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Volume 15, issue 12
Atmos. Chem. Phys., 15, 6707–6720, 2015
https://doi.org/10.5194/acp-15-6707-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 15, 6707–6720, 2015
https://doi.org/10.5194/acp-15-6707-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 17 Jun 2015

Research article | 17 Jun 2015

Vertical variation of optical properties of mixed Asian dust/pollution plumes according to pathway of air mass transport over East Asia

S.-K. Shin1,*, D. Müller2,**, C. Lee3, K. H. Lee4, D. Shin5, Y. J. Kim1, and Y. M. Noh6 S.-K. Shin et al.
  • 1School of Environmental Science and Engineering, Gwangju Institute of Science & Technology, Gwangju, Republic of Korea
  • 2School of Physics, Astronomy and Mathematics, University of Hertfordshire, Hertfordshire, UK
  • 3Korea Meteorological Administration, Seoul, Republic of Korea
  • 4Department of Atmospheric and Environmental Sciences, Gangneung-Wonju National University, Gangneung, Republic of Korea
  • 5Air Quality Forecasting Centre, Climate and Air Quality Research Department, National Institute of Environmental Research, Incheon, Republic of Korea
  • 6International Environmental Research Centre (IERC), Gwangju Institute of Science & Technology, Gwangju, Republic of Korea
  • *now at: Department of Atmospheric and Environmental Sciences, Gangneung-Wonju National University, Gangneung, Republic of Korea
  • **formerly at: School of Environmental Science and Engineering, Gwangju Institute of Science & Technology, Gwangju, Republic of Korea

Abstract. We use five years (2009–2013) of multiwavelength Raman lidar measurements at Gwangju, South Korea (35.10° N, 126.53° E) for the identification of changes of optical properties of East Asian dust depending on its transport path over China. Profiles of backscatter and extinction coefficients, lidar ratios, and backscatter-related Ångström exponents (wavelength pair 355/532 nm) were measured at Gwangju. Linear particle depolarization ratios were used to identify East Asian dust layers. We used backward trajectory modeling to identify the pathway and the vertical position of dust-laden air masses over China during long-range transport. Most cases of Asian dust events can be described by the emission of dust in desert areas and subsequent transport over highly polluted regions of China. The Asian dust plumes could be categorized into two classes according to the height above ground at which these plumes were transported: (case I) the dust layers passed over China at high altitude levels (> 3 km) until arrival over Gwangju, and (case II) the Asian dust layers were transported near the surface and within the lower troposphere (< 3 km) over industrialized areas before they arrived over Gwangju. We find that the optical characteristics of these mixed Asian dust layers over Gwangju differ depending on their vertical position above ground over China and the change of height above ground during transport. The mean linear particle depolarization ratio was 0.21 ± 0.06 (at 532 nm), the mean lidar ratios were 52 ± 7 sr at 355 nm and 53 ± 8 sr at 532 nm, and the mean Ångström exponent was 0.74 ± 0.31 for case I. In contrast, plumes transported at lower altitudes (case II) showed low depolarization ratios (0.13 ± 0.04 at 532 nm), and higher lidar ratio (63 ± 9 sr at 355 nm and 62 ± 8 sr at 532 nm) and Ångström exponents (0.98 ± 0.51). These numbers show that the optical characteristics of mixed Asian plumes are more similar to optical characteristics of urban pollution. We find a decrease of the linear depolarization ratio of the mixed dust/pollution plume depending on transport time if the pollution layer traveled over China at low heights, i.e., below approximately 3 km above ground. In contrast, we do not find such a trend if the dust plumes traveled at heights above 3 km over China. We need a longer time series of lidar measurements in order to determine in a quantitative way the change of optical properties of dust with transport time.

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The measurements from 2009 to 2013 using a multiwavelength Raman lidar were conducted to identify the changes in optical properties of East Asian dust. We found that the optical properties of Asian dust change depending on the dust plume's vertical position and the change of vertical position during transport over China. We believe this paper provides a better understanding of the optical properties of mixed Asian dust plums and the effect of long-range transport on dust properties.
The measurements from 2009 to 2013 using a multiwavelength Raman lidar were conducted to...
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