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Volume 17, issue 13
Atmos. Chem. Phys., 17, 8453–8471, 2017
https://doi.org/10.5194/acp-17-8453-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 17, 8453–8471, 2017
https://doi.org/10.5194/acp-17-8453-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 11 Jul 2017

Research article | 11 Jul 2017

Diffusivity measurements of volatile organics in levitated viscous aerosol particles

Sandra Bastelberger et al.

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Bateman, A. P., Bertram, A. K., and Martin, S. T.: Hygroscopic Influence on the Semisolid-to-Liquid Transition of Secondary Organic Materials, J. Phys. Chem. A, 119, 4386–4395, https://doi.org/10.1021/jp508521c, 2015.
Bateman, A. P., Gong, Z., Liu, P., Sato, B., Cirino, G., Zhang, Y., Artaxo, P., Bertram, A. K., Manzi, A. O., Rizzo, L. V., Souza, R. A. F., Zaveri, R. A., and Martin, S. T.: Sub-micrometre particulate matter is primarily in liquid form over Amazon rainforest, Nat. Geosci., 9, 34–37, https://doi.org/10.1038/NGEO2599, 2016.
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We present quantitative condensed-phase diffusivity measurements of a volatile organic (tetraethylene glycol) in highly viscous single aerosol particles (aqueous sucrose). The condensed-phase diffusivity exhibits a strong temperature and humidity dependence. Our results suggest that diffusion limitations of volatile organics in highly viscous organic aerosol may severely impact gas–particle partitioning under cold and dry conditions.
We present quantitative condensed-phase diffusivity measurements of a volatile organic...
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