Articles | Volume 17, issue 4
https://doi.org/10.5194/acp-17-2509-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Special issue:
https://doi.org/10.5194/acp-17-2509-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Aerosol vertical distribution and optical properties over China from long-term satellite and ground-based remote sensing
Pengfei Tian
Key Laboratory for Semi-Arid Climate Change of the Ministry of
Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou
730000, China
Department of Atmospheric Sciences, Texas A&M University, College
Station, Texas 77843, USA
Xianjie Cao
Key Laboratory for Semi-Arid Climate Change of the Ministry of
Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou
730000, China
Lei Zhang
CORRESPONDING AUTHOR
Key Laboratory for Semi-Arid Climate Change of the Ministry of
Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou
730000, China
Naixiu Sun
Key Laboratory for Semi-Arid Climate Change of the Ministry of
Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou
730000, China
Lu Sun
Department of Atmospheric Sciences, Texas A&M University, College
Station, Texas 77843, USA
Timothy Logan
Department of Atmospheric Sciences, Texas A&M University, College
Station, Texas 77843, USA
Jinsen Shi
Key Laboratory for Semi-Arid Climate Change of the Ministry of
Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou
730000, China
Yuan Wang
Division of Geological and Planetary Sciences, California Institute of Technology, Pasadena, CA 91106, USA
Yuemeng Ji
Department of Atmospheric Sciences, Texas A&M University, College
Station, Texas 77843, USA
Institute of Environmental Health and Pollution Control, School of
Environmental Science and Engineering, Guangdong University of Technology,
Guangzhou 510006, China
Department of Atmospheric Sciences, Texas A&M University, College
Station, Texas 77843, USA
Zhongwei Huang
Key Laboratory for Semi-Arid Climate Change of the Ministry of
Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou
730000, China
Tian Zhou
Key Laboratory for Semi-Arid Climate Change of the Ministry of
Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou
730000, China
Yingying Shi
Key Laboratory for Semi-Arid Climate Change of the Ministry of
Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou
730000, China
Department of Atmospheric Sciences, Texas A&M University, College
Station, Texas 77843, USA
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Hsiang-He Lee, Xue Zheng, Shaoyue Qiu, and Yuan Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-3199, https://doi.org/10.5194/egusphere-2024-3199, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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The study investigates how aerosol-cloud interactions affect warm boundary layer stratiform clouds over the Eastern North Atlantic. High-resolution WRF-Chem simulations reveal that non-rain clouds at the edges of cloud systems are prone to evaporation, leading to an aerosol drying effect and a transition of aerosols back to accumulation mode for future activation. The study emphasizes that this dynamic behavior is often not adequately represented in most previous prescribed-aerosol simulations.
Xiaojian Zheng, Xiquan Dong, Baike Xi, Timothy Logan, and Yuan Wang
Atmos. Chem. Phys., 24, 10323–10347, https://doi.org/10.5194/acp-24-10323-2024, https://doi.org/10.5194/acp-24-10323-2024, 2024
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The marine boundary layer aerosol–cloud interactions (ACIs) are examined using in situ measurements from two aircraft campaigns over the eastern North Atlantic (ACE-ENA) and Southern Ocean (SOCRATES). The SOCRATES clouds have more and smaller cloud droplets. The ACE-ENA clouds exhibit stronger drizzle formation and growth. Results found distinctive aerosol–cloud interactions for two campaigns. The drizzle processes significantly alter sub-cloud aerosol budgets and impact the ACI assessments.
Weina Zhang, Jianhua Mai, Zhichao Fan, Yongpeng Ji, Yuemeng Ji, Guiying Li, Yanpeng Gao, and Taicheng An
Atmos. Chem. Phys., 24, 9019–9030, https://doi.org/10.5194/acp-24-9019-2024, https://doi.org/10.5194/acp-24-9019-2024, 2024
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This study reveals heterogeneous oxidation causes further radiative forcing effect (RFE) enhancement of amine–mineral mixed particles. Note that RFE increment is higher under clean conditions than that under polluted conditions, which is contributed to high-oxygen-content products. The enhanced RFE of amine–mineral particles caused by heterogenous oxidation is expected to alleviate warming effects.
Jianzhong Xu, Xinghua Zhang, Wenhui Zhao, Lixiang Zhai, Miao Zhong, Jinsen Shi, Junying Sun, Yanmei Liu, Conghui Xie, Yulong Tan, Kemei Li, Xinlei Ge, Qi Zhang, and Shichang Kang
Earth Syst. Sci. Data, 16, 1875–1900, https://doi.org/10.5194/essd-16-1875-2024, https://doi.org/10.5194/essd-16-1875-2024, 2024
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A comprehensive aerosol observation project was carried out in the Tibetan Plateau (TP) and its surroundings in recent years to investigate the properties and sources of atmospheric aerosols as well as their regional differences by performing multiple intensive field observations. The release of this dataset can provide basic and systematic data for related research in the atmospheric, cryospheric, and environmental sciences in this unique region.
Guangyao Dai, Songhua Wu, Wenrui Long, Jiqiao Liu, Yuan Xie, Kangwen Sun, Fanqian Meng, Xiaoquan Song, Zhongwei Huang, and Weibiao Chen
Atmos. Meas. Tech., 17, 1879–1890, https://doi.org/10.5194/amt-17-1879-2024, https://doi.org/10.5194/amt-17-1879-2024, 2024
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An overview is given of the main algorithms applied to derive the aerosol and cloud optical property product of the Aerosol and Carbon Detection Lidar (ACDL), which is capable of globally profiling aerosol and cloud optical properties with high accuracy. The paper demonstrates the observational capabilities of ACDL for aerosol and cloud vertical structure and global distribution through two optical property product measurement cases and global aerosol optical depth profile observations.
Yuemeng Ji, Zhang Shi, Wenjian Li, Jiaxin Wang, Qiuju Shi, Yixin Li, Lei Gao, Ruize Ma, Weijun Lu, Lulu Xu, Yanpeng Gao, Guiying Li, and Taicheng An
Atmos. Chem. Phys., 24, 3079–3091, https://doi.org/10.5194/acp-24-3079-2024, https://doi.org/10.5194/acp-24-3079-2024, 2024
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The formation mechanisms for secondary brown carbon (SBrC) contributed by multifunctional reduced nitrogen compounds (RNCs) remain unclear. Hence, from combined laboratory experiments and quantum chemical calculations, we investigated the heterogeneous reactions of glyoxal (GL) with multifunctional RNCs, which are driven by four-step indirect nucleophilic addition reactions. Our results show a possible missing source for SBrC formation on urban, regional, and global scales.
Qiantao Liu, Zhongwei Huang, Jiqiao Liu, Weibiao Chen, Qingqing Dong, Songhua Wu, Guangyao Dai, Meishi Li, Wuren Li, Ze Li, Xiaodong Song, and Yuan Xie
Atmos. Meas. Tech., 17, 1403–1417, https://doi.org/10.5194/amt-17-1403-2024, https://doi.org/10.5194/amt-17-1403-2024, 2024
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The achieved results revealed that the ACDL observations were in good agreement with the ground-based lidar measurements during dust events. The heights of cloud top and bottom from these two measurements were well matched and comparable. This study proves that the ACDL provides reliable observations of aerosol and cloud in the presence of various climatic conditions, which helps to further evaluate the impacts of aerosol on climate and the environment, as well as on the ecosystem in the future.
Honglin Pan, Jianping Huang, Jiming Li, Zhongwei Huang, Minzhong Wang, Ali Mamtimin, Wen Huo, Fan Yang, Tian Zhou, and Kanike Raghavendra Kumar
Earth Syst. Sci. Data, 16, 1185–1207, https://doi.org/10.5194/essd-16-1185-2024, https://doi.org/10.5194/essd-16-1185-2024, 2024
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We applied several correction procedures and rigorously checked for data quality constraints during the long observation period spanning almost 14 years (2007–2020). Nevertheless, some uncertainties remain, mainly due to technical constraints and limited documentation of the measurements. Even though not completely accurate, this strategy is expected to at least reduce the inaccuracy of the computed characteristic value of aerosol optical parameters.
Elyse A. Pennington, Yuan Wang, Benjamin C. Schulze, Karl M. Seltzer, Jiani Yang, Bin Zhao, Zhe Jiang, Hongru Shi, Melissa Venecek, Daniel Chau, Benjamin N. Murphy, Christopher M. Kenseth, Ryan X. Ward, Havala O. T. Pye, and John H. Seinfeld
Atmos. Chem. Phys., 24, 2345–2363, https://doi.org/10.5194/acp-24-2345-2024, https://doi.org/10.5194/acp-24-2345-2024, 2024
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To assess the air quality in Los Angeles (LA), we improved the CMAQ model by using dynamic traffic emissions and new secondary organic aerosol schemes to represent volatile chemical products. Source apportionment demonstrates that the urban areas of the LA Basin and vicinity are NOx-saturated, with the largest sensitivity of O3 to changes in volatile organic compounds in the urban core. The improvement and remaining issues shed light on the future direction of the model development.
Xiaoli Gong, Liyao Zhu, and Renyi Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2023-3113, https://doi.org/10.5194/egusphere-2023-3113, 2024
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Citric acid participates in and enhances the multi-component nucleation of SA·AM·Wn·CAm, SA·DMA·Wn·CAm, and SA·AM·DMA·Wn·CAm (m=0–1, n = 0–4) clusters using the M06-2X/6-311+G(2d, p) level. Three COOH and one OH groups of CA can act as both hydrogen donors and acceptors, participate in the formation of the hydrogen bonds, lower the nucleation barriers. Addition of a CA molecule to above clusters resulted in negative Gibbs free energies for all reactions.
Da Gao, Bin Zhao, Shuxiao Wang, Yuan Wang, Brian Gaudet, Yun Zhu, Xiaochun Wang, Jiewen Shen, Shengyue Li, Yicong He, Dejia Yin, and Zhaoxin Dong
Atmos. Chem. Phys., 23, 14359–14373, https://doi.org/10.5194/acp-23-14359-2023, https://doi.org/10.5194/acp-23-14359-2023, 2023
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Surface PM2.5 concentrations can be enhanced by aerosol–radiation interactions (ARIs) and aerosol–cloud interactions (ACIs). In this study, we found PM2.5 enhancement induced by ACIs shows a significantly smaller decrease ratio than that induced by ARIs in China with anthropogenic emission reduction from 2013 to 2021, making ACIs more important for enhancing PM2.5 concentrations. ACI-induced PM2.5 enhancement needs to be emphatically considered to meet the national PM2.5 air quality standard.
Yun Lin, Yuan Wang, Jen-Shan Hsieh, Jonathan H. Jiang, Qiong Su, Lijun Zhao, Michael Lavallee, and Renyi Zhang
Atmos. Chem. Phys., 23, 13835–13852, https://doi.org/10.5194/acp-23-13835-2023, https://doi.org/10.5194/acp-23-13835-2023, 2023
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Tropical cyclones (TCs) can cause catastrophic damage to coastal regions. We used a numerical model that explicitly simulates aerosol–cloud interaction and atmosphere–ocean coupling. We show that aerosols and ocean coupling work together to make TC storms bigger but weaker. Moreover, TCs in polluted air have more rainfall and higher sea levels, leading to more severe storm surges and flooding. Our research highlights the roles of aerosols and ocean-coupling feedbacks in TC hazard assessment.
Yuan Wang, Xiaojian Zheng, Xiquan Dong, Baike Xi, and Yuk L. Yung
Atmos. Chem. Phys., 23, 8591–8605, https://doi.org/10.5194/acp-23-8591-2023, https://doi.org/10.5194/acp-23-8591-2023, 2023
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Marine boundary layer clouds remain poorly predicted in global climate models due to multiple entangled uncertainty sources. This study uses the in situ observations from a recent field campaign to constrain and evaluate cloud physics in a simplified version of a climate model. Progress and remaining issues in the cloud physics parameterizations are identified. We systematically evaluate the impacts of large-scale forcing, microphysical scheme, and aerosol concentrations on the cloud property.
Jingyu Wang, Xianfeng Wang, Edward Park, and Yun Lin
Nat. Hazards Earth Syst. Sci. Discuss., https://doi.org/10.5194/nhess-2023-100, https://doi.org/10.5194/nhess-2023-100, 2023
Manuscript not accepted for further review
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Building upon the findings in a preceding study by the authors (Wang et al., 2023), this brief communication successfully applied the soil moisture-based tornado damage track detection method to the 24–25 March 2023 Mississippi outbreak. This study also found that the notable discrepancies between spotter reports and ground survey assessments at the tornado early stage can be reconciled using the new method.
Shikuan Jin, Yingying Ma, Zhongwei Huang, Jianping Huang, Wei Gong, Boming Liu, Weiyan Wang, Ruonan Fan, and Hui Li
Atmos. Chem. Phys., 23, 8187–8210, https://doi.org/10.5194/acp-23-8187-2023, https://doi.org/10.5194/acp-23-8187-2023, 2023
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To better understand the Asian aerosol environment, we studied distributions and trends of aerosol with different sizes and types. Over the past 2 decades, dust, sulfate, and sea salt aerosol decreased by 5.51 %, 3.07 %, and 9.80 %, whereas organic carbon and black carbon aerosol increased by 17.09 % and 6.23 %, respectively. The increase in carbonaceous aerosols was a feature of Asia. An exception is found in East Asia, where the carbonaceous aerosols reduced, owing largely to China's efforts.
Yunshu Zhang, Jiening Liang, Zhida Zhang, Bentao Li, Haotian Zhang, Xianjie Cao, Pengfei Tian, and Lei Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2022-776, https://doi.org/10.5194/egusphere-2022-776, 2022
Preprint archived
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This paper used the WRF-Chem model to simulate different climatic regions of the Tibetan Plateau with finer resolution from 2004 to 2006 and fond that the dust sources are mainly concentrated in the western part of the plateau, while the dust loading of the northern part is the highest. This suggests that dust in the western area can rapidly fall back to the ground after being blown up, while dust in the north can stay in the atmosphere for a long time. That would be useful to future research.
Yixin Li, Jiayun Zhao, Mario Gomez-Hernandez, Michael Lavallee, Natalie M. Johnson, and Renyi Zhang
Atmos. Chem. Phys., 22, 9843–9857, https://doi.org/10.5194/acp-22-9843-2022, https://doi.org/10.5194/acp-22-9843-2022, 2022
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Here we elucidate the production of COOs and their roles in SOA and brown carbon formation from m-xylene oxidation by simultaneously monitoring the evolution of gas-phase products and aerosol properties in an environmental chamber. A kinetic framework is developed to predict SOA production from the concentrations and uptake coefficients for COOs. This functionality-based approach reproduces SOA formation from m-xylene oxidation well and is applicable to VOC oxidation for other species.
Xinghua Zhang, Wenhui Zhao, Lixiang Zhai, Miao Zhong, Jinsen Shi, Junying Sun, Yanmei Liu, Conghui Xie, Yulong Tan, Kemei Li, Xinlei Ge, Qi Zhang, Shichang Kang, and Jianzhong Xu
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2022-211, https://doi.org/10.5194/essd-2022-211, 2022
Manuscript not accepted for further review
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A comprehensive aerosol observation project was carried out in the Tibetan Plateau (TP) in recent years to investigate the properties and sources of atmospheric aerosols as well as their regional differences by performing multiple short-term intensive field observations. The real-time online high-time-resolution (hourly) data of aerosol properties in the different TP region are integrated in a new dataset and can provide supporting for related studies in in the TP.
Huige Di, Yun Yuan, Qing Yan, Wenhui Xin, Shichun Li, Jun Wang, Yufeng Wang, Lei Zhang, and Dengxin Hua
Atmos. Meas. Tech., 15, 3555–3567, https://doi.org/10.5194/amt-15-3555-2022, https://doi.org/10.5194/amt-15-3555-2022, 2022
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It is necessary to correctly evaluate the amount of cloud water resources in an area. Currently, there is a lack of effective observation methods for atmospheric column condensate evaluation. We propose a method for atmospheric column condensate by combining millimetre cloud radar, lidar and microwave radiometers. The method can realise determination of atmospheric column condensate. The variation of cloud before precipitation is considered, and the atmospheric column is deduced and obtained.
Yuemeng Ji, Qiuju Shi, Xiaohui Ma, Lei Gao, Jiaxin Wang, Yixin Li, Yanpeng Gao, Guiying Li, Renyi Zhang, and Taicheng An
Atmos. Chem. Phys., 22, 7259–7271, https://doi.org/10.5194/acp-22-7259-2022, https://doi.org/10.5194/acp-22-7259-2022, 2022
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The formation mechanisms of secondary organic aerosol and brown carbon from small α-carbonyls are still unclear. Thus, the mechanisms and kinetics of aqueous-phase reactions of glyoxal were investigated using quantum chemical and kinetic rate calculations. Several essential isomeric processes were identified, including protonation to yield diol/tetrol and carbenium ions as well as nucleophilic addition of carbenium ions to diol/tetrol and free methylamine/ammonia.
Yun Lin, Jiwen Fan, Pengfei Li, Lai-yung Ruby Leung, Paul J. DeMott, Lexie Goldberger, Jennifer Comstock, Ying Liu, Jong-Hoon Jeong, and Jason Tomlinson
Atmos. Chem. Phys., 22, 6749–6771, https://doi.org/10.5194/acp-22-6749-2022, https://doi.org/10.5194/acp-22-6749-2022, 2022
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How sea spray aerosols may affect cloud and precipitation over the region by acting as ice-nucleating particles (INPs) is unknown. We explored the effects of INPs from marine aerosols on orographic cloud and precipitation for an atmospheric river event observed during the 2015 ACAPEX field campaign. The marine INPs enhance the formation of ice and snow, leading to less shallow warm clouds but more mixed-phase and deep clouds. This work suggests models need to consider the impacts of marine INPs.
Yun Lin, Yuan Wang, Bowen Pan, Jiaxi Hu, Song Guo, Misti Levy Zamora, Pengfei Tian, Qiong Su, Yuemeng Ji, Jiayun Zhao, Mario Gomez-Hernandez, Min Hu, and Renyi Zhang
Atmos. Chem. Phys., 22, 4951–4967, https://doi.org/10.5194/acp-22-4951-2022, https://doi.org/10.5194/acp-22-4951-2022, 2022
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Severe regional haze events, which are characterized by exceedingly high levels of fine particulate matter (PM), occur frequently in many developing countries (such as China and India), with profound implications for human health, weather, and climate. Our work establishes a synthetic view for the dominant regional features during severe haze events, unraveling rapid in situ PM production and inefficient transport, both of which are amplified by atmospheric stagnation.
Xiaojian Zheng, Baike Xi, Xiquan Dong, Peng Wu, Timothy Logan, and Yuan Wang
Atmos. Chem. Phys., 22, 335–354, https://doi.org/10.5194/acp-22-335-2022, https://doi.org/10.5194/acp-22-335-2022, 2022
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This study uses ground-based observations to investigate the physical processes in the aerosol–cloud interactions in non-precipitating marine boundary layer clouds, over the eastern North Atlantic Ocean. Results show that the cloud responses to the aerosols are diminished with limited water vapor supply, while they are enhanced with increasing water vapor availability. The clouds are found to be most sensitive to the aerosols under sufficient water vapor and strong boundary layer turbulence.
Jiarui Wu, Naifang Bei, Yuan Wang, Xia Li, Suixin Liu, Lang Liu, Ruonan Wang, Jiaoyang Yu, Tianhao Le, Min Zuo, Zhenxing Shen, Junji Cao, Xuexi Tie, and Guohui Li
Atmos. Chem. Phys., 21, 2229–2249, https://doi.org/10.5194/acp-21-2229-2021, https://doi.org/10.5194/acp-21-2229-2021, 2021
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A source-oriented version of the WRF-Chem model is developed to conduct source identification of wintertime PM2.5 in the North China Plain. Trans-boundary transport of air pollutants generally dominates the haze pollution in Beijing and Tianjin. The air quality in Hebei, Shandong, and Shanxi is generally controlled by local emissions. Primary aerosol species, such as EC and POA, are generally controlled by local emissions, while secondary aerosol shows evident regional characteristics.
Yuan Wang, Xiaojian Zheng, Xiquan Dong, Baike Xi, Peng Wu, Timothy Logan, and Yuk L. Yung
Atmos. Chem. Phys., 20, 14741–14755, https://doi.org/10.5194/acp-20-14741-2020, https://doi.org/10.5194/acp-20-14741-2020, 2020
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A recent aircraft field campaign near the Azores in the summer of 2017 provides ample observations of aerosols and clouds with detailed vertical information. This study utilizes those observational data in combination with the aerosol-aware large-eddy simulations and aerosol reanalysis data to examine the significance of the long-range-transported aerosol effect on marine-boundary-layer clouds. It is the first time that the ACE-ENA aircraft campaign data are used for this topic.
Brigitte Rooney, Yuan Wang, Jonathan H. Jiang, Bin Zhao, Zhao-Cheng Zeng, and John H. Seinfeld
Atmos. Chem. Phys., 20, 14597–14616, https://doi.org/10.5194/acp-20-14597-2020, https://doi.org/10.5194/acp-20-14597-2020, 2020
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Wildfires have become increasingly prevalent. Intense smoke consisting of particulate matter (PM) leads to an increased risk of morbidity and mortality. The record-breaking Camp Fire ravaged Northern California for two weeks in 2018. Here, we employ a comprehensive chemical transport model along with ground-based and satellite observations to characterize the PM concentrations across Northern California and to investigate the pollution sensitivity predictions to key parameters of the model.
Dale M. Ward, Xiquan Dong, Baike Xi, Peng Wu, Xiaojian Zheng, and Yuan Wang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-817, https://doi.org/10.5194/acp-2020-817, 2020
Preprint withdrawn
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Marine boundary layer clouds in subtropical regions strongly impact global energy balance, but complete understanding of the processes that control their development remain elusive. We analyze aircraft in-situ measurements of clouds collected in a field campaign for cases that contain organized structures tens of kilometres in extent embedded within a larger overcast cloud field. Failure to account for these structures can lead to misrepresentation in models and satellite retrievals.
Xiaojian Zheng, Baike Xi, Xiquan Dong, Timothy Logan, Yuan Wang, and Peng Wu
Atmos. Chem. Phys., 20, 3483–3501, https://doi.org/10.5194/acp-20-3483-2020, https://doi.org/10.5194/acp-20-3483-2020, 2020
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The continental low-level stratiform cloud susceptibilities to aerosols were investigated under different absorptive aerosol regimes. The weakly absorbing aerosols, which are more hygroscopic, can better activate as cloud condensation nuclei. The favorable thermodynamic condition enhances the cloud susceptibility, while the cloud-layer heating effect induced by strongly absorbing aerosols dampens the cloud susceptibility. Overall, the clouds are more susceptible to the weakly absorbing aerosols.
Misti Levy Zamora, Jianfei Peng, Min Hu, Song Guo, Wilmarie Marrero-Ortiz, Dongjie Shang, Jing Zheng, Zhuofei Du, Zhijun Wu, and Renyi Zhang
Atmos. Chem. Phys., 19, 14329–14338, https://doi.org/10.5194/acp-19-14329-2019, https://doi.org/10.5194/acp-19-14329-2019, 2019
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Severe haze formation in Beijing during wintertime is attributed to explosive secondary aerosol formation including particle nucleation and subsequent particle growth. Organic matter is responsible for producing nucleation mode particles, while secondary organic and inorganic components jointly contribute to the high aerosol mass during haze episodes. High levels of gaseous precursors and stagnant air mass are responsible for fast secondary aerosol formation.
Yun Lin, Yuemeng Ji, Yixin Li, Jeremiah Secrest, Wen Xu, Fei Xu, Yuan Wang, Taicheng An, and Renyi Zhang
Atmos. Chem. Phys., 19, 8003–8019, https://doi.org/10.5194/acp-19-8003-2019, https://doi.org/10.5194/acp-19-8003-2019, 2019
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We have investigated the molecular interactions between succinic acid and sulfuric acid–base clusters in the presence of hydration, including ammonia and dimethylamine. Our results indicate that the multicomponent nucleation involving organic acids, sulfuric acid, and base species promotes new particle formation in the atmosphere, particularly under polluted conditions.
Brigitte Rooney, Ran Zhao, Yuan Wang, Kelvin H. Bates, Ajay Pillarisetti, Sumit Sharma, Seema Kundu, Tami C. Bond, Nicholas L. Lam, Bora Ozaltun, Li Xu, Varun Goel, Lauren T. Fleming, Robert Weltman, Simone Meinardi, Donald R. Blake, Sergey A. Nizkorodov, Rufus D. Edwards, Ankit Yadav, Narendra K. Arora, Kirk R. Smith, and John H. Seinfeld
Atmos. Chem. Phys., 19, 7719–7742, https://doi.org/10.5194/acp-19-7719-2019, https://doi.org/10.5194/acp-19-7719-2019, 2019
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Approximately 3 billion people worldwide cook with solid fuels, such as wood, charcoal, and agricultural residues, that are often combusted in inefficient cookstoves. Here, we simulate the distribution of the two major health-damaging outdoor pollution species (PM2.5 and O3) using state-of-the-science emissions databases and atmospheric chemical transport models to estimate the impact of household combustion on ambient air quality in India.
Hao Guo, Sri Harsha Kota, Kaiyu Chen, Shovan Kumar Sahu, Jianlin Hu, Qi Ying, Yuan Wang, and Hongliang Zhang
Atmos. Chem. Phys., 18, 15219–15229, https://doi.org/10.5194/acp-18-15219-2018, https://doi.org/10.5194/acp-18-15219-2018, 2018
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A total of 1.04 million premature mortalities and up to 2 years of life lost (YLL) per person were estimated in India in 2015 due to PM2.5. Premature mortality due to cerebrovascular disease (CEVD) was the highest (0.44 million), followed by ischaemic heart disease (IHD, 0.40 million). The residential sector was the largest contributor, followed by industry, agriculture and energy. Reducing PM2.5 concentrations would lead to a significant reduction in premature mortality and YLL.
Gehui Wang, Fang Zhang, Jianfei Peng, Lian Duan, Yuemeng Ji, Wilmarie Marrero-Ortiz, Jiayuan Wang, Jianjun Li, Can Wu, Cong Cao, Yuan Wang, Jun Zheng, Jeremiah Secrest, Yixin Li, Yuying Wang, Hong Li, Na Li, and Renyi Zhang
Atmos. Chem. Phys., 18, 10123–10132, https://doi.org/10.5194/acp-18-10123-2018, https://doi.org/10.5194/acp-18-10123-2018, 2018
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Several studies using thermodynamic models estimated pH and sulfate formation rate during pollution periods in China are highly conflicting. Here we show distinct sulfate formation for organic seed particles from that of (NH4)2SO4 seeds, when the particles are exposed to SO2, NO2, and NH3 at high RH. Our results reveal that the pH value of ambient organics-dominated aerosols is sufficiently high to promote efficient SO2 oxidation by NO2 with NH3 neutralization under polluted conditions in China.
Pengfei Tian, Lei Zhang, Jianmin Ma, Kai Tang, Lili Xu, Yuan Wang, Xianjie Cao, Jiening Liang, Yuemeng Ji, Jonathan H. Jiang, Yuk L. Yung, and Renyi Zhang
Atmos. Chem. Phys., 18, 7815–7825, https://doi.org/10.5194/acp-18-7815-2018, https://doi.org/10.5194/acp-18-7815-2018, 2018
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The mixing of dust and anthropogenic pollution over East Asia plays a significant yet poorly quantified role in aerosol radiative effects. We have found that radiative absorption of the East Asian aerosol mixtures are significantly enhanced. Our results show that the interaction between dust and anthropogenic pollution not only represents a viable aerosol formation pathway but also results in unfavorable dispersion conditions, both exacerbating the regional air pollution in East Asia.
Kai Tang, Zhongwei Huang, Jianping Huang, Teruya Maki, Shuang Zhang, Atsushi Shimizu, Xiaojun Ma, Jinsen Shi, Jianrong Bi, Tian Zhou, Guoyin Wang, and Lei Zhang
Atmos. Chem. Phys., 18, 7131–7148, https://doi.org/10.5194/acp-18-7131-2018, https://doi.org/10.5194/acp-18-7131-2018, 2018
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To our knowledge, this is the first simultaneous field measurement of bioaerosols in dust events at four sites along the transport pathway of Asian dust. The samples were analyzed by means of fluorescence microscopy, scanning electron microscopy, and MiSeq sequencing analysis. The results indicate that dust clouds can carry many bacteria of various types into downwind regions, the alpha and beta diversity of which were investigated.
Xin Wang, Hui Wen, Jinsen Shi, Jianrong Bi, Zhongwei Huang, Beidou Zhang, Tian Zhou, Kaiqi Fu, Quanliang Chen, and Jinyuan Xin
Atmos. Chem. Phys., 18, 2119–2138, https://doi.org/10.5194/acp-18-2119-2018, https://doi.org/10.5194/acp-18-2119-2018, 2018
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A ground-based mobile laboratory was deployed near the dust source regions over northwestern China.
We not only captured natural dust but also characterized the properties of anthropogenic soil dust produced by agricultural cultivations.
The results indicate that large differences were found between the optical and microphysical properties of anthropogenic and natural dust.
Jianzhong Xu, Qi Zhang, Jinsen Shi, Xinlei Ge, Conghui Xie, Junfeng Wang, Shichang Kang, Ruixiong Zhang, and Yuhang Wang
Atmos. Chem. Phys., 18, 427–443, https://doi.org/10.5194/acp-18-427-2018, https://doi.org/10.5194/acp-18-427-2018, 2018
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This manuscript presents results from a comprehensive field study using an HR-AMS coupled with a suite of other instruments in central Tibetan Plateau. The study discusses the chemical composition, sources, and processes of submicron aerosol during the transition from pre-monsoon to monsoon. Organic aerosol was overall highly oxidized during the entire study with higher O / C ratios during the pre-monsoon period. Sensitivity of air pollution transport with synoptic process was also evaluated.
Zhijuan Zhang, Bin Chen, Jianping Huang, Jingjing Liu, Jianrong Bi, Tian Zhou, and Zhongwei Huang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-1000, https://doi.org/10.5194/acp-2017-1000, 2017
Revised manuscript not accepted
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Environmental problems caused by aerosols such as dust aerosols are influencing people's lives and work. Due to different radiative effects of different types of aerosols, detection of the aerosol type is vital for improving our air quality. In this study, the optical properties of pure dust and transported anthropogenic dust are compared by using ground-based Lidar data. Based on our conclusion, detection of different dust aerosols will be more accurate using satellite-based Lidar.
Jianfei Peng, Min Hu, Song Guo, Zhuofei Du, Dongjie Shang, Jing Zheng, Jun Zheng, Limin Zeng, Min Shao, Yusheng Wu, Don Collins, and Renyi Zhang
Atmos. Chem. Phys., 17, 10333–10348, https://doi.org/10.5194/acp-17-10333-2017, https://doi.org/10.5194/acp-17-10333-2017, 2017
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Rapid growth of BC particles was observed in Beijing using a new outdoor chamber, with an average growth rate of 26 ± 11 nm h−1. Secondary organic aerosol (SOA) accounted for more than 90 % of the coating mass. The hygroscopic growth factor of BC particles increased to 1.06–1.08 upon ageing. The κ (kappa) values for BC particles were calculated as only 0.035, indicating that initial photochemical ageing of BC particles does not appreciably alter the particle hygroscopicity in Beijing.
Yujiao Zhu, Caiqing Yan, Renyi Zhang, Zifa Wang, Mei Zheng, Huiwang Gao, Yang Gao, and Xiaohong Yao
Atmos. Chem. Phys., 17, 9469–9484, https://doi.org/10.5194/acp-17-9469-2017, https://doi.org/10.5194/acp-17-9469-2017, 2017
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This study reports the distinct effects of street canyons on new particle formation (NPF) under warm or cold ambient temperature conditions because of on-road vehicle emissions; i.e., stronger condensation sinks are responsible for the reduced NPF in the springtime, but efficient nucleation and partitioning of gaseous species contribute to the enhanced NPF in the wintertime. The oxidization of biogenic organics is suggested to play an important role in growing new particles.
Jinming Ge, Zeen Zhu, Chuang Zheng, Hailing Xie, Tian Zhou, Jianping Huang, and Qiang Fu
Atmos. Chem. Phys., 17, 9035–9047, https://doi.org/10.5194/acp-17-9035-2017, https://doi.org/10.5194/acp-17-9035-2017, 2017
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A modified method with a new noise reduction scheme that can reduce the noise distribution to a narrow range is proposed to distinguish clouds and other hydrometeors from noise and recognize more features with weak signal in cloud radar observations. It was found that our method has significant advantages in reducing the rates of both failed negative and false positive hydrometeor identifications in simulated clouds and recognizing clouds with weak signal from our cloud radar observations.
Jianrong Bi, Jianping Huang, Jinsen Shi, Zhiyuan Hu, Tian Zhou, Guolong Zhang, Zhongwei Huang, Xin Wang, and Hongchun Jin
Atmos. Chem. Phys., 17, 7775–7792, https://doi.org/10.5194/acp-17-7775-2017, https://doi.org/10.5194/acp-17-7775-2017, 2017
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We conducted a field campaign on exploring dust aerosol in Dunhuang farmland nearby Gobi deserts. The anthropogenic dust produced by agricultural cultivations exerted a significant superimposed effect on elevated dust loadings. Strong south wind in daytime scavenged the pollution and weak northeast wind at night favorably accumulated air pollutants near the surface. The local emissions remarkably modified the absorptive and optical characteristics of mineral dust in desert source region.
Wei Pu, Xin Wang, Hailun Wei, Yue Zhou, Jinsen Shi, Zhiyuan Hu, Hongchun Jin, and Quanliang Chen
The Cryosphere, 11, 1213–1233, https://doi.org/10.5194/tc-11-1213-2017, https://doi.org/10.5194/tc-11-1213-2017, 2017
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We conducted a large field campaign to collect snow samples in Xinjiang. We measured insoluble light-absorbing particles with estimated black carbon concentrations of 10–150 ngg-1. We found a probable shift in emission sources with the progression of winter and dominated contributions of BC and OC to light absorption. A PMF model indicated an optimal three-factor/source solution that included industrial pollution, biomass burning, and soil dust.
Siyu Chen, Jianping Huang, Litai Kang, Hao Wang, Xiaojun Ma, Yongli He, Tiangang Yuan, Ben Yang, Zhongwei Huang, and Guolong Zhang
Atmos. Chem. Phys., 17, 2401–2421, https://doi.org/10.5194/acp-17-2401-2017, https://doi.org/10.5194/acp-17-2401-2017, 2017
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Compared with the TD dust, the importance of the GD dust in eastern China, Japan, and Korea is always neglected. We focused primarily on the dynamic and thermodynamics mechanisms of dust emission and transport over TD and GD and further elucidate the influence of TD and GD dust on the entire East Asia based on a case study using WRF-Chem model in the study.
Xin Wang, Wei Pu, Yong Ren, Xuelei Zhang, Xueying Zhang, Jinsen Shi, Hongchun Jin, Mingkai Dai, and Quanliang Chen
Atmos. Chem. Phys., 17, 2279–2296, https://doi.org/10.5194/acp-17-2279-2017, https://doi.org/10.5194/acp-17-2279-2017, 2017
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A 2014 snow survey was performed across northeastern China to analyze light absorption of ILAPs in seasonal snow, and modeling studies were conducted to compare snow albedo reduction due to assumptions of internal–external mixing of BC in snow and different snow grain shapes. The results show that the simulated snow albedos from both SAMDS and SNICAR agree well with the observed values at low ILAP mixing ratios, but they tend to be higher than surface observations at high ILAP mixing ratios.
Jianzhong Xu, Jinsen Shi, Qi Zhang, Xinlei Ge, Francesco Canonaco, André S. H. Prévôt, Matthias Vonwiller, Sönke Szidat, Jinming Ge, Jianmin Ma, Yanqing An, Shichang Kang, and Dahe Qin
Atmos. Chem. Phys., 16, 14937–14957, https://doi.org/10.5194/acp-16-14937-2016, https://doi.org/10.5194/acp-16-14937-2016, 2016
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This study deployed an AMS field study in Lanzhou, a city in northwestern China, evaluating the chemical composition, sources, and processes of urban aerosols during wintertime. In comparison with the results during summer in Lanzhou, the air pollution during winter was more severe and the sources were more complex. In addition, this paper estimates the contributions of fossil and non-fossil sources of organic carbon to primary and secondary organic carbon using the carbon isotopic method.
C. He, K.-N. Liou, Y. Takano, R. Zhang, M. Levy Zamora, P. Yang, Q. Li, and L. R. Leung
Atmos. Chem. Phys., 15, 11967–11980, https://doi.org/10.5194/acp-15-11967-2015, https://doi.org/10.5194/acp-15-11967-2015, 2015
T. Logan, B. Xi, and X. Dong
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-13-32269-2013, https://doi.org/10.5194/acpd-13-32269-2013, 2013
Revised manuscript not accepted
T. Logan, B. Xi, X. Dong, Z. Li, and M. Cribb
Atmos. Chem. Phys., 13, 2253–2265, https://doi.org/10.5194/acp-13-2253-2013, https://doi.org/10.5194/acp-13-2253-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
The role of refractive indices in measuring mineral dust with high-spectral-resolution infrared satellite sounders: application to the Gobi Desert
Influence of covariance of aerosol and meteorology on co-located precipitating and non-precipitating clouds over the Indo-Gangetic Plain
Light-absorbing black carbon and brown carbon components of smoke aerosol from DSCOVR EPIC measurements over North America and central Africa
Fluorescence properties of long-range transported smoke: Insights from five-channel lidar observations over Moscow during the 2023 wildfire season
Distinct effects of Fine and Coarse Aerosols on Microphysical Processes of Shallow Precipitation Systems in Summer over Southern China
The emission, transport, and impacts of the extreme Saharan dust storm of 2015
Increased number concentrations of small particles explains perceived stagnation in air quality over Korea
California wildfire smoke contributes to a positive atmospheric temperature anomaly over the western United States
Remote Sensing detectability of airborne Arctic dust
Dust storms from the Taklamakan Desert significantly darken snow surface on surrounding mountains
Opposite effects of aerosols and meteorological parameters on warm clouds in two contrasting regions over eastern China
Effect of wind speed on marine aerosol optical properties over remote oceans with use of spaceborne lidar observations
Assessment of smoke plume height products derived from multisource satellite observations using lidar-derived height metrics for wildfires in the western US
A remote sensing algorithm for vertically resolved cloud condensation nuclei number concentrations from airborne and spaceborne lidar observations
Opinion: Aerosol remote sensing over the next 20 years
Monitoring biomass burning aerosol transport using CALIOP observations and reanalysis models: a Canadian wildfire event in 2019
Thermal infrared observations of a western United States biomass burning aerosol plume
A new look into the impacts of dust radiative effects on the energetics of tropical easterly waves
Wind-driven emissions of coarse-mode particles in an urban environment
Measurement report: Dust and anthropogenic aerosols' vertical distributions over northern China dense aerosols gathered at the top of the mixing layer
Climatological assessment of the vertically resolved optical and microphysical aerosol properties by lidar measurements, sun photometer, and in situ observations over 17 years at Universitat Politècnica de Catalunya (UPC) Barcelona
Aerosol optical depth climatology from the high-resolution MAIAC product over Europe: differences between major European cities and their surrounding environments
Impact of assimilating NOAA VIIRS aerosol optical depth (AOD) observations on global AOD analysis from the Copernicus Atmosphere Monitoring Service (CAMS)
Spectral dependence of birch and pine pollen optical properties using a synergy of lidar instruments
Validation activities of Aeolus wind products on the southeastern Iberian Peninsula
Thermal infrared dust optical depth and coarse-mode effective diameter over oceans retrieved from collocated MODIS and CALIOP observations
A comprehensive reappraisal of long-term aerosol characteristics, trends, and variability in Asia
Satellite (GOSAT-2 CAI-2) retrieval and surface (ARFINET) observations of aerosol black carbon over India
Spatiotemporal variation characteristics of global fires and their emissions
The (mis)identification of high-latitude dust events using remote sensing methods in the Yukon, Canada: a sub-daily variability analysis
Comparison of dust optical depth from multi-sensor products and MONARCH (Multiscale Online Non-hydrostatic AtmospheRe CHemistry) dust reanalysis over North Africa, the Middle East, and Europe
Understanding day–night differences in dust aerosols over the dust belt of North Africa, the Middle East, and Asia
Satellite observations of smoke–cloud–radiation interactions over the Amazon rainforest
Single-scattering properties of ellipsoidal dust aerosols constrained by measured dust shape distributions
Validation of the TROPOMI/S5P aerosol layer height using EARLINET lidars
Vertical characterization of fine and coarse dust particles during an intense Saharan dust outbreak over the Iberian Peninsula in springtime 2021
Aerosol optical depth regime over megacities of the world
South American 2020 regional smoke plume: intercomparison with previous years, impact on solar radiation, and the role of Pantanal biomass burning season
Circular polarization in atmospheric aerosols
Spatiotemporal continuous estimates of daily 1 km PM2.5 from 2000 to present under the Tracking Air Pollution in China (TAP) framework
Robust evidence for reversal of the trend in aerosol effective climate forcing
Simultaneous retrievals of biomass burning aerosols and trace gases from the ultraviolet to near-infrared over northern Thailand during the 2019 pre-monsoon season
A decadal assessment of the climatology of aerosol and cloud properties over South Africa
Aerosol characterisation in the subtropical eastern North Atlantic region using long-term AERONET measurements
Long-range transport of Asian dust to the Arctic: identification of transport pathways, evolution of aerosol optical properties, and impact assessment on surface albedo changes
Canadian and Alaskan wildfire smoke particle properties, their evolution, and controlling factors, from satellite observations
Evaluation of aerosol optical depths and clear-sky radiative fluxes of the CERES Edition 4.1 SYN1deg data product
Arctic spring and summertime aerosol optical depth baseline from long-term observations and model reanalyses – Part 1: Climatology and trend
Vertical structure of biomass burning aerosol transported over the southeast Atlantic Ocean
Arctic spring and summertime aerosol optical depth baseline from long-term observations and model reanalyses – Part 2: Statistics of extreme AOD events, and implications for the impact of regional biomass burning processes
Perla Alalam, Fabrice Ducos, and Hervé Herbin
Atmos. Chem. Phys., 24, 12277–12294, https://doi.org/10.5194/acp-24-12277-2024, https://doi.org/10.5194/acp-24-12277-2024, 2024
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This study dives into the impact of mineral dust laboratory complex refractive indices (CRIs) on quantifying the dust microphysical properties using satellite infrared remote sensing. Results show that using CRIs obtained by advanced realistic techniques can improve the accuracy of these measurements, emphasizing the importance of choosing the suitable CRI in atmospheric models. This improvement is crucial for better predicting the dust radiative effect and impact on the climate.
Nabia Gulistan, Khan Alam, and Yangang Liu
Atmos. Chem. Phys., 24, 11333–11349, https://doi.org/10.5194/acp-24-11333-2024, https://doi.org/10.5194/acp-24-11333-2024, 2024
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This study looks at the influence of aerosol and meteorology on precipitating and non-precipitating clouds over the Indo-Gangetic Plain (IGP). A major finding of this study was that the high loading of aerosols led to a high occurrence of precipitating clouds under unstable conditions in summer. The study has the potential to open a new avenue for the scientific community to further explore and understand the complications of aerosol–cloud–precipitation over the complex topography of the IGP.
Myungje Choi, Alexei Lyapustin, Gregory L. Schuster, Sujung Go, Yujie Wang, Sergey Korkin, Ralph Kahn, Jeffrey S. Reid, Edward J. Hyer, Thomas F. Eck, Mian Chin, David J. Diner, Olga Kalashnikova, Oleg Dubovik, Jhoon Kim, and Hans Moosmüller
Atmos. Chem. Phys., 24, 10543–10565, https://doi.org/10.5194/acp-24-10543-2024, https://doi.org/10.5194/acp-24-10543-2024, 2024
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This paper introduces a retrieval algorithm to estimate two key absorbing components in smoke (black carbon and brown carbon) using DSCOVR EPIC measurements. Our analysis reveals distinct smoke properties, including spectral absorption, layer height, and black carbon and brown carbon, over North America and central Africa. The retrieved smoke properties offer valuable observational constraints for modeling radiative forcing and informing health-related studies.
Igor Veselovskii, Mikhail Korenskiy, Nikita Kasianik, Boris Barchunov, Qiaoyun Hu, Philippe Goloub, and Thierry Podvin
EGUsphere, https://doi.org/10.5194/egusphere-2024-2874, https://doi.org/10.5194/egusphere-2024-2874, 2024
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A fluorescence lidar was utilized to study transported smoke during the wildfire season from May to September 2023. The lidar performs fluorescence measurements at 5 wavelengths. Observations reveal that the fluorescence capacity increases with altitude, suggesting higher concentration of organic compounds in the UTLS compared to the lower troposphere. And urban aerosol fluorescence tends to decrease with wavelength, while the peak of smoke fluorescence is observed at 513 or 560 nm channels.
Fengjiao Chen, Yuanjian Yang, Lu Yu, Yang Li, Weiguang Liu, Yan Liu, and Simone Lolli
EGUsphere, https://doi.org/10.5194/egusphere-2024-2206, https://doi.org/10.5194/egusphere-2024-2206, 2024
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The precipitation microphysical mechanisms responsible for the varied impacts of aerosols on shallow precipitation remain unclear. This study reveals that coarse aerosols invigorate shallow rainfall through enhanced coalescence processes, whereas fine aerosols suppress shallow rainfall via intensified breakup microphysical processes. These impacts are independent of thermodynamic environments but are more significant in low-humidity conditions.
Brian Harr, Bing Pu, and Qinjian Jin
Atmos. Chem. Phys., 24, 8625–8651, https://doi.org/10.5194/acp-24-8625-2024, https://doi.org/10.5194/acp-24-8625-2024, 2024
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We found that the formation of the extreme trans-Atlantic African dust event in June 2015 was associated with a brief surge in dust emissions over western North Africa and extreme circulation patterns, including intensified easterly jets, which facilitated the westward transport of dust. The dust plume modified radiative flux along its transport pathway but had minor impacts on air quality in the US due to the record-high Caribbean low-level jet advecting part of the plume to the Pacific.
Sohee Joo, Juseon Shin, Matthias Tesche, Dehkhoda Naghmeh, Taegyeong Kim, and Youngmin Noh
EGUsphere, https://doi.org/10.5194/egusphere-2024-1208, https://doi.org/10.5194/egusphere-2024-1208, 2024
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In our study, we investigated why, in Northeast Asia, visibility has not improved even though air pollution levels have decreased. By examining trends in Seoul and Ulsan, we found that the particles in the air are getting smaller, which scatters light more effectively and reduces how far we can see. Our findings suggest that changes in particle properties adversely affected public perception of air quality improvement even though the PM2.5 mass concentration is continuously decreasing.
James L. Gomez, Robert J. Allen, and King-Fai Li
Atmos. Chem. Phys., 24, 6937–6963, https://doi.org/10.5194/acp-24-6937-2024, https://doi.org/10.5194/acp-24-6937-2024, 2024
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Wildfires in California (CA) have grown very large during the past 20 years. These fires emit sunlight-absorbing aerosols. Analyzing observational data, our study finds that aerosols emitted from large fires in northern CA spread throughout CA and Nevada and heat the atmosphere. This heating is consistent with larger-than-normal temperatures and dry conditions. Further study is needed to determine how much the aerosols heat the atmosphere and whether they are drying the atmosphere as well.
Norman T. O’Neill, Keyvan Ranjbar, Liviu Ivănescu, Yann Blanchard, Seyed Ali Sayedain, and Yasmin AboEl-Fetouh
EGUsphere, https://doi.org/10.5194/egusphere-2024-1057, https://doi.org/10.5194/egusphere-2024-1057, 2024
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Dust from mid-latitude deserts or from local drainage basins is a weak component of atmospheric aerosols in the Arctic. Satellite-based dust estimates are often overestimated because dust and cloud measurements can be confused. Illustrations are given with an emphasis on the flawed claim that a classic indicator of dust (negative brightness temperature differences) is proof of the presence of airborne Arctic dust. Low altitude “warm” water plumes are the likely source of such negative values.
Yuxuan Xing, Yang Chen, Shirui Yan, Xiaoyi Cao, Yong Zhou, Xueying Zhang, Tenglong Shi, Xiaoying Niu, Dongyou Wu, Jiecan Cui, Yue Zhou, Xin Wang, and Wei Pu
Atmos. Chem. Phys., 24, 5199–5219, https://doi.org/10.5194/acp-24-5199-2024, https://doi.org/10.5194/acp-24-5199-2024, 2024
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This study investigated the impact of dust storms from the Taklamakan Desert on surrounding high mountains and regional radiation balance. Using satellite data and simulations, researchers found that dust storms significantly darken the snow surface in the Tien Shan, Kunlun, and Qilian mountains, reaching mountains up to 1000 km away. This darkening occurs not only in spring but also during summer and autumn, leading to increased absorption of solar radiation.
Yuqin Liu, Tao Lin, Jiahua Zhang, Fu Wang, Yiyi Huang, Xian Wu, Hong Ye, Guoqin Zhang, Xin Cao, and Gerrit de Leeuw
Atmos. Chem. Phys., 24, 4651–4673, https://doi.org/10.5194/acp-24-4651-2024, https://doi.org/10.5194/acp-24-4651-2024, 2024
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A new method, the geographical detector method (GDM), has been applied to satellite data, in addition to commonly used statistical methods, to study the sensitivity of cloud properties to aerosol over China. Different constraints for aerosol and cloud liquid water path apply over polluted and clean areas. The GDM shows that cloud parameters are more sensitive to combinations of parameters than to individual parameters, but confounding effects due to co-variation of parameters cannot be excluded.
Kangwen Sun, Guangyao Dai, Songhua Wu, Oliver Reitebuch, Holger Baars, Jiqiao Liu, and Suping Zhang
Atmos. Chem. Phys., 24, 4389–4409, https://doi.org/10.5194/acp-24-4389-2024, https://doi.org/10.5194/acp-24-4389-2024, 2024
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This paper investigates the correlation between marine aerosol optical properties and wind speeds over remote oceans using the spaceborne lidars ALADIN and CALIOP. Three remote ocean areas are selected. Pure marine aerosol optical properties at 355 nm are derived from ALADIN. The relationships between marine aerosol optical properties and wind speeds are analyzed within and above the marine atmospheric boundary layer, revealing the effect of wind speed on marine aerosols over remote oceans.
Jingting Huang, S. Marcela Loría-Salazar, Min Deng, Jaehwa Lee, and Heather A. Holmes
Atmos. Chem. Phys., 24, 3673–3698, https://doi.org/10.5194/acp-24-3673-2024, https://doi.org/10.5194/acp-24-3673-2024, 2024
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Increased wildfire intensity has resulted in taller wildfire smoke plumes. We investigate the vertical structure of wildfire smoke plumes using aircraft lidar data and establish two effective smoke plume height metrics. Four novel satellite-based plume height products are evaluated for wildfires in the western US. Our results provide guidance on the strengths and limitations of these satellite products and set the stage for improved plume rise estimates by leveraging satellite products.
Piyushkumar N. Patel, Jonathan H. Jiang, Ritesh Gautam, Harish Gadhavi, Olga Kalashnikova, Michael J. Garay, Lan Gao, Feng Xu, and Ali Omar
Atmos. Chem. Phys., 24, 2861–2883, https://doi.org/10.5194/acp-24-2861-2024, https://doi.org/10.5194/acp-24-2861-2024, 2024
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Global measurements of cloud condensation nuclei (CCN) are essential for understanding aerosol–cloud interactions and predicting climate change. To address this gap, we introduced a remote sensing algorithm that retrieves vertically resolved CCN number concentrations from airborne and spaceborne lidar systems. This innovation offers a global distribution of CCN concentrations from space, facilitating model evaluation and precise quantification of aerosol climate forcing.
Lorraine A. Remer, Robert C. Levy, and J. Vanderlei Martins
Atmos. Chem. Phys., 24, 2113–2127, https://doi.org/10.5194/acp-24-2113-2024, https://doi.org/10.5194/acp-24-2113-2024, 2024
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Aerosols are small liquid or solid particles suspended in the atmosphere, including smoke, particulate pollution, dust, and sea salt. Today, we rely on satellites viewing Earth's atmosphere to learn about these particles. Here, we speculate on the future to imagine how satellite viewing of aerosols will change. We expect more public and private satellites with greater capabilities, better ways to infer information from satellites, and merging of data with models.
Xiaoxia Shang, Antti Lipponen, Maria Filioglou, Anu-Maija Sundström, Mark Parrington, Virginie Buchard, Anton S. Darmenov, Ellsworth J. Welton, Eleni Marinou, Vassilis Amiridis, Michael Sicard, Alejandro Rodríguez-Gómez, Mika Komppula, and Tero Mielonen
Atmos. Chem. Phys., 24, 1329–1344, https://doi.org/10.5194/acp-24-1329-2024, https://doi.org/10.5194/acp-24-1329-2024, 2024
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In June 2019, smoke particles from a Canadian wildfire event were transported to Europe. The long-range-transported smoke plumes were monitored with a spaceborne lidar and reanalysis models. Based on the aerosol mass concentrations estimated from the observations, the reanalysis models had difficulties in reproducing the amount and location of the smoke aerosols during the transport event. Consequently, more spaceborne lidar missions are needed for reliable monitoring of aerosol plumes.
Blake T. Sorenson, Jeffrey S. Reid, Jianglong Zhang, Robert E. Holz, William L. Smith Sr., and Amanda Gumber
Atmos. Chem. Phys., 24, 1231–1248, https://doi.org/10.5194/acp-24-1231-2024, https://doi.org/10.5194/acp-24-1231-2024, 2024
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Smoke particles are typically submicron in size and assumed to have negligible impacts at the thermal infrared spectrum. However, we show that infrared signatures can be observed over dense smoke plumes from satellites. We found that giant particles are unlikely to be the dominant cause. Rather, co-transported water vapor injected to the middle to upper troposphere and surface cooling beneath the plume due to shadowing are significant, with the surface cooling effect being the most dominant.
Farnaz Hosseinpour and Eric M. Wilcox
Atmos. Chem. Phys., 24, 707–724, https://doi.org/10.5194/acp-24-707-2024, https://doi.org/10.5194/acp-24-707-2024, 2024
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This study shows mechanistic relationships between the radiative effect of dust aerosols in the Saharan air layer and the kinetic energy of the African easterly waves across the tropical Atlantic Ocean using 22 years of daily satellite observations and reanalysis data based on satellite assimilation. Our findings suggest that dust aerosols not merely are transported by these waves but also contribute to the growth of waves through the enhancement of diabatic heating induced by dust.
Markus D. Petters, Tyas Pujiastuti, Ajmal Rasheeda Satheesh, Sabin Kasparoglu, Bethany Sutherland, and Nicholas Meskhidze
Atmos. Chem. Phys., 24, 745–762, https://doi.org/10.5194/acp-24-745-2024, https://doi.org/10.5194/acp-24-745-2024, 2024
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This work introduces a new method that uses remote sensing techniques to obtain surface number emissions of particles with a diameter greater than 500 nm. The technique was applied to study particle emissions at an urban site near Houston, TX, USA. The emissions followed a diurnal pattern and peaked near noon local time. The daily averaged emissions correlated with wind speed. The source is likely due to wind-driven erosion of material situated on asphalted and other hard surfaces.
Zhuang Wang, Chune Shi, Hao Zhang, Yujia Chen, Xiyuan Chi, Congzi Xia, Suyao Wang, Yizhi Zhu, Kaidi Zhang, Xintong Chen, Chengzhi Xing, and Cheng Liu
Atmos. Chem. Phys., 23, 14271–14292, https://doi.org/10.5194/acp-23-14271-2023, https://doi.org/10.5194/acp-23-14271-2023, 2023
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The annual cycle of dust and anthropogenic aerosols' vertical distributions was revealed by polarization Raman lidar in Beijing. Anthropogenic aerosols typically accumulate at the top of the mixing layer (ML) due to the hygroscopic growth of atmospheric particles, and this is most significant in summer. There is no significant relationship between bottom dust mass concentration and ML height, while the dust in the upper air tends to be distributed near the mixing layer.
Simone Lolli, Michaël Sicard, Francesco Amato, Adolfo Comeron, Cristina Gíl-Diaz, Tony C. Landi, Constantino Munoz-Porcar, Daniel Oliveira, Federico Dios Otin, Francesc Rocadenbosch, Alejandro Rodriguez-Gomez, Andrés Alastuey, Xavier Querol, and Cristina Reche
Atmos. Chem. Phys., 23, 12887–12906, https://doi.org/10.5194/acp-23-12887-2023, https://doi.org/10.5194/acp-23-12887-2023, 2023
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We evaluated the long-term trends and seasonal variability of the vertically resolved aerosol properties over the past 17 years in Barcelona. Results shows that air quality is improved, with a consistent drop in PM concentrations at the surface, as well as the column aerosol optical depth. The results also show that natural dust outbreaks are more likely in summer, with aerosols reaching an altitude of 5 km, while in winter, aerosols decay as an exponential with a scale height of 600 m.
Ludovico Di Antonio, Claudia Di Biagio, Gilles Foret, Paola Formenti, Guillaume Siour, Jean-François Doussin, and Matthias Beekmann
Atmos. Chem. Phys., 23, 12455–12475, https://doi.org/10.5194/acp-23-12455-2023, https://doi.org/10.5194/acp-23-12455-2023, 2023
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Long-term (2000–2021) 1 km resolution satellite data have been used to investigate the climatological aerosol optical depth (AOD) variability and trends at different scales in Europe. Average enhancements of the local-to-regional AOD ratio at 550 nm of 57 %, 55 %, 39 % and 32 % are found for large metropolitan areas such as Barcelona, Lisbon, Paris and Athens, respectively, suggesting a non-negligible enhancement of the aerosol burden through local emissions.
Sebastien Garrigues, Melanie Ades, Samuel Remy, Johannes Flemming, Zak Kipling, Istvan Laszlo, Mark Parrington, Antje Inness, Roberto Ribas, Luke Jones, Richard Engelen, and Vincent-Henri Peuch
Atmos. Chem. Phys., 23, 10473–10487, https://doi.org/10.5194/acp-23-10473-2023, https://doi.org/10.5194/acp-23-10473-2023, 2023
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The Copernicus Atmosphere Monitoring Service (CAMS) provides global monitoring of aerosols using the ECMWF forecast model constrained by the assimilation of satellite aerosol optical depth (AOD). This work aims at evaluating the assimilation of the NOAA VIIRS AOD product in the ECMWF model. It shows that the introduction of VIIRS in the CAMS data assimilation system enhances the accuracy of the aerosol analysis, particularly over Europe and desert and maritime sites.
Maria Filioglou, Ari Leskinen, Ville Vakkari, Ewan O'Connor, Minttu Tuononen, Pekko Tuominen, Samuli Laukkanen, Linnea Toiviainen, Annika Saarto, Xiaoxia Shang, Petri Tiitta, and Mika Komppula
Atmos. Chem. Phys., 23, 9009–9021, https://doi.org/10.5194/acp-23-9009-2023, https://doi.org/10.5194/acp-23-9009-2023, 2023
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Pollen impacts climate and public health, and it can be detected in the atmosphere by lidars which measure the linear particle depolarization ratio (PDR), a shape-relevant optical parameter. As aerosols also cause depolarization, surface aerosol and pollen observations were combined with measurements from ground-based lidars operating at different wavelengths to determine the optical properties of birch and pine pollen and quantify their relative contribution to the PDR.
Jesús Abril-Gago, Pablo Ortiz-Amezcua, Diego Bermejo-Pantaleón, Juana Andújar-Maqueda, Juan Antonio Bravo-Aranda, María José Granados-Muñoz, Francisco Navas-Guzmán, Lucas Alados-Arboledas, Inmaculada Foyo-Moreno, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 23, 8453–8471, https://doi.org/10.5194/acp-23-8453-2023, https://doi.org/10.5194/acp-23-8453-2023, 2023
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Validation activities of Aeolus wind products were performed in Granada with different upward-probing instrumentation (Doppler lidar system and radiosondes) and spatiotemporal collocation criteria. Specific advantages and disadvantages of each instrument were identified, and an optimal comparison criterion is proposed. Aeolus was proven to provide reliable wind products, and the upward-probing instruments were proven to be useful for Aeolus wind product validation activities.
Jianyu Zheng, Zhibo Zhang, Hongbin Yu, Anne Garnier, Qianqian Song, Chenxi Wang, Claudia Di Biagio, Jasper F. Kok, Yevgeny Derimian, and Claire Ryder
Atmos. Chem. Phys., 23, 8271–8304, https://doi.org/10.5194/acp-23-8271-2023, https://doi.org/10.5194/acp-23-8271-2023, 2023
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We developed a multi-year satellite-based retrieval of dust optical depth at 10 µm and the coarse-mode dust effective diameter over global oceans. It reveals climatological coarse-mode dust transport patterns and regional differences over the North Atlantic, the Indian Ocean and the North Pacific.
Shikuan Jin, Yingying Ma, Zhongwei Huang, Jianping Huang, Wei Gong, Boming Liu, Weiyan Wang, Ruonan Fan, and Hui Li
Atmos. Chem. Phys., 23, 8187–8210, https://doi.org/10.5194/acp-23-8187-2023, https://doi.org/10.5194/acp-23-8187-2023, 2023
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To better understand the Asian aerosol environment, we studied distributions and trends of aerosol with different sizes and types. Over the past 2 decades, dust, sulfate, and sea salt aerosol decreased by 5.51 %, 3.07 %, and 9.80 %, whereas organic carbon and black carbon aerosol increased by 17.09 % and 6.23 %, respectively. The increase in carbonaceous aerosols was a feature of Asia. An exception is found in East Asia, where the carbonaceous aerosols reduced, owing largely to China's efforts.
Mukunda M. Gogoi, S. Suresh Babu, Ryoichi Imasu, and Makiko Hashimoto
Atmos. Chem. Phys., 23, 8059–8079, https://doi.org/10.5194/acp-23-8059-2023, https://doi.org/10.5194/acp-23-8059-2023, 2023
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Considering the climate warming potential of atmospheric black carbon (BC), satellite-based retrieval is a novel idea. This study highlights the regional distribution of BC based on observations by the Cloud and Aerosol Imager-2 on board the GOSAT-2 satellite and near-surface measurements of BC in ARFINET. The satellite retrieval fairly depicts the regional and seasonal features of BC over the Indian region, which are similar to those recorded by surface observations.
Hao Fan, Xingchuan Yang, Chuanfeng Zhao, Yikun Yang, and Zhenyao Shen
Atmos. Chem. Phys., 23, 7781–7798, https://doi.org/10.5194/acp-23-7781-2023, https://doi.org/10.5194/acp-23-7781-2023, 2023
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Using 20-year multi-source data, this study shows pronounced regional and seasonal variations in fire activities and emissions. Seasonal variability of fires is larger with increasing latitude. The increase in temperature in the Northern Hemisphere's middle- and high-latitude forest regions was primarily responsible for the increase in fires and emissions, while the changes in fire occurrence in tropical regions were more influenced by the decrease in precipitation and relative humidity.
Rosemary Huck, Robert G. Bryant, and James King
Atmos. Chem. Phys., 23, 6299–6318, https://doi.org/10.5194/acp-23-6299-2023, https://doi.org/10.5194/acp-23-6299-2023, 2023
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This study shows that mineral aerosol (dust) emission events in high-latitude areas are under-represented in both ground- and space-based detecting methods. This is done through a suite of ground-based data to prove that dust emissions from the proglacial area, Lhù’ààn Mân, occur almost daily but are not always recorded at different timescales. Dust has multiple effects on atmospheric processes; therefore, accurate quantification is important in the calibration and validation of climate models.
Michail Mytilinaios, Sara Basart, Sergio Ciamprone, Juan Cuesta, Claudio Dema, Enza Di Tomaso, Paola Formenti, Antonis Gkikas, Oriol Jorba, Ralph Kahn, Carlos Pérez García-Pando, Serena Trippetta, and Lucia Mona
Atmos. Chem. Phys., 23, 5487–5516, https://doi.org/10.5194/acp-23-5487-2023, https://doi.org/10.5194/acp-23-5487-2023, 2023
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Multiscale Online Non-hydrostatic AtmospheRe CHemistry model (MONARCH) dust reanalysis provides a high-resolution 3D reconstruction of past dust conditions, allowing better quantification of climate and socioeconomic dust impacts. We assess the performance of the reanalysis needed to reproduce dust optical depth using dust-related products retrieved from satellite and ground-based observations and show that it reproduces the spatial distribution and seasonal variability of atmospheric dust well.
Jacob Z. Tindan, Qinjian Jin, and Bing Pu
Atmos. Chem. Phys., 23, 5435–5466, https://doi.org/10.5194/acp-23-5435-2023, https://doi.org/10.5194/acp-23-5435-2023, 2023
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We use the Infrared Atmospheric Sounder Interferometer (IASI) retrievals of dust variables (dust optical depth and dust layer height) and surface observations to understand the day- and nighttime variations in dust aerosols over the dust belt. Our results show that daytime dust aerosols are significantly different from nighttime, and such day–night variations are influenced by meteorological factors such as wind speed, precipitation, and turbulent motions within the atmospheric boundary layer.
Ross Herbert and Philip Stier
Atmos. Chem. Phys., 23, 4595–4616, https://doi.org/10.5194/acp-23-4595-2023, https://doi.org/10.5194/acp-23-4595-2023, 2023
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We provide robust evidence from multiple sources showing that smoke from fires in the Amazon rainforest significantly modifies the diurnal cycle of convection and cools the climate. Low to moderate amounts of smoke increase deep convective clouds and rain, whilst beyond a threshold amount, the smoke starts to suppress the convection and rain. We are currently at this threshold, suggesting increases in fires from agricultural practices or droughts will reduce cloudiness and rain over the region.
Yue Huang, Jasper F. Kok, Masanori Saito, and Olga Muñoz
Atmos. Chem. Phys., 23, 2557–2577, https://doi.org/10.5194/acp-23-2557-2023, https://doi.org/10.5194/acp-23-2557-2023, 2023
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Global aerosol models and remote sensing retrievals use dust optical models with inconsistent and inaccurate dust shape approximations. Here, we present a new dust optical model constrained by measured dust shape distributions. This new dust optical model is an improvement on the current dust optical models used in models and retrieval algorithms, as quantified by comparisons against laboratory and field observations of dust optics.
Konstantinos Michailidis, Maria-Elissavet Koukouli, Dimitris Balis, J. Pepijn Veefkind, Martin de Graaf, Lucia Mona, Nikolaos Papagianopoulos, Gesolmina Pappalardo, Ioanna Tsikoudi, Vassilis Amiridis, Eleni Marinou, Anna Gialitaki, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Daniele Bortoli, Maria João Costa, Vanda Salgueiro, Alexandros Papayannis, Maria Mylonaki, Lucas Alados-Arboledas, Salvatore Romano, Maria Rita Perrone, and Holger Baars
Atmos. Chem. Phys., 23, 1919–1940, https://doi.org/10.5194/acp-23-1919-2023, https://doi.org/10.5194/acp-23-1919-2023, 2023
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Comparisons with ground-based correlative lidar measurements constitute a key component in the validation of satellite aerosol products. This paper presents the validation of the TROPOMI aerosol layer height (ALH) product, using archived quality assured ground-based data from lidar stations that belong to the EARLINET network. Comparisons between the TROPOMI ALH and co-located EARLINET measurements show good agreement over the ocean.
María Ángeles López-Cayuela, Carmen Córdoba-Jabonero, Diego Bermejo-Pantaleón, Michaël Sicard, Vanda Salgueiro, Francisco Molero, Clara Violeta Carvajal-Pérez, María José Granados-Muñoz, Adolfo Comerón, Flavio T. Couto, Rubén Barragán, María-Paz Zorzano, Juan Antonio Bravo-Aranda, Constantino Muñoz-Porcar, María João Costa, Begoña Artíñano, Alejandro Rodríguez-Gómez, Daniele Bortoli, Manuel Pujadas, Jesús Abril-Gago, Lucas Alados-Arboledas, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 23, 143–161, https://doi.org/10.5194/acp-23-143-2023, https://doi.org/10.5194/acp-23-143-2023, 2023
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An intense Saharan dust outbreak crossing the Iberian Peninsula in springtime was monitored to determinine the specific contribution of fine and coarse dust particles at five lidar stations, strategically covering its SW–central–NE pathway. Expected dust ageing along the transport started unappreciated. A different fine-dust impact on optical (~30 %) and mass (~10 %) properties was found. Use of polarized lidar measurements (mainly in elastic systems) for fine/coarse dust separation is crucial.
Kyriakoula Papachristopoulou, Ioannis-Panagiotis Raptis, Antonis Gkikas, Ilias Fountoulakis, Akriti Masoom, and Stelios Kazadzis
Atmos. Chem. Phys., 22, 15703–15727, https://doi.org/10.5194/acp-22-15703-2022, https://doi.org/10.5194/acp-22-15703-2022, 2022
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Megacities' air quality is determined by atmospheric aerosols. We focus on changes over the last two decades in the 81 largest cities, using satellite data. European and American cities have lower aerosol compared to African and Asian cities. For European, North American and East Asian cities, aerosols are decreasing over time, especially in China and the US. In the remaining cities, aerosol loads are increasing, particularly in India.
Nilton Évora do Rosário, Elisa Thomé Sena, and Marcia Akemi Yamasoe
Atmos. Chem. Phys., 22, 15021–15033, https://doi.org/10.5194/acp-22-15021-2022, https://doi.org/10.5194/acp-22-15021-2022, 2022
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The 2020 burning season in Brazil was marked by an atypically high number of fire spots across Pantanal, leading to high amounts of smoke within the biome. This study shows that smoke over Pantanal, usually a fraction of that over Amazonia, was higher and resulted mainly from fires in conservation and indigenous areas. It also contributes to highlighting Pantanal's 2020 burning season as the worst combination of a climate extreme scenario and inadequately enforced environmental regulations.
Santiago Gassó and Kirk D. Knobelspiesse
Atmos. Chem. Phys., 22, 13581–13605, https://doi.org/10.5194/acp-22-13581-2022, https://doi.org/10.5194/acp-22-13581-2022, 2022
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Atmospheric particles interact with light resulting in observable optical polarization. Thus, we can learn about their composition from space. New satellite sensor technology measures full polarization of reflected sunlight. This paper considers circular polarization, an overlooked category of polarization with distinctive features that could bring new insights. We review existing literature and make novel computations to consider this previously underappreciated category of polarization.
Qingyang Xiao, Guannan Geng, Shigan Liu, Jiajun Liu, Xia Meng, and Qiang Zhang
Atmos. Chem. Phys., 22, 13229–13242, https://doi.org/10.5194/acp-22-13229-2022, https://doi.org/10.5194/acp-22-13229-2022, 2022
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We provided complete coverage PM2.5 concentrations at a 1-km resolution from 2000 to the present, carefully considering the significant changes in land use characteristics in China. This high-resolution PM2.5 data successfully revealed the local-scale PM2.5 variations. We noticed changes in PM2.5 spatial patterns in association with the clean air policies, with the pollution hotspots having transferred from urban centers to rural regions with limited air quality monitoring.
Johannes Quaas, Hailing Jia, Chris Smith, Anna Lea Albright, Wenche Aas, Nicolas Bellouin, Olivier Boucher, Marie Doutriaux-Boucher, Piers M. Forster, Daniel Grosvenor, Stuart Jenkins, Zbigniew Klimont, Norman G. Loeb, Xiaoyan Ma, Vaishali Naik, Fabien Paulot, Philip Stier, Martin Wild, Gunnar Myhre, and Michael Schulz
Atmos. Chem. Phys., 22, 12221–12239, https://doi.org/10.5194/acp-22-12221-2022, https://doi.org/10.5194/acp-22-12221-2022, 2022
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Pollution particles cool climate and offset part of the global warming. However, they are washed out by rain and thus their effect responds quickly to changes in emissions. We show multiple datasets to demonstrate that aerosol emissions and their concentrations declined in many regions influenced by human emissions, as did the effects on clouds. Consequently, the cooling impact on the Earth energy budget became smaller. This change in trend implies a relative warming.
Ukkyo Jeong, Si-Chee Tsay, N. Christina Hsu, David M. Giles, John W. Cooper, Jaehwa Lee, Robert J. Swap, Brent N. Holben, James J. Butler, Sheng-Hsiang Wang, Somporn Chantara, Hyunkee Hong, Donghee Kim, and Jhoon Kim
Atmos. Chem. Phys., 22, 11957–11986, https://doi.org/10.5194/acp-22-11957-2022, https://doi.org/10.5194/acp-22-11957-2022, 2022
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Ultraviolet (UV) measurements from satellite and ground are important for deriving information on several atmospheric trace and aerosol characteristics. Simultaneous retrievals of aerosol and trace gases in this study suggest that water uptake by aerosols is one of the important phenomena affecting aerosol properties over northern Thailand, which is important for regional air quality and climate. Obtained aerosol properties covering the UV are also important for various satellite algorithms.
Abdulaziz Tunde Yakubu and Naven Chetty
Atmos. Chem. Phys., 22, 11065–11087, https://doi.org/10.5194/acp-22-11065-2022, https://doi.org/10.5194/acp-22-11065-2022, 2022
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This study examined the source of atmospheric aerosols and their role in forming clouds and rainfall over South Africa. The research provided answers to the cause of low precipitation, mainly linked to drought and water shortages experienced over the region. Further insight into the cause of occasional flooding that occurs in other parts of the area is provided. Finally, the study described the relationship between aerosol–cloud precipitation based on observation over the region.
África Barreto, Rosa D. García, Carmen Guirado-Fuentes, Emilio Cuevas, A. Fernando Almansa, Celia Milford, Carlos Toledano, Francisco J. Expósito, Juan P. Díaz, and Sergio F. León-Luis
Atmos. Chem. Phys., 22, 11105–11124, https://doi.org/10.5194/acp-22-11105-2022, https://doi.org/10.5194/acp-22-11105-2022, 2022
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A comprehensive characterization of atmospheric aerosols in the subtropical eastern North Atlantic has been carried out in this paper using long-term ground AERONET photometric observations over the period 2005–2020 from a unique network made up of four stations strategically located from sea level to 3555 m height on the island of Tenerife. This is a region that can be considered a key location to study the seasonal dependence of dust transport from the Sahel-Sahara.
Xiaoxi Zhao, Kan Huang, Joshua S. Fu, and Sabur F. Abdullaev
Atmos. Chem. Phys., 22, 10389–10407, https://doi.org/10.5194/acp-22-10389-2022, https://doi.org/10.5194/acp-22-10389-2022, 2022
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Long-range transport of Asian dust to the Arctic was considered an important source of Arctic air pollution. Different transport routes to the Arctic had divergent effects on the evolution of aerosol properties. Depositions of long-range-transported dust particles can reduce the Arctic surface albedo considerably. This study implied that the ubiquitous long-transport dust from China exerted considerable aerosol indirect effects on the Arctic and may have potential biogeochemical significance.
Katherine T. Junghenn Noyes, Ralph A. Kahn, James A. Limbacher, and Zhanqing Li
Atmos. Chem. Phys., 22, 10267–10290, https://doi.org/10.5194/acp-22-10267-2022, https://doi.org/10.5194/acp-22-10267-2022, 2022
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We compare retrievals of wildfire smoke particle size, shape, and light absorption from the MISR satellite instrument to modeling and other satellite data on land cover type, drought conditions, meteorology, and estimates of fire intensity (fire radiative power – FRP). We find statistically significant differences in the particle properties based on burning conditions and land cover type, and we interpret how changes in these properties point to specific aerosol aging mechanisms.
David W. Fillmore, David A. Rutan, Seiji Kato, Fred G. Rose, and Thomas E. Caldwell
Atmos. Chem. Phys., 22, 10115–10137, https://doi.org/10.5194/acp-22-10115-2022, https://doi.org/10.5194/acp-22-10115-2022, 2022
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This paper presents an evaluation of the aerosol analysis incorporated into the Clouds and the Earth's Radiant Energy System (CERES) data products as well as the aerosols' impact on solar radiation reaching the surface. CERES is a NASA Earth observation mission with instruments flying on various polar-orbiting satellites. Its primary objective is the study of the radiative energy balance of the climate system as well as examination of the influence of clouds and aerosols on this balance.
Peng Xian, Jianglong Zhang, Norm T. O'Neill, Travis D. Toth, Blake Sorenson, Peter R. Colarco, Zak Kipling, Edward J. Hyer, James R. Campbell, Jeffrey S. Reid, and Keyvan Ranjbar
Atmos. Chem. Phys., 22, 9915–9947, https://doi.org/10.5194/acp-22-9915-2022, https://doi.org/10.5194/acp-22-9915-2022, 2022
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The study provides baseline Arctic spring and summertime aerosol optical depth climatology, trend, and extreme event statistics from 2003 to 2019 using a combination of aerosol reanalyses, remote sensing, and ground observations. Biomass burning smoke has an overwhelming contribution to black carbon (an efficient climate forcer) compared to anthropogenic sources. Burning's large interannual variability and increasing summer trend have important implications for the Arctic climate.
Harshvardhan Harshvardhan, Richard Ferrare, Sharon Burton, Johnathan Hair, Chris Hostetler, David Harper, Anthony Cook, Marta Fenn, Amy Jo Scarino, Eduard Chemyakin, and Detlef Müller
Atmos. Chem. Phys., 22, 9859–9876, https://doi.org/10.5194/acp-22-9859-2022, https://doi.org/10.5194/acp-22-9859-2022, 2022
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The evolution of aerosol in biomass burning smoke plumes that travel over marine clouds off the Atlantic coast of central Africa was studied using measurements made by a lidar deployed on a high-altitude aircraft. The main finding was that the physical properties of aerosol do not change appreciably once the plume has left land and travels over the ocean over a timescale of 1 to 2 d. Almost all particles in the plume are of radius less than 1 micrometer and spherical in shape.
Peng Xian, Jianglong Zhang, Norm T. O'Neill, Jeffrey S. Reid, Travis D. Toth, Blake Sorenson, Edward J. Hyer, James R. Campbell, and Keyvan Ranjbar
Atmos. Chem. Phys., 22, 9949–9967, https://doi.org/10.5194/acp-22-9949-2022, https://doi.org/10.5194/acp-22-9949-2022, 2022
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The study provides a baseline Arctic spring and summertime aerosol optical depth climatology, trend, and extreme event statistics from 2003 to 2019 using a combination of aerosol reanalyses, remote sensing, and ground observations. Biomass burning smoke has an overwhelming contribution to black carbon (an efficient climate forcer) compared to anthropogenic sources. Burning's large interannual variability and increasing summer trend have important implications for the Arctic climate.
Cited articles
Boucher, O., Randall, D., Artaxo, P., Bretherton, C., Feingold, G., Forster, P., Kerminen, V.-M., Kondo, Y., Liao, H., Lohmann, U., Rasch, P., Satheesh, S. K., Sherwood, S., Stevens, B., and Zhang, X. Y.: Clouds and Aerosols, in: Climate Change 2013: The Physical Science Basis. Contribution of Working Group I to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Stocker, T. F., Qin, D., Plattner, G.-K., Tignor, M., Allen, S. K., Boschung, J., Nauels, A., Xia, Y., Bex, V., and Midgley, P. M., Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, 2013.
Cao, X., Wang, Z., Tian, P., Wang, J., Zhang, L., and Quan, X.: Statistics of aerosol extinction coefficient profiles and optical depth using lidar measurement over Lanzhou, China since 2005–2008, J. Quant. Spectrosc. Ra., 122, 150–154, https://doi.org/10.1016/j.jqsrt.2012.09.016, 2013.
Che, H., Zhang, X.-Y., Xia, X., Goloub, P., Holben, B., Zhao, H., Wang, Y., Zhang, X.-C., Wang, H., Blarel, L., Damiri, B., Zhang, R., Deng, X., Ma, Y., Wang, T., Geng, F., Qi, B., Zhu, J., Yu, J., Chen, Q., and Shi, G.: Ground-based aerosol climatology of China: aerosol optical depths from the China Aerosol Remote Sensing Network (CARSNET) 2002–2013, Atmos. Chem. Phys., 15, 7619–7652, https://doi.org/10.5194/acp-15-7619-2015, 2015.
Cui, Y., Lin, J., Song, C., Liu, M., Yan, Y., Xu, Y., and Huang, B.: Rapid growth in nitrogen dioxide pollution over Western China, 2005–2013, Atmos. Chem. Phys., 16, 6207–6221, https://doi.org/10.5194/acp-16-6207-2016, 2016.
Ding, A., Huang, X., Nie, W., Sun, J., Kerminen, V. M., Petäjä, T., Su, H., Cheng, Y., Yang, X., Wang, M., Chi, X., Wang, J., Virkkula, A., Guo, W., Yuan, J., Wang, S., Zhang, R., Wu, Y., Song, Y., Zhu, T., Zilitinkevich, S., Kulmala, M., and Fu, C.: Enhanced haze pollution by black carbon in megacities in China, Geophys. Res. Lett., 43, 287–2879, https://doi.org/10.1002/2016GL067745, 2016.
Eck, T. F., Holben, B. N., Dubovik, O., Smirnov, A., Goloub, P., Chen, H. B., Chatenet, B., Gomes, L., Zhang, X. Y., Tsay, S. C., Ji, Q., Giles, D., and Slutsker, I.: Columnar aerosol optical properties at AERONET sites in central eastern Asia and aerosol transport to the tropical mid-Pacific, J. Geophys. Res., 110, D06202, https://doi.org/10.1029/2004JD005274, 2005.
Fernald, F. G.: Analysis of atmospheric lidar observations: some comments, Appl. Optics, 23, 652–653, https://doi.org/10.1364/AO.23.000652, 1984.
Garrett, T. J. and Zhao, C.: Increased Arctic cloud longwave emissivity associated with pollution from mid-latitudes, Nature, 440, 787–789, https://doi.org/10.1038/nature04636, 2006.
Garrett, T. J., Zhao, C., and Novelli P. C.:, Assessing the relative contributions of transport efficiency and scavenging to seasonal variability in Arctic aerosol, Tellus B, 62, 190–196, https://doi.org/10.1111/j.1600-0889.2010.00453.x, 2010.
Ge, J. M., Huang, J. P., Xu, C. P., Qi, Y. L., and Liu, H. Y.: Characteristics of Taklimakan dust emission and distribution: A satellite and reanalysis field perspective, J. Geophys. Res., 119, 11772–11783, https://doi.org/10.1002/2014JD022280, 2014.
Ge, J. M., Liu, H., Huang, J., and Fu, Q.: Taklimakan Desert nocturnal low-level jet: climatology and dust activity, Atmos. Chem. Phys., 16, 7773–7783, https://doi.org/10.5194/acp-16-7773-2016, 2016.
Groß, S., Tesche, M., Freudenthaler, V., Toledano, C., Wiegner, M., Ansmann, A., Althausen, D., and Seefeldner, M.: Characterization of Saharan dust, marine aerosols and mixtures of biomass-burning aerosols and dust by means of multi-wavelength depolarization and Raman lidar measurements during SAMUM 2, Tellus B, 63, 706–724, https://doi.org/10.1111/j.1600-0889.2011.00556.x, 2011.
Guo, J., Liu, H., Wang, F., Huang, J., Xia, F., Lou, M., Wu, Y., Jiang, J. H., Xie, T., Zhaxi, Y., and Yung, Y. L.: Three-dimensional structure of aerosol in China: A perspective from multi-satellite observations, Atmos. Res., 178–179, 580–589, https://doi.org/10.1016/j.atmosres.2016.05.010, 2016a.
Guo, J., Miao, Y., Zhang, Y., Liu, H., Li, Z., Zhang, W., He, J., Lou, M., Yan, Y., Bian, L., and Zhai, P.: The climatology of planetary boundary layer height in China derived from radiosonde and reanalysis data, Atmos. Chem. Phys., 16, 13309–13319, https://doi.org/10.5194/acp-16-13309-2016, 2016b.
Guo, S., Hu, M., Zamora, M. L., Peng, J., Shang, D., Zheng, J., Du, Z., Wu, Z., Shao, M., Zeng, L., Molina, M. J., and Zhang, R.: Elucidating severe urban haze formation in China, P. Natl. Acad. Sci. USA, 111, 17373–17378, https://doi.org/10.1073/pnas.1419604111, 2014.
Gustafsson, Ö. and Ramanathan, V.: Convergence on climate warming by black carbon aerosols, P. Natl. Acad. Sci. USA, 113, 4243–4245, https://doi.org/10.1073/pnas.1603570113, 2016.
Hara, Y., Uno, I., Shimizu, A., Sugimoto, N., Matsui, I., Yumimoto, K., Kurokawa, J.-i., Ohara, T., and Liu, Z.: Seasonal Characteristics of Spherical Aerosol Distribution in Eastern Asia: Integrated Analysis Using Ground/Space-Based Lidars and a Chemical Transport Model, SOLA, 7, 121–124, https://doi.org/10.2151/sola.2011-031, 2011.
He, Q. S., Li, C. C., Mao, J. T., Lau, A. K. H., and Chu, D. A.: Analysis of aerosol vertical distribution and variability in Hong Kong, J. Geophys. Res., 113, D14211, https://doi.org/10.1029/2008JD009778, 2008.
Heese, B., Baars, H., Bohlmann, S., Althausen, D., and Deng, R.: Continuous vertical aerosol profiling with a multi-wavelength Raman polarization lidar over the Pearl River Delta, China, Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-733, in review, 2016.
Huang, C., Chen, C. H., Li, L., Cheng, Z., Wang, H. L., Huang, H. Y., Streets, D. G., Wang, Y. J., Zhang, G. F., and Chen, Y. R.: Emission inventory of anthropogenic air pollutants and VOC species in the Yangtze River Delta region, China, Atmos. Chem. Phys., 11, 4105–4120, https://doi.org/10.5194/acp-11-4105-2011, 2011.
Huang, J., Huang, Z., Bi, J., Zhang, W., and Zhang, L.: Micro-Pulse Lidar Measurements of Aerosol Vertical Structure over the Loess Plateau, Atmos. Oceanic Sci. Lett., 1, 8–11, https://doi.org/10.1080/16742834.2008.11446756, 2008a.
Huang, J., Zhang, W., Zuo, J., Bi, J., Shi, J., Wang, X., Chang, Z., Huang, Z., Yang, S., Zhang, B., Wang, G., Feng, G., Yuan, J., Zhang, L., Zuo, H., Wang, S., Fu, C., and Chou, J.: An overview of the Semi-arid Climate and Environment Research Observatory over the Loess Plateau, Adv. Atmos. Sci., 25, 906–921, https://doi.org/10.1007/s00376-008-0906-7, 2008b.
Huang, J. P., Liu, J. J., Chen, B., and Nasiri, S. L.: Detection of anthropogenic dust using CALIPSO lidar measurements, Atmos. Chem. Phys., 15, 11653–11665, https://doi.org/10.5194/acp-15-11653-2015, 2015.
Huang, Z., Huang, J., Bi, J., Wang, G., Wang, W., Fu, Q., Li, Z., Tsay, S.-C., and Shi, J.: Dust aerosol vertical structure measurements using three MPL lidars during 2008 China-U.S. joint dust field experiment, J. Geophys. Res., 115, D00K15, https://doi.org/10.1029/2009JD013273, 2010.
Huang, Z., Huang, J., Hayasaka, T., Wang, S., Zhou, T., and Jin, H.: Short-cut transport path for Asian dust directly to the Arctic: a case study, Environ. Res. Lett., 10, 114018, https://doi.org/10.1088/1748-9326/10/11/114018, 2015.
Huneeus, N., Schulz, M., Balkanski, Y., Griesfeller, J., Prospero, J., Kinne, S., Bauer, S., Boucher, O., Chin, M., Dentener, F., Diehl, T., Easter, R., Fillmore, D., Ghan, S., Ginoux, P., Grini, A., Horowitz, L., Koch, D., Krol, M. C., Landing, W., Liu, X., Mahowald, N., Miller, R., Morcrette, J.-J., Myhre, G., Penner, J., Perlwitz, J., Stier, P., Takemura, T., and Zender, C. S.: Global dust model intercomparison in AeroCom phase I, Atmos. Chem. Phys., 11, 7781–7816, https://doi.org/10.5194/acp-11-7781-2011, 2011.
Jia, R., Liu, Y. Z., Chen, B., Zhang, Z. J., and Huang, J. P.: Source and transportation of summer dust over the Tibetan Plateau, Atmos. Environ., 123, 210–219, https://doi.org/10.1016/j.atmosenv.2015.10.038, 2015.
Kandler, K., Lieke, K., Benker, N., Emmel, C., Kupper, M., Muller-Ebert, D., Ebert, M., Scheuvens, D., Schladitz, A., Schutz, L., and Weinbruch, S.: Electron microscopy of particles collected at Praia, Cape Verde, during the Saharan Mineral Dust Experiment: particle chemistry, shape, mixing state and complex refractive index, Tellus B, 63, 475–496, https://doi.org/10.1111/j.1600-0889.2011.00550.x, 2011.
Khalizov, A. F., Xue, H., and Zhang, R.: Enhanced light absorption and scattering by carbon soot aerosols internally mixed with sulfuric acid, J. Phys. Chem. 113, 1066–1074, https://doi.org/10.1021/jp807531n, 2009.
Kipling, Z., Stier, P., Johnson, C. E., Mann, G. W., Bellouin, N., Bauer, S. E., Bergman, T., Chin, M., Diehl, T., Ghan, S. J., Iversen, T., Kirkevåg, A., Kokkola, H., Liu, X., Luo, G., van Noije, T., Pringle, K. J., von Salzen, K., Schulz, M., Seland, Ø., Skeie, R. B., Takemura, T., Tsigaridis, K., and Zhang, K.: What controls the vertical distribution of aerosol? Relationships between process sensitivity in HadGEM3–UKCA and inter-model variation from AeroCom Phase II, Atmos. Chem. Phys., 16, 2221–2241, https://doi.org/10.5194/acp-16-2221-2016, 2016.
Koffi, B., Schulz, M., Bréon, F.-M., Griesfeller, J., Winker, D., Balkanski, Y., Bauer, S., Berntsen, T., Chin, M., Collins, W. D., Dentener, F., Diehl, T., Easter, R., Ghan, S., Ginoux, P., Gong, S., Horowitz, L. W., Iversen, T., Kirkevåg, A., Koch, D., Krol, M., Myhre, G., Stier, P., and Takemura, T.: Application of the CALIOP layer product to evaluate the vertical distribution of aerosols estimated by global models: AeroCom phase I results, J. Geophys. Res., 117, D10201, https://doi.org/10.1029/2011JD016858, 2012.
Lei, W., Derecskei-Kovacs, A., and Zhang, R.: Ab initio study of OH addition reaction to isoprene, J. Chem. Phys., 113, 5354–5360, https://doi.org/10.1063/1.1290020, 2000.
Li, G., Wang, Y., and Zhang, R.: Implementation of a two-moment bulk microphysics scheme to the WRF model to investigate aerosol-cloud interaction, J. Geophys. Res., 113, D15211, https://doi.org/10.1029/2007JD009361, 2008.
Li, J., Carlson, B. E., and Lacis, A. A.: Using single-scattering albedo spectral curvature to characterize East Asian aerosol mixtures, J. Geophys. Res., 120, 2037–2052, https://doi.org/10.1002/2014JD022433, 2015.
Li, Z., Chen, H., Cribb, M., Dickerson, R., Holben, B., Li, C., Lu, D., Luo, Y., Maring, H., Shi, G., Tsay, S. C., Wang, P., Wang, Y., Xia, X., Zheng, Y., Yuan, T., and Zhao, F.: Preface to special section on East Asian Studies of Tropospheric Aerosols: An International Regional Experiment (EAST-AIRE), J. Geophys. Res., 112, D22S00, https://doi.org/10.1029/2007JD008853, 2007.
Li, Z., Niu, F., Fan, J., Liu, Y., Rosenfeld, D., and Ding, Y.: Long-term impacts of aerosols on the vertical development of clouds and precipitation, Nat. Geosci., 4, 888–894, https://doi.org/10.1038/ngeo1313, 2011.
Liu, C., Shen, X., Gao, W., Liu, P., and Sun, Z.: Evaluation of CALIPSO aerosol optical depth using AERONET and MODIS data over China, In SPIE Optical Engineering Applications 2014 Oct 2 (92210F-92210F), International Society for Optics and Photonics, https://doi.org/10.1117/12.2058929, 2014.
Liu, X. H., Zhang, Y., Xing, J., Zhang, Q. A., Wang, K., Streets, D. G., Jang, C., Wang, W. X., and Hao, J. M.: Understanding of regional air pollution over China using CMAQ, part II. Process analysis and sensitivity of ozone and particulate matter to precursor emissions, Atmos. Environ., 44, 3719–3727, https://doi.org/10.1016/j.atmosenv.2010.03.036, 2010.
Liu, Z., Liu, D., Huang, J., Vaughan, M., Uno, I., Sugimoto, N., Kittaka, C., Trepte, C., Wang, Z., Hostetler, C., and Winker, D.: Airborne dust distributions over the Tibetan Plateau and surrounding areas derived from the first year of CALIPSO lidar observations, Atmos. Chem. Phys., 8, 5045–5060, https://doi.org/10.5194/acp-8-5045-2008, 2008.
Logan, T., Xi, B., Dong, X., Obrecht, R., Li, Z., and Cribb, M.: A study of Asian dust plumes using satellite, surface, and aircraft measurements during the INTEX-B field experiment, J. Geophys. Res., 115, D00K25, https://doi.org/10.1029/2010JD014134, 2010.
Logan, T., Xi, B., Dong, X., Li, Z., and Cribb, M.: Classification and investigation of Asian aerosol absorptive properties, Atmos. Chem. Phys., 13, 2253–2265, https://doi.org/10.5194/acp-13-2253-2013, 2013.
Luo, Y. X., Zheng, X. B., Zhao, T. L., and Chen, J.: A climatology of aerosol optical depth over China from recent 10 years of MODIS remote sensing data, Int. J. Climatol. 34, 863–870, https://doi.org/10.1002/joc.3728, 2014.
Ma, Z. W., Hu, X. F., Sayer, A. M., Levy, R., Zhang, Q., Xue, Y. G., Tong, S. L., Bi, J., Huang, L., and Liu, Y.: Satellite-Based Spatiotemporal Trends in PM2.5 Concentrations: China, 2004–2013, Environ. Health Persp., 124, 184–192, https://doi.org/10.1289/ehp.1409481, 2016.
Miao, Y., Hu, X.-M., Liu, S., Qian, T., Xue, M., Zheng, Y., and Wang, S.: Seasonal variation of local atmospheric circulations and boundary layer structure in the Beijing-Tianjin-Hebei region and implications for air quality, J. Adv. Model Earth Sy., 7, 1602–1626, https://doi.org/10.1002/2015MS000522, 2015.
Mielonen, T., Arola, A., Komppula, M., Kukkonen, J., Koskinen, J., de Leeuw, G., and Lehtinen, K.: Comparison of CALIOP level 2 aerosol subtypes to aerosol types derived from AERONET inversion data, Geophys. Res. Lett., 36, L18804, https://doi.org/10.1029/2009GL039609, 2009.
Nemuc, A., Vasilescu, J., Talianu, C., Belegante, L., and Nicolae, D.: Assessment of aerosol's mass concentrations from measured linear particle depolarization ratio (vertically resolved) and simulations, Atmos. Meas. Tech., 6, 3243–3255, https://doi.org/10.5194/amt-6-3243-2013, 2013.
Nesbitt, S. W., Zhang, R., and Orville, R. E.: Seasonal and global NOx production by lightning estimated from the Optical Transient Detector (OTD), Tellus B, 52, 1206–1215, https://doi.org/10.1034/j.1600-0889.2000.01121.x, 2000.
Omar, A. H., Won, J.-G., Winker, D. M., Yoon, S.-C., Dubovik, O., and McCormick, M. P.: Development of global aerosol models using cluster analysis of Aerosol Robotic Network (AERONET) measurements, J. Geophys. Res., 110, D10S14, https://doi.org/10.1029/2004JD004874, 2005.
Omar, A. H., Winker, D. M., Vaughan, M. A., Hu, Y., Trepte, C. R., Ferrare, R. A., Lee, K.-P., Hostetler, C. A., Kittaka, C., Rogers, R. R., Kuehn, R. E., and Liu, Z.: The CALIPSO Automated Aerosol Classification and Lidar Ratio Selection Algorithm, J. Atmos. Ocean. Tech., 26, 1994–2014, https://doi.org/10.1175/2009JTECHA1231.1, 2009.
Pan, X., Uno, I., Hara, Y., Kuribayashi, M., Kobayashi, H., Sugimoto, N., Yamamoto, S., Shimohara, T., and Wang, Z.: Observation of the simultaneous transport of Asian mineral dust aerosols with anthropogenic pollutants using a POPC during a long-lasting dust event in late spring 2014, Geophys. Res. Lett., 42, 1593–1598, https://doi.org/10.1002/2014GL062491, 2015.
Papagiannopoulos, N., Mona, L., Alados-Arboledas, L., Amiridis, V., Baars, H., Binietoglou, I., Bortoli, D., D'Amico, G., Giunta, A., Guerrero-Rascado, J. L., Schwarz, A., Pereira, S., Spinelli, N., Wandinger, U., Wang, X., and Pappalardo, G.: CALIPSO climatological products: evaluation and suggestions from EARLINET, Atmos. Chem. Phys., 16, 2341–2357, https://doi.org/10.5194/acp-16-2341-2016, 2016.
Peng, J., Hu, M., Guo, S., Du, Z., Zheng, J., Shang, D., Levy Zamora, M., Zeng, L., Shao, M., Wu, Y.-S., Zheng, J., Wang, Y., Glen, C. R., Collins, D. R., Molina, M. J., and Zhang, R.: Markedly enhanced absorption and direct radiative forcing of black carbon under polluted urban environments, P. Natl. Acad. Sci. USA, 113, 4266–4271, https://doi.org/10.1073/pnas.1602310113, 2016.
Petäjä, T., Järvi, L., Kerminen, V. M., Ding, A. J., Sun, J. N., Nie, W., Kujansuu, J., Virkkula, A., Yang, X., and Fu, C. B., Zilitinkevich, S., and Kulmala, M.: Enhanced air pollution via aerosol-boundary layer feedback in China, Sci. Rep., 6, 18998, https://doi.org/10.1038/srep18998, 2016.
Porter, J. N. and Clarke, A. D.: Aerosol size distribution models based on in situ measurements, J. Geophys. Res., 102, 6035–6045, https://doi.org/10.1029/96JD03403, 1997.
Qi, Y., Ge, J., and Huang, J.: Spatial and temporal distribution of MODIS and MISR aerosol optical depth over northern China and comparison with AERONET, Chinese Sci. Bull., 58, 2497–2506, https://doi.org/10.1007/s11434-013-5678-5, 2013.
Qiu, C. and Zhang, R.: Multiphase chemistry of atmospheric amines, Phys. Chem. Chem. Phys., 15, 5738–5752, https://doi.org/10.1039/C3CP43446J, 2013.
Qiu, Q., Wang, L., Lal, V., Khalizov, A. F., and Zhang, R.: Heterogeneous chemistry of alkylamines on ammonium sulfate and ammonium bisulfate, Environ. Sci. Technol., 45, 4748–4755, https://doi.org/10.1021/es1043112, 2011.
Rosenfeld, D., Sherwood, S., Wood, R., and Donner, L.: Climate Effects of Aerosol-Cloud Interactions, Science, 343, 379–380, https://doi.org/10.1126/science.1247490, 2014.
Sasano, Y. and Browell, E. V.: Light scattering characteristics of various aerosol types derived from multiple wavelength lidar observations, Appl. Optics, 28, 1670–1679, https://doi.org/10.1364/AO.28.001670, 1989.
Schleicher, N., Norra, S., Fricker, M., Kaminski, U., Chen, Y., Chai, F., Wang, S., Yu, Y., and Cen, K.: Spatio-temporal variations of black carbon concentrations in the Megacity Beijing, Environ. Pollut., 182, 392–401, https://doi.org/10.1016/j.envpol.2013.07.042, 2013.
Su, X., Cao, J., Li, Z., Lin, M., and Wang, G.: Column-Integrated Aerosol Optical Properties during Summer and Autumn of 2012 in Xi'an, China, Aerosol Air Qual. Res., 14, 850–861, https://doi.org/10.4209/aaqr.2013.03.0093, 2014.
Sugimoto, N. and Huang, Z.: Lidar methods for observing mineral dust, J. Meteor. Res., 28, 173–184, https://doi.org/10.1007/s13351-014-3068-9, 2014.
Sugimoto, N., Matsui, I., Shimizu, A., Uno, I., Asai, K., Endoh, T., and Nakajima, T.: Observation of dust and anthropogenic aerosol plumes in the Northwest Pacific with a two-wavelength polarization lidar on board the research vessel Mirai, Geophys. Res. Lett., 29, 1901, https://doi.org/10.1029/2002GL015112, 2002.
Suh, I., Zhang, R., Molina, L. T., and Molina, M. J.: Oxidation Mechanism of Aromatic Peroxy and Bicyclic Radicals from OH−Toluene Reactions, J. Am. Chem. Soc., 125, 12655–12665, https://doi.org/10.1021/ja0350280, 2003.
Takamura, T., Sasano, Y., and Hayasaka, T.: Tropospheric aerosol optical properties derived from lidar, sun photometer, and optical particle counter measurements, Appl. Optics, 33, 7132–7140, https://doi.org/10.1364/AO.33.007132, 1994.
Tao, M., Chen, L., Wang, Z., Tao, J., Che, H., Wang, X., and Wang, Y.: Comparison and evaluation of the MODIS Collection 6 aerosol data in China, J. Geophys. Res., 120, 6992–7005, https://doi.org/10.1002/2015JD023360, 2015.
Tian, P., Cao, X., Liang, J., Zhang, L., Yi, N., Wang, L., and Cheng, X.: Improved empirical mode decomposition based denoising method for lidar signals, Opt. Commun., 325, 54–59, https://doi.org/10.1016/j.optcom.2014.03.083, 2014.
Wang, G., Zhang, R., Gomez, M. E., Yang, L., Zamora, M. L., Hu, M., Lin, Y., Peng, J., Guo, S., Meng, J., Li, J., Cheng, C., Hu, T., Ren, Y., Wang, Y., Gao, J., Cao, J., An, Z., Zhou, W., Li, G., Wang, J., Tian, P., Marrero-Ortiz, W., Secrest, J., Du, Z., Zheng, J., Shang, D., Zeng, L., Shao, M., Wang, W., Huang, Y., Wang, Y., Zhu, Y., Li, Y., Hu, J., Pan, B., Cai, L., Cheng, Y., Ji, Y., Zhang, F., Rosenfeld, D., Liss, P. S., Duce, R. A., Kolb, C. E., Molina, M. J.: Persistent sulfate formation from London Fog to Chinese Haze, P. Natl. Acad. Sci. USA, 113, 13630–13635, doi/10.1073/pnas.1616540113, 2016.
Wang, H., Zhang, L., Cao, X., Zhang, Z., and Liang, J.: A-Train satellite measurements of dust aerosol distributions over northern China, J. Quant. Spectrosc. Ra., 122, 170–179, https://doi.org/10.1016/j.jqsrt.2012.08.011, 2013.
Wang, S., Zhang, Q., Martin, R. V., Philip, S., Liu, F., Li, M., Jiang, X., and He, K.: Satellite measurements oversee China's sulfur dioxide emission reductions from coal-fired power plants, Environ. Res. Lett., 10, 114015, https://doi.org/10.1088/1748-9326/10/11/114015, 2015.
Wang, Y., Wan, Q., Meng, W., Liao, F., Tan, H., and Zhang, R.: Long-term impacts of aerosols on precipitation and lightning over the Pearl River Delta megacity area in China, Atmos. Chem. Phys., 11, 12421–12436, https://doi.org/10.5194/acp-11-12421-2011, 2011.
Wang, Y., Khalizov, A., Levy, M., and Zhang, R.: New Directions: Light absorbing aerosols and their atmospheric impacts, Atmos. Environ., 81, 713–715, https://doi.org/10.1016/j.atmosenv.2013.09.034, 2013.
Wang, Y., Zhang, R. Y., and Saravanan, R.: Asian pollution climatically modulates mid-latitude cyclones following hierarchical modelling and observational analysis, Nat. Commun., 5, 3098, https://doi.org/10.1038/ncomms4098, 2014.
Winker, D. M., Vaughan, M. A., Omar, A., Hu, Y. X., Powell, K. A., Liu, Z. Y., Hunt, W. H., and Young, S. A.: Overview of the CALIPSO Mission and CALIOP Data Processing Algorithms, J. Atmos. Ocean. Tech., 26, 2310–2323, https://doi.org/10.1175/2009JTECHA1281.1, 2009.
Winker, D. M., Tackett, J. L., Getzewich, B. J., Liu, Z., Vaughan, M. A., and Rogers, R. R.: The global 3-D distribution of tropospheric aerosols as characterized by CALIOP, Atmos. Chem. Phys., 13, 3345–3361, https://doi.org/10.5194/acp-13-3345-2013, 2013.
Wu, D., Zhou, J., Liu, D., Wang, Z., Zhong, Z., Xie, C., Qi, F., Fan, A., and Wang, Y.: 12-year lidar Observations of Tropospheric Aerosol over Hefei (31.9° N, 117.2° E), China, J. Opt. Soc. Korea, 15, 90–95, https://doi.org/10.3807/JOSK.2011.15.1.090, 2011.
Wu, G., Li, Z., Fu, C., Zhang, X., Zhang, R., Zhang, R., Zhou, T., Li, J., Li, J., Zhou, D., Wu, L., Zhou, L., He, B., and Huang, R.: Advances in studying interactions between aerosols and monsoon in China, Sci. China Earth Sci., 59, 1–16, https://doi.org/10.1007/s11430-015-5198-z, 2016.
Wu, M., Wu, D., Fan, Q., Wang, B. M., Li, H. W., and Fan, S. J.: Observational studies of the meteorological characteristics associated with poor air quality over the Pearl River Delta in China, Atmos. Chem. Phys., 13, 10755–10766, https://doi.org/10.5194/acp-13-10755-2013, 2013.
Xie, C. B., Nishizawa, T., Sugimoto, N., Matsui, I., and Wang, Z. F.: Characteristics of aerosol optical properties in pollution and Asian dust episodes over Beijing, China, Appl. Optics, 47, 4945–4951, https://doi.org/10.1364/AO.47.004945, 2008.
Xie, S., Liu, X., Zhao, C., and Zhang, Y.: Sensitivity of CAM5-Simulated Arctic Clouds and Radiation to Ice Nucleation Parameterization, J. Climate, 26, 5981–5999, https://doi.org/10.1175/jcli-d-12-00517.1, 2013.
Xin, J., Wang, Y., Pan, Y., Ji, D., Liu, Z., Wen, T., Wang, Y., Li, X., Sun, Y., Sun, J., Wang, P., Wang, G., Wang, X., Cong, Z., Song, T., Hu, B., Wang, L., Tang, G., Gao, W., Guo, Y., Miao, H., Tian, S., and Wang, L.: The Campaign on Atmospheric Aerosol Research Network of China: CARE-China, B. Am. Meteorol. Soc., 96, 1137–1155, https://doi.org/10.1175/BAMS-D-14-00039.1, 2015.
Xu, Z., Xue, L. K., Wang, T., Xia, T., Gao, Y., Louie, P. K. K., and Luk, C. W. Y.: Measurements of Peroxyacetyl Nitrate at a Background Site in the Pearl River Delta Region: Production Efficiency and Regional Transport, Aerosol Air Qual. Res., 15, 833–841, https://doi.org/10.4209/aaqr.2014.11.0275, 2015.
Yang, X., Zhao, C., Guo, J., and Wang, Y.: Intensification of aerosol pollution associated with its feedback with surface solar radiation and winds in Beijing, J. Geophys. Res., 121, 4093–4099, https://doi.org/10.1002/2015JD024645, 2016.
Yu, H., Chin, M., Winker, D. M., Omar, A. H., Liu, Z., Kittaka, C., and Diehl, T.: Global view of aerosol vertical distributions from CALIPSO lidar measurements and GOCART simulations: Regional and seasonal variations, J. Geophys. Res., 115, D00H30, https://doi.org/10.1029/2009JD013364, 2010.
Yue, D. L., Hu, M., Zhang, R. Y., Wang, Z. B., Zheng, J., Wu, Z. J., Wiedensohler, A., He, L. Y., Huang, X. F., and Zhu, T.: The roles of sulfuric acid in new particle formation and growth in the mega-city of Beijing, Atmos. Chem. Phys., 10, 4953–4960, https://doi.org/10.5194/acp-10-4953-2010, 2010.
Zhao, C. and Garrett T. J.: Effects of Arctic haze on surface cloud radiative forcing, Geophys. Res. Lett., 42, 557–564, https://doi.org/10.1002/2014GL062015, 2015.
Zhang, D. and Zhang, R.: Laboratory Investigation of Heterogeneous Interaction of Sulfuric Acid with Soot, Environ. Sci. Technol., 39, 5722–5728, https://doi.org/10.1021/es050372d, 2005.
Zhang, D., Zhang, R., Park, J., and North, S. W.: Hydroxy Peroxy Nitrites and Nitrates from OH Initiated Reactions of Isoprene, J. Am. Chem. Soc., 124, 9600–9605, https://doi.org/10.1021/ja0255195, 2002.
Zhang, H., Hu, D., Chen, J., Ye, X., Wang, S., Hao, J. M., Wang, L., Zhang, R., and An, Z.: Particle size distribution and polycyclic aromatic hydrocarbons emissions from agricultural crop residue burning, Environ. Sci. Technol., 45, 5477–5482, https://doi.org/10.1021/es1037904, 2011.
Zhang, R., Leu, M. T., and Keyser, L. F.: Heterogeneous chemistry of HONO on liquid sulfuric acid: A new mechanism of chlorine activation on stratospheric sulfate aerosols, J. Phys. Chem., 100, 339–345, https://doi.org/10.1021/jp952060a, 1996.
Zhang, R., Li, G., Fan, J., Wu, D. L., and Molina, M. J.: Intensification of Pacific storm track linked to Asian pollution, P. Natl. Acad. Sci. USA, 104, 5295–5299, https://doi.org/10.1073/pnas.0700618104, 2007.
Zhang, R., Khalizov, A. F., Pagels, J., Zhang, D., Xue, H., and McMurry, P. H.: Variability in morphology, hygroscopicity, and optical properties of soot aerosols during atmospheric processing, P. Natl. Acad. Sci. USA, 105, 10291–10296, https://doi.org/10.1073/pnas.0804860105, 2008.
Zhang, R., Wang, G. H., Guo, S., Zarnora, M. L., Ying, Q., Lin, Y., Wang, W. G., Hu, M., and Wang, Y.: Formation of Urban Fine Particulate Matter, Chem. Rev., 115, 3803–3855, https://doi.org/10.1021/acs.chemrev.5b00067, 2015.
Zhang, X. Y., Wang, Y. Q., Niu, T., Zhang, X. C., Gong, S. L., Zhang, Y. M., and Sun, J. Y.: Atmospheric aerosol compositions in China: spatial/temporal variability, chemical signature, regional haze distribution and comparisons with global aerosols, Atmos. Chem. Phys., 12, 779–799, https://doi.org/10.5194/acp-12-779-2012, 2012.
Zhang, Y. and Cao, F.: Fine particulate matter (PM2.5) in China at a city level, Sci. Rep., 5, 14884, https://doi.org/10.1038/srep14884, 2015.
Zhao, J., Levitt, N. P., Zhang, R., and Chen, J.: Heterogeneous Reactions of Methylglyoxal in Acidic Media:? Implications for Secondary Organic Aerosol Formation, Environ. Sci. Technol., 40, 7682–7687, https://doi.org/10.1021/es060610k, 2006.
Zhou, T., Huang, J., Huang, Z., Liu, J., Wang, W., and Lin, L.: The depolarization–attenuated backscatter relationship for dust plumes, Opt. Express, 21, 15195–15204, https://doi.org/10.1364/OE.21.015195, 2013.
Short summary
We have investigated the vertical distribution and optical properties of aerosols over China using long-term satellite observations from the Cloud–Aerosol Lidar with Orthogonal Polarization, ground-based lidar observations and Aerosol Robotic Network data. Our results provide key information on the long-term aerosol seasonal and spatial variations, optical properties, regional types, long-range transport and atmospheric stability in China for air quality and climate studies.
We have investigated the vertical distribution and optical properties of aerosols over China...
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