 6339–6356, https://doi.org/10.5194/acp-20-6339-2020, https://doi.org/10.5194/acp-20-6339-2020, 2020
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Fundamental disagreements among bottom-up emission inventories exist about the sign of the black carbon emissions trend from China over the past decade. Our decadal observations on Fukue Island clearly indicate its rapid reduction, after correcting for interannual meteorological variability, which supports inventories reflecting governmental clean air actions after 2010. The reduction pace surpasses those of SSP1 scenarios for 2015–2030, suggesting highly successful emission control policies.
Masahiro Momoi, Rei Kudo, Kazuma Aoki, Tatsuhiro Mori, Kazuhiko Miura, Hiroshi Okamoto, Hitoshi Irie, Yoshinori Shoji, Akihiro Uchiyama, Osamu Ijima, Matsumi Takano, and Teruyuki Nakajima
Atmos. Meas. Tech., 13, 2635–2658, https://doi.org/10.5194/amt-13-2635-2020, https://doi.org/10.5194/amt-13-2635-2020, 2020
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The water vapor channel of sun photometers, such as a sky radiometer, has been calibrated at limited observation sites (e.g., Mauna Loa) in previous studies, but our procedure has made on-site calibration possible by using sky radiances in addition to direct solar irradiance. The retrieved precipitable water vapor values correspond well to those derived from a global-navigation-satellite-system–global-positioning-system receiver, a microwave radiometer, and an AERONET sun–sky radiometer.
Karin Kreher, Michel Van Roozendael, Francois Hendrick, Arnoud Apituley, Ermioni Dimitropoulou, Udo Frieß, Andreas Richter, Thomas Wagner, Johannes Lampel, Nader Abuhassan, Li Ang, Monica Anguas, Alkis Bais, Nuria Benavent, Tim Bösch, Kristof Bognar, Alexander Borovski, Ilya Bruchkouski, Alexander Cede, Ka Lok Chan, Sebastian Donner, Theano Drosoglou, Caroline Fayt, Henning Finkenzeller, David Garcia-Nieto, Clio Gielen, Laura Gómez-Martín, Nan Hao, Bas Henzing, Jay R. Herman, Christian Hermans, Syedul Hoque, Hitoshi Irie, Junli Jin, Paul Johnston, Junaid Khayyam Butt, Fahim Khokhar, Theodore K. Koenig, Jonas Kuhn, Vinod Kumar, Cheng Liu, Jianzhong Ma, Alexis Merlaud, Abhishek K. Mishra, Moritz Müller, Monica Navarro-Comas, Mareike Ostendorf, Andrea Pazmino, Enno Peters, Gaia Pinardi, Manuel Pinharanda, Ankie Piters, Ulrich Platt, Oleg Postylyakov, Cristina Prados-Roman, Olga Puentedura, Richard Querel, Alfonso Saiz-Lopez, Anja Schönhardt, Stefan F. Schreier, André Seyler, Vinayak Sinha, Elena Spinei, Kimberly Strong, Frederik Tack, Xin Tian, Martin Tiefengraber, Jan-Lukas Tirpitz, Jeroen van Gent, Rainer Volkamer, Mihalis Vrekoussis, Shanshan Wang, Zhuoru Wang, Mark Wenig, Folkard Wittrock, Pinhua H. Xie, Jin Xu, Margarita Yela, Chengxin Zhang, and Xiaoyi Zhao
Atmos. Meas. Tech., 13, 2169–2208, https://doi.org/10.5194/amt-13-2169-2020, https://doi.org/10.5194/amt-13-2169-2020, 2020
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In September 2016, 36 spectrometers from 24 institutes measured a number of key atmospheric pollutants during an instrument intercomparison campaign (CINDI-2) at Cabauw, the Netherlands. Here we report on the outcome of this intercomparison exercise. The three major goals were to characterise the differences between the participating instruments, to define a robust methodology for performance assessment, and to contribute to the harmonisation of the measurement settings and retrieval methods.
Fanhao Meng, Min Qin, Ke Tang, Jun Duan, Wu Fang, Shuaixi Liang, Kaidi Ye, Pinhua Xie, Yele Sun, Conghui Xie, Chunxiang Ye, Pingqing Fu, Jianguo Liu, and Wenqing Liu
Atmos. Chem. Phys., 20, 5071–5092, https://doi.org/10.5194/acp-20-5071-2020, https://doi.org/10.5194/acp-20-5071-2020, 2020
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Nitrous acid (HONO), a major precursor of the OH radical, plays a key role in atmospheric chemistry, but its sources are still debated. The first high-resolution vertical measurements of HONO and NO2 were conducted in Beijing to investigate the nocturnal sources of HONO at different stages of pollution. The ground surface dominated HONO production by heterogeneous conversion of NO2 during clean episodes, but the aerosol production was an important nighttime HONO source during haze episodes.
Bin Yao, Chao Liu, Yan Yin, Zhiquan Liu, Chunxiang Shi, Hironobu Iwabuchi, and Fuzhong Weng
Atmos. Meas. Tech., 13, 1033–1049, https://doi.org/10.5194/amt-13-1033-2020, https://doi.org/10.5194/amt-13-1033-2020, 2020
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Due to the complex spatiotemporal and physical properties of clouds, their quantitative depictions in different atmospheric reanalysis datasets are still highly uncertain. A radiance-based evaluation approach is developed to evaluate the quality of cloud properties by directly comparing them with satellite radiance observations. ERA5 and CRA are found to have great capability in representing the cloudy atmosphere over East Asia, and MERRA-2 tends to slightly overestimate clouds over the region.
Sebastian Donner, Jonas Kuhn, Michel Van Roozendael, Alkiviadis Bais, Steffen Beirle, Tim Bösch, Kristof Bognar, Ilya Bruchkouski, Ka Lok Chan, Steffen Dörner, Theano Drosoglou, Caroline Fayt, Udo Frieß, François Hendrick, Christian Hermans, Junli Jin, Ang Li, Jianzhong Ma, Enno Peters, Gaia Pinardi, Andreas Richter, Stefan F. Schreier, André Seyler, Kimberly Strong, Jan-Lukas Tirpitz, Yang Wang, Pinhua Xie, Jin Xu, Xiaoyi Zhao, and Thomas Wagner
Atmos. Meas. Tech., 13, 685–712, https://doi.org/10.5194/amt-13-685-2020, https://doi.org/10.5194/amt-13-685-2020, 2020
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The calibration of the elevation angles of MAX-DOAS instruments is important for the correct interpretation of such MAX-DOAS measurements. We present and evaluate different methods for the elevation calibration of MAX-DOAS instruments which were applied during the CINDI-2 field campaign.
Chunmao Zhu, Yugo Kanaya, Masayuki Takigawa, Kohei Ikeda, Hiroshi Tanimoto, Fumikazu Taketani, Takuma Miyakawa, Hideki Kobayashi, and Ignacio Pisso
Atmos. Chem. Phys., 20, 1641–1656, https://doi.org/10.5194/acp-20-1641-2020, https://doi.org/10.5194/acp-20-1641-2020, 2020
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Black carbon is believed to be one of the causes of the rapid warming and glacier melting in the Arctic. The results of our study show that processes associated with the petroleum industry, such as gas flaring in Russia, are the main BC source at the Arctic surface. Emissions in East Asia are the main BC sources at high altitudes in the Arctic. Wildfires in Siberia, Alaska, and Canada are another important Arctic BC source in summer.
Kazuyuki Miyazaki, Kevin W. Bowman, Keiya Yumimoto, Thomas Walker, and Kengo Sudo
Atmos. Chem. Phys., 20, 931–967, https://doi.org/10.5194/acp-20-931-2020, https://doi.org/10.5194/acp-20-931-2020, 2020
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We introduce a multi-model, multi-constituent chemical data assimilation framework that directly accounts for model error in transport and chemistry by integrating a portfolio of forward chemical transport models. The assimilation was able to reduce ensemble forward model spread and bias relative to independent measurements. Diagnostic information readily available from the framework has the potential to improve chemical predictions through relationships such as emergent constraints.
Lei Kong, Xiao Tang, Jiang Zhu, Zifa Wang, Joshua S. Fu, Xuemei Wang, Syuichi Itahashi, Kazuyo Yamaji, Tatsuya Nagashima, Hyo-Jung Lee, Cheol-Hee Kim, Chuan-Yao Lin, Lei Chen, Meigen Zhang, Zhining Tao, Jie Li, Mizuo Kajino, Hong Liao, Zhe Wang, Kengo Sudo, Yuesi Wang, Yuepeng Pan, Guiqian Tang, Meng Li, Qizhong Wu, Baozhu Ge, and Gregory R. Carmichael
Atmos. Chem. Phys., 20, 181–202, https://doi.org/10.5194/acp-20-181-2020, https://doi.org/10.5194/acp-20-181-2020, 2020
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Evaluation and uncertainty investigation of NO2, CO and NH3 modeling over China were conducted in this study using 14 chemical transport model results from MICS-Asia III. All models largely underestimated CO concentrations and showed very poor performance in reproducing the observed monthly variations of NH3 concentrations. Potential factors related to such deficiencies are investigated and discussed in this paper.
Yongjoo Choi, Yugo Kanaya, Seung-Myung Park, Atsushi Matsuki, Yasuhiro Sadanaga, Sang-Woo Kim, Itsushi Uno, Xiaole Pan, Meehye Lee, Hyunjae Kim, and Dong Hee Jung
Atmos. Chem. Phys., 20, 83–98, https://doi.org/10.5194/acp-20-83-2020, https://doi.org/10.5194/acp-20-83-2020, 2020
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The relationship between black carbon (BC) and carbon monoxide (CO) can differ by the different structure of fuel consumption. By investigating the representativeness of the BC and CO emission inventory for real-world comparison with reliable observations, this study suggested that accurate CO emissions should be preferentially investigated to enhance the accuracy of the BC emission rate over East Asia.
Leigh R. Crilley, Louisa J. Kramer, Bin Ouyang, Jun Duan, Wenqian Zhang, Shengrui Tong, Maofa Ge, Ke Tang, Min Qin, Pinhua Xie, Marvin D. Shaw, Alastair C. Lewis, Archit Mehra, Thomas J. Bannan, Stephen D. Worrall, Michael Priestley, Asan Bacak, Hugh Coe, James Allan, Carl J. Percival, Olalekan A. M. Popoola, Roderic L. Jones, and William J. Bloss
Atmos. Meas. Tech., 12, 6449–6463, https://doi.org/10.5194/amt-12-6449-2019, https://doi.org/10.5194/amt-12-6449-2019, 2019
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Nitrous acid (HONO) is key species for understanding tropospheric chemistry, yet accurate and precise measurements are challenging. Here we report an inter–comparison exercise of a number of instruments that measured HONO in a highly polluted location (Beijing). All instruments agreed on the temporal trends yet displayed divergence in absolute concentrations. The cause of this divergence was unclear, but it may in part be due to spatial variability in instrument location.
Pradeep Khatri, Hironobu Iwabuchi, Tadahiro Hayasaka, Hitoshi Irie, Tamio Takamura, Akihiro Yamazaki, Alessandro Damiani, Husi Letu, and Qin Kai
Atmos. Meas. Tech., 12, 6037–6047, https://doi.org/10.5194/amt-12-6037-2019, https://doi.org/10.5194/amt-12-6037-2019, 2019
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In an attempt to make cloud retrievals from the surface more common and convenient, we developed a cloud retrieval algorithm applicable for sky radiometers. It is based on an optimum method by fitting measured transmittances with modeled values. Further, a cost-effective and easy-to-use calibration procedure is proposed and validated using data obtained from the standard method. A detailed error analysis and quality assessment are also performed.
Xianyi Yang, Huizheng Che, Hitoshi Irie, Quanliang Chen, Ke Gui, Ying Cai, Yu Zheng, Linchang An, Hujia Zhao, Lei Li, Yuanxin Liang, Yaqiang Wang, Hong Wang, and Xiaoye Zhang
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2019-339, https://doi.org/10.5194/amt-2019-339, 2019
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This study assesses the performance of SKYNET in comparison to AERONET (Aerosol Robotic Network) for retrieving aerosol optical properties (AOPs) in Beijing, China. SKYNET data retrieved by SR-CEReS analysis package are used to analyze a serious pollution event in winter over Beijing. The AOPs under three weather conditions (clean, dusty, haze) in Beijing are discussed. Measurements from the SKYNET skyradiometer can be used to analyze the AOPs over Beijing reasonably.
Kévin Lamy, Thierry Portafaix, Béatrice Josse, Colette Brogniez, Sophie Godin-Beekmann, Hassan Bencherif, Laura Revell, Hideharu Akiyoshi, Slimane Bekki, Michaela I. Hegglin, Patrick Jöckel, Oliver Kirner, Ben Liley, Virginie Marecal, Olaf Morgenstern, Andrea Stenke, Guang Zeng, N. Luke Abraham, Alexander T. Archibald, Neil Butchart, Martyn P. Chipperfield, Glauco Di Genova, Makoto Deushi, Sandip S. Dhomse, Rong-Ming Hu, Douglas Kinnison, Michael Kotkamp, Richard McKenzie, Martine Michou, Fiona M. O'Connor, Luke D. Oman, Giovanni Pitari, David A. Plummer, John A. Pyle, Eugene Rozanov, David Saint-Martin, Kengo Sudo, Taichu Y. Tanaka, Daniele Visioni, and Kohei Yoshida
Atmos. Chem. Phys., 19, 10087–10110, https://doi.org/10.5194/acp-19-10087-2019, https://doi.org/10.5194/acp-19-10087-2019, 2019
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In this study, we simulate the ultraviolet radiation evolution during the 21st century on Earth's surface using the output from several numerical models which participated in the Chemistry-Climate Model Initiative. We present four possible futures which depend on greenhouse gases emissions. The role of ozone-depleting substances, greenhouse gases and aerosols are investigated. Our results emphasize the important role of aerosols for future ultraviolet radiation in the Northern Hemisphere.
Hiroaki Tatebe, Tomoo Ogura, Tomoko Nitta, Yoshiki Komuro, Koji Ogochi, Toshihiko Takemura, Kengo Sudo, Miho Sekiguchi, Manabu Abe, Fuyuki Saito, Minoru Chikira, Shingo Watanabe, Masato Mori, Nagio Hirota, Yoshio Kawatani, Takashi Mochizuki, Kei Yoshimura, Kumiko Takata, Ryouta O'ishi, Dai Yamazaki, Tatsuo Suzuki, Masao Kurogi, Takahito Kataoka, Masahiro Watanabe, and Masahide Kimoto
Geosci. Model Dev., 12, 2727–2765, https://doi.org/10.5194/gmd-12-2727-2019, https://doi.org/10.5194/gmd-12-2727-2019, 2019
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For a deeper understanding of a wide range of climate science issues, the latest version of the Japanese climate model, called MIROC6, was developed. The climate model represents observed mean climate and climate variations well, for example tropical precipitation, the midlatitude westerlies, and the East Asian monsoon, which influence human activity all over the world. The improved climate simulations could add reliability to climate predictions under global warming.
Zhiyan Li, Renzhi Hu, Pinhua Xie, Hao Chen, Xiaoyan Liu, Shuaixi Liang, Dan Wang, Fengyang Wang, Yihui Wang, Chuan Lin, Jianguo Liu, and Wenqing Liu
Atmos. Meas. Tech., 12, 3223–3236, https://doi.org/10.5194/amt-12-3223-2019, https://doi.org/10.5194/amt-12-3223-2019, 2019
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A dual-channel CRDS system for NO2 and NO detection is reported. The detection limits of the developed CRDS system for NO2 and NOx measurements are estimated to be about 0.030 ppb (1σ, 1 s) and 0.040 ppb (1σ, 1 s), respectively. The measurements of on-road vehicle emission plumes by this mobile CRDS instrument show the different emission characteristics in the urban and suburban areas of Hefei. The instrument provides a new method for retrieving fast variations in NO and NO2 plumes.
Keiichiro Hara, Kengo Sudo, Takato Ohnishi, Kazuo Osada, Masanori Yabuki, Masataka Shiobara, and Takashi Yamanouchi
Atmos. Chem. Phys., 19, 7817–7837, https://doi.org/10.5194/acp-19-7817-2019, https://doi.org/10.5194/acp-19-7817-2019, 2019
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We measured equivalent black carbon (EBC) concentrations at Syowa Station, Antarctica, from February 2005. EBC might be transported directly to Syowa Station from mid-latitudes mainly via the boundary layer and the lower free troposphere. Some BC was transported to Antarctic regions via the upper free troposphere. Biomass burning in South America and southern Africa is the most dominant source. Fossil fuel combustion in South America and southern Africa also have important contributions.
Zongbo Shi, Tuan Vu, Simone Kotthaus, Roy M. Harrison, Sue Grimmond, Siyao Yue, Tong Zhu, James Lee, Yiqun Han, Matthias Demuzere, Rachel E. Dunmore, Lujie Ren, Di Liu, Yuanlin Wang, Oliver Wild, James Allan, W. Joe Acton, Janet Barlow, Benjamin Barratt, David Beddows, William J. Bloss, Giulia Calzolai, David Carruthers, David C. Carslaw, Queenie Chan, Lia Chatzidiakou, Yang Chen, Leigh Crilley, Hugh Coe, Tie Dai, Ruth Doherty, Fengkui Duan, Pingqing Fu, Baozhu Ge, Maofa Ge, Daobo Guan, Jacqueline F. Hamilton, Kebin He, Mathew Heal, Dwayne Heard, C. Nicholas Hewitt, Michael Hollaway, Min Hu, Dongsheng Ji, Xujiang Jiang, Rod Jones, Markus Kalberer, Frank J. Kelly, Louisa Kramer, Ben Langford, Chun Lin, Alastair C. Lewis, Jie Li, Weijun Li, Huan Liu, Junfeng Liu, Miranda Loh, Keding Lu, Franco Lucarelli, Graham Mann, Gordon McFiggans, Mark R. Miller, Graham Mills, Paul Monk, Eiko Nemitz, Fionna O'Connor, Bin Ouyang, Paul I. Palmer, Carl Percival, Olalekan Popoola, Claire Reeves, Andrew R. Rickard, Longyi Shao, Guangyu Shi, Dominick Spracklen, David Stevenson, Yele Sun, Zhiwei Sun, Shu Tao, Shengrui Tong, Qingqing Wang, Wenhua Wang, Xinming Wang, Xuejun Wang, Zifang Wang, Lianfang Wei, Lisa Whalley, Xuefang Wu, Zhijun Wu, Pinhua Xie, Fumo Yang, Qiang Zhang, Yanli Zhang, Yuanhang Zhang, and Mei Zheng
Atmos. Chem. Phys., 19, 7519–7546, https://doi.org/10.5194/acp-19-7519-2019, https://doi.org/10.5194/acp-19-7519-2019, 2019
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APHH-Beijing is a collaborative international research programme to study the sources, processes and health effects of air pollution in Beijing. This introduction to the special issue provides an overview of (i) the APHH-Beijing programme, (ii) the measurement and modelling activities performed as part of it and (iii) the air quality and meteorological conditions during joint intensive field campaigns as a core activity within APHH-Beijing.
Yugo Kanaya, Kazuyuki Miyazaki, Fumikazu Taketani, Takuma Miyakawa, Hisahiro Takashima, Yuichi Komazaki, Xiaole Pan, Saki Kato, Kengo Sudo, Takashi Sekiya, Jun Inoue, Kazutoshi Sato, and Kazuhiro Oshima
Atmos. Chem. Phys., 19, 7233–7254, https://doi.org/10.5194/acp-19-7233-2019, https://doi.org/10.5194/acp-19-7233-2019, 2019
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Ozone and carbon monoxide levels were uniquely observed (for > 10 000 h) over oceans from 67° S to 75° N. Tropospheric chemistry reanalysis v2 reproduced the observed evolution of pollution plumes from continents but underpredicted and overpredicted ozone levels in the Arctic and in the western Pacific equatorial region, respectively. Processes to explain the gaps are proposed, including halogen-mediated destruction in the low latitudes. Our open data set will complement the TOAR data collection.
Zainab Q. Hakim, Scott Archer-Nicholls, Gufran Beig, Gerd A. Folberth, Kengo Sudo, Nathan Luke Abraham, Sachin Ghude, Daven K. Henze, and Alexander T. Archibald
Atmos. Chem. Phys., 19, 6437–6458, https://doi.org/10.5194/acp-19-6437-2019, https://doi.org/10.5194/acp-19-6437-2019, 2019
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Surface ozone is an important air pollutant and recent work has calculated that large numbers of people die prematurely because of exposure to high levels of surface ozone in India. However, these calculations require model simulations of ozone as key inputs.
Here we perform the most thorough evaluation of global model surface ozone over India to date. These analyses of model simulations and observations highlight some successes and shortcomings and the need for further process-based studies.
Shuaixi Liang, Min Qin, Pinhua Xie, Jun Duan, Wu Fang, Yabai He, Jin Xu, Jingwei Liu, Xin Li, Ke Tang, Fanhao Meng, Kaidi Ye, Jianguo Liu, and Wenqing Liu
Atmos. Meas. Tech., 12, 2499–2512, https://doi.org/10.5194/amt-12-2499-2019, https://doi.org/10.5194/amt-12-2499-2019, 2019
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A home-built instrument of an incoherent broadband cavity-enhanced absorption spectrometer is reported for sensitive detection of CHOCHO and NO2 in China's highly polluted environment. An NO2 spectral profile measured using the same spectrometer is applied as a reference spectral profile in the subsequent atmospheric spectral analysis and retrieval of NO2 and CHOCHO. This will provide an idea for solving the problem of cross-interference of strongly absorbing gases in weakly absorbing gases.
Xin Tian, Pinhua Xie, Jin Xu, Yang Wang, Ang Li, Fengcheng Wu, Zhaokun Hu, Cheng Liu, and Qiong Zhang
Atmos. Chem. Phys., 19, 3375–3393, https://doi.org/10.5194/acp-19-3375-2019, https://doi.org/10.5194/acp-19-3375-2019, 2019
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We used the MAX-DOAS instrument installed at the UCAS, Beijing, to evaluate effects on HCHO. The daily variation, transport, sources, and the effect of APEC emission control measures on HCHO were analyzed. Dependences of HCHO VCDs on wind fields indicated that the HCHO values were affected by the transport of pollutants from the south. The results from comparing the MAX-DOAS with the CAMS model indicate the CAMS model can simulate the effects of transport and the secondary sources of HCHO well.
Kai-Lan Chang, Owen R. Cooper, J. Jason West, Marc L. Serre, Martin G. Schultz, Meiyun Lin, Virginie Marécal, Béatrice Josse, Makoto Deushi, Kengo Sudo, Junhua Liu, and Christoph A. Keller
Geosci. Model Dev., 12, 955–978, https://doi.org/10.5194/gmd-12-955-2019, https://doi.org/10.5194/gmd-12-955-2019, 2019
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We developed a new method for combining surface ozone observations from thousands of monitoring sites worldwide with the output from multiple atmospheric chemistry models. The result is a global surface ozone distribution with greater accuracy than any single model can achieve. We focused on an ozone metric relevant to human mortality caused by long-term ozone exposure. Our method can be applied to studies that quantify the impacts of ozone on human health and mortality.
Hitoshi Irie, Hossain Mohammed Syedul Hoque, Alessandro Damiani, Hiroshi Okamoto, Al Mashroor Fatmi, Pradeep Khatri, Tamio Takamura, and Thanawat Jarupongsakul
Atmos. Meas. Tech., 12, 599–606, https://doi.org/10.5194/amt-12-599-2019, https://doi.org/10.5194/amt-12-599-2019, 2019
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The first intensive multicomponent observation by sky radiometer and MAX-DOAS was performed in Thailand during the 2016 dry season. We found that the concentration of formaldehyde (HCHO) was a useful tracer for biomass burning plumes. With the HCHO enhancement, the ratio of gaseous glyoxal to HCHO concentrations decreased and the aerosol absorption optical depths (AAODs) increased. The wavelength dependence of AAODs was quantified, providing evidence for the presence of brown carbon aerosols.
Mengyao Liu, Jintai Lin, K. Folkert Boersma, Gaia Pinardi, Yang Wang, Julien Chimot, Thomas Wagner, Pinhua Xie, Henk Eskes, Michel Van Roozendael, François Hendrick, Pucai Wang, Ting Wang, Yingying Yan, Lulu Chen, and Ruijing Ni
Atmos. Meas. Tech., 12, 1–21, https://doi.org/10.5194/amt-12-1-2019, https://doi.org/10.5194/amt-12-1-2019, 2019
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China has become the world’s largest emitter of NOx, which mainly comes from vehicle exhaust, power plants, etc. However, there are no official ground-based measurements before 2013, so satellites have been widely used to monitor and analyze NOx pollution here. Aerosol is the key factor influencing the accuracy of the satellite NOx product. Our study provides a more accurate way to account for aerosol's influence compared to current widely used products.
K. Folkert Boersma, Henk J. Eskes, Andreas Richter, Isabelle De Smedt, Alba Lorente, Steffen Beirle, Jos H. G. M. van Geffen, Marina Zara, Enno Peters, Michel Van Roozendael, Thomas Wagner, Joannes D. Maasakkers, Ronald J. van der A, Joanne Nightingale, Anne De Rudder, Hitoshi Irie, Gaia Pinardi, Jean-Christopher Lambert, and Steven C. Compernolle
Atmos. Meas. Tech., 11, 6651–6678, https://doi.org/10.5194/amt-11-6651-2018, https://doi.org/10.5194/amt-11-6651-2018, 2018
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This paper describes a new, improved data record of 22+ years of coherent nitrogen dioxide (NO2) pollution measurements from different satellite instruments. Our work helps to ensure that climate data are of sufficient quality to draw reliable conclusions and shape decisions. It shows how dedicated intercomparisons of retrieval sub-steps have led to improved NO2 measurements from the GOME, SCIAMACHY, GOME-2(A), and OMI sensors, and how quality assurance of the new data product is achieved.
Xinyi Dong, Joshua S. Fu, Qingzhao Zhu, Jian Sun, Jiani Tan, Terry Keating, Takashi Sekiya, Kengo Sudo, Louisa Emmons, Simone Tilmes, Jan Eiof Jonson, Michael Schulz, Huisheng Bian, Mian Chin, Yanko Davila, Daven Henze, Toshihiko Takemura, Anna Maria Katarina Benedictow, and Kan Huang
Atmos. Chem. Phys., 18, 15581–15600, https://doi.org/10.5194/acp-18-15581-2018, https://doi.org/10.5194/acp-18-15581-2018, 2018
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We have applied the HTAP phase II multi-model data to investigate the long-range transport impacts on surface concentration and column density of PM from Europe and Russia, Belarus, and Ukraine to eastern Asia, with a special focus on the long-range transport contribution during haze episodes in China. We found that long-range transport plays a more important role in elevating the background concentration of surface PM during the haze days.
Jan Eiof Jonson, Michael Schulz, Louisa Emmons, Johannes Flemming, Daven Henze, Kengo Sudo, Marianne Tronstad Lund, Meiyun Lin, Anna Benedictow, Brigitte Koffi, Frank Dentener, Terry Keating, Rigel Kivi, and Yanko Davila
Atmos. Chem. Phys., 18, 13655–13672, https://doi.org/10.5194/acp-18-13655-2018, https://doi.org/10.5194/acp-18-13655-2018, 2018
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Focusing on Europe, this HTAP 2 study computes ozone in several global models when reducing anthropogenic emissions by 20 % in different world regions. The differences in model results are explored
by use of a novel stepwise approach combining a tracer, CO and ozone. For ozone the contributions from the rest of the world are larger than from Europe, with the largest contributions from North America and eastern Asia. Contributions do, however, depend on the choice of ozone metric.
Pakawat Phalitnonkiat, Peter G. M. Hess, Mircea D. Grigoriu, Gennady Samorodnitsky, Wenxiu Sun, Ellie Beaudry, Simone Tilmes, Makato Deushi, Beatrice Josse, David Plummer, and Kengo Sudo
Atmos. Chem. Phys., 18, 11927–11948, https://doi.org/10.5194/acp-18-11927-2018, https://doi.org/10.5194/acp-18-11927-2018, 2018
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The co-occurrence of heat waves and pollution events and the resulting high mortality rates emphasize the importance of the co-occurrence of pollution and temperature extremes. We analyze ozone and temperature extremes and their joint occurrence over the United States during the summer months (JJA) in measurement data and in model simulations of the present and future climates.
Wenfu Tang, Avelino F. Arellano, Joshua P. DiGangi, Yonghoon Choi, Glenn S. Diskin, Anna Agustí-Panareda, Mark Parrington, Sebastien Massart, Benjamin Gaubert, Youngjae Lee, Danbi Kim, Jinsang Jung, Jinkyu Hong, Je-Woo Hong, Yugo Kanaya, Mindo Lee, Ryan M. Stauffer, Anne M. Thompson, James H. Flynn, and Jung-Hun Woo
Atmos. Chem. Phys., 18, 11007–11030, https://doi.org/10.5194/acp-18-11007-2018, https://doi.org/10.5194/acp-18-11007-2018, 2018
Jun Duan, Min Qin, Bin Ouyang, Wu Fang, Xin Li, Keding Lu, Ke Tang, Shuaixi Liang, Fanhao Meng, Zhaokun Hu, Pinhua Xie, Wenqing Liu, and Rolf Häsler
Atmos. Meas. Tech., 11, 4531–4543, https://doi.org/10.5194/amt-11-4531-2018, https://doi.org/10.5194/amt-11-4531-2018, 2018
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We report a custom-built instrument for simultaneous unambiguous measurements of HONO and NO2 based on incoherent broadband cavity enhanced absorption spectroscopy (IBBCEAS). The current IBBCEAS instrument has made significant improvements in terms of efficient sampling as well as resistance against vibration; temperature change and the measurement precisions (2σ) for HONO are about 180 and 340 ppt in 30 s, respectively. The field inter-comparison and the mobile measurements are present.
Ciao-Kai Liang, J. Jason West, Raquel A. Silva, Huisheng Bian, Mian Chin, Yanko Davila, Frank J. Dentener, Louisa Emmons, Johannes Flemming, Gerd Folberth, Daven Henze, Ulas Im, Jan Eiof Jonson, Terry J. Keating, Tom Kucsera, Allen Lenzen, Meiyun Lin, Marianne Tronstad Lund, Xiaohua Pan, Rokjin J. Park, R. Bradley Pierce, Takashi Sekiya, Kengo Sudo, and Toshihiko Takemura
Atmos. Chem. Phys., 18, 10497–10520, https://doi.org/10.5194/acp-18-10497-2018, https://doi.org/10.5194/acp-18-10497-2018, 2018
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Emissions from one continent affect air quality and health elsewhere. Here we quantify the effects of intercontinental PM2.5 and ozone transport on human health using a new multi-model ensemble, evaluating the health effects of emissions from six world regions and three emission source sectors. Emissions from one region have significant health impacts outside of that source region; similarly, foreign emissions contribute significantly to air-pollution-related deaths in several world regions.
Juan Cuesta, Yugo Kanaya, Masayuki Takigawa, Gaëlle Dufour, Maxim Eremenko, Gilles Foret, Kazuyuki Miyazaki, and Matthias Beekmann
Atmos. Chem. Phys., 18, 9499–9525, https://doi.org/10.5194/acp-18-9499-2018, https://doi.org/10.5194/acp-18-9499-2018, 2018
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This paper tackles a major issue for air quality over East Asia: ozone pollution produced over a major source, like the North China Plain, and the contribution of ozone produced while being transported across the continent and the surrounding seas. The main originality of the paper lays in the fact that this photochemical production of ozone is observationally quantified with new multispectral satellite observations offering unique skills to observe the ozone pollution plumes near the surface.
Stefano Galmarini, Ioannis Kioutsioukis, Efisio Solazzo, Ummugulsum Alyuz, Alessandra Balzarini, Roberto Bellasio, Anna M. K. Benedictow, Roberto Bianconi, Johannes Bieser, Joergen Brandt, Jesper H. Christensen, Augustin Colette, Gabriele Curci, Yanko Davila, Xinyi Dong, Johannes Flemming, Xavier Francis, Andrea Fraser, Joshua Fu, Daven K. Henze, Christian Hogrefe, Ulas Im, Marta Garcia Vivanco, Pedro Jiménez-Guerrero, Jan Eiof Jonson, Nutthida Kitwiroon, Astrid Manders, Rohit Mathur, Laura Palacios-Peña, Guido Pirovano, Luca Pozzoli, Marie Prank, Martin Schultz, Rajeet S. Sokhi, Kengo Sudo, Paolo Tuccella, Toshihiko Takemura, Takashi Sekiya, and Alper Unal
Atmos. Chem. Phys., 18, 8727–8744, https://doi.org/10.5194/acp-18-8727-2018, https://doi.org/10.5194/acp-18-8727-2018, 2018
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An ensemble of model results relating to ozone concentrations in Europe in 2010 has been produced and studied. The novelty consists in the fact that the ensemble is made of results of models working at two different scales (regional and global), therefore contributing in detail two different parts of the atmospheric spectrum. The ensemble defined as a hybrid has been studied in detail and shown to bring additional value to the assessment of air quality.
Sandip S. Dhomse, Douglas Kinnison, Martyn P. Chipperfield, Ross J. Salawitch, Irene Cionni, Michaela I. Hegglin, N. Luke Abraham, Hideharu Akiyoshi, Alex T. Archibald, Ewa M. Bednarz, Slimane Bekki, Peter Braesicke, Neal Butchart, Martin Dameris, Makoto Deushi, Stacey Frith, Steven C. Hardiman, Birgit Hassler, Larry W. Horowitz, Rong-Ming Hu, Patrick Jöckel, Beatrice Josse, Oliver Kirner, Stefanie Kremser, Ulrike Langematz, Jared Lewis, Marion Marchand, Meiyun Lin, Eva Mancini, Virginie Marécal, Martine Michou, Olaf Morgenstern, Fiona M. O'Connor, Luke Oman, Giovanni Pitari, David A. Plummer, John A. Pyle, Laura E. Revell, Eugene Rozanov, Robyn Schofield, Andrea Stenke, Kane Stone, Kengo Sudo, Simone Tilmes, Daniele Visioni, Yousuke Yamashita, and Guang Zeng
Atmos. Chem. Phys., 18, 8409–8438, https://doi.org/10.5194/acp-18-8409-2018, https://doi.org/10.5194/acp-18-8409-2018, 2018
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We analyse simulations from the Chemistry-Climate Model Initiative (CCMI) to estimate the return dates of the stratospheric ozone layer from depletion by anthropogenic chlorine and bromine. The simulations from 20 models project that global column ozone will return to 1980 values in 2047 (uncertainty range 2042–2052). Return dates in other regions vary depending on factors related to climate change and importance of chlorine and bromine. Column ozone in the tropics may continue to decline.
Jiani Tan, Joshua S. Fu, Frank Dentener, Jian Sun, Louisa Emmons, Simone Tilmes, Kengo Sudo, Johannes Flemming, Jan Eiof Jonson, Sylvie Gravel, Huisheng Bian, Yanko Davila, Daven K. Henze, Marianne T. Lund, Tom Kucsera, Toshihiko Takemura, and Terry Keating
Atmos. Chem. Phys., 18, 6847–6866, https://doi.org/10.5194/acp-18-6847-2018, https://doi.org/10.5194/acp-18-6847-2018, 2018
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We study the distributions of sulfur and nitrogen deposition, which are associated with current environmental issues such as formation of acid rain and ecosystem eutrophication and result in widespread problems such as loss of environmental diversity, harming the crop yield and even food insecurity. According to our study, both the amount and distribution of sulfate and nitrogen deposition have changed significantly in the last decade, particularly in East Asia, South Asia and Southeast Asia.
Alessandro Damiani, Hitoshi Irie, Takashi Horio, Tamio Takamura, Pradeep Khatri, Hideaki Takenaka, Takashi Nagao, Takashi Y. Nakajima, and Raul R. Cordero
Atmos. Meas. Tech., 11, 2501–2521, https://doi.org/10.5194/amt-11-2501-2018, https://doi.org/10.5194/amt-11-2501-2018, 2018
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The Tohoku Earthquake of March 2011 stressed the need for energy source diversity, and the governmental policy in Japan has been stimulating a broader use of
renewable energy. Solar power is potentially able to mitigate climate change triggered by greenhouse gas emissions, but its instability caused by cloudiness
is a critical issue for suppliers. To develop an appropriate control system, surface solar radiation data must be made available as accurately as possible.
Jungbin Mok, Nickolay A. Krotkov, Omar Torres, Hiren Jethva, Zhanqing Li, Jhoon Kim, Ja-Ho Koo, Sujung Go, Hitoshi Irie, Gordon Labow, Thomas F. Eck, Brent N. Holben, Jay Herman, Robert P. Loughman, Elena Spinei, Seoung Soo Lee, Pradeep Khatri, and Monica Campanelli
Atmos. Meas. Tech., 11, 2295–2311, https://doi.org/10.5194/amt-11-2295-2018, https://doi.org/10.5194/amt-11-2295-2018, 2018
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Measuring aerosol absorption from the shortest ultraviolet (UV) to the near-infrared (NIR) wavelengths is important for studies of climate, tropospheric photochemistry, human health, and agricultural productivity. We estimate the accuracy and demonstrate consistency of aerosol absorption retrievals from different instruments, after accounting for spectrally varying surface albedo and gaseous absorption.
Theano Drosoglou, Maria Elissavet Koukouli, Natalia Kouremeti, Alkiviadis F. Bais, Irene Zyrichidou, Dimitris Balis, Ronald J. van der A, Jin Xu, and Ang Li
Atmos. Meas. Tech., 11, 2239–2255, https://doi.org/10.5194/amt-11-2239-2018, https://doi.org/10.5194/amt-11-2239-2018, 2018
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A diurnal pattern of tropospheric NO2 with two maxima around late morning and late afternoon is revealed, reflecting high anthropogenic emissions, and a minimum at noon, due to photochemical destruction of tropospheric NO2. GOME-2B shows the smallest underestimation despite its large pixel size. The distance between the measurement location and the satellite pixel center affects mostly GOME-2B data selection. The effect of clouds is more profound on the selection of OMI overpass data.
Tomohiro O. Sato, Takao M. Sato, Hideo Sagawa, Katsuyuki Noguchi, Naoko Saitoh, Hitoshi Irie, Kazuyuki Kita, Mona E. Mahani, Koji Zettsu, Ryoichi Imasu, Sachiko Hayashida, and Yasuko Kasai
Atmos. Meas. Tech., 11, 1653–1668, https://doi.org/10.5194/amt-11-1653-2018, https://doi.org/10.5194/amt-11-1653-2018, 2018
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Air pollution is one of the world's greatest environmental health risks. Ozone adversely affects human health and agricultural production, and the tropospheric ozone has been increasing globally over the past few decades. We report an advanced method to derive the ozone amount in the lowermost troposphere using multi-spectral measurements (UV, thermal infrared and microwave). Combining the MW measurement with the UV and thermal infrared measurements certainly increased the sensitivity.
Takashi Sekiya, Kazuyuki Miyazaki, Koji Ogochi, Kengo Sudo, and Masayuki Takigawa
Geosci. Model Dev., 11, 959–988, https://doi.org/10.5194/gmd-11-959-2018, https://doi.org/10.5194/gmd-11-959-2018, 2018
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We evaluate global tropospheric NO2 simulations using a chemical transport model (CTM) at horizontal resolutions of 0.56, 1.1, and 2.8°. Agreement against satellite retrievals improved greatly at 0.56 and 1.1° resolutions (compared to 2.8°) over polluted and biomass burning regions, especially over areas with strong local sources, such as a megacity. The evaluations demonstrate the potential of using a high-resolution global CTM for studying megacity-scale air pollutants across the entire globe.
Fengcheng Wu, Pinhua Xie, Ang Li, Fusheng Mou, Hao Chen, Yi Zhu, Tong Zhu, Jianguo Liu, and Wenqing Liu
Atmos. Chem. Phys., 18, 1535–1554, https://doi.org/10.5194/acp-18-1535-2018, https://doi.org/10.5194/acp-18-1535-2018, 2018
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Investigating the temporal and spatial distribution of pollutants, emissions, and pollution transport is necessary to better understand the effect of various sources on air quality. We report on mobile differential optical absorption spectroscopy (mobile DOAS) observations of precursors SO2 and NO2 vertical columns in NCP in the summer of 2013 (from 11 June to 7 July) in this study.
Olaf Morgenstern, Kane A. Stone, Robyn Schofield, Hideharu Akiyoshi, Yousuke Yamashita, Douglas E. Kinnison, Rolando R. Garcia, Kengo Sudo, David A. Plummer, John Scinocca, Luke D. Oman, Michael E. Manyin, Guang Zeng, Eugene Rozanov, Andrea Stenke, Laura E. Revell, Giovanni Pitari, Eva Mancini, Glauco Di Genova, Daniele Visioni, Sandip S. Dhomse, and Martyn P. Chipperfield
Atmos. Chem. Phys., 18, 1091–1114, https://doi.org/10.5194/acp-18-1091-2018, https://doi.org/10.5194/acp-18-1091-2018, 2018
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We assess how ozone as simulated by a group of chemistry–climate models responds to variations in man-made climate gases and ozone-depleting substances. We find some agreement, particularly in the middle and upper stratosphere, but also considerable disagreement elsewhere. Such disagreement affects the reliability of future ozone projections based on these models, and also constitutes a source of uncertainty in climate projections using prescribed ozone derived from these simulations.
Rintaro Okamura, Hironobu Iwabuchi, and K. Sebastian Schmidt
Atmos. Meas. Tech., 10, 4747–4759, https://doi.org/10.5194/amt-10-4747-2017, https://doi.org/10.5194/amt-10-4747-2017, 2017
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Three-dimensional (3-D) radiative transfer effects are a major source of retrieval errors in satellite-based optical remote sensing of clouds. Multi-pixel, multispectral approaches based on deep learning are proposed for retrieval of cloud optical thickness and droplet effective radius. A feasibility test shows that proposed retrieval methods are effective to obtain accurate cloud properties. Use of the convolutional neural network is effective to reduce 3-D radiative transfer effects.
Itsushi Uno, Kazuo Osada, Keiya Yumimoto, Zhe Wang, Syuichi Itahashi, Xiaole Pan, Yukari Hara, Yugo Kanaya, Shigekazu Yamamoto, and Thomas Duncan Fairlie
Atmos. Chem. Phys., 17, 14181–14197, https://doi.org/10.5194/acp-17-14181-2017, https://doi.org/10.5194/acp-17-14181-2017, 2017
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We analyzed long-term fine- and coarse-mode nitrate and related aerosols synergetic observations at Fukuoka, Japan. GEOS Chem model including dust and sea-salt acid uptake processes was used to assess the observed seasonal variation, and the impact of long-range transport from the Asian continent. A numerical model reproduced the seasonal variations of fine aerosols. For coarse nitrate, large-scale dust-nitrate outflow from China was confirmed during all dust events between January and June.
Xiaole Pan, Yugo Kanaya, Fumikazu Taketani, Takuma Miyakawa, Satoshi Inomata, Yuichi Komazaki, Hiroshi Tanimoto, Zhe Wang, Itsushi Uno, and Zifa Wang
Atmos. Chem. Phys., 17, 13001–13016, https://doi.org/10.5194/acp-17-13001-2017, https://doi.org/10.5194/acp-17-13001-2017, 2017
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Characteristics of refractory black carbon (rBC) from open biomass burning (OBB) have a great impact on regional pollution and climate, in particular in East Asia. However, experimental study on characteristics of rBC from agricultural residue burning in East China was limited. This study performed laboratory experiments: we found that emission of rBC is highly related to flaming burning, and non-rBC to smoldering burning. Rapid condensation of semi-volatile organics resulted in coated rBC.
Huisheng Bian, Mian Chin, Didier A. Hauglustaine, Michael Schulz, Gunnar Myhre, Susanne E. Bauer, Marianne T. Lund, Vlassis A. Karydis, Tom L. Kucsera, Xiaohua Pan, Andrea Pozzer, Ragnhild B. Skeie, Stephen D. Steenrod, Kengo Sudo, Kostas Tsigaridis, Alexandra P. Tsimpidi, and Svetlana G. Tsyro
Atmos. Chem. Phys., 17, 12911–12940, https://doi.org/10.5194/acp-17-12911-2017, https://doi.org/10.5194/acp-17-12911-2017, 2017
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Atmospheric nitrate contributes notably to total aerosol mass in the present day and is likely to be more important over the next century, with a projected decline in SO2 and NOx emissions and increase in NH3 emissions. This paper investigates atmospheric nitrate using multiple global models and measurements. The study is part of the AeroCom phase III activity. The study is the first attempt to look at global atmospheric nitrate simulation at physical and chemical process levels.
Yang Wang, Steffen Beirle, Francois Hendrick, Andreas Hilboll, Junli Jin, Aleksandra A. Kyuberis, Johannes Lampel, Ang Li, Yuhan Luo, Lorenzo Lodi, Jianzhong Ma, Monica Navarro, Ivan Ortega, Enno Peters, Oleg L. Polyansky, Julia Remmers, Andreas Richter, Olga Puentedura, Michel Van Roozendael, André Seyler, Jonathan Tennyson, Rainer Volkamer, Pinhua Xie, Nikolai F. Zobov, and Thomas Wagner
Atmos. Meas. Tech., 10, 3719–3742, https://doi.org/10.5194/amt-10-3719-2017, https://doi.org/10.5194/amt-10-3719-2017, 2017
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Slant column densities of nitrous acid (HONO) derived from different MAX-DOAS instruments and retrieval software are systematically compared for the first time during the Multi Axis DOAS – Comparison campaign for Aerosols and Trace gases (MAD-CAT) campaign held at MPIC in Mainz, Germany, from June to October 2013. Through the inter-comparisons and sensitivity studies we quantified the uncertainties in the DOAS fits of HONO from different sources and concluded a recommended setting.
Kohei Ikeda, Hiroshi Tanimoto, Takafumi Sugita, Hideharu Akiyoshi, Yugo Kanaya, Chunmao Zhu, and Fumikazu Taketani
Atmos. Chem. Phys., 17, 10515–10533, https://doi.org/10.5194/acp-17-10515-2017, https://doi.org/10.5194/acp-17-10515-2017, 2017
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Black carbon (BC), also known as soot particles, plays a key role in Arctic warming; hence, an understanding of the major source regions and types is important for its mitigation. We found that Russia was the dominant contributor to Arctic BC at the surface level, while the East Asian contribution was the largest in the middle troposphere and the burden over the Arctic, suggesting that BC emission reduction from Russia and East Asia can help mitigate warming in the Arctic.
Wei Wang, Yuan Tian, Cheng Liu, Youwen Sun, Wenqing Liu, Pinhua Xie, Jianguo Liu, Jin Xu, Isamu Morino, Voltaire A. Velazco, David W. T. Griffith, Justus Notholt, and Thorsten Warneke
Atmos. Meas. Tech., 10, 2627–2643, https://doi.org/10.5194/amt-10-2627-2017, https://doi.org/10.5194/amt-10-2627-2017, 2017
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A ground-based high-resolution Fourier transform spectrometer (FTS) station has been established in Hefei, China to remotely measure CO2, CO and other greenhouse gases. Our research aim is to provide information for constraining regional sources and sinks, and validate satellite data, such as GOSAT, OCO-2 and TANSAT. We investigate the potential of FTS to determine the temporal variability of atmospheric CO2 and CO, and assess the ability of our observations to validate satellite data.
Tatsuya Nagashima, Kengo Sudo, Hajime Akimoto, Junichi Kurokawa, and Toshimasa Ohara
Atmos. Chem. Phys., 17, 8231–8246, https://doi.org/10.5194/acp-17-8231-2017, https://doi.org/10.5194/acp-17-8231-2017, 2017
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We showed the large contribution of different source regions in Asia to the recent increasing trend in surface ozone over Japan by using a global chemical transport model. China accounted for the largest part of the increasing trend, not only through the domestic ozone production (36 %) but also the ozone production in the adjacent countries due to the ozone precursors emitted in China (10 %). Other factors such as temporal change in climate and methane concentration were also investigated.
Takuma Miyakawa, Naga Oshima, Fumikazu Taketani, Yuichi Komazaki, Ayako Yoshino, Akinori Takami, Yutaka Kondo, and Yugo Kanaya
Atmos. Chem. Phys., 17, 5851–5864, https://doi.org/10.5194/acp-17-5851-2017, https://doi.org/10.5194/acp-17-5851-2017, 2017
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We have deployed a single particle soot photometer (SP2) to characterize black carbon (BC) aerosols near industrial sources in Japan in the early summer of 2014 and at a remote island in the spring of 2015. The observed changes in the SP2-derived size distributions and mixing state of BC-containing particles with air mass transport are connected to meteorological variability (transport pathways and air mass histories) in spring in east Asia.
Min Huang, Gregory R. Carmichael, R. Bradley Pierce, Duseong S. Jo, Rokjin J. Park, Johannes Flemming, Louisa K. Emmons, Kevin W. Bowman, Daven K. Henze, Yanko Davila, Kengo Sudo, Jan Eiof Jonson, Marianne Tronstad Lund, Greet Janssens-Maenhout, Frank J. Dentener, Terry J. Keating, Hilke Oetjen, and Vivienne H. Payne
Atmos. Chem. Phys., 17, 5721–5750, https://doi.org/10.5194/acp-17-5721-2017, https://doi.org/10.5194/acp-17-5721-2017, 2017
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In support of the HTAP phase 2 experiment, we conducted a number of regional-scale Sulfur Transport and dEposition Model base and sensitivity simulations over North America during May–June 2010. The STEM chemical boundary conditions were downscaled from three (GEOS-Chem, RAQMS, and ECMWF C-IFS) global chemical transport models' simulations. Analyses were performed on large spatial–temporal scales relative to HTAP1 and also on subcontinental and event scales including the use of satellite data.
Yang Wang, Steffen Beirle, Johannes Lampel, Mariliza Koukouli, Isabelle De Smedt, Nicolas Theys, Ang Li, Dexia Wu, Pinhua Xie, Cheng Liu, Michel Van Roozendael, Trissevgeni Stavrakou, Jean-François Müller, and Thomas Wagner
Atmos. Chem. Phys., 17, 5007–5033, https://doi.org/10.5194/acp-17-5007-2017, https://doi.org/10.5194/acp-17-5007-2017, 2017
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A long-term MAX-DOAS measurement from 2011 to 2014 was operated in Wuxi, part of the most industrialized area of the Yangtze River delta region of China. The tropospheric VCDs and vertical profiles of NO2, SO2 and HCHO derived from the MAX-DOAS are used to validate the products derived from OMI and GOME-2A/B by different scientific teams (daily- and bimonthly-averaged data). We investigate the effects of clouds, aerosols and a priori profile shapes on satellite retrievals of tropospheric VCDs.
Syuichi Itahashi, Itsushi Uno, Kazuo Osada, Yusuke Kamiguchi, Shigekazu Yamamoto, Kei Tamura, Zhe Wang, Yasunori Kurosaki, and Yugo Kanaya
Atmos. Chem. Phys., 17, 3823–3843, https://doi.org/10.5194/acp-17-3823-2017, https://doi.org/10.5194/acp-17-3823-2017, 2017
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Over East Asia, the transboundary air pollution of SO42− has been recognized. The importance of the transboundary air pollution of NO3− in winter was demonstrated in this study through synergetic ground-based observations with state-of-the-art measurements of secondary inorganic aerosols (SO42−, NO3−, and NH4+) and a regional chemical transport model analysis. This study will help to refine the understanding of transboundary heavy PM2.5 pollution in winter.
Enno Peters, Gaia Pinardi, André Seyler, Andreas Richter, Folkard Wittrock, Tim Bösch, Michel Van Roozendael, François Hendrick, Theano Drosoglou, Alkiviadis F. Bais, Yugo Kanaya, Xiaoyi Zhao, Kimberly Strong, Johannes Lampel, Rainer Volkamer, Theodore Koenig, Ivan Ortega, Olga Puentedura, Mónica Navarro-Comas, Laura Gómez, Margarita Yela González, Ankie Piters, Julia Remmers, Yang Wang, Thomas Wagner, Shanshan Wang, Alfonso Saiz-Lopez, David García-Nieto, Carlos A. Cuevas, Nuria Benavent, Richard Querel, Paul Johnston, Oleg Postylyakov, Alexander Borovski, Alexander Elokhov, Ilya Bruchkouski, Haoran Liu, Cheng Liu, Qianqian Hong, Claudia Rivera, Michel Grutter, Wolfgang Stremme, M. Fahim Khokhar, Junaid Khayyam, and John P. Burrows
Atmos. Meas. Tech., 10, 955–978, https://doi.org/10.5194/amt-10-955-2017, https://doi.org/10.5194/amt-10-955-2017, 2017
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This work is about harmonization of differential optical absorption spectroscopy retrieval codes, which is a remote sensing technique widely used to derive atmospheric trace gas amounts. The study is based on ground-based measurements performed during the Multi-Axis DOAS Comparison campaign for Aerosols and Trace gases (MAD-CAT) in Mainz, Germany, in summer 2013. In total, 17 international groups working in the field of the DOAS technique participated in this study.
Yang Wang, Johannes Lampel, Pinhua Xie, Steffen Beirle, Ang Li, Dexia Wu, and Thomas Wagner
Atmos. Chem. Phys., 17, 2189–2215, https://doi.org/10.5194/acp-17-2189-2017, https://doi.org/10.5194/acp-17-2189-2017, 2017
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The air pollution in the Yangtze River delta (YRD), the largest economic region in China, threatens the health of the inhabitants in this region. A long-term MAX-DOAS observation in Wuxi, China (belonging to YRD), is used to characterize vertical distributions (VD) of the aerosols and the precursor trace gases in the boundary to identify the dominating sources. The results are valuable for further validation of satellite products and chemical transport modelings.
Olaf Morgenstern, Michaela I. Hegglin, Eugene Rozanov, Fiona M. O'Connor, N. Luke Abraham, Hideharu Akiyoshi, Alexander T. Archibald, Slimane Bekki, Neal Butchart, Martyn P. Chipperfield, Makoto Deushi, Sandip S. Dhomse, Rolando R. Garcia, Steven C. Hardiman, Larry W. Horowitz, Patrick Jöckel, Beatrice Josse, Douglas Kinnison, Meiyun Lin, Eva Mancini, Michael E. Manyin, Marion Marchand, Virginie Marécal, Martine Michou, Luke D. Oman, Giovanni Pitari, David A. Plummer, Laura E. Revell, David Saint-Martin, Robyn Schofield, Andrea Stenke, Kane Stone, Kengo Sudo, Taichu Y. Tanaka, Simone Tilmes, Yousuke Yamashita, Kohei Yoshida, and Guang Zeng
Geosci. Model Dev., 10, 639–671, https://doi.org/10.5194/gmd-10-639-2017, https://doi.org/10.5194/gmd-10-639-2017, 2017
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We present a review of the make-up of 20 models participating in the Chemistry–Climate Model Initiative (CCMI). In comparison to earlier such activities, most of these models comprise a whole-atmosphere chemistry, and several of them include an interactive ocean module. This makes them suitable for studying the interactions of tropospheric air quality, stratospheric ozone, and climate. The paper lays the foundation for other studies using the CCMI simulations for scientific analysis.
Kazuyuki Miyazaki, Henk Eskes, Kengo Sudo, K. Folkert Boersma, Kevin Bowman, and Yugo Kanaya
Atmos. Chem. Phys., 17, 807–837, https://doi.org/10.5194/acp-17-807-2017, https://doi.org/10.5194/acp-17-807-2017, 2017
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Global surface emissions of nitrogen oxides (NOx) over a 10-year period (2005–2014) are estimated from assimilation of multiple satellite datasets. We present detailed distributions of the estimated NOx emission distributions for all major regions, the diurnal, seasonal, and decadal variability. The estimated emissions show a positive trend over India, China, and the Middle East, and a negative trend over the United States, southern Africa, and western Europe.
Shi Song, K. Sebastian Schmidt, Peter Pilewskie, Michael D. King, Andrew K. Heidinger, Andi Walther, Hironobu Iwabuchi, Gala Wind, and Odele M. Coddington
Atmos. Chem. Phys., 16, 13791–13806, https://doi.org/10.5194/acp-16-13791-2016, https://doi.org/10.5194/acp-16-13791-2016, 2016
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The radiative effects of spatially complex cloud fields are notoriously difficult to estimate and are afflicted with errors up to ±50 % of the incident solar radiation. We find that horizontal photon transport, the leading cause for these three-dimensional effects, manifests itself through a spectral fingerprint – a new observable that holds promise for reducing the errors associated with spatial complexity by moving the problem to the spectral dimension.
Qianqian Hong, Zhouqing Xie, Cheng Liu, Feiyue Wang, Pinhua Xie, Hui Kang, Jin Xu, Jiancheng Wang, Fengcheng Wu, Pengzhen He, Fusheng Mou, Shidong Fan, Yunsheng Dong, Haicong Zhan, Xiawei Yu, Xiyuan Chi, and Jianguo Liu
Atmos. Chem. Phys., 16, 13807–13821, https://doi.org/10.5194/acp-16-13807-2016, https://doi.org/10.5194/acp-16-13807-2016, 2016
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It is known that rapid industrialization in developing countries has led to an increase in air pollution. Here we firstly report the speciated atmospheric mercury during haze days based upon 1-year synchronous observations in an inland city in China. The findings provide direct evidence to understand the biogeochemical cycles of atmospheric mercury related to air pollution and an opportunity to evaluate the potential health risks of atmospheric mercury.
Camilla Weum Stjern, Bjørn Hallvard Samset, Gunnar Myhre, Huisheng Bian, Mian Chin, Yanko Davila, Frank Dentener, Louisa Emmons, Johannes Flemming, Amund Søvde Haslerud, Daven Henze, Jan Eiof Jonson, Tom Kucsera, Marianne Tronstad Lund, Michael Schulz, Kengo Sudo, Toshihiko Takemura, and Simone Tilmes
Atmos. Chem. Phys., 16, 13579–13599, https://doi.org/10.5194/acp-16-13579-2016, https://doi.org/10.5194/acp-16-13579-2016, 2016
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Air pollution can reach distant regions through intercontinental transport. Here we first present results from the Hemispheric Transport of Air Pollution Phase 2 exercise, where many models performed the same set of coordinated emission-reduction experiments. We find that mitigations have considerable extra-regional effects, and show that this is particularly true for black carbon emissions, as long-range transport elevates aerosols to higher levels where their radiative influence is stronger.
Yugo Kanaya, Xiaole Pan, Takuma Miyakawa, Yuichi Komazaki, Fumikazu Taketani, Itsushi Uno, and Yutaka Kondo
Atmos. Chem. Phys., 16, 10689–10705, https://doi.org/10.5194/acp-16-10689-2016, https://doi.org/10.5194/acp-16-10689-2016, 2016
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Wet removal of atmospheric black carbon particles was quantitatively characterized in terms of accumulated precipitation along a backward trajectory (APT) using long-term observations at Fukue Island, western Japan, receiving Asian continental outflow with variable degrees of influence from precipitation. The emission inventory of BC over East Asia was assessed in terms of the observed BC/CO ratios. Model simulations should be diagnosed with these improved knowledge on the emission and removal.
Raquel A. Silva, J. Jason West, Jean-François Lamarque, Drew T. Shindell, William J. Collins, Stig Dalsoren, Greg Faluvegi, Gerd Folberth, Larry W. Horowitz, Tatsuya Nagashima, Vaishali Naik, Steven T. Rumbold, Kengo Sudo, Toshihiko Takemura, Daniel Bergmann, Philip Cameron-Smith, Irene Cionni, Ruth M. Doherty, Veronika Eyring, Beatrice Josse, Ian A. MacKenzie, David Plummer, Mattia Righi, David S. Stevenson, Sarah Strode, Sophie Szopa, and Guang Zengast
Atmos. Chem. Phys., 16, 9847–9862, https://doi.org/10.5194/acp-16-9847-2016, https://doi.org/10.5194/acp-16-9847-2016, 2016
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Using ozone and PM2.5 concentrations from the ACCMIP ensemble of chemistry-climate models for the four Representative Concentration Pathway scenarios (RCPs), together with projections of future population and baseline mortality rates, we quantify the human premature mortality impacts of future ambient air pollution in 2030, 2050 and 2100, relative to 2000 concentrations. We also estimate the global mortality burden of ozone and PM2.5 in 2000 and each future period.
U. Frieß, H. Klein Baltink, S. Beirle, K. Clémer, F. Hendrick, B. Henzing, H. Irie, G. de Leeuw, A. Li, M. M. Moerman, M. van Roozendael, R. Shaiganfar, T. Wagner, Y. Wang, P. Xie, S. Yilmaz, and P. Zieger
Atmos. Meas. Tech., 9, 3205–3222, https://doi.org/10.5194/amt-9-3205-2016, https://doi.org/10.5194/amt-9-3205-2016, 2016
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This article describes the first direct comparison of aerosol extinction profiles from Multi-Axis DOAS measurements of the oxygen collision complex using five different retrieval algorithms. A comparison of the retrieved profiles with co-located aerosol measurements shows good agreement with respect to profile shape and aerosol optical thickness. This study shows that MAX-DOAS is a simple, versatile and cost-effective method for the measurement of aerosol properties in the lower troposphere.
Youwen Sun, Cheng Liu, Pinhua Xie, Andreas Hartl, Kalok Chan, Yuan Tian, Wei Wang, Min Qin, Jianguo Liu, and Wenqing Liu
Atmos. Meas. Tech., 9, 1167–1180, https://doi.org/10.5194/amt-9-1167-2016, https://doi.org/10.5194/amt-9-1167-2016, 2016
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SO2 variability over a large concentration range and interferences from other gases have been major limitations in industrial SO2 emission monitoring. This study demonstrates accurate industrial SO2 emission monitoring through a portable multichannel gas analyzer with an optimized retrieval algorithm. The developed instrument shows good performance in both the linear and nonlinear ranges.
Y. Wang, M. Penning de Vries, P. H. Xie, S. Beirle, S. Dörner, J. Remmers, A. Li, and T. Wagner
Atmos. Meas. Tech., 8, 5133–5156, https://doi.org/10.5194/amt-8-5133-2015, https://doi.org/10.5194/amt-8-5133-2015, 2015
G. G. Matvienko, B. D. Belan, M. V. Panchenko, O. A. Romanovskii, S. M. Sakerin, D. M. Kabanov, S. A. Turchinovich, Y. S. Turchinovich, T. A. Eremina, V. S. Kozlov, S. A. Terpugova, V. V. Pol'kin, E. P. Yausheva, D. G. Chernov, T. B. Zhuravleva, T. V. Bedareva, S. L. Odintsov, V. D. Burlakov, A. V. Nevzorov, M. Y. Arshinov, G. A. Ivlev, D. E. Savkin, A. V. Fofonov, V. A. Gladkikh, A. P. Kamardin, Y. S. Balin, G. P. Kokhanenko, I. E. Penner, S. V. Samoilova, P. N. Antokhin, V. G. Arshinova, D. K. Davydov, A. V. Kozlov, D. A. Pestunov, T. M. Rasskazchikova, D. V. Simonenkov, T. K. Sklyadneva, G. N. Tolmachev, S. B. Belan, V. P. Shmargunov, A. S. Kozlov, and S. B. Malyshkin
Atmos. Meas. Tech., 8, 4507–4520, https://doi.org/10.5194/amt-8-4507-2015, https://doi.org/10.5194/amt-8-4507-2015, 2015
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The primary objective of the Complex Aerosol Experiment was measurement of microphysical, chemical, and optical properties of aerosol particles in the surface air layer and free atmosphere. The measurement data were used to retrieve the whole set of aerosol optical parameters, necessary for radiation calculations. Three measurement cycles were performed within the experiment during 2013: in spring, summer (July), and in late summer/early autumn.
M. Saito and H. Iwabuchi
Atmos. Meas. Tech., 8, 4295–4311, https://doi.org/10.5194/amt-8-4295-2015, https://doi.org/10.5194/amt-8-4295-2015, 2015
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A new algorithm for aerosol retrievals from twilight photographs taken by a digital single reflex-lens camera is developed. A radiative transfer model taking spherical-shell atmosphere, multiple scattering and refraction into account is used as a forward model, and the optimal estimation is used as an inversion calculation to infer the aerosol optical and radiative properties. The AOTs are inferred with small uncertainties and agree very well with that from the skyradiometer.
G. Dufour, M. Eremenko, J. Cuesta, C. Doche, G. Foret, M. Beekmann, A. Cheiney, Y. Wang, Z. Cai, Y. Liu, M. Takigawa, Y. Kanaya, and J.-M. Flaud
Atmos. Chem. Phys., 15, 10839–10856, https://doi.org/10.5194/acp-15-10839-2015, https://doi.org/10.5194/acp-15-10839-2015, 2015
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We identify the stratospheric and the photochemical sources contributing to the late-spring O3 distribution over East Asia using IASI O3 and CO observations. Reversible subsiding O3 transfers in the UTLS associated with low-pressure systems impact lower-tropospheric O3 north of 40°N. By contrast, photochemical production from primary pollutants significantly contributes to the enhanced lower-tropospheric O3 over the NCP and photochemical processing occurs within the plume exported from the NCP.
J. L. Schnell, M. J. Prather, B. Josse, V. Naik, L. W. Horowitz, P. Cameron-Smith, D. Bergmann, G. Zeng, D. A. Plummer, K. Sudo, T. Nagashima, D. T. Shindell, G. Faluvegi, and S. A. Strode
Atmos. Chem. Phys., 15, 10581–10596, https://doi.org/10.5194/acp-15-10581-2015, https://doi.org/10.5194/acp-15-10581-2015, 2015
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We test global chemistry--climate models in their ability to simulate present-day surface ozone. Models are tested against observed hourly ozone from 4217 stations in North America and Europe that are averaged over 1°x1° grid cells. Using novel metrics, we find most models match the shape but not the amplitude of regional summertime diurnal and annual cycles and match the pattern but not the magnitude of summer ozone enhancement. Most also match the observed distribution of extreme episode sizes
K. Miyazaki, H. J. Eskes, and K. Sudo
Atmos. Chem. Phys., 15, 8315–8348, https://doi.org/10.5194/acp-15-8315-2015, https://doi.org/10.5194/acp-15-8315-2015, 2015
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This paper reports on an 8-year reanalysis of tropospheric chemistry based on an assimilation of multiple satellite-derived data sets. The reanalysis performed well on regional and global scales and for seasonal and interannual variations. The simultaneous assimilation of multiple-species data, involving the optimisation of both concentration and emission fields, provides unique information on year-to-year variations in the atmospheric environment.
K. Ishijima, M. Takigawa, K. Sudo, S. Toyoda, N. Yoshida, T. Röckmann, J. Kaiser, S. Aoki, S. Morimoto, S. Sugawara, and T. Nakazawa
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-15-19947-2015, https://doi.org/10.5194/acpd-15-19947-2015, 2015
Revised manuscript not accepted
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We developed an atmospheric N2O isotopocule model based on a chemistry-coupled atmospheric general circulation model and a simple method to optimize the model, and estimated the isotopic signatures of surface sources at the hemispheric scale. Data obtained from ground-based observations, measurements of firn air, and balloon and aircraft flights were used to optimize the long-term trends, interhemispheric gradients, and photolytic fractionation, respectively, in the model.
H. Irie, T. Nakayama, A. Shimizu, A. Yamazaki, T. Nagai, A. Uchiyama, Y. Zaizen, S. Kagamitani, and Y. Matsumi
Atmos. Meas. Tech., 8, 2775–2788, https://doi.org/10.5194/amt-8-2775-2015, https://doi.org/10.5194/amt-8-2775-2015, 2015
S.-K. Shin, D. Müller, C. Lee, K. H. Lee, D. Shin, Y. J. Kim, and Y. M. Noh
Atmos. Chem. Phys., 15, 6707–6720, https://doi.org/10.5194/acp-15-6707-2015, https://doi.org/10.5194/acp-15-6707-2015, 2015
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The measurements from 2009 to 2013 using a multiwavelength Raman lidar were conducted to identify the changes in optical properties of East Asian dust. We found that the optical properties of Asian dust change depending on the dust plume's vertical position and the change of vertical position during transport over China. We believe this paper provides a better understanding of the optical properties of mixed Asian dust plums and the effect of long-range transport on dust properties.
X. Pan, Y. Kanaya, H. Tanimoto, S. Inomata, Z. Wang, S. Kudo, and I. Uno
Atmos. Chem. Phys., 15, 6101–6111, https://doi.org/10.5194/acp-15-6101-2015, https://doi.org/10.5194/acp-15-6101-2015, 2015
D. Shin, D. Müller, K. Lee, S. Shin, Y. J. Kim, C. K. Song, and Y. M. Noh
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-15-1171-2015, https://doi.org/10.5194/acpd-15-1171-2015, 2015
Preprint withdrawn
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We present for the first time results of Raman lidar observations of the temporal evolution of a stratospheric aerosol layer observed in the upper troposphere and lower stratosphere over Korea. We find what non-spherical particles may have been present in the lower stratosphere for at least six months after the eruption on the volcano. Our study adds to the limited information on volcanic aerosols over East Asia.
L. N. Lamsal, N. A. Krotkov, E. A. Celarier, W. H. Swartz, K. E. Pickering, E. J. Bucsela, J. F. Gleason, R. V. Martin, S. Philip, H. Irie, A. Cede, J. Herman, A. Weinheimer, J. J. Szykman, and T. N. Knepp
Atmos. Chem. Phys., 14, 11587–11609, https://doi.org/10.5194/acp-14-11587-2014, https://doi.org/10.5194/acp-14-11587-2014, 2014
K. Noguchi, A. Richter, V. Rozanov, A. Rozanov, J. P. Burrows, H. Irie, and K. Kita
Atmos. Meas. Tech., 7, 3497–3508, https://doi.org/10.5194/amt-7-3497-2014, https://doi.org/10.5194/amt-7-3497-2014, 2014
H. Matsui, M. Koike, Y. Kondo, A. Takami, J. D. Fast, Y. Kanaya, and M. Takigawa
Atmos. Chem. Phys., 14, 9513–9535, https://doi.org/10.5194/acp-14-9513-2014, https://doi.org/10.5194/acp-14-9513-2014, 2014
Y. Wang, A. Li, P. H. Xie, T. Wagner, H. Chen, W. Q. Liu, and J. G. Liu
Atmos. Meas. Tech., 7, 1663–1680, https://doi.org/10.5194/amt-7-1663-2014, https://doi.org/10.5194/amt-7-1663-2014, 2014
S. Itahashi, I. Uno, H. Irie, J.-I. Kurokawa, and T. Ohara
Atmos. Chem. Phys., 14, 3623–3635, https://doi.org/10.5194/acp-14-3623-2014, https://doi.org/10.5194/acp-14-3623-2014, 2014
K. Miyazaki, H. J. Eskes, K. Sudo, and C. Zhang
Atmos. Chem. Phys., 14, 3277–3305, https://doi.org/10.5194/acp-14-3277-2014, https://doi.org/10.5194/acp-14-3277-2014, 2014
J.-T. Lin, R. V. Martin, K. F. Boersma, M. Sneep, P. Stammes, R. Spurr, P. Wang, M. Van Roozendael, K. Clémer, and H. Irie
Atmos. Chem. Phys., 14, 1441–1461, https://doi.org/10.5194/acp-14-1441-2014, https://doi.org/10.5194/acp-14-1441-2014, 2014
F. C. Wu, P. H. Xie, A. Li, K. L. Chan, A. Hartl, Y. Wang, F. Q. Si, Y. Zeng, M. Qin, J. Xu, J. G. Liu, W. Q. Liu, and M. Wenig
Atmos. Meas. Tech., 6, 2277–2292, https://doi.org/10.5194/amt-6-2277-2013, https://doi.org/10.5194/amt-6-2277-2013, 2013
Y. Kanaya, H. Akimoto, Z.-F. Wang, P. Pochanart, K. Kawamura, Y. Liu, J. Li, Y. Komazaki, H. Irie, X.-L. Pan, F. Taketani, K. Yamaji, H. Tanimoto, S. Inomata, S. Kato, J. Suthawaree, K. Okuzawa, G. Wang, S. G. Aggarwal, P. Q. Fu, T. Wang, J. Gao, Y. Wang, and G. Zhuang
Atmos. Chem. Phys., 13, 8265–8283, https://doi.org/10.5194/acp-13-8265-2013, https://doi.org/10.5194/acp-13-8265-2013, 2013
K. Kawamura, E. Tachibana, K. Okuzawa, S. G. Aggarwal, Y. Kanaya, and Z. F. Wang
Atmos. Chem. Phys., 13, 8285–8302, https://doi.org/10.5194/acp-13-8285-2013, https://doi.org/10.5194/acp-13-8285-2013, 2013
Y. M. Noh, H. Lee, D. Mueller, K. Lee, D. Shin, S. Shin, T. J. Choi, Y. J. Choi, and K. R. Kim
Atmos. Chem. Phys., 13, 7619–7629, https://doi.org/10.5194/acp-13-7619-2013, https://doi.org/10.5194/acp-13-7619-2013, 2013
N. He, K. Kawamura, K. Okuzawa, Y. Kanaya, and Z. F. Wang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-13-16699-2013, https://doi.org/10.5194/acpd-13-16699-2013, 2013
Revised manuscript not accepted
K. Kawamura, K. Okuzawa, S. G. Aggarwal, H. Irie, Y. Kanaya, and Z. Wang
Atmos. Chem. Phys., 13, 5369–5380, https://doi.org/10.5194/acp-13-5369-2013, https://doi.org/10.5194/acp-13-5369-2013, 2013
H. Irie, K. Yamaji, K. Ikeda, I. Uno, S. Itahashi, T. Ohara, and J. Kurokawa
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-13-14037-2013, https://doi.org/10.5194/acpd-13-14037-2013, 2013
Preprint withdrawn
V. Naik, A. Voulgarakis, A. M. Fiore, L. W. Horowitz, J.-F. Lamarque, M. Lin, M. J. Prather, P. J. Young, D. Bergmann, P. J. Cameron-Smith, I. Cionni, W. J. Collins, S. B. Dalsøren, R. Doherty, V. Eyring, G. Faluvegi, G. A. Folberth, B. Josse, Y. H. Lee, I. A. MacKenzie, T. Nagashima, T. P. C. van Noije, D. A. Plummer, M. Righi, S. T. Rumbold, R. Skeie, D. T. Shindell, D. S. Stevenson, S. Strode, K. Sudo, S. Szopa, and G. Zeng
Atmos. Chem. Phys., 13, 5277–5298, https://doi.org/10.5194/acp-13-5277-2013, https://doi.org/10.5194/acp-13-5277-2013, 2013
K. W. Bowman, D. T. Shindell, H. M. Worden, J.F. Lamarque, P. J. Young, D. S. Stevenson, Z. Qu, M. de la Torre, D. Bergmann, P. J. Cameron-Smith, W. J. Collins, R. Doherty, S. B. Dalsøren, G. Faluvegi, G. Folberth, L. W. Horowitz, B. M. Josse, Y. H. Lee, I. A. MacKenzie, G. Myhre, T. Nagashima, V. Naik, D. A. Plummer, S. T. Rumbold, R. B. Skeie, S. A. Strode, K. Sudo, S. Szopa, A. Voulgarakis, G. Zeng, S. S. Kulawik, A. M. Aghedo, and J. R. Worden
Atmos. Chem. Phys., 13, 4057–4072, https://doi.org/10.5194/acp-13-4057-2013, https://doi.org/10.5194/acp-13-4057-2013, 2013
D. T. Shindell, J.-F. Lamarque, M. Schulz, M. Flanner, C. Jiao, M. Chin, P. J. Young, Y. H. Lee, L. Rotstayn, N. Mahowald, G. Milly, G. Faluvegi, Y. Balkanski, W. J. Collins, A. J. Conley, S. Dalsoren, R. Easter, S. Ghan, L. Horowitz, X. Liu, G. Myhre, T. Nagashima, V. Naik, S. T. Rumbold, R. Skeie, K. Sudo, S. Szopa, T. Takemura, A. Voulgarakis, J.-H. Yoon, and F. Lo
Atmos. Chem. Phys., 13, 2939–2974, https://doi.org/10.5194/acp-13-2939-2013, https://doi.org/10.5194/acp-13-2939-2013, 2013
D. S. Stevenson, P. J. Young, V. Naik, J.-F. Lamarque, D. T. Shindell, A. Voulgarakis, R. B. Skeie, S. B. Dalsoren, G. Myhre, T. K. Berntsen, G. A. Folberth, S. T. Rumbold, W. J. Collins, I. A. MacKenzie, R. M. Doherty, G. Zeng, T. P. C. van Noije, A. Strunk, D. Bergmann, P. Cameron-Smith, D. A. Plummer, S. A. Strode, L. Horowitz, Y. H. Lee, S. Szopa, K. Sudo, T. Nagashima, B. Josse, I. Cionni, M. Righi, V. Eyring, A. Conley, K. W. Bowman, O. Wild, and A. Archibald
Atmos. Chem. Phys., 13, 3063–3085, https://doi.org/10.5194/acp-13-3063-2013, https://doi.org/10.5194/acp-13-3063-2013, 2013
Y. H. Lee, J.-F. Lamarque, M. G. Flanner, C. Jiao, D. T. Shindell, T. Berntsen, M. M. Bisiaux, J. Cao, W. J. Collins, M. Curran, R. Edwards, G. Faluvegi, S. Ghan, L. W. Horowitz, J. R. McConnell, J. Ming, G. Myhre, T. Nagashima, V. Naik, S. T. Rumbold, R. B. Skeie, K. Sudo, T. Takemura, F. Thevenon, B. Xu, and J.-H. Yoon
Atmos. Chem. Phys., 13, 2607–2634, https://doi.org/10.5194/acp-13-2607-2013, https://doi.org/10.5194/acp-13-2607-2013, 2013
A. Voulgarakis, V. Naik, J.-F. Lamarque, D. T. Shindell, P. J. Young, M. J. Prather, O. Wild, R. D. Field, D. Bergmann, P. Cameron-Smith, I. Cionni, W. J. Collins, S. B. Dalsøren, R. M. Doherty, V. Eyring, G. Faluvegi, G. A. Folberth, L. W. Horowitz, B. Josse, I. A. MacKenzie, T. Nagashima, D. A. Plummer, M. Righi, S. T. Rumbold, D. S. Stevenson, S. A. Strode, K. Sudo, S. Szopa, and G. Zeng
Atmos. Chem. Phys., 13, 2563–2587, https://doi.org/10.5194/acp-13-2563-2013, https://doi.org/10.5194/acp-13-2563-2013, 2013
P. J. Young, A. T. Archibald, K. W. Bowman, J.-F. Lamarque, V. Naik, D. S. Stevenson, S. Tilmes, A. Voulgarakis, O. Wild, D. Bergmann, P. Cameron-Smith, I. Cionni, W. J. Collins, S. B. Dalsøren, R. M. Doherty, V. Eyring, G. Faluvegi, L. W. Horowitz, B. Josse, Y. H. Lee, I. A. MacKenzie, T. Nagashima, D. A. Plummer, M. Righi, S. T. Rumbold, R. B. Skeie, D. T. Shindell, S. A. Strode, K. Sudo, S. Szopa, and G. Zeng
Atmos. Chem. Phys., 13, 2063–2090, https://doi.org/10.5194/acp-13-2063-2013, https://doi.org/10.5194/acp-13-2063-2013, 2013
J.-F. Lamarque, D. T. Shindell, B. Josse, P. J. Young, I. Cionni, V. Eyring, D. Bergmann, P. Cameron-Smith, W. J. Collins, R. Doherty, S. Dalsoren, G. Faluvegi, G. Folberth, S. J. Ghan, L. W. Horowitz, Y. H. Lee, I. A. MacKenzie, T. Nagashima, V. Naik, D. Plummer, M. Righi, S. T. Rumbold, M. Schulz, R. B. Skeie, D. S. Stevenson, S. Strode, K. Sudo, S. Szopa, A. Voulgarakis, and G. Zeng
Geosci. Model Dev., 6, 179–206, https://doi.org/10.5194/gmd-6-179-2013, https://doi.org/10.5194/gmd-6-179-2013, 2013
G. Pinardi, M. Van Roozendael, N. Abuhassan, C. Adams, A. Cede, K. Clémer, C. Fayt, U. Frieß, M. Gil, J. Herman, C. Hermans, F. Hendrick, H. Irie, A. Merlaud, M. Navarro Comas, E. Peters, A. J. M. Piters, O. Puentedura, A. Richter, A. Schönhardt, R. Shaiganfar, E. Spinei, K. Strong, H. Takashima, M. Vrekoussis, T. Wagner, F. Wittrock, and S. Yilmaz
Atmos. Meas. Tech., 6, 167–185, https://doi.org/10.5194/amt-6-167-2013, https://doi.org/10.5194/amt-6-167-2013, 2013
Related subject area
Subject: Gases | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Vertical profiles of global tropospheric nitrogen dioxide (NO2) obtained by cloud slicing the TROPOspheric Monitoring Instrument (TROPOMI)
Opinion: Beyond global means – novel space-based approaches to indirectly constrain the concentrations of and trends and variations in the tropospheric hydroxyl radical (OH)
Satellite-observed relationships between land cover, burned area, and atmospheric composition over the southern Amazon
Ammonia emission estimates using CrIS satellite observations over Europe
Insights into the long-term (2005–2021) spatiotemporal evolution of summer ozone production sensitivity in the Northern Hemisphere derived with the Ozone Monitoring Instrument (OMI)
Tropical tropospheric ozone distribution and trends from in situ and satellite data
Estimation of ground-level NO2 and its spatiotemporal variations in China using GEMS measurements and a nested machine learning model
Unleashing the Potential of Geostationary Satellite Observations in Air Quality Forecasting Through Artificial Intelligence Techniques
Investigation of the impact of satellite vertical sensitivity on long-term retrieved lower-tropospheric ozone trends
Quantifying the diurnal variation in atmospheric NO2 from Geostationary Environment Monitoring Spectrometer (GEMS) observations
Global seasonal urban, industrial, and background NO2 estimated from TROPOMI satellite observations
What can we learn about tropospheric OH from satellite observations of methane?
Feasibility of robust estimates of ozone production rates using satellite observations
Identifying Missing Sources and Reducing NOx Emissions Uncertainty over China using Daily Satellite Data and a Mass-Conserving Method
Ammonia in the upper troposphere–lower stratosphere (UTLS): GLORIA airborne measurements for CAMS model evaluation in the Asian monsoon and in biomass burning plumes above the South Atlantic
A lightweight NO2-to-NOx conversion model for quantifying NOx emissions of point sources from NO2 satellite observations
Towards a sector-specific CO∕CO2 emission ratio: satellite-based observations of CO release from steel production in Germany
Monitoring European anthropogenic NOx emissions from space
Upper tropospheric pollutants observed by MIPAS: geographic and seasonal variations
Comparing space-based to reported carbon monoxide emission estimates for Europe’s iron & steel plants
Opposite variations of peak and low ozone concentrations in eastern China: Positive effects of NOx control on ozone pollution
Pyrogenic HONO seen from space: insights from global IASI observations
First evaluation of the GEMS formaldehyde product against TROPOMI and ground-based column measurements during the in-orbit test period
High-resolution mapping of nitrogen oxide emissions in large US cities from TROPOMI retrievals of tropospheric nitrogen dioxide columns
Quantifying the tropospheric ozone radiative effect and its temporal evolution in the satellite era
Tropical upper tropospheric trends in ozone and carbon monoxide (2005–2020): observational and model results
A satellite chronology of plumes from the April 2021 eruption of La Soufrière, St Vincent
Investigation of spatial and temporal variability in lower tropospheric ozone from RAL Space UV–Vis satellite products
Two years of satellite-based carbon dioxide emission quantification at the world's largest coal-fired power plants
Tropical tropospheric ozone and carbon monoxide distributions: characteristics, origins, and control factors, as seen by IAGOS and IASI
Investigation of the summer 2018 European ozone air pollution episodes using novel satellite data and modelling
Bridging the spatial gaps of the Ammonia Monitoring Network using satellite ammonia measurements
A roadmap to estimating agricultural ammonia volatilization over Europe using satellite observations and simulation data
Investigation of meteorological conditions and BrO during ozone depletion events in Ny-Ålesund between 2010 and 2021
Quantification of carbon monoxide emissions from African cities using TROPOMI
Nitrogen oxides emissions from selected cities in North America, Europe, and East Asia observed by the TROPOspheric Monitoring Instrument (TROPOMI) before and after the COVID-19 pandemic
Remotely sensed and surface measurement- derived mass-conserving inversion of daily NOx emissions and inferred combustion technologies in energy-rich northern China
Examining TROPOMI formaldehyde to nitrogen dioxide ratios in the Lake Michigan region: implications for ozone exceedances
Impact of different sources of precursors on an ozone pollution outbreak over Europe analysed with IASI+GOME2 multispectral satellite observations and model simulations
Monitoring and quantifying CO2 emissions of isolated power plants from space
Technical note: Constraining the hydroxyl (OH) radical in the tropics with satellite observations of its drivers – first steps toward assessing the feasibility of a global observation strategy
Significant contribution of inland ships to the total NOx emissions along the Yangtze River
Characteristics of interannual variability in space-based XCO2 global observations
Toward a versatile spaceborne architecture for immediate monitoring of the global methane pledge
Methane emissions are predominantly responsible for record-breaking atmospheric methane growth rates in 2020 and 2021
Ground solar absorption observations of total column CO, CO2, CH4, and aerosol optical depth from California's Sequoia Lightning Complex Fire: emission factors and modified combustion efficiency at regional scales
Potential of TROPOMI for understanding spatio-temporal variations in surface NO2 and their dependencies upon land use over the Iberian Peninsula
Mobile MAX-DOAS observations of tropospheric NO2 and HCHO during summer over the Three Rivers' Source region in China
Estimating enhancement ratios of nitrogen dioxide, carbon monoxide and carbon dioxide using satellite observations
Source mechanisms and transport patterns of tropospheric bromine monoxide: findings from long-term multi-axis differential optical absorption spectroscopy measurements at two Antarctic stations
Rebekah P. Horner, Eloise A. Marais, Nana Wei, Robert G. Ryan, and Viral Shah
Atmos. Chem. Phys., 24, 13047–13064, https://doi.org/10.5194/acp-24-13047-2024, https://doi.org/10.5194/acp-24-13047-2024, 2024
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Nitrogen oxides (NOx ≡ NO + NO2) affect tropospheric ozone and the hydroxyl radical, influencing climate and atmospheric oxidation. To address the lack of routine observations of NOx, we cloud slice satellite observations of NO2 to derive a new dataset of global vertical profiles of NO2. We evaluate our data against in situ aircraft observations and use these data to critique the contemporary understanding of tropospheric NOx, as simulated by the GEOS-Chem model.
Bryan N. Duncan, Daniel C. Anderson, Arlene M. Fiore, Joanna Joiner, Nickolay A. Krotkov, Can Li, Dylan B. Millet, Julie M. Nicely, Luke D. Oman, Jason M. St. Clair, Joshua D. Shutter, Amir H. Souri, Sarah A. Strode, Brad Weir, Glenn M. Wolfe, Helen M. Worden, and Qindan Zhu
Atmos. Chem. Phys., 24, 13001–13023, https://doi.org/10.5194/acp-24-13001-2024, https://doi.org/10.5194/acp-24-13001-2024, 2024
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Trace gases emitted to or formed within the atmosphere may be chemically or physically removed from the atmosphere. One trace gas, the hydroxyl radical (OH), is responsible for initiating the chemical removal of many trace gases, including some greenhouse gases. Despite its importance, scientists have not been able to adequately measure OH. In this opinion piece, we discuss promising new methods to indirectly constrain OH using satellite data of trace gases that control the abundance of OH.
Emma Sands, Richard J. Pope, Ruth M. Doherty, Fiona M. O'Connor, Chris Wilson, and Hugh Pumphrey
Atmos. Chem. Phys., 24, 11081–11102, https://doi.org/10.5194/acp-24-11081-2024, https://doi.org/10.5194/acp-24-11081-2024, 2024
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Changes in vegetation alongside biomass burning impact regional atmospheric composition and air quality. Using satellite remote sensing, we find a clear linear relationship between forest cover and isoprene and a pronounced non-linear relationship between burned area and nitrogen dioxide in the southern Amazon, a region of substantial deforestation. These quantified relationships can be used for model evaluation and further exploration of biosphere-atmosphere interactions in Earth System Models.
Jieying Ding, Ronald van der A, Henk Eskes, Enrico Dammers, Mark Shephard, Roy Wichink Kruit, Marc Guevara, and Leonor Tarrason
Atmos. Chem. Phys., 24, 10583–10599, https://doi.org/10.5194/acp-24-10583-2024, https://doi.org/10.5194/acp-24-10583-2024, 2024
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Here we applied the existing Daily Emissions Constrained by Satellite Observations (DECSO) inversion algorithm to NH3 observations from the CrIS satellite instrument to estimate NH3 emissions. As NH3 in the atmosphere is influenced by NOx, we implemented DECSO to estimate NOx and NH3 emissions simultaneously. The emissions are derived over Europe for 2020 at a spatial resolution of 0.2° using daily observations from CrIS and TROPOMI. Results are compared to bottom-up emission inventories.
Matthew S. Johnson, Sajeev Philip, Scott Meech, Rajesh Kumar, Meytar Sorek-Hamer, Yoichi P. Shiga, and Jia Jung
Atmos. Chem. Phys., 24, 10363–10384, https://doi.org/10.5194/acp-24-10363-2024, https://doi.org/10.5194/acp-24-10363-2024, 2024
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Satellites, like the Ozone Monitoring Instrument (OMI), retrieve proxy species of ozone (O3) formation (formaldehyde and nitrogen dioxide) and the ratios (FNRs) which can define O3 production sensitivity regimes. Here we investigate trends of OMI FNRs from 2005 to 2021, and they have increased in major cities, suggesting a transition from radical- to NOx-limited regimes. OMI also observed the impact of reduced emissions during the 2020 COVID-19 lockdown that resulted in increased FNRs.
Audrey Gaudel, Ilann Bourgeois, Meng Li, Kai-Lan Chang, Jerald Ziemke, Bastien Sauvage, Ryan M. Stauffer, Anne M. Thompson, Debra E. Kollonige, Nadia Smith, Daan Hubert, Arno Keppens, Juan Cuesta, Klaus-Peter Heue, Pepijn Veefkind, Kenneth Aikin, Jeff Peischl, Chelsea R. Thompson, Thomas B. Ryerson, Gregory J. Frost, Brian C. McDonald, and Owen R. Cooper
Atmos. Chem. Phys., 24, 9975–10000, https://doi.org/10.5194/acp-24-9975-2024, https://doi.org/10.5194/acp-24-9975-2024, 2024
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The study examines tropical tropospheric ozone changes. In situ data from 1994–2019 display increased ozone, notably over India, Southeast Asia, and Malaysia and Indonesia. Sparse in situ data limit trend detection for the 15-year period. In situ and satellite data, with limited sampling, struggle to consistently detect trends. Continuous observations are vital over the tropical Pacific Ocean, Indian Ocean, western Africa, and South Asia for accurate ozone trend estimation in these regions.
Naveed Ahmad, Changqing Lin, Alexis K. H. Lau, Jhoon Kim, Tianshu Zhang, Fangqun Yu, Chengcai Li, Ying Li, Jimmy C. H. Fung, and Xiang Qian Lao
Atmos. Chem. Phys., 24, 9645–9665, https://doi.org/10.5194/acp-24-9645-2024, https://doi.org/10.5194/acp-24-9645-2024, 2024
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This study developed a nested machine learning model to convert the GEMS NO2 column measurements into ground-level concentrations across China. The model directly incorporates the NO2 mixing height (NMH) into the methodological framework. The study underscores the importance of considering NMH when estimating ground-level NO2 from satellite column measurements and highlights the significant advantages of new-generation geostationary satellites in air quality monitoring.
Chengxin Zhang, Xinhan Niu, Hongyu Wu, Zhipeng Ding, Ka Lok Chan, Jhoon Kim, Thomas Wagner, and Cheng Liu
EGUsphere, https://doi.org/10.5194/egusphere-2024-2620, https://doi.org/10.5194/egusphere-2024-2620, 2024
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This research utilizes hourly air pollution observations from the world’s first geostationary satellite to develop a spatiotemporal neural network model for full-coverage surface NO2 pollution prediction over the next 24 hours, achieving outstanding forecasting performance and efficacy. These results highlight the profound impact of geostationary satellite observations in advancing air quality forecasting models, thereby contributing to future models for health exposure to air pollution.
Richard J. Pope, Fiona M. O'Connor, Mohit Dalvi, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Brice Barret, Eric Le Flochmoen, Anne Boynard, Martyn P. Chipperfield, Wuhu Feng, Matilda A. Pimlott, Sandip S. Dhomse, Christian Retscher, Catherine Wespes, and Richard Rigby
Atmos. Chem. Phys., 24, 9177–9195, https://doi.org/10.5194/acp-24-9177-2024, https://doi.org/10.5194/acp-24-9177-2024, 2024
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Ozone is a potent air pollutant in the lower troposphere, with adverse impacts on human health. Satellite records of tropospheric ozone currently show large-scale inconsistencies in long-term trends. Our detailed study of the potential factors (e.g. satellite errors, where the satellite can observe ozone) potentially driving these inconsistencies found that, in North America, Europe, and East Asia, the underlying trends are typically small with large uncertainties.
David P. Edwards, Sara Martínez-Alonso, Duseong S. Jo, Ivan Ortega, Louisa K. Emmons, John J. Orlando, Helen M. Worden, Jhoon Kim, Hanlim Lee, Junsung Park, and Hyunkee Hong
Atmos. Chem. Phys., 24, 8943–8961, https://doi.org/10.5194/acp-24-8943-2024, https://doi.org/10.5194/acp-24-8943-2024, 2024
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Until recently, satellite observations of atmospheric pollutants at any location could only be obtained once a day. New geostationary satellites stare at a region of the Earth to make hourly measurements, and the Geostationary Environment Monitoring Spectrometer is the first looking at Asia. These data and model simulations show how the change seen for one important pollutant that determines air quality depends on a combination of pollution emissions, atmospheric chemistry, and meteorology.
Vitali Fioletov, Chris A. McLinden, Debora Griffin, Xiaoyi Zhao, and Henk Eskes
EGUsphere, https://doi.org/10.5194/egusphere-2024-1991, https://doi.org/10.5194/egusphere-2024-1991, 2024
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Satellite data were used to estimate urban per capita emissions for 261 major cities worldwide. Three components in tropospheric NO2 data: background NO2, NO2 from urban sources, and from industrial point sources were isolated and then each of these components was analyzed separately. The largest per capita emissions were found at the Middle East and the smallest were in India and South Africa. Urban weekend emissions are 20 %–50 % less than workday emissions for all regions except China.
Elise Penn, Daniel J. Jacob, Zichong Chen, James D. East, Melissa P. Sulprizio, Lori Bruhwiler, Joannes D. Maasakkers, Hannah Nesser, Zhen Qu, Yuzhong Zhang, and John Worden
EGUsphere, https://doi.org/10.5194/egusphere-2024-2260, https://doi.org/10.5194/egusphere-2024-2260, 2024
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The hydroxyl radical (OH), destroys many air pollutants, including methane. Global mean OH cannot be directly measured, so it is inferred with the methyl chloroform (MCF) proxy. MCF is decreasing, and a replacement is needed. We use satellite observations of methane in two spectral ranges as a proxy for OH instead. We find shortwave infrared observations can characterize yearly OH and its seasonality, but not the latitudinal distribution. Thermal infrared observations add little information.
Amir H. Souri, Gonzalo González Abad, Glenn M. Wolfe, Tijl Verhoelst, Corinne Vigouroux, Gaia Pinardi, Steven Compernolle, Bavo Langerock, Bryan N. Duncan, and Matthew S. Johnson
EGUsphere, https://doi.org/10.5194/egusphere-2024-1947, https://doi.org/10.5194/egusphere-2024-1947, 2024
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We establish a simple yet robust relationship between ozone production rates and several geophysical parameters obtained from several intensive atmospheric composition campaigns. We have shown that satellite remote sensing data can effectively constrain these parameters, enabling us to produce the first global maps of ozone production rates with unprecedented resolution.
Lingxiao Lu, Jason Blake Cohen, Kai Qin, Xiaolu Li, and Qin He
EGUsphere, https://doi.org/10.5194/egusphere-2024-1903, https://doi.org/10.5194/egusphere-2024-1903, 2024
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This study assimilates NO2 observations from TROPOMI in a mass-conserving manner and inverts daily NOx emissions. The results are presented over rapidly changing regions in China. Attribution is quantified using local observations and inverted proxy of combustion temperature. There are significant sources identified in some areas which are not in existing databases, especially small and medium industries along the Yangtze River. We also demonstrate which emissions are robust and which are not.
Sören Johansson, Michael Höpfner, Felix Friedl-Vallon, Norbert Glatthor, Thomas Gulde, Vincent Huijnen, Anne Kleinert, Erik Kretschmer, Guido Maucher, Tom Neubert, Hans Nordmeyer, Christof Piesch, Peter Preusse, Martin Riese, Björn-Martin Sinnhuber, Jörn Ungermann, Gerald Wetzel, and Wolfgang Woiwode
Atmos. Chem. Phys., 24, 8125–8138, https://doi.org/10.5194/acp-24-8125-2024, https://doi.org/10.5194/acp-24-8125-2024, 2024
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We present airborne infrared limb sounding GLORIA measurements of ammonia (NH3) in the upper troposphere of air masses within the Asian monsoon and of those connected with biomass burning. Comparing CAMS (Copernicus Atmosphere Monitoring Service) model data, we find that the model reproduces the measured enhanced NH3 within the Asian monsoon well but not that within biomass burning plumes, where no enhanced NH3 is measured in the upper troposphere but considerable amounts are simulated by CAMS.
Sandro Meier, Erik F. M. Koene, Maarten Krol, Dominik Brunner, Alexander Damm, and Gerrit Kuhlmann
Atmos. Chem. Phys., 24, 7667–7686, https://doi.org/10.5194/acp-24-7667-2024, https://doi.org/10.5194/acp-24-7667-2024, 2024
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Nitrogen oxides (NOx = NO + NO2) are important air pollutants. This study addresses the challenge of accurately estimating NOx emissions from NO2 satellite observations. We develop a realistic model to convert NO2 to NOx by using simulated plumes from various power plants. We apply the model to satellite NO2 observations, significantly reducing biases in estimated NOx emissions. The study highlights the potential for a consistent, high-resolution estimation of NOx emissions using satellite data.
Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Michael Weimer, Heinrich Bovensmann, John P. Burrows, and Hartmut Bösch
Atmos. Chem. Phys., 24, 7609–7621, https://doi.org/10.5194/acp-24-7609-2024, https://doi.org/10.5194/acp-24-7609-2024, 2024
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Large quantities of CO and CO2 are emitted during conventional steel production. As satellite-based estimates of CO2 emissions at the facility level are challenging, co-emitted CO can indicate the carbon footprint of steel plants. We estimate CO emissions for German steelworks and use CO2 emissions from emissions trading data to derive a sector-specific CO/CO2 emission ratio for the steel industry; it is a prerequisite to use CO as a proxy for CO2 emissions from similar steel production sites.
Ronald J. van der A, Jieying Ding, and Henk Eskes
Atmos. Chem. Phys., 24, 7523–7534, https://doi.org/10.5194/acp-24-7523-2024, https://doi.org/10.5194/acp-24-7523-2024, 2024
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Using observations of the Sentinel-5P satellite and the latest version of the inversion algorithm DECSO, anthropogenic NOx emissions are derived for Europe for the years 2019–2022 with a spatial resolution of 0.2°. The results are compared with European emissions of the Copernicus Atmosphere Monitoring Service.
Norbert Glatthor, Gabriele P. Stiller, Thomas von Clarmann, Bernd Funke, Sylvia Kellmann, and Andrea Linden
EGUsphere, https://doi.org/10.5194/egusphere-2024-1793, https://doi.org/10.5194/egusphere-2024-1793, 2024
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We present global upper tropospheric distributions of the pollutants HCN, CO, C2H2, C2H6, PAN and HCOOH, observed by MIPAS/Envisat between 2002 and 2012. This common view allows conclusions on the sources of the different pollutants, like, e.g., biomass burning, anthropogenic sources or biogenic release. For this purpose we compare their VMR distributions and additionally perform global correlation and regression analyses.
Gijs Leguijt, Joannes D. Maasakkers, Hugo A. C. Denier van der Gon, Arjo J. Segers, Tobias Borsdorff, Ivar R. van der Velde, and Ilse Aben
EGUsphere, https://doi.org/10.5194/egusphere-2024-1561, https://doi.org/10.5194/egusphere-2024-1561, 2024
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The production of steel coincides with large emissions of greenhouse gases and air pollutants including carbon monoxide. European facilities are required to report their emissions, which are estimated using a variety of methods. We evaluate these estimates using carbon monoxide concentrations measured using a satellite. We find generally good agreement between our values and those reported but also identify some uncertainties, showing that satellites can provide insights on these emissions.
Zhuang Wang, Chune Shi, Hao Zhang, Xianguang Ji, Yizhi Zhu, Congzi Xia, Xiaoyun Sun, Xinfeng Lin, Shaowei Yan, Suyao Wang, Yuan Zhou, Chengzhi Xing, Yujia Chen, and Cheng Liu
EGUsphere, https://doi.org/10.5194/egusphere-2024-341, https://doi.org/10.5194/egusphere-2024-341, 2024
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This study attempts to explain the surface ozone background, typical, and peak trends in eastern China by combining a large amount of ground–based and satellite observations, and found substantial reductions in nitrogen oxides emissions have diametrically opposed effects on peak (decreasing) and low (increasing) ozone concentrations.
Bruno Franco, Lieven Clarisse, Nicolas Theys, Juliette Hadji-Lazaro, Cathy Clerbaux, and Pierre Coheur
Atmos. Chem. Phys., 24, 4973–5007, https://doi.org/10.5194/acp-24-4973-2024, https://doi.org/10.5194/acp-24-4973-2024, 2024
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Using IASI global infrared measurements, we retrieve nitrous acid (HONO) in fire plumes from space. We detect large enhancements of pyrogenic HONO worldwide, especially from intense wildfires at Northern Hemisphere mid- and high latitudes. Predominance of IASI nighttime over daytime measurements sheds light on HONO's extended lifetime and secondary formation during long-range transport in smoke plumes. Our findings deepen the understanding of atmospheric HONO, crucial for air quality assessment.
Gitaek T. Lee, Rokjin J. Park, Hyeong-Ahn Kwon, Eunjo S. Ha, Sieun D. Lee, Seunga Shin, Myoung-Hwan Ahn, Mina Kang, Yong-Sang Choi, Gyuyeon Kim, Dong-Won Lee, Deok-Rae Kim, Hyunkee Hong, Bavo Langerock, Corinne Vigouroux, Christophe Lerot, Francois Hendrick, Gaia Pinardi, Isabelle De Smedt, Michel Van Roozendael, Pucai Wang, Heesung Chong, Yeseul Cho, and Jhoon Kim
Atmos. Chem. Phys., 24, 4733–4749, https://doi.org/10.5194/acp-24-4733-2024, https://doi.org/10.5194/acp-24-4733-2024, 2024
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This study evaluates the Geostationary Environment Monitoring Spectrometer (GEMS) HCHO product by comparing its vertical column densities (VCDs) with those of TROPOMI and ground-based observations. Based on some sensitivity tests, obtaining radiance references under clear-sky conditions significantly improves HCHO retrieval quality. GEMS HCHO VCDs captured seasonal and diurnal variations well during the first year of observation, showing consistency with TROPOMI and ground-based observations.
Fei Liu, Steffen Beirle, Joanna Joiner, Sungyeon Choi, Zhining Tao, K. Emma Knowland, Steven J. Smith, Daniel Q. Tong, Siqi Ma, Zachary T. Fasnacht, and Thomas Wagner
Atmos. Chem. Phys., 24, 3717–3728, https://doi.org/10.5194/acp-24-3717-2024, https://doi.org/10.5194/acp-24-3717-2024, 2024
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Using satellite data, we developed a coupled method independent of the chemical transport model to map NOx emissions across US cities. After validating our technique with synthetic data, we charted NOx emissions from 2018–2021 in 39 cities. Our results closely matched EPA estimates but also highlighted some inconsistencies in both magnitude and spatial distribution. This research can help refine strategies for monitoring and managing air quality.
Richard J. Pope, Alexandru Rap, Matilda A. Pimlott, Brice Barret, Eric Le Flochmoen, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Anne Boynard, Christian Retscher, Wuhu Feng, Richard Rigby, Sandip S. Dhomse, Catherine Wespes, and Martyn P. Chipperfield
Atmos. Chem. Phys., 24, 3613–3626, https://doi.org/10.5194/acp-24-3613-2024, https://doi.org/10.5194/acp-24-3613-2024, 2024
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Tropospheric ozone is an important short-lived climate forcer which influences the incoming solar short-wave radiation and the outgoing long-wave radiation in the atmosphere (8–15 km) where the balance between the two yields a net positive (i.e. warming) effect at the surface. Overall, we find that the tropospheric ozone radiative effect ranges between 1.21 and 1.26 W m−2 with a negligible trend (2008–2017), suggesting that tropospheric ozone influences on climate have remained stable with time.
Lucien Froidevaux, Douglas E. Kinnison, Benjamin Gaubert, Michael J. Schwartz, Nathaniel J. Livesey, William G. Read, Charles G. Bardeen, Jerry R. Ziemke, and Ryan A. Fuller
EGUsphere, https://doi.org/10.5194/egusphere-2024-525, https://doi.org/10.5194/egusphere-2024-525, 2024
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We compare observed changes in ozone (O3) and carbon monoxide (CO) in the tropical upper troposphere (10–15 km altitude) for 2005–2020 to predictions from model simulations that track the evolution of natural and industrial emissions transported to this region. An increasing trend in measured upper tropospheric O3 is generally well matched by the model trends. We also find that changes in modeled industrial CO surface emissions lead to better model agreement with observed decreasing CO trends.
Isabelle A. Taylor, Roy G. Grainger, Andrew T. Prata, Simon R. Proud, Tamsin A. Mather, and David M. Pyle
Atmos. Chem. Phys., 23, 15209–15234, https://doi.org/10.5194/acp-23-15209-2023, https://doi.org/10.5194/acp-23-15209-2023, 2023
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This study looks at sulfur dioxide (SO2) and ash emissions from the April 2021 eruption of La Soufrière on St Vincent. Using satellite data, 35 eruptive events were identified. Satellite data were used to track SO2 as it was transported around the globe. The majority of SO2 was emitted into the upper troposphere and lower stratosphere. Similarities with the 1979 eruption of La Soufrière highlight the value of studying these eruptions to be better prepared for future eruptions.
Richard J. Pope, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Martyn P. Chipperfield, Wuhu Feng, Matilda A. Pimlott, Sandip S. Dhomse, Christian Retscher, and Richard Rigby
Atmos. Chem. Phys., 23, 14933–14947, https://doi.org/10.5194/acp-23-14933-2023, https://doi.org/10.5194/acp-23-14933-2023, 2023
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Ozone is a potent air pollutant, and we present the first study to investigate long-term changes in lower tropospheric column ozone (LTCO3) from space. We have constructed a merged LTCO3 dataset from GOME-1, SCIAMACHY and OMI between 1996 and 2017. Comparing LTCO3 between the 1996–2000 and 2013–2017 5-year averages, we find significant positive increases in the tropics/sub-tropics, while in the northern mid-latitudes, we find small-scale differences.
Daniel H. Cusworth, Andrew K. Thorpe, Charles E. Miller, Alana K. Ayasse, Ralph Jiorle, Riley M. Duren, Ray Nassar, Jon-Paul Mastrogiacomo, and Robert R. Nelson
Atmos. Chem. Phys., 23, 14577–14591, https://doi.org/10.5194/acp-23-14577-2023, https://doi.org/10.5194/acp-23-14577-2023, 2023
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Carbon dioxide (CO2) emissions from combustion sources are uncertain in many places across the globe. Satellites have the ability to detect and quantify emissions from large CO2 point sources, including coal-fired power plants. In this study, we tasked two satellites to routinely observe CO2 emissions at 30 coal-fired power plants between 2021 and 2022. These results present the largest dataset of space-based CO2 emission estimates to date.
Maria Tsivlidou, Bastien Sauvage, Yasmine Bennouna, Romain Blot, Damien Boulanger, Hannah Clark, Eric Le Flochmoën, Philippe Nédélec, Valérie Thouret, Pawel Wolff, and Brice Barret
Atmos. Chem. Phys., 23, 14039–14063, https://doi.org/10.5194/acp-23-14039-2023, https://doi.org/10.5194/acp-23-14039-2023, 2023
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The tropics are a region where the ozone increase has been most apparent since 1980 and where observations are sparse. Using aircraft, satellite, and model data, we document the characteristics of tropospheric ozone and CO over the whole tropics for the last 2 decades. We explore the origin of the observed CO anomalies and investigate transport processes driving the tropical CO and O3 distribution. Our study highlights the importance of anthropogenic emissions, mostly over the northern tropics.
Richard J. Pope, Brian J. Kerridge, Martyn P. Chipperfield, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Matilda A. Pimlott, Wuhu Feng, Edward Comyn-Platt, Garry D. Hayman, Stephen R. Arnold, and Ailish M. Graham
Atmos. Chem. Phys., 23, 13235–13253, https://doi.org/10.5194/acp-23-13235-2023, https://doi.org/10.5194/acp-23-13235-2023, 2023
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In the summer of 2018, Europe experienced several persistent large-scale ozone (O3) pollution episodes. Satellite tropospheric O3 and surface O3 data recorded substantial enhancements in 2018 relative to other years. Targeted model simulations showed that meteorological processes and emissions controlled the elevated surface O3, while mid-tropospheric O3 enhancements were dominated by stratospheric O3 intrusion and advection of North Atlantic O3-rich air masses into Europe.
Rui Wang, Da Pan, Xuehui Guo, Kang Sun, Lieven Clarisse, Martin Van Damme, Pierre-François Coheur, Cathy Clerbaux, Melissa Puchalski, and Mark A. Zondlo
Atmos. Chem. Phys., 23, 13217–13234, https://doi.org/10.5194/acp-23-13217-2023, https://doi.org/10.5194/acp-23-13217-2023, 2023
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Ammonia (NH3) is a key precursor for fine particulate matter (PM2.5) and a primary form of reactive nitrogen, yet it has sparse ground measurements. We perform the first comprehensive comparison between ground observations and satellite retrievals in the US, demonstrating that satellite NH3 data can help fill spatial gaps in the current ground monitoring networks. Trend analyses using both datasets highlight increasing NH3 trends across the US, including the NH3 hotspots and urban areas.
Rimal Abeed, Camille Viatte, William C. Porter, Nikolaos Evangeliou, Cathy Clerbaux, Lieven Clarisse, Martin Van Damme, Pierre-François Coheur, and Sarah Safieddine
Atmos. Chem. Phys., 23, 12505–12523, https://doi.org/10.5194/acp-23-12505-2023, https://doi.org/10.5194/acp-23-12505-2023, 2023
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Ammonia emissions from agricultural activities will inevitably increase with the rise in population. We use a variety of datasets (satellite, reanalysis, and model simulation) to calculate the first regional map of ammonia emission potential during the start of the growing season in Europe. We then apply our developed method using a climate model to show the effect of the temperature increase on future ammonia columns under two possible climate scenarios.
Bianca Zilker, Andreas Richter, Anne-Marlene Blechschmidt, Peter von der Gathen, Ilias Bougoudis, Sora Seo, Tim Bösch, and John Philip Burrows
Atmos. Chem. Phys., 23, 9787–9814, https://doi.org/10.5194/acp-23-9787-2023, https://doi.org/10.5194/acp-23-9787-2023, 2023
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During Arctic spring, near-surface ozone is depleted by bromine released from salty sea ice and/or snow-covered areas under certain meteorological conditions. To study this ozone depletion and the prevailing meteorological conditions, two ozone data sets from Ny-Ålesund, Svalbard, have been evaluated. We found that during ozone depletion events lower pressure over the Barents Sea and higher pressure in the Icelandic Low area led to a transport of cold polar air from the north to Ny-Ålesund.
Gijs Leguijt, Joannes D. Maasakkers, Hugo A. C. Denier van der Gon, Arjo J. Segers, Tobias Borsdorff, and Ilse Aben
Atmos. Chem. Phys., 23, 8899–8919, https://doi.org/10.5194/acp-23-8899-2023, https://doi.org/10.5194/acp-23-8899-2023, 2023
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We present a fast method to evaluate carbon monoxide emissions from cities in Africa. Carbon monoxide is important for climate change in an indirect way, as it is linked to ozone, methane, and carbon dioxide. Our measurements are made with a satellite that sees the entire globe every single day. This means that we can check from space whether the current knowledge of emission rates is up to date. We make the comparison and show that the emission rates in northern Africa are underestimated.
Chantelle R. Lonsdale and Kang Sun
Atmos. Chem. Phys., 23, 8727–8748, https://doi.org/10.5194/acp-23-8727-2023, https://doi.org/10.5194/acp-23-8727-2023, 2023
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The COVID-19 pandemic, which was caused by the SARS-CoV-2 virus, emerged in 2019, and its still evolving variants have resulted in unprecedented shifts in human activities and anthropogenic emissions into the Earth's atmosphere. We present monthly nitrogen oxide emissions over three major continents from May 2018 to January 2023 to capture variations before and after the COVID-19 pandemic. We focus on a diverse collection of 54 cities to quantify the post-COVID-19 perturbations.
Xiaolu Li, Jason Blake Cohen, Kai Qin, Hong Geng, Xiaohui Wu, Liling Wu, Chengli Yang, Rui Zhang, and Liqin Zhang
Atmos. Chem. Phys., 23, 8001–8019, https://doi.org/10.5194/acp-23-8001-2023, https://doi.org/10.5194/acp-23-8001-2023, 2023
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Remotely sensed NO2 and surface NOx are combined with a mathematical method to estimate daily NOx emissions. The results identify new sources and improve existing estimates. The estimation is driven by three flexible factors: thermodynamics of combustion, chemical loss, and atmospheric transport. The thermodynamic term separates power, iron, and cement from coking, boilers, and aluminum. This work finds three causes for the extremes: emissions, UV radiation, and transport.
Juanito Jerrold Mariano Acdan, Robert Bradley Pierce, Angela F. Dickens, Zachariah Adelman, and Tsengel Nergui
Atmos. Chem. Phys., 23, 7867–7885, https://doi.org/10.5194/acp-23-7867-2023, https://doi.org/10.5194/acp-23-7867-2023, 2023
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Ozone is an air pollutant that is harmful to human health. Near the surface of Earth, ozone is created when other pollutants react in the presence of sunlight. This study uses satellite data to investigate how ozone levels can be decreased in the Lake Michigan region of the United States. Our results indicate that ozone levels can be decreased by decreasing volatile organic compound emissions in urban areas and decreasing nitrogen oxide emissions in the region as a whole.
Sachiko Okamoto, Juan Cuesta, Matthias Beekmann, Gaëlle Dufour, Maxim Eremenko, Kazuyuki Miyazaki, Cathy Boonne, Hiroshi Tanimoto, and Hajime Akimoto
Atmos. Chem. Phys., 23, 7399–7423, https://doi.org/10.5194/acp-23-7399-2023, https://doi.org/10.5194/acp-23-7399-2023, 2023
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We present a detailed analysis of the daily evolution of the lowermost tropospheric ozone documented by IASI+GOME2 multispectral satellite observations and that of its precursors from TCR-2 tropospheric chemistry reanalysis. It reveals that the ozone outbreak across Europe in July 2017 was produced during favorable condition for photochemical production of ozone and was associated with multiple sources of ozone precursors: biogenic, anthropogenic, and biomass burning emissions.
Xiaojuan Lin, Ronald van der A, Jos de Laat, Henk Eskes, Frédéric Chevallier, Philippe Ciais, Zhu Deng, Yuanhao Geng, Xuanren Song, Xiliang Ni, Da Huo, Xinyu Dou, and Zhu Liu
Atmos. Chem. Phys., 23, 6599–6611, https://doi.org/10.5194/acp-23-6599-2023, https://doi.org/10.5194/acp-23-6599-2023, 2023
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Satellite observations provide evidence for CO2 emission signals from isolated power plants. We use these satellite observations to quantify emissions. We found that for power plants with multiple observations, the correlation of estimated and reported emissions is significantly improved compared to a single observation case. This demonstrates that accurate estimation of power plant emissions can be achieved by monitoring from future satellite missions with more frequent observations.
Daniel C. Anderson, Bryan N. Duncan, Julie M. Nicely, Junhua Liu, Sarah A. Strode, and Melanie B. Follette-Cook
Atmos. Chem. Phys., 23, 6319–6338, https://doi.org/10.5194/acp-23-6319-2023, https://doi.org/10.5194/acp-23-6319-2023, 2023
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We describe a methodology that combines machine learning, satellite observations, and 3D chemical model output to infer the abundance of the hydroxyl radical (OH), a chemical that removes many trace gases from the atmosphere. The methodology successfully captures the variability of observed OH, although further observations are needed to evaluate absolute accuracy. Current satellite observations are of sufficient quality to infer OH, but retrieval validation in the remote tropics is needed.
Xiumei Zhang, Ronald van der A, Jieying Ding, Xin Zhang, and Yan Yin
Atmos. Chem. Phys., 23, 5587–5604, https://doi.org/10.5194/acp-23-5587-2023, https://doi.org/10.5194/acp-23-5587-2023, 2023
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We compiled a ship emission inventory based on automatic identification system (AIS) signals in the Jiangsu section of the Yangtze River. This ship emission inventory was compared with Chinese bottom-up inventories and the satellite-derived emissions from TROPOMI. The result shows a consistent spatial distribution, with riverine cities having high NOx emissions. Inland ship emissions of NOx are shown to contribute at least 40 % to air pollution along the river.
Yifan Guan, Gretchen Keppel-Aleks, Scott C. Doney, Christof Petri, Dave Pollard, Debra Wunch, Frank Hase, Hirofumi Ohyama, Isamu Morino, Justus Notholt, Kei Shiomi, Kim Strong, Rigel Kivi, Matthias Buschmann, Nicholas Deutscher, Paul Wennberg, Ralf Sussmann, Voltaire A. Velazco, and Yao Té
Atmos. Chem. Phys., 23, 5355–5372, https://doi.org/10.5194/acp-23-5355-2023, https://doi.org/10.5194/acp-23-5355-2023, 2023
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We characterize spatial–temporal patterns of interannual variability (IAV) in atmospheric CO2 based on NASA’s Orbiting Carbon Observatory-2 (OCO-2). CO2 variation is strongly impacted by climate events, with higher anomalies during El Nino years. We show high correlation in IAV between space-based and ground-based CO2 from long-term sites. Because OCO-2 has near-global coverage, our paper provides a roadmap to study IAV where in situ observation is sparse, such as open oceans and remote lands.
Yuchen Wang, Xvli Guo, Yajie Huo, Mengying Li, Yuqing Pan, Shaocai Yu, Alexander Baklanov, Daniel Rosenfeld, John H. Seinfeld, and Pengfei Li
Atmos. Chem. Phys., 23, 5233–5249, https://doi.org/10.5194/acp-23-5233-2023, https://doi.org/10.5194/acp-23-5233-2023, 2023
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Substantial advances have been made in recent years toward detecting and quantifying methane super-emitters from space. However, such advances have rarely been expanded to measure the global methane pledge because large-scale swaths and high-resolution sampling have not been coordinated. Here we present a versatile spaceborne architecture that can juggle planet-scale and plant-level methane retrievals, challenge official emission reports, and remain relevant for stereoscopic measurements.
Liang Feng, Paul I. Palmer, Robert J. Parker, Mark F. Lunt, and Hartmut Bösch
Atmos. Chem. Phys., 23, 4863–4880, https://doi.org/10.5194/acp-23-4863-2023, https://doi.org/10.5194/acp-23-4863-2023, 2023
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Our understanding of recent changes in atmospheric methane has defied explanation. Since 2007, the atmospheric growth of methane has accelerated to record-breaking values in 2020 and 2021. We use satellite observations of methane to show that (1) increasing emissions over the tropics are mostly responsible for these recent atmospheric changes, and (2) changes in the OH sink during the 2020 Covid-19 lockdown can explain up to 34% of changes in atmospheric methane for that year.
Isis Frausto-Vicencio, Sajjan Heerah, Aaron G. Meyer, Harrison A. Parker, Manvendra Dubey, and Francesca M. Hopkins
Atmos. Chem. Phys., 23, 4521–4543, https://doi.org/10.5194/acp-23-4521-2023, https://doi.org/10.5194/acp-23-4521-2023, 2023
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Wildfires are increasing in the western USA, making it critical to understand the impacts of greenhouse gases and air pollutants on the atmosphere. We used a ground-based remote sensing technique to measure the greenhouse gases and aerosol in the atmosphere. We isolate a large smoke plume from a nearby wildfire and calculate variables to understand the fuel properties and combustion phases. We find that a significant amount of methane is emitted from the 2020 California wildfire season.
Hervé Petetin, Marc Guevara, Steven Compernolle, Dene Bowdalo, Pierre-Antoine Bretonnière, Santiago Enciso, Oriol Jorba, Franco Lopez, Albert Soret, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 23, 3905–3935, https://doi.org/10.5194/acp-23-3905-2023, https://doi.org/10.5194/acp-23-3905-2023, 2023
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This study analyses the potential of the TROPOMI space sensor for monitoring the variability of NO2 pollution over the Iberian Peninsula. A reduction of NO2 levels is observed during the weekend and in summer, especially over most urbanized areas, in agreement with surface observations. An enhancement of NO2 is found during summer with TROPOMI over croplands, potentially related to natural soil NO emissions, which illustrates the outstanding value of TROPOMI for complementing surface networks.
Siyang Cheng, Xinghong Cheng, Jianzhong Ma, Xiangde Xu, Wenqian Zhang, Jinguang Lv, Gang Bai, Bing Chen, Siying Ma, Steffen Ziegler, Sebastian Donner, and Thomas Wagner
Atmos. Chem. Phys., 23, 3655–3677, https://doi.org/10.5194/acp-23-3655-2023, https://doi.org/10.5194/acp-23-3655-2023, 2023
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We made mobile MAX-DOAS measurements in the background atmosphere over the Tibetan Plateau in summer 2021. We retrieved the tropospheric NO2 and HCHO vertical column densities (VCDs) along extended driving routes and found a decreasing trend of the VCDs with altitude. Elevated NO2 VCDs along the driving routes could be attributed to enhanced traffic emissions from the towns crossed. The spatio-temporal distribution of the HCHO VCDs correlated strongly with the surface temperature.
Cameron G. MacDonald, Jon-Paul Mastrogiacomo, Joshua L. Laughner, Jacob K. Hedelius, Ray Nassar, and Debra Wunch
Atmos. Chem. Phys., 23, 3493–3516, https://doi.org/10.5194/acp-23-3493-2023, https://doi.org/10.5194/acp-23-3493-2023, 2023
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We use three satellites measuring carbon dioxide (CO2), carbon monoxide (CO) and nitrogen dioxide (NO2) to calculate atmospheric enhancements of these gases from 27 urban areas. We calculate enhancement ratios between the species and compare those to ratios derived from four globally gridded anthropogenic emission inventories. We find that the global inventories generally underestimate CO emissions in many North American and European cities relative to our observed enhancement ratios.
Udo Frieß, Karin Kreher, Richard Querel, Holger Schmithüsen, Dan Smale, Rolf Weller, and Ulrich Platt
Atmos. Chem. Phys., 23, 3207–3232, https://doi.org/10.5194/acp-23-3207-2023, https://doi.org/10.5194/acp-23-3207-2023, 2023
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Reactive bromine compounds, emitted by the sea ice during polar spring, play an important role in the atmospheric chemistry of the coastal regions of Antarctica. We investigate the sources and impacts of reactive bromine in detail using many years of measurements at two Antarctic sites located at opposite sides of the Antarctic continent. Using a multitude of meteorological observations, we were able to identify the main triggers and source regions for reactive bromine in Antarctica.
Cited articles
Beirle, S., Platt, U., Wenig, M., and Wagner, T.: Weekly cycle of NO2 by GOME measurements: a signature of anthropogenic sources, Atmos. Chem. Phys., 3, 2225–2232, https://doi.org/10.5194/acp-3-2225-2003, 2003.
Boersma, K. F., Eskes, H. J., Veefkind, J. P., Brinksma, E. J., van der A, R. J., Sneep, M., van den Oord, G. H. J., Levelt, P. F., Stammes, P., Gleason, J. F., and Bucsela, E. J.: Near-real time retrieval of tropospheric NO2 from OMI, Atmos. Chem. Phys., 7, 2103–2118, https://doi.org/10.5194/acp-7-2103-2007, 2007.
Boersma, K. F., Jacob, D. J., Trainic, M., Rudich, Y., DeSmedt, I., Dirksen, R., and Eskes, H. J.: Validation of urban NO2 concentrations and their diurnal and seasonal variations observed from the SCIAMACHY and OMI sensors using in situ surface measurements in Israeli cities, Atmos. Chem. Phys., 9, 3867–3879, https://doi.org/10.5194/acp-9-3867-2009, 2009.
Boersma, K. F., Eskes, H. J., Dirksen, R. J., van der A, R. J., Veefkind, J. P., Stammes, P., Huijnen, V., Kleipool, Q. L., Sneep, M., Claas, J., Leitão, J., Richter, A., Zhou, Y., and Brunner, D.: An improved tropospheric NO2 column retrieval algorithm for the Ozone Monitoring Instrument, Atmos. Meas. Tech., 4, 19050–1928, https://doi.org/10.5194/amt-4-1905-2011, 2011.
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