Articles | Volume 12, issue 1
https://doi.org/10.5194/acp-12-591-2012
© Author(s) 2012. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Special issue:
https://doi.org/10.5194/acp-12-591-2012
© Author(s) 2012. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
11 Jan 2012
Research article |
| 11 Jan 2012
Gas-particle partitioning of atmospheric Hg(II) and its effect on global mercury deposition
H. M. Amos
Department of Earth and Planetary Sciences, Harvard University, Cambridge, MA, USA
D. J. Jacob
Department of Earth and Planetary Sciences, Harvard University, Cambridge, MA, USA
School of Engineering and Applied Sciences, Harvard University, Boston, MA, USA
C. D. Holmes
Department of Earth System Science, University of California, Irvine, CA, USA
J. A. Fisher
Department of Earth and Planetary Sciences, Harvard University, Cambridge, MA, USA
Q. Wang
School of Engineering and Applied Sciences, Harvard University, Boston, MA, USA
R. M. Yantosca
School of Engineering and Applied Sciences, Harvard University, Boston, MA, USA
E. S. Corbitt
Department of Earth and Planetary Sciences, Harvard University, Cambridge, MA, USA
E. Galarneau
Air Quality Research Division, Environment Canada, Toronto, Ont., Canada
A. P. Rutter
Civil and Environmental Engineering Department, Rice University, Houston, TX, USA
M. S. Gustin
Department of Natural Resources and Environmental Sciences, University of Nevada, Reno, NV, USA
A. Steffen
Air Quality Research Division, Environment Canada, Toronto, Ont., Canada
J. J. Schauer
Department of Civil and Environmental Engineering, University of Wisconsin, Madison, WI, USA
J. A. Graydon
Department of Biological Sciences, University of Alberta, Edmonton, Alberta, Canada
V. L. St. Louis
Department of Biological Sciences, University of Alberta, Edmonton, Alberta, Canada
R. W. Talbot
Department of Earth and Atmospheric Sciences, University of Houston, Houston, TX, USA
E. S. Edgerton
Atmospheric Research & Analysis, Inc., Cary, NC, USA
Y. Zhang
Department of Atmospheric Sciences, University of Washington, Seattle, USA
E. M. Sunderland
School of Engineering and Applied Sciences, Harvard University, Boston, MA, USA
Department of Environmental Health, Harvard University, Boston, MA, USA
Related subject area
Subject: Gases | Research Activity: Atmospheric Modelling | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Impacts of urbanization on air quality and the related health risks in a city with complex terrain
Optimizing 4 years of CO2 biospheric fluxes from OCO-2 and in situ data in TM5: fire emissions from GFED and inferred from MOPITT CO data
Development and application of a multi-scale modeling framework for urban high-resolution NO2 pollution mapping
Towards monitoring the CO2 source–sink distribution over India via inverse modelling: quantifying the fine-scale spatiotemporal variability in the atmospheric CO2 mole fraction
Evaluation of simulated CO2 power plant plumes from six high-resolution atmospheric transport models
Methane emissions from China: a high-resolution inversion of TROPOMI satellite observations
Estimated regional CO2 flux and uncertainty based on an ensemble of atmospheric CO2 inversions
Technical note: The CAMS greenhouse gas reanalysis from 2003 to 2020
Assessing the representativity of NH3 measurements influenced by boundary-layer dynamics and the turbulent dispersion of a nearby emission source
Analysis of CO2, CH4, and CO surface and column concentrations observed at Réunion Island by assessing WRF-Chem simulations
Technical note: Interpretation of field observations of point-source methane plume using observation-driven large-eddy simulations
Quantifying fossil fuel methane emissions using observations of atmospheric ethane and an uncertain emission ratio
The impact of peripheral circulation characteristics of typhoon on sustained ozone episodes over the Pearl River Delta region, China
Updated Global Fuel Exploitation Inventory (GFEI) for methane emissions from the oil, gas, and coal sectors: evaluation with inversions of atmospheric methane observations
High-resolution mapping of regional traffic emissions using land-use machine learning models
Land use and anthropogenic heat modulate ozone by meteorology: a perspective from the Yangtze River Delta region
Four years of global carbon cycle observed from the Orbiting Carbon Observatory 2 (OCO-2) version 9 and in situ data and comparison to OCO-2 version 7
Data assimilation of CrIS NH3 satellite observations for improving spatiotemporal NH3 distributions in LOTOS-EUROS
On the cross-tropopause transport of water by tropical convective overshoots: a mesoscale modelling study constrained by in situ observations during the TRO-Pico field campaign in Brazil
Effects of ozone–vegetation interactions on meteorology and air quality in China using a two-way coupled land–atmosphere model
The drivers and health risks of unexpected surface ozone enhancements over the Sichuan Basin, China, in 2020
Estimating 2010–2015 anthropogenic and natural methane emissions in Canada using ECCC surface and GOSAT satellite observations
Technical note: AQMEII4 Activity 1: evaluation of wet and dry deposition schemes as an integral part of regional-scale air quality models
Evaluating the impact of storage-and-release on aircraft-based mass-balance methodology using a regional air-quality model
The regional impact of urban emissions on air quality in Europe: the role of the urban canopy effects
A new inverse modeling approach for emission sources based on the DDM-3D and 3DVAR techniques: an application to air quality forecasts in the Beijing–Tianjin–Hebei region
Assessing urban methane emissions using column-observing portable Fourier transform infrared (FTIR) spectrometers and a novel Bayesian inversion framework
Evidence of a recent decline in UK emissions of hydrofluorocarbons determined by the InTEM inverse model and atmospheric measurements
Vehicle-induced turbulence and atmospheric pollution
A comparative study to reveal the influence of typhoons on the transport, production and accumulation of O3 in the Pearl River Delta, China
Sensitivity to the sources of uncertainties in the modeling of atmospheric CO2 concentration within and in the vicinity of Paris
Estimating Upper Silesian coal mine methane emissions from airborne in situ observations and dispersion modeling
Analysis of CO2 spatio-temporal variations in China using a weather–biosphere online coupled model
Mobile monitoring of urban air quality at high spatial resolution by low-cost sensors: impacts of COVID-19 pandemic lockdown
Linking global terrestrial CO2 fluxes and environmental drivers: inferences from the Orbiting Carbon Observatory 2 satellite and terrestrial biospheric models
Uncertainties in the Emissions Database for Global Atmospheric Research (EDGAR) emission inventory of greenhouse gases
Using TROPOspheric Monitoring Instrument (TROPOMI) measurements and Weather Research and Forecasting (WRF) CO modelling to understand the contribution of meteorology and emissions to an extreme air pollution event in India
Global methane budget and trend, 2010–2017: complementarity of inverse analyses using in situ (GLOBALVIEWplus CH4 ObsPack) and satellite (GOSAT) observations
COVID-19 lockdowns highlight a risk of increasing ozone pollution in European urban areas
Large-eddy simulation of traffic-related air pollution at a very high resolution in a mega-city: evaluation against mobile sensors and insights for influencing factors
Technical note: Emission mapping of key sectors in Ho Chi Minh City, Vietnam, using satellite-derived urban land use data
Impact of western Pacific subtropical high on ozone pollution over eastern China
High-resolution hybrid inversion of IASI ammonia columns to constrain US ammonia emissions using the CMAQ adjoint model
Simulation of radon-222 with the GEOS-Chem global model: emissions, seasonality, and convective transport
Regional CO2 fluxes from 2010 to 2015 inferred from GOSAT XCO2 retrievals using a new version of the Global Carbon Assimilation System
The friagem event in the central Amazon and its influence on micrometeorological variables and atmospheric chemistry
Modeling atmospheric ammonia using agricultural emissions with improved spatial variability and temporal dynamics
Quantifying methane emissions from Queensland's coal seam gas producing Surat Basin using inventory data and a regional Bayesian inversion
Errors in top-down estimates of emissions using a known source
The impact of urban land-surface on extreme air pollution over central Europe
Chenchao Zhan, Min Xie, Hua Lu, Bojun Liu, Zheng Wu, Tijian Wang, Bingliang Zhuang, Mengmeng Li, and Shu Li
Atmos. Chem. Phys., 23, 771–788, https://doi.org/10.5194/acp-23-771-2023, https://doi.org/10.5194/acp-23-771-2023, 2023
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With the development of urbanization, urban land use and anthropogenic
emissions increase, affecting urban air quality and, in turn, the health risks associated with air pollutants. In this study, we systematically evaluate the impacts of urbanization on air quality and the corresponding health risks in a highly urbanized city with severe air pollution and complex terrain. This work focuses on the health risks caused by urbanization and can provide valuable insight for air pollution strategies.
Hélène Peiro, Sean Crowell, and Berrien Moore III
Atmos. Chem. Phys., 22, 15817–15849, https://doi.org/10.5194/acp-22-15817-2022, https://doi.org/10.5194/acp-22-15817-2022, 2022
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CO data can provide a powerful constraint on fire fluxes, supporting more accurate estimation of biospheric CO2 fluxes. We converted CO fire flux into CO2 fire prior, which is then used to adjust CO2 respiration. We applied this to two other fire flux products. CO2 inversions constrained by satellites or in situ data are then performed. Results show larger variations among the data assimilated than across the priors, but tropical flux from in situ inversions is sensitive to priors.
Zhaofeng Lv, Zhenyu Luo, Fanyuan Deng, Xiaotong Wang, Junchao Zhao, Lucheng Xu, Tingkun He, Yingzhi Zhang, Huan Liu, and Kebin He
Atmos. Chem. Phys., 22, 15685–15702, https://doi.org/10.5194/acp-22-15685-2022, https://doi.org/10.5194/acp-22-15685-2022, 2022
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This study developed a hybrid model, CMAQ-RLINE_URBAN, to predict the urban NO2 concentrations at a high spatial resolution. To estimate the influence of various street canyons on the dispersion of air pollutants, a new parameterization scheme was established based on computational fluid dynamics and machine learning methods. This work created a new method to identify the characteristics of vehicle-related air pollution at both city and street scales simultaneously and accurately.
Vishnu Thilakan, Dhanyalekshmi Pillai, Christoph Gerbig, Michal Galkowski, Aparnna Ravi, and Thara Anna Mathew
Atmos. Chem. Phys., 22, 15287–15312, https://doi.org/10.5194/acp-22-15287-2022, https://doi.org/10.5194/acp-22-15287-2022, 2022
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This paper demonstrates how we can use atmospheric observations to improve the CO2 flux estimates in India. This is achieved by improving the representation of terrain, mesoscale transport, and flux variations. We quantify the impact of the unresolved variations in the current models on optimally estimated fluxes via inverse modelling and quantify the associated flux uncertainty. We illustrate how a parameterization scheme captures this variability in the coarse models.
Dominik Brunnner, Gerrit Kuhlmann, Stephan Henne, Erik Koene, Bastian Kern, Sebastian Wolff, Christiane Voigt, Patrick Jöckel, Christoph Kiemle, Anke Roiger, Alina Fiehn, Sven Krautwurst, Konstantin Gerilowski, Heinrich Bovensmann, Jakob Borchardt, Michal Galkowski, Christoph Gerbig, Julia Marshall, Andrzej Klonecki, Pascal Prunet, Robert Hanfland, Margit Pattantyús-Ábrahám, Andrzej Wyszogrodzki, and Andreas Fix
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-645, https://doi.org/10.5194/acp-2022-645, 2022
Revised manuscript accepted for ACP
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Six atmospheric transport models were evaluated for their capability to simulate the CO2 plumes from two of the largest power plants in Europe by comparing the models against aircraft observations collected during the CoMet campaign in 2018. The study analysed how realistically such plumes can be simulated at different model resolutions and how well the planned European satellite mission CO2M will be able to quantify emissions from power plants.
Zichong Chen, Daniel J. Jacob, Hannah Nesser, Melissa P. Sulprizio, Alba Lorente, Daniel J. Varon, Xiao Lu, Lu Shen, Zhen Qu, Elise Penn, and Xueying Yu
Atmos. Chem. Phys., 22, 10809–10826, https://doi.org/10.5194/acp-22-10809-2022, https://doi.org/10.5194/acp-22-10809-2022, 2022
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We quantify methane emissions in China and contributions from different sectors by inverse analysis of 2019 TROPOMI satellite observations of atmospheric methane. We find that anthropogenic methane emissions for China are underestimated in the national inventory. Our estimate of emissions indicates a small life-cycle loss rate, implying net climate benefits from the current
coal-to-gasenergy transition in China. However, this small loss rate can be misleading given China's high gas imports.
Naveen Chandra, Prabir K. Patra, Yousuke Niwa, Akihiko Ito, Yosuke Iida, Daisuke Goto, Shinji Morimoto, Masayuki Kondo, Masayuki Takigawa, Tomohiro Hajima, and Michio Watanabe
Atmos. Chem. Phys., 22, 9215–9243, https://doi.org/10.5194/acp-22-9215-2022, https://doi.org/10.5194/acp-22-9215-2022, 2022
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This paper is intended to accomplish two goals: (1) quantify mean and uncertainty in non-fossil-fuel CO2 fluxes estimated by inverse modeling and (2) provide in-depth analyses of regional CO2 fluxes in support of emission mitigation policymaking. CO2 flux variability and trends are discussed concerning natural climate variability and human disturbances using multiple lines of evidence.
Anna Agusti-Panareda, Jérôme Barré, Sébastien Massart, Antje Inness, Ilse Aben, Melanie Ades, Bianca C. Baier, Gianpaolo Balsamo, Tobias Borsdorff, Nicolas Bousserez, Souhail Boussetta, Michael Buchwitz, Luca Cantarello, Cyril Crevoisier, Richard Engelen, Henk Eskes, Johannes Flemming, Sébastien Garrigues, Otto Hasekamp, Vincent Huijnen, Luke Jones, Zak Kipling, Bavo Langerock, Joe McNorton, Nicolas Meilhac, Stefan Noel, Mark Parrington, Vincent-Henri Peuch, Michel Ramonet, Miha Ratzinger, Maximilian Reuter, Roberto Ribas, Martin Suttie, Colm Sweeney, Jérôme Tarniewicz, and Lianghai Wu
EGUsphere, https://doi.org/10.5194/egusphere-2022-283, https://doi.org/10.5194/egusphere-2022-283, 2022
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We present a global dataset of atmospheric CO2 and CH4, the two most important human-made greenhouse gases, which covers almost two decades (2003–2020). It is produced by combining satellite data of CO2 and CH4 with a weather and air composition prediction model, and it has been carefully evaluated against independent observations to ensure validity and point out deficiencies to the user. This dataset can be used for scientific studies in the field of climate change and the global carbon cycle.
Ruben B. Schulte, Margreet C. van Zanten, Bart J. H. van Stratum, and Jordi Vilà-Guerau de Arellano
Atmos. Chem. Phys., 22, 8241–8257, https://doi.org/10.5194/acp-22-8241-2022, https://doi.org/10.5194/acp-22-8241-2022, 2022
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We present a fine-scale simulation framework, utilizing large-eddy simulations, to assess NH3 measurements influenced by boundary-layer dynamics and turbulent dispersion of a nearby emission source. The minimum required distance from an emission source differs for concentration and flux measurements, from 0.5–3.0 km and 0.75–4.5 km, respectively. The simulation framework presented here proves to be a powerful and versatile tool for future NH3 research at high spatio-temporal resolutions.
Sieglinde Callewaert, Jérôme Brioude, Bavo Langerock, Valentin Duflot, Dominique Fonteyn, Jean-François Müller, Jean-Marc Metzger, Christian Hermans, Nicolas Kumps, Michel Ramonet, Morgan Lopez, Emmanuel Mahieu, and Martine De Mazière
Atmos. Chem. Phys., 22, 7763–7792, https://doi.org/10.5194/acp-22-7763-2022, https://doi.org/10.5194/acp-22-7763-2022, 2022
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A regional atmospheric transport model is used to analyze the factors contributing to CO2, CH4, and CO observations at Réunion Island. We show that the surface observations are dominated by local fluxes and dynamical processes, while the column data are influenced by larger-scale mechanisms such as biomass burning plumes. The model is able to capture the measured time series well; however, the results are highly dependent on accurate boundary conditions and high-resolution emission inventories.
Anja Ražnjević, Chiel van Heerwaarden, Bart van Stratum, Arjan Hensen, Ilona Velzeboer, Pim van den Bulk, and Maarten Krol
Atmos. Chem. Phys., 22, 6489–6505, https://doi.org/10.5194/acp-22-6489-2022, https://doi.org/10.5194/acp-22-6489-2022, 2022
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Mobile measurement techniques (e.g., instruments placed in cars) are often employed to identify and quantify individual sources of greenhouse gases. Due to road restrictions, those observations are often sparse (temporally and spatially). We performed high-resolution simulations of plume dispersion, with realistic weather conditions encountered in the field, to reproduce the measurement process of a methane plume emitted from an oil well and provide additional information about the plume.
Alice E. Ramsden, Anita L. Ganesan, Luke M. Western, Matthew Rigby, Alistair J. Manning, Amy Foulds, James L. France, Patrick Barker, Peter Levy, Daniel Say, Adam Wisher, Tim Arnold, Chris Rennick, Kieran M. Stanley, Dickon Young, and Simon O'Doherty
Atmos. Chem. Phys., 22, 3911–3929, https://doi.org/10.5194/acp-22-3911-2022, https://doi.org/10.5194/acp-22-3911-2022, 2022
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Quantifying methane emissions from different sources is a key focus of current research. We present a method for estimating sectoral methane emissions that uses ethane as a tracer for fossil fuel methane. By incorporating variable ethane : methane emission ratios into this model, we produce emissions estimates with improved uncertainty characterisation. This method will be particularly useful for studying methane emissions in areas with complex distributions of sources.
Ying Li, Xiangjun Zhao, Xuejiao Deng, and Jinhui Gao
Atmos. Chem. Phys., 22, 3861–3873, https://doi.org/10.5194/acp-22-3861-2022, https://doi.org/10.5194/acp-22-3861-2022, 2022
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This study finds a new phenomenon of weak wind deepening (WWD) associated with the peripheral circulation of typhoon and gives the influence mechanism of WWD on its contribution to daily variation during sustained ozone episodes. The WWD provides the premise for pollution accumulation in the whole PBL and continued enhancement of ground-level ozone via vertical mixing processes. These findings could benefit the daily daytime ozone forecast in the PRD region and other areas.
Tia R. Scarpelli, Daniel J. Jacob, Shayna Grossman, Xiao Lu, Zhen Qu, Melissa P. Sulprizio, Yuzhong Zhang, Frances Reuland, Deborah Gordon, and John R. Worden
Atmos. Chem. Phys., 22, 3235–3249, https://doi.org/10.5194/acp-22-3235-2022, https://doi.org/10.5194/acp-22-3235-2022, 2022
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We present a spatially explicit version of the national inventories of oil, gas, and coal methane emissions as submitted by individual countries to the United Nations Framework Convention on Climate Change (UNFCCC) in 2021. We then use atmospheric modeling to compare our inventory emissions to atmospheric methane observations with the goal of identifying potential under- and overestimates of oil–gas methane emissions in the national inventories.
Xiaomeng Wu, Daoyuan Yang, Ruoxi Wu, Jiajun Gu, Yifan Wen, Shaojun Zhang, Rui Wu, Renjie Wang, Honglei Xu, K. Max Zhang, Ye Wu, and Jiming Hao
Atmos. Chem. Phys., 22, 1939–1950, https://doi.org/10.5194/acp-22-1939-2022, https://doi.org/10.5194/acp-22-1939-2022, 2022
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Our work pioneered land-use machine learning methods for developing link-level emission inventories, utilizing hourly traffic profiles, including volume, speed, and fleet mix, obtained from the governmental intercity highway monitoring network in the "capital circles" of China. This research provides a platform to realize the near-real-time process of establishing high-resolution vehicle emission inventories for policy makers to engage in sophisticated traffic management.
Chenchao Zhan and Min Xie
Atmos. Chem. Phys., 22, 1351–1371, https://doi.org/10.5194/acp-22-1351-2022, https://doi.org/10.5194/acp-22-1351-2022, 2022
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The changes of land use and anthropogenic heat (AH) derived from urbanization can affect meteorology and in turn O3 evolution. In this study, we briefly describe the general features of O3 pollution in the Yangtze River Delta (YRD) based on in situ observational data. Then, the impacts of land use and anthropogenic heat on O3 via changing the meteorological factors and local circulations are investigated in this region using the WRF-Chem model.
Hélène Peiro, Sean Crowell, Andrew Schuh, David F. Baker, Chris O'Dell, Andrew R. Jacobson, Frédéric Chevallier, Junjie Liu, Annmarie Eldering, David Crisp, Feng Deng, Brad Weir, Sourish Basu, Matthew S. Johnson, Sajeev Philip, and Ian Baker
Atmos. Chem. Phys., 22, 1097–1130, https://doi.org/10.5194/acp-22-1097-2022, https://doi.org/10.5194/acp-22-1097-2022, 2022
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Satellite CO2 observations are constantly improved. We study an ensemble of different atmospheric models (inversions) from 2015 to 2018 using separate ground-based data or two versions of the OCO-2 satellite. Our study aims to determine if different satellite data corrections can yield different estimates of carbon cycle flux. A difference in the carbon budget between the two versions is found over tropical Africa, which seems to show the impact of corrections applied in satellite data.
Shelley van der Graaf, Enrico Dammers, Arjo Segers, Richard Kranenburg, Martijn Schaap, Mark W. Shephard, and Jan Willem Erisman
Atmos. Chem. Phys., 22, 951–972, https://doi.org/10.5194/acp-22-951-2022, https://doi.org/10.5194/acp-22-951-2022, 2022
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CrIS NH3 satellite observations are assimilated into the LOTOS-EUROS model using two different methods. In the first method the data are used to fit spatially varying NH3 emission time factors. In the second method a local ensemble transform Kalman filter is used. Compared to in situ observations, combining both methods led to the most significant improvements in the modeled concentrations and deposition, illustrating the usefulness of CrIS NH3 to improve the spatiotemporal distribution of NH3.
Abhinna K. Behera, Emmanuel D. Rivière, Sergey M. Khaykin, Virginie Marécal, Mélanie Ghysels, Jérémie Burgalat, and Gerhard Held
Atmos. Chem. Phys., 22, 881–901, https://doi.org/10.5194/acp-22-881-2022, https://doi.org/10.5194/acp-22-881-2022, 2022
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Deep convection overshooting the stratosphere's contribution to the global stratospheric water budget is still being quantified. We ran three different cloud-resolving simulations of an observed case of overshoots in Bauru during the TRO-Pico balloon campaign in the context of upscaling the impact of overshoots at a large scale. These simulations, which have been validated with balloon-borne and S-band radar measurements, shed light on the local-scale variability and composition of overshoots.
Jiachen Zhu, Amos P. K. Tai, and Steve Hung Lam Yim
Atmos. Chem. Phys., 22, 765–782, https://doi.org/10.5194/acp-22-765-2022, https://doi.org/10.5194/acp-22-765-2022, 2022
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This study assessed O3 damage to plant and the subsequent effects on meteorology and air quality in China, whereby O3, meteorology, and vegetation can co-evolve with each other. We provided comprehensive understanding about how O3–vegetation impacts adversely affect plant growth and crop production, and contribute to global warming and severe O3 air pollution in China. Our findings clearly pinpoint the need to consider the O3 damage effects in both air quality studies and climate change studies.
Youwen Sun, Hao Yin, Xiao Lu, Justus Notholt, Mathias Palm, Cheng Liu, Yuan Tian, and Bo Zheng
Atmos. Chem. Phys., 21, 18589–18608, https://doi.org/10.5194/acp-21-18589-2021, https://doi.org/10.5194/acp-21-18589-2021, 2021
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This study uses high-resolution nested-grid GEOS-Chem simulation, the eXtreme Gradient Boosting (XGBoost) machine learning method, and the exposure–response relationship to determine the drivers and evaluate the health risks of the unexpected surface O3 enhancements over the Sichuan Basin in 2020. These unexpected O3 enhancements were induced by meteorological anomalies and caused dramatically high health risks.
Sabour Baray, Daniel J. Jacob, Joannes D. Maasakkers, Jian-Xiong Sheng, Melissa P. Sulprizio, Dylan B. A. Jones, A. Anthony Bloom, and Robert McLaren
Atmos. Chem. Phys., 21, 18101–18121, https://doi.org/10.5194/acp-21-18101-2021, https://doi.org/10.5194/acp-21-18101-2021, 2021
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We use 2010–2015 surface and satellite observations to disentangle methane from anthropogenic and natural sources in Canada. Using a chemical transport model (GEOS-Chem), the mismatch between modelled and observed methane concentrations can be used to infer emissions according to Bayesian statistics. Compared to prior knowledge, we show higher anthropogenic emissions attributed to energy and/or agriculture in Western Canada and lower natural emissions from Boreal wetlands.
Stefano Galmarini, Paul Makar, Olivia E. Clifton, Christian Hogrefe, Jesse O. Bash, Roberto Bellasio, Roberto Bianconi, Johannes Bieser, Tim Butler, Jason Ducker, Johannes Flemming, Alma Hodzic, Christopher D. Holmes, Ioannis Kioutsioukis, Richard Kranenburg, Aurelia Lupascu, Juan Luis Perez-Camanyo, Jonathan Pleim, Young-Hee Ryu, Roberto San Jose, Donna Schwede, Sam Silva, and Ralf Wolke
Atmos. Chem. Phys., 21, 15663–15697, https://doi.org/10.5194/acp-21-15663-2021, https://doi.org/10.5194/acp-21-15663-2021, 2021
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This technical note presents the research protocols for phase 4 of the Air Quality Model Evaluation International Initiative (AQMEII4). This initiative has three goals: (i) to define the state of wet and dry deposition in regional models, (ii) to evaluate how dry deposition influences air concentration and flux predictions, and (iii) to identify the causes for prediction differences. The evaluation compares LULC-specific dry deposition and effective conductances and fluxes.
Sepehr Fathi, Mark Gordon, Paul A. Makar, Ayodeji Akingunola, Andrea Darlington, John Liggio, Katherine Hayden, and Shao-Meng Li
Atmos. Chem. Phys., 21, 15461–15491, https://doi.org/10.5194/acp-21-15461-2021, https://doi.org/10.5194/acp-21-15461-2021, 2021
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We have investigated the accuracy of aircraft-based mass balance methodologies through computer model simulations of the atmosphere and air quality at a regional high-resolution scale. We have defined new quantitative metrics to reduce emission retrieval uncertainty by evaluating top-down mass balance estimates against the known simulated meteorology and input emissions. We also recommend methodologies and flight strategies for improved retrievals in future aircraft-based studies.
Peter Huszar, Jan Karlický, Jana Marková, Tereza Nováková, Marina Liaskoni, and Lukáš Bartík
Atmos. Chem. Phys., 21, 14309–14332, https://doi.org/10.5194/acp-21-14309-2021, https://doi.org/10.5194/acp-21-14309-2021, 2021
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Urban areas are strong hot spots of emissions influencing local and regional air quality. Cities furthermore influence the meteorological conditions due to their characteristic surface properties and geometry. We found that if these latter effects are not included in the quantification of the impact of urban emissions on regional air quality, this impact will be overestimated, and this overestimation is mainly due to the enhanced turbulence that is present in cities compared to rural areas.
Xinghong Cheng, Zilong Hao, Zengliang Zang, Zhiquan Liu, Xiangde Xu, Shuisheng Wang, Yuelin Liu, Yiwen Hu, and Xiaodan Ma
Atmos. Chem. Phys., 21, 13747–13761, https://doi.org/10.5194/acp-21-13747-2021, https://doi.org/10.5194/acp-21-13747-2021, 2021
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We develop a new inversion method of emission sources based on sensitivity analysis and the three-dimension variational technique. The novel explicit observation operator matrix between emission sources and the receptor’s concentrations is established. Then this method is applied to a typical heavy haze episode in North China, and spatiotemporal variations of SO2, NO2, and O3 concentrations simulated using a posterior emission sources are compared with results using an a priori inventory.
Taylor S. Jones, Jonathan E. Franklin, Jia Chen, Florian Dietrich, Kristian D. Hajny, Johannes C. Paetzold, Adrian Wenzel, Conor Gately, Elaine Gottlieb, Harrison Parker, Manvendra Dubey, Frank Hase, Paul B. Shepson, Levi H. Mielke, and Steven C. Wofsy
Atmos. Chem. Phys., 21, 13131–13147, https://doi.org/10.5194/acp-21-13131-2021, https://doi.org/10.5194/acp-21-13131-2021, 2021
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Methane emissions from leaks in natural gas pipes are often a large source in urban areas, but they are difficult to measure on a city-wide scale. Here we use an array of innovative methane sensors distributed around the city of Indianapolis and a new method of combining their data with an atmospheric model to accurately determine the magnitude of these emissions, which are about 70 % larger than predicted. This method can serve as a framework for cities trying to account for their emissions.
Alistair J. Manning, Alison L. Redington, Daniel Say, Simon O'Doherty, Dickon Young, Peter G. Simmonds, Martin K. Vollmer, Jens Mühle, Jgor Arduini, Gerard Spain, Adam Wisher, Michela Maione, Tanja J. Schuck, Kieran Stanley, Stefan Reimann, Andreas Engel, Paul B. Krummel, Paul J. Fraser, Christina M. Harth, Peter K. Salameh, Ray F. Weiss, Ray Gluckman, Peter N. Brown, John D. Watterson, and Tim Arnold
Atmos. Chem. Phys., 21, 12739–12755, https://doi.org/10.5194/acp-21-12739-2021, https://doi.org/10.5194/acp-21-12739-2021, 2021
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This paper estimates UK emissions of important greenhouse gases (hydrofluorocarbons (HFCs)) using high-quality atmospheric observations and atmospheric modelling. We compare these estimates with those submitted by the UK to the United Nations. We conclude that global concentrations of these gases are still increasing. Our estimates for the UK are 73 % of those reported and that the UK emissions are now falling, demonstrating an impact of UK government policy.
Paul A. Makar, Craig Stroud, Ayodeji Akingunola, Junhua Zhang, Shuzhan Ren, Philip Cheung, and Qiong Zheng
Atmos. Chem. Phys., 21, 12291–12316, https://doi.org/10.5194/acp-21-12291-2021, https://doi.org/10.5194/acp-21-12291-2021, 2021
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Vehicle pollutant emissions occur in an environment where upward transport can be enhanced due to the turbulence created by the vehicles as they move through the atmosphere. An approach for including these turbulence effects in regional air pollution forecast models has been derived from theoretical, observation, and higher-resolution modeling. The enhanced mixing, which occurs in the immediate vicinity of roadways, changes pollutant concentrations on the regional to continental scale.
Kun Qu, Xuesong Wang, Yu Yan, Jin Shen, Teng Xiao, Huabin Dong, Limin Zeng, and Yuanhang Zhang
Atmos. Chem. Phys., 21, 11593–11612, https://doi.org/10.5194/acp-21-11593-2021, https://doi.org/10.5194/acp-21-11593-2021, 2021
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Typhoons above the Northwest Pacific frequently lead to severe ambient ozone pollution in the Pearl River Delta, China, in autumn and summer. However, typhoons do not enhance ozone transport, production and accumulation at the same time, and differences also exist between these influences in two seasons. Through systematic comparisons, we revealed the complex interactions between local meteorology and ozone processes, which is essential for understanding the causes of regional ozone pollution.
Jinghui Lian, François-Marie Bréon, Grégoire Broquet, Thomas Lauvaux, Bo Zheng, Michel Ramonet, Irène Xueref-Remy, Simone Kotthaus, Martial Haeffelin, and Philippe Ciais
Atmos. Chem. Phys., 21, 10707–10726, https://doi.org/10.5194/acp-21-10707-2021, https://doi.org/10.5194/acp-21-10707-2021, 2021
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Currently there is growing interest in monitoring city-scale CO2 emissions based on atmospheric CO2 measurements, atmospheric transport modeling, and inversion technique. We analyze the various sources of uncertainty that impact the atmospheric CO2 modeling and that may compromise the potential of this method for the monitoring of CO2 emission over Paris. Results suggest selection criteria for the assimilation of CO2 measurements into the inversion system that aims at retrieving city emissions.
Julian Kostinek, Anke Roiger, Maximilian Eckl, Alina Fiehn, Andreas Luther, Norman Wildmann, Theresa Klausner, Andreas Fix, Christoph Knote, Andreas Stohl, and André Butz
Atmos. Chem. Phys., 21, 8791–8807, https://doi.org/10.5194/acp-21-8791-2021, https://doi.org/10.5194/acp-21-8791-2021, 2021
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Abundant mining and industrial activities in the Upper Silesian Coal Basin lead to large emissions of the potent greenhouse gas methane. This study quantifies these emissions with continuous, high-precision airborne measurements and dispersion modeling. Our emission estimates are in line with values reported in the European Pollutant Release and Transfer Register (E-PRTR 2017) but significantly lower than values reported in the Emissions Database for Global Atmospheric Research (EDGAR v4.3.2).
Xinyi Dong, Man Yue, Yujun Jiang, Xiao-Ming Hu, Qianli Ma, Jingjiao Pu, and Guangqiang Zhou
Atmos. Chem. Phys., 21, 7217–7233, https://doi.org/10.5194/acp-21-7217-2021, https://doi.org/10.5194/acp-21-7217-2021, 2021
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The dynamics of CO2 has received considerable attention in the literature, yet uncertainties remain. We applied an online coupled weather-biosphere model to simulate biosphere processes and meteorology simultaneously to characterize CO2 dynamics in China. Anthropogenic emission was more influential in upper air, and the biosphere flux played a more important role in surface CO2, suggesting a significant influence of the boundary layer thermal structure on the accumulation and depletion of CO2.
Shibao Wang, Yun Ma, Zhongrui Wang, Lei Wang, Xuguang Chi, Aijun Ding, Mingzhi Yao, Yunpeng Li, Qilin Li, Mengxian Wu, Ling Zhang, Yongle Xiao, and Yanxu Zhang
Atmos. Chem. Phys., 21, 7199–7215, https://doi.org/10.5194/acp-21-7199-2021, https://doi.org/10.5194/acp-21-7199-2021, 2021
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Mobile monitoring with low-cost sensors is a promising approach to garner high-spatial-resolution observations representative of the community scale. We develop a grid analysis method to obtain 50 m resolution maps of major air pollutants (CO, NO2, and O3) based on GIS technology. Our results demonstrate the sensing power of mobile monitoring for urban air pollution, which provides detailed information for source attribution and accurate traceability at the urban micro-scale.
Zichong Chen, Junjie Liu, Daven K. Henze, Deborah N. Huntzinger, Kelley C. Wells, Stephen Sitch, Pierre Friedlingstein, Emilie Joetzjer, Vladislav Bastrikov, Daniel S. Goll, Vanessa Haverd, Atul K. Jain, Etsushi Kato, Sebastian Lienert, Danica L. Lombardozzi, Patrick C. McGuire, Joe R. Melton, Julia E. M. S. Nabel, Benjamin Poulter, Hanqin Tian, Andrew J. Wiltshire, Sönke Zaehle, and Scot M. Miller
Atmos. Chem. Phys., 21, 6663–6680, https://doi.org/10.5194/acp-21-6663-2021, https://doi.org/10.5194/acp-21-6663-2021, 2021
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NASA's Orbiting Carbon Observatory 2 (OCO-2) satellite observes atmospheric CO2 globally. We use a multiple regression and inverse model to quantify the relationships between OCO-2 and environmental drivers within individual years for 2015–2018 and within seven global biomes. Our results point to limitations of current space-based observations for inferring environmental relationships but also indicate the potential to inform key relationships that are very uncertain in process-based models.
Efisio Solazzo, Monica Crippa, Diego Guizzardi, Marilena Muntean, Margarita Choulga, and Greet Janssens-Maenhout
Atmos. Chem. Phys., 21, 5655–5683, https://doi.org/10.5194/acp-21-5655-2021, https://doi.org/10.5194/acp-21-5655-2021, 2021
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We conducted an extensive analysis of the structural uncertainty of the Emissions Database for Global Atmospheric Research (EDGAR) emission inventory of greenhouse gases, which adds a much needed reliability dimension to the accuracy of the emission estimates. The study undertakes in-depth analyses of the implication of aggregating emissions from different sources and/or countries on the accuracy. Results are presented for all emissions sectors according to IPCC definitions.
Ashique Vellalassery, Dhanyalekshmi Pillai, Julia Marshall, Christoph Gerbig, Michael Buchwitz, Oliver Schneising, and Aparnna Ravi
Atmos. Chem. Phys., 21, 5393–5414, https://doi.org/10.5194/acp-21-5393-2021, https://doi.org/10.5194/acp-21-5393-2021, 2021
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We investigate factors contributing to the severe and persistent air quality degradation in northern India that has worsened during every winter over the last decade. This is achieved by implementing atmospheric modelling and using recently available Sentinel-5 P satellite data for carbon monoxide. We see a minimal role of biomass burning, except for the state of Punjab. The aim is to focus on residential and industrial emission reduction strategies to tackle air pollution over northern India.
Xiao Lu, Daniel J. Jacob, Yuzhong Zhang, Joannes D. Maasakkers, Melissa P. Sulprizio, Lu Shen, Zhen Qu, Tia R. Scarpelli, Hannah Nesser, Robert M. Yantosca, Jianxiong Sheng, Arlyn Andrews, Robert J. Parker, Hartmut Boesch, A. Anthony Bloom, and Shuang Ma
Atmos. Chem. Phys., 21, 4637–4657, https://doi.org/10.5194/acp-21-4637-2021, https://doi.org/10.5194/acp-21-4637-2021, 2021
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We use an analytical solution to the Bayesian inverse problem to quantitatively compare and combine the information from satellite and in situ observations, and to estimate global methane budget and their trends over the 2010–2017 period. We find that satellite and in situ observations are to a large extent complementary in the inversion for estimating global methane budget, and reveal consistent corrections of regional anthropogenic and wetland methane emissions relative to the prior inventory.
Stuart K. Grange, James D. Lee, Will S. Drysdale, Alastair C. Lewis, Christoph Hueglin, Lukas Emmenegger, and David C. Carslaw
Atmos. Chem. Phys., 21, 4169–4185, https://doi.org/10.5194/acp-21-4169-2021, https://doi.org/10.5194/acp-21-4169-2021, 2021
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The changes in mobility across Europe due to the COVID-19 lockdowns had consequences for air quality. We compare what was experienced to estimates of "what would have been" without the lockdowns. Nitrogen dioxide (NO2), an important vehicle-sourced pollutant, decreased by a third. However, ozone (O3) increased in response to lower NO2. Because NO2 is decreasing over time, increases in O3 can be expected in European urban areas and will require management to avoid future negative outcomes.
Yanxu Zhang, Xingpei Ye, Shibao Wang, Xiaojing He, Lingyao Dong, Ning Zhang, Haikun Wang, Zhongrui Wang, Yun Ma, Lei Wang, Xuguang Chi, Aijun Ding, Mingzhi Yao, Yunpeng Li, Qilin Li, Ling Zhang, and Yongle Xiao
Atmos. Chem. Phys., 21, 2917–2929, https://doi.org/10.5194/acp-21-2917-2021, https://doi.org/10.5194/acp-21-2917-2021, 2021
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Urban air quality varies drastically at street scale, but traditional methods are too coarse to resolve it. We develop a 10 m resolution air quality model and apply it for traffic-related carbon monoxide air quality in Nanjing megacity. The model reveals a detailed geographical dispersion pattern of air pollution in and out of the road network and agrees well with a validation dataset. The model can be a vigorous part of the smart city system and inform urban planning and air quality management.
Trang Thi Quynh Nguyen, Wataru Takeuchi, Prakhar Misra, and Sachiko Hayashida
Atmos. Chem. Phys., 21, 2795–2818, https://doi.org/10.5194/acp-21-2795-2021, https://doi.org/10.5194/acp-21-2795-2021, 2021
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This study provides annual emissions of transportation, manufacturing industries and construction, and residential areas at 1 km resolution from 2009 to 2016 for Ho Chi Minh City, Vietnam. Our originality is our use of satellite-derived urban land use morphological maps. These maps which are based on building height provided by a coarse-resolution satellite-derived digital surface model (DSM) and urban built-up area classified from Landsat images allow spatial disaggregation of annual emissions.
Zhongjing Jiang, Jing Li, Xiao Lu, Cheng Gong, Lin Zhang, and Hong Liao
Atmos. Chem. Phys., 21, 2601–2613, https://doi.org/10.5194/acp-21-2601-2021, https://doi.org/10.5194/acp-21-2601-2021, 2021
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This study demonstrates that the intensity of the western Pacific subtropical high (WPSH), a major synoptic pattern in the northern Pacific during summer, can induce a dipole change in surface ozone pollution over eastern China. Ozone concentration increases in the north and decreases in the south during the strong WPSH phase, and vice versa. The change in chemical processes associated with the WPSH change plays a decisive role, whereas the natural emission of ozone precursors accounts for ~ 30 %.
Yilin Chen, Huizhong Shen, Jennifer Kaiser, Yongtao Hu, Shannon L. Capps, Shunliu Zhao, Amir Hakami, Jhih-Shyang Shih, Gertrude K. Pavur, Matthew D. Turner, Daven K. Henze, Jaroslav Resler, Athanasios Nenes, Sergey L. Napelenok, Jesse O. Bash, Kathleen M. Fahey, Gregory R. Carmichael, Tianfeng Chai, Lieven Clarisse, Pierre-François Coheur, Martin Van Damme, and Armistead G. Russell
Atmos. Chem. Phys., 21, 2067–2082, https://doi.org/10.5194/acp-21-2067-2021, https://doi.org/10.5194/acp-21-2067-2021, 2021
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Ammonia (NH3) emissions can exert adverse impacts on air quality and ecosystem well-being. NH3 emission inventories are viewed as highly uncertain. Here we optimize the NH3 emission estimates in the US using an air quality model and NH3 measurements from the IASI satellite instruments. The optimized NH3 emissions are much higher than the National Emissions Inventory estimates in April. The optimized NH3 emissions improved model performance when evaluated against independent observation.
Bo Zhang, Hongyu Liu, James H. Crawford, Gao Chen, T. Duncan Fairlie, Scott Chambers, Chang-Hee Kang, Alastair G. Williams, Kai Zhang, David B. Considine, Melissa P. Sulprizio, and Robert M. Yantosca
Atmos. Chem. Phys., 21, 1861–1887, https://doi.org/10.5194/acp-21-1861-2021, https://doi.org/10.5194/acp-21-1861-2021, 2021
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We simulate atmospheric 222Rn using the GEOS-Chem model to improve understanding of 222Rn emissions and characterize convective transport in the model. We demonstrate the potential of a customized global 222Rn emission scenario to improve simulated surface 222Rn concentrations and seasonality. We assess convective transport using observed 222Rn vertical profiles. Results have important implications for using chemical transport models to interpret the transport of trace gases and aerosols.
Fei Jiang, Hengmao Wang, Jing M. Chen, Weimin Ju, Xiangjun Tian, Shuzhuang Feng, Guicai Li, Zhuoqi Chen, Shupeng Zhang, Xuehe Lu, Jane Liu, Haikun Wang, Jun Wang, Wei He, and Mousong Wu
Atmos. Chem. Phys., 21, 1963–1985, https://doi.org/10.5194/acp-21-1963-2021, https://doi.org/10.5194/acp-21-1963-2021, 2021
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We present a 6-year inversion from 2010 to 2015 for the global and regional carbon fluxes using only the GOSAT XCO2 retrievals. We find that the XCO2 retrievals could significantly improve the modeling of atmospheric CO2 concentrations and that the inferred interannual variations in the terrestrial carbon fluxes in most land regions have a better relationship with the changes in severe drought area or leaf area index, or are more consistent with the previous estimates about drought impact.
Guilherme F. Camarinha-Neto, Julia C. P. Cohen, Cléo Q. Dias-Júnior, Matthias Sörgel, José Henrique Cattanio, Alessandro Araújo, Stefan Wolff, Paulo A. F. Kuhn, Rodrigo A. F. Souza, Luciana V. Rizzo, and Paulo Artaxo
Atmos. Chem. Phys., 21, 339–356, https://doi.org/10.5194/acp-21-339-2021, https://doi.org/10.5194/acp-21-339-2021, 2021
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It was observed that friagem phenomena (incursion of cold waves from the high latitudes of the Southern Hemisphere to the Amazon region), very common in the dry season of the Amazon region, produced significant changes in microclimate and atmospheric chemistry. Moreover, the effects of the friagem change the surface O3 and CO2 mixing ratios and therefore interfere deeply in the microclimatic conditions and the chemical composition of the atmosphere above the rainforest.
Xinrui Ge, Martijn Schaap, Richard Kranenburg, Arjo Segers, Gert Jan Reinds, Hans Kros, and Wim de Vries
Atmos. Chem. Phys., 20, 16055–16087, https://doi.org/10.5194/acp-20-16055-2020, https://doi.org/10.5194/acp-20-16055-2020, 2020
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This article is about improving the modeling of agricultural ammonia emissions. By considering land use, meteorology and agricultural practices, ammonia emission totals officially reported by countries are distributed in space and time. We illustrated the first step for a better understanding of the variability of ammonia emission, with the possibility of being applied at a European scale, which is of great significance for ammonia budget research and future policy-making.
Ashok K. Luhar, David M. Etheridge, Zoë M. Loh, Julie Noonan, Darren Spencer, Lisa Smith, and Cindy Ong
Atmos. Chem. Phys., 20, 15487–15511, https://doi.org/10.5194/acp-20-15487-2020, https://doi.org/10.5194/acp-20-15487-2020, 2020
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With the sharp rise in coal seam gas (CSG) production in Queensland’s Surat Basin, there is much interest in quantifying methane emissions from this area and from unconventional gas production in general. We develop and apply a regional Bayesian inverse model that uses hourly methane concentration data from two sites and modelled backward dispersion to quantify emissions. The model requires a narrow prior and suggests that the emissions from the CSG areas are 33% larger than bottom-up estimates.
Wayne M. Angevine, Jeff Peischl, Alice Crawford, Christopher P. Loughner, Ilana B. Pollack, and Chelsea R. Thompson
Atmos. Chem. Phys., 20, 11855–11868, https://doi.org/10.5194/acp-20-11855-2020, https://doi.org/10.5194/acp-20-11855-2020, 2020
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Emissions of air pollutants must be known for a wide variety of applications. Different methods of estimating emissions often disagree substantially. In this study, we apply standard methods to a well-known source, a power plant. We explore the uncertainty implied by the different answers that come from the different methods, different samples taken over several years, and different pollutants. We find that the overall uncertainty of emissions estimates is about 30 %.
Peter Huszar, Jan Karlický, Jana Ďoubalová, Tereza Nováková, Kateřina Šindelářová, Filip Švábik, Michal Belda, Tomáš Halenka, and Michal Žák
Atmos. Chem. Phys., 20, 11655–11681, https://doi.org/10.5194/acp-20-11655-2020, https://doi.org/10.5194/acp-20-11655-2020, 2020
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The paper shows how extreme meteorological conditions change due to the urban land-cover forcing and how this translates to the impact on the extreme air pollution over central European cities. It focuses on ozone, nitrogen dioxide, and particulate matter with a diameter of less than 2.5 μm and shows that, while for the extreme daily maximum 8 h ozone, changes are same as for the mean ones, much larger modifications are calculated for extreme NO2 and PM2.5 compared to their mean changes.
Cited articles
Alegría, N., Herranz, M., Idoeta, R., and Legarda, F.: Study of Be-7 activity concentration in the air of northern Spain, J. Radioanal. Nucl. Chem., 286, 347–351, https://doi.org/10.1007/s10967-010-0710-6, 2010.
AMAP/UNEP: Technical Background Report to the Global Atmospheric Mercury Assessment. Arctic Monitoring and Assessment Programme/UNEP Chemical Branch. 159 pp., 2008.
Arnott, W., Gyawali, M., and Arnold, I.: Aerosol extinction and single scattering albedo downwind of the summer 2008 California wildfires measured with photoacoustic spectrometers and sunphotometers from 355 nm to 1047 nm. Eos, 89, AGU Fall Meeting Supplement, Abstract A11D-0169, 2008.
Balkanski, Y. J., Jacob, D. J., and Gardner, G. M.: Transport and residence times of tropospheric aerosols inferred from a global three-dimensional simulation of Pb-210, J. Geophys. Res., 98, 20573–20586, 1993.
Bergan, T. and Rodhe, H.: Oxidation of elemental mercury in the atmosphere; constraints imposed by global scale modeling, J. Atmos. Chem., 40, 191–212, 2001.
Bullock, O. R. and Brehme, K. A.: Atmospheric mercury simulation using the CMAQ model: Formulation description and analysis of wet deposition results, Atmos. Environ., 36, 2135–2146, 2002.
Calvert, J. G., and Lindberg, S. E.: Mechanisms of mercury removal by O-3 and OH in the atmosphere, Atmos. Environ., 39, 3355–3367, https://doi.org/10.1016/j.atmosenv.2005.01.055, 2005.
Chung, S. H. and Seinfeld, J. H.: Global distribution and climate forcing of carbonaceous aerosols, J. Geophys. Res., 107, 4407, https://doi.org/10.1029/2001JD001397, 2002.
Clarkson, T. W. and Magos, L.: The toxicology of mercury and its chemical compounds, Crit. Rev. Toxic. , 36, 609–662, 2006.
Clever, H. L., Johnson, S. A., and Derrick, M. E.: The solubility of mercury and some sparingly soluble mercury salts in water and aqueous-electrolyte solutions, J. Phys. Chem. Ref. Data, 14, 631–681, 1985.
Dastoor, A. P. and Larocque, Y.: Global circulation of atmospheric mercury: A modeling study, Atmos. Environ., 38, 147–161, https://doi.org/10.1016/j.atmosenv.2003.08.037, 2004.
Edgerton, E. S., Hartsell, B. E., and Jansen, J. J.: Mercury speciation in coal-fired power plant plumes observed at three surface sites in the southeastern US, Environ. Sci. Technol., 40, 4563–4570, https://doi.org/10.1021/es0515607, 2006.
Engle, M. A., Tate, M. T., Krabbenhoft, D. P., Schauer, J. J., Kolker, A., Shanley, J. B., and Bothner, M. H.: Comparison of atmospheric mercury speciation and deposition at nine sites across central and eastern North America, J. Geophys. Res., 115, D18306, https://doi.org/10.1029/2010jd014064, 2010.
Faïn, X., Obrist, D., Hallar, A. G., McCubbin, I., and Rahn, T.: High levels of reactive gaseous mercury observed at a high elevation research laboratory in the Rocky Mountains, Atmos. Chem. Phys., 9, 8049–8060, https://doi.org/10.5194/acp-9-8049-2009, 2009.
Faïn, X., Obrist, D., Pierce, A., Barth, C., Gustin, M. S., and Boyle, D. P.: Whole-watershed mercury balance at Sagehen Creek, Sierra Nevada, CA, Geochim. Cosmochim. Acta, 75, 2379–2392, https://doi.org/10.1016/j.gca.2011.01.041, 2011.
Finley, B. D., Swartzendruber, P. C., and Jaffe, D. A.: Particulate mercury emissions in regional wildfire plumes observed at the Mount Bachelor Observatory, Atmos. Environ., 43, 6074–6083, https://doi.org/10.1016/j.atmosenv.2009.08.046, 2009.
Friedli, H. R., Radke, L. F., Lu, J. Y., Banic, C. M., Leaitch, W. R., and MacPherson, J. I.: Mercury emissions from burning of biomass from temperate North American forests: Laboratory and airborne measurements, Atmos. Environ., 37, 253–267, https://doi.org/10.1016/s1352-2310(02)00819-1, 2003a.
Friedli, H. R., Radke, L. F., Prescott, R., Hobbs, P. V., and Sinha, P.: Mercury emissions from the August 2001 wildfires in Washington State and an agricultural waste fire in Oregon and atmospheric mercury budget estimates, Glob. Biogeochem. Cy, 17, 1039, https://doi.org/10.1029/2002GB001972, 2003b.
Galarneau, E., Bidleman, T. F., and Blanchard, P.: Seasonality and interspecies differences in particle/gas partitioning of PAHs observed by the Integrated Atmospheric Deposition Network (IADN), Atmos. Environ., 40, 182–197, https://doi.org/10.1016/j.atmosenv.2005.09.034, 2006.
Graydon, J. A., Louis, V. L. S., Hintelmann, H., Lindberg, S. E., Sandilands, K. A., Rudd, J. W. M., Kelly, C. A., Hall, B. D., and Mowat, L. D.: Long-term wet and dry deposition of total and methyl mercury in the remote boreal ecoregion of Canada, Environ. Sci. Technol., 42, 8345–8351, https://doi.org/10.1021/es801056j, 2008.
Gustin, M. and Jaffe, D.: Reducing the uncertainty in measurement and understanding of mercury in the atmosphere, Environ. Sci. Technol., 44, 2222–2227, https://doi.org/10.1021/es902736k, 2010.
Hall, B.: The gas-phase oxidation of elemental mercury by ozone, Water Air Soil Pollut., 80, 301–315, https://doi.org/10.1007/bf01189680, 1995.
Hedgecock, I. M. and Pirrone, N.: Mercury and photochemistry in the marine boundary layer-modeling studies suggest the in situ production of reactive gas phase mercury, Atmos. Environ., 35, 3055–3062, https://doi.org/10.1016/s1352-2310(01)00109-1, 2001.
Holmes, C. D., Jacob, D. J., Mason, R. P., and Jaffe, D. A.: Sources and deposition of reactive gaseous mercury in the marine atmosphere, Atmos. Environ., 43, 2278–2285, https://doi.org/10.1016/j.atmosenv.2009.01.051, 2009.
Holmes, C. D., Jacob, D. J., Corbitt, E. S., Mao, J., Yang, X., Talbot, R., and Slemr, F.: Global atmospheric model for mercury including oxidation by bromine atoms, Atmos. Chem. Phys., 10, 12037–12057, https://doi.org/10.5194/acp-10-12037-2010, 2010.
Hynes, A., Donohoue, D., Goodsite, M., Hedgecock, I., Pirrone, N., and Mason, R.: Our current understanding of major chemical and physical processes affecting mercury dynamics in the atmosphere and at air-water/terrestrial interfaces, in: Mercury Fate and Transport in the Global Atmosphere, edited by: Pirrone, N. and Mason, R. P., chap. 14, Springer, 322–344, 2009.
Keeler, G., Glinsorn, G., and Pirrone, N.: Particulate mercury in the atmosphere – its significance, transport, transformation and sources, Water Air Soil Pollut., 80, 159–168, https://doi.org/10.1007/bf01189664, 1995.
Keeler, G. J., Gratz, L. E., and Al-Wali, K.: Long-term atmospheric mercury wet deposition at Underhill, Vermont, Ecotoxicology, 14, 71–83, https://doi.org/10.1007/s10646-004-6260-3, 2005.
Koch, D. M., Jacob, D. J., and Graustein, W. C.: Vertical transport of tropospheric aerosols as indicated by Be-7 and Pb-210 in a chemical tracer model, J. Geophys. Res., 101, 18651–18666, https://doi.org/10.1029/96jd01176, 1996.
Kos, G., Ryzhkov, A., and Dastoor, A.: Analysis of uncertainties in measurements and mode for oxidised and particle-bound mercury, 10th International Conference on Mercury as a Global Pollutant, Halifax, Nova Scotia, Canada, 2011.
Lamborg, C. H., Fitzgerald, W. F., Vandal, G. M., and Rolfhus, K. R.: Atmospheric mercury in northern Wisconsin – sources and species, Water Air Soil Pollut., 80, 189–198, https://doi.org/10.1007/bf01189667, 1995.
Landis, M. S., Stevens, R. K., Schaedlich, F., and Prestbo, E. M.: Development and characterization of an annular denuder methodology for the measurement of divalent inorganic reactive gaseous mercury in ambient air, Environ. Sci. Technol., 36, 3000–3009, https://doi.org/10.1021/es015887t, 2002.
Levine, S. Z. and Schwartz, S. E.: In-cloud and below-cloud scavenging of nitric acid vapor, Atmos. Environ., 16, 1725–1734, 1982.
Lin, C. J., Pongprueksa, P., Lindberg, S. E., Pehkonen, S. O., Byun, D., and Jang, C.: Scientific uncertainties in atmospheric mercury models I: Model science evaluation, Atmos. Environ., 40, 2911–2928, https://doi.org/10.1016/j.atmosenv.2006.01.009, 2006.
Lindberg, S. E. and Stratton, W. J.: Atmospheric mercury speciation: Concentrations and behavior of reactive gaseous mercury in ambient air, Environ. Sci. Technol., 32, 49–57, https://doi.org/10.1021/es970546u, 1998.
Lindqvist, O. and Rodhe, H.: Atmospheric mercury - a review, Tellus B-Chem. Phys. Meteorol., 37, 136–159, 1985.
Liu, H. Y., Jacob, D. J., Bey, I., and Yantosca, R. M.: Constraints from Pb-210 and Be-7 on wet deposition and transport in a global three-dimensional chemical tracer model driven by assimilated meteorological fields, J. Geophys. Res., 106, 12109–12128, https://doi.org/10.1029/2000jd900839, 2001.
Lohman, K., Seigneur, C., Edgerton, E., and Jansen, J.: Modeling mercury in power plant plumes, Environ. Sci. Technol., 40, 3848–3854, https://doi.org/10.1021/es051556v, 2006.
Lombard, M. A. S., Bryce, J. G., Mao, H., and Talbot, R.: Mercury deposition in southern New Hampshire, 2006–2009, Atmos. Chem. Phys., 11, 7657–7668, https://doi.org/10.5194/acp-11-7657-2011, 2011.
Lyman, S. N., Gustin, M. S., Prestbo, E. M., and Marsik, F. J.: Estimation of dry deposition of atmospheric mercury in Nevada by direct and indirect methods, Environ. Sci. Technol., 41, 1970–1976, https://doi.org/10.1021/es062323m, 2007.
Lyman, S. N., Gustin, M. S., Prestbo, E. M., Kilner, P. I., Edgerton, E., and Hartsell, B.: Testing and application of surrogate surfaces for understanding potential gaseous oxidized mercury dry deposition, Environ. Sci. Technol., 43, 6235–6241, https://doi.org/10.1021/es901192e, 2009.
Lyman, S. N. and Gustin, M. S.: Determinants of atmospheric mercury concentrations in Reno, Nevada, USA, Sci. Total Environ., 408, 431–438, https://doi.org/10.1016/j.scitotenv.2009.09.045, 2009.
Lyman, S. N., Jaffe, D. A., and Gustin, M. S.: Release of mercury halides from KCl denuders in the presence of ozone, Atmos. Chem. Phys., 10, 8197–8204, 10.5194/acp-10-8197-2010, 2010.
Lynam, M. M. and Keeler, G. J.: Artifacts associated with the measurement of particulate mercury in an urban environment: The influence of elevated ozone concentrations, Atmos. Environ., 39, 3081–3088, https://doi.org/10.1016/j.atmosenv.2005.01.036, 2005
Mahaffey, K. R., Clickner, R. P., and Bodurow, C. C.: Blood organic mercury and dietary mercury intake: National health and nutrition examination survey, 1999 and 2000, Environ. Health Persp., 112, 562–570, 2004.
Mahaffey, K. R., Clickner, R. P., and Jeffries, R. A.: Adult women's blood mercury concentrations vary regionally in the United States: Association with patterns of fish consumption (NHANES 1999–2004), Environ. Health Persp., 117, 47–53, 10.1289/ehp.11674, 2009.
Malcolm, E. G. and Keeler, G. J.: Evidence for a sampling artifact for particulate-phase mercury in the marine atmosphere, Atmos. Environ., 41, 3352–3359, https://doi.org/10.1016/j.atmosenv.2006.12.024, 2007.
Mao, H., Talbot, R., Hegarty, J., and Koermer, J.: Speciated mercury at marine, coastal, and inland sites in New England - Part 2: Relationships with atmospheric physical parameters, Atmos. Chem. Phys. Discuss., 11, 28395–28443, http://dx.doi.org/10.5194/acpd-11-28395-2011https://doi.org/10.5194/acpd-11-28395-2011, 2011.
Mason, R. P. and Sheu, G. R.: Role of the ocean in the global mercury cycle, Global Biogeochem. Cy., 16, 1093, https://doi.org/10.1029/2001gb001440, 2002.
Mergler, D., Anderson, H. A., Chan, L. H. M., Mahaffey, K. R., Murray, M., Sakamoto, M., and Stern, A. H.: Methylmercury exposure and health effects in humans: A worldwide concern, Ambio, 36, 3–11, 2007.
Muramatsu, H., Yoshizawa, S., Abe, T., Ishii, T., Wada, M., Horiuchi, Y., and Kanekatsu, R.: Variation of Be-7 concentration in surface air at Nagano, Japan, J. Radioanal. Nucl. Chem., 275, 299–307, https://doi.org/10.1007/s10967-007-7056-8, 2008.
National Atmospheric Deposition Program: Mercury Deposition Network (MDN): A NADP Network, available online at: http://nadp.sws.uiuc.edu/MDN/, 2011.
Odum, J. R., Hoffmann, T., Bowman, F., Collins, D., Flagan, R. C., and Seinfeld, J. H.: Gas/particle partitioning and secondary organic aerosol yields, Environ. Sci. Technol., 30, 2580–2585, https://doi.org/10.1021/es950943, 1996.
Pacyna, E. G., Pacyna, J. M., Sundseth, K., Munthe, J., Kindbom, K., Wilson, S., Steenhuisen, F., and Maxson, P.: Global emission of mercury to the atmosphere from anthropogenic sources in 2005 and projections to 2020, Atmos. Environ., 44, 2487–2499, https://doi.org/10.1016/j.atmosenv.2009.06.009, 2010.
Pankow, J. F.: Review and comparative-analysis if the theories on partitioning between the gas and aerosol particulate phases in the atmosphere, Atmos. Environ., 21, 2275–2283, https://doi.org/10.1016/0004-6981(87)90363-5, 1987.
Pankow, J. F., Storey, J. M. E., and Yamasaki, H.: Effects of relative-humidity on gas-particle partitioning of semivolatile organic-compounds to urban particulate matter, Environ. Sci. Technol., 27, 2220–2226, https://doi.org/10.1021/es00047a032, 1993.
Pankow, J. F.: An absorption-model of the gas aerosol partitioning involved in the formation of secondary organic aerosol, Atmos. Environ., 28, 189–193, https://doi.org/10.1016/1352-2310(94)90094-9, 1994.
Petersen, G., Munthe, J., Pleijel, K., Bloxam, R., and Kumar, A. V.: A comprehensive Eulerian modeling framework for airborne mercury species: Development and testing of the tropospheric chemistry module (TCM), Atmos. Environ., 32, 829–843, https://doi.org/10.1016/s1352-2310(97)00049-6, 1998.
Petersen, G., Iverfeldt, A., and Munthe, J.: Atmospheric mercury species over central and northern Europe – model-calculations and comparison with observations from the Nordic Air and Precipitation Network for 1987 and 1988, Atmos. Environ., 29, 47–67, https://doi.org/10.1016/1352-2310(94)00223-8, 1995.
Poissant, L., Pilote, M., Xu, X. H., Zhang, H., and Beauvais, C.: Atmospheric mercury speciation and deposition in the Bay St. Francois wetlands, J. Geophys. Res., 109, D11301, 10.1029/2003jd004364, 2004.
Pongprueksa, P., Lin, C. J., Lindberg, S. E., Jang, C., Braverman, T., Bullock, O. R., Ho, T. C., and Chu, H. W.: Scientific uncertainties in atmospheric mercury models III: Boundary and initial conditions, model grid resolution, and Hg(II) reduction mechanism, Atmos. Environ., 42, 1828–1845, https://doi.org/10.1016/j.atmosenv.2007.11.020, 2008.
Rutter, A. P. and Schauer, J. J.: The impact of aerosol composition on the particle to gas partitioning of reactive mercury, Environ. Sci. Technol., 41, 3934–3939, https://doi.org/10.1021/es062439i, 2007a.
Rutter, A. P. and Schauer, J. J.: The effect of temperature on the gas-particle partitioning of reactive mercury in atmospheric aerosols, Atmos. Environ., 41, 8647–8657, https://doi.org/10.1016/j.atmosenv.2007.07.024, 2007b.
Rutter, A. P., Hanford, K. L., Zwers, J. T., Perillo-Nicholas, A. L., Schauer, J. J., and Olson, M. L.: Evaluation of an offline method for the analysis of atmospheric reactive gaseous mercury and particulate mercury, J. Air Waste Manage. Assoc., 58, 377–383, 10.3155/1047-3289.58.3.377, 2008a.
Rutter, A. P., Schauer, J. J., Lough, G. C., Snyder, D. C., Kolb, C. J., Von Klooster, S., Rudolf, T., Manolopoulos, H., and Olson, M. L.: A comparison of speciated atmospheric mercury at an urban center and an upwind rural location, J. Environ. Monit., 10, 102–108, https://doi.org/10.1039/b710247j, 2008b.
Sanei, H., Outridge, P. M., Goodarzi, F., Wang, F., Armstrong, D., Warren, K., and Fishback, L.: Wet deposition mercury fluxes in the Canadian sub-Arctic and southern Alberta, measured using an automated precipitation collector adapted to cold regions, Atmos. Environ., 44, 1672–1681, https://doi.org/10.1016/j.atmosenv.2010.01.030, 2010.
Scheuhammer, A. M., Meyer, M. W., Sandheinrich, M. B., and Murray, M. W.: Effects of environmental methylmercury on the health of wild birds, mammals, and fish, Ambio, 36, 12–18, https://doi.org/10.1579/0044-7447(2007)36[12:eoemot]2.0.co;2, 2007.
Schroeder, W. H. and Munthe, J.: Atmospheric mercury – an overview, Atmos. Environ., 32, 809–822, https://doi.org/10.1016/s1352-2310(97)00293-8, 1998.
Seigneur, C., Abeck, H., Chia, G., Reinhard, M., Bloom, N. S., Prestbo, E., and Saxena, P.: Mercury adsorption to elemental carbon (soot) particles and atmospheric particulate matter, Atmos. Environ., 32, 2649–2657, https://doi.org/10.1016/s1352-2310(97)00415-9, 1998.
Seigneur, C., Karamchandani, P., Lohman, K., Vijayaraghavan, K., and Shia, R. L.: Multiscale modeling of the atmospheric fate and transport of mercury, J. Geophys. Res., 106, 27795–27809, https://doi.org/10.1029/2000jd000273, 2001.
Seigneur, C., Karamchandani, P., Vijayaraghavan, K., Lohman, K., Shia, R. L., and Levin, L.: On the effect of spatial resolution on atmospheric mercury modeling, Sci. Total Environ., 304, 73–81, https://doi.org/10.1016/s0048-9697(02)00558-2, 2003.
Seigneur, C., Vijayaraghavan, K., and Lohman, K.: Atmospheric mercury chemistry: Sensitivity of global model simulations to chemical reactions, J. Geophys. Res., 111, D22306, https://doi.org/10.1029/2005jd006780, 2006.
Seinfeld, J. H. and Pandis, S. N.: Atmospheric chemistry and physics: From air pollution to climate change, 2nd ed., John Wiley & Sons, Inc., 1203 pp., 2006.
Selin, N. E., Jacob, D. J., Park, R. J., Yantosca, R. M., Strode, S., Jaegle, L., and Jaffe, D.: Chemical cycling and deposition of atmospheric mercury: Global constraints from observations, J. Geophys. Res., 112, D02308, https://doi.org/10.1029/2006jd007450, 2007.
Selin, N. E. and Jacob, D. J.: Seasonal and spatial patterns of mercury wet deposition in the United States: Constraints on the contribution from North American anthropogenic sources, Atmos. Environ., 42, 5193–5204, 2008.
Selin, N. E., Jacob, D. J., Yantosca, R. M., Strode, S., Jaegle, L., and Sunderland, E. M.: Global 3-D land-ocean-atmosphere model for mercury: Present-day versus preindustrial cycles and anthropogenic enrichment factors for deposition, Global Biogeochem. Cycles, 22, GB3099, https://doi.org/10.1029/2008gb003282, 2008.
Sigler, J. M., Mao, H., and Talbot, R.: Gaseous elemental and reactive mercury in southern New Hampshire, Atmos. Chem. Phys., 9, 1929–1942, https://doi.org/10.5194/acp-9-1929-2009, 2009.
Skov, H., Brooks, S. B., Goodsite, M. E., Lindberg, S. E., Meyers, T. P., Landis, M. S., Larsen, M. R. B., Jensen, B., McConville, G., and Christensen, J.: Fluxes of reactive gaseous mercury measured with a newly developed method using relaxed eddy accumulation, Atmos. Environ., 40, 5452–5463, https://doi.org/10.1016/j.atmosenv.2006.04.061, 2006.
Soerensen, A. L., Sunderland, E. M., Holmes, C. D., Jacob, D. J., Yantosca, R. M., Skov, H., Christensen, J. H., Strode, S. A., and Mason, R. P.: An improved global model for air-sea exchange of mercury: High concentrations over the North Atlantic, Environ. Sci. Technol., 44, 8574–8580, https://doi.org/10.1021/es102032g, 2010.
Sommar, J., Gardfeldt, K., Stromberg, D., and Feng, X. B.: A kinetic study of the gas-phase reaction between the hydroxyl radical and atomic mercury, Atmos. Environ., 35, 3049–3054, https://doi.org/10.1016/s1352-2310(01)00108-x, 2001.
Subir, M., Ariya, P. A., and Dastoor, A. P.: A review of uncertainties in atmospheric modeling of mercury chemistry I. Uncertainties in existing kinetic parameters - fundamental limitations and the importance of heterogeneous chemistry, Atmos. Environ., 45, 5664–5676, https://doi.org/10.1016/j.atmosenv.2011.04.046, 2011.
Sunderland, E. M., and Mason, R. P.: Human impacts on open ocean mercury concentrations, Global Biogeochem. Cy., 21, GB4022, 10.1029/2006GB002876, 2007.
Swartzendruber, P. C., Jaffe, D. A., Prestbo, E. M., Weiss-Penzias, P., Selin, N. E., Park, R., Jacob, D. J., Strode, S., and Jaegle, L.: Observations of reactive gaseous mercury in the free troposphere at the Mount Bachelor Observatory, J. Geophys. Res., 111, D24302, https://doi.org/10.1029/2006jd007415, 2006.
Talbot, R., Mao, H., Feddersen, D., Smith, M., Kim, S. Y., Sive, B. C., Haase, K., Ambrose, J., Zhou, Y., and Russo, R.: Comparison of particulate mercury measured with manual and automated methods, Atmosphere, 2, 1–20, https://doi.org/10.3390/atmos2010001, 2011.
ter Schure, A., Caffrey, J., Gustin, M. S., Holmes, C. D., Hynes, A., Landing, B., Landis, M. S., Laudel, D., Levin, L., Nair, U., Jansen, J., Ryan, J., Walters, J., Schauer, J. J., Volkamer, R., Waters, D., and Weiss, P.: An integrated approach to assess elevated mercury wet deposition and concentrations in the southeastern United States, 10th International Conference on Mercury as a Global Pollutant, Halifax, Nova Scotia, Canada, 2011.
Vijayaraghavan, K., Karamchandani, P., Seigneur, C., Balmori, R., and Chen, S. Y.: Plume-in-grid modeling of atmospheric mercury, J. Geophys. Res., 113, D24305, https://doi.org/10.1029/2008jd010580, 2008.
Wang, Q., Jacob, D. J., Fisher, J. A., Mao, J., Leibensperger, E. M., Carouge, C. C., Le Sager, P., Kondo, Y., Jimenez, J. L., Cubison, M. J., and Doherty, S. J.: Sources of carbonaceous aerosols and deposited black carbon in the Arctic in winter-spring: Implications for radiative forcing, Atmos. Chem. Phys., 11, 12453–12473, https://doi.org/10.5194/acp-11-12453-2011, 2011.
Wang, Y. H., Jacob, D. J., and Logan, J. A.: Global simulation of tropospheric O3-NOx-hydrocarbon chemistry 1. Model formulation, J. Geophys. Res., 103, 10713–10725, https://doi.org/10.1029/98jd00158, 1998.
Weiss-Penzias, P., Gustin, M. S., and Lyman, S. N.: Observations of speciated atmospheric mercury at three sites in Nevada: Evidence for a free tropospheric source of reactive gaseous mercury, J. Geophys. Res., 114, D14302, https://doi.org/10.1029/2008jd011607, 2009.
Weiss-Penzias, P. S., Gustin, M. S., and Lyman, S. N.: Sources of gaseous oxidized mercury and mercury dry deposition at two southeastern US sites, Atmos. Environ., 45, 4569–4579, https://doi.org/10.1016/j.atmosenv.2011.05.069, 2011.
Wesely, M. L.: Parameterization of surface resistances to gaseous dry deposition in regional-scale numerical-models, Atmos. Environ., 23, 1293–1304, https://doi.org/10.1016/0004-6981(89)90153-4, 1989.
Yamasaki, H., Kuwata, K., and Miyamoto, H.: Effects of ambient temperature on aspects of airborne polycyclic aromatic hydrocarbons, Environ. Sci. Technol., 16, 189–194, https://doi.org/10.1021/es00098a003, 1982.
Yoshimori, M.: Beryllium 7 radionucleide as a tracer of vertical air mass transport in the troposphere, Atmos. Remote Sens., 828–832, 2005.
Zhang, L., Jacob, D. J., Downey, N. V., Wood, D. A., Blewitt, D., Carouge, C. C., van Donkelaar, A., Jones, D. B. A., Murray, L. T., and Wang, Y.: Improved estimate of the policy-relevant background ozone in the United States using the GEOS-Chem global model with 1/2$^{\circ}{\times}$2/3° horizontal resolution over North America, Atmos. Environ., 45, 6769–6776, 2011a.
Zhang, L. Jacob, D. J., Knipping, E. M., Kumar, N., Munger, J. W., Carouge, C. C., van Donkelaar, A., Wang, Y., and D. Chen: Nitrogen deposition to the United States: distribution, sources, and processes, Atmos. Chem. Phys., submitted, 2011b.
Zhang, Y., Jaeglé, L., van Donkelaar, A., Martin, R. V., Holmes, C. D., Amos, H. M., Wang, Q., Jacob, D. J., Talbot, R., Artz, R., Holson, T. M., Felton, D., Miller, E. K., Perry, K. D., Schmeltz, D., Steffen, A., and Tordon, R.: Nested-grid simulation of mercury over North America, Atmos. Chem. Phys., submitted, 2011.
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